TY - JOUR A1 - Kniepert, Juliane A1 - Lange, Ilja A1 - van der Kaap, Niels J. A1 - Koster, L. Jan Anton A1 - Neher, Dieter T1 - A conclusive view on charge generation, recombination, and extraction in As-prepared and annealed P3HT:PCBM blends: combined experimental and simulation work JF - dvanced energy materials N2 - Time-delayed collection field (TDCF) and bias-amplified charge extraction (BACE) are applied to as-prepared and annealed poly(3-hexylthiophene):[6,6]-phenyl C-71 butyric acid methyl ester (P3HT:PCBM) blends coated from chloroform. Despite large differences in fill factor, short-circuit current, and power conversion efficiency, both blends exhibit a negligible dependence of photogeneration on the electric field and strictly bimolecular recombination (BMR) with a weak dependence of the BMR coefficient on charge density. Drift-diffusion simulations are performed using the measured coefficients and mobilities, taking into account bimolecular recombination and the possible effects of surface recombination. The excellent agreement between the simulation and the experimental data for an intensity range covering two orders of magnitude indicates that a field-independent generation rate and a density-independent recombination coefficient describe the current-voltage characteristics of the annealed P3HT: PCBM devices, while the performance of the as-prepared blend is shown to be limited by space charge effects due to a low hole mobility. Finally, even though the bimolecular recombination coefficient is small, surface recombination is found to be a negligible loss mechanism in these solar cells. Y1 - 2014 U6 - https://doi.org/10.1002/aenm.201301401 SN - 1614-6832 SN - 1614-6840 VL - 4 IS - 7 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Stephan, Christoph A. T1 - A dark sector extension of the almost-commutative standard model JF - International journal of modern physics : A, Particles and fields, gravitation, cosmology, nuclear physics N2 - We consider an extension of the Standard Model within the framework of Noncommutative Geometry. The model is based on an older model [C. A. Stephan, Phys. Rev. D 79, 065013 (2009)] which extends the Standard Model by new fermions, a new U(1)-gauge group and, crucially, a new scalar field which couples to the Higgs field. This new scalar field allows to lower the mass of the Higgs mass from similar to 170 GeV, as predicted by the Spectral Action for the Standard Model, to a value of 120-130 GeV. The shortcoming of the previous model lay in its inability to meet all the constraints on the gauge couplings implied by the Spectral Action. These shortcomings are cured in the present model which also features a "dark sector" containing fermions and scalar particles. KW - Noncommutative geometry KW - spectral triple KW - beyond Standard Model KW - Higgs boson KW - scalar fields Y1 - 2014 U6 - https://doi.org/10.1142/S0217751X14500055 SN - 0217-751X SN - 1793-656X VL - 29 IS - 1 PB - World Scientific CY - Singapore ER - TY - JOUR A1 - Naze, Yael A1 - Wang, Q. Daniel A1 - Chu, You-Hua A1 - Gruendl, Robert A1 - Oskinova, Lida T1 - A deep chandra observation of the giant HII region N11. I. x-ray sorces in the field JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Supplement series N2 - A very sensitive X-ray investigation of the giant HII region N11 in the Large Megallanic Cloud was performed using the Chandra X-ray Observatory. The 300 ks observation reveals X-ray sources with luminosities down to 10(32) erg s(-1), increasing the number of known point sources in the field by more than a factor of five. Among these detections are 13 massive stars (3 compact groups of massive stars, 9 O stars, and one early B star) with log(L-X/L-BOL) similar to -6.5 to -7, which may suggest that they are highly magnetic or colliding-wind systems. On the other hand, the stacked signal for regions corresponding to undetected O stars yields log(L-X/L-BOL) similar to -7.3, i.e., an emission level comparable to similar Galactic stars despite the lower metallicity. Other point sources coincide with 11 foreground stars, 6 late-B/A stars in N11, and many background objects. This observation also uncovers the extent and detailed spatial properties of the soft, diffuse emission regions, but the presence of some hotter plasma in their spectra suggests contamination by the unresolved stellar population. KW - galaxies: star clusters: general KW - ISM: individual objects (LMC N11) KW - Magellanic Clouds KW - X-rays: stars Y1 - 2014 U6 - https://doi.org/10.1088/0067-0049/213/2/23 SN - 0067-0049 SN - 1538-4365 VL - 213 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Meier, Patrick A1 - Kriegel, Hendrik A1 - Motschmann, Uwe A1 - Schmidt, Jürgen A1 - Spahn, Frank A1 - Hill, Thomas W. A1 - Dong, Yaxue A1 - Jones, Geraint H. T1 - A model of the spatial and size distribution of Enceladus' dust plume JF - Planetary and space science KW - Enceladus KW - Plume KW - Nanograins KW - Cassini KW - Tail Y1 - 2014 U6 - https://doi.org/10.1016/j.pss.2014.09.016 SN - 0032-0633 VL - 104 SP - 216 EP - 233 PB - Elsevier CY - Oxford ER - TY - JOUR A1 - Aliu, E. A1 - Archambault, S. A1 - Aune, T. A1 - Benbow, W. A1 - Berger, K. A1 - Bird, R. A1 - Bouvier, A. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cerruti, M. A1 - Chen, Xuhui A1 - Ciupik, L. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dumm, J. A1 - Errando, M. A1 - Falcone, A. A1 - Federici, Simone A1 - Feng, Q. A1 - Finley, J. P. A1 - Fortin, P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gillanders, G. H. A1 - Griffin, S. A1 - Griffiths, S. T. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Kertzman, M. A1 - Khassen, Y. A1 - Kieda, D. A1 - Krennrich, F. A1 - Kumar, S. A1 - Lang, M. J. A1 - Lyutikov, M. A1 - Maier, G. A1 - McArthur, S. A1 - McCann, A. A1 - Meagher, K. A1 - Millis, J. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, M. A1 - Popkow, A. A1 - Quinn, J. A1 - Ragan, K. A1 - Rajotte, J. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Sembroski, G. H. A1 - Sheidaei, F. A1 - Smith, A. W. A1 - Staszak, D. A1 - Telezhinsky, Igor O. A1 - Theiling, M. A1 - Tucci, J. V. A1 - Tyler, J. A1 - Varlotta, A. A1 - Wakely, S. P. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Welsing, R. A1 - Williams, D. A. A1 - Zajczyk, A. A1 - Zitzer, B. T1 - A search for enhanced very high energy GAMMA-RAY emission from the 2013 march crab nebula flare JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - In 2013 March, a flaring episode from the Crab Nebula lasting similar to 2 weeks was detected by Fermi-LAT (Large Area Telescope on board the Fermi Gamma-ray Space Telescope). The Very Energetic Radiation Imaging Telescope Array System (VERITAS) provides simultaneous observations throughout this period. During the flare, Fermi-LAT detected a 20 fold increase in flux above the average synchrotron flux >100 MeV seen from the Crab Nebula. Simultaneous measurements with VERITAS are consistent with the non-variable long-term average Crab Nebula flux at TeV energies. Assuming a linear correlation between the very high energy flux change >1 TeV and the flux change seen in the Fermi-LAT band >100 MeV during the period of simultaneous observations, the linear correlation factor can be constrained to be at most 8.6 x 10(-3) with 95% confidence. KW - gamma rays: general KW - ISM: individual objects (Crab Nebula) Y1 - 2014 U6 - https://doi.org/10.1088/2041-8205/781/1/L11 SN - 2041-8205 SN - 2041-8213 VL - 781 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Spahn, Frank A1 - Vieira Neto, E. A1 - Guimaraes, A. H. F. A1 - Gorban, A. N. A1 - Brilliantov, Nikolai V. T1 - A statistical model of aggregate fragmentation JF - New journal of physics : the open-access journal for physics N2 - A statistical model of fragmentation of aggregates is proposed, based on the stochastic propagation of cracks through the body. The propagation rules are formulated on a lattice and mimic two important features of the process-a crack moves against the stress gradient while dissipating energy during its growth. We perform numerical simulations of the model for two-dimensional lattice and reveal that the mass distribution for small-and intermediate-size fragments obeys a power law, F(m) proportional to m(-3/2), in agreement with experimental observations. We develop an analytical theory which explains the detected power law and demonstrate that the overall fragment mass distribution in our model agrees qualitatively with that one observed in experiments. Y1 - 2014 U6 - https://doi.org/10.1088/1367-2630/16/1/013031 SN - 1367-2630 VL - 16 PB - IOP Publ. Ltd. CY - Bristol ER - TY - THES A1 - Herenz, Peter T1 - A study of the absorption characteristics of gaseous galaxy halos in the local Universe T1 - Untersuchung von Absorptionsstrukturen in den gasförmigen Halos von Galaxien im lokalen Universum. N2 - Today, it is well known that galaxies like the Milky Way consist not only of stars but also of gas and dust. The galactic halo, a sphere of gas that surrounds the stellar disk of a galaxy, is especially interesting. It provides a wealth of information about in and outflowing gaseous material towards and away from galaxies and their hierarchical evolution. For the Milky Way, the so-called high-velocity clouds (HVCs), fast moving neutral gas complexes in the halo that can be traced by absorption-line measurements, are believed to play a crucial role in the overall matter cycle in our Galaxy. Over the last decades, the properties of these halo structures and their connection to the local circumgalactic and intergalactic medium (CGM and IGM, respectively) have been investigated in great detail by many different groups. So far it remains unclear, however, to what extent the results of these studies can be transferred to other galaxies in the local Universe. In this thesis, we study the absorption properties of Galactic HVCs and compare the HVC absorption characteristics with those of intervening QSO absorption-line systems at low redshift. The goal of this project is to improve our understanding of the spatial extent and physical conditions of gaseous galaxy halos in the local Universe. In the first part of the thesis we use HST /STIS ultraviolet spectra of more than 40 extragalactic background sources to statistically analyze the absorption properties of the HVCs in the Galactic halo. We determine fundamental absorption line parameters including covering fractions of different weakly/intermediately/highly ionized metals with a particular focus on SiII and MgII. Due to the similarity in the ionization properties of SiII and MgII, we are able to estimate the contribution of HVC-like halo structures to the cross section of intervening strong MgII absorbers at z = 0. Our study implies that only the most massive HVCs would be regarded as strong MgII absorbers, if the Milky Way halo would be seen as a QSO absorption line system from an exterior vantage point. Combining the observed absorption-cross section of Galactic HVCs with the well-known number density of intervening strong MgII absorbers at z = 0, we conclude that the contribution of infalling gas clouds (i.e., HVC analogs) in the halos of Milky Way-type galaxies to the cross section of strong MgII absorbers is 34%. This result indicates that only about one third of the strong MgII absorption can be associated with HVC analogs around other galaxies, while the majority of the strong MgII systems possibly is related to galaxy outflows and winds. The second part of this thesis focuses on the properties of intervening metal absorbers at low redshift. The analysis of the frequency and physical conditions of intervening metal systems in QSO spectra and their relation to nearby galaxies offers new insights into the typical conditions of gaseous galaxy halos. One major aspect in our study was to regard intervening metal systems as possible HVC analogs. We perform a detailed analysis of absorption line properties and line statistics for 57 metal absorbers along 78 QSO sightlines using newly-obtained ultraviolet spectra obtained with HST /COS. We find clear evidence for bimodal distribution in the HI column density in the absorbers, a trend that we interpret as sign for two different classes of absorption systems (with HVC analogs at the high-column density end). With the help of the strong transitions of SiII λ1260, SiIII λ1206, and CIII λ977 we have set up Cloudy photoionization models to estimate the local ionization conditions, gas densities, and metallicities. We find that the intervening absorption systems studied by us have, on average, similar physical conditions as Galactic HVC absorbers, providing evidence that many of them represent HVC analogs in the vicinity of other galaxies. We therefore determine typical halo sizes for SiII, SiIII, and CIII for L = 0.01L∗ and L = 0.05L∗ galaxies. Based on the covering fractions of the different ions in the Galactic halo, we find that, for example, the typical halo size for SiIII is ∼ 160 kpc for L = 0.05L∗ galaxies. We test the plausibility of this result by searching for known galaxies close to the QSO sightlines and at similar redshifts as the absorbers. We find that more than 34% of the measured SiIII absorbers have galaxies associated with them, with the majority of the absorbers indeed being at impact parameters ρ ≤160 kpc. N2 - Galaxien bestehen nicht nur aus Planeten und Sternen, sondern sind u.a. auch von einer Hülle aus Gas und Staub, dem Halo, umgeben. Dieser Halo spielt für die Entwicklung der Galaxie eine zentrale Rolle, da er mit der galaktischen Scheibe wechselwirken kann. Für das Verständnis des galaktischen Materiekreislaufs ist es daher entscheidend, die Prozesse und Vorgänge sowie das Zusammenspiel der verschiedenen Gasphasen in diesem Übergangsbereich zum intergalaktischen Medium charakterisieren und verstehen zu können. In der vorliegenden Arbeit werden lokale Phänomene, die sogenannten Hochgeschwindigkeitswolken (HVCs), im Halo der Milchstraße mit Hilfe des Hubble-Weltraumteleskops analysiert und ausgewertet. Im Gegensatz zu dem normalen Halo Gas bewegen sich diese HVCs mit ungewöhnlich hohen Geschwindigkeiten durch die ̈ äußeren Bereiche der Milchstraße. Sie passen daher nicht in das Galaktische Ge- schwindigkeitsmodell und stellen eine eigene, wichtige Klasse von Objekten dar, welche mit der Galaxie wechselwirken und diese beeinflussen. Für die Analyse dieser HVCs werden mehr als 40 Spektren von extragalaktischen Hintergrundquellen statistisch untersucht, um u.a. den Bedeckungsanteil von verschiedenen niedrig-/mittel- und hochionisierten Metallen zu ermitteln. Wegen der Ähnlichkeit der Ionisationsparameter von einfach ionisiertem Silizium, SiII, und einfach ionisiertem Magnesium, MgII, ist es möglich, den Beitrag von HVCs zum Wirkungsquerschnitt von starken MgII Absorbern im lokalen Universum zu bestimmen. Es stellt sich heraus, dass, würde man von außen auf die Milchstraße schauen, Galaktische HVCs etwa 52 % zum totalen Wirkungsquerschnitt von starken MgII Absorptionssystemen in der Milchstraße beitragen. Weiterhin ergibt sich, dass nur etwa ein Drittel der starken MgII Absorptionssysteme in der Umgebung von Milchstraßen-ähnlichen Galaxien als HVC Gegenstücke identifziert werden kann. Betrachtet man die große Anzahl an bekannten MgII Absorptionssystemen folgt daraus, dass das HVC-Phänomen nicht alleine auf unsere Galaxie beschränkt ist, sondern im Gegenteil, weit verbreitet zu sein scheint. Weiterhin werden die Eigenschaften von Metallsystemen bei niedriger Rotverschiebung in Quasarspektren analysiert. Die Suche nach extragalaktischen Metallsystemen in einer Vielzahl von Spektren und deren statistische Auswertung bezogen auf ihre Ursprungsgalaxien ermöglicht es, neue Erkenntnisse über die typische Struktur von Halos Milchstraßen-ähnlicher Galaxien zu erlangen. Eine der Hauptfragestellungen ist die Identifizierung von entfernten Metallsystemen als HVC-Analoga. Dazu wurden weitere Quasarspektren des Hubble-Teleskops ausgewertet und mit den Ergebnissen über Galaktische HVCs verglichen. Es zeigt sich hierbei, dass z.B. in der Säulendichteverteilung von neutralem Wasserstoff eine deutliche zweikomponentige Struktur zu erkennen ist. Diese könnte das Resultat von zwei verschiedenen Absorber Populationen sein, wobei eine HVC-ähnliche Eigenschaften aufweist. Diese Absorptionssysteme besitzen im Mittel sehr ähnliche Eigenschaften wie Galaktische Absorber, z.B. in Bezug auf die Eigenschaften des Gases oder dessen Zusammensetzung. Das impliziert u.a., dass sich auch dazugehörige Galaxien innerhalb eines bestimmten Abstandes um diese Absorber befinden sollten. Diese Vermutung wird anhand der Daten exemplarisch für zweichfach ionisiertes Silizium, SiII, untersucht. Es stellt sich heraus, dass sich in mehr als 34 % der Fälle zugehörige Galaxien bei SiIII Absorbern befinden, wobei die Mehrheit sogar innerhalb des von uns ermittelten mittleren Detektionsradius von 160 kpc zu finden ist. Allgemein können wir viele Hinweise darauf finden, dass das HVC-Phänomen nicht nur auf die Milchstraße beschränkt, sondern weit verbreitet ist. Zusätzlich scheinen Metallsysteme in Quasarspektren gute Indikatoren für HVC-Analoga in der Umgebung von anderen entfernten Galaxien zu sein. KW - Halo KW - Hochgeschwindigkeitswolken KW - Galaxien KW - Spektroskopie KW - halo KW - high-velocity-clouds KW - galaxies KW - spectroscopy Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus-70513 ER - TY - JOUR A1 - Aliu, E. A1 - Archambault, S. A1 - Arlen, T. A1 - Aune, T. A1 - Behera, B. A1 - Beilicke, M. A1 - Benbow, W. A1 - Berger, K. A1 - Bird, R. A1 - Bouvier, A. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cerruti, M. A1 - Chen, Xuhui A1 - Ciupik, L. A1 - Connolly, M. P. A1 - Cui, W. A1 - Duke, C. A1 - Dumm, J. A1 - Errando, M. A1 - Falcone, A. A1 - Federici, S. A1 - Feng, Q. A1 - Finley, J. P. A1 - Fleischhack, H. A1 - Fortin, P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gillanders, G. H. A1 - Griffin, S. A1 - Griffiths, S. T. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Humensky, T. B. A1 - Johnson, C. A. A1 - Kaaret, P. A1 - Kertzman, M. A1 - Khassen, Y. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Madhavan, A. S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Meagher, K. A1 - Millis, J. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nieto, D. A1 - Ong, R. A. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, M. A1 - Popkow, A. A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Sembroski, G. H. A1 - Smith, A. W. A1 - Staszak, D. A1 - Telezhinsky, Igor O. A1 - Theiling, M. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Wakely, S. P. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Welsing, R. A1 - Williams, D. A. A1 - Zajczyk, A. A1 - Zitzer, B. T1 - A three-year multi-wavelenght study of the very-high-energy gamma-ray Blazar 1ES 0229+200 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics KW - BL Lacertae objects: general KW - BL Lacertae objects: individual (1ES 0229+200, VER J0232+202) KW - diffuse radiation KW - galaxies: active KW - gamma rays: general KW - magnetic fields Y1 - 2014 U6 - https://doi.org/10.1088/0004-637X/782/1/13 SN - 0004-637X SN - 1538-4357 VL - 782 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Gerhardt, Matthias A1 - Ecke, Mary A1 - Walz, Michael A1 - Stengl, Andreas A1 - Beta, Carsten A1 - Gerisch, Günther T1 - Actin and PIP3 waves in giant cells reveal the inherent length scale of an excited state JF - Journal of cell science N2 - The membrane and actin cortex of a motile cell can autonomously differentiate into two states, one typical of the front, the other of the tail. On the substrate-attached surface of Dictyostelium discoideum cells, dynamic patterns of front-like and tail-like states are generated that are well suited to monitor transitions between these states. To image large-scale pattern dynamics independently of boundary effects, we produced giant cells by electric-pulse-induced cell fusion. In these cells, actin waves are coupled to the front and back of phosphatidylinositol (3,4,5)-trisphosphate (PIP3)-rich bands that have a finite width. These composite waves propagate across the plasma membrane of the giant cells with undiminished velocity. After any disturbance, the bands of PIP3 return to their intrinsic width. Upon collision, the waves locally annihilate each other and change direction; at the cell border they are either extinguished or reflected. Accordingly, expanding areas of progressing PIP3 synthesis become unstable beyond a critical radius, their center switching from a front-like to a tail-like state. Our data suggest that PIP3 patterns in normal-sized cells are segments of the self-organizing patterns that evolve in giant cells. KW - Actin waves KW - PIP3 signals KW - Excitable systems KW - Cell polarity KW - Cell fusion Y1 - 2014 U6 - https://doi.org/10.1242/jcs.156000 SN - 0021-9533 SN - 1477-9137 VL - 127 IS - 20 SP - 4507 EP - 4517 PB - Company of Biologists Limited CY - Cambridge ER - TY - THES A1 - Yadavalli, Nataraja Sekhar T1 - Advances in experimental methods to probe surface relief grating formation mechanism in photosensitive materials T1 - Entstehung von Oberflächengittern in lichtempfindlichen Materialien N2 - When azobenzene-modified photosensitive polymer films are irradiated with light interference patterns, topographic variations in the film develop that follow the electric field vector distribution resulting in the formation of surface relief grating (SRG). The exact correspondence of the electric field vector orientation in interference pattern in relation to the presence of local topographic minima or maxima of SRG is in general difficult to determine. In my thesis, we have established a systematic procedure to accomplish the correlation between different interference patterns and the topography of SRG. For this, we devise a new setup combining an atomic force microscope and a two-beam interferometer (IIAFM). With this set-up, it is possible to track the topography change in-situ, while at the same time changing polarization and phase of the impinging interference pattern. To validate our results, we have compared two photosensitive materials named in short as PAZO and trimer. This is the first time that an absolute correspondence between the local distribution of electric field vectors of interference pattern and the local topography of the relief grating could be established exhaustively. In addition, using our IIAFM we found that for a certain polarization combination of two orthogonally polarized interfering beams namely SP (↕, ↔) interference pattern, the topography forms SRG with only half the period of the interference patterns. Exploiting this phenomenon we are able to fabricate surface relief structures below diffraction limit with characteristic features measuring only 140 nm, by using far field optics with a wavelength of 491 nm. We have also probed for the stresses induced during the polymer mass transport by placing an ultra-thin gold film on top (5–30 nm). During irradiation, the metal film not only deforms along with the SRG formation, but ruptures in regular and complex manner. The morphology of the cracks differs strongly depending on the electric field distribution in the interference pattern even when the magnitude and the kinetic of the strain are kept constant. This implies a complex local distribution of the opto-mechanical stress along the topography grating. The neutron reflectivity measurements of the metal/polymer interface indicate the penetration of metal layer within the polymer resulting in the formation of bonding layer that confirms the transduction of light induced stresses in the polymer layer to a metal film. N2 - Azobenzolhaltige Polymere gehören zu einer Klasse funktionaler Materialien, bei denen durch ein äußeres Strahlungsfeld eine starke mechanische Reaktion ausgelöst werden kann. Durch die Bindung an das Polymerrückgrat können die Azobenzole, die unter UV-Belichtung eine Photoisomerisierung ausführen, was zum Teil drastische Effekte zur Folge hat. Unter Belichtung mit Intensitätsmustern, d.h. mit räumlich variierender Verteilung der Polarisation oder der Intensität des einfallenden Lichts verändert sich die Topographie der azobenzolhaltigen Filme, was zur Bildung von Oberflächengittern (engl. Surface Relief Gratings, SRG) führt. In dieser Arbeit wurde eine neue Methode vorgeschlagen, bei der das Verhalten elastischer/morphologischer Eigenschaften unter verschiedenen Belichtungsbedingungen, d.h. mit unterschiedlicher Verteilung der Polarisation und der Intensität in situ lokal als Funktion der Position entlang der SRG aufgenommen werden kann. Außerdem wurde hier vorgeschlagen, opto-mechanische Spannungen, die innerhalb der photosensitiven Polymerfilme während der Belichtung entstehen, mit Hilfe dünner aufgebrachter metallischen Schichten abzubilden und zu analysieren. KW - Azobenzolhaltige Polymerfilme KW - Oberflächengitter KW - In-situ Rasterkraftmikroskopie KW - Opto-mechanische Spannungen KW - Metall/Graphen/Polymer Grenzfläch KW - azobenzene polymer films KW - surface relief grating KW - in-situ atomic force microscopy KW - opto-mechanical stresses KW - metal/polymer interfaces Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus-71213 ER - TY - THES A1 - Schmidt, Lukas T1 - Aerosols and boundary layer structure over Arctic sea ice based on airborne lidar and dropsonde measurements T1 - Aerosol und Grenzschichtstruktur über arktischem Meereis anhand von Flugzeuggetragenen Lidar- und Dropsonden- Messungen N2 - The atmosphere over the Arctic Ocean is strongly influenced by the distribution of sea ice and open water. Leads in the sea ice produce strong convective fluxes of sensible and latent heat and release aerosol particles into the atmosphere. They increase the occurrence of clouds and modify the structure and characteristics of the atmospheric boundary layer (ABL) and thereby influence the Arctic climate. In the course of this study aircraft measurements were performed over the western Arctic Ocean as part of the campaign PAMARCMIP 2012 of the Alfred Wegener Institute for Polar and Marine Research (AWI). Backscatter from aerosols and clouds within the lower troposphere and the ABL were measured with the nadir pointing Airborne Mobile Aerosol Lidar (AMALi) and dropsondes were launched to obtain profiles of meteorological variables. Furthermore, in situ measurements of aerosol properties, meteorological variables and turbulence were part of the campaign. The measurements covered a broad range of atmospheric and sea ice conditions. In this thesis, properties of the ABL over Arctic sea ice with a focus on the influence of open leads are studied based on the data from the PAMARCMIP campaign. The height of the ABL is determined by different methods that are applied to dropsonde and AMALi backscatter profiles. ABL heights are compared for different flights representing different conditions of the atmosphere and of sea ice and open water influence. The different criteria for ABL height that are applied show large variation in terms of agreement among each other, depending on the characteristics of the ABL and its history. It is shown that ABL height determination from lidar backscatter by methods commonly used under mid-latitude conditions is applicable to the Arctic ABL only under certain conditions. Aerosol or clouds within the ABL are needed as a tracer for ABL height detection from backscatter. Hence an aerosol source close to the surface is necessary, that is typically found under the present influence of open water and therefore convective conditions. However it is not always possible to distinguish residual layers from the actual ABL. Stable boundary layers are generally difficult to detect. To illustrate the complexity of the Arctic ABL and processes therein, four case studies are analyzed each of which represents a snapshot of the interplay between atmosphere and underlying sea ice or water surface. Influences of leads and open water on the aerosol and clouds within the ABL are identified and discussed. Leads are observed to cause the formation of fog and cloud layers within the ABL by humidity emission. Furthermore they decrease the stability and increase the height of the ABL and consequently facilitate entrainment of air and aerosol layers from the free troposphere. N2 - Die Verteilung von Meereis und offenem Wasser hat einen starken Einfluss auf die Atmosphäre über dem arktischen Ozean. Eisrinnen (sog. Leads) verursachen konvektive Flüsse von latenter und sensibler Wärme und führen zum Eintrag von Aerosolpartikeln in die Atmosphäre. Dadurch führen sie zum vermehrten Auftreten von Wolken und modifizieren die Struktur und die Eigenschaften der atmosphärischen Grenzschicht (ABL), wodurch das arktische Klima beeinflusst wird. Im Rahmen der Messkampagne PAMARCMIP 2012 des Alfred-Wegener-Instituts (AWI) wurden als Teil dieser Arbeit über dem westlichen arktischen Ozean Flugzeugmessungen durchgeführt. Mithilfe des nach unten gerichteten Airborne Mobile Aerosol Lidar (AMALi) wurde die Rückstreuung von Aerosolen und Wolken in der unteren Troposphäre und ABL gemessen. Dropsonden wurden verwendet, um Profile meteorologischer Größen zu erhalten. Zudem wurden in situ Messungen von Aerosoleigenschaften, meteorologischen Variablen und der Turbulenz durchgeführt. In dieser Arbeit werden die Eigenschaften der ABL über arktischem Meereis basierend auf den Daten der PAMARCMIP Kampagne untersucht. Dabei liegt der Fokus auf dem Einfluss offener Leads auf die ABL. Aus den gewonnenen Dropsondendaten und AMALi Rückstreuprofilen wird die Höhe der ABL mithilfe verschiedener Methoden bestimmt. Die für verschiedene Messflüge und somit unterschiedliche atmosphärische Bedingungen sowie Meereisverteilungen berechneten ABL Höhen werden miteinander verglichen, und somit der Einfluss von offenem Wasser auf die ABL untersucht. Die verschiedenen Methoden zur Bestimmung der ABL Höhe führen zu unterschiedlichen Ergebnissen, je nach Eigenschaften der ABL und ihrer Geschichte. Es wird gezeigt, dass die Methoden für die ABL Höhen-Bestimmung aus der Lidar Rückstreuung, die gewöhnlich für die mittleren Breiten verwendet werden, nur bedingt für arktische Bedingungen geeignet ist. Um die ABL Höhe aus der Rückstreuung ableiten zu können, müssen Aerosole oder Wolken in der Grenzschicht als Tracer vorhanden sein. Dazu ist eine Aerosolquelle nahe der Oberfläche notwendig, welche typischerweise unter dem Einfluss von offenem Wasser und konvektiven Bedingungen vorliegt. Dennoch ist es nicht immer möglich, die aktuelle Grenzschicht von residualen Schichten zu unterscheiden. Stabile Grenzschichten sind im Allgemeinen schwer zu detektieren. Um die Komplexität der arktischen Grenzschicht und die beteiligten Prozesse zu veranschaulichen, werden vier Fallstudien detailliert analysiert, welche jeweils eine Momentaufnahme des Zusammenspiels von Atmosphäre und Meereis oder Wasseroberfläche darstellen. Der Einfluss von Leads und offenem Wasser auf Aerosol und Wolken in der ABL werden identifiziert und diskutiert. Die Bildung von Wolken- und Nebelschichten, verursacht durch den Feuchteeintrag über offenen Leads, wird beobachtet. Zudem verringern leads die Stabilität der ABL, führen zu einer Zunahme ihrer Höhe und begünstigen dadurch Entrainment von Luft und Aerosolschichten aus der freien Troposphäre. KW - polar KW - atmosphere KW - AMALi KW - Polar 5 KW - lead KW - polar KW - Atmosphäre KW - AMALi KW - Polar 5 KW - Eisrinne Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-75076 ER - TY - JOUR A1 - Cherstvy, Andrey G. A1 - Chechkin, Aleksei V. A1 - Metzler, Ralf T1 - Ageing and confinement in non-ergodic heterogeneous diffusion processes JF - Journal of physics : A, Mathematical and theoretical N2 - We study the effects of ageing-the time delay between initiation of the physical process at t = 0 and start of observation at some time t(a) > 0-and spatial confinement on the properties of heterogeneous diffusion processes (HDPs) with deterministic power-law space-dependent diffusivities, D(x) = D-0 vertical bar x vertical bar(alpha). From analysis of the ensemble and time averaged mean squared displacements and the ergodicity breaking parameter quantifying the inherent degree of irreproducibility of individual realizations of the HDP we obtain striking similarities to ageing subdiffusive continuous time random walks with scale-free waiting time distributions. We also explore how both processes can be distinguished. For confined HDPs we study the long-time saturation of the ensemble and time averaged particle displacements as well as the magnitude of the inherent scatter of time averaged displacements and contrast the outcomes to the results known for other anomalous diffusion processes under confinement. KW - stochastic processes KW - anomalous diffusion KW - ageing KW - weak ergodicity breaking Y1 - 2014 U6 - https://doi.org/10.1088/1751-8113/47/48/485002 SN - 1751-8113 SN - 1751-8121 VL - 47 IS - 48 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Metzler, Ralf A1 - Sanders, L. A1 - Lomholt, M. A. A1 - Lizana, L. A1 - Fogelmark, K. A1 - Ambjoernsson, Tobias T1 - Ageing single file motion JF - The European physical journal Y1 - 2014 U6 - https://doi.org/10.1140/epjst/e2014-02333-5 SN - 1951-6355 SN - 1951-6401 VL - 223 IS - 14 SP - 3287 EP - 3293 PB - Springer CY - Heidelberg ER - TY - JOUR A1 - Schulz, Johannes H. P. A1 - Barkai, Eli A1 - Metzler, Ralf T1 - Aging renewal theory and application to random walks JF - Physical review : X, Expanding access N2 - We discuss a renewal process in which successive events are separated by scale-free waiting time periods. Among other ubiquitous long-time properties, this process exhibits aging: events counted initially in a time interval [0, t] statistically strongly differ from those observed at later times [t(a,) t(a) + t]. The versatility of renewal theory is owed to its abstract formulation. Renewals can be interpreted as steps of a random walk, switching events in two-state models, domain crossings of a random motion, etc. In complex, disordered media, processes with scale-free waiting times play a particularly prominent role. We set up a unified analytical foundation for such anomalous dynamics by discussing in detail the distribution of the aging renewal process. We analyze its half-discrete, half-continuous nature and study its aging time evolution. These results are readily used to discuss a scale-free anomalous diffusion process, the continuous-time random walk. By this, we not only shed light on the profound origins of its characteristic features, such as weak ergodicity breaking, along the way, we also add an extended discussion on aging effects. In particular, we find that the aging behavior of time and ensemble averages is conceptually very distinct, but their time scaling is identical at high ages. Finally, we show how more complex motion models are readily constructed on the basis of aging renewal dynamics. Y1 - 2014 U6 - https://doi.org/10.1103/PhysRevX.4.011028 SN - 2160-3308 VL - 4 IS - 1 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Zhao, Qiang A1 - Dunlop, John William Chapman A1 - Qiu, Xunlin A1 - Huang, Feihe A1 - Zhang, Zibin A1 - Heyda, Jan A1 - Dzubiella, Joachim A1 - Antonietti, Markus A1 - Yuan, Jiayin T1 - An instant multi-responsive porous polymer actuator driven by solvent molecule sorption JF - Nature Communications N2 - Fast actuation speed, large-shape deformation and robust responsiveness are critical to synthetic soft actuators. A simultaneous optimization of all these aspects without trade-offs remains unresolved. Here we describe porous polymer actuators that bend in response to acetone vapour (24 kPa, 20 degrees C) at a speed of an order of magnitude faster than the state-of-the-art, coupled with a large-scale locomotion. They are meanwhile multi-responsive towards a variety of organic vapours in both the dry and wet states, thus distinctive from the traditional gel actuation systems that become inactive when dried. The actuator is easy-to-make and survives even after hydrothermal processing (200 degrees C, 24 h) and pressing-pressure (100 MPa) treatments. In addition, the beneficial responsiveness is transferable, being able to turn 'inert' objects into actuators through surface coating. This advanced actuator arises from the unique combination of porous morphology, gradient structure and the interaction between solvent molecules and actuator materials. Y1 - 2014 U6 - https://doi.org/10.1038/ncomms5293 SN - 2041-1723 VL - 5 PB - Nature Publ. Group CY - London ER - TY - JOUR A1 - Goychuk, Igor A1 - Kharchenko, Vasyl O. T1 - Anomalous features of diffusion in corrugated potentials with spatial correlations: Faster than normal, and other surprises JF - Physical review letters N2 - Normal diffusion in corrugated potentials with spatially uncorrelated Gaussian energy disorder famously explains the origin of non-Arrhenius exp[-sigma(2)/(k(B)T(2))] temperature dependence in disordered systems. Here we show that unbiased diffusion remains asymptotically normal also in the presence of spatial correlations decaying to zero. However, because of a temporal lack of self-averaging, transient subdiffusion emerges on the mesoscale, and it can readily reach macroscale even for moderately strong disorder fluctuations of sigma similar to 4 - 5k(B)T. Because of its nonergodic origin, such subdiffusion exhibits a large scatter in single-trajectory averages. However, at odds with intuition, it occurs essentially faster than one expects from the normal diffusion in the absence of correlations. We apply these results to diffusion of regulatory proteins on DNA molecules and predict that such diffusion should be anomalous, but much faster than earlier expected on a typical length of genes for a realistic energy disorder of several room k(B)T, or merely 0.05-0.075 eV. Y1 - 2014 U6 - https://doi.org/10.1103/PhysRevLett.113.100601 SN - 0031-9007 SN - 1079-7114 VL - 113 IS - 10 PB - American Physical Society CY - College Park ER - TY - THES A1 - Zhou, Xu T1 - Atmospheric interactions with land surface in the arctic based on regional climate model solutions Y1 - 2014 ER - TY - JOUR A1 - Kruglov, Vyacheslav P. A1 - Kuznetsov, Sergey P. A1 - Pikovskij, Arkadij T1 - Attractor of Smale - Williams type in an autonomous distributed system JF - Regular and chaotic dynamics : international scientific journal N2 - We consider an autonomous system of partial differential equations for a one-dimensional distributed medium with periodic boundary conditions. Dynamics in time consists of alternating birth and death of patterns with spatial phases transformed from one stage of activity to another by the doubly expanding circle map. So, the attractor in the Poincar, section is uniformly hyperbolic, a kind of Smale - Williams solenoid. Finite-dimensional models are derived as ordinary differential equations for amplitudes of spatial Fourier modes (the 5D and 7D models). Correspondence of the reduced models to the original system is demonstrated numerically. Computational verification of the hyperbolicity criterion is performed for the reduced models: the distribution of angles of intersection for stable and unstable manifolds on the attractor is separated from zero, i.e., the touches are excluded. The example considered gives a partial justification for the old hopes that the chaotic behavior of autonomous distributed systems may be associated with uniformly hyperbolic attractors. KW - Smale - Williams solenoid KW - hyperbolic attractor KW - chaos KW - Swift - Hohenberg equation KW - Lyapunov exponent Y1 - 2014 U6 - https://doi.org/10.1134/S1560354714040042 SN - 1560-3547 SN - 1468-4845 VL - 19 IS - 4 SP - 483 EP - 494 PB - Pleiades Publ. CY - New York ER - TY - JOUR A1 - Hubrig, Swetlana A1 - Fossati, Luca A1 - Carroll, Thorsten Anthony A1 - Castro, Norberto A1 - Gonzalez, J. F. A1 - Ilyin, Ilya A1 - Przybilla, Norbert A1 - Schoeller, M. A1 - Oskinova, Lida A1 - Morel, T. A1 - Langer, N. A1 - Scholz, Ralf-Dieter A1 - Kharchenko, N. V. A1 - Nieva, M. -F. T1 - B fields in OB stars (BOB): The discovery of a magnetic field in a multiple system in the Trifid nebula, one of the youngest star forming regions JF - Astronomy and astrophysics : an international weekly journal N2 - Aims. Recent magnetic field surveys in O- and B-type stars revealed that about 10% of the core-hydrogen-burning massive stars host large-scale magnetic fields. The physical origin of these fields is highly debated. To identify and model the physical processes responsible for the generation of magnetic fields in massive stars, it is important to establish whether magnetic massive stars are found in very young star-forming regions or whether they are formed in close interacting binary systems. Methods. In the framework of our ESO Large Program, we carried out low-resolution spectropolarimetric observations with FORS 2 in 2013 April of the three most massive central stars in the Trifid nebula, HD 164492A, HD 164492C, and HD 164492D. These observations indicated a strong longitudinal magnetic field of about 500-600 G in the poorly studied component HD 164492C. To confirm this detection, we used HARPS in spectropolarimetric mode on two consecutive nights in 2013 June. Results. Our HARPS observations confirmed the longitudinal magnetic field in HD 164492C. Furthermore, the HARPS observations revealed that HD 164492C cannot be considered as a single star as it possesses one or two companions. The spectral appearance indicates that the primary is most likely of spectral type B1-B1.5 V. Since in both observing nights most spectral lines appear blended, it is currently unclear which components are magnetic. Long-term monitoring using high-resolution spectropolarimetry is necessary to separate the contribution of each component to the magnetic signal. Given the location of the system HD 164492C in one of the youngest star formation regions, this system can be considered as a Rosetta Stone for our understanding of the origin of magnetic fields in massive stars. KW - binaries: close KW - stars: early-type KW - stars: fundamental parameters KW - stars: magnetic field KW - stars: variables: general KW - stars: individual: HD 164492C Y1 - 2014 U6 - https://doi.org/10.1051/0004-6361/201423490 SN - 0004-6361 SN - 1432-0746 VL - 564 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Rosenau, Philip A1 - Pikovskij, Arkadij T1 - Breathers in strongly anharmonic lattices JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - We present and study a family of finite amplitude breathers on a genuinely anharmonic Klein-Gordon lattice embedded in a nonlinear site potential. The direct numerical simulations are supported by a quasilinear Schrodinger equation (QLS) derived by averaging out the fast oscillations assuming small, albeit finite, amplitude vibrations. The genuinely anharmonic interlattice forces induce breathers which are strongly localized with tails evanescing at a doubly exponential rate and are either close to a continuum, with discrete effects being suppressed, or close to an anticontinuum state, with discrete effects being enhanced. Whereas the D-QLS breathers appear to be always stable, in general there is a stability threshold which improves with spareness of the lattice. Y1 - 2014 U6 - https://doi.org/10.1103/PhysRevE.89.022924 SN - 1539-3755 SN - 1550-2376 VL - 89 IS - 2 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Talukder, Srijeeta A1 - Sen, Shrabani A1 - Chakraborti, Prantik A1 - Metzler, Ralf A1 - Banik, Suman K. A1 - Chaudhury, Pinaki T1 - Breathing dynamics based parameter sensitivity analysis of hetero-polymeric DNA JF - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - We study the parameter sensitivity of hetero-polymeric DNA within the purview of DNA breathing dynamics. The degree of correlation between the mean bubble size and the model parameters is estimated for this purpose for three different DNA sequences. The analysis leads us to a better understanding of the sequence dependent nature of the breathing dynamics of hetero-polymeric DNA. Out of the 14 model parameters for DNA stability in the statistical Poland-Scheraga approach, the hydrogen bond interaction epsilon(hb)(AT) for an AT base pair and the ring factor. turn out to be the most sensitive parameters. In addition, the stacking interaction epsilon(st)(TA-TA) for an TA-TA nearest neighbor pair of base-pairs is found to be the most sensitive one among all stacking interactions. Moreover, we also establish that the nature of stacking interaction has a deciding effect on the DNA breathing dynamics, not the number of times a particular stacking interaction appears in a sequence. We show that the sensitivity analysis can be used as an effective measure to guide a stochastic optimization technique to find the kinetic rate constants related to the dynamics as opposed to the case where the rate constants are measured using the conventional unbiased way of optimization. (c) 2014 AIP Publishing LLC. Y1 - 2014 U6 - https://doi.org/10.1063/1.4869112 SN - 0021-9606 SN - 1089-7690 VL - 140 IS - 12 PB - American Institute of Physics CY - Melville ER - TY - GEN A1 - Talukder, Srijeeta A1 - Sen, Shrabani A1 - Chakraborti, Prantik A1 - Metzler, Ralf A1 - Banik, Suman K. A1 - Chaudhury, Pinaki T1 - Breathing dynamics based parameter sensitivity analysis of hetero-polymeric DNA T2 - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - We study the parameter sensitivity of hetero-polymeric DNA within the purview of DNA breathing dynamics. The degree of correlation between the mean bubble size and the model parameters is estimated for this purpose for three different DNA sequences. The analysis leads us to a better understanding of the sequence dependent nature of the breathing dynamics of hetero-polymeric DNA. Out of the 14 model parameters for DNA stability in the statistical Poland-Scheraga approach, the hydrogen bond interaction epsilon(hb)(AT) for an AT base pair and the ring factor. turn out to be the most sensitive parameters. In addition, the stacking interaction epsilon(st)(TA-TA) for an TA-TA nearest neighbor pair of base-pairs is found to be the most sensitive one among all stacking interactions. Moreover, we also establish that the nature of stacking interaction has a deciding effect on the DNA breathing dynamics, not the number of times a particular stacking interaction appears in a sequence. We show that the sensitivity analysis can be used as an effective measure to guide a stochastic optimization technique to find the kinetic rate constants related to the dynamics as opposed to the case where the rate constants are measured using the conventional unbiased way of optimization. Y1 - 2014 U6 - https://doi.org/10.1063/1.4871297 SN - 0021-9606 SN - 1089-7690 VL - 140 IS - 14 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Zink, Christof A1 - Niebuhr, Mario A1 - Jechow, Andreas A1 - Heuer, Axel A1 - Menzel, Ralf T1 - Broad area diode laser with on-chip transverse Bragg grating stabilized in an off-axis external cavity JF - Optics express : the international electronic journal of optics N2 - The emission characteristics of a novel, specially designed broad area diode laser (BAL) with on-chip transversal Bragg resonance (TBR) grating in lateral direction were investigated in an off-axis external cavity setup. The internal TBR grating defines a low loss transversal mode at a specific angle of incidence and a certain wavelength. By providing feedback at this specific angle with an external mirror, it is possible to select this low loss transverse mode and stabilize the BAL. Near diffraction limited emission with an almost single lobed far field pattern could be realized, in contrast to the double lobed far field pattern of similar setups using standard BALs or phase-locked diode laser arrays. Furthermore, we could achieve a narrow bandwidth emission with a simplified setup without external frequency selective elements. (C) 2014 Optical Society of America Y1 - 2014 U6 - https://doi.org/10.1364/OE.22.014108 SN - 1094-4087 VL - 22 IS - 12 SP - 14108 EP - 14113 PB - Optical Society of America CY - Washington ER - TY - JOUR A1 - Kliem, Bernhard A1 - Lin, J. A1 - Forbes, T. G. A1 - Priest, E. R. A1 - Toeroek, T. T1 - Catastrophe versus instability for the eruption of a toroadal solar magnetic flux JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - The onset of a solar eruption is formulated here as either a magnetic catastrophe or as an instability. Both start with the same equation of force balance governing the underlying equilibria. Using a toroidal flux rope in an external bipolar or quadrupolar field as a model for the current-carrying flux, we demonstrate the occurrence of a fold catastrophe by loss of equilibrium for several representative evolutionary sequences in the stable domain of parameter space. We verify that this catastrophe and the torus instability occur at the same point; they are thus equivalent descriptions for the onset condition of solar eruptions. KW - magnetohydrodynamics (MHD) KW - Sun: corona KW - Sun: coronal mass ejections (CMEs) KW - Sun: filaments, prominences KW - Sun: flares KW - Sun: magnetic fields Y1 - 2014 U6 - https://doi.org/10.1088/0004-637X/789/1/46 SN - 0004-637X SN - 1538-4357 VL - 789 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - GEN A1 - Liu, W. A1 - Tkachov, R. A1 - Komber, H. A1 - Senkovskyy, V. A1 - Schubert, M. A1 - Wei, Z. A1 - Facchetti, A. A1 - Neher, Dieter A1 - Kiriy, A. T1 - Chain-growth polycondensation of perylene diimide-based copolymers BT - a new route to regio-regular perylene diimide-based acceptors for all-polymer solar cells and n-type transistors N2 - Herein, we report the chain-growth tin-free room temperature polymerization method to synthesize n-type perylene diimide-dithiophene-based conjugated polymers (PPDIT2s) suitable for solar cell and transistor applications. The palladium/electron-rich tri-tert-butylphosphine catalyst is effective to enable the chain-growth polymerization of anion-radical monomer Br-TPDIT-Br/Zn to PPDIT2 with a molecular weight up to Mw ≈ 50 kg mol−1 and moderate polydispersity. This is the second example of the polymerization of unusual anion-radical aromatic complexes formed in a reaction of active Zn and electron-deficient diimide-based aryl halides. As such, the discovered polymerization method is not a specific reactivity feature of the naphthalene-diimide derivatives but is rather a general polymerization tool. This is an important finding, given the significantly higher maximum external quantum efficiency that can be reached with PDI-based copolymers (32–45%) in all-polymer solar cells compared to NDI-based materials (15–30%). Our studies revealed that PPDIT2 synthesized by the new method and the previously published polymer prepared by step-growth Stille polycondensation show similar electron mobility and all-polymer solar cell performance. At the same time, the polymerization reported herein has several technological advantages as it proceeds relatively fast at room temperature and does not involve toxic tin-based compounds. Because several chain-growth polymerization reactions are well-suited for the preparation of well-defined multi-functional polymer architectures, the next target is to explore the utility of the discovered polymerization in the synthesis of end-functionalized polymers and block copolymers. Such materials would be helpful to improve the nanoscale morphology of polymer blends in all-polymer solar cells. T3 - Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe - 273 Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-98724 ER - TY - JOUR A1 - Liu, W. A1 - Tkachov, R. A1 - Komber, H. A1 - Senkovskyy, V. A1 - Schubert, M. A1 - Wei, Z. A1 - Facchetti, A. A1 - Neher, Dieter A1 - Kiriy, A. T1 - Chain-growth polycondensation of perylene diimide-based copolymers: a new route to regio-regular perylene diimide-based acceptors for all-polymer solar cells and n-type transistors JF - Polymer Chemistry N2 - Herein, we report the chain-growth tin-free room temperature polymerization method to synthesize n-type perylene diimide-dithiophene-based conjugated polymers (PPDIT2s) suitable for solar cell and transistor applications. The palladium/electron-rich tri-tert-butylphosphine catalyst is effective to enable the chain-growth polymerization of anion-radical monomer Br-TPDIT-Br/Zn to PPDIT2 with a molecular weight up to M-w approximate to 50 kg mol(-1) and moderate polydispersity. This is the second example of the polymerization of unusual anion-radical aromatic complexes formed in a reaction of active Zn and electron-deficient diimide-based aryl halides. As such, the discovered polymerization method is not a specific reactivity feature of the naphthalene-diimide derivatives but is rather a general polymerization tool. This is an important finding, given the significantly higher maximum external quantum efficiency that can be reached with PDI-based copolymers (32-45%) in all-polymer solar cells compared to NDI-based materials (15-30%). Our studies revealed that PPDIT2 synthesized by the new method and the previously published polymer prepared by step-growth Stille polycondensation show similar electron mobility and all-polymer solar cell performance. At the same time, the polymerization reported herein has several technological advantages as it proceeds relatively fast at room temperature and does not involve toxic tin-based compounds. Because several chain-growth polymerization reactions are well-suited for the preparation of well-defined multi-functional polymer architectures, the next target is to explore the utility of the discovered polymerization in the synthesis of end-functionalized polymers and block copolymers. Such materials would be helpful to improve the nanoscale morphology of polymer blends in all-polymer solar cells. Y1 - 2014 U6 - https://doi.org/10.1039/c3py01707a SN - 1759-9954 SN - 1759-9962 VL - 5 IS - 10 SP - 3404 EP - 3411 PB - Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Kraffert, Felix A1 - Steyrleuthner, Robert A1 - Albrecht, Steve A1 - Neher, Dieter A1 - Scharber, Markus C. A1 - Bittl, Robert A1 - Behrends, Jan T1 - Charge Separation in PCPDTBT : PCBM Blends from an EPR Perspective JF - The journal of physical chemistry Y1 - 2014 U6 - https://doi.org/10.1021/jp509650v SN - 1932-7447 VL - 118 IS - 49 SP - 28482 EP - 28493 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Tremel, Kim A1 - Fischer, Florian S. U. A1 - Kayunkid, Navaphun A1 - Di Pietro, Riccardo A1 - Tkachov, Roman A1 - Kiriy, Anton A1 - Neher, Dieter A1 - Ludwigs, Sabine A1 - Brinkmann, Martin T1 - Charge transport anisotropy in highly oriented thin films of the acceptor polymer P(NDI2OD-T2) JF - dvanced energy materials N2 - The nanomorphology of the high mobility polymer poly{[N,N'-bis(2-octyldodecyl)-1,4,5,8-naphthalenedicarboximide-2,6-diyl]-alt-5,5'-(2,2'-bithiophene)} P(NDI2OD-T2) in thin films is explored as a function of different annealing conditions and correlated to optical and electrical properties. While nanofibrils with face-on orientation in form I are obtained directly after spin-coating and annealing below the melt transition temperature, clear evidence of lamellar structures is found after melt-annealing followed by slow cooling to room temperature. Interestingly these structural changes are accompanied by distinct changes in the absorption patterns. Electron diffraction measurements further show clear transitions towards predominant edge-on oriented chains in form II upon melt-annealing. Large-scale alignment with dichroic ratios up to 10 and improved order is achieved by high temperature rubbing and subsequent post-rubbing annealing. These highly oriented morphologies allow anisotropic in-plane charge transport to be probed with top-gate transistors parallel and perpendicular to the polymer chain direction. Mobilities up to 0.1 cm(2) V-1 s(-1) are observed parallel to the polymer chain, which is up to 10 times higher than those perpendicular to the polymer chain. Y1 - 2014 U6 - https://doi.org/10.1002/aenm.201301659 SN - 1614-6832 SN - 1614-6840 VL - 4 IS - 10 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Yeldesbay, Azamat A1 - Pikovskij, Arkadij A1 - Rosenblum, Michael T1 - Chimeralike states in an ensemble of globally coupled oscillators JF - Physical review letters N2 - We demonstrate the emergence of a complex state in a homogeneous ensemble of globally coupled identical oscillators, reminiscent of chimera states in nonlocally coupled oscillator lattices. In this regime some part of the ensemble forms a regularly evolving cluster, while all other units irregularly oscillate and remain asynchronous. We argue that the chimera emerges because of effective bistability, which dynamically appears in the originally monostable system due to internal delayed feedback in individual units. Additionally, we present two examples of chimeras in bistable systems with frequency-dependent phase shift in the global coupling. Y1 - 2014 U6 - https://doi.org/10.1103/PhysRevLett.112.144103 SN - 0031-9007 SN - 1079-7114 VL - 112 IS - 14 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Massa, D. A1 - Oskinova, Lida A1 - Fullerton, A. W. A1 - Prinja, R. K. A1 - Bohlender, D. A. A1 - Morrison, N. D. A1 - Blake, M. A1 - Pych, W. T1 - CIR modulation of the X-ray flux from the O7.5 III(n)((f)) star xi Persei(a similar to...)? JF - Monthly notices of the Royal Astronomical Society N2 - We analyse a 162 ks high energy transmission grating Chandra observation of the O7.5 III(n)((f)) star xi Per, together with contemporaneous H alpha observations. The X-ray spectrum of this star is similar to other single O stars, and not pathological in any way. Its UV wind lines are known to display cyclical time variability, with a period of 2.086 d, which is thought to be associated with corotating interaction regions (CIRs). We examine the Chandra and H alpha data for variability on this time-scale. We find that the X-rays vary by similar to 15 per cent over the course of the observations and that this variability is out of phase with variable absorption on the blue wing of the H alpha profiles (assumed to be a surrogate for the UV absorption associated with CIRs). While not conclusive, both sets of data are consistent with models where the CIRs are either a source of X-rays or modulate them. KW - stars: early-type KW - stars: individual: xi Persei KW - stars: mass loss KW - stars: winds, outflows KW - X-rays: stars Y1 - 2014 U6 - https://doi.org/10.1093/mnras/stu565 SN - 0035-8711 SN - 1365-2966 VL - 441 IS - 3 SP - 2173 EP - 2180 PB - Oxford Univ. Press CY - Oxford ER - TY - JOUR A1 - Kaiser, Eurika A1 - Noack, Bernd R. A1 - Cordier, Laurent A1 - Spohn, Andreas A1 - Segond, Marc A1 - Abel, Markus A1 - Daviller, Guillaume A1 - Osth, Jan A1 - Krajnovic, Sinisa A1 - Niven, Robert K. T1 - Cluster-based reduced-order modelling of a mixing layer JF - Journal of fluid mechanics KW - low-dimensional models KW - nonlinear dynamical systems KW - shear layers Y1 - 2014 U6 - https://doi.org/10.1017/jfm.2014.355 SN - 0022-1120 SN - 1469-7645 VL - 754 SP - 365 EP - 414 PB - Cambridge Univ. Press CY - New York ER - TY - JOUR A1 - Levanova, T. A. A1 - Osipov, Grigory V. A1 - Pikovskij, Arkadij T1 - Coherence properties of cycling chaos JF - Communications in nonlinear science & numerical simulation N2 - Cycling chaos is a heteroclinic connection between several chaotic attractors, at which switchings between the chaotic sets occur at growing time intervals. Here we characterize the coherence properties of these switchings, considering nearly periodic regimes that appear close to the cycling chaos due to imperfections or to instability. Using numerical simulations of coupled Lorenz, Roessler, and logistic map models, we show that the coherence is high in the case of imperfection (so that asymptotically the cycling chaos is very regular), while it is low close to instability of the cycling chaos. (C) 2014 Elsevier B. V. All rights reserved. KW - Heteroclinic cycle KW - Chaos KW - Coherence Y1 - 2014 U6 - https://doi.org/10.1016/j.cnsns.2014.01.011 SN - 1007-5704 SN - 1878-7274 VL - 19 IS - 8 SP - 2734 EP - 2739 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Godec, Aljaz A1 - Bauer, Maximilian A1 - Metzler, Ralf T1 - Collective dynamics effect transient subdiffusion of inert tracers in flexible gel networks JF - New journal of physics : the open-access journal for physics N2 - Based on extensive Brownian dynamics simulations we study the thermal motion of a tracer bead in a cross-linked, flexible gel in the limit when the tracer particle size is comparable to or even larger than the equilibrium mesh size of the gel. The analysis of long individual trajectories of the tracer demonstrates the existence of pronounced transient anomalous diffusion. From the time averaged mean squared displacement and the time averaged van Hove correlation functions we elucidate the many-body origin of the non-Brownian tracer bead dynamics. Our results shed new light onto the ongoing debate over the physical origin of steric tracer interactions with structured environments. KW - anomalous diffusion KW - gel network KW - van Hove correlation Y1 - 2014 U6 - https://doi.org/10.1088/1367-2630/16/9/092002 SN - 1367-2630 VL - 16 PB - IOP Publ. Ltd. CY - Bristol ER - TY - INPR A1 - Bürger, Gerd T1 - Comment on "Bias correction, quantile mapping, and downscaling: revisiting the inflation issue" T2 - Journal of climate N2 - In a recent paper, Maraun describes the adverse effects of quantile mapping on downscaling. He argues that when large-scale GCM variables are rescaled directly to small-scale fields or even station data, genuine small-scale covariability is lost and replaced by uniform variability inherited from the larger scales. This leads to a misrepresentation mainly of areal means and long-term trends. This comment acknowledges the former point, although the argument is relatively old, but disagrees with the latter, showing that grid-size long-term trends can be different from local trends. Finally, because it is partly incorrectly addressed, some clarification is added regarding the inflation issue, stressing that neither randomization nor inflation is free of unverified assumptions. KW - Climate change KW - Statistics KW - Climate variability Y1 - 2014 U6 - https://doi.org/10.1175/JCLI-D-13-00184.1 SN - 0894-8755 SN - 1520-0442 VL - 27 IS - 4 SP - 1819 EP - 1820 PB - American Meteorological Soc. CY - Boston ER - TY - INPR A1 - Föhlisch, Alexander A1 - de Groot, F. M. F. A1 - Odelius, Michael A1 - Techert, Simone A1 - Wernet, P. T1 - Comment on "state-dependent electron delocalization dynamics at the solute-solvent interface: soft-x-ray absorption spectroscopy and lambda b initio calculations" T2 - Physical review letters Y1 - 2014 U6 - https://doi.org/10.1103/PhysRevLett.112.129302 SN - 0031-9007 SN - 1079-7114 VL - 112 IS - 12 PB - American Physical Society CY - College Park ER - TY - THES A1 - Brem, Patrick T1 - Compact objects in dense astrophysical environments BT - numerical simulations and implications for gravitational wave astronomy Y1 - 2014 ER - TY - THES A1 - Yeldesbay, Azamat T1 - Complex regimes of synchronization T1 - Komplexe Synchronisationszustände BT - modeling and analysis N2 - Synchronization is a fundamental phenomenon in nature. It can be considered as a general property of self-sustained oscillators to adjust their rhythm in the presence of an interaction. In this work we investigate complex regimes of synchronization phenomena by means of theoretical analysis, numerical modeling, as well as practical analysis of experimental data. As a subject of our investigation we consider chimera state, where due to spontaneous symmetry-breaking of an initially homogeneous oscillators lattice split the system into two parts with different dynamics. Chimera state as a new synchronization phenomenon was first found in non-locally coupled oscillators system, and has attracted a lot of attention in the last decade. However, the recent studies indicate that this state is also possible in globally coupled systems. In the first part of this work, we show under which conditions the chimera-like state appears in a system of globally coupled identical oscillators with intrinsic delayed feedback. The results of the research explain how initially monostable oscillators became effectivly bistable in the presence of the coupling and create a mean field that sustain the coexistence of synchronized and desynchronized states. Also we discuss other examples, where chimera-like state appears due to frequency dependence of the phase shift in the bistable system. In the second part, we make further investigation of this topic by modeling influence of an external periodic force to an oscillator with intrinsic delayed feedback. We made stability analysis of the synchronized state and constructed Arnold tongues. The results explain formation of the chimera-like state and hysteric behavior of the synchronization area. Also, we consider two sets of parameters of the oscillator with symmetric and asymmetric Arnold tongues, that correspond to mono- and bi-stable regimes of the oscillator. In the third part, we demonstrate the results of the work, which was done in collaboration with our colleagues from Psychology Department of University of Potsdam. The project aimed to study the effect of the cardiac rhythm on human perception of time using synchronization analysis. From our part, we made a statistical analysis of the data obtained from the conducted experiment on free time interval reproduction task. We examined how ones heartbeat influences the time perception and searched for possible phase synchronization between heartbeat cycles and time reproduction responses. The findings support the prediction that cardiac cycles can serve as input signals, and is used for reproduction of time intervals in the range of several seconds. N2 - Synchronisation ist ein fundamentales Naturphänomen. Es ist die grundlegende Eigenschaft sich selbsterhaltender Oszillatoren, in Gegenwart einer Wechselwirkung, danach zu streben, ihre Rhythmen anzupassen. In dieser Arbeit betrachten wir komplexe Synchronisationszustände sowohl mit Hilfe analytischer Methoden als auch durch numerische Simulation und in experimentellen Daten. Unser Untersuchungsobjekt sind die sogenannten Chimera Zustände, in welchen sich Ensemble von gekoppelten, identischen Oszillatoren auf Grund eines Symmetriebruches spontan in Gruppen mit unterschiedlicher Dynamik aufteilen. Die Entdeckung von Chimeras in zunächst nichtlokal gekoppelten Systemen hat in den letzten zehn Jahren ein großes Interesse an neuartigen Synchronisationsphänomenen geweckt. Neueste Forschungsergebnisse belegen, dass diese Zustände unter bestimmten Bedingungen auch in global gekoppelten Systemen existieren können. Solche Bedingungen werden im ersten Teil der Arbeit in Ensemblen global gekoppelter Oszillatoren mit zusätzlicher, zeitverzögerter Selbstkopplung untersucht. Wir zeigen, wie zunächst monostabile Oszillatoren in Gegenwart von dem Treiben der globalen Kopplung effektiv bistabil werden, und sich so in zwei Gruppen organisieren. Das mittlere Feld, welches durch diese Gruppen aufgebaut wird, ist quasiperiodisch wodurch der Chimera Zustand sich selbst stabilisiert. In einem anderen Beispiel zeigen wir, dass der Chimera Zustand auch durch einen frequenzabhängigen Phasenunterschied in der globalen Kopplung erreicht werden kann. Zur genaueren Untersuchung der Mechanismen, die zur effektiven Bistabilität führen, betrachten wir im zweiten Teil der Arbeit den Einfluss einer externen periodischen Kraft auf einzelne Oszillatoren mit zeitverzögerter Selbstkopplung. Wir führen die Stabilitätanalyse des synchronen Zustands durch, und stellen die Arnoldzunge dar. Im dritten Teil der Arbeit stellen wir die Ergebnisse einer Synchronisationsanalyse vor, welche in Kooperation mit Wissenschaftlern der Psychologischen Fakultät der Universität Potsdam durchgeführt wurde. In dem Projekt wurde die Auswirkung des Herzrhythmus auf die menschliche Zeitwahrnehmung erforscht. Unsere Aufgabe war es, die experimentellen Daten statistisch zu analysieren. Im Experiment sollten Probanden ein gegebenes Zeitintervall reproduzieren während gleichzeitig ihr Herzschlag aufgezeichnet wurde. Durch eine Phasenanalyse haben wir den Zusammenhang zwischen dem Herzschlag und der Start- bzw. Stoppzeit der zu reproduzierenden Zeitintervalle untersucht. Es stellt sich heraus, dass Herzschläge bei Zeitintervallen über einige Sekunden als Taktgeber dienen können. KW - synchronization KW - phase oscillators KW - chimera state KW - time perception KW - Synchronisation KW - Phasen Oszillatoren KW - chimera Zustände KW - zeitverzögerte Selbstkopplung KW - Synchronisationsanalyse KW - Zeitwahrnehmung Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-73348 ER - TY - JOUR A1 - Di Florio, G. A1 - Bruendermann, E. A1 - Yadavalli, Nataraja Sekhar A1 - Santer, Svetlana A1 - Havenith, Martina T1 - Confocal raman microscopy and AFM study of the interface between the photosensitive polymer layer and multilayer graphene JF - Soft materials N2 - In this paper we report on the interaction between photosensitive azobenzene-containing polymer films and on top adsorbed graphene multilayers. The photosensitive polymer film changes its topography under irradiation with light interference patterns according to their polarization distribution. The multilayer graphene follows the deformation of the polymer film and stretches accordingly. Using confocal Raman microspectroscopy we can detect the appearance of additional peaks in the Raman spectrum of the photosensitive polymer film upon irradiation indicating a molecular interaction at the interface between the graphene multilayer and the polymer matrix. Multi-component analysis of the specific Raman bands shows that the interaction involves the graphene rings and the aromatic rings of the azobenzenes causing the strong adhesion between the two materials. KW - Graphene KW - Multilayer graphene KW - Photosensitive polymer film KW - Confocal Raman microscopy KW - AFM KW - Surface Relief Grating KW - Interfacial molecular interaction Y1 - 2014 U6 - https://doi.org/10.1080/1539445X.2014.945040 SN - 1539-445X SN - 1539-4468 VL - 12 SP - S98 EP - S105 PB - Taylor & Francis Group CY - Philadelphia ER - TY - JOUR A1 - Kang, Yu A1 - Barbirz, Stefanie A1 - Lipowsky, Reinhard A1 - Santer, Mark T1 - Conformational Diversity of O-Antigen Polysaccharides of the Gram-Negative Bacterium Shigella flexneri Serotype Y JF - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry Y1 - 2014 U6 - https://doi.org/10.1021/jp4111713 SN - 1520-6106 VL - 118 IS - 9 SP - 2523 EP - 2534 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Wendt, Martin T1 - Constraints on variations of m(p)/m(e) based on UVES observations of H-2 JF - Astronomische Nachrichten = Astronomical notes N2 - This article summarizes the latest results on the proton-to-electron mass ratio derived from H-2 observations at high redshift in the light of possible variations of fundamental physical constants. The focus lies on UVES observations of the past years as enormous progress was achieved since the first positive results on / were published. With the better understanding of systematics, dedicated observation runs, and numerous approaches to improve wavelength calibration accuracy, all current findings are in reasonable good agreement with no variation and provide an upper limit of / < 1 x 10(-5) for the redshift range of 2 < z < 3. (( KW - cosmology: observations KW - early Universe KW - quasars: absorption lines Y1 - 2014 U6 - https://doi.org/10.1002/asna.201312008 SN - 0004-6337 SN - 1521-3994 VL - 335 IS - 1 SP - 106 EP - 112 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Aliu, E. A1 - Aune, T. A1 - Barnacka, Anna A1 - Beilicke, M. A1 - Benbow, W. A1 - Berger, K. A1 - Biteau, Jonathan A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cardenzana, J. V. A1 - Cerruti, M. A1 - Chen, Xuhui A1 - Ciupik, L. A1 - Connaughton, V. A1 - Cui, W. A1 - Dickinson, H. J. A1 - Eisch, J. D. A1 - Errando, M. A1 - Falcone, A. A1 - Federici, Simone A1 - Feng, Q. A1 - Finley, J. P. A1 - Fleischhack, H. A1 - Fortin, P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gillanders, G. H. A1 - Griffin, S. A1 - Griffiths, S. T. A1 - Grube, J. A1 - Gyuk, G. A1 - Hakansson, Nils A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Humensky, T. B. A1 - Johnson, C. A. A1 - Kaaret, P. A1 - Kar, P. A1 - Kertzman, M. A1 - Khassen, Y. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Madhavan, A. S. A1 - Maier, G. A1 - McArthur, S. A1 - McCann, A. A1 - Meagher, K. A1 - Millis, J. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nieto, D. A1 - Ong, R. A. A1 - Otte, A. N. A1 - Park, N. A1 - Pohl, Martin A1 - Popkow, A. A1 - Prokoph, H. A1 - Pueschel, Elisa A1 - Quinn, J. A1 - Ragan, K. A1 - Rajotte, J. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Sembroski, G. H. A1 - Shahinyan, K. A1 - Smith, A. W. A1 - Staszak, D. A1 - Telezhinsky, Igor O. A1 - Tucci, J. V. A1 - Tyler, J. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Wakely, S. P. A1 - Weiner, O. M. A1 - Weinstein, A. A1 - Welsing, R. A1 - Wilhelm, Alina A1 - Williams, D. A. A1 - Zitzer, B. A1 - McEnery, J. E. A1 - Perkins, J. S. A1 - Veres, P. A1 - Zhu, S. T1 - Constraints on very high energy emission from GRB 130427A JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - Prompt emission from the very fluent and nearby (z = 0.34) gamma-ray burst GRB130427A was detected by several orbiting telescopes and by ground-based, wide-field-of-view optical transient monitors. Apart from the intensity and proximity of this GRB, it is exceptional due to the extremely long-lived high-energy (100 MeV to 100 GeV) gamma-ray emission, which was detected by the Large Area Telescope on the Fermi Gamma-Ray Space Telescope for similar to 70 ks after the initial burst. The persistent, hard-spectrum, high-energy emission suggests that the highest-energy gamma rays may have been produced via synchrotron self-Compton processes though there is also evidence that the high-energy emission may instead be an extension of the synchrotron spectrum. VERITAS, a ground-based imaging atmospheric Cherenkov telescope array, began follow-up observations of GRB130427A similar to 71 ks (similar to 20 hr) after the onset of the burst. The GRB was not detected with VERITAS; however, the high elevation of the observations, coupled with the low redshift of the GRB, make VERITAS a very sensitive probe of the emission from GRB130427A for E > 100 GeV. The non-detection and consequent upper limit derived place constraints on the synchrotron self-Compton model of high-energy gamma-ray emission from this burst. KW - gamma-ray burst: individual (GRB 130427A) Y1 - 2014 U6 - https://doi.org/10.1088/2041-8205/795/1/L3 SN - 2041-8205 SN - 2041-8213 VL - 795 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - THES A1 - Steinhaus, Sebastian Peter T1 - Constructing quantum spacetime T1 - Konstruktion der Quantenraumzeit BT - relation to classical gravity BT - Relation zur klassischen Gravitation N2 - Despite remarkable progress made in the past century, which has revolutionized our understanding of the universe, there are numerous open questions left in theoretical physics. Particularly important is the fact that the theories describing the fundamental interactions of nature are incompatible. Einstein's theory of general relative describes gravity as a dynamical spacetime, which is curved by matter and whose curvature determines the motion of matter. On the other hand we have quantum field theory, in form of the standard model of particle physics, where particles interact via the remaining interactions - electromagnetic, weak and strong interaction - on a flat, static spacetime without gravity. A theory of quantum gravity is hoped to cure this incompatibility by heuristically replacing classical spacetime by quantum spacetime'. Several approaches exist attempting to define such a theory with differing underlying premises and ideas, where it is not clear which is to be preferred. Yet a minimal requirement is the compatibility with the classical theory, they attempt to generalize. Interestingly many of these models rely on discrete structures in their definition or postulate discreteness of spacetime to be fundamental. Besides the direct advantages discretisations provide, e.g. permitting numerical simulations, they come with serious caveats requiring thorough investigation: In general discretisations break fundamental diffeomorphism symmetry of gravity and are generically not unique. Both complicates establishing the connection to the classical continuum theory. The main focus of this thesis lies in the investigation of this relation for spin foam models. This is done on different levels of the discretisation / triangulation, ranging from few simplices up to the continuum limit. In the regime of very few simplices we confirm and deepen the connection of spin foam models to discrete gravity. Moreover, we discuss dynamical, e.g. diffeomorphism invariance in the discrete, to fix the ambiguities of the models. In order to satisfy these conditions, the discrete models have to be improved in a renormalisation procedure, which also allows us to study their continuum dynamics. Applied to simplified spin foam models, we uncover a rich, non--trivial fixed point structure, which we summarize in a phase diagram. Inspired by these methods, we propose a method to consistently construct the continuum theory, which comes with a unique vacuum state. N2 - Trotz bemerkenswerter Fortschritte im vergangenen Jahrhundert, die unser Verständnis des Universums revolutioniert haben, gibt es noch zahlreiche ungeklärte Fragen in der theoretischen Physik. Besondere Bedeutung kommt der Tatsache zu, dass die Theorien, welche die fundamentalen Wechselwirkungen der Natur beschreiben, inkompatibel sind. Nach Einsteins allgemeiner Relativitätstheorie wird die Gravitation durch eine dynamische Raumzeit dargestellt, die von Materie gekrümmt wird und ihrerseits durch die Krümmung die Bewegung der Materie bestimmt. Dem gegenüber steht die Quantenfeldtheorie, die die verbliebenen Wechselwirkungen - elektromagnetische, schwache und starke Wechselwirkung - im Standardmodell der Teilchenphysik beschreibt, in dem Teilchen auf einer statischen Raumzeit -- ohne Gravitation -- miteinander interagieren. Die Hoffnung ist, dass eine Theorie der Quantengravitation diese Inkompatibilität beheben kann, indem, heuristisch, die klassische Raumzeit durch eine 'Quantenraumzeit' ersetzt wird. Es gibt zahlreiche Ansätze eine solche Theorie zu definieren, die auf unterschiedlichen Prämissen und Ideen beruhen, wobei a priori nicht klar ist, welche zu bevorzugen sind. Eine Minimalanforderung an diese Theorien ist Kompatibilität mit der klassischen Theorie, die sie verallgemeinern sollen. Interessanterweise basieren zahlreiche Modelle in ihrer Definition auf Diskretisierungen oder postulieren eine fundamentale Diskretheit der Raumzeit. Neben den unmittelbaren Vorteilen, die Diskretisierungen bieten, z.B. das Ermöglichen numerischer Simulationen, gibt es auch gravierende Nachteile, die einer ausführlichen Untersuchung bedürfen: Im Allgemeinen brechen Diskretisierungen die fundamentale Diffeomorphismensymmetrie der Gravitation und sind in der Regel nicht eindeutig definiert. Beides erschwert die Wiederherstellung der Verbindung zur klassischen, kontinuierlichen Theorie. Das Hauptaugenmerk dieser Doktorarbeit liegt darin diese Verbindung insbesondere für Spin-Schaum-Modelle (spin foam models) zu untersuchen. Dies geschieht auf sehr verschiedenen Ebenen der Diskretisierung / Triangulierung, angefangen bei wenigen Simplizes bis hin zum Kontinuumslimes. Im Regime weniger Simplizes wird die bekannte Verbindung von Spin--Schaum--Modellen zu diskreter Gravitation bestätigt und vertieft. Außerdem diskutieren wir dynamische Prinzipien, z.B. Diffeomorphismeninvarianz im Diskreten, um die Ambiguitäten der Modelle zu fixieren. Um diese Bedingungen zu erfüllen, müssen die diskreten Modelle durch Renormierungsverfahren verbessert werden, wodurch wir auch ihre Kontinuumsdynamik untersuchen können. Angewandt auf vereinfachte Spin-Schaum-Modelle finden wir eine reichhaltige, nicht-triviale Fixpunkt-Struktur, die wir in einem Phasendiagramm zusammenfassen. Inspiriert von diesen Methoden schlagen wir zu guter Letzt eine konsistente Konstruktionsmethode für die Kontinuumstheorie vor, die einen eindeutigen Vakuumszustand definiert. KW - Quantengravitation KW - Spin-Schaum-Modelle KW - Regge Kalkül KW - Renormierung KW - Verfeinerungslimes KW - quantum gravity KW - spin foams KW - regge calculus KW - renormalization and refinement limit Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus-72558 ER - TY - JOUR A1 - Beim Graben, Peter T1 - Contextual emergence of intentionality JF - Journal of consciousness studies : controversies in science & the humanities ; an international multi-disciplinary journal N2 - By means of an intriguing physical example, magnetic surface swimmers, that can be described in terms of Dennett's intentional stance, I reconstruct a hierarchy of necessary and sufficient conditions for the applicability of the intentional strategy. It turns out that the different levels of the intentional hierarchy are contextually emergent from their respective subjacent levels by imposing stability constraints upon them. At the lowest level of the hierarchy, phenomenal physical laws emerge for the coarse-grained description of open, nonlinear, and dissipative non-equilibrium systems in critical states. One level higher, dynamic patterns, such as, for example, magnetic surface swimmers, are contextually emergent as they are invariant under certain symmetry operations. Again one level up, these patterns behave apparently rationally by selecting optimal pathways for the dissipation of energy that is delivered by external gradients. This is in accordance with the restated Second Law of thermodynamics as a stability criterion. At the highest level, true believers are intentional systems that are stable under exchanging their observation conditions. Y1 - 2014 SN - 1355-8250 VL - 21 IS - 5-6 SP - 75 EP - 96 PB - Imprint Academic CY - Exeter ER - TY - JOUR A1 - van Driel-Gesztelyi, L. A1 - Baker, Daniel N. A1 - Toeroek, T. A1 - Pariat, E. A1 - Green, L. M. A1 - Williams, D. R. A1 - Carlyle, J. A1 - Valori, G. A1 - Demoulin, Pascal A1 - Kliem, Bernhard A1 - Long, D. M. A1 - Matthews, S. A. A1 - Malherbe, J. -M. T1 - Coronal magnetic reconnection driven by CME expansion-the 2011 June 7 event JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - Coronal mass ejections (CMEs) erupt and expand in a magnetically structured solar corona. Various indirect observational pieces of evidence have shown that the magnetic field of CMEs reconnects with surrounding magnetic fields, forming, e.g., dimming regions distant from the CME source regions. Analyzing Solar Dynamics Observatory (SDO) observations of the eruption from AR 11226 on 2011 June 7, we present the first direct evidence of coronal magnetic reconnection between the fields of two adjacent active regions during a CME. The observations are presented jointly with a data-constrained numerical simulation, demonstrating the formation/intensification of current sheets along a hyperbolic flux tube at the interface between the CME and the neighboring AR 11227. Reconnection resulted in the formation of new magnetic connections between the erupting magnetic structure from AR 11226 and the neighboring active region AR 11227 about 200 Mm from the eruption site. The onset of reconnection first becomes apparent in the SDO/AIA images when filament plasma, originally contained within the erupting flux rope, is redirected toward remote areas in AR 11227, tracing the change of large-scale magnetic connectivity. The location of the coronal reconnection region becomes bright and directly observable at SDO/AIA wavelengths, owing to the presence of down-flowing cool, dense (1010 cm(-3)) filament plasma in its vicinity. The high-density plasma around the reconnection region is heated to coronal temperatures, presumably by slow-mode shocks and Coulomb collisions. These results provide the first direct observational evidence that CMEs reconnect with surrounding magnetic structures, leading to a large-scale reconfiguration of the coronal magnetic field. KW - magnetic reconnection KW - magnetohydrodynamics (MHD) KW - Sun: corona KW - Sun: coronal mass ejections (CMEs) KW - Sun: magnetic fields KW - Sun: UV radiation Y1 - 2014 U6 - https://doi.org/10.1088/0004-637X/788/1/85 SN - 0004-637X SN - 1538-4357 VL - 788 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Schubert, Marcel A1 - Collins, Brian A. A1 - Mangold, Hannah A1 - Howard, Ian A. A1 - Schindler, Wolfram A1 - Vandewal, Koen A1 - Roland, Steffen A1 - Behrends, Jan A1 - Kraffert, Felix A1 - Steyrleuthner, Robert A1 - Chen, Zhihua A1 - Fostiropoulos, Konstantinos A1 - Bittl, Robert A1 - Salleo, Alberto A1 - Facchetti, Antonio A1 - Laquai, Frederic A1 - Ade, Harald W. A1 - Neher, Dieter T1 - Correlated donor/acceptor crystal orientation controls photocurrent generation in all-polymer solar cells JF - Advanced functional materials N2 - New polymers with high electron mobilities have spurred research in organic solar cells using polymeric rather than fullerene acceptors due to their potential of increased diversity, stability, and scalability. However, all-polymer solar cells have struggled to keep up with the steadily increasing power conversion efficiency of polymer: fullerene cells. The lack of knowledge about the dominant recombination process as well as the missing concluding picture on the role of the semi-crystalline microstructure of conjugated polymers in the free charge carrier generation process impede a systematic optimization of all-polymer solar cells. These issues are examined by combining structural and photo-physical characterization on a series of poly(3-hexylthiophene) (donor) and P(NDI2OD-T2) (acceptor) blend devices. These experiments reveal that geminate recombination is the major loss channel for photo-excited charge carriers. Advanced X-ray and electron-based studies reveal the effect of chloronaphthalene co-solvent in reducing domain size, altering domain purity, and reorienting the acceptor polymer crystals to be coincident with those of the donor. This reorientation correlates well with the increased photocurrent from these devices. Thus, effi cient split-up of geminate pairs at polymer/polymer interfaces may necessitate correlated donor/acceptor crystal orientation, which represents an additional requirement compared to the isotropic fullerene acceptors. Y1 - 2014 U6 - https://doi.org/10.1002/adfm.201304216 SN - 1616-301X SN - 1616-3028 VL - 24 IS - 26 SP - 4068 EP - 4081 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Sandev, Trifce A1 - Metzler, Ralf A1 - Tomovski, Zivorad T1 - Correlation functions for the fractional generalized Langevin equation in the presence of internal and external noise JF - Journal of mathematical physics N2 - We study generalized fractional Langevin equations in the presence of a harmonic potential. General expressions for the mean velocity and particle displacement, the mean squared displacement, position and velocity correlation functions, as well as normalized displacement correlation function are derived. We report exact results for the cases of internal and external friction, that is, when the driving noise is either internal and thus the fluctuation-dissipation relation is fulfilled or when the noise is external. The asymptotic behavior of the generalized stochastic oscillator is investigated, and the case of high viscous damping (overdamped limit) is considered. Additional behaviors of the normalized displacement correlation functions different from those for the regular damped harmonic oscillator are observed. In addition, the cases of a constant external force and the force free case are obtained. The validity of the generalized Einstein relation for this process is discussed. The considered fractional generalized Langevin equation may be used to model anomalous diffusive processes including single file-type diffusion. Y1 - 2014 U6 - https://doi.org/10.1063/1.4863478 SN - 0022-2488 SN - 1089-7658 VL - 55 IS - 2 PB - American Institute of Physics CY - Melville ER - TY - THES A1 - Balzer, Arnim T1 - Crab flare observations with H.E.S.S. phase II T1 - Crab Flare Observations with H.E.S.S. Phase II N2 - The H.E.S.S. array is a third generation Imaging Atmospheric Cherenkov Telescope (IACT) array. It is located in the Khomas Highland in Namibia, and measures very high energy (VHE) gamma-rays. In Phase I, the array started data taking in 2004 with its four identical 13 m telescopes. Since then, H.E.S.S. has emerged as the most successful IACT experiment to date. Among the almost 150 sources of VHE gamma-ray radiation found so far, even the oldest detection, the Crab Nebula, keeps surprising the scientific community with unexplained phenomena such as the recently discovered very energetic flares of high energy gamma-ray radiation. During its most recent flare, which was detected by the Fermi satellite in March 2013, the Crab Nebula was simultaneously observed with the H.E.S.S. array for six nights. The results of the observations will be discussed in detail during the course of this work. During the nights of the flare, the new 24 m × 32 m H.E.S.S. II telescope was still being commissioned, but participated in the data taking for one night. To be able to reconstruct and analyze the data of the H.E.S.S. Phase II array, the algorithms and software used by the H.E.S.S. Phase I array had to be adapted. The most prominent advanced shower reconstruction technique developed by de Naurois and Rolland, the template-based model analysis, compares real shower images taken by the Cherenkov telescope cameras with shower templates obtained using a semi-analytical model. To find the best fitting image, and, therefore, the relevant parameters that describe the air shower best, a pixel-wise log-likelihood fit is done. The adaptation of this advanced shower reconstruction technique to the heterogeneous H.E.S.S. Phase II array for stereo events (i.e. air showers seen by at least two telescopes of any kind), its performance using MonteCarlo simulations as well as its application to real data will be described. N2 - Das H.E.S.S. Experiment misst sehr hochenergetische Gammastrahlung im Khomas Hochland von Namibia. Es ist ein sogenanntes abbildendes atmosphärisches Cherenkov-Teleskopsystem welches in der 1. Phase, die im Jahr 2004 mit der Datennahme begann, aus vier identischen 13 m Spiegelteleskopen bestand. Seitdem hat sich H.E.S.S. als das erfolgreichstes Experiment in der bodengebundenen Gammastrahlungsastronomie etabliert. Selbst die älteste der mittlerweile fast 150 entdeckten Quellen von sehr hochenergetischer Gammastrahlung, der Krebsnebel, fasziniert immernoch Wissenschaftler mit neuen bisher unbekannten und unerwarteten Phänomenen. Ein Beispiel dafür sind die vor kurzem entdeckten sehr energiereichen Ausbrüche von hochenergetischer Gammastrahlung. Bei dem letzten deratigen Ausbruch des Krebsnebels im März 2013 hat das H.E.S.S. Experiment für sechs Nächte simultan mit dem Fermi-Satelliten, welcher den Ausbruch entdeckte, Daten genommen. Die Analyse der Daten, deren Ergebnis und deren Interpretation werden im Detail in dieser Arbeit vorgestellt. Während dieser Beobachtungen befand sich ein neues 24 m × 32 m großes Spiegelteleskop, das H.E.S.S. II- Teleskop, noch in seiner Inbetriebnahme, trotzdem hat es für eine dieser sechs Nächte an der Datennahme des gesamten Teleskopsystems teilgenommen. Um die Daten rekonstruieren und analysieren zu können, mussten die für die 1. Phase des Experiments entwickelten Algorithmen und die Software des H.E.S.S.- Experiments angepasst werden. Die fortschrittlichste Schauerrekonstruktionsmethode, welche von de Naurois und Rolland entwickelt wurde, basiert auf dem Vergleich von echten Schauerbildern, die mit Hilfe der Cherenkov-Kameras der einzelnen Teleskope aufgenommen wurden, mit Schauerschablonen die mit Hilfe eines semianalytischen Modells erzeugt wurden. Das am besten passende Bild und damit auch alle relevanten Schauerparameter, wird mit Hilfe einer pixelweisen Loglikelihood-Anpassung ermittelt. Die nötigen Änderungen um Multiteleskopereignisse, welche vom heterogenen H.E.S.S. Phase II Detektor gemessen wurden, mit Hilfe dieser fortschrittlichen Schauerrekonstruktionsmethode analysieren zu können, sowie die resultierenden Ergebnisse von MonteCarlo-Simulationen, als auch die Anwendung auf echte Daten, werden im Rahmen dieser Arbeit präsentiert. KW - Gammastrahlungsastronomie KW - Rekonstruktionsmethoden KW - Datenanalyse KW - Krebsnebel KW - gamma-ray astronomy KW - reconstruction methods KW - data analysis KW - Crab Nebula Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus-72545 ER - TY - JOUR A1 - de Carvalho, Sidney J. A1 - Metzler, Ralf A1 - Cherstvy, Andrey G. T1 - Critical adsorption of polyelectrolytes onto charged Janus nanospheres JF - Physical chemistry, chemical physics : a journal of European Chemical Societies N2 - Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two equally but oppositely charged hemispheres. The critical binding conditions for polyelectrolyte chains are analysed as function of the radius of the Janus particle and its surface charge density, as well as the salt concentration in the ambient solution. Specifically for the adsorption of finite-length polyelectrolyte chains onto Janus nanoparticles, we demonstrate that the critical adsorption conditions drastically differ when the size of the Janus particle or the screening length of the electrolyte are varied. We compare the scaling laws obtained for the adsorption-desorption threshold to the known results for uniformly charged spherical particles, observing significant disparities. We also contrast the changes to the polyelectrolyte chain conformations close to the surface of the Janus nanoparticles as compared to those for simple spherical particles. Finally, we discuss experimentally relevant physicochemical systems for which our simulations results may become important. In particular, we observe similar trends with polyelectrolyte complexation with oppositely but heterogeneously charged proteins. Y1 - 2014 U6 - https://doi.org/10.1039/c4cp02207f SN - 1463-9076 SN - 1463-9084 VL - 16 IS - 29 SP - 15539 EP - 15550 PB - Royal Society of Chemistry CY - Cambridge ER - TY - GEN A1 - de Carvalho, Sidney J. A1 - Metzler, Ralf A1 - Cherstvy, Andrey G. T1 - Critical adsorption of polyelectrolytes onto charged Janus nanospheres N2 - Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two equally but oppositely charged hemispheres. The critical binding conditions for polyelectrolyte chains are analysed as function of the radius of the Janus particle and its surface charge density, as well as the salt concentration in the ambient solution. Specifically for the adsorption of finite-length polyelectrolyte chains onto Janus nanoparticles, we demonstrate that the critical adsorption conditions drastically differ when the size of the Janus particle or the screening length of the electrolyte are varied. We compare the scaling laws obtained for the adsorption–desorption threshold to the known results for uniformly charged spherical particles, observing significant disparities. We also contrast the changes to the polyelectrolyte chain conformations close to the surface of the Janus nanoparticles as compared to those for simple spherical particles. Finally, we discuss experimentally relevant physico-chemical systems for which our simulations results may become important. In particular, we observe similar trends with polyelectrolyte complexation with oppositely but heterogeneously charged proteins. T3 - Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe - 278 Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-98783 ER - TY - JOUR A1 - Archambault, S. A1 - Aune, T. A1 - Behera, B. A1 - Beilicke, M. A1 - Benbow, W. A1 - Berger, K. A1 - Bird, R. A1 - Biteau, Jonathan A1 - Bugaev, V. A1 - Byrum, K. A1 - Cardenzana, J. V. A1 - Cerruti, M. A1 - Chen, Xuhui A1 - Ciupik, L. A1 - Connolly, M. P. A1 - Cui, Wei A1 - Dumm, J. A1 - Errando, M. A1 - Falcone, A. A1 - Federici, Simone A1 - Feng, Q. A1 - Finley, J. P. A1 - Fleischhack, H. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gillanders, G. H. A1 - Griffin, S. A1 - Griffiths, S. T. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Humensky, T. B. A1 - Johnson, C. A. A1 - Kaaret, P. A1 - Kertzman, M. A1 - Khassen, Y. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Kumar, S. A1 - Lang, M. J. A1 - Madhavan, A. S. A1 - Maier, G. A1 - McCann, A. A1 - Meagher, K. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nieto, Daniel A1 - Ong, R. A. A1 - Otte, A. N. A1 - Park, N. A1 - Pohl, Martin A1 - Popkow, A. A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Rajotte, J. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Sembroski, G. H. A1 - Shahinyan, K. A1 - Staszak, D. A1 - Telezhinsky, Igor O. A1 - Tucci, J. V. A1 - Tyler, J. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Wakely, S. P. A1 - Weinstein, A. A1 - Welsing, R. A1 - Wilhelm, Alina A1 - Williams, D. A. A1 - Ackermann, Margit A1 - Ajello, M. A1 - Albert, A. A1 - Baldini, L. A1 - Bastieri, D. A1 - Bellazzini, R. A1 - Bissaldi, E. A1 - Bregeon, Johan A1 - Buehler, R. A1 - Buson, S. A1 - Caliandro, G. A. A1 - Cameron, R. A. A1 - Caraveo, P. A. A1 - Cavazzuti, E. A1 - Charles, E. A1 - Chiang, J. A1 - Ciprini, S. A1 - Claus, R. A1 - Cutini, S. A1 - de Angelis, A. A1 - de Palma, F. A1 - Dermer, C. D. A1 - Digel, S. W. A1 - Di Venere, L. A1 - Drell, P. S. A1 - Favuzzi, C. A1 - Franckowiak, A. A1 - Fusco, P. A1 - Gargano, F. A1 - Gasparrini, D. A1 - Giglietto, N. A1 - Giordano, F. A1 - Giroletti, M. A1 - Grenier, I. A. A1 - Guiriec, S. A1 - Jogler, T. A1 - Kuss, M. A1 - Larsson, S. A1 - Latronico, L. A1 - Longo, F. A1 - Loparco, F. A1 - Lubrano, P. A1 - Madejski, G. M. A1 - Mayer, M. A1 - Mazziotta, Mario Nicola A1 - Michelson, P. F. A1 - Mizuno, T. A1 - Monzani, M. E. A1 - Morselli, Aldo A1 - Murgia, S. A1 - Nuss, E. A1 - Ohsugi, T. A1 - Ormes, J. F. A1 - Paneque, D. A1 - Perkins, J. S. A1 - Piron, F. A1 - Pivato, G. A1 - Raino, S. A1 - Razzano, M. A1 - Reimer, A. A1 - Reimer, Olaf A1 - Ritz, S. A1 - Schaal, M. A1 - Sgro, C. A1 - Siskind, E. J. A1 - Spinelli, P. A1 - Takahashi, H. A1 - Tibaldo, L. A1 - Tinivella, M. A1 - Troja, E. A1 - Vianello, G. A1 - Werner, M. A1 - Wood, M. T1 - Deep broadband observations of the distant gamma-ray blazar PKS 1424+240 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - We present deep VERITAS observations of the blazar PKS 1424+240, along with contemporaneous Fermi Large Area Telescope, Swift X-ray Telescope, and Swift UV Optical Telescope data between 2009 February 19 and 2013 June 8. This blazar resides at a redshift of z >= 0.6035, displaying a significantly attenuated gamma-ray flux above 100 GeV due to photon absorption via pair-production with the extragalactic background light. We present more than 100 hr of VERITAS observations over three years, a multiwavelength light curve, and the contemporaneous spectral energy distributions. The source shows a higher flux of (2.1 +/- 0.3) x 10(-7) photons m(-2) s(-1) above 120 GeV in 2009 and 2011 as compared to the flux measured in 2013, corresponding to (1.02 +/- 0.08) x 10-7 photons m(-2) s(-1) above 120 GeV. The measured differential very high energy (VHE; E >= 100 GeV) spectral indices are Gamma = 3.8 +/- 0.3, 4.3 +/- 0.6 and 4.5 +/- 0.2 in 2009, 2011, and 2013, respectively. No significant spectral change across the observation epochs is detected. We find no evidence for variability at gamma-ray opacities of greater than tau = 2, where it is postulated that any variability would be small and occur on timescales longer than a year if hadronic cosmic-ray interactions with extragalactic photon fields provide a secondary VHE photon flux. The data cannot rule out such variability due to low statistics. KW - BL Lacertae objects: individual (PKS 1424+240)-cosmic background radiation KW - gamma rays: galaxies Y1 - 2014 U6 - https://doi.org/10.1088/2041-8205/785/1/L16 SN - 2041-8205 SN - 2041-8213 VL - 785 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER -