TY - JOUR A1 - Rettig, L. A1 - Dornes, C. A1 - Thielemann-Kuehn, Nele A1 - Pontius, N. A1 - Zabel, Hartmut A1 - Schlagel, D. L. A1 - Lograsso, T. A. A1 - Chollet, M. A1 - Robert, A. A1 - Sikorski, M. A1 - Song, S. A1 - Glownia, J. M. A1 - Schuessler-Langeheine, Christian A1 - Johnson, S. L. A1 - Staub, U. T1 - Itinerant and Localized Magnetization Dynamics in Antiferromagnetic Ho JF - Physical review letters N2 - Using femtosecond time-resolved resonant magnetic x-ray diffraction at the Ho L-3 absorption edge, we investigate the demagnetization dynamics in antiferromagnetically ordered metallic Ho after femtosecond optical excitation. Tuning the x-ray energy to the electric dipole (E1, 2p -> 5d) or quadrupole (E2, 2p -> 4f) transition allows us to selectively and independently study the spin dynamics of the itinerant 5d and localized 4f electronic subsystems via the suppression of the magnetic (2 1 3-tau) satellite peak. We find demagnetization time scales very similar to ferromagnetic 4f systems, suggesting that the loss of magnetic order occurs via a similar spin-flip process in both cases. The simultaneous demagnetization of both subsystems demonstrates strong intra-atomic 4f-5d exchange coupling. In addition, an ultrafast lattice contraction due to the release of magneto-striction leads to a transient shift of the magnetic satellite peak. Y1 - 2016 U6 - https://doi.org/10.1103/PhysRevLett.116.257202 SN - 0031-9007 SN - 1079-7114 VL - 116 SP - 6382 EP - 6389 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Siebrecht, R. A1 - Schreyer, A. A1 - Englisch, Uwe A1 - Pietsch, Ullrich A1 - Zabel, Hartmut T1 - The new reflectometer ADAM at the ILL Y1 - 1997 ER - TY - JOUR A1 - Thielemann-Kühn, Nele A1 - Schick, Daniel A1 - Pontius, Niko A1 - Trabant, Christoph A1 - Mitzner, Rolf A1 - Holldack, Karsten A1 - Zabel, Hartmut A1 - Föhlisch, Alexander A1 - Schuessler-Langeheine, Christian T1 - Ultrafast and Energy-Efficient Quenching of Spin Order: Antiferromagnetism Beats Ferromagnetism JF - Physical review letters N2 - By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material-metallic dysprosium-we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much more efficiently reduced by optical excitation than its ferromagnetic counterpart. We assign the fast and extremely efficient process in the antiferromagnet to an interatomic transfer of angular momentum within the spin system. Our findings imply that this angular momentum transfer channel is effective in other magnetic metals with nonparallel spin alignment. They also point out a possible route towards energy-efficient spin manipulation for magnetic devices. Y1 - 2017 U6 - https://doi.org/10.1103/PhysRevLett.119.197202 SN - 0031-9007 SN - 1079-7114 VL - 119 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Pudell, Jan-Etienne A1 - von Reppert, Alexander A1 - Schick, D. A1 - Zamponi, F. A1 - Rössle, Matthias A1 - Herzog, Marc A1 - Zabel, Hartmut A1 - Bargheer, Matias T1 - Ultrafast negative thermal expansion driven by spin disorder JF - Physical review : B, Condensed matter and materials physics N2 - We measure the transient strain profile in a nanoscale multilayer system composed of yttrium, holmium, and niobium after laser excitation using ultrafast x-ray diffraction. The strain propagation through each layer is determined by transient changes in the material-specific Bragg angles. We experimentally derive the exponentially decreasing stress profile driving the strain wave and show that it closely matches the optical penetration depth. Below the Neel temperature of Ho, the optical excitation triggers negative thermal expansion, which is induced by a quasi-instantaneous contractive stress and a second contractive stress contribution increasing on a 12-ps timescale. These two timescales were recently measured for the spin disordering in Ho [Rettig et al., Phys. Rev. Lett. 116, 257202 (2016)]. As a consequence, we observe an unconventional bipolar strain pulse with an inverted sign traveling through the heterostructure. Y1 - 2019 U6 - https://doi.org/10.1103/PhysRevB.99.094304 SN - 2469-9950 SN - 2469-9969 VL - 99 IS - 9 PB - American Physical Society CY - College Park ER -