TY  - JOUR
A1  - Rettig, L.
A1  - Dornes, C.
A1  - Thielemann-Kuehn, Nele
A1  - Pontius, N.
A1  - Zabel, Hartmut
A1  - Schlagel, D. L.
A1  - Lograsso, T. A.
A1  - Chollet, M.
A1  - Robert, A.
A1  - Sikorski, M.
A1  - Song, S.
A1  - Glownia, J. M.
A1  - Schuessler-Langeheine, Christian
A1  - Johnson, S. L.
A1  - Staub, U.
T1  - Itinerant and Localized Magnetization Dynamics in Antiferromagnetic Ho
JF  - Physical review letters
N2  - Using femtosecond time-resolved resonant magnetic x-ray diffraction at the Ho L-3 absorption edge, we investigate the demagnetization dynamics in antiferromagnetically ordered metallic Ho after femtosecond optical excitation. Tuning the x-ray energy to the electric dipole (E1, 2p -> 5d) or quadrupole (E2, 2p -> 4f) transition allows us to selectively and independently study the spin dynamics of the itinerant 5d and localized 4f electronic subsystems via the suppression of the magnetic (2 1 3-tau) satellite peak. We find demagnetization time scales very similar to ferromagnetic 4f systems, suggesting that the loss of magnetic order occurs via a similar spin-flip process in both cases. The simultaneous demagnetization of both subsystems demonstrates strong intra-atomic 4f-5d exchange coupling. In addition, an ultrafast lattice contraction due to the release of magneto-striction leads to a transient shift of the magnetic satellite peak.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.116.257202
SN  - 0031-9007
SN  - 1079-7114
VL  - 116
SP  - 6382
EP  - 6389
PB  - American Physical Society
CY  - College Park
ER  -