TY - JOUR A1 - Blakesley, James C. A1 - Neher, Dieter T1 - Relationship between energetic disorder and open-circuit voltage in bulk heterojunction organic solar cells JF - Physical review : B, Condensed matter and materials physics N2 - We simulate organic bulk heterojunction solar cells. The effects of energetic disorder are incorporated through a Gaussian or exponential model of density of states. Analytical models of open-circuit voltage (V(OC)) are derived from the splitting of quasi-Fermi potentials. Their predictions are backed up by more complex numerical device simulations including effects such as carrier-density-dependent charge-carrier mobilities. It is predicted that the V(OC) depends on: (1) the donor-acceptor energy gap; (2) charge-carrier recombination rates; (3) illumination intensity; (4) the contact work functions (if not in the pinning regime); and (5) the amount of energetic disorder. A large degree of energetic disorder, or a high density of traps, is found to cause significant reductions in V(OC). This can explain why V(OC) is often less than expected in real devices. Energetic disorder also explains the nonideal temperature and intensity dependence of V(OC) and the superbimolecular recombination rates observed in many real bulk heterojunction solar cells. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.84.075210 SN - 1098-0121 VL - 84 IS - 7 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Burylko, Oleksandr A1 - Pikovskij, Arkadij T1 - Desynchronization transitions in nonlinearly coupled phase oscillators JF - Physica :D, Nonlinear phenomena N2 - We consider the nonlinear extension of the Kuramoto model of globally coupled phase oscillators where the phase shift in the coupling function depends on the order parameter. A bifurcation analysis of the transition from fully synchronous state to partial synchrony is performed. We demonstrate that for small ensembles it is typically mediated by stable cluster states, that disappear with creation of heteroclinic cycles, while for a larger number of oscillators a direct transition from full synchrony to a periodic or a quasiperiodic regime occurs. KW - Coupled oscillators KW - Oscillator ensembles KW - Kuramoto model KW - Nonlinear coupling KW - Bifurcations Y1 - 2011 U6 - https://doi.org/10.1016/j.physd.2011.05.016 SN - 0167-2789 VL - 240 IS - 17 SP - 1352 EP - 1361 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Sun, Y-P A1 - Pietzsch, Annette A1 - Hennies, Franz A1 - Rinkevicius, Z. A1 - Karlsson, Hans O. A1 - Schmitt, Thorsten A1 - Strocov, Vladimir N. A1 - Andersson, Joakim A1 - Kennedy, B. A1 - Schlappa, J. A1 - Föhlisch, Alexander A1 - Gel'mukhanov, F. A1 - Rubensson, Jan-Erik T1 - Internal symmetry and selection rules in resonant inelastic soft x-ray scattering JF - Journal of physics : B, Atomic, molecular and optical physics N2 - Resonant inelastic soft x-ray scattering spectra excited at the dissociative 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O(2) are presented and discussed in terms of state-of-the-art molecular theory. A new selection rule due to internal spin coupling is established, facilitating a deep analysis of the valence excited final states. Furthermore, it is found that a commonly accepted symmetry selection rule due to orbital parity breaks down, as the core hole and excited electron swap parity, thereby opening the symmetry forbidden 3 sigma(g) decay channel. Y1 - 2011 U6 - https://doi.org/10.1088/0953-4075/44/16/161002 SN - 0953-4075 VL - 44 IS - 16 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Acciari, V. A. A1 - Aliu, E. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dickherber, R. A1 - Duke, C. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Finnegan, G. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Guenette, R. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - LeBohec, S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Senturk, G. D. A1 - Smith, A. W. A1 - Staszak, D. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. A1 - Zitzer, B. T1 - VERITAS OBSERVATIONS OF THE TeV BINARY LS I+61 degrees 303 DURING 2008-2010 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We present the results of observations of the TeV binary LS I + 61 degrees 303 with the VERITAS telescope array between 2008 and 2010, at energies above 300 GeV. In the past, both ground-based gamma-ray telescopes VERITAS and MAGIC have reported detections of TeV emission near the apastron phases of the binary orbit. The observations presented here show no strong evidence for TeV emission during these orbital phases; however, during observations taken in late 2010, significant emission was detected from the source close to the phase of superior conjunction (much closer to periastron passage) at a 5.6 standard deviation (5.6 sigma) post-trials significance. In total, between 2008 October and 2010 December a total exposure of 64.5 hr was accumulated with VERITAS on LS I + 61 degrees 303, resulting in an excess at the 3.3 sigma significance level for constant emission over the entire integrated data set. The flux upper limits derived for emission during the previously reliably active TeV phases (i.e., close to apastron) are less than 5% of the Crab Nebula flux in the same energy range. This result stands in apparent contrast to previous observations by both MAGIC and VERITAS which detected the source during these phases at 10% of the Crab Nebula flux. During the two year span of observations, a large amount of X-ray data were also accrued on LS I + 61 degrees 303 by the Swift X-ray Telescope and the Rossi X-ray Timing Explorer Proportional Counter Array. We find no evidence for a correlation between emission in the X-ray and TeV regimes during 20 directly overlapping observations. We also comment on data obtained contemporaneously by the Fermi Large Area Telescope. KW - binaries: general KW - gamma rays: general KW - X-rays: binaries Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/738/1/3 SN - 0004-637X VL - 738 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Stich, Michael A1 - Beta, Carsten T1 - Standing waves in a complex Ginzburg-Landau equation with time-delay feedback JF - Discrete and continuous dynamical systems : a journal bridging mathematics and sciences N2 - Standing waves are studied as solutions of a complex Ginsburg-Landau equation subjected to local and global time-delay feedback terms. The onset of standing waves is studied at the instability of the homogeneous periodic solution with respect to spatially periodic perturbations. The solution of this spatiotemporal wave pattern is given and is compared to the homogeneous periodic solution. KW - pattern formation KW - reaction-diffusion system KW - control Y1 - 2011 SN - 1078-0947 SN - 1553-5231 IS - 1 SP - 1329 EP - 1334 PB - American Institute of Mathematical Sciences CY - Springfield ER - TY - JOUR A1 - Hübener, Robert A1 - Kruszynska, Caroline A1 - Hartmann, Lorenz A1 - Duer, Wolfgang A1 - Plenio, Martin B. A1 - Eisert, Jens T1 - Tensor network methods with graph enhancement JF - Physical review : B, Condensed matter and materials physics N2 - We present applications of the renormalization algorithm with graph enhancement (RAGE). This analysis extends the algorithms and applications given for approaches based on matrix product states introduced in [Phys. Rev. A 79, 022317 (2009)] to other tensor-network states such as the tensor tree states (TTS) and projected entangled pair states. We investigate the suitability of the bare TTS to describe ground states, showing that the description of certain graph states and condensed-matter models improves. We investigate graph-enhanced tensor-network states, demonstrating that in some cases (disturbed graph states and for certain quantum circuits) the combination of weighted graph states with TTS can greatly improve the accuracy of the description of ground states and time-evolved states. We comment on delineating the boundary of the classically efficiently simulatable states of quantum many-body systems. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.84.125103 SN - 1098-0121 VL - 84 IS - 12 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Schmah, Tanya A1 - Marwan, Norbert A1 - Thomsen, Jesper Skovhus A1 - Saparin, Peter T1 - Long range node-strut analysis of trabecular bone microarchitecture JF - Medical physics : the international journal of medical physics research and practice N2 - Purpose: We present a new morphometric measure of trabecular bone microarchitecture, called mean node strength (NdStr), which is part of a newly developed approach called long range nodestrut analysis. Our general aim is to describe and quantify the apparent "latticelike" microarchitecture of the trabecular bone network. Methods: Similar in some ways to the topological node-strut analysis introduced by Garrahan et al. [J. Microsc. 142, 341-349 (1986)], our method is distinguished by an emphasis on long-range trabecular connectivity. Thus, while the topological classification of a pixel (after skeletonization) as a node, strut, or terminus, can be determined from the 3 x 3 neighborhood of that pixel, our method, which does not involve skeletonization, takes into account a much larger neighborhood. In addition, rather than giving a discrete classification of each pixel as a node, strut, or terminus, our method produces a continuous variable, node strength. The node strength is averaged over a region of interest to produce the mean node strength of the region. Results: We have applied our long range node-strut analysis to a set of 26 high-resolution peripheral quantitative computed tomography (pQCT) axial images of human proximal tibiae acquired 17 mm below the tibial plateau. We found that NdStr has a strong positive correlation with trabecular volumetric bone mineral density (BMD). After an exponential transformation, we obtain a Pearson's correlation coefficient of r - 0.97. Qualitative comparison of images with similar BMD but with very different NdStr values suggests that the latter measure has successfully quantified the prevalence of the "latticelike" microarchitecture apparent in the image. Moreover, we found a strong correlation (r - 0.62) between NdStr and the conventional node-terminus ratio (Nd/Tm) of Garrahan et al. The Nd/Tm ratios were computed using traditional histomorphometry performed on bone biopsies obtained at the same location as the pQCT scans. Conclusions: The newly introduced morphometric measure allows a quantitative assessment of the long-range connectivity of trabecular bone. One advantage of this method is that it is based on pQCT images that can be obtained noninvasively from patients, i.e., without having to obtain a bone biopsy from the patient. KW - trabecular bone KW - osteoporosis KW - structure analysis KW - histomorphometry KW - pQCT Y1 - 2011 U6 - https://doi.org/10.1118/1.3622600 SN - 0094-2405 VL - 38 IS - 9 SP - 5003 EP - 5011 PB - American Association of Physicists in Medicine CY - Melville ER - TY - JOUR A1 - Oskinova, Lida A1 - Todt, Helge Tobias A1 - Ignace, Richard A1 - Brown, John C. A1 - Cassinelli, Joseph P. A1 - Hamann, Wolf-Rainer T1 - Early magnetic B-type stars X-ray emission and wind properties JF - Monthly notices of the Royal Astronomical Society N2 - We present a comprehensive study of X-ray emission by, and wind properties of, massive magnetic early B-type stars. Dedicated XMM-Newton observations were obtained for three early-type B-type stars, xi(1) CMa, V2052 Oph and zeta Cas, with recently discovered magnetic fields. We report the first detection of X-ray emission from V2052 Oph and zeta Cas. The latter is one the softest X-ray sources among the early-type stars, while the former is one of the X-ray faintest. The observations show that the X-ray spectra of our programme stars are quite soft with the bulk of X-ray emitting material having a temperature of about 1 MK. We compile the complete sample of early B-type stars with detected magnetic fields to date and existing X-ray measurements, in order to study whether the X-ray emission can be used as a general proxy for stellar magnetism. We find that the X-ray properties of early massive B-type magnetic stars are diverse, and that hard and strong X-ray emission does not necessarily correlate with the presence of a magnetic field, corroborating similar conclusions reached earlier for the classical chemically peculiar magnetic Bp-Ap stars. We analyse the ultraviolet (UV) spectra of five non-supergiant B stars with magnetic fields (tau Sco, beta Cep, xi(1) CMa, V2052 Oph and zeta Cas) by means of non-local thermodynamic equilibrium (non-LTE) iron-blanketed model atmospheres. The latter are calculated with the Potsdam Wolf-Rayet (PoWR) code, which treats the photosphere as well as the wind, and also accounts for X-rays. With the exception of t Sco, this is the first analysis of these stars by means of stellar wind models. Our models accurately fit the stellar photospheric spectra in the optical and the UV. The parameters of X-ray emission, temperature and flux are included in the model in accordance with observations. We confirm the earlier findings that the filling factors of X-ray emitting material are very high. Our analysis reveals that the magnetic early-type B stars studied here have weak winds with velocities not significantly exceeding upsilon(esc). The mass-loss rates inferred from the analysis of UV lines are significantly lower than predicted by hydrodynamically consistent models. We find that, although the X-rays strongly affect the ionization structure of the wind, this effect is not sufficient in reducing the total radiative acceleration. When the X-rays are accounted for at the intensity and temperatures observed, there is still sufficient radiative acceleration to drive a stronger mass-loss than we empirically infer from the UV spectral lines. KW - techniques: spectroscopic KW - stars: magnetic field KW - stars: massive KW - stars: mass loss KW - X-rays: stars Y1 - 2011 U6 - https://doi.org/10.1111/j.1365-2966.2011.19143.x SN - 0035-8711 VL - 416 IS - 2 SP - 1456 EP - 1474 PB - Wiley-Blackwell CY - Hoboken ER - TY - JOUR A1 - Winkel, B. A1 - Ben Bekhti, Nadya A1 - Darmstaedter, V. A1 - Floeer, L. A1 - Kerp, J. A1 - Richter, Philipp T1 - The high-velocity cloud complex Galactic center negative as seen by EBHIS and GASS I. Cloud catalog and global properties JF - Astronomy and astrophysics : an international weekly journal N2 - Using Milky Way data of the new Effelsberg-Bonn HI Survey (EBHIS) and the Galactic All-Sky Survey (GASS), we present a revised picture of the high-velocity cloud (HVC) complex Galactic center negative (GCN). Owing to the higher angular resolution of these surveys compared to previous studies (e.g., the Leiden Dwingeloo Survey), we resolve complex GCN into lots of individual tiny clumps, that mostly have relatively broad line widths of more than 15 km s(-1). We do not detect a diffuse extended counterpart, which is unusual for an HVC complex. In total 243 clumps were identified and parameterized which allows us to statistically analyze the data. Cold-line components (i.e.,Delta upsilon(fwhm) < 7.5 km s(-1)) are found in about 5% only of the identified cloudlets. Our analysis reveals that complex GCN is likely built up of several subpopulations that do not share a common origin. Furthermore, complex GCN might be a prime example for warm-gas accretion onto the Milky Way, where neutral HI clouds are not stable against interaction with the Milky Way gas halo and become ionized prior to accretion. KW - ISM: clouds KW - Galaxy: halo Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201117357 SN - 0004-6361 VL - 533 IS - 18 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Sun, Zhongkui A1 - Yang, Xiaoli T1 - Generating and enhancing lag synchronization of chaotic systems by white noise JF - Chaos : an interdisciplinary journal of nonlinear science N2 - In this paper, we study the crucial impact of white noise on lag synchronous regime in a pair of time-delay unidirectionally coupled systems. Our result demonstrates that merely via white-noise-based coupling lag synchronization could be achieved between the coupled systems (chaotic or not). And it is also demonstrated that a conventional lag synchronous regime can be enhanced by white noise. Sufficient conditions are further proved mathematically for noise-inducing and noise-enhancing lag synchronization, respectively. Additionally, the influence of parameter mismatch on the proposed lag synchronous regime is studied, by which we announce the robustness and validity of the new strategy. Two numerical examples are provided to illustrate the validity and some possible applications of the theoretical result. Y1 - 2011 U6 - https://doi.org/10.1063/1.3623440 SN - 1054-1500 SN - 1089-7682 VL - 21 IS - 3 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Schuh, Christian A1 - Lomadze, Nino A1 - Rühe, Jürgen A1 - Kopyshev, Alexey A1 - Santer, Svetlana T1 - Photomechanical degrafting of Azo-functionalized Poly(methacrylic acid) (PMAA) brushes JF - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry N2 - We report on the preparation and characterization of photosensitive polymer brushes. The brushes are synthesized through polymer analogous attachment of azobenzene groups to surface-attached poly(methacrylic acid) (PMAA) chains. The topography of the photosensitive brushes shows a strong reaction upon irradiation with UV light. While homogeneous illumination leaves the polymer topography unchanged, irradiation of the samples with interference patterns with periodically varying light intensity leads to the formation of surface relief gratings (SRG). The height of the stripes of the grating can be controlled by adjusting the irradiation time. The SRG pattern can be erased through solvent treatment when the periodicity of the stripe pattern is less than the length of the fully stretched polymer chains. In the opposite case, photomechanical scission of receding polymer chains is observed during SRG formation, and the inscribed patterns are permanent. Y1 - 2011 U6 - https://doi.org/10.1021/jp2041229 SN - 1520-6106 VL - 115 IS - 35 SP - 10431 EP - 10438 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Schuch, Norbert A1 - Harrison, Sarah K. A1 - Osborne, Tobias J. A1 - Eisert, Jens T1 - Information propagation for interacting-particle systems JF - Physical review : A, Atomic, molecular, and optical physics N2 - We study the speed at which information propagates through systems of interacting quantum particles moving on a regular lattice and show that for a certain class of initial conditions there exists a maximum speed of sound at which information can propagate. Our argument applies equally to quantum spins, bosons such as in the Bose-Hubbard model, fermions, anyons, and general mixtures thereof, on arbitrary lattices of any dimension. It also pertains to dissipative dynamics on the lattice, and generalizes to the continuum for quantum fields. Our result can be seen as an analog of the Lieb-Robinson bound for strongly correlated models. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevA.84.032309 SN - 1050-2947 VL - 84 IS - 3 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Eichler, David A1 - Pohl, Martin T1 - Can ultrahigh-energy cosmic rays come from Gamma-ray bursts? - cosmic rays below the ankle and galactic gamma-ray bursts JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - The maximum cosmic-ray energy achievable by acceleration by a relativistic blast wave is derived. It is shown that forward shocks from long gamma-ray bursts (GRBs) in the interstellar medium accelerate protons to large enough energies, and have a sufficient energy budget, to produce the Galactic cosmic-ray component just below the ankle at 4 x 10(18) eV, as per an earlier suggestion. It is further argued that, were extragalactic long GRBs responsible for the component above the ankle as well, the occasional Galactic GRB within the solar circle would contribute more than the observational limits on the outward flux from the solar circle, unless an avoidance scenario, such as intermittency and/or beaming, allows the present-day local flux to be less than 10(-3) of the average. Difficulties with these avoidance scenarios are noted. KW - cosmic rays KW - galaxies: general KW - gamma-ray burst: general Y1 - 2011 U6 - https://doi.org/10.1088/2041-8205/738/2/L21 SN - 2041-8205 VL - 738 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Aliu, E. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Boettcher, Markus A1 - Bouvier, A. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dickherber, R. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Huan, H. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Madhavan, A. S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pichel, A. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Skole, C. A1 - Smith, A. W. A1 - Staszak, D. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Tyler, J. A1 - Varlotta, A. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. T1 - Veritas observations of unusual extragalactic transient swift J164449.3+573451 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - We report on very high energy (>100 GeV) gamma-ray observations of Swift J164449.3+573451, an unusual transient object first detected by the Swift Observatory and later detected by multiple radio, optical, and X-ray observatories. A total exposure of 28 hr was obtained on Swift J164449.3+573451 with the Very Energetic Radiation Imaging Telescope Array System ( VERITAS) during 2011 March 28-April 15. We do not detect the source and place a differential upper limit on the emission at 500 GeV during these observations of 1.4 x 10(-12) erg cm(-2) s(-1) (99% confidence level). We also present time-resolved upper limits and use a flux limit averaged over the X-ray flaring period to constrain various emission scenarios that can accommodate both the radio-through-X-ray emission detected from the source and the lack of detection by VERITAS. KW - accretion, accretion disks KW - galaxies: active KW - gamma rays: galaxies KW - radiation mechanisms: non-thermal Y1 - 2011 U6 - https://doi.org/10.1088/2041-8205/738/2/L30 SN - 2041-8205 VL - 738 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Kliesch, Martin A1 - Barthel, Thomas A1 - Gogolin, C. A1 - Kastoryano, M. A1 - Eisert, J. T1 - Dissipative quantum church-turing theorem JF - Physical review letters N2 - We show that the time evolution of an open quantum system, described by a possibly time dependent Liouvillian, can be simulated by a unitary quantum circuit of a size scaling polynomially in the simulation time and the size of the system. An immediate consequence is that dissipative quantum computing is no more powerful than the unitary circuit model. Our result can be seen as a dissipative Church-Turing theorem, since it implies that under natural assumptions, such as weak coupling to an environment, the dynamics of an open quantum system can be simulated efficiently on a quantum computer. Formally, we introduce a Trotter decomposition for Liouvillian dynamics and give explicit error bounds. This constitutes a practical tool for numerical simulations, e.g., using matrix-product operators. We also demonstrate that most quantum states cannot be prepared efficiently. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.107.120501 SN - 0031-9007 VL - 107 IS - 12 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Shayduk, Roman A1 - Navirian, Hengameh A1 - Leitenberger, Wolfram A1 - Goldshteyn, Jevgenij A1 - Vrejoiu, Ionela A1 - Weinelt, Martin A1 - Gaal, Peter A1 - Herzog, Marc A1 - von Korff Schmising, Clemens A1 - Bargheer, Matias T1 - Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction JF - New journal of physics : the open-access journal for physics N2 - We report on synchrotron-based high-repetition rate ultrafast x-ray diffraction (UXRD) experiments monitoring the transport of heat from an epitaxial La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice (SL) into the substrate on timescales from 100 ps to 4 mu s. Transient thermal lattice expansion was determined with an accuracy of 10(-7), corresponding to a sensitivity to temperature changes down to 0.01 K. We follow the heat flow within the SL and into the substrate after the impulsive laser heating leads to a small temperature rise of Delta T = 6 K. The transient lattice temperature can be simulated very well using the bulk heat conductivities. This contradicts the interpretation of previous UXRD measurements, which predicted a long-lasting expansion of SrRuO(3) for more than 200 ps. The disagreement could be resolved by assuming that the heat conductivity changes in the first hundred picoseconds. Y1 - 2011 U6 - https://doi.org/10.1088/1367-2630/13/9/093032 SN - 1367-2630 VL - 13 IS - 11 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Lomadze, Nino A1 - Kopyshev, Alexey A1 - Rühe, Jürgen A1 - Santer, Svetlana T1 - Light-Induced chain scission in photosensitive polymer brushes JF - Macromolecules : a publication of the American Chemical Society N2 - We report on a process inducing photomechanical fracture of chemical bonds in photosensitive PMAA polymer brushes. The photosensitive PMAA polymer brushes were prepared by covalent attachment of azobenzene groups to poly(methylacrylic acid) (PMAA) chains generated by surface-initiated polymerization. While homogeneous irradiation leaves the polymer topography unchanged, the azo-PMAA brushes show a strong response upon irradiation with UV interference patterns. The photoisomerization process in the surface-attached polymer films results in the irreversible formation of surface relief gratings (SRG), which are strongly enhanced upon washing with a good solvent for the polymer. The photomechanical forces during mass transport induced by the irradiation lead to the scission of covalent bounds and accordingly to a degrafting of the polymer chains in areas where the polymer is receding from. It is observed that the number of ruptured chains depends strongly on the amount of azo side chains in the polymer. Y1 - 2011 U6 - https://doi.org/10.1021/ma201016q SN - 0024-9297 VL - 44 IS - 18 SP - 7372 EP - 7377 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Sun, Zhuanlan A1 - Zhang, Xiaoqing A1 - Xia, Zhongfu A1 - Qiu, Xunlin A1 - Wirges, Werner A1 - Gerhard, Reimund A1 - Zeng, Changchun A1 - Zhang, Chuck A1 - Wang, Ben T1 - Polarization and piezoelectricity in polymer films with artificial void structure JF - Applied physics : A, Materials science & processing N2 - Laminated polymer-film systems with well-defined void structures were prepared from fluoroethylenepropylene (FEP) and polytetrafluoroethylene (PTFE) layers. First the PTFE films were patterned and then fusion-bonded with the FEP films. The laminates were subjected to either corona or contact charging in order to obtain the desired piezoelectricity. The build-up of the "macro-dipoles" in the laminated films was studied by recording the electric hysteresis loops. The resulting electro-mechanical properties were investigated by means of dielectric resonance spectroscopy (DRS) and direct measurements of the stress-strain relationship. Moreover, the thermal stability of the piezoelectric d (33) coefficient was investigated at elevated temperatures and via thermally stimulated discharge (TSD) current measurements in short circuit. For 150 mu m thick laminated films, consisting of one 25 mu m thick PTFE layer, two 12.5 mu m thick FEP layers, and a void of 100 mu m height, the critical voltage necessary for the build-up of the "macro-dipoles" in the inner voids was approximately 1400 V, which agrees with the value calculated from the Paschen Law. A quasi-static piezoelectric d (33) coefficient up to 300 pC/N was observed after corona charging. The mechanical properties of the film systems are highly anisotropic. At room temperature, the Young's moduli of the laminated film system are around 0.37 MPa in the thickness direction and 274 MPa in the lateral direction, respectively. Using these values, the theoretical shape anisotropy ratio of the void was calculated, which agrees well with experimental observation. Compared with films that do not exhibit structural regularity, the laminates showed improved thermal stability of the d (33) coefficients. The thermal stability of d (33) can be further improved by pre-aging. E.g., the reduction of the d (33) value in the sample pre-aged at 150A degrees C for 5 h was less than 5% after annealing for 30 h at a temperature of 90A degrees C. Y1 - 2011 U6 - https://doi.org/10.1007/s00339-011-6481-2 SN - 0947-8396 VL - 105 IS - 1 SP - 197 EP - 205 PB - Springer CY - New York ER - TY - JOUR A1 - Koseska, Aneta A1 - Volkov, Evgenii A1 - Kurths, Jürgen T1 - Synthetic multicellular oscillatory systems controlling protein dynamics with genetic circuits JF - Physica scripta : an international journal for experimental and theoretical physics N2 - Synthetic biology is a relatively new research discipline that combines standard biology approaches with the constructive nature of engineering. Thus, recent efforts in the field of synthetic biology have given a perspective to consider cells as 'programmable matter'. Here, we address the possibility of using synthetic circuits to control protein dynamics. In particular, we show how intercellular communication and stochasticity can be used to manipulate the dynamical behavior of a population of coupled synthetic units and, in this manner, finely tune the expression of specific proteins of interest, e.g. in large bioreactors. Y1 - 2011 U6 - https://doi.org/10.1088/0031-8949/84/04/045007 SN - 0031-8949 VL - 84 IS - 4 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Baushev, Anton N. T1 - Principal properties of the velocity distribution of dark matter particles on the outskirts of the Solar system JF - Monthly notices of the Royal Astronomical Society N2 - The velocity distribution of the dark matter particles on the outskirts of the Solar system remains unclear. We suggest to determine it using experimentally found properties of the oldest halo objects. Indeed, the oldest halo stars and globular clusters form a collisionless system, as well as dark matter particles do, and they evolved in the same gravitational field. If we accept this analogy, we can show that the velocity distribution of the dark matter particles should be highly anisotropic and have a sharp maximum near upsilon similar to 500 km s(-1). The distribution is totally different from the Maxwell one. We analyse the influence of the distribution function on the results of dark matter detection experiments. It is found that the direct detection signal should differ noticeably from the one calculated from the Maxwell distribution with similar or equal to 220 km s(-1), which is conventional for direct detection experiments (the ratio depends on the detector properties and typically falls within the range between 6 and 0.2). Moreover, the sharp distinction from the Maxwell distribution can be very essential to the observations of dark matter annihilation. KW - elementary particles KW - methods: analytical KW - dark matter Y1 - 2011 U6 - https://doi.org/10.1111/j.1745-3933.2011.01125.x SN - 0035-8711 VL - 417 IS - 1 SP - L83 EP - L87 PB - Wiley-Blackwell CY - Malden ER -