TY  - JOUR
A1  - Sadovnichii, V. A.
A1  - Panasyuk, M. I.
A1  - Amelyushkin, A. M.
A1  - Bogomolov, V. V.
A1  - Benghin, V. V.
A1  - Garipov, G. K.
A1  - Kalegaev, V. V.
A1  - Klimov, P. A.
A1  - Khrenov, B. A.
A1  - Petrov, V. L.
A1  - Sharakin, S. A.
A1  - Shirokov, A. V.
A1  - Svertilov, S. I.
A1  - Zotov, M. Y.
A1  - Yashin, I. V.
A1  - Gorbovskoy, E. S.
A1  - Lipunov, V. M.
A1  - Park, I. H.
A1  - Lee, J.
A1  - Jeong, S.
A1  - Kim, M. B.
A1  - Jeong, H. M.
A1  - Shprits, Yuri Y.
A1  - Angelopoulos, V.
A1  - Russell, C. T.
A1  - Runov, A.
A1  - Turner, D.
A1  - Strangeway, R. J.
A1  - Caron, R.
A1  - Biktemerova, S.
A1  - Grinyuk, A.
A1  - Lavrova, M.
A1  - Tkachev, L.
A1  - Tkachenko, A.
A1  - Martinez, O.
A1  - Salazar, H.
A1  - Ponce, E.
T1  - "Lomonosov" Satellite-Space Observatory to Study Extreme Phenomena in Space
JF  - Space science reviews
N2  - The "Lomonosov" space project is lead by Lomonosov Moscow State University in collaboration with the following key partners: Joint Institute for Nuclear Research, Russia, University of California, Los Angeles (USA), University of Pueblo (Mexico), Sungkyunkwan University (Republic of Korea) and with Russian space industry organi-zations to study some of extreme phenomena in space related to astrophysics, astroparticle physics, space physics, and space biology. The primary goals of this experiment are to study: -Ultra-high energy cosmic rays (UHECR) in the energy range of the Greizen-ZatsepinKuzmin (GZK) cutoff; -Ultraviolet (UV) transient luminous events in the upper atmosphere; -Multi-wavelength study of gamma-ray bursts in visible, UV, gamma, and X-rays; -Energetic trapped and precipitated radiation (electrons and protons) at low-Earth orbit (LEO) in connection with global geomagnetic disturbances; -Multicomponent radiation doses along the orbit of spacecraft under different geomagnetic conditions and testing of space segments of optical observations of space-debris and other space objects; -Instrumental vestibular-sensor conflict of zero-gravity phenomena during space flight. This paper is directed towards the general description of both scientific goals of the project and scientific equipment on board the satellite. The following papers of this issue are devoted to detailed descriptions of scientific instruments.
KW  - Gamma-ray bursts
KW  - Ultra-high energy cosmic rays
KW  - Radiation belts
KW  - Space mission
Y1  - 2017
U6  - https://doi.org/10.1007/s11214-017-0425-x
SN  - 0038-6308
SN  - 1572-9672
VL  - 212
SP  - 1705
EP  - 1738
PB  - Springer
CY  - Dordrecht
ER  - 
TY  - JOUR
A1  - Chen, Zupeng
A1  - Savateev, Aleksandr
A1  - Pronkin, Sergey
A1  - Papaefthimiou, Vasiliki
A1  - Wolff, Christian Michael
A1  - Willinger, Marc Georg
A1  - Willinger, Elena
A1  - Neher, Dieter
A1  - Antonietti, Markus
A1  - Dontsova, Dariya
T1  - "The Easier the Better" Preparation of Efficient Photocatalysts-Metastable Poly(heptazine imide) Salts
JF  - Advanced materials
N2  - Cost-efficient, visible-light-driven hydrogen production from water is an attractive potential source of clean, sustainable fuel. Here, it is shown that thermal solid state reactions of traditional carbon nitride precursors (cyanamide, melamine) with NaCl, KCl, or CsCl are a cheap and straightforward way to prepare poly(heptazine imide) alkali metal salts, whose thermodynamic stability decreases upon the increase of the metal atom size. The chemical structure of the prepared salts is confirmed by the results of X-ray photoelectron and infrared spectroscopies, powder X-ray diffraction and electron microscopy studies, and, in the case of sodium poly(heptazine imide), additionally by atomic pair distribution function analysis and 2D powder X-ray diffraction pattern simulations. In contrast, reactions with LiCl yield thermodynamically stable poly(triazine imides). Owing to the metastability and high structural order, the obtained heptazine imide salts are found to be highly active photo-catalysts in Rhodamine B and 4-chlorophenol degradation, and Pt-assisted sacrificial water reduction reactions under visible light irradiation. The measured hydrogen evolution rates are up to four times higher than those provided by a benchmark photocatalyst, mesoporous graphitic carbon nitride. Moreover, the products are able to photocatalytically reduce water with considerable reaction rates, even when glycerol is used as a sacrificial hole scavenger.
KW  - carbon nitride
KW  - glycerol oxidation
KW  - mesocrystals
KW  - poly(heptazine imide)
KW  - water reduction reactions
Y1  - 2017
U6  - https://doi.org/10.1002/adma.201700555
SN  - 0935-9648
SN  - 1521-4095
VL  - 29
SP  - 21800
EP  - 21806
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - THES
A1  - Ehrig, Sebastian
T1  - 3D curvature and its role on tissue organization
N2  - Shape change is a fundamental process occurring in biological tissues during embryonic development and regeneration of tissues and organs. This process is regulated by cells that are constrained within a complex environment of biochemical and physical cues. The spatial constraint due to geometry has a determining role on tissue mechanics and the spatial distribution of force patterns that, in turn, influences the organization of the tissue structure. An understanding of the underlying principles of tissue organization may have wide consequences for the understanding of healing processes and the development of organs and, as such, is of fundamental interest for the tissue engineering community.
This thesis aims to further our understanding of how the collective behaviour of cells is influenced by the 3D geometry of the environment. Previous research studying the role of geometry on tissue growth has mainly focused either on flat surfaces or on substrates where at least one of the principal curvatures is zero. In the present work, tissue growth from MC3T3-E1 pre-osteoblasts was investigated on surfaces of controlled mean curvature. 
One key aspect of this thesis was the development of substrates of controlled mean curvature and their visualization in 3D. It was demonstrated that substrates of controlled mean curvature suitable for cell culture can be fabricated using liquid polymers and surface tension effects.
Using these substrates, it was shown that the mean surface curvature has a strong impact on the rate of tissue growth and on the organization of the tissue structure. It was thereby not only demonstrated that the amount of tissue produced (i.e. growth rates) by the cells depends on the mean curvature of the substrate but also that the tissue surface behaves like a viscous fluid with an equilibrium shape governed by the Laplace-Young-law. It was observed that more tissue was formed on highly concave surfaces compared to flat or convex surfaces.
Motivated by these observations, an analytical model was developed, where the rate of tissue growth is a function of the mean curvature, which could successfully describe the growth kinetics. This model was also able to reproduce the growth kinetics of previous experiments where tissues have been cultured in straight-sided prismatic pores.
A second part of this thesis focuses on the tissue structure, which influences the mechanical properties of the mature bone tissue. Since the extracellular matrix is produced by the cells, the cell orientation has a strong impact on the direction of the tissue fibres. In addition, it was recently shown that some cell types exhibit collective alignment similar to liquid crystals. 
Based on this observation, a computational model of self-propelled active particles was developed to explore in an abstract manner how the collective behaviour of cells is influenced by 3D curvature. It was demonstrated that the 3D curvature has a strong impact on the self-organization of active particles and gives, therefore, first insights into the principles of self-organization of cells on curved surfaces.
N2  - Formänderung ist ein fundamentaler Vorgang während der embryonalen Entwicklung und der Regeneration von Geweben und Organen. Dieser Prozess wird von Zellen reguliert die in einer komplexen Umgebung von biochemischen und physikalischen Signalen eingebettet sind. Die räumliche Begrenzung der Zellen führt dabei zu Unterschieden in der Gewebemechanik und der räumlichen Verteilung von Kräften und hat damit einen Einfluss auf die Organisation der Gewebestruktur. Ein Verständnis der Organisationsprozesse von Geweben hat weitreichende Konsequenzen im Hinblick auf das Verständnis von Heilungsprozessen und der Entwicklung von Organen bis hin zu medizinischen Anwendungen wie der Entwicklung von Implantaten.
Die vorliegende Arbeit zielt auf ein besseres Verständnis wie das kollektive Verhalten von Gewebezellen von der dreidimensionalen Krümmung der Umgebung beeinflusst wird. Die bisherige Forschung war bislang limitiert auf flache Oberflächen oder auf Substrate in denen zumindest eine der beiden Hauptkrümmungen Null ist. In dieser Arbeit wurde daher das Gewebewachstum von MC3T3-E1 Pre-Osteoblasten auf Oberflächen mit konstanter mittlerer Krümmung studiert.
Ein wichtiger Teil der Arbeit war die Entwicklung von Substraten mit kontrollierter mittlerer Krümmung und deren Visualisierung in 3D. Es wurde gezeigt, dass sich die Oberflächen- spannung von Polymerlösungen nutzen lässt um eben solche Substrate zu erzeugen. 
Mit Hilfe dieser Substrate wurde gezeigt, dass die mittlere Krümmung der Oberfläche einen entscheidenden Einfluss auf die Wachstumsrate und die Organisation der Gewebestruktur hat. Es konnte nicht nur gezeigt werden dass die Menge an gebildetem Gewebe von der mittleren Krümmung abhängig ist, sondern auch dass die Oberfläche des Gewebes sich dabei wie eine Flüssigkeit verhält und dem Laplace-Young Gesetz folgt. Es wurde beobachtet dass sich mehr Gewebe auf konkaven als auf flachen oder konvexen Oberflächen gebildet hat.
Basierend auf diesen Beobachtungen wurde ein analytisches Modell entwickelt, welches die Wachstumsrate als Funktion der mittleren Krümmung beschreibt und mit Hilfe dessen sich das Gewebewachstum erfolgreich beschreiben lässt. Dieses Modell kann auch die Ergebnisse früherer Arbeiten reproduzieren, in denen Gewebe in prismatischen Poren kultiviert wurden.
Ein weiterer Teil der Arbeit befasste sich mit der Struktur des Gewebes, welche einen Einfluss auf die späteren mechanischen Eigenschaften des maturierten Knochengewebes hat. Da die extrazelluläre Matrix des Gewebes von den Zellen gebildet wird, hat die Orientierung der Zellen einen entscheidenden Einfluss auf die Ausrichtung der Gewebefasern. Außerdem wurde vor kurzem gezeigt, dass sich manche Zellen wie Flüssigkristalle anordnen können. 
Basierend auf dieser Beobachtung wurde ein Computermodell aktiver Partikel entwickelt, mit dessen Hilfe sich der Einfluss des kollektiven Verhaltens der Zellen auf dreidimensional gekrümmten Oberflächen abstrahieren lässt. Es konnte dabei gezeigt werden, dass die dreidimensionale Krümmung einen entscheidenden Einfluss auf die Selbstorganisation dieser Partikel hat und gibt damit erste Einblicke in ein mögliches Organisationsverhalten von Zellen auf 3D Oberflächen.
KW  - biophysics
KW  - tissue engineering
KW  - mechanobiology
Y1  - 2017
ER  - 
TY  - JOUR
A1  - Seiler, Martin
A1  - Sremcevic, Miodrag
A1  - Seiss, Martin
A1  - Hoffmann, Holger
A1  - Spahn, Frank
T1  - A Librational Model for the Propeller Bleriot in the Saturnian Ring System
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters
KW  - planets and satellites: individual (Saturn)
KW  - planets and satellites: rings
Y1  - 2017
U6  - https://doi.org/10.3847/2041-8213/aa6d73
SN  - 2041-8205
SN  - 2041-8213
VL  - 840
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Abeysekara, A. U.
A1  - Archambault, S.
A1  - Archer, A.
A1  - Benbow, Wystan
A1  - Bird, Ralph
A1  - Buchovecky, M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cerruti, M.
A1  - Chen, X.
A1  - Ciupik, L.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Eisch, J. D.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Gillanders, G. H.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Hutten, M.
A1  - Hakansson, N.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Humensky, T. B.
A1  - Johnson, C. A.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krause, M.
A1  - Krennrich, F.
A1  - Kumar, S.
A1  - Lang, M. J.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Meagher, K.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nguyen, T.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Pelassa, V.
A1  - Pohl, Martin
A1  - Popkow, A.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Rulten, C.
A1  - Santander, M.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Wakely, S. P.
A1  - Weiner, O. M.
A1  - Weinstein, A.
A1  - Wilhelm, Alina
A1  - Williams, D. A.
A1  - Fegan, S.
A1  - Giebels, B.
A1  - Horan, D.
A1  - Berdyugin, A.
A1  - Kuan, J.
A1  - Lindfors, E.
A1  - Nilsson, K.
A1  - Oksanen, A.
A1  - Prokoph, H.
A1  - Reinthal, R.
A1  - Takalo, L.
A1  - Zefi, F.
T1  - A Luminous and Isolated Gamma-Ray Flare from the Blazar B2 1215+30
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - B2 1215+30 is a BL-Lac-type blazar that was first detected at TeV energies by the MAGIC atmospheric Cherenkov telescopes and subsequently confirmed by the Very Energetic Radiation Imaging Telescope Array System (VERITAS) observatory with data collected between 2009 and 2012. In 2014 February 08, VERITAS detected a large-amplitude flare from B2. 1215+30 during routine monitoring observations of the blazar 1ES. 1218+304, located in the same field of view. The TeV flux reached 2.4 times the Crab Nebula flux with a variability timescale of <3.6 hr. Multiwavelength observations with Fermi-LAT, Swift, and the Tuorla Observatory revealed a correlated high GeV flux state and no significant optical counterpart to the flare, with a spectral energy distribution where the gamma-ray luminosity exceeds the synchrotron luminosity. When interpreted in the framework of a onezone leptonic model, the observed emission implies a high degree of beaming, with Doppler factor delta > 10, and an electron population with spectral index p < 2.3.
KW  - BL Lacertae objects: individual (B2 1215+30, VER J1217+301)
KW  - galaxies: active
KW  - galaxies: jets
KW  - galaxies: nuclei
KW  - gamma rays: galaxies
Y1  - 2017
U6  - https://doi.org/10.3847/1538-4357/836/2/205
SN  - 0004-637X
SN  - 1538-4357
VL  - 836
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Vieyro, Florencia L.
A1  - Romero, Gustavo Esteban
A1  - Bosch-Ramon, Valentin
A1  - Marcote, Benito
A1  - del Valle, Maria Victoria
T1  - A model for the repeating FRB 121102 in the AGN scenario
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Fast radio bursts (FRBs) are transient sources of unknown origin. Recent radio and optical observations have provided strong evidence for an extragalactic origin of the phenomenon and the precise localization of the repeating FRB 121102. Observations using the Karl G. Jansky Very Large Array (VLA) and very-long-baseline interferometry (VLBI) have revealed the existence of a continuum non-thermal radio source consistent with the location of the bursts in a dwarf galaxy. All these new data rule out several models that were previously proposed, and impose stringent constraints to new models. Aims. We aim to model FRB 121102 in light of the new observational results in the active galactic nucleus (AGN) scenario. Methods. We propose a model for repeating FRBs in which a non-steady relativistic e(+)-beam, accelerated by an impulsive magneto-hydrodynamic driven mechanism, interacts with a cloud at the centre of a star-forming dwarf galaxy. The interaction generates regions of high electrostatic field called cavitons in the plasma cloud. Turbulence is also produced in the beam. These processes, plus particle isotropization, the interaction scale, and light retardation effects, provide the necessary ingredients for short-lived, bright coherent radiation bursts. Results. The mechanism studied in this work explains the general properties of FRB 121102, and may also be applied to other repetitive FRBs. Conclusions. Coherent emission from electrons and positrons accelerated in cavitons provides a plausible explanation of FRBs.
KW  - radio continuum: general
KW  - galaxies: dwarf
KW  - galaxies: jets
KW  - radiation mechanisms: non-thermal
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201730556
SN  - 1432-0746
VL  - 602
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Hintsche, Marius
A1  - Waljor, Veronika
A1  - Grossmann, Robert
A1  - Kühn, Marco J.
A1  - Thormann, Kai M.
A1  - Peruani, Fernando
A1  - Beta, Carsten
T1  - A polar bundle of flagella can drive bacterial swimming by pushing, pulling, or coiling around the cell body
JF  - Scientific reports
N2  - Bacteria swim in sequences of straight runs that are interrupted by turning events. They drive their swimming locomotion with the help of rotating helical flagella. Depending on the number of flagella and their arrangement across the cell body, different run-and-turn patterns can be observed. Here, we present fluorescence microscopy recordings showing that cells of the soil bacterium Pseudomonas putida that are decorated with a polar tuft of helical flagella, can alternate between two distinct swimming patterns. On the one hand, they can undergo a classical push-pull-push cycle that is well known from monopolarly flagellated bacteria but has not been reported for species with a polar bundle of multiple flagella. Alternatively, upon leaving the pulling mode, they can enter a third slow swimming phase, where they propel themselves with their helical bundle wrapped around the cell body. A theoretical estimate based on a random-walk model shows that the spreading of a population of swimmers is strongly enhanced when cycling through a sequence of pushing, pulling, and wrapped flagellar configurations as compared to the simple push-pull-push pattern.
Y1  - 2017
U6  - https://doi.org/10.1038/s41598-017-16428-9
SN  - 2045-2322
VL  - 7
PB  - Macmillan Publishers Limited, part of Springer Nature
CY  - London
ER  - 
TY  - JOUR
A1  - Postnov, K.
A1  - Oskinova, Lida
A1  - Torrejon, J. M.
T1  - A propelling neutron star in the enigmatic Be-star gamma Cassiopeia
JF  - Monthly notices of the Royal Astronomical Society
N2  - gamma Cassiopeia (gamma Cas), is known to be a binary system consisting of a Be-type star and a low-mass (M similar to 1M(circle dot)) companion of unknown nature orbiting in the Be-disc plane. Here, we apply the quasi-spherical accretion theory on to a compact magnetized star and show that if the low-mass companion of gamma Cas is a fast spinning neutron star, the key observational signatures of. Cas are remarkably well reproduced. Direct accretion on to this fast rotating neutron star is impeded by the propeller mechanism. In this case, around the neutron star magnetosphere a hot shell is formed which emits thermal X-rays in qualitative and quantitative agreement with observed properties of the X-ray emission from gamma Cas. We suggest that gamma Cas and its analogues constitute a new subclass of Be-type X-ray binaries hosting rapidly rotating neutron stars formed in supernova explosions with small kicks. The subsequent evolutionary stage of gamma Cas and its analogues should be the X Per-type binaries comprising low-luminosity slowly rotating X-ray pulsars. The model explains the enigmatic X-ray emission from gamma Cas, and also establishes evolutionary connections between various types of rotating magnetized neutron stars in Be-binaries.
KW  - stars: emission-line, Be
KW  - stars: neutron
Y1  - 2017
U6  - https://doi.org/10.1093/mnrasl/slw223
SN  - 0035-8711
SN  - 1365-2966
VL  - 465
IS  - 1
SP  - L119
EP  - L123
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Jaervinen, S. P.
A1  - Hubrig, Swetlana
A1  - Ilyin, Ilya
A1  - Shenar, Tomer
A1  - Schoeller, M.
T1  - A search for spectral variability in the highly magnetized O9.7 V star HD 54879
JF  - Astronomische Nachrichten = Astronomical notes
N2  - The O9.7 V star HD 54879 possesses the second strongest magnetic field among the single, magnetic, O-type stars. In contrast to other magnetic O-type stars, the chemical abundance analysis of HD 54879 indicated a rather normal optical spectrum without obvious element enhancements or depletions. Furthermore, spectral variability was detected only in lines partly formed in the magnetosphere. As this star shows such a deviate, almost nonvariable, spectral behavior, we performed a deeper analysis of its spectral variability on different timescales using all currently available HARPSpol and FORS 2 spectropolarimetric observations. The longitudinal magnetic field strengths measured at different epochs indicate the presence of variability possibly related to stellar rotation, but the current data do not allow us yet to identify the periodicity of the field variation. As spectropolarimetric observations obtained at different epochs consist of subexposures with different integration times, we investigated spectral variability on timescales of minutes. The detected level of variability in line profiles of different elements is rather low, between 0.2 and 1.7%, depending on the integration time of the exposures and the considered element.
KW  - stars: magnetic fields
KW  - stars: oscillations
KW  - techniques: polarimetric
KW  - stars: individual (HD 54879)
Y1  - 2017
U6  - https://doi.org/10.1002/asna.201713402
SN  - 0004-6337
SN  - 1521-3994
VL  - 338
SP  - 952
EP  - 958
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Herrmann, Carl J. J.
A1  - Metzler, Ralf
A1  - Engbert, Ralf
T1  - A self-avoiding walk with neural delays as a model of fixational eye movements
JF  - Scientific reports
N2  - Fixational eye movements show scaling behaviour of the positional mean-squared displacement with a characteristic transition from persistence to antipersistence for increasing time-lag. These statistical patterns were found to be mainly shaped by microsaccades (fast, small-amplitude movements). However, our re-analysis of fixational eye-movement data provides evidence that the slow component (physiological drift) of the eyes exhibits scaling behaviour of the mean-squared displacement that varies across human participants. These results suggest that drift is a correlated movement that interacts with microsaccades. Moreover, on the long time scale, the mean-squared displacement of the drift shows oscillations, which is also present in the displacement auto-correlation function. This finding lends support to the presence of time-delayed feedback in the control of drift movements. Based on an earlier non-linear delayed feedback model of fixational eye movements, we propose and discuss different versions of a new model that combines a self-avoiding walk with time delay. As a result, we identify a model that reproduces oscillatory correlation functions, the transition from persistence to antipersistence, and microsaccades.
Y1  - 2017
U6  - https://doi.org/10.1038/s41598-017-13489-8
SN  - 2045-2322
VL  - 7
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Herrmann, Carl J. J.
A1  - Metzler, Ralf
T1  - A self-avoiding walk with neural delays as a model of fixational eye movements
JF  - Scientific reports
N2  - Fixational eye movements show scaling behaviour of the positional mean-squared displacement with a characteristic transition from persistence to antipersistence for increasing time-lag. These statistical patterns were found to be mainly shaped by microsaccades (fast, small-amplitude movements). However, our re-analysis of fixational eye-movement data provides evidence that the slow component (physiological drift) of the eyes exhibits scaling behaviour of the mean-squared displacement that varies across human participants. These results suggest that drift is a correlated movement that interacts with microsaccades. Moreover, on the long time scale, the mean-squared displacement of the drift shows oscillations, which is also present in the displacement auto-correlation function. This finding lends support to the presence of time-delayed feedback in the control of drift movements. Based on an earlier non-linear delayed feedback model of fixational eye movements, we propose and discuss different versions of a new model that combines a self-avoiding walk with time delay. As a result, we identify a model that reproduces oscillatory correlation functions, the transition from persistence to antipersistence, and microsaccades.
Y1  - 2017
U6  - https://doi.org/10.1038/s41598-017-13489-8
SN  - 2045-2322
VL  - 7
SP  - 1
EP  - 17
PB  - Springer Nature
CY  - London
ER  - 
TY  - JOUR
A1  - Kamann, Sebastian
A1  - Husser, T. -O.
A1  - Dreizler, S.
A1  - Emsellem, E.
A1  - Weilbacher, Peter Michael
A1  - Martens, S.
A1  - Bacon, R.
A1  - den Brok, M.
A1  - Giesers, B.
A1  - Krajnovic, Davor
A1  - Roth, Martin M.
A1  - Wendt, Martin
A1  - Wisotzki, Lutz
T1  - A stellar census in globular clusters with MUSE
BT  - the contribution of rotation to cluster dynamics studied with 200 000 stars
JF  - Monthly notices of the Royal Astronomical Society
N2  - This is the first of a series of papers presenting the results from our survey of 25 Galactic globular clusters with the MUSE integral-field spectrograph. In combination with our dedicated algorithm for source deblending, MUSE provides unique multiplex capabilities in crowded stellar fields and allows us to acquire samples of up to 20 000 stars within the half-light radius of each cluster. The present paper focuses on the analysis of the internal dynamics of 22 out of the 25 clusters, using about 500 000 spectra of 200 000 individual stars. Thanks to the large stellar samples per cluster, we are able to perform a detailed analysis of the central rotation and dispersion fields using both radial profiles and two-dimensional maps. The velocity dispersion profiles we derive show a good general agreement with existing radial velocity studies but typically reach closer to the cluster centres. By comparison with proper motion data, we derive or update the dynamical distance estimates to 14 clusters. Compared to previous dynamical distance estimates for 47 Tuc, our value is in much better agreement with other methods. We further find significant (>3 sigma) rotation in the majority (13/22) of our clusters. Our analysis seems to confirm earlier findings of a link between rotation and the ellipticities of globular clusters. In addition, we find a correlation between the strengths of internal rotation and the relaxation times of the clusters, suggesting that the central rotation fields are relics of the cluster formation that are gradually dissipated via two-body relaxation.
KW  - techniques: imaging spectroscopy
KW  - stars: kinematics and dynamics
KW  - globular clusters: general
Y1  - 2017
U6  - https://doi.org/10.1093/mnras/stx2719
SN  - 0035-8711
SN  - 1365-2966
VL  - 473
IS  - 4
SP  - 5591
EP  - 5616
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Vaz da Cruz, Vinicius
A1  - Ertan, Emelie
A1  - Couto, Rafael C.
A1  - Eckert, Sebastian
A1  - Fondell, Mattis
A1  - Dantz, Marcus
A1  - Kennedy, Brian
A1  - Schmitt, Thorsten
A1  - Pietzsch, Annette
A1  - Guimaraes, Freddy F.
A1  - Ågren, Hans
A1  - Odelius, Michael
A1  - Föhlisch, Alexander
A1  - Kimberg, Victor
T1  - A study of the water molecule using frequency control over nuclear dynamics in resonant X-ray scattering
JF  - Physical chemistry, chemical physics : a journal of European Chemical Societies
N2  - In this combined theoretical and experimental study we report a full analysis of the resonant inelastic X-ray scattering (RIXS) spectra of H2O, D2O and HDO. We demonstrate that electronically-elastic RIXS has an inherent capability to map the potential energy surface and to perform vibrational analysis of the electronic ground state in multimode systems. We show that the control and selection of vibrational excitation can be performed by tuning the X-ray frequency across core-excited molecular bands and that this is clearly reflected in the RIXS spectra. Using high level ab initio electronic structure and quantum nuclear wave packet calculations together with high resolution RIXS measurements, we discuss in detail the mode coupling, mode localization and anharmonicity in the studied systems.
Y1  - 2017
U6  - https://doi.org/10.1039/c7cp01215b
SN  - 1463-9076
SN  - 1463-9084
VL  - 19
SP  - 19573
EP  - 19589
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Vandewal, Koen
A1  - Benduhn, Johannes
A1  - Schellhammer, Karl Sebastian
A1  - Vangerven, Tim
A1  - Rückert, Janna E.
A1  - Piersimoni, Fortunato
A1  - Scholz, Reinhard
A1  - Zeika, Olaf
A1  - Fan, Yeli
A1  - Barlow, Stephen
A1  - Neher, Dieter
A1  - Marder, Seth R.
A1  - Manca, Jean
A1  - Spoltore, Donato
A1  - Cuniberti, Gianaurelio
A1  - Ortmann, Frank
T1  - Absorption Tails of Donor
BT  - C-60 Blends Provide Insight into Thermally Activated Charge-Transfer Processes and Polaron Relaxation
JF  - Journal of the American Chemical Society
N2  - In disordered organic semiconductors, the transfer of a rather localized charge carrier from one site to another triggers a deformation of the molecular structure quantified by the intramolecular relaxation energy. A similar structural relaxation occurs upon population of intermolecular charge-transfer (CT) states formed at organic electron donor (D)-acceptor (A) interfaces. Weak CT absorption bands for D A complexes occur at photon energies below the optical gaps of both the donors and the C-60 acceptor as a result of optical transitions from the neutral ground state to the ionic CT state. In this work, we show that temperature-activated intramolecular vibrations of the ground state play a major role in determining the line shape of such CT absorption bands. This allows us to extract values for the relaxation energy related to the geometry change from neutral to ionic CT complexes. Experimental values for the relaxation energies of 20 D:C-60 CT complexes correlate with values calculated within density functional theory. These results provide an experimental method for determining the polaron relaxation energy in solid-state organic D-A blends and show the importance of a reduced relaxation energy, which we introduce to characterize thermally activated CT processes.
Y1  - 2017
U6  - https://doi.org/10.1021/jacs.6b12857
SN  - 0002-7863
VL  - 139
IS  - 4
SP  - 1699
EP  - 1704
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Kar, Prathitha
A1  - Cherstvy, Andrey G.
A1  - Metzler, Ralf
T1  - Acceleration of bursty multiprotein target search kinetics on DNA by colocalisation
JF  - Physical chemistry, chemical physics : a journal of European Chemical Societies
N2  - Proteins are capable of locating specific targets on DNA by employing a facilitated diffusion process with intermittent 1D and 3D search steps. Gene colocalisation and coregulation-i.e. the spatial proximity of two communicating genes-is one factor capable of accelerating the target search process along the DNA. We perform Monte Carlo computer simulations and demonstrate the benefits of gene colocalisation for minimising the search time in a model DNA-protein system. We use a simple diffusion model to mimic the search for targets by proteins, produced initially in bursts of multiple proteins and performing the first-passage search on the DNA chain. The behaviour of the mean first-passage times to the target is studied as a function of distance between the initial position of proteins and the DNA target position, as well as versus the concentration of proteins. We also examine the properties of bursty target search kinetics for varying physical-chemical protein-DNA binding affinity. Our findings underline the relevance of colocalisation of production and binding sites for protein search inside biological cells.
Y1  - 2017
U6  - https://doi.org/10.1039/c7cp06922g
SN  - 1463-9076
SN  - 1463-9084
VL  - 20
IS  - 12
SP  - 7931
EP  - 7946
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Anielski, Alexander
A1  - Barbosa Pfannes, Eva Katharina
A1  - Beta, Carsten
T1  - Adaptive microfluidic gradient generator for quantitative chemotaxis experiments
JF  - Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques
N2  - Chemotactic motion in a chemical gradient is an essential cellular function that controls many processes in the living world. For a better understanding and more detailed modelling of the underlying mechanisms of chemotaxis, quantitative investigations in controlled environments are needed. We developed a setup that allows us to separately address the dependencies of the chemotactic motion on the average background concentration and on the gradient steepness of the chemoattractant. In particular, both the background concentration and the gradient steepness can be kept constant at the position of the cell while it moves along in the gradient direction. This is achieved by generating a well-defined chemoattractant gradient using flow photolysis. In this approach, the chemoattractant is released by a light-induced reaction from a caged precursor in a microfluidic flow chamber upstream of the cell. The flow photolysis approach is combined with an automated real-time cell tracker that determines changes in the cell position and triggers movement of the microscope stage such that the cell motion is compensated and the cell remains at the same position in the gradient profile. The gradient profile can be either determined experimentally using a caged fluorescent dye or may be alternatively determined by numerical solutions of the corresponding physical model. To demonstrate the function of this adaptive microfluidic gradient generator, we compare the chemotactic motion of Dictyostelium discoideum cells in a static gradient and in a gradient that adapts to the position of the moving cell. Published by AIP Publishing.
Y1  - 2017
U6  - https://doi.org/10.1063/1.4978535
SN  - 0034-6748
SN  - 1089-7623
VL  - 88
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Chechkin, Aleksei V.
A1  - Kantz, Holger
A1  - Metzler, Ralf
T1  - Ageing effects in ultraslow continuous time random walks
JF  - The European physical journal : B, Condensed matter and complex systems
N2  - In ageing systems physical observables explicitly depend on the time span elapsing between the original initiation of the system and the actual start of the recording of the particle motion. We here study the signatures of ageing in the framework of ultraslow continuous time random walk processes with super-heavy tailed waiting time densities. We derive the density for the forward or recurrent waiting time of the motion as function of the ageing time, generalise the Montroll-Weiss equation for this process, and analyse the ageing behaviour of the ensemble and time averaged mean squared displacements.
Y1  - 2017
U6  - https://doi.org/10.1140/epjb/e2017-80270-9
SN  - 1434-6028
SN  - 1434-6036
VL  - 90
PB  - Springer
CY  - New York
ER  - 
TY  - JOUR
A1  - Safdari, Hadiseh
A1  - Cherstvy, Andrey G.
A1  - Chechkin, Aleksei V.
A1  - Bodrova, Anna
A1  - Metzler, Ralf
T1  - Aging underdamped scaled Brownian motion
BT  - Ensemble- and time-averaged particle displacements, nonergodicity, and the failure of the overdamping approximation
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - We investigate both analytically and by computer simulations the ensemble- and time-averaged, nonergodic, and aging properties of massive particles diffusing in a medium with a time dependent diffusivity. We call this stochastic diffusion process the (aging) underdamped scaled Brownian motion (UDSBM). We demonstrate how the mean squared displacement (MSD) and the time-averaged MSD of UDSBM are affected by the inertial term in the Langevin equation, both at short, intermediate, and even long diffusion times. In particular, we quantify the ballistic regime for the MSD and the time-averaged MSD as well as the spread of individual time-averaged MSD trajectories. One of the main effects we observe is that, both for the MSD and the time-averaged MSD, for superdiffusive UDSBM the ballistic regime is much shorter than for ordinary Brownian motion. In contrast, for subdiffusive UDSBM, the ballistic region extends to much longer diffusion times. Therefore, particular care needs to be taken under what conditions the overdamped limit indeed provides a correct description, even in the long time limit. We also analyze to what extent ergodicity in the Boltzmann-Khinchin sense in this nonstationary system is broken, both for subdiffusive and superdiffusive UDSBM. Finally, the limiting case of ultraslow UDSBM is considered, with a mixed logarithmic and power-law dependence of the ensemble-and time-averaged MSDs of the particles. In the limit of strong aging, remarkably, the ordinary UDSBM and the ultraslow UDSBM behave similarly in the short time ballistic limit. The approaches developed here open ways for considering other stochastic processes under physically important conditions when a finite particle mass and aging in the system cannot be neglected.
Y1  - 2017
U6  - https://doi.org/10.1103/PhysRevE.95.012120
SN  - 2470-0045
SN  - 2470-0053
VL  - 95
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Mishurova, Tatiana
A1  - Cabeza, Sandra
A1  - Artzt, Katia
A1  - Haubrich, Jan
A1  - Klaus, Manuela
A1  - Genzel, Christoph
A1  - Requena, Guillermo
A1  - Bruno, Giovanni
T1  - An Assessment of Subsurface Residual Stress Analysis in SLM Ti-6Al-4V
JF  - Materials
N2  - Ti-6Al-4V bridges were additively fabricated by selective laser melting (SLM) under different scanning speed conditions, to compare the effect of process energy density on the residual stress state. Subsurface lattice strain characterization was conducted by means of synchrotron diffraction in energy dispersive mode. High tensile strain gradients were found at the frontal surface for samples in an as-built condition. The geometry of the samples promotes increasing strains towards the pillar of the bridges. We observed that the higher the laser energy density during fabrication, the lower the lattice strains. A relief of lattice strains takes place after heat treatment.
KW  - selective laser melting
KW  - additive manufacturing
KW  - heat treatment
KW  - Ti-6Al-4V
KW  - synchrotron X-ray diffraction
KW  - residual stress
Y1  - 2017
U6  - https://doi.org/10.3390/ma10040348
SN  - 1996-1944
VL  - 10
PB  - MDPI
CY  - Basel
ER  - 
TY  - JOUR
A1  - Richter, Philipp
A1  - Nuza, S. E.
A1  - Fox, Andrew J.
A1  - Wakker, Bart P.
A1  - Lehner, N.
A1  - Ben Bekhti, Nadya
A1  - Fechner, Cora
A1  - Wendt, Martin
A1  - Howk, J. Christopher
A1  - Muzahid, S.
A1  - Ganguly, R.
A1  - Charlton, Jane C.
T1  - An HST/COS legacy survey of high-velocity ultraviolet absorption in the
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Context. The Milky Way is surrounded by large amounts of diffuse gaseous matter that connects the stellar body of our Galaxy with its large-scale Local Group (LG) environment. Aims. To characterize the absorption properties of this circumgalactic medium (CGM) and its relation to the LG we present the so-far largest survey of metal absorption in Galactic high-velocity clouds (HVCs) using archival ultraviolet (UV) spectra of extragalactic background sources. The UV data are obtained with the Cosmic Origins Spectrograph (COS) onboard the Hubble Space Telescope (HST) and are supplemented by 21 cm radio observations of neutral hydrogen. Methods. Along 270 sightlines we measure metal absorption in the lines of Si II, Si III, C II, and C IV and associated H I 21 cm emission in HVCs in the velocity range vertical bar v(LSR)vertical bar = 100-500 km s(-1). With this unprecedented large HVC sample we were able to improve the statistics on HVC covering fractions, ionization conditions, small-scale structure, CGM mass, and inflow rate. For the first time, we determine robustly the angular two point correlation function of the high-velocity absorbers, systematically analyze antipodal sightlines on the celestial sphere, and compare the HVC absorption characteristics with that of damped Lyman alpha absorbers (DLAs) and constrained cosmological simulations of the LG (CLUES project).
KW  - Galaxy: halo
KW  - Galaxy: structure
KW  - Galaxy: evolution
KW  - ISM: kinematics and dynamics
KW  - techniques: spectroscopic
KW  - ultraviolet: ISM
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201630081
SN  - 1432-0746
VL  - 607
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Ignace, R.
A1  - Hole, K. T.
A1  - Oskinova, Lida
A1  - Rotter, J. P.
T1  - An X-Ray Study of Two B plus B Binaries: AH Cep and CW Cep
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - AH Cep and CW Cep are both early B-type binaries with short orbital periods of 1.8. days and 2.7. days, respectively. All four components are B0.5V types. The binaries are also double-lined spectroscopic and eclipsing. Consequently, solutions for orbital and stellar parameters make the pair of binaries ideal targets for a study of the colliding winds between two B. stars. Chandra ACIS-I observations were obtained to determine X-ray luminosities. AH. Cep was detected with an unabsorbed X-ray luminosity at a 90% confidence interval of (9-33) x 10(30) erg s(-1), or (0.5-1.7) x 10(-7) L-Bol , relative to the combined Bolometric luminosities of the two components. While formally consistent with expectations for embedded wind shocks, or binary wind collision, the near-twin system of CW Cep was a surprising nondetection. For CW Cep, an upper limit was determined with L-X/L-Bol < 10(-8), again for the combined components. One difference between these two systems is that AH Cep is part of a multiple system. The X-rays from AH. Cep may not arise from standard wind shocks nor wind collision, but perhaps instead from magnetism in any one of the four components of the system. The possibility could be tested by searching for cyclic X-ray variability in AH. Cep on the short orbital period of the inner B. stars.
KW  - stars: early-type
KW  - stars: individual (AH Cep, CW Cep)
KW  - stars: massive
KW  - stars: winds
KW  - outflows X-rays: binaries
Y1  - 2017
U6  - https://doi.org/10.3847/1538-4357/aa93ea
SN  - 0004-637X
SN  - 1538-4357
VL  - 850
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Stange, Maike
A1  - Hintsche, Marius
A1  - Sachse, Kirsten
A1  - Gerhardt, Matthias
A1  - Valleriani, Angelo
A1  - Beta, Carsten
T1  - Analyzing the spatial positioning of nuclei in polynuclear giant cells
JF  - Journal of Physics D: Applied Physics
N2  - How cells establish and maintain a well-defined size is a fundamental question of cell biology. Here we investigated to what extent the microtubule cytoskeleton can set a predefined cell size, independent of an enclosing cell membrane. We used electropulse-induced cell fusion to form giant multinuclear cells of the social amoeba Dictyostelium discoideum. Based on dual-color confocal imaging of cells that expressed fluorescent markers for the cell nucleus and the microtubules, we determined the subcellular distributions of nuclei and centrosomes in the giant cells. Our two- and three-dimensional imaging results showed that the positions of nuclei in giant cells do not fall onto a regular lattice. However, a comparison with model predictions for random positioning showed that the subcellular arrangement of nuclei maintains a low but still detectable degree of ordering. This can be explained by the steric requirements of the microtubule cytoskeleton, as confirmed by the effect of a microtubule degrading drug.
KW  - Dictyostelium
KW  - cell nucleus
KW  - positioning
KW  - imaging
KW  - spatial poisson distribution
Y1  - 2017
U6  - https://doi.org/10.1088/1361-6463/aa8da0
SN  - 0022-3727
SN  - 1361-6463
VL  - 50
IS  - 46
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - THES
A1  - Buschhüter, David
T1  - Anforderungsrelevante mathematik- und physikbezogene Leistungsdispositionen von Physikanfängerinnen und  - anfängern
BT  - Zeitlicher Wandel mathematischer und physikalischer Kentnisse und Fähigkeiten (1978/2013) und inkrementelle Validität von Physikbezogenen Leistungsdispositionen für Studienleistungen und Studienabbruch
Y1  - 2017
ER  - 
TY  - GEN
A1  - Metzler, Ralf
T1  - Anomalous Diffusion in Membranes and the Cytoplasm of Biological Cells
T2  - Biophysical journal
Y1  - 2017
U6  - https://doi.org/10.1016/j.bpj.2016.11.2577
SN  - 0006-3495
SN  - 1542-0086
VL  - 112
IS  - 3
SP  - 476A
EP  - 476A
PB  - Cell Press
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Stolterfoht, Martin
A1  - Wolff, Christian Michael
A1  - Amir, Yohai
A1  - Paulke, Andreas
A1  - Perdigon-Toro, Lorena
A1  - Caprioglio, Pietro
A1  - Neher, Dieter
T1  - Approaching the fill factor Shockley-Queisser limit in stable, dopant-free triple cation perovskite solar cells
JF  - Energy & Environmental Science
N2  - Perovskite solar cells now compete with their inorganic counterparts in terms of power conversion efficiency, not least because of their small open-circuit voltage (V-OC) losses. A key to surpass traditional thin-film solar cells is the fill factor (FF). Therefore, more insights into the physical mechanisms that define the bias dependence of the photocurrent are urgently required. In this work, we studied charge extraction and recombination in efficient triple cation perovskite solar cells with undoped organic electron/hole transport layers (ETL/HTL). Using integral time of flight we identify the transit time through the HTL as the key figure of merit for maximizing the fill factor (FF) and efficiency. Complementarily, intensity dependent photocurrent and V-OC measurements elucidate the role of the HTL on the bias dependence of non-radiative and transport-related loss channels. We show that charge transport losses can be completely avoided under certain conditions, yielding devices with FFs of up to 84%. Optimized cells exhibit power conversion efficiencies of above 20% for 6 mm(2) sized pixels and 18.9% for a device area of 1 cm(2). These are record efficiencies for hybrid perovskite devices with dopant-free transport layers, highlighting the potential of this device technology to avoid charge-transport limitations and to approach the Shockley-Queisser limit.
Y1  - 2017
U6  - https://doi.org/10.1039/c7ee00899f
SN  - 1754-5692
SN  - 1754-5706
VL  - 10
SP  - 1530
EP  - 1539
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Zacharias, Michael
A1  - Chen, Xuhui
A1  - Wagner, Stefan
T1  - Attenuation of TeV gamma-rays by the starlight photon field of the host galaxy
JF  - Monthly notices of the Royal Astronomical Society
N2  - The absorption of TeV gamma-ray photons produced in relativistic jets by surrounding soft photon fields is a long-standing problem of jet physics. In some cases, the most likely emission site close to the central black hole is ruled out because of the high opacity caused by strong optical and infrared photon sources, such as the broad-line region. Mostly neglected for jet modelling is the absorption of gamma-rays in the starlight photon field of the host galaxy. Analysing the absorption for arbitrary locations and observation angles of the gamma-ray emission site within the host galaxy, we find that the distance to the galaxy centre, the observation angle, and the distribution of starlight in the galaxy are crucial for the amount of absorption. We derive the absorption value for a sample of 20 TeV-detected blazars with a redshift z(r) < 0.2. The absorption value of the gamma-ray emission located in the galaxy centre may be as high as 20 per cent, with an average value of 6 per cent. This is important in order to determine the intrinsic blazar parameters. We see no significant trends in our sample between the degree of absorption and host properties, such as starlight emissivity, galactic size, half-light radius, and redshift. While the uncertainty of the spectral properties of the extragalactic background light exceeds the effect of absorption by stellar light from the host galaxy in distant objects, the latter is a dominant effect in nearby sources. It may also be revealed in a differential comparison of sources with similar redshifts.
KW  - opacity
KW  - radiation mechanisms: non-thermal
KW  - galaxies: active
KW  - gamma-rays: galaxies
Y1  - 2016
U6  - https://doi.org/10.1093/mnras/stw3032
SN  - 0035-8711
SN  - 1365-2966
VL  - 465
IS  - 3
SP  - 3767
EP  - 3774
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Schöller, Markus
A1  - Hubrig, Swetlana
A1  - Fossati, L.
A1  - Carroll, Thorsten Anthony
A1  - Briquet, Maryline
A1  - Oskinova, Lida
A1  - Järvinen, S.
A1  - Ilyin, Ilya
A1  - Castro, N.
A1  - Morel, T.
A1  - Langer, N.
A1  - Przybilla, N.
A1  - Nieva, M. -F.
A1  - Kholtygin, A. F.
A1  - Sana, H.
A1  - Herrero, A.
A1  - Barba, R. H.
A1  - de Koter, A.
T1  - B fields in OB stars (BOB)
BT  - Concluding the FORS2 observing campaign
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Aims. The B fields in OB stars (BOB) Collaboration is based on an ESO Large Programme to study the occurrence rate, properties, and ultimately the origin of magnetic fields in massive stars. Methods. In the framework of this program, we carried out low-resolution spectropolarimetric observations of a large sample of massive stars using FORS2 installed at the ESO VLT 8m telescope. Results. We determined the magnetic field values with two completely independent reduction and analysis pipelines. Our in-depth study of the magnetic field measurements shows that differences between our two pipelines are usually well within 3 sigma errors. From the 32 observations of 28 OB stars, we were able to monitor the magnetic fields in CPD -57 degrees 3509 and HD164492C, confirm the magnetic field in HD54879, and detect a magnetic field in CPD -62 degrees 2124. We obtain a magnetic field detection rate of 6 +/- 3% for the full sample of 69 OB stars observed with FORS 2 within the BOB program. For the preselected objects with a nu sin i below 60 km s(-1), we obtain a magnetic field detection rate of 5 +/- 5%. We also discuss X-ray properties and multiplicity of the objects in our FORS2 sample with respect to the magnetic field detections.
KW  - polarization
KW  - stars: early-type
KW  - stars: magnetic field
KW  - stars: massive
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201628905
SN  - 1432-0746
VL  - 599
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Delle Side, Domenico
A1  - Nassisi, Vincenzo
A1  - Pennetta, Cecilia
A1  - Alifano, Pietro
A1  - Di Salvo, Marco
A1  - Tala, Adelfia
A1  - Chechkin, Aleksei V.
A1  - Seno, Flavio
A1  - Trovato, Antonio
T1  - Bacterial bioluminescence onset and quenching: a dynamical model for a quorum sensing-mediated property
JF  - Royal Society Open Science
N2  - We present an effective dynamical model for the onset of bacterial bioluminescence, one of the most studied quorum sensing-mediated traits. Our model is built upon simple equations that describe the growth of the bacterial colony, the production and accumulation of autoinducer signal molecules, their sensing within bacterial cells, and the ensuing quorum activation mechanism that triggers bioluminescent emission. The model is directly tested to quantitatively reproduce the experimental distributions of photon emission times, previously measured for bacterial colonies of Vibrio jasicida, a luminescent bacterium belonging to the Harveyi clade, growing in a highly drying environment. A distinctive and novel feature of the proposed model is bioluminescence ‘quenching’ after a given time elapsed from activation. Using an advanced fitting procedure based on the simulated annealing algorithm, we are able to infer from the experimental observations the biochemical parameters used in the model. Such parameters are in good agreement with the literature data. As a further result, we find that, at least in our experimental conditions, light emission in bioluminescent bacteria appears to originate from a subtle balance between colony growth and quorum activation due to autoinducers diffusion, with the two phenomena occurring on the same time scale. This finding is consistent with a negative feedback mechanism previously reported for Vibrio harveyi.
KW  - quorum sensing
KW  - bioluminescence
KW  - biophysical model
KW  - Vibrio Harveyi clade
KW  - oxygen quenching
KW  - Gompertz growth function
Y1  - 2017
U6  - https://doi.org/10.1098/rsos.171586
SN  - 2054-5703
VL  - 4
PB  - Royal Society
CY  - London
ER  - 
TY  - JOUR
A1  - Sandev, Trifce
A1  - Sokolov, Igor M.
A1  - Metzler, Ralf
A1  - Chechkin, Aleksei V.
T1  - Beyond monofractional kinetics
JF  - Chaos, solitons & fractals : applications in science and engineering ; an interdisciplinary journal of nonlinear science
N2  - We discuss generalized integro-differential diffusion equations whose integral kernels are not of a simple power law form, and thus these equations themselves do not belong to the family of fractional diffusion equations exhibiting a monoscaling behavior. They instead generate a broad class of anomalous nonscaling patterns, which correspond either to crossovers between different power laws, or to a non-power-law behavior as exemplified by the logarithmic growth of the width of the distribution. We consider normal and modified forms of these generalized diffusion equations and provide a brief discussion of three generic types of integral kernels for each form, namely, distributed order, truncated power law and truncated distributed order kernels. For each of the cases considered we prove the non-negativity of the solution of the corresponding generalized diffusion equation and calculate the mean squared displacement. (C) 2017 Elsevier Ltd. All rights reserved.
KW  - Distributed order diffusion-wave equations
KW  - Complete Bernstein function
KW  - Completely monotone function
Y1  - 2017
U6  - https://doi.org/10.1016/j.chaos.2017.05.001
SN  - 0960-0779
SN  - 1873-2887
VL  - 102
SP  - 210
EP  - 217
PB  - Elsevier
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Bolotov, Maxim I.
A1  - Smirnov, Lev A.
A1  - Osipov, Grigory V.
A1  - Pikovskij, Arkadij
T1  - Breathing chimera in a system of phase oscillators
JF  - JETP Letters
N2  - Chimera states consisting of synchronous and asynchronous domains in a medium of nonlinearly coupled phase oscillators have been considered. Stationary inhomogeneous solutions of the Ott-Antonsen equation for a complex order parameter that correspond to fundamental chimeras have been constructed. The direct numerical simulation has shown that these structures under certain conditions are transformed to oscillatory (breathing) chimera regimes because of the development of instability.
Y1  - 2017
U6  - https://doi.org/10.1134/S0021364017180059
SN  - 0021-3640
SN  - 1090-6487
VL  - 106
SP  - 393
EP  - 399
PB  - Pleiades Publ.
CY  - New York
ER  - 
TY  - JOUR
A1  - Chechkin, Aleksei V.
A1  - Seno, Flavio
A1  - Metzler, Ralf
A1  - Sokolov, Igor M.
T1  - Brownian yet Non-Gaussian Diffusion: From Superstatistics to Subordination of Diffusing Diffusivities
JF  - Physical review : X, Expanding access
N2  - A growing number of biological, soft, and active matter systems are observed to exhibit normal diffusive dynamics with a linear growth of the mean-squared displacement, yet with a non-Gaussian distribution of increments. Based on the Chubinsky-Slater idea of a diffusing diffusivity, we here establish and analyze a minimal model framework of diffusion processes with fluctuating diffusivity. In particular, we demonstrate the equivalence of the diffusing diffusivity process with a superstatistical approach with a distribution of diffusivities, at times shorter than the diffusivity correlation time. At longer times, a crossover to a Gaussian distribution with an effective diffusivity emerges. Specifically, we establish a subordination picture of Brownian but non-Gaussian diffusion processes, which can be used for a wide class of diffusivity fluctuation statistics. Our results are shown to be in excellent agreement with simulations and numerical evaluations.
Y1  - 2017
U6  - https://doi.org/10.1103/PhysRevX.7.021002
SN  - 2160-3308
VL  - 7
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Kuckein, Christoph
A1  - Diercke, Andrea
A1  - González Manrique, Sergio Javier
A1  - Verma, Meetu
A1  - Loehner-Boettcher, Johannes
A1  - Socas-Navarro, H.
A1  - Balthasar, Horst
A1  - Sobotka, M.
A1  - Denker, Carsten
T1  - Ca II 8542 angstrom brightenings induced by a solar microflare
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Aims. We study small-scale brightenings in Ca II 8542 angstrom line-core images to determine their nature and effect on localized heating and mass transfer in active regions. Methods. High-resolution two-dimensional spectroscopic observations of a solar active region in the near-infrared Ca II 8542 angstrom line were acquired with the GREGOR Fabry-Perot Interferometer attached to the 1.5-m GREGOR telescope. Inversions of the spectra were carried out using the NICOLE code to infer temperatures and line-of-sight (LOS) velocities. Response functions of the Ca II line were computed for temperature and LOS velocity variations. Filtergrams of the Atmospheric Imaging Assembly (AIA) and magnetograms of the Helioseismic and Magnetic Imager (HMI) were coaligned to match the ground-based observations and to follow the Ca II brightenings along all available layers of the atmosphere. Results. We identified three brightenings of sizes up to 2 ' x 2 ' that appeared in the Ca II 8542 angstrom line-core images. Their lifetimes were at least 1.5 min. We found evidence that the brightenings belonged to the footpoints of a microflare (MF). The properties of the observed brightenings disqualified the scenarios of Ellerman bombs or Interface Region Imaging Spectrograph (IRIS) bombs. However, this MF shared some common properties with flaring active-region fibrils or flaring arch filaments (FAFs): (1) FAFs and MFs are both apparent in chromospheric and coronal layers according to the AIA channels; and (2) both show flaring arches with lifetimes of about 3.0-3.5 min and lengths of similar to 20 ' next to the brightenings. The inversions revealed heating by 600 K at the footpoint location in the ambient chromosphere during the impulsive phase. Connecting the footpoints, a dark filamentary structure appeared in the Ca II line-core images. Before the start of the MF, the spectra of this structure already indicated average blueshifts, meaning upward motions of the plasma along the LOS. During the impulsive phase, these velocities increased up to -2.2 km s(-1). The structure did not disappear during the observations. Downflows dominated at the footpoints. However, in the upper photosphere, slight upflows occurred during the impulsive phase. Hence, bidirectional flows are present in the footpoints of the MF.
KW  - Sun: photosphere
KW  - Sun: chromosphere
KW  - Sun: corona
KW  - Sun: activity
KW  - techniques: imaging spectroscopy
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201731319
SN  - 1432-0746
VL  - 608
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Yin, Zhong
A1  - Inhester, Ludger
A1  - Veedu, Sreevidya Thekku
A1  - Quevedo, Wilson
A1  - Pietzsch, Annette
A1  - Wernet, Philippe
A1  - Groenhof, Gerrit
A1  - Föhlisch, Alexander
A1  - Grubmueller, Helmut
A1  - Techert, Simone
T1  - Cationic and Anionic Impact on the Electronic Structure of Liquid Water
JF  - The journal of physical chemistry letters
N2  - Hydration shells around ions are crucial for many fundamental biological and chemical processes. Their local physicochemical properties are quite different from those of bulk water and hard to probe experimentally. We address this problem by combining soft X-ray spectroscopy using a liquid jet and molecular dynamics (MD) simulations together with ab initio electronic structure calculations to elucidate the water ion interaction in a MgCl2 solution at the molecular level. Our results reveal that salt ions mainly affect the electronic properties of water molecules in close vicinity and that the oxygen K-edge X-ray emission spectrum of water molecules in the first solvation shell differs significantly from that of bulk water. Ion-specific effects are identified by fingerprint features in the water X-ray emission spectra. While Mg2+ ions cause a bathochromic shift of the water lone pair orbital, the 3p orbital of the Cl- ions causes an additional peak in the water emission spectrum at around 528 eV.
Y1  - 2017
U6  - https://doi.org/10.1021/acs.jpclett.7b01392
SN  - 1948-7185
VL  - 8
SP  - 3759
EP  - 3764
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Petereit, Johannes
A1  - Pikovskij, Arkadij
T1  - Chaos synchronization by nonlinear coupling
JF  - Communications in nonlinear science & numerical simulation
N2  - We study synchronization properties of three nonlinearly coupled chaotic maps. Coupling is introduced in such a way, that it cannot be reduced to pairwise terms, but includes combined action of all interacting units. For two models of nonlinear coupling we characterize the transition to complete synchrony, as well as partially synchronized states. Relation to hypernetworks of chaotic units is also discussed.
KW  - Chaos synchronization
KW  - Partial synchrony
KW  - Intermittency
KW  - Hypernetwork
Y1  - 2016
U6  - https://doi.org/10.1016/j.cnsns.2016.09.002
SN  - 1007-5704
SN  - 1878-7274
VL  - 44
SP  - 344
EP  - 351
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Politi, Antonio
A1  - Pikovskij, Arkadij
A1  - Ullner, Ekkehard
T1  - Chaotic macroscopic phases in one-dimensional oscillators
JF  - European physical journal special topics
N2  - The connection between the macroscopic description of collective chaos and the underlying microscopic dynamics is thoroughly analysed in mean-field models of one-dimensional oscillators. We investigate to what extent infinitesimal perturbations of the microscopic configurations can provide information also on the stability of the corresponding macroscopic phase. In ensembles of identical one-dimensional dynamical units, it is possible to represent the microscopic configurations so as to make transparent their connection with the macroscopic world. As a result, we find evidence of an intermediate, mesoscopic, range of distances, over which the instability is neither controlled by the microscopic equations nor by the macroscopic ones. We examine a whole series of indicators, ranging from the usual microscopic Lyapunov exponents, to the collective ones, including finite-amplitude exponents. A system of pulse-coupled oscillators is also briefly reviewed as an example of non-identical phase oscillators where collective chaos spontaneously emerges.
Y1  - 2017
U6  - https://doi.org/10.1140/epjst/e2017-70056-4
SN  - 1951-6355
SN  - 1951-6401
VL  - 226
SP  - 1791
EP  - 1810
PB  - Springer
CY  - Heidelberg
ER  - 
TY  - JOUR
A1  - Abdalla, H.
A1  - Abramowski, A.
A1  - Aharonian, Felix A.
A1  - Benkhali, F. Ait
A1  - Akhperjanian, A. G.
A1  - Andersson, T.
A1  - Anguener, E. O.
A1  - Arrieta, M.
A1  - Aubert, P.
A1  - Backes, M.
A1  - Balzer, A.
A1  - Barnard, M.
A1  - Becherini, Y.
A1  - Tjus, J. Becker
A1  - Berge, D.
A1  - Bernhard, S.
A1  - Bernlorhr, K.
A1  - Blackwell, R.
A1  - Bottcher, M.
A1  - Boisson, C.
A1  - Bolmont, J.
A1  - Bordas, Pol
A1  - Bregeon, J.
A1  - Brun, F.
A1  - Brun, P.
A1  - Bryan, M.
A1  - Bulik, T.
A1  - Capasso, M.
A1  - Carr, J.
A1  - Casanova, Sabrina
A1  - Cerruti, M.
A1  - Chakraborty, N.
A1  - Chalme-Calvet, R.
A1  - Chaves, R. C. G.
A1  - Chen, A.
A1  - Chevalier, J.
A1  - Chretien, M.
A1  - Colafrancesco, S.
A1  - Cologna, G.
A1  - Condon, B.
A1  - Conrad, J.
A1  - Cui, Y.
A1  - Davids, I. D.
A1  - Decock, J.
A1  - Degrange, B.
A1  - Deil, C.
A1  - Devin, J.
A1  - deWilt, P.
A1  - Dirson, L.
A1  - Djannati-Atai, A.
A1  - Domainko, W.
A1  - Donath, A.
A1  - Dubus, G.
A1  - Dutson, K.
A1  - Dyks, J.
A1  - Edwards, T.
A1  - Egberts, Kathrin
A1  - Eger, P.
A1  - Ernenwein, J. -P.
A1  - Eschbach, S.
A1  - Farnier, C.
A1  - Fegan, S.
A1  - Fernandes, M. V.
A1  - Fiasson, A.
A1  - Fontaine, G.
A1  - Foerster, A.
A1  - Funk, S.
A1  - Fuessling, M.
A1  - Gabici, S.
A1  - Gajdus, M.
A1  - Gallant, Y. A.
A1  - Garrigoux, T.
A1  - Giavitto, G.
A1  - Giebels, B.
A1  - Glicenstein, J. F.
A1  - Gottschall, D.
A1  - Goyal, A.
A1  - Grondin, M. -H.
A1  - Hadasch, D.
A1  - Hahn, J.
A1  - Haupt, M.
A1  - Hawkes, J.
A1  - Heinzelmann, G.
A1  - Henri, G.
A1  - Hermann, G.
A1  - Hervet, O.
A1  - Hinton, J. A.
A1  - Hofmann, W.
A1  - Hoischen, Clemens
A1  - Holler, M.
A1  - Horns, D.
A1  - Ivascenko, A.
A1  - Jacholkowska, A.
A1  - Jamrozy, M.
A1  - Janiak, M.
A1  - Jankowsky, D.
A1  - Jankowsky, F.
A1  - Jingo, M.
A1  - Jogler, T.
A1  - Jouvin, L.
A1  - Jung-Richardt, I.
A1  - Kastendieck, M. A.
A1  - Katarzynski, K.
A1  - Katz, U.
A1  - Kerszberg, D.
A1  - Khelifi, B.
A1  - Er, M. Kie Ff
A1  - King, J.
A1  - Klepser, S.
A1  - Klochkov, D.
A1  - Kluzniak, W.
A1  - Kolitzus, D.
A1  - Komin, Nu.
A1  - Kosack, K.
A1  - Krakau, S.
A1  - Kraus, M.
A1  - Krayzel, F.
A1  - Kruger, P. P.
A1  - Laffon, H.
A1  - Lamanna, G.
A1  - Lau, J.
A1  - Lees, J. -P.
A1  - Lefaucheur, J.
A1  - Lefranc, V.
A1  - Lemiere, A.
A1  - Lemoine-Goumard, M.
A1  - Lenain, J. -P.
A1  - Leser, E.
A1  - Lohse, T.
A1  - Lorentz, M.
A1  - Liu, R.
A1  - Lopez-Coto, R.
A1  - Lypova, I.
A1  - Marandon, V.
A1  - Marcowith, Alexandre
A1  - Mariaud, C.
A1  - Marx, R.
A1  - Maurin, G.
A1  - Maxted, N.
A1  - Mayer, M.
A1  - Meintjes, P. J.
A1  - Meyer, M.
A1  - Mitchell, A. M. W.
A1  - Moderski, R.
A1  - Mohamed, M.
A1  - Mohrmann, L.
A1  - Mora, K.
A1  - Moulin, Emmanuel
A1  - Murach, T.
A1  - de Naurois, M.
A1  - Niederwanger, F.
A1  - Niemiec, J.
A1  - Oakes, L.
A1  - Odaka, H.
A1  - Oettl, S.
A1  - Ohm, S.
A1  - Ostrowski, M.
A1  - Oya, I.
A1  - Padovani, M.
A1  - Panter, M.
A1  - Parsons, R. D.
A1  - Pekeur, N. W.
A1  - Pelletier, G.
A1  - Perennes, C.
A1  - Petrucci, P. -O.
A1  - Peyaud, B.
A1  - Piel, Q.
A1  - Pita, S.
A1  - Poon, H.
A1  - Prokhorov, D.
A1  - Prokoph, H.
A1  - Puehlhofer, G.
A1  - Punch, M.
A1  - Quirrenbach, A.
A1  - Raab, S.
A1  - Reimer, A.
A1  - Reimer, O.
A1  - Renaud, M.
A1  - de los Reyes, R.
A1  - Rieger, F.
A1  - Romoli, C.
A1  - Rosier-Lees, S.
A1  - Rowell, G.
A1  - Rudak, B.
A1  - Rulten, C. B.
A1  - Sahakian, V.
A1  - Salek, D.
A1  - Sanchez, D. A.
A1  - Santangelo, A.
A1  - Sasaki, M.
A1  - Schlickeiser, R.
A1  - Schussler, F.
A1  - Schulz, A.
A1  - Schwanke, U.
A1  - Schwemmer, S.
A1  - Settimo, M.
A1  - Seyffert, A. S.
A1  - Shafi, N.
A1  - Shilon, I.
A1  - Simoni, R.
A1  - Sol, H.
A1  - Spanier, F.
A1  - Spengler, G.
A1  - Spies, F.
A1  - Ert, Ff
A1  - Stawarz, L.
A1  - Steenkamp, R.
A1  - Stegmann, Christian Michael
A1  - Stinzing, F.
A1  - Stycz, K.
A1  - Sushch, I.
A1  - Tavernet, J. -P.
A1  - Tavernier, T.
A1  - Taylor, A. M.
A1  - Terrier, R.
A1  - Tibaldo, L.
A1  - Tiziani, D.
A1  - Tluczykont, M.
A1  - Trichard, C.
A1  - Tuffs, R.
A1  - Uchiyama, Y.
A1  - van der Walt, D. J.
A1  - van Eldik, C.
A1  - van Rensburg, C.
A1  - van Soelen, B.
A1  - Vasileiadis, G.
A1  - Veh, J.
A1  - Venter, C.
A1  - Viana, A.
A1  - Vincent, P.
A1  - Vink, J.
A1  - Voisin, F.
A1  - Voelk, H. J.
A1  - Vuillaume, T.
A1  - Wadiasingh, Z.
A1  - Wagner, S. J.
A1  - Wagner, P.
A1  - Wagner, R. M.
A1  - White, R.
A1  - Wierzcholska, A.
A1  - Willmann, P.
A1  - Woernlein, A.
A1  - Wouters, D.
A1  - Yang, R.
A1  - Zabalza, V.
A1  - Zaborov, D.
A1  - Zacharias, M.
A1  - Zdziarski, A. A.
A1  - Zech, Alraune
A1  - Zefi, F.
A1  - Ziegler, A.
A1  - Zywucka, N.
T1  - Characterizing the gamma-ray long-term variability of PKS2155 304 with HESS and Fermi-LAT
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Studying the temporal variability of BL Lac objects at the highest energies provides unique insights into the extreme physical processes occurring in relativistic jets and in the vicinity of super-massive black holes. To this end, the long-term variability of the BL Lac object PKS 2155 304 is analyzed in the high (HE, 100MeV < E < 300 GeV) and very high energy (VHE, E > 200 GeV) gamma-ray domain. Over the course of similar to 9 yr of H. E. S. S. observations the VHE light curve in the quiescent state is consistent with a log-normal behavior. The VHE variability in this state is well described by flicker noise (power-spectral-density index beta(VHE) = 1 .10(+ 0 : 10) (0 : 13)) on timescales larger than one day. An analysis of similar to 5.5 yr of HE Fermi-LAT data gives consistent results (beta(HE) = 1 : 20(+ 0 : 21) (0 : 23), on timescales larger than 10 days) compatible with the VHE findings. The HE and VHE power spectral densities show a scale invariance across the probed time ranges. A direct linear correlation between the VHE and HE fluxes could neither be excluded nor firmly established. These long-term-variability properties are discussed and compared to the red noise behavior (beta similar to 2) seen on shorter timescales during VHE-flaring states. The difference in power spectral noise behavior at VHE energies during quiescent and flaring states provides evidence that these states are influenced by different physical processes, while the compatibility of the HE and VHE long-term results is suggestive of a common physical link as it might be introduced by an underlying jet-disk connection.
KW  - galaxies: active
KW  - BL Lacertae objects: individual: PKS 2155-304
KW  - gamma rays: galaxies
KW  - galaxies: jets
KW  - galaxies: nuclei
KW  - radiation mechanisms: non-thermal
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201629419
SN  - 1432-0746
SN  - 0004-6361
VL  - 598
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Laquai, Frederic
A1  - Andrienko, Denis
A1  - Deibel, Carsten
A1  - Neher, Dieter
T1  - Charge carrier generation, recombination, and extraction in polymer-fullerene bulk heterojunction organic solar cells
JF  - Elementary processes in organic photovoltaics
N2  - In this chapter we review the basic principles of photocurrent generation in bulk heterojunction organic solar cells, discuss the loss channels limiting their efficiency, and present case studies of several polymer-fullerene blends. Using steady-state and transient, optical, and electrooptical techniques, we create a precise picture of the fundamental processes that ultimately govern solar cell efficiency.
KW  - Charge extraction
KW  - Charge generation
KW  - Charge recombination
KW  - Organic solar cells
KW  - PBT7
KW  - PBTTT
KW  - PCPDTBT
Y1  - 2026
SN  - 978-3-319-28338-8
SN  - 978-3-319-28336-4
U6  - https://doi.org/10.1007/978-3-319-28338-8_11
SN  - 0065-3195
VL  - 272
SP  - 267
EP  - 291
PB  - Springer
CY  - Berlin
ER  - 
TY  - JOUR
A1  - Roland, Steffen
A1  - Yan, Liang
A1  - Zhang, Qianqian
A1  - Jiao, Xuechen
A1  - Hunt, Adrian
A1  - Ghasemi, Masoud
A1  - Ade, Harald
A1  - You, Wei
A1  - Neher, Dieter
T1  - Charge Generation and Mobility-Limited Performance of Bulk Heterojunction Solar Cells with a Higher Adduct Fullerene
JF  - The journal of physical chemistry : C, Nanomaterials and interfaces
N2  - Alternative electron acceptors are being actively explored in order to advance the development of bulk-heterojunction (BHJ) organic solar cells (OSCs). The indene-C-60 bisadduct (ICBA) has been regarded as a promising candidate, as it provides high open-circuit voltage in BHJ solar cells; however, the photovoltaic performance of such ICBA-based devices is often inferior when compared to cells with the omnipresent PCBM electron acceptor. Here, by pairing the high performance polymer (FTAZ) as the donor with either PCBM or ICBA as the acceptor, we explore the physical mechanism behind the reduced performance of the ICBA-based device. Time delayed collection field (TDCF) experiments reveal reduced, yet field-independent free charge generation in the FTAZ:ICBA system, explaining the overall lower photocurrent in its cells. Through the analysis of the photoluminescence, photogeneration, and electroluminescence, we find that the lower generation efficiency is neither caused by inefficient exciton splitting, nor do we find evidence for significant energy back-transfer from the CT state to singlet excitons. In fact, the increase in open circuit voltage when replacing PCBM by ICBA is entirely caused by the increase in the CT energy, related to the shift in the LUMO energy, while changes in the radiative and nonradiative recombination losses are nearly absent. On the other hand, space charge limited current (SCLC) and bias-assisted charge extraction (BACE) measurements consistently reveal a severely lower electron mobilitiy in the FTAZ:ICBA blend. Studies of the blends with resonant soft X-ray scattering (R-SoXS), grazing incident wide-angle X-ray scattering (GIWAXS), and scanning transmission X-ray microscopy (STXM) reveal very little differences in the mesoscopic morphology but significantly less nanoscale molecular ordering of the fullerene domains in the ICBA based blends, which we propose as the main cause for the lower generation efficiency and smaller electron mobility. Calculations of the JV curves with an analytical model, using measured values, show good agreement with the experimentally determined JV characteristics, proving that these devices suffer from slow carrier extraction, resulting in significant bimolecular recombination losses. Therefore, this study highlights the importance of high charge carrier mobility for newly synthesized acceptor materials, in addition to having suitable energy levels.
Y1  - 2017
U6  - https://doi.org/10.1021/acs.jpcc.7b02288
SN  - 1932-7447
VL  - 121
SP  - 10305
EP  - 10316
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Koopman, Wouter-Willem Adriaan
A1  - Natali, Marco
A1  - Donati, Giovanni P.
A1  - Muccini, Michele
A1  - Toffanin, Stefano
T1  - Charge-exciton interaction rate in organic field-effect transistors by means of transient photoluminescence electromodulated spectroscopy
JF  - ACS photonics
N2  - Organic light-emitting transistors (OLETs) offer a huge potential for the design of highly integrated multifunctional optoelectronic systems and of intense nano scale light sources, such as the long-searched-for electrically pumped organic laser. In order to fulfill these promises, the efficiency and brightness of the current state-of-the-art devices have to be increased significantly. The dominating quenching process limiting the external quantum efficiency in OLETs is charge-exciton interaction. A comprehensive understanding of this quenching process is therefore of paramount importance. The present article reports a systematic investigation of charge-exciton interaction in organic transistors employing time resolved photoluminescence electro-modulation (PLEM) spectroscopy on the picosecond time scale. The results show that the injected charges reduce the exciton radiative recombination in two ways: (i) charges may prevent the generation of excitons and (ii) charges activate a further nonradiative channel for the exciton decay. Moreover, the transient PLEM measurements clearly reveal that not only trapped charges, as already reported in literature, but rather the entire injected charge density contributes to the quenching of the exciton population.
KW  - photoluminescence quenching
KW  - charge density
KW  - exciton dynamics
KW  - organic
KW  - field-effect transistor
KW  - light emission
KW  - optical spectroscopy
Y1  - 2017
U6  - https://doi.org/10.1021/acsphotonics.6b00573
SN  - 2330-4022
VL  - 4
IS  - 2
SP  - 282
EP  - 291
PB  - American Chemical Society
CY  - Washington, DC
ER  - 
TY  - JOUR
A1  - Wang, Jingwen
A1  - Rychkov, Dmitry
A1  - Gerhard, Reimund
T1  - Chemical modification with orthophosphoric acid enhances surface-charge stability on polypropylene electrets
JF  - Applied physics letters
N2  - The low surface-charge stability of polypropylene (PP) frequently limits its application as an electret material. In this paper, we demonstrate how the treatment of PP-film surfaces with orthophosphoric acid (H3PO4) enhances their charge stability. To discriminate between the effects of chemical modification and thermal treatment, as-received and annealed PP films are used as reference samples. The electret properties of treated and non-treated PP films are characterized with thermally stimulated discharge (TSD) and isothermal surface-potential decay (ISPD) experiments, from which considerable improvement in thermal and temporal charge stability is observed for samples modified with H3PO4. The half-value temperature (T-1/2) observed on TSD curves of chemically treated PP increases to 131 and 145 degrees C for positive and negative charges, respectively. The enhancement might be attributed to the phosphoric compounds detected on the H3PO4-modified surfaces via attenuated-total-reflection infrared spectroscopy. Deeper surface traps formed at the "foreign" phosphorus-containing structures are able to capture the charges over longer time periods and at higher temperatures, thus leading to significant improvements in the temporal and thermal surface-charge stabilities of PP electrets. Published by AIP Publishing.
Y1  - 2017
U6  - https://doi.org/10.1063/1.4983348
SN  - 0003-6951
SN  - 1077-3118
VL  - 110
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Smirnov, Lev A.
A1  - Osipov, Grigory V.
A1  - Pikovskij, Arkadij
T1  - Chimera patterns in the Kuramoto-Battogtokh model
JF  - Journal of physics : A, Mathematical and theoretical
N2  - Kuramoto and Battogtokh (2002 Nonlinear Phenom. Complex Syst. 5 380) discovered chimera states represented by stable coexisting synchrony and asynchrony domains in a lattice of coupled oscillators. After a reformulation in terms of a local order parameter, the problem can be reduced to partial differential equations. We find uniformly rotating, spatially periodic chimera patterns as solutions of a reversible ordinary differential equation, and demonstrate a plethora of such states. In the limit of neutral coupling they reduce to analytical solutions in the form of one-and two-point chimera patterns as well as localized chimera solitons. Patterns at weakly attracting coupling are characterized by virtue of a perturbative approach. Stability analysis reveals that only the simplest chimeras with one synchronous region are stable.
KW  - nonlocal coupled oscillators
KW  - chimera state
KW  - coarse-grained order parameter
KW  - Ott-Antonsen reduction
KW  - perturbation approach
KW  - linear stability analysis
Y1  - 2017
U6  - https://doi.org/10.1088/1751-8121/aa55f1
SN  - 1751-8113
SN  - 1751-8121
VL  - 50
IS  - 8
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Zaks, Michael
A1  - Pikovskij, Arkadij
T1  - Chimeras and complex cluster states in arrays of spin-torque oscillators
JF  - Scientific reports
N2  - We consider synchronization properties of arrays of spin-torque nano-oscillators coupled via an RC load. We show that while the fully synchronized state of identical oscillators may be locally stable in some parameter range, this synchrony is not globally attracting. Instead, regimes of different levels of compositional complexity are observed. These include chimera states (a part of the array forms a cluster while other units are desynchronized), clustered chimeras (several clusters plus desynchronized oscillators), cluster state (all oscillators form several clusters), and partial synchronization (no clusters but a nonvanishing mean field). Dynamically, these states are also complex, demonstrating irregular and close to quasiperiodic modulation. Remarkably, when heterogeneity of spin-torque oscillators is taken into account, dynamical complexity even increases: close to the onset of a macroscopic mean field, the dynamics of this field is rather irregular.
Y1  - 2017
U6  - https://doi.org/10.1038/s41598-017-04918-9
SN  - 2045-2322
VL  - 7
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Zaks, Michael A.
A1  - Pikovskij, Arkadij
T1  - Chimeras and complex cluster states in arrays of spin-torque oscillators
JF  - Scientific reports
N2  - We consider synchronization properties of arrays of spin-torque nano-oscillators coupled via an RC load. We show that while the fully synchronized state of identical oscillators may be locally stable in some parameter range, this synchrony is not globally attracting. Instead, regimes of different levels of compositional complexity are observed. These include chimera states (a part of the array forms a cluster while other units are desynchronized), clustered chimeras (several clusters plus desynchronized oscillators), cluster state (all oscillators form several clusters), and partial synchronization (no clusters but a nonvanishing mean field). Dynamically, these states are also complex, demonstrating irregular and close to quasiperiodic modulation. Remarkably, when heterogeneity of spin-torque oscillators is taken into account, dynamical complexity even increases: close to the onset of a macroscopic mean field, the dynamics of this field is rather irregular.
Y1  - 2017
U6  - https://doi.org/10.1038/s41598-017-04918-9
SN  - 2045-2322
VL  - 7
PB  - Macmillan Publishers Limited
CY  - London
ER  - 
TY  - GEN
A1  - Kubatova, B.
A1  - Kubát, Jiří
A1  - Hamann, Wolf-Rainer
A1  - Oskinova, Lida
T1  - Clumping in Massive Star Winds and its Possible Connection to the B[e] Phenomenon
T2  - The B(e) Phenomenon: Forty Years of Studies : proceedings of a conference held at Charles University, Prague, Czech Republic, 27 June-1 July 2016
N2  - It has been observationally established that winds of hot massive stars have highly variable characteristics. The variability evident in the winds is believed to be caused by structures on a broad range of spatial scales. Small-scale structures (clumping) in stellar winds of hot stars are possible consequence of an instability appearing in their radiation hydrodynamics. To understand how clumping may influence calculation of theoretical spectra, different clumping properties and their 3D nature have to be taken into account. Properties of clumping have been examined using our 3D radiative transfer calculations. Effects of clumping for the case of the B[e] phenomenon are discussed.
Y1  - 2017
SN  - 978-1-58381-900-5
SN  - 978-1-58381-901-2
VL  - 508
SP  - 45
EP  - 50
PB  - Astronomical Soceity of the Pacific
CY  - San Fransisco
ER  - 
TY  - JOUR
A1  - Wernet, Philippe
A1  - Leitner, T.
A1  - Josefsson, Ida
A1  - Mazza, T.
A1  - Miedema, P. S.
A1  - Schroder, H.
A1  - Beye, Martin
A1  - Kunnus, K.
A1  - Schreck, S.
A1  - Radcliffe, P.
A1  - Dusterer, S.
A1  - Meyer, M.
A1  - Odelius, Michael
A1  - Fohlisch, Alexander
T1  - Communication: Direct evidence for sequential dissociation of gas-phase Fe(CO)(5) via a singlet pathway upon excitation at 266 nm
JF  - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr
N2  - We prove the hitherto hypothesized sequential dissociation of Fe(CO)(5) in the gas phase upon photoexcitation at 266 nm via a singlet pathway with time-resolved valence and core-level photoelectron spectroscopy with an x-ray free-electron laser. Valence photoelectron spectra are used to identify free CO molecules and to determine the time constants of stepwise dissociation to Fe(CO)(4) within the temporal resolution of the experiment and further to Fe(CO)(3) within 3 ps. Fe 3p core-level photoelectron spectra directly reflect the singlet spin state of the Fe center in Fe(CO)(5), Fe(CO)(4), and Fe(CO)(3) showing that the dissociation exclusively occurs along a singlet pathway without triplet-state contribution. Our results are important for assessing intra- and intermolecular relaxation processes in the photodissociation dynamics of the prototypical Fe(CO)(5) complex in the gas phase and in solution, and they establish time-resolved core-level photoelectron spectroscopy as a powerful tool for determining the multiplicity of transition metals in photochemical reactions of coordination complexes. Published by AIP Publishing.
Y1  - 2017
U6  - https://doi.org/10.1063/1.4984774
SN  - 0021-9606
SN  - 1089-7690
VL  - 146
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Schimka, Selina
A1  - Gordievskaya, Yulia D.
A1  - Lomadze, Nino
A1  - Lehmann, Maren
A1  - von Klitzing, Regine
A1  - Rumyantsev, Artem M.
A1  - Kramarenko, Elena Yu.
A1  - Santer, Svetlana
T1  - Communication: Light driven remote control of microgels’ size in the  presence of photosensitive surfactant: Complete phase diagram
JF  - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr
N2  - Here we report on a light triggered remote control of microgel size in the presence of photosensitive surfactant. The hydrophobic tail of the cationic surfactant contains azobenzene group that undergoes a reversible photo-isomerization reaction from a trans-to a cis-state accompanied by a change in the hydrophobicity of the surfactant. We have investigated light assisted behaviour and the complex formation of the microgels with azobenzene containing surfactant over the broad concentrational range starting far below and exceeding several times of the critical micelle concentration (CMC). At small surfactant concentration in solution (far below CMC), the surfactant in the trans-state accommodates within the microgel causing its compaction, while the cis-isomer desorbs out of microgel resulting in its swelling. The process of the microgel size change can be described as swelling on UV irradiation (trans-cis isomerization) and shrinking on irradiation with blue light (cis-trans isomerization). However, at the surfactant concentrations larger than CMC, the opposite behaviour is observed: the microgel swells on blue irradiation and shrinks during exposure to UV light. We explain this behaviour theoretically taking into account isomer dependent micellization of surfactant within the microgels. Published by AIP Publishing.
Y1  - 2017
U6  - https://doi.org/10.1063/1.4986143
SN  - 0021-9606
SN  - 1089-7690
VL  - 147
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Palyulin, Vladimir V.
A1  - Mantsevich, Vladimir N.
A1  - Klages, Rainer
A1  - Metzler, Ralf
A1  - Chechkin, Aleksei V.
T1  - Comparison of pure and combined search strategies for single and multiple targets
JF  - The European physical journal : B, Condensed matter and complex systems
N2  - We address the generic problem of random search for a point-like target on a line. Using the measures of search reliability and efficiency to quantify the random search quality, we compare Brownian search with Levy search based on long-tailed jump length distributions. We then compare these results with a search process combined of two different long-tailed jump length distributions. Moreover, we study the case of multiple targets located by a Levy searcher.
Y1  - 2017
U6  - https://doi.org/10.1140/epjb/e2017-80372-4
SN  - 1434-6028
SN  - 1434-6036
VL  - 90
SP  - 20
EP  - 37
PB  - Springer
CY  - New York
ER  - 
TY  - JOUR
A1  - Goldobin, Denis S.
A1  - Pimenova, Anastasiya V.
A1  - Rosenblum, Michael
A1  - Pikovskij, Arkadij
T1  - Competing influence of common noise and desynchronizing coupling on synchronization in the Kuramoto-Sakaguchi ensemble
JF  - European physical journal special topics
N2  - We describe analytically synchronization and desynchronization effects in an ensemble of phase oscillators driven by common noise and by global coupling. Adopting the Ott-Antonsen ansatz, we reduce the dynamics to closed stochastic equations for the order parameters, and study these equations for the cases of populations of identical and nonidentical oscillators. For nonidentical oscillators we demonstrate a counterintuitive effect of divergence of individual frequencies for moderate repulsive coupling, while the order parameter remains large.
Y1  - 2017
U6  - https://doi.org/10.1140/epjst/e2017-70039-y
SN  - 1951-6355
SN  - 1951-6401
VL  - 226
SP  - 1921
EP  - 1937
PB  - Springer
CY  - Heidelberg
ER  - 
TY  - JOUR
A1  - Menzel, Ralf
A1  - Puhlmann, Dirk
A1  - Heuer, Axel
T1  - Complementarity in single photon interference – the role of the mode function and vacuum fields
JF  - Journal of the European Optical Society-Rapid
N2  - Background
In earlier experiments the role of the vacuum fields could be demonstrated as the source of complementarity with respect to the temporal properties (Heuer et al., Phys. Rev. Lett. 114:053601, 2015).

Methods
Single photon first order interferences of spatially separated regions from the cone structure of spontaneous parametric down conversion allow for analyzing the role of the mode function in quantum optics regarding the complementarity principle.

Results
Here the spatial coherence properties of these vacuum fields are demonstrated as the physical reason for complementarity in these single photon quantum optical experiments. These results are directly connected to the mode picture in classical optics.

Conclusion
The properties of the involved vacuum fields selected via the measurement process are the physical background of the complementarity principle in quantum optics.
KW  - Quantum optics
KW  - Complementarity
KW  - Mode function
KW  - Vacuum fields
Y1  - 2017
U6  - https://doi.org/10.1186/s41476-017-0036-x
SN  - 1990-2573
VL  - 13
PB  - Springer
ER  - 
TY  - GEN
A1  - Waldrip, Steven H.
A1  - Niven, Robert K.
A1  - Abel, Markus
A1  - Schlegel, Michael
T1  - Consistent maximum entropy representations of pipe flow networks
T2  - AIP conference proceedings
N2  - The maximum entropy method is used to predict flows on water distribution networks. This analysis extends the water distribution network formulation of Waldrip et al. (2016) Journal of Hydraulic Engineering (ASCE), by the use of a continuous relative entropy defined on a reduced parameter set. This reduction in the parameters that the entropy is defined over ensures consistency between different representations of the same network. The performance of the proposed reduced parameter method is demonstrated with a one-loop network case study.
Y1  - 2017
SN  - 978-0-7354-1527-0
U6  - https://doi.org/10.1063/1.4985365
SN  - 0094-243X
VL  - 1853
IS  - 1
PB  - American Institute of Physics
CY  - Melville
ER  -