TY  - JOUR
A1  - Liebig, Ferenc
A1  - Sarhan, Radwan Mohamed
A1  - Prietzel, Claudia Christina
A1  - Reinecke, Antje
A1  - Koetz, Joachim
T1  - "Green" gold nanotriangles: synthesis, purification by polyelectrolyte/micelle depletion flocculation and performance in surface-enhanced Raman scattering
JF  - RSC Advances
N2  - The aim of this study was to develop a one-step synthesis of gold nanotriangles (NTs) in the presence of mixed phospholipid vesicles followed by a separation process to isolate purified NTs. Negatively charged vesicles containing AOT and phospholipids, in the absence and presence of additional reducing agents (polyampholytes, polyanions or low molecular weight compounds), were used as a template phase to form anisotropic gold nanoparticles. Upon addition of the gold chloride solution, the nucleation process is initiated and both types of particles, i.e., isotropic spherical and anisotropic gold nanotriangles, are formed simultaneously. As it was not possible to produce monodisperse nanotriangles with such a one-step procedure, the anisotropic nanoparticles needed to be separated from the spherical ones. Therefore, a new type of separation procedure using combined polyelectrolyte/micelle depletion flocculation was successfully applied. As a result of the different purification steps, a green colored aqueous dispersion was obtained containing highly purified, well-defined negatively charged flat nanocrystals with a platelet thickness of 10 nm and an edge length of about 175 nm. The NTs produce promising results in surface-enhanced Raman scattering.
Y1  - 2016
U6  - https://doi.org/10.1039/c6ra04808k
SN  - 2046-2069
VL  - 6
SP  - 33561
EP  - 33568
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Yadavalli, Nataraja Sekhar
A1  - Loebner, Sarah
A1  - Papke, Thomas
A1  - Sava, Elena
A1  - Hurduc, Nicolae
A1  - Santer, Svetlana
T1  - A comparative study of photoinduced deformation in azobenzene containing polymer films
JF  - Soft matter
N2  - In this paper two groups supporting different views on the mechanism of light induced polymer deformation argue about the respective underlying theoretical conceptions, in order to bring this interesting debate to the attention of the scientific community. The group of Prof. Nicolae Hurduc supports the model claiming that the cyclic isomerization of azobenzenes may cause an athermal transition of the glassy azobenzene containing polymer into a fluid state, the so-called photo-fluidization concept. This concept is quite convenient for an intuitive understanding of the deformation process as an anisotropic flow of the polymer material. The group of Prof. Svetlana Santer supports the re-orientational model where the mass-transport of the polymer material accomplished during polymer deformation is stated to be generated by the light-induced re-orientation of the azobenzene side chains and as a consequence of the polymer backbone that in turn results in local mechanical stress, which is enough to irreversibly deform an azobenzene containing material even in the glassy state. For the debate we chose three polymers differing in the glass transition temperature, 32 degrees C, 87 degrees C and 95 degrees C, representing extreme cases of flexible and rigid materials. Polymer film deformation occurring during irradiation with different interference patterns is recorded using a homemade set-up combining an optical part for the generation of interference patterns and an atomic force microscope for acquiring the kinetics of film deformation. We also demonstrated the unique behaviour of azobenzene containing polymeric films to switch the topography in situ and reversibly by changing the irradiation conditions. We discuss the results of reversible deformation of three polymers induced by irradiation with intensity (IIP) and polarization (PIP) interference patterns, and the light of homogeneous intensity in terms of two approaches: the re-orientational and the photo-fluidization concepts. Both agree in that the formation of opto-mechanically induced stresses is a necessary prerequisite for the process of deformation. Using this argument, the deformation process can be characterized either as a flow or mass transport.
Y1  - 2016
U6  - https://doi.org/10.1039/c6sm00029k
SN  - 1744-683X
SN  - 1744-6848
VL  - 12
SP  - 2593
EP  - 2603
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Clusella, Pau
A1  - Politi, Antonio
A1  - Rosenblum, Michael
T1  - A minimal model of self-consistent partial synchrony
JF  - NEW JOURNAL OF PHYSICS
N2  - We show that self-consistent partial synchrony in globally coupled oscillatory ensembles is a general phenomenon. We analyze in detail appearance and stability properties of this state in possibly the simplest setup of a biharmonic Kuramoto-Daido phase model as well as demonstrate the effect in limit-cycle relaxational Rayleigh oscillators. Such a regime extends the notion of splay state from a uniform distribution of phases to an oscillating one. Suitable collective observables such as the Kuramoto order parameter allow detecting the presence of an inhomogeneous distribution. The characteristic and most peculiar property of self-consistent partial synchrony is the difference between the frequency of single units and that of the macroscopic field.
KW  - synchronization
KW  - collective dynamics
KW  - coupled oscillators
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/9/093037
SN  - 1367-2630
VL  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Neher, Dieter
A1  - Kniepert, Juliane
A1  - Elimelech, Arik
A1  - Koster, L. Jan Anton
T1  - A New Figure of Merit for Organic Solar Cells with Transport-limited Photocurrents
JF  - Scientific reports
N2  - Compared to their inorganic counterparts, organic semiconductors suffer from relatively low charge carrier mobilities. Therefore, expressions derived for inorganic solar cells to correlate characteristic performance parameters to material properties are prone to fail when applied to organic devices. This is especially true for the classical Shockley-equation commonly used to describe current-voltage (JV)-curves, as it assumes a high electrical conductivity of the charge transporting material. Here, an analytical expression for the JV-curves of organic solar cells is derived based on a previously published analytical model. This expression, bearing a similar functional dependence as the Shockley-equation, delivers a new figure of merit a to express the balance between free charge recombination and extraction in low mobility photoactive materials. This figure of merit is shown to determine critical device parameters such as the apparent series resistance and the fill factor.
Y1  - 2016
U6  - https://doi.org/10.1038/srep24861
SN  - 2045-2322
VL  - 6
SP  - E2348
EP  - E2349
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Neher, Dieter
A1  - Kniepert, Juliane
A1  - Elimelech, Arik
A1  - Koster, L. Jan Anton
T1  - A New Figure of Merit for Organic Solar Cells with Transport-limited Photocurrents
JF  - Scientific reports
N2  - Compared to their inorganic counterparts, organic semiconductors suffer from relatively low charge carrier mobilities. Therefore, expressions derived for inorganic solar cells to correlate characteristic performance parameters to material properties are prone to fail when applied to organic devices. This is especially true for the classical Shockley-equation commonly used to describe current-voltage (JV)-curves, as it assumes a high electrical conductivity of the charge transporting material. Here, an analytical expression for the JV-curves of organic solar cells is derived based on a previously published analytical model. This expression, bearing a similar functional dependence as the Shockley-equation, delivers a new figure of merit α to express the balance between free charge recombination and extraction in low mobility photoactive materials. This figure of merit is shown to determine critical device parameters such as the apparent series resistance and the fill factor.
KW  - Electronic and spintronic devices
KW  - Semiconductors
Y1  - 2016
U6  - https://doi.org/10.1038/srep24861
SN  - 2045-2322
VL  - 6
PB  - Nature Publishing Group
CY  - London
ER  - 
TY  - JOUR
A1  - Abeysekara, A. U.
A1  - Archambault, S.
A1  - Archer, A.
A1  - Benbow, W.
A1  - Bird, R.
A1  - Buchovecky, M.
A1  - Buckley, J. H.
A1  - Byrum, K.
A1  - Cardenzana, J. V.
A1  - Cerruti, M.
A1  - Chen, Xuhui
A1  - Christiansen, J. L.
A1  - Ciupik, L.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Eisch, J. D.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Fegan, D. J.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Fortin, P.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Gillanders, G. H.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Huetten, M.
A1  - Hakansson, Nils
A1  - Hanna, D.
A1  - Holder, J.
A1  - Humensky, T. B.
A1  - Johnson, C. A.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kelley-Hoskins, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krause, M.
A1  - Krennrich, F.
A1  - Kumar, S.
A1  - Lang, M. J.
A1  - Lin, T. T. Y.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Meagher, K.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Petrashyk, A.
A1  - Pohl, Martin
A1  - Popkow, A.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Ratliff, G.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Santander, M.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Vincent, S.
A1  - Wakely, S. P.
A1  - Weiner, O. M.
A1  - Weinstein, A.
A1  - Williams, D. A.
A1  - Zitzer, B.
T1  - A SEARCH FOR BRIEF OPTICAL FLASHES ASSOCIATED WITH THE SETI TARGET KIC 8462852
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters
N2  - The F-type star KIC. 8462852 has recently been identified as an exceptional target for search for extraterrestrial intelligence (SETI) observations. We describe an analysis methodology for optical SETI, which we have used to analyze nine hours of serendipitous archival observations of KIC. 8462852 made with the VERITAS gamma-ray observatory between 2009 and 2015. No evidence of pulsed optical beacons, above a pulse intensity at the Earth of approximately 1 photon m(-2), is found. We also discuss the potential use of imaging atmospheric Cherenkov telescope arrays in searching for extremely short duration optical transients in general.
KW  - astrobiology
KW  - extraterrestrial intelligence
KW  - methods: observational
KW  - stars: individual ( KIC 8462852)
KW  - techniques: photometric
Y1  - 2016
U6  - https://doi.org/10.3847/2041-8205/818/2/L33
SN  - 2041-8205
SN  - 2041-8213
VL  - 818
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Aliu, E.
A1  - Archambault, S.
A1  - Archer, A.
A1  - Benbow, W.
A1  - Bird, R.
A1  - Biteau, Jonathan
A1  - Buchovecky, M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cardenzana, J. V.
A1  - Cerruti, M.
A1  - Chen, Xuhui
A1  - Ciupik, L.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Eisch, J. D.
A1  - Falcone, A.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Flinders, A.
A1  - Fortin, P.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Gillanders, G. H.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Huetten, M.
A1  - Hakansson, Nils
A1  - Holder, J.
A1  - Humensky, T. B.
A1  - Johnson, C. A.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kelley-Hoskins, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krause, M.
A1  - Lang, M. J.
A1  - Loo, A.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Meagher, K.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nguyen, T.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, A. N.
A1  - Pandel, D.
A1  - Park, N.
A1  - Pelassa, V.
A1  - Petrashyk, A.
A1  - Pohl, M.
A1  - Popkow, A.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Rulten, C.
A1  - Santander, M.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Varlotta, A.
A1  - Vincent, S.
A1  - Wakely, S. P.
A1  - Weiner, O. M.
A1  - Weinstein, A.
A1  - Wilhelm, Alina
A1  - Williams, D. A.
A1  - Zitzer, B.
A1  - Chernyakova, M.
A1  - Roberts, M. S. E.
T1  - A SEARCH FOR VERY HIGH ENERGY GAMMA RAYS FROM THE MISSING LINK BINARY PULSAR J1023+0038 WITH VERITAS
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - The binary millisecond radio pulsar PSR J1023+0038 exhibits many characteristics similar to the gamma-ray binary system PSR B1259-63/LS 2883, making it an ideal candidate for the study of high-energy nonthermal emission. It has been the subject of multiwavelength campaigns following the disappearance of the pulsed radio emission in 2013 June, which revealed the appearance of an accretion disk around the neutron star. We present the results of very high energy (VHE) gamma-ray observations carried out by the Very Energetic Radiation Imaging Telescope Array System before and after this change of state. Searches for steady and pulsed emission of both data sets yield no significant gamma-ray signal above 100 GeV, and upper limits are given for both a steady and pulsed gamma-ray flux. These upper limits are used to constrain the magnetic field strength in the shock region of the PSR J1023+0038 system. Assuming that VHE gamma rays are produced via an inverse Compton mechanism in the shock region, we constrain the shock magnetic field to be greater than similar to 2 G before the disappearance of the radio pulsar and greater than similar to 10 G afterward.
KW  - binaries: general
KW  - gamma rays: general
KW  - pulsars: general
KW  - pulsars: individual (PSR J1023+0038)
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/831/2/193
SN  - 0004-637X
SN  - 1538-4357
VL  - 831
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Levermann, Anders
A1  - Winkelmann, Ricarda
T1  - A simple equation for the melt elevation feedback of ice sheets
JF  - The Cryosphere : TC ; an interactive open access journal of the European Geosciences Union
N2  - In recent decades, the Greenland Ice Sheet has been losing mass and has thereby contributed to global sea-level rise. The rate of ice loss is highly relevant for coastal protection worldwide. The ice loss is likely to increase under future warming. Beyond a critical temperature threshold, a meltdown of the Greenland Ice Sheet is induced by the self-enforcing feedback between its lowering surface elevation and its increasing surface mass loss: the more ice that is lost, the lower the ice surface and the warmer the surface air temperature, which fosters further melting and ice loss. The computation of this rate so far relies on complex numerical models which are the appropriate tools for capturing the complexity of the problem. By contrast we aim here at gaining a conceptual understanding by deriving a purposefully simple equation for the self-enforcing feedback which is then used to estimate the melt time for different levels of warming using three observable characteristics of the ice sheet itself and its surroundings. The analysis is purely conceptual in nature. It is missing important processes like ice dynamics for it to be useful for applications to sea-level rise on centennial timescales, but if the volume loss is dominated by the feedback, the resulting logarithmic equation unifies existing numerical simulations and shows that the melt time depends strongly on the level of warming with a critical slow-down near the threshold: the median time to lose 10% of the present-day ice volume varies between about 3500 years for a temperature level of 0.5 degrees C above the threshold and 500 years for 5 degrees C. Unless future observations show a significantly higher melting sensitivity than currently observed, a complete meltdown is unlikely within the next 2000 years without significant ice-dynamical contributions.
Y1  - 2016
U6  - https://doi.org/10.5194/tc-10-1799-2016
SN  - 1994-0416
SN  - 1994-0424
VL  - 10
SP  - 1799
EP  - 1807
PB  - Copernicus
CY  - Göttingen
ER  - 
TY  - JOUR
A1  - Schwarzl, Maria
A1  - Godec, Aljaz
A1  - Oshanin, Gleb
A1  - Metzler, Ralf
T1  - A single predator charging a herd of prey: effects of self volume and predator-prey decision-making
JF  - Journal of physics : A, Mathematical and theoretical
N2  - We study the degree of success of a single predator hunting a herd of prey on a two-dimensional square lattice landscape. We explicitly consider the self volume of the prey restraining their dynamics on the lattice. The movement of both predator and prey is chosen to include an intelligent, decision making step based on their respective sighting ranges, the radius in which they can detect the other species (prey cannot recognise each other besides the self volume interaction): after spotting each other the motion of prey and predator turns from a nearest neighbour random walk into directed escape or chase, respectively. We consider a large range of prey densities and sighting ranges and compute the mean first passage time for a predator to catch a prey as well as characterise the effective dynamics of the hunted prey. We find that the prey's sighting range dominates their life expectancy and the predator profits more from a bad eyesight of the prey than from his own good eye sight. We characterise the dynamics in terms of the mean distance between the predator and the nearest prey. It turns out that effectively the dynamics of this distance coordinate can be captured in terms of a simple Ornstein–Uhlenbeck picture. Reducing the many-body problem to a simple two-body problem by imagining predator and nearest prey to be connected by an effective Hookean bond, all features of the model such as prey density and sighting ranges merge into the effective binding constant.
KW  - first passage process
KW  - diffusion
KW  - predator-prey model
Y1  - 2016
U6  - https://doi.org/10.1088/1751-8113/49/22/225601
SN  - 1751-8113
SN  - 1751-8121
VL  - 49
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Abramowski, Attila
A1  - Aharonian, Felix A.
A1  - Benkhali, Faical  Ait
A1  - Akhperjanian, A. G.
A1  - Angüner, Ekrem Oǧuzhan
A1  - Backes, Michael
A1  - Balzer, Arnim
A1  - Becherini, Yvonne
A1  - Tjus, J. Becker
A1  - Berge, David
A1  - Bernhard, Sabrina
A1  - Bernlöhr, K.
A1  - Birsin, E.
A1  - Blackwell, R.
A1  - Boettcher, Markus
A1  - Boisson, Catherine
A1  - Bolmont, J.
A1  - Bordas, Pol
A1  - Bregeon, Johan
A1  - Brun, Francois
A1  - Brun, Pierre
A1  - Bryan, Mark
A1  - Bulik, Tomasz
A1  - Carr, John
A1  - Casanova, Sabrina
A1  - Chakraborty, N.
A1  - Chalme-Calvet, R.
A1  - Chaves, Ryan C. G.
A1  - Chen, Andrew
A1  - Chretien, M.
A1  - Colafrancesco, Sergio
A1  - Cologna, Gabriele
A1  - Conrad, Jan
A1  - Couturier, C.
A1  - Cui, Y.
A1  - Davids, I. D.
A1  - Degrange, B.
A1  - Deil, C.
A1  - deWilt, P.
A1  - Djannati-Ata, A.
A1  - Domainko, W.
A1  - Donath, A.
A1  - Dubus, G.
A1  - Dutson, K.
A1  - Dyks, J.
A1  - Dyrda, M.
A1  - Edwards, T.
A1  - Egberts, Kathrin
A1  - Eger, P.
A1  - Ernenwein, J-P.
A1  - Espigat, P.
A1  - Farnier, C.
A1  - Fegan, S.
A1  - Feinstein, F.
A1  - Fernandes, M. V.
A1  - Fernandez, D.
A1  - Fiasson, A.
A1  - Fontaine, G.
A1  - Foerster, A.
A1  - Fuessling, M.
A1  - Gabici, S.
A1  - Gajdus, M.
A1  - Gallant, Y. A.
A1  - Garrigoux, T.
A1  - Giavitto, G.
A1  - Giebels, B.
A1  - Glicenstein, J. F.
A1  - Gottschall, D.
A1  - Goyal, A.
A1  - Grondin, M-H.
A1  - Grudzinska, M.
A1  - Hadasch, D.
A1  - Haeffner, S.
A1  - Hahn, J.
A1  - Hawkes, J.
A1  - Heinzelmann, G.
A1  - Henri, G.
A1  - Hermann, G.
A1  - Hervet, O.
A1  - Hillert, A.
A1  - Hinton, James Anthony
A1  - Hofmann, W.
A1  - Hofverberg, P.
A1  - Hoischen, Clemens
A1  - Holler, M.
A1  - Horns, D.
A1  - Ivascenko, A.
A1  - Jacholkowska, A.
A1  - Jamrozy, M.
A1  - Janiak, M.
A1  - Jankowsky, F.
A1  - Jung-Richardt, I.
A1  - Kastendieck, M. A.
A1  - Katarzynski, K.
A1  - Katz, U.
A1  - Kerszberg, D.
A1  - Khelifi, B.
A1  - Kieffer, M.
A1  - Klepser, S.
A1  - Klochkov, D.
A1  - Kluzniak, W.
A1  - Kolitzus, D.
A1  - Komin, Nu.
A1  - Kosack, K.
A1  - Krakau, S.
A1  - Krayzel, F.
A1  - Krueger, P. P.
A1  - Laffon, H.
A1  - Lamanna, G.
A1  - Lau, J.
A1  - Lefaucheur, J.
A1  - Lefranc, V.
A1  - Lemiere, A.
A1  - Lemoine-Goumard, M.
A1  - Lenain, J-P.
A1  - Lohse, T.
A1  - Lopatin, A.
A1  - Lu, C-C.
A1  - Lui, R.
A1  - Marandon, V.
A1  - Marcowith, Alexandre
A1  - Mariaud, C.
A1  - Marx, R.
A1  - Maurin, G.
A1  - Maxted, N.
A1  - Mayer, M.
A1  - Meintjes, P. J.
A1  - Menzler, U.
A1  - Meyer, M.
A1  - Mitchell, A. M. W.
A1  - Moderski, R.
A1  - Mohamed, M.
A1  - Mora, K.
A1  - Moulin, Emmanuel
A1  - Murach, T.
A1  - de Naurois, M.
A1  - Niemiec, J.
A1  - Oakes, L.
A1  - Odaka, H.
A1  - Oettl, S.
A1  - Ohm, S.
A1  - Opitz, B.
A1  - Ostrowski, M.
A1  - Oya, I.
A1  - Panter, M.
A1  - Parsons, R. D.
A1  - Arribas, M. Paz
A1  - Pekeur, N. W.
A1  - Pelletier, G.
A1  - Petrucci, P-O.
A1  - Peyaud, B.
A1  - Pita, S.
A1  - Poon, H.
A1  - Prokoph, H.
A1  - Puehlhofer, G.
A1  - Punch, M.
A1  - Quirrenbach, A.
A1  - Raab, S.
A1  - Reichardt, I.
A1  - Reimer, A.
A1  - Reimer, O.
A1  - Renaud, M.
A1  - de los Reyes, R.
A1  - Rieger, F.
A1  - Romoli, C.
A1  - Rosier-Lees, S.
A1  - Rowell, G.
A1  - Rudak, B.
A1  - Rulten, C. B.
A1  - Sahakian, V.
A1  - Salek, D.
A1  - Sanchez, David M.
A1  - Santangelo, A.
A1  - Sasaki, M.
A1  - Schlickeiser, R.
A1  - Schuessler, F.
A1  - Schulz, A.
A1  - Schwanke, U.
A1  - Schwemmer, S.
A1  - Seyffert, A. S.
A1  - Simoni, R.
A1  - Sol, H.
A1  - Spanier, F.
A1  - Spengler, G.
A1  - Spies, F.
A1  - Stawarz, L.
A1  - Steenkamp, R.
A1  - Stegmann, Christian
A1  - Stinzing, F.
A1  - Stycz, K.
A1  - Sushch, Iurii
A1  - Tavernet, J-P.
A1  - Tavernier, T.
A1  - Taylor, A. M.
A1  - Terrier, R.
A1  - Tluczykont, M.
A1  - Trichard, C.
A1  - Tuffs, R.
A1  - Valerius, K.
A1  - van der Walt, J.
A1  - van Eldik, C.
A1  - van Soelen, B.
A1  - Vasileiadis, G.
A1  - Veh, J.
A1  - Venter, C.
A1  - Viana, A.
A1  - Vincent, P.
A1  - Vink, J.
A1  - Voisin, F.
A1  - Voelk, H. J.
A1  - Vuillaume, T.
A1  - Wagner, S. J.
A1  - Wagner, P.
A1  - Wagner, R. M.
A1  - Weidinger, M.
A1  - Weitzel, Q.
A1  - White, R.
A1  - Wierzcholska, A.
A1  - Willmann, P.
A1  - Woernlein, A.
A1  - Wouters, D.
A1  - Yang, R.
A1  - Zabalza, V.
A1  - Zaborov, D.
A1  - Zacharias, M.
A1  - Zdziarski, A. A.
A1  - Zech, Alraune
A1  - Zefi, F.
A1  - Zywucka, N.
T1  - Acceleration of petaelectronvolt protons in the Galactic Centre
JF  - Nature : the international weekly journal of science
N2  - Galactic cosmic rays reach energies of at least a few petaelectronvolts (of the order of 1015 electronvolts). This implies that our Galaxy contains petaelectronvolt accelerators (‘PeVatrons’), but all proposed models of Galactic cosmic-ray accelerators encounter difficulties at exactly these energies. Dozens of Galactic accelerators capable of accelerating particles to energies of tens of teraelectronvolts (of the order of 1013 electronvolts) were inferred from recent γ-ray observations3. However, none of the currently known accelerators—not even the handful of shell-type supernova remnants commonly believed to supply most Galactic cosmic rays—has shown the characteristic tracers of petaelectronvolt particles, namely, power-law spectra of γ-rays extending without a cut-off or a spectral break to tens of teraelectronvolts4. Here we report deep γ-ray observations with arcminute angular resolution of the region surrounding the Galactic Centre, which show the expected tracer of the presence of petaelectronvolt protons within the central 10 parsecs of the Galaxy. We propose that the supermassive black hole Sagittarius A* is linked to this PeVatron. Sagittarius A* went through active phases in the past, as demonstrated by X-ray outbursts5and an outflow from the Galactic Centre6. Although its current rate of particle acceleration is not sufficient to provide a substantial contribution to Galactic cosmic rays, Sagittarius A* could have plausibly been more active over the last 106–107 years, and therefore should be considered as a viable alternative to supernova remnants as a source of petaelectronvolt Galactic cosmic rays.
Y1  - 2016
U6  - https://doi.org/10.1038/nature17147
SN  - 0028-0836
SN  - 1476-4687
VL  - 531
SP  - 476
EP  - +
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Godec, Aljaz
A1  - Metzler, Ralf
T1  - Active transport improves the precision of linear long distance molecular signalling
JF  - Journal of physics : A, Mathematical and theoretical
N2  - Molecular signalling in living cells occurs at low copy numbers and is thereby inherently limited by the noise imposed by thermal diffusion. The precision at which biochemical receptors can count signalling molecules is intimately related to the noise correlation time. In addition to passive thermal diffusion, messenger RNA and vesicle-engulfed signalling molecules can transiently bind to molecular motors and are actively transported across biological cells. Active transport is most beneficial when trafficking occurs over large distances, for instance up to the order of 1 metre in neurons. Here we explain how intermittent active transport allows for faster equilibration upon a change in concentration triggered by biochemical stimuli. Moreover, we show how intermittent active excursions induce qualitative changes in the noise in effectively one-dimensional systems such as dendrites. Thereby they allow for significantly improved signalling precision in the sense of a smaller relative deviation in the concentration read-out by the receptor. On the basis of linear response theory we derive the exact mean field precision limit for counting actively transported molecules. We explain how intermittent active excursions disrupt the recurrence in the molecular motion, thereby facilitating improved signalling accuracy. Our results provide a deeper understanding of how recurrence affects molecular signalling precision in biological cells and novel medical-diagnostic devices.
KW  - noise in biochemical signalling
KW  - Brownian motion
KW  - active transport
KW  - linear response theory
KW  - fluctuation-dissipation theorem
KW  - generalised Langevin equation
KW  - recurrence
Y1  - 2016
U6  - https://doi.org/10.1088/1751-8113/49/36/364001
SN  - 1751-8113
SN  - 1751-8121
VL  - 49
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Fischer, Jost Leonhardt
A1  - Bader, Rolf
A1  - Abel, Markus
T1  - Aeroacoustical coupling and synchronization of organ pipes
JF  - The journal of the Acoustical Society of America
N2  - A synchronization experiment on two mutual interacting organ pipes is compared with a theoretical model which takes into account the coupling mechanisms by the underlying first principles of fluid mechanics and aeroacoustics. The focus is on the Arnold-tongue, a mathematical object in the parameter space of detuning and coupling strength which quantitatively captures the interaction of the synchronized sound sources. From the experiment, a nonlinearly shaped Arnold-tongue is obtained, describing the coupling of the synchronized pipe-pipe system. This is in contrast to the linear shaped Arnold-tongue found in a preliminary experiment of the coupled system pipe-loudspeaker. To understand the experimental result, a coarse-grained model of two nonlinear coupled self-sustained oscillators is developed. The model, integrated numerically, is in very good agreement with the synchronization experiment for separation distances of the pipes in the far field and in the intermediate field. The methods introduced open the door for a deeper understanding of the fundamental processes of sound generation and the coupling mechanisms on mutual interacting acoustic oscillators. (C) 2016 Acoustical Society of America.
Y1  - 2016
U6  - https://doi.org/10.1121/1.4964135
SN  - 0001-4966
SN  - 1520-8524
VL  - 140
SP  - 2344
EP  - 2351
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Kruesemann, Henning
A1  - Schwarzl, Richard
A1  - Metzler, Ralf
T1  - Ageing Scher-Montroll Transport
JF  - Transport in Porous Media
N2  - We study the properties of ageing Scher-Montroll transport in terms of a biased subdiffusive continuous time random walk in which the waiting times between consecutive jumps of the charge carriers are distributed according to the power law probability with . As we show, the dynamical properties of the Scher-Montroll transport depend on the ageing time span between the initial preparation of the system and the start of the observation. The Scher-Montroll transport theory was originally shown to describe the photocurrent in amorphous solids in the presence of an external electric field, but it has since been used in many other fields of physical sciences, in particular also in the geophysical context for the description of the transport of tracer particles in subsurface aquifers. In the absence of ageing () the photocurrent of the classical Scher-Montroll model or the breakthrough curves in the groundwater context exhibit a crossover between two power law regimes in time with the scaling exponents and . In the presence of ageing a new power law regime and an initial plateau regime of the current emerge. We derive the different power law regimes and crossover times of the ageing Scher-Montroll transport and show excellent agreement with simulations of the process. Experimental data of ageing Scher-Montroll transport in polymeric semiconductors are shown to agree well with the predictions of our theory.
KW  - Anomalous diffusion
KW  - Ageing
KW  - Scher-Montroll transport
Y1  - 2016
U6  - https://doi.org/10.1007/s11242-016-0686-y
SN  - 0169-3913
SN  - 1573-1634
VL  - 115
SP  - 327
EP  - 344
PB  - Springer
CY  - New York
ER  - 
TY  - JOUR
A1  - Kuik, Friderike
A1  - Lauer, Axel
A1  - Churkina, Galina
A1  - Van der Gon, Hugo A. C. Denier
A1  - Fenner, Daniel
A1  - Mar, Kathleen A.
A1  - Butler, Tim M.
T1  - Air quality modelling in the Berlin-Brandenburg region using WRF-Chem v3.7.1: sensitivity to resolution of model grid and input data
JF  - Geoscientific model development : an interactive open access journal of the European Geosciences Union
N2  - Air pollution is the number one environmental cause of premature deaths in Europe. Despite extensive regulations, air pollution remains a challenge, especially in urban areas. For studying summertime air quality in the Berlin–Brandenburg region of Germany, the Weather Research and Forecasting Model with Chemistry (WRF-Chem) is set up and evaluated against meteorological and air quality observations from monitoring stations as well as from a field campaign conducted in 2014. The objective is to assess which resolution and level of detail in the input data is needed for simulating urban background air pollutant concentrations and their spatial distribution in the Berlin–Brandenburg area. The model setup includes three nested domains with horizontal resolutions of 15, 3 and 1 km and anthropogenic emissions from the TNO-MACC III inventory. We use RADM2 chemistry and the MADE/SORGAM aerosol scheme. Three sensitivity simulations are conducted updating input parameters to the single-layer urban canopy model based on structural data for Berlin, specifying land use classes on a sub-grid scale (mosaic option) and downscaling the original emissions to a resolution of ca. 1 km × 1 km for Berlin based on proxy data including traffic density and population density. The results show that the model simulates meteorology well, though urban 2 m temperature and urban wind speeds are biased high and nighttime mixing layer height is biased low in the base run with the settings described above. We show that the simulation of urban meteorology can be improved when specifying the input parameters to the urban model, and to a lesser extent when using the mosaic option. On average, ozone is simulated reasonably well, but maximum daily 8 h mean concentrations are underestimated, which is consistent with the results from previous modelling studies using the RADM2 chemical mechanism. Particulate matter is underestimated, which is partly due to an underestimation of secondary organic aerosols. NOx (NO + NO2) concentrations are simulated reasonably well on average, but nighttime concentrations are overestimated due to the model's underestimation of the mixing layer height, and urban daytime concentrations are underestimated. The daytime underestimation is improved when using downscaled, and thus locally higher emissions, suggesting that part of this bias is due to deficiencies in the emission input data and their resolution. The results further demonstrate that a horizontal resolution of 3 km improves the results and spatial representativeness of the model compared to a horizontal resolution of 15 km. With the input data (land use classes, emissions) at the level of detail of the base run of this study, we find that a horizontal resolution of 1 km does not improve the results compared to a resolution of 3 km. However, our results suggest that a 1 km horizontal model resolution could enable a detailed simulation of local pollution patterns in the Berlin–Brandenburg region if the urban land use classes, together with the respective input parameters to the urban canopy model, are specified with a higher level of detail and if urban emissions of higher spatial resolution are used.
Y1  - 2016
U6  - https://doi.org/10.5194/gmd-9-4339-2016
SN  - 1991-959X
SN  - 1991-9603
VL  - 9
SP  - 4339
EP  - 4363
PB  - Copernicus
CY  - Göttingen
ER  - 
TY  - JOUR
A1  - Vafin, Sergei
A1  - Schlickeiser, R.
A1  - Yoon, P. H.
T1  - AMPLIFICATION OF COLLECTIVE MAGNETIC FLUCTUATIONS IN MAGNETIZED BI-MAXWELLIAN PLASMAS FOR PARALLEL WAVE VECTORS. I. ELECTRON-PROTON PLASMA
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - The general electromagnetic fluctuation theory is a powerful tool to analyze the magnetic fluctuation spectrum of a plasma. Recent works utilizing this theory for a magnetized non-relativistic isotropic Maxwellian electron-proton plasma have demonstrated that the equilibrium ratio of vertical bar delta B vertical bar/B-0 can be as high as 10(-12). This value results from the balance between spontaneous emission of fluctuations and their damping, and it is considerably smaller than the observed value vertical bar delta B vertical bar/B-0 in the solar wind at 1 au, where 10(-3) less than or similar to vertical bar delta B vertical bar/B-0 less than or similar to 10(-1). In the present manuscript, we consider an anisotropic bi-Maxwellian distribution function to investigate the effect of plasma instabilities on the magnetic field fluctuations. We demonstrate that these instabilities strongly amplify the magnetic field fluctuations and provide a sufficient mechanism to explain the observed value of vertical bar delta B vertical bar/B-0 in the solar wind at 1 au.
KW  - instabilities
KW  - magnetic fields
KW  - solar wind
KW  - turbulence
KW  - waves
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/829/1/41
SN  - 0004-637X
SN  - 1538-4357
VL  - 829
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Aldoretta, E. J.
A1  - St-Louis, N.
A1  - Richardson, N. D.
A1  - Moffat, Anthony F. J.
A1  - Eversberg, T.
A1  - Hill, G. M.
A1  - Shenar, Tomer
A1  - Artigau, E.
A1  - Gauza, B.
A1  - Knapen, J. H.
A1  - Kubat, Jiří
A1  - Kubatova, Brankica
A1  - Maltais-Tariant, R.
A1  - Munoz, M.
A1  - Pablo, H.
A1  - Ramiaramanantsoa, T.
A1  - Richard-Laferriere, A.
A1  - Sablowski, D. P.
A1  - Simon-Diaz, S.
A1  - St-Jean, L.
A1  - Bolduan, F.
A1  - Dias, F. M.
A1  - Dubreuil, P.
A1  - Fuchs, D.
A1  - Garrel, T.
A1  - Grutzeck, G.
A1  - Hunger, T.
A1  - Kuesters, D.
A1  - Langenbrink, M.
A1  - Leadbeater, R.
A1  - Li, D.
A1  - Lopez, A.
A1  - Mauclaire, B.
A1  - Moldenhawer, T.
A1  - Potter, M.
A1  - dos Santos, E. M.
A1  - Schanne, L.
A1  - Schmidt, J.
A1  - Sieske, H.
A1  - Strachan, J.
A1  - Stinner, E.
A1  - Stinner, P.
A1  - Stober, B.
A1  - Strandbaek, K.
A1  - Syder, T.
A1  - Verilhac, D.
A1  - Waldschlaeger, U.
A1  - Weiss, D.
A1  - Wendt, A.
T1  - An extensive spectroscopic time series of three Wolf-Rayet stars - I. The lifetime of large-scale structures in the wind of WR 134
JF  - Monthly notices of the Royal Astronomical Society
N2  - During the summer of 2013, a 4-month spectroscopic campaign took place to observe the variabilities in three Wolf-Rayet stars. The spectroscopic data have been analysed for WR 134 (WN6b), to better understand its behaviour and long-term periodicity, which we interpret as arising from corotating interaction regions (CIRs) in the wind. By analysing the variability of the He ii lambda 5411 emission line, the previously identified period was refined to P = 2.255 +/- 0.008 (s.d.) d. The coherency time of the variability, which we associate with the lifetime of the CIRs in the wind, was deduced to be 40 +/- 6 d, or similar to 18 cycles, by cross-correlating the variability patterns as a function of time. When comparing the phased observational grey-scale difference images with theoretical grey-scales previously calculated from models including CIRs in an optically thin stellar wind, we find that two CIRs were likely present. A separation in longitude of Delta I center dot a parts per thousand integral 90A degrees was determined between the two CIRs and we suggest that the different maximum velocities that they reach indicate that they emerge from different latitudes. We have also been able to detect observational signatures of the CIRs in other spectral lines (C iv lambda lambda 5802,5812 and He i lambda 5876). Furthermore, a DAC was found to be present simultaneously with the CIR signatures detected in the He i lambda 5876 emission line which is consistent with the proposed geometry of the large-scale structures in the wind. Small-scale structures also show a presence in the wind, simultaneously with the larger scale structures, showing that they do in fact co-exist.
KW  - instabilities
KW  - methods: data analysis
KW  - techniques: spectroscopic
KW  - stars: individual: WR 134
KW  - stars: massive
KW  - stars: Wolf-Rayet
Y1  - 2016
U6  - https://doi.org/10.1093/mnras/stw1188
SN  - 0035-8711
SN  - 1365-2966
VL  - 460
SP  - 3407
EP  - 3417
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Richter, Philipp
A1  - Wakker, Bart P.
A1  - Fechner, Cora
A1  - Herenz, Peter
A1  - Tepper-Garcia, T.
A1  - Fox, Andrew J.
T1  - An HST/COS legacy survey of intervening Si III absorption in the extended gaseous halos of low-redshift galaxies
JF  - Climate : open access journal
N2  - Aims. Doubly ionized silicon (Si III) is a powerful tracer of diffuse ionized gas inside and outside of galaxies. It can be observed in the local Universe in ultraviolet (UV) absorption against bright extragalactic background sources. We here present an extensive study of intervening Si III-selected absorbers and study the properties of the warm circumgalactic medium (CGM) around low-redshift (z <= 0.1) galaxies. Methods. We analyzed the UV absorption spectra of 303 extragalactic background sources, as obtained with the Cosmic Origins Spectrograph (COS) on-board the Hubble Space Telescope (HST). We developed a geometrical model for the absorption-cross section of the CGM around the local galaxy population and compared the observed Si III absorption statistics with predictions provided by the model. We also compared redshifts and positions of the absorbers with those of similar to 64 000 galaxies using archival galaxy-survey data to investigate the relation between intervening Si III absorbers and the CGM. Results. Along a total redshift path of Delta z approximate to 24, we identify 69 intervening Si III systems that all show associated absorption from other low and high ions (e.g., H I, Si II, Si IV, C II, C IV). We derive a bias-corrected number density of dN/dz(Si III) = 2.5 +/- 0.4 for absorbers with column densities log N(Si III) > 12.2, which is similar to 3 times the number density of strong Mg II systems at z = 0. This number density matches the expected cross section of a Si III absorbing CGM around the local galaxy population with a mean covering fraction of < f(c)> = 0.69. For the majority (similar to 60 percent) of the absorbers, we identify possible host galaxies within 300 km s(-1) of the absorbers and derive impact parameters rho < 200 kpc, demonstrating that the spatial distributions of Si III absorbers and galaxies are highly correlated. Conclusions. Our study indicates that the majority of Si III-selected absorbers in our sample trace the CGM of nearby galaxies within their virial radii at a typical covering fraction of similar to 70 percent. We estimate that diffuse gas in the CGM around galaxies, as traced by Si III, contains substantially more (more than twice as much) baryonic mass than their neutral interstellar medium.
KW  - galaxies: halos
KW  - galaxies: formation
KW  - intergalactic medium
KW  - quasars: absorption lines
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527038
SN  - 1432-0746
VL  - 590
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Schick, Daniel
A1  - Le Guyader, Loic
A1  - Pontius, Niko
A1  - Radu, Ilie
A1  - Kachel, Torsten
A1  - Mitzner, Rolf
A1  - Zeschke, Thomas
A1  - Schuessler-Langeheine, Christian
A1  - Föhlisch, Alexander
A1  - Holldack, Karsten
T1  - Analysis of the halo background in femtosecond slicing experiments
JF  - Journal of synchrotron radiation
N2  - The slicing facility FemtoSpeX at BESSY II offers unique opportunities to study photo-induced dynamics on femtosecond time scales by means of X-ray magnetic circular dichroism, resonant and non-resonant X-ray diffraction, and X-ray absorption spectroscopy experiments in the soft X-ray regime. Besides femtosecond X-ray pulses, slicing sources inherently also produce a so-called `halo' background with a different time structure, polarization and pointing. Here a detailed experimental characterization of the halo radiation is presented, and a method is demonstrated for its correct and unambiguous removal from femtosecond time-resolved data using a special laser triggering scheme as well as analytical models. Examples are given for time-resolved measurements with corresponding halo correction, and errors of the relevant physical quantities caused by either neglecting or by applying a simplified model to describe this background are estimated.
KW  - femtosecond slicing
KW  - halo
KW  - pump-probe
KW  - XMCD
KW  - X-ray scattering
Y1  - 2016
U6  - https://doi.org/10.1107/S160057751600401X
SN  - 1600-5775
VL  - 23
SP  - 700
EP  - 711
PB  - International Union of Crystallography
CY  - Chester
ER  - 
TY  - JOUR
A1  - Steinke, Martin
A1  - Oskinova, Lida
A1  - Hamann, Wolf-Rainer
A1  - Sander, Andreas Alexander Christoph
A1  - Liermann, A.
A1  - Todt, Helge Tobias
T1  - Analysis of the WN star WR102c, its WR nebula, and the associated cluster of massive stars in the Sickle Nebula
JF  - Tectonophysics : international journal of geotectonics and the geology and physics of the interior of the earth
N2  - Context. The massive Wolf-Rayet type star WR102c is located near the Quintuplet Cluster, one of the three massive star clusters in the Galactic centre region. Previous studies indicated that WR102c may have a dusty circumstellar nebula and is among the main ionising sources of the Sickle Nebula associated with the Quintuplet Cluster. Aims. The goals of our study are to derive the stellar parameters of WR102c from the analysis of its spectrum and to investigate its stellar and nebular environment. Methods. We obtained observations with the ESO VLT integral field spectrograph SINFONI in the K-band, extracted the stellar spectra, and analysed them by means of stellar atmosphere models. Results. Our new analysis supersedes the results previously reported for WR102c. We significantly decrease its bolometric luminosity and hydrogen content. We detect four early OB type stars close to WR102c. These stars have radial velocities similar to that of WR102c. We suggest that together with WR102c these stars belong to a distinct star cluster with a total mass of similar to 1000 M-circle dot. We identify a new WR nebula around WR102c in the SINFONI map of the di ff use Br gamma emission and in the HST Pa ff images. The Br gamma line at di ff erent locations is not significantly broadened and similar to the width of nebular emission elsewhere in the H i i region around WR102c. Conclusions. The massive star WR102c located in the Galactic centre region resides in a star cluster containing additional early-type stars. The stellar parameters of WR102c are typical for hydrogen-free WN6 stars. We identify a nebula surrounding WR102c that has a morphology similar to other nebulae around hydrogen-free WR stars, and propose that the formation of this nebula is linked to interaction of the fast stellar wind with the matter ejected at a previous evolutionary stage of WR102c.
KW  - stars: early-type
KW  - stars: individual: WR 102c
KW  - stars: Wolf
KW  - Rayet
KW  - Galaxy: center
KW  - HII regions
KW  - infrared: stars
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527692
SN  - 1432-0746
VL  - 588
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Cherstvy, Andrey G.
A1  - Metzler, Ralf
T1  - Anomalous diffusion in time-fluctuating non-stationary diffusivity landscapes
JF  - Physical chemistry, chemical physics : PCCP ; a journal of European chemical societies
N2  - We investigate the ensemble and time averaged mean squared displacements for particle diffusion in a simple model for disordered media by assuming that the local diffusivity is both fluctuating in time and has a deterministic average growth or decay in time. In this study we compare computer simulations of the stochastic Langevin equation for this random diffusion process with analytical results. We explore the regimes of normal Brownian motion as well as anomalous diffusion in the sub- and superdiffusive regimes. We also consider effects of the inertial term on the particle motion. The investigation of the resulting diffusion is performed for unconfined and confined motion.
Y1  - 2016
U6  - https://doi.org/10.1039/C6CP03101C
SN  - 1463-9084
SN  - 1463-9076
VL  - 18
SP  - 23840
EP  - 23852
PB  - RSC Publ.
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Cherstvy, Andrey G.
A1  - Metzler, Ralf
T1  - Anomalous diffusion in time-fluctuating non-stationary diffusivity landscapes
JF  - Physical chemistry, chemical physics : a journal of European Chemical Societies
N2  - We investigate the ensemble and time averaged mean squared displacements for particle diffusion in a simple model for disordered media by assuming that the local diffusivity is both fluctuating in time and has a deterministic average growth or decay in time. In this study we compare computer simulations of the stochastic Langevin equation for this random diffusion process with analytical results. We explore the regimes of normal Brownian motion as well as anomalous diffusion in the sub- and superdiffusive regimes. We also consider effects of the inertial term on the particle motion. The investigation of the resulting diffusion is performed for unconfined and confined motion.
Y1  - 2016
U6  - https://doi.org/10.1039/c6cp03101c
SN  - 1463-9076
SN  - 1463-9084
VL  - 18
SP  - 23840
EP  - 23852
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Poeschke, Patrick
A1  - Sokolov, Igor M.
A1  - Nepomnyashchy, Alexander A.
A1  - Zaks, Michael A.
T1  - Anomalous transport in cellular flows: The role of initial conditions and aging
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - We consider the diffusion-advection problem in two simple cellular flow models ( often invoked as examples of subdiffusive tracer motion) and concentrate on the intermediate time range, in which the tracer motion indeed may show subdiffusion. We perform extensive numerical simulations of the systems under different initial conditions and show that the pure intermediate-time subdiffusion regime is only evident when the particles start at the border between different cells, i.e., at the separatrix, and is less pronounced or absent for other initial conditions. The motion moreover shows quite peculiar aging properties, which are also mirrored in the behavior of the time-averaged mean squared displacement for single trajectories. This kind of behavior is due to the complex motion of tracers trapped inside the cell and is absent in classical models based on continuous-time random walks with no dynamics in the trapped state.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevE.94.032128
SN  - 2470-0045
SN  - 2470-0053
VL  - 94
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Ghosh, Surya K.
A1  - Cherstvy, Andrey G.
A1  - Grebenkov, Denis S.
A1  - Metzler, Ralf
T1  - Anomalous, non-Gaussian tracer diffusion in crowded two-dimensional environments
JF  - NEW JOURNAL OF PHYSICS
N2  - A topic of intense current investigation pursues the question of how the highly crowded environment of biological cells affects the dynamic properties of passively diffusing particles. Motivated by recent experiments we report results of extensive simulations of the motion of a finite sized tracer particle in a heterogeneously crowded environment made up of quenched distributions of monodisperse crowders of varying sizes in finite circular two-dimensional domains. For given spatial distributions of monodisperse crowders we demonstrate how anomalous diffusion with strongly non-Gaussian features arises in this model system. We investigate both biologically relevant situations of particles released either at the surface of an inner domain or at the outer boundary, exhibiting distinctly different features of the observed anomalous diffusion for heterogeneous distributions of crowders. Specifically we reveal an asymmetric spreading of tracers even at moderate crowding. In addition to the mean squared displacement (MSD) and local diffusion exponent we investigate the magnitude and the amplitude scatter of the time averaged MSD of individual tracer trajectories, the non-Gaussianity parameter, and the van Hove correlation function. We also quantify how the average tracer diffusivity varies with the position in the domain with a heterogeneous radial distribution of crowders and examine the behaviour of the survival probability and the dynamics of the tracer survival probability. Inter alia, the systems we investigate are related to the passive transport of lipid molecules and proteins in two-dimensional crowded membranes or the motion in colloidal solutions or emulsions in effectively two-dimensional geometries, as well as inside supercrowded, surface adhered cells.
KW  - anomalous diffusion
KW  - crowded fluids
KW  - stochastic processes
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/1/013027
SN  - 1367-2630
VL  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Kunnus, Kristjan
A1  - Josefsson, Ida
A1  - Rajkovic, Ivan
A1  - Schreck, Simon
A1  - Quevedo, Wilson
A1  - Beye, Martin
A1  - Grübel, Sebastian
A1  - Scholz, Mirko
A1  - Nordlund, Dennis
A1  - Zhang, Wenkai
A1  - Hartsock, Robert W.
A1  - Gaffney, Kelly J.
A1  - Schlotter, William F.
A1  - Turner, Joshua J.
A1  - Kennedy, Brian
A1  - Hennies, Franz
A1  - Techert, Simone
A1  - Wernet, Philippe
A1  - Odelius, Michael
A1  - Föhlisch, Alexander
T1  - Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics
JF  - NEW JOURNAL OF PHYSICS
N2  - Ultrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)(5) in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given-which will be covered experimentally by upcoming transform-limited x-ray sources.
KW  - ultrafast photochemistry
KW  - excited state selectivity
KW  - anti-Stokes resonant x-ray raman scattering
KW  - free electron lasers
KW  - resonant inelastic x-ray scattering
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/10/103011
SN  - 1367-2630
VL  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Zhelavskaya, Irina
A1  - Spasojevic, M.
A1  - Shprits, Yuri Y.
A1  - Kurth, William S.
T1  - Automated determination of electron density from electric field measurements on the Van Allen Probes spacecraft
JF  - Journal of geophysical research : Space physics
N2  - We present the Neural-network-based Upper hybrid Resonance Determination (NURD) algorithm for automatic inference of the electron number density from plasma wave measurements made on board NASA's Van Allen Probes mission. A feedforward neural network is developed to determine the upper hybrid resonance frequency, fuhr, from electric field measurements, which is then used to calculate the electron number density. In previous missions, the plasma resonance bands were manually identified, and there have been few attempts to do robust, routine automated detections. We describe the design and implementation of the algorithm and perform an initial analysis of the resulting electron number density distribution obtained by applying NURD to 2.5 years of data collected with the Electric and Magnetic Field Instrument Suite and Integrated Science (EMFISIS) instrumentation suite of the Van Allen Probes mission. Densities obtained by NURD are compared to those obtained by another recently developed automated technique and also to an existing empirical plasmasphere and trough density model.
KW  - Van Allen Probes
KW  - electron number density
KW  - neural networks
Y1  - 2016
U6  - https://doi.org/10.1002/2015JA022132
SN  - 2169-9380
SN  - 2169-9402
VL  - 121
SP  - 4611
EP  - 4625
PB  - American Geophysical Union
CY  - Washington
ER  - 
TY  - JOUR
A1  - Pavlenko, Elena S.
A1  - Sander, Mathias
A1  - Mitzscherling, S.
A1  - Pudell, Jan-Etienne
A1  - Zamponi, Flavio
A1  - Roessle, M.
A1  - Bojahr, Andre
A1  - Bargheer, Matias
T1  - Azobenzene - functionalized polyelectrolyte nanolayers as ultrafast optoacoustic transducers
JF  - Nanoscale
N2  - We introduce azobenzene-functionalized polyelectrolyte multilayers as efficient, inexpensive optoacoustic transducers for hyper-sound strain waves in the GHz range. By picosecond transient reflectivity measurements we study the creation of nanoscale strain waves, their reflection from interfaces, damping by scattering from nanoparticles and propagation in soft and hard adjacent materials like polymer layers, quartz and mica. The amplitude of the generated strain epsilon similar to 5 x 10(-4) is calibrated by ultrafast X-ray diffraction.
Y1  - 2016
U6  - https://doi.org/10.1039/c6nr01448h
SN  - 2040-3364
SN  - 2040-3372
VL  - 8
SP  - 13297
EP  - 13302
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Przybilla, Norbert
A1  - Fossati, Luca
A1  - Hubrig, Swetlana
A1  - Nieva, M. -F.
A1  - Jaervinen, S. P.
A1  - Castro, Norberto
A1  - Schoeller, M.
A1  - Ilyin, Ilya
A1  - Butler, Keith
A1  - Schneider, F. R. N.
A1  - Oskinova, Lida
A1  - Morel, T.
A1  - Langer, N.
A1  - de Koter, A.
T1  - B fields in OB stars (BOB): Detection of a magnetic field in the He-strong star CPD-57 degrees 3509
JF  - Organic letters
N2  - Methods. Spectropolarimetric observations with FORS2 and HARPSpol are analysed using two independent approaches to quantify the magnetic field strength. A high-S/N FLAMES/GIRAFFE spectrum is analysed using a hybrid non-LTE model atmosphere technique. Comparison with stellar evolution models constrains the fundamental parameters of the star. Results. We obtain a firm detection of a surface averaged longitudinal magnetic field with a maximum amplitude of about 1 kG. Assuming a dipolar configuration of the magnetic field, this implies a dipolar field strength larger than 3.3 kG. Moreover, the large amplitude and fast variation (within about 1 day) of the longitudinal magnetic field implies that CPD-57 degrees 3509 is spinning very fast despite its apparently slow projected rotational velocity. The star should be able to support a centrifugal magnetosphere, yet the spectrum shows no sign of magnetically confined material; in particular, emission in H alpha is not observed. Apparently, the wind is either not strong enough for enough material to accumulate in the magnetosphere to become observable or, alternatively, some leakage process leads to loss of material from the magnetosphere. The quantitative spectroscopic analysis of the star yields an effective temperature and a logarithmic surface gravity of 23 750 +/- 250 K and 4.05 +/- 0.10, respectively, and a surface helium fraction of 0.28 +/- 0.02 by number. The surface abundances of C, N, O, Ne, S, and Ar are compatible with the cosmic abundance standard, whereas Mg, Al, Si, and Fe are depleted by about a factor of 2. This abundance pattern can be understood as the consequence of a fractionated stellar wind. CPD-57 degrees 3509 is one of the most evolved He-strong stars known with an independent age constraint due to its cluster membership.
KW  - stars: abundances
KW  - stars: atmospheres
KW  - stars: evolution
KW  - stars: magnetic field
KW  - stars: individual: CPD-57 degrees 3509
KW  - stars: massive
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527646
SN  - 1432-0746
VL  - 587
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Reindl, Nicole
A1  - Rauch, Thomas
A1  - Miller Bertolami, Marcelo Miguel
A1  - Todt, Helge Tobias
A1  - Werner, K.
T1  - Breaking news from the HST
BT  - the central star of the Stingray Nebula is now returning towards the AGB
JF  - Monthly notices of the Royal Astronomical Society
N2  - SAO 244567 is a rare example of a star that allows us to witness stellar evolution in real time. Between 1971 and 1990, it changed from a B-type star into the hot central star of the Stingray Nebula. This observed rapid heating has been a mystery for decades, since it is in strong contradiction with the low mass of the star and canonical post-asymptotic giant branch (AGB) evolution. We speculated that SAO 244567 might have suffered from a late thermal pulse (LTP) and obtained new observations with Hubble Space Telescope (HST)/COS to follow the evolution of the surface properties of SAO 244567 and to verify the LTP hypothesis. Our non-LTE spectral analysis reveals that the star cooled significantly since 2002 and that its envelope is now expanding. Therefore, we conclude that SAO 244567 is currently on its way back towards the AGB, which strongly supports the LTP hypothesis. A comparison with state-of-the-art LTP evolutionary calculations shows that these models cannot fully reproduce the evolution of all surface parameters simultaneously, pointing out possible shortcomings of stellar evolution models. Thereby, SAO 244567 keeps on challenging stellar evolution theory and we highly encourage further investigations.
KW  - stars: AGB and post-AGB
KW  - stars: atmospheres
KW  - stars: evolution
Y1  - 2016
U6  - https://doi.org/10.1093/mnrasl/slw175
SN  - 0035-8711
SN  - 1365-2966
VL  - 464
SP  - L51
EP  - L55
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Baushev, Anton N.
T1  - Can the dark matter annihilation signal be significantly boosted by substructures?
JF  - Journal of cosmology and astroparticle physics
N2  - A very general cosmological consideration suggests that, along with galactic dark matter halos, much smaller dark matter structures may exist. These structures are usually called `clumps', and their mass extends to 10&#8722;6 M &#8857; or even lower. The clumps should give the main contribution into the signal of dark matter annihilation, provided that they have survived until the present time. Recent observations favor a cored profile for low-mass astrophysical halos. We consider cored clumps and show that they are significantly less firm than the standard NFW ones. In contrast to the standard scenario, the cored clumps should have been completely destroyed inside ~ 20 kpc from the Milky Way center. The dwarf spheroidals should not contain any dark matter clumps. On the other hand, even under the most pessimistic assumption about the clump structure, the clumps should have survived in the Milky Way at a distance exceeding 50 kpc from the center, as well as in low-density cosmic structures. There they significantly boost the dark matter annihilation. We show that at least 70% of the clumps endured the primordial structure formation should still exist untouched in the present-day Universe.
KW  - dark matter theory
KW  - particle physics - cosmology connection
KW  - supersymmetry and cosmology
KW  - cosmic ray theory
Y1  - 2016
U6  - https://doi.org/10.1088/1475-7516/2016/01/018
SN  - 1475-7516
VL  - 30
SP  - 12
EP  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Leonhardt, Helmar
A1  - Gerhardt, Matthias
A1  - Hoeppner, Nadine
A1  - Krüger, Kirsten
A1  - Tarantola, Marco
A1  - Beta, Carsten
T1  - Cell-substrate impedance fluctuations of single amoeboid cells encode cell-shape and adhesion dynamics
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - We show systematic electrical impedance measurements of single motile cells on microelectrodes. Wild-type cells and mutant strains were studied that differ in their cell-substrate adhesion strength. We recorded the projected cell area by time-lapse microscopy and observed irregular oscillations of the cell shape. These oscillations were correlated with long-term variations in the impedance signal. Superposed to these long-term trends, we observed fluctuations in the impedance signal. Their magnitude clearly correlated with the adhesion strength, suggesting that strongly adherent cells display more dynamic cell-substrate interactions.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevE.93.012414
SN  - 2470-0045
SN  - 2470-0053
VL  - 93
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Puhlmann, Dirk
A1  - Henkel, Carsten
A1  - Heuer, Axel
A1  - Pieplow, Gregor
A1  - Menzel, Ralf
T1  - Characterization of a remote optical element with bi-photons
JF  - Physica scripta : an international journal for experimental and theoretical physics
N2  - We present a simple setup that exploits the interference of entangled photon pairs. 'Signal' photons are sent through a Mach–Zehnder-like interferometer, while 'idlers' are detected in a variable polarization state. Two-photon interference (in coincidence detection) is observed with very high contrast and for significant time delays between signal and idler detection events. This is explained by quantum erasure of the polarization tag and a delayed choice protocol involving a non-local virtual polarizer. The phase of the two-photon fringes is scanned by varying the path length in the signal beam or by rotating a birefringent crystal in the idler beam. We exploit this to characterize one beam splitter of the signal photon interferometer (reflection and transmission amplitudes including losses), using only information about coincidences and control parameters in the idler path. This is possible because our bi-photon state saturates the Greenberger–Yelin–Englert inequality between contrast and predictability.
KW  - quantum optics
KW  - quantum eraser
KW  - entanglement
KW  - bi-photons
Y1  - 2016
U6  - https://doi.org/10.1088/0031-8949/91/2/023006
SN  - 0031-8949
SN  - 1402-4896
VL  - 91
SP  - 113
EP  - 114
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Sander, Mathias
A1  - Koc, A.
A1  - Kwamen, C. T.
A1  - Michaels, H.
A1  - von Reppert, Alexander
A1  - Pudell, Jan-Etienne
A1  - Zamponi, Flavio
A1  - Bargheer, Matias
A1  - Sellmann, J.
A1  - Schwarzkopf, J.
A1  - Gaal, P.
T1  - Characterization of an ultrafast Bragg-Switch for shortening hard x-ray pulses
JF  - Journal of applied physics
N2  - We present a nanostructured device that functions as photoacoustic hard x-ray switch. The device is triggered by femtosecond laser pulses and allows for temporal gating of hard x-rays on picosecond (ps) timescales. It may be used for pulse picking or even pulse shortening in 3rd generation synchrotron sources. Previous approaches mainly suffered from insufficient switching contrasts due to excitation-induced thermal distortions. We present a new approach where thermal distortions are spatially separated from the functional switching layers in the structure. Our measurements yield a switching contrast of 14, which is sufficient for efficient hard x-ray pulse shortening. The optimized structure also allows for utilizing the switch at high repetition rates of up to 208 kHz. Published by AIP Publishing.
Y1  - 2016
U6  - https://doi.org/10.1063/1.4967835
SN  - 0021-8979
SN  - 1089-7550
VL  - 120
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Paulke, Andreas
A1  - Stranks, Samuel D.
A1  - Kniepert, Juliane
A1  - Kurpiers, Jona
A1  - Wolff, Christian Michael
A1  - Schön, Natalie
A1  - Snaith, Henry J.
A1  - Brenner, Thomas J. K.
A1  - Neher, Dieter
T1  - Charge carrier recombination dynamics in perovskite and polymer solar cells
JF  - Applied physics letters
N2  - Time-delayed collection field experiments are applied to planar organometal halide perovskite (CH3NH3PbI3) based solar cells to investigate charge carrier recombination in a fully working solar cell at the nanosecond to microsecond time scale. Recombination of mobile (extractable) charges is shown to follow second-order recombination dynamics for all fluences and time scales tested. Most importantly, the bimolecular recombination coefficient is found to be time-dependent, with an initial value of ca. 10(-9) cm(3)/s and a progressive reduction within the first tens of nanoseconds. Comparison to the prototypical organic bulk heterojunction device PTB7:PC71BM yields important differences with regard to the mechanism and time scale of free carrier recombination. (C) 2016 AIP Publishing LLC.
Y1  - 2016
U6  - https://doi.org/10.1063/1.4944044
SN  - 0003-6951
SN  - 1077-3118
VL  - 108
SP  - 252
EP  - 262
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Mueller, Lars
A1  - Nanova, Diana
A1  - Glaser, Tobias
A1  - Beck, Sebastian
A1  - Pucci, Annemarie
A1  - Kast, Anne K.
A1  - Schroeder, Rasmus R.
A1  - Mankel, Eric
A1  - Pingel, Patrick
A1  - Neher, Dieter
A1  - Kowalsky, Wolfgang
A1  - Lovrincic, Robert
T1  - Charge-Transfer-Solvent Interaction Predefines Doping Efficiency in p-Doped P3HT Films
JF  - Chemistry of materials : a publication of the American Chemical Society
N2  - Efficient electrical doping of organic semiconductors is a necessary prerequisite for the fabrication of high performance organic electronic devices. In this work, we study p-type doping of poly(3-hexylthiophene) (P3HT) with 2,3,5,6-tetrafluoro-7,7,8,8-tetracyanoquinodimethane (F(4)TCNQ) spin-cast from two different solvents. Using electron diffraction, we find strong dopant-induced pi-pi-stacking for films from the solvent chloroform, but not from chlorobenzene. This image is confirmed and expanded by the analysis of vibrational features of P3HT and polaron absorptions using optical spectroscopy. Here, a red-shifted polaron absorption is found in doped films from chloroform, caused by a higher conjugation length of the polymer backbone. These differences result in a higher conductivity of films from chloroform. We use optical spectroscopy on the corresponding blend solutions to shed light on the origin of this effect and propose a model to explain why solutions of doped P3HT reveal more aggregation of charged molecules in chlorobenzene, whereas more order is finally observed in dried films from chloroform. Our study emphasizes the importance of solvent parameters exceeding the bare solubility of pure dopant and host material for the preparation of highly conductive doped films.
Y1  - 2016
U6  - https://doi.org/10.1021/acs.chemmater.6b01629
SN  - 0897-4756
SN  - 1520-5002
VL  - 28
SP  - 4432
EP  - 4439
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Dzhanoev, Arsen R.
A1  - Schmidt, J.
A1  - Liu, X.
A1  - Spahn, Frank
T1  - Charging of small grains in a space plasma: Application to Jovian stream particles
JF  - International psychogeriatrics
N2  - Context. Most theoretical investigations of dust charging processes in space have treated the current balance condition as independent of grain size. However, for small grains, since they are often observed in space environments, a dependence on grain size is expected owing to secondary electron emission (SEE). Here, by the term "small" we mean a particle size comparable to the typical penetration depth for given primary electron energy. The results are relevant for the dynamics of small, charged dust particles emitted by the volcanic moon Io, which forms the Jovian dust streams. Aims. We revise the theory of charging of small (submicron sized) micrometeoroids to take into account a high production of secondary electrons for small grains immersed in an isotropic flux of electrons. We apply our model to obtain an improved estimate for the charge of the dust streams leaving the Jovian system, detected by several spacecraft. Methods. We apply a continuum model to describe the penetration of primary electrons in a grain and the emission of secondary electrons along the path. Averaging over an isotropic flux of primaries, we derive a new expression for the secondary electron yield, which can be used to express the secondary electron current on a grain. Results. For the Jupiter plasma environment we derive the surface potential of grains composed of NaCl (believed to be the major constituent of Jovian dust stream particles) or silicates. For small particles, the potential depends on grain size and the secondary electron current induces a sensitivity to material properties. As a result of the small particle effect, the estimates for the charging times and for the fractional charge fluctuations of NaCl grains obtained using our general approach to SEE give results qualitatively different from the analogous estimates derived from the traditional approach to SEE. We find that for the charging environment considered in this paper field emission does not limit the charging of NaCl grains.
KW  - plasmas
KW  - planets and satellites: individual: Jupiter
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527891
SN  - 1432-0746
VL  - 591
SP  - 647
EP  - 684
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Beye, Martin
A1  - Öberg, Henrik
A1  - Xin, Hongliang
A1  - Dakovski, Georgi L.
A1  - Föhlisch, Alexander
A1  - Gladh, Jorgen
A1  - Hantschmann, Markus
A1  - Hieke, Florian
A1  - Kaya, Sarp
A1  - Kühn, Danilo
A1  - LaRue, Jerry
A1  - Mercurio, Giuseppe
A1  - Minitti, Michael P.
A1  - Mitra, Ankush
A1  - Moeller, Stefan P.
A1  - Ng, May Ling
A1  - Nilsson, Anders
A1  - Nordlund, Dennis
A1  - Norskov, Jens
A1  - Öström, Henrik
A1  - Ogasawara, Hirohito
A1  - Persson, Mats
A1  - Schlotter, William F.
A1  - Sellberg, Jonas A.
A1  - Wolf, Martin
A1  - Abild-Pedersen, Frank
A1  - Pettersson, Lars G. M.
A1  - Wurth, Wilfried
T1  - Chemical Bond Activation Observed with an X-ray Laser
JF  - The journal of physical chemistry letters
N2  - The concept of bonding and antibonding orbitals is fundamental in chemistry. The population of those orbitals and the energetic difference between the two reflect the strength of the bonding interaction. Weakening the bond is expected to reduce this energetic splitting, but the transient character of bond-activation has so far prohibited direct experimental access. Here we apply time-resolved soft X-ray spectroscopy at a free electron laser to directly observe the decreased bonding antibonding splitting following bond-activation using an ultrashort optical laser pulse.
Y1  - 2016
U6  - https://doi.org/10.1021/acs.jpclett.6b01543
SN  - 1948-7185
VL  - 7
SP  - 3647
EP  - 3651
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Bozzo, Enrico
A1  - Oskinova, Lida
A1  - Feldmeier, Achim
A1  - Falanga, M.
T1  - Clumpy wind accretion in supergiant neutron star high mass X-ray binaries
JF  - BMC neuroscience
N2  - The accretion of the stellar wind material by a compact object represents the main mechanism powering the X-ray emission in classical supergiant high mass X-ray binaries and supergiant fast X-ray transients. In this work we present the first attempt to simulate the accretion process of a fast and dense massive star wind onto a neutron star, taking into account the effects of the centrifugal and magnetic inhibition of accretion ("gating") due to the spin and magnetic field of the compact object. We made use of a radiative hydrodynamical code to model the nonstationary radiatively driven wind of an O-B supergiant star and then place a neutron star characterized by a fixed magnetic field and spin period at a certain distance from the massive companion. Our calculations follow, as a function of time (on a total timescale of several hours), the transitions of the system through all different accretion regimes that are triggered by the intrinsic variations in the density and velocity of the nonstationary wind. The X-ray luminosity released by the system is computed at each time step by taking into account the relevant physical processes occurring in the different accretion regimes. Synthetic lightcurves are derived and qualitatively compared with those observed from classical supergiant high mass X-ray binaries and supergiant fast X-ray transients. Although a number of simplifications are assumed in these calculations, we show that taking into account the effects of the centrifugal and magnetic inhibition of accretion significantly reduces the average X-ray luminosity expected for any neutron star wind-fed binary. The present model calculations suggest that long spin periods and stronger magnetic fields are favored in order to reproduce the peculiar behavior of supergiant fast X-ray transients in the X-ray domain.
KW  - stars: neutron
KW  - X-rays: binaries
KW  - supergiants
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201628341
SN  - 1432-0746
VL  - 589
SP  - 369
EP  - 389
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Schleussner, Carl-Friedrich
A1  - Donges, Jonathan
A1  - Engemann, Denis A.
A1  - Levermann, Anders
T1  - Clustered marginalization of minorities during social transitions induced by co-evolution of behaviour and network structure
JF  - Scientific reports
N2  - Large-scale transitions in societies are associated with both individual behavioural change and restructuring of the social network. These two factors have often been considered independently, yet recent advances in social network research challenge this view. Here we show that common features of societal marginalization and clustering emerge naturally during transitions in a co-evolutionary adaptive network model. This is achieved by explicitly considering the interplay between individual interaction and a dynamic network structure in behavioural selection. We exemplify this mechanism by simulating how smoking behaviour and the network structure get reconfigured by changing social norms. Our results are consistent with empirical findings: The prevalence of smoking was reduced, remaining smokers were preferentially connected among each other and formed increasingly marginalized clusters. We propose that self-amplifying feedbacks between individual behaviour and dynamic restructuring of the network are main drivers of the transition. This generative mechanism for co-evolution of individual behaviour and social network structure may apply to a wide range of examples beyond smoking.
Y1  - 2016
U6  - https://doi.org/10.1038/srep30790
SN  - 2045-2322
VL  - 6
SP  - 3407
EP  - 3417
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Sandev, Trifce
A1  - Iomin, Alexander
A1  - Kantz, Holger
A1  - Metzler, Ralf
A1  - Chechkin, Aleksei V.
T1  - Comb Model with Slow and Ultraslow Diffusion
JF  - Mathematical modelling of natural phenomena
N2  - We consider a generalized diffusion equation in two dimensions for modeling diffusion on a comb-like structures. We analyze the probability distribution functions and we derive the mean squared displacement in x and y directions. Different forms of the memory kernels (Dirac delta, power-law, and distributed order) are considered. It is shown that anomalous diffusion may occur along both x and y directions. Ultraslow diffusion and some more general diffusive processes are observed as well. We give the corresponding continuous time random walk model for the considered two dimensional diffusion-like equation on a comb, and we derive the probability distribution functions which subordinate the process governed by this equation to the Wiener process.
KW  - comb-like model
KW  - anomalous diffusion
KW  - mean squared displacement
KW  - probability density function
Y1  - 2016
U6  - https://doi.org/10.1051/mmnp/201611302
SN  - 0973-5348
SN  - 1760-6101
VL  - 11
SP  - 18
EP  - 33
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Sebek, Michael
A1  - Tönjes, Ralf
A1  - Kiss, Istvan Z.
T1  - Complex Rotating Waves and Long Transients in a Ring Network of Electrochemical Oscillators with Sparse Random Cross-Connections
JF  - Physical review letters
N2  - We perform experiments and phase model simulations with a ring network of oscillatory electrochemical reactions to explore the effect of random connections and nonisochronicity of the interactions on the pattern formation. A few additional links facilitate the emergence of the fully synchronized state. With larger nonisochronicity, complex rotating waves or persistent irregular phase dynamics can derail the convergence to global synchronization. The observed long transients of irregular phase dynamics exemplify the possibility of a sudden onset of hypersynchronous behavior without any external stimulus or network reorganization.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.116.068701
SN  - 0031-9007
SN  - 1079-7114
VL  - 116
SP  - 3001
EP  - 3009
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Clark, Peter U.
A1  - Shakun, Jeremy D.
A1  - Marcott, Shaun A.
A1  - Mix, Alan C.
A1  - Eby, Michael
A1  - Kulp, Scott
A1  - Levermann, Anders
A1  - Milne, Glenn A.
A1  - Pfister, Patrik L.
A1  - Santer, Benjamin D.
A1  - Schrag, Daniel P.
A1  - Solomon, Susan
A1  - Stocker, Thomas F.
A1  - Strauss, Benjamin H.
A1  - Weaver, Andrew J.
A1  - Winkelmann, Ricarda
A1  - Archer, David
A1  - Bard, Edouard
A1  - Goldner, Aaron
A1  - Lambeck, Kurt
A1  - Pierrehumbert, Raymond T.
A1  - Plattner, Gian-Kasper
T1  - Consequences of twenty-first-century policy for multi-millennial climate
and sea-level change
JF  - Nature climate change
N2  - Most of the policy debate surrounding the actions needed to mitigate and adapt to anthropogenic climate change has been framed by observations of the past 150 years as well as climate and sea-level projections for the twenty-first century. The focus on this 250-year window, however, obscures some of the most profound problems associated with climate change. Here, we argue that the twentieth and twenty-first centuries, a period during which the overwhelming majority of human-caused carbon emissions are likely to occur, need to be placed into a long-term context that includes the past 20 millennia, when the last Ice Age ended and human civilization developed, and the next ten millennia, over which time the projected impacts of anthropogenic climate change will grow and persist. This long-term perspective illustrates that policy decisions made in the next few years to decades will have profound impacts on global climate, ecosystems and human societies - not just for this century, but for the next ten millennia and beyond.
Y1  - 2016
U6  - https://doi.org/10.1038/NCLIMATE2923
SN  - 1758-678X
SN  - 1758-6798
VL  - 6
SP  - 360
EP  - 369
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Kronberg, Elena A.
A1  - Rashev, M. V.
A1  - Daly, P. W.
A1  - Shprits, Yuri Y.
A1  - Turner, D. L.
A1  - Drozdov, Alexander
A1  - Dobynde, M.
A1  - Kellerman, Adam C.
A1  - Fritz, T. A.
A1  - Pierrard, V.
A1  - Borremans, K.
A1  - Klecker, B.
A1  - Friedel, R.
T1  - Contamination in electron observations of the silicon detector on board
JF  - Space Weather: The International Journal of Research and Applications
N2  - Since more than 15 years, the Cluster mission passes through Earth's radiation belts at least once every 2 days for several hours, measuring the electron intensity at energies from 30 to 400 keV. These data have previously been considered not usable due to contamination caused by penetrating energetic particles (protons at >100 keV and electrons at >400 keV). In this study, we assess the level of distortion of energetic electron spectra from the Research with Adaptive Particle Imaging Detector (RAPID)/Imaging Electron Spectrometer (IES) detector, determining the efficiency of its shielding. We base our assessment on the analysis of experimental data and a radiation transport code (Geant4). In simulations, we use the incident particle energy distribution of the AE9/AP9 radiation belt models. We identify the Roederer L values, L&#8902;, and energy channels that should be used with caution: at 3&#8804;L&#8902;&#8804;4, all energy channels (40–400 keV) are contaminated by protons (&#8771;230 to 630 keV and >600 MeV); at L&#8902;&#8771;1 and 4–6, the energy channels at 95–400 keV are contaminated by high-energy electrons (>400 keV). Comparison of the data with electron and proton observations from RBSP/MagEIS indicates that the subtraction of proton fluxes at energies &#8771; 230–630 keV from the IES electron data adequately removes the proton contamination. We demonstrate the usefulness of the corrected data for scientific applications.
Y1  - 2016
U6  - https://doi.org/10.1002/2016SW001369
SN  - 1542-7390
VL  - 14
SP  - 449
EP  - 462
PB  - American Geophysical Union
CY  - Washington
ER  - 
TY  - JOUR
A1  - Di Pietro, Riccardo
A1  - Nasrallah, Iyad
A1  - Carpenter, Joshua
A1  - Gann, Eliot
A1  - Kölln, Lisa Sophie
A1  - Thomsen, Lars
A1  - Venkateshvaran, Deepak
A1  - Sadhanala, Aditya
A1  - Chabinyc, Michael
A1  - McNeill, Christopher R.
A1  - Facchetti, Antonio
A1  - Ade, Harald W.
A1  - Sirringhaus, Henning
A1  - Neher, Dieter
T1  - Coulomb Enhanced Charge Transport in Semicrystalline Polymer Semiconductors
JF  - Advanced functional materials
Y1  - 2016
U6  - https://doi.org/10.1002/adfm.201602080
SN  - 1616-301X
SN  - 1616-3028
VL  - 26
SP  - 8011
EP  - 8022
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - de Carvalho, Sidney J.
A1  - Metzler, Ralf
A1  - Cherstvy, Andrey G.
T1  - Critical adsorption of polyelectrolytes onto planar and convex highly charged surfaces
BT  - the nonlinear Poisson–Boltzmann approach
JF  - New journal of physics : the open-access journal for physics
N2  - We study the adsorption–desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the well known scaling relations for the threshold transition—demarcating the adsorbed and desorbed domains of a polyelectrolyte near weakly charged surfaces—are altered for highly charged interfaces. In virtue of high surface potentials and large surface charge densities, the Debye–Hückel approximation is often not feasible and the nonlinear Poisson–Boltzmann approach should be implemented. At low salt conditions, for instance, the electrostatic potential from the nonlinear Poisson–Boltzmann equation is smaller than the Debye–Hückel result, such that the required critical surface charge density for polyelectrolyte adsorption σc increases. The nonlinear relation between the surface charge density and electrostatic potential leads to a sharply increasing critical surface charge density with growing ionic strength, imposing an additional limit to the critical salt concentration above which no polyelectrolyte adsorption occurs at all. We contrast our simulations findings with the known scaling results for weak critical polyelectrolyte adsorption onto oppositely charged surfaces for the three standard geometries. Finally, we discuss some applications of our results for some physical–chemical and biophysical systems.
KW  - polyelectrolyte adsorption
KW  - electrostatic interactions
KW  - critical phenomena
KW  - Debye screening
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/8/083037
SN  - 1367-2630
VL  - 18
PB  - IOP Publ.
CY  - London
ER  - 
TY  - JOUR
A1  - de Carvalho, Sidney J.
A1  - Metzler, Ralf
A1  - Cherstvy, Andrey G.
T1  - Critical adsorption of polyelectrolytes onto planar and convex highly charged surfaces: the nonlinear Poisson-Boltzmann approach
JF  - NEW JOURNAL OF PHYSICS
N2  - We study the adsorption-desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the well known scaling relations for the threshold transition demarcating the adsorbed and desorbed domains of a polyelectrolyte near weakly charged surfaces-are altered for highly charged interfaces. In virtue of high surface potentials and large surface charge densities, the Debye-Huckel approximation is often not feasible and the nonlinear Poisson-Boltzmann approach should be implemented. At low salt conditions, for instance, the electrostatic potential from the nonlinear Poisson-Boltzmann equation is smaller than the Debye-Huckel result, such that the required critical surface charge density for polyelectrolyte adsorption sigma(c) increases. The nonlinear relation between the surface charge density and electrostatic potential leads to a sharply increasing critical surface charge density with growing ionic strength, imposing an additional limit to the critical salt concentration above which no polyelectrolyte adsorption occurs at all. We contrast our simulations findings with the known scaling results for weak critical polyelectrolyte adsorption onto oppositely charged surfaces for the three standard geometries. Finally, we discuss some applications of our results for some physical-chemical and biophysical systems.
KW  - polyelectrolyte adsorption
KW  - electrostatic interactions
KW  - critical phenomena
KW  - Debye screening
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/8/083037
SN  - 1367-2630
VL  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Ganopolski, A.
A1  - Winkelmann, Ricarda
A1  - Schellnhuber, Hans Joachim
T1  - Critical insolation-CO2 relation for diagnosing past and future glacial inception
JF  - Nature : the international weekly journal of science
N2  - The past rapid growth of Northern Hemisphere continental ice sheets, which terminated warm and stable climate periods, is generally attributed to reduced summer insolation in boreal latitudes(1-3). Yet such summer insolation is near to its minimum at present(4), and there are no signs of a new ice age(5). This challenges our understanding of the mechanisms driving glacial cycles and our ability to predict the next glacial inception(6). Here we propose a critical functional relationship between boreal summer insolation and global carbon dioxide (CO2) concentration, which explains the beginning of the past eight glacial cycles and might anticipate future periods of glacial inception. Using an ensemble of simulations generated by an Earth system model of intermediate complexity constrained by palaeoclimatic data, we suggest that glacial inception was narrowly missed before the beginning of the Industrial Revolution. The missed inception can be accounted for by the combined effect of relatively high late-Holocene CO2 concentrations and the low orbital eccentricity of the Earth(7). Additionally, our analysis suggests that even in the absence of human perturbations no substantial build-up of ice sheets would occur within the next several thousand years and that the current interglacial would probably last for another 50,000 years. However, moderate anthropogenic cumulative CO2 emissions of 1,000 to 1,500 gigatonnes of carbon will postpone the next glacial inception by at least 100,000 years(8,9). Our simulations demonstrate that under natural conditions alone the Earth system would be expected to remain in the present delicately balanced interglacial climate state, steering clear of both large-scale glaciation of the Northern Hemisphere and its complete deglaciation, for an unusually long time.
Y1  - 2016
U6  - https://doi.org/10.1038/nature16494
SN  - 0028-0836
SN  - 1476-4687
VL  - 529
SP  - 200
EP  - U159
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Xu, Siyao
A1  - Yan, Huirong
A1  - Lazarian, A.
T1  - DAMPING OF MAGNETOHYDRODYNAMIC TURBULENCE IN PARTIALLY IONIZED PLASMA: IMPLICATIONS FOR COSMIC RAY PROPAGATION
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - We study the damping processes of both incompressible and compressible magnetohydrodynamic (MHD) turbulence in a partially ionized medium. We start from the linear analysis of MHD waves, applying both single-fluid and two-fluid treatments. The damping rates derived from the linear analysis are then used in determining the damping scales of MHD turbulence. The physical connection between the damping scale of MHD turbulence and the cutoff boundary of linear MHD waves is investigated. We find two branches of slow modes propagating in ions and neutrals, respectively, below the damping scale of slow MHD turbulence, and offer a thorough discussion of their propagation and dissipation behavior. Our analytical results are shown to be applicable in a variety of partially ionized interstellar medium (ISM) phases and the solar chromosphere. The importance of neutral viscosity in damping the Alfvenic turbulence in the interstellar warm neutral medium and the solar chromosphere is demonstrated. As a significant astrophysical utility, we introduce damping effects to the propagation of cosmic rays in partially ionized ISM. The important role of turbulence damping in both transit-time damping and gyroresonance is identified.
KW  - cosmic rays
KW  - magnetohydrodynamics (MHD)
KW  - turbulence
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/826/2/166
SN  - 0004-637X
SN  - 1538-4357
VL  - 826
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Frieler, Katja
A1  - Mengel, M.
A1  - Levermann, Anders
T1  - Delaying future sea-level rise by storing water in Antarctica
JF  - Earth system dynamics
N2  - Even if greenhouse gas emissions were stopped today, sea level would continue to rise for centuries, with the long-term sea-level commitment of a 2 degrees C warmer world significantly exceeding 2 m. In view of the potential implications for coastal populations and ecosystems worldwide, we investigate, from an ice-dynamic perspective, the possibility of delaying sea-level rise by pumping ocean water onto the surface of the Antarctic ice sheet. We find that due to wave propagation ice is discharged much faster back into the ocean than would be expected from a pure advection with surface velocities. The delay time depends strongly on the distance from the coastline at which the additional mass is placed and less strongly on the rate of sea-level rise that is mitigated. A millennium-scale storage of at least 80% of the additional ice requires placing it at a distance of at least 700 km from the coastline. The pumping energy required to elevate the potential energy of ocean water to mitigate the currently observed 3 mmyr(-1) will exceed 7% of the current global primary energy supply. At the same time, the approach offers a comprehensive protection for entire coastlines particularly including regions that cannot be protected by dikes.
Y1  - 2016
U6  - https://doi.org/10.5194/esd-7-203-2016
SN  - 2190-4979
SN  - 2190-4987
VL  - 7
SP  - 203
EP  - 210
PB  - Copernicus
CY  - Göttingen
ER  - 
TY  - JOUR
A1  - Steinmetz, Matthias
T1  - Die Vermessung des Universums
JF  - Vision als Aufgabe : das Leibniz-Universum im 21. Jahrhundert
Y1  - 2016
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:b4-opus4-25899
SN  - 978-3-939818-67-0
SP  - 197
EP  - 210
PB  - Berlin-Brandenburgische Akademie der Wissenschaften
CY  - Berlin
ER  - 
TY  - JOUR
A1  - Yang, Jie
A1  - Gühr, Markus
A1  - Vecchione, Theodore
A1  - Robinson, Matthew Scott
A1  - Li, Renkai
A1  - Hartmann, Nick
A1  - Shen, Xiaozhe
A1  - Coffee, Ryan
A1  - Corbett, Jeff
A1  - Fry, Alan
A1  - Gaffney, Kelly
A1  - Gorkhover, Tais
A1  - Hast, Carsten
A1  - Jobe, Keith
A1  - Makasyuk, Igor
A1  - Reid, Alexander
A1  - Robinson, Joseph
A1  - Vetter, Sharon
A1  - Wang, Fenglin
A1  - Weathersby, Stephen
A1  - Yoneda, Charles
A1  - Centurion, Martin
A1  - Wang, Xijie
T1  - Diffractive imaging of a rotational wavepacket in nitrogen molecules
with femtosecond megaelectronvolt electron pulses
JF  - Nature Communications
N2  - Imaging changes in molecular geometries on their natural femtosecond timescale with sub-Angstrom spatial precision is one of the critical challenges in the chemical sciences, as the nuclear geometry changes determine the molecular reactivity. For photoexcited molecules, the nuclear dynamics determine the photoenergy conversion path and efficiency. Here we report a gas-phase electron diffraction experiment using megaelectronvolt (MeV) electrons, where we captured the rotational wavepacket dynamics of nonadiabatically laser-aligned nitrogen molecules. We achieved a combination of 100 fs root-mean-squared temporal resolution and sub-Angstrom (0.76 angstrom) spatial resolution that makes it possible to resolve the position of the nuclei within the molecule. In addition, the diffraction patterns reveal the angular distribution of the molecules, which changes from prolate (aligned) to oblate (anti-aligned) in 300 fs. Our results demonstrate a significant and promising step towards making atomically resolved movies of molecular reactions.
Y1  - 2016
U6  - https://doi.org/10.1038/ncomms11232
SN  - 2041-1723
VL  - 7
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Yang, Jie
A1  - Guehr, Markus
A1  - Shen, Xiaozhe
A1  - Li, Renkai
A1  - Vecchione, Theodore
A1  - Coffee, Ryan
A1  - Corbett, Jeff
A1  - Fry, Alan
A1  - Hartmann, Nick
A1  - Hast, Carsten
A1  - Hegazy, Kareem
A1  - Jobe, Keith
A1  - Makasyuk, Igor
A1  - Robinson, Joseph
A1  - Robinson, Matthew Scott
A1  - Vetter, Sharon
A1  - Weathersby, Stephen
A1  - Yoneda, Charles
A1  - Wang, Xijie
A1  - Centurion, Martin
T1  - Diffractive Imaging of Coherent Nuclear Motion in Isolated Molecules
JF  - Physical review letters
N2  - Observing the motion of the nuclear wave packets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational wave packet in isolated iodine molecules using ultrafast electron diffraction with relativistic electrons. The time-varying interatomic distance was measured with a precision 0.07 angstrom and temporal resolution of 230 fs full width at half maximum. The method is not only sensitive to the position but also the shape of the nuclear wave packet.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.117.153002
SN  - 0031-9007
SN  - 1079-7114
VL  - 117
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Hamaguchi, K.
A1  - Oskinova, Lida
A1  - Russell, C. M. P.
A1  - Petre, R.
A1  - Enoto, T.
A1  - Morihana, K.
A1  - Ishida, M.
T1  - DISCOVERY OF RAPIDLY MOVING PARTIAL X-RAY ABSORBERS WITHIN GAMMA CASSIOPEIAE
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - detected six rapid X-ray spectral hardening events called "softness dips" in a similar to 100 ks observation in 2011. All the softness dip events show symmetric softness-ratio variations, and some of them have flat bottoms apparently due to saturation. The softness dip spectra are best described by either similar to 40% or similar to 70% partial covering absorption to kT similar to 12 keV plasma emission by matter with a neutral hydrogen column density of similar to(2-8) x 10(21) cm(-2), while the spectrum outside these dips is almost free of absorption. This result suggests the presence of two distinct X-ray-emitting spots in the.. Cas system, perhaps on a white dwarf (WD) companion with dipole mass accretion. The partial covering absorbers may be blobs in the Be stellar wind, the Be disk, or rotating around the WD companion. Weak correlations of the softness ratios to the hard X-ray flux suggest the presence of stable plasmas at kT similar to 0.9 and 5 keV, which may originate from the Be or WD winds. The formation of a Be star and WD binary system requires mass transfer between two stars; gamma Cas may have experienced such activity in the past.
KW  - blue stragglers
KW  - stars: emission-line, Be
KW  - stars: individual (gamma Cassiopeiae)
KW  - stars: winds, outflows
KW  - white dwarfs
KW  - X-rays: stars
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/832/2/140
SN  - 0004-637X
SN  - 1538-4357
VL  - 832
SP  - 33
EP  - 49
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Archambault, S.
A1  - Archer, A.
A1  - Barnacka, Anna
A1  - Behera, B.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Berger, K.
A1  - Bird, R.
A1  - Böttcher, Markus
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Cardenzana, J. V.
A1  - Cerruti, M.
A1  - Chen, Xuhui
A1  - Christiansen, J. L.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Dumm, J.
A1  - Eisch, J. D.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Federici, Simone
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Gillanders, G. H.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Griffiths, S. T.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Hakansson, Nils
A1  - Hanna, D.
A1  - Holder, J.
A1  - Hughes, G.
A1  - Johnson, C. A.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kertzman, M.
A1  - Khassen, Y.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Kumar, S.
A1  - Lang, M. J.
A1  - Madhavan, A. S.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Meagher, K.
A1  - Millis, J.
A1  - Moriarty, P.
A1  - Nelson, T.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pohl, Martin
A1  - Popkow, A.
A1  - Prokoph, H.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Rajotte, J.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Sweeney, K.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Varlotta, A.
A1  - Vassiliev, V. V.
A1  - Wakely, S. P.
A1  - Welsing, R.
A1  - Wilhelm, Alina
A1  - Williams, D. A.
A1  - Zitzer, B.
T1  - Discovery of very high energy gamma rays from 1ES 1440+122
JF  - Monthly notices of the Royal Astronomical Society
KW  - BL Lacertae objects: general
KW  - gamma-rays: general
Y1  - 2016
U6  - https://doi.org/10.1093/mnras/stw1319
SN  - 0035-8711
SN  - 1365-2966
VL  - 461
SP  - 202
EP  - 208
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Kurpiers, Jona
A1  - Neher, Dieter
T1  - Dispersive Non-Geminate Recombination in an Amorphous Polymer: Fullerene Blend
JF  - Scientific reports
N2  - Recombination of free charge is a key process limiting the performance of solar cells. For low mobility materials, such as organic semiconductors, the kinetics of non-geminate recombination (NGR) is strongly linked to the motion of charges. As these materials possess significant disorder, thermalization of photogenerated carriers in the inhomogeneously broadened density of state distribution is an unavoidable process. Despite its general importance, knowledge about the kinetics of NGR in complete organic solar cells is rather limited. We employ time delayed collection field (TDCF) experiments to study the recombination of photogenerated charge in the high-performance polymer: fullerene blend PCDTBT:PCBM. NGR in the bulk of this amorphous blend is shown to be highly dispersive, with a continuous reduction of the recombination coefficient throughout the entire time scale, until all charge carriers have either been extracted or recombined. Rapid, contact-mediated recombination is identified as an additional loss channel, which, if not properly taken into account, would erroneously suggest a pronounced field dependence of charge generation. These findings are in stark contrast to the results of TDCF experiments on photovoltaic devices made from ordered blends, such as P3HT:PCBM, where non-dispersive recombination was proven to dominate the charge carrier dynamics under application relevant conditions.
Y1  - 2016
U6  - https://doi.org/10.1038/srep26832
SN  - 2045-2322
VL  - 6
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Kurpiers, Jona
A1  - Neher, Dieter
T1  - Dispersive Non-Geminate Recombination in an Amorphous Polymer:Fullerene Blend
JF  - Scientific reports
N2  - Recombination of free charge is a key process limiting the performance of solar cells. For low mobility materials, such as organic semiconductors, the kinetics of non-geminate recombination (NGR) is strongly linked to the motion of charges. As these materials possess significant disorder, thermalization of photogenerated carriers in the inhomogeneously broadened density of state distribution is an unavoidable process. Despite its general importance, knowledge about the kinetics of NGR in complete organic solar cells is rather limited. We employ time delayed collection field (TDCF) experiments to study the recombination of photogenerated charge in the high-performance polymer:fullerene blend PCDTBT:PCBM. NGR in the bulk of this amorphous blend is shown to be highly dispersive, with a continuous reduction of the recombination coefficient throughout the entire time scale, until all charge carriers have either been extracted or recombined. Rapid, contact-mediated recombination is identified as an additional loss channel, which, if not properly taken into account, would erroneously suggest a pronounced field dependence of charge generation. These findings are in stark contrast to the results of TDCF experiments on photovoltaic devices made from ordered blends, such as P3HT:PCBM, where non-dispersive recombination was proven to dominate the charge carrier dynamics under application relevant conditions.
Y1  - 2016
U6  - https://doi.org/10.1038/srep26832
SN  - 2045-2322
VL  - 6
PB  - Nature Publishing Group
CY  - London
ER  - 
TY  - JOUR
A1  - Lu, Guanghao
A1  - Di Pietro, Riccardo
A1  - Kölln, Lisa Sophie
A1  - Nasrallah, Iyad
A1  - Zhou, Ling
A1  - Mollinger, Sonya
A1  - Himmelberger, Scott
A1  - Koch, Norbert
A1  - Salleo, Alberto
A1  - Neher, Dieter
T1  - Dual-Characteristic Transistors Based on Semiconducting Polymer Blends
JF  - Advanced electronic materials
N2  - A dual-characteristic polymer field-effect transistor has markedly different characteristics in low and high voltage operations. In the low-voltage range (<5 V) it shows sharp subthreshold slopes (0.3–0.4 V dec&#8722;1), using which a low-voltage inverter with gain 8 is realized, while high-voltage (>5 V) induces symmetric current with regard to drain and gate voltages, leading to discrete differential (trans) conductances.
KW  - charge accumulation
KW  - crystalline ordering
KW  - field-effect-transistor
KW  - semiconducting polymers
Y1  - 2016
U6  - https://doi.org/10.1002/aelm.201600267
SN  - 2199-160X
VL  - 2
SP  - 2344
EP  - 2351
PB  - Wiley-Blackwell
CY  - Hoboken
ER  - 
TY  - JOUR
A1  - Guber, Christoph R.
A1  - Richter, Philipp
T1  - Dust depletion of Ca and Ti in QSO absorption-line systems
JF  - Wiley Interdisciplinary Reviews : Water
N2  - Aims. To explore the role of titanium-and calcium-dust depletion in gas in and around galaxies, we systematically study Ti/Ca abundance ratios in intervening absorption-line systems at low and high redshift. Methods. We investigate high-resolution optical spectra obtained by the UVES instrument at the Very Large Telescope (VLT) and spectroscopically analyze 34 absorption-line systems at z <= 0.5 to measure column densities (or limits) for Ca II and Ti II. We complement our UVES data set with previously published absorption-line data on Ti/Ca for redshifts up to z similar to 3.8. Our absorber sample contains 110 absorbers including damped Lyman alpha systems (DLAs), sub-DLAs, and Lyman-Limit systems (LLS). We compare our Ti/Ca findings with results from the MilkyWay and the Magellanic Clouds and discuss the properties of Ti/Ca absorbers in the general context of quasar absorption-line systems. Results. Our analysis indicates that there are two distinct populations of absorbers with either high or low Ti/Ca ratios with a separation at [Ti/Ca] approximate to 1. While the calcium-dust depletion in most of the absorbers appears to be severe, the titanium depletions are mild in systems with high Ti/Ca ratios. The derived trend indicates that absorbers with high Ti/Ca ratios have dust-to-gas ratios that are substantially lower than in the Milky Way. We characterize the overall nature of the absorbers by correlating Ti/Ca with other observables (e.g., metallicity, velocity-component structure) and by modeling the ionization properties of singly-ionized Ca and Ti in different environments. Conclusions. We conclude that Ca II and Ti II bearing absorption-line systems trace predominantly neutral gas in the disks and inner halo regions of galaxies, where the abundance of Ca and Ti reflects the local metal and dust content of the gas. Our study suggests that the Ti/Ca ratio represents a useful measure for the gas-to-dust ratio and overall metallicity in intervening absorption-line systems.
KW  - quasars: absorption lines
KW  - dust, extinction
KW  - galaxies: abundances
KW  - galaxies: ISM
KW  - intergalactic medium
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201628466
SN  - 1432-0746
VL  - 591
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Liu, Xiaodong
A1  - Sachse, Manuel
A1  - Spahn, Frank
A1  - Schmidt, Jurgen
T1  - Dynamics and distribution of Jovian dust ejected from the Galilean satellites
JF  - Journal of geophysical research, Planets
N2  - In this paper, the dynamical analysis of the Jovian dust originating from the four Galilean moons is presented. High-accuracy orbital integrations of dust particles are used to determine their dynamical evolution. A variety of forces are taken into account, including the Lorentz force, solar radiation pressure, Poynting-Robertson drag, solar gravity, the satellites' gravity, plasma drag, and gravitational effects due to nonsphericity of Jupiter. More than 20,000 dust particles from each source moon in the size range from 0.05 &#956;m to 1 cm are simulated over 8000 (Earth) years until each dust grain hits a sink (moons, Jupiter, or escape from the system). Configurations of dust number density in the Jovicentric equatorial inertial frame are calculated and shown. In a Jovicentric frame rotating with the Sun the dust distributions are found to be asymmetric. For certain small particle sizes, the dust population is displaced towards the Sun, while for certain larger sizes, the dust population is displaced away from the Sun. The average lifetime as a function of particle size for ejecta from each source moon is derived, and two sharp jumps in the average lifetime are analyzed. Transport of dust between the Galilean moons and to Jupiter is investigated. Most of the orbits for dust particles from Galilean moons are prograde, while, surprisingly, a small fraction of orbits are found to become retrograde mainly due to solar radiation pressure and Lorentz force. The distribution of orbital elements is also analyzed.
Y1  - 2016
U6  - https://doi.org/10.1002/2016JE004999
SN  - 2169-9097
SN  - 2169-9100
VL  - 121
SP  - 1141
EP  - 1173
PB  - American Geophysical Union
CY  - Washington
ER  - 
TY  - JOUR
A1  - Vlasov, Vladimir
A1  - Rosenblum, Michael
A1  - Pikovskij, Arkadij
T1  - Dynamics of weakly inhomogeneous oscillator populations: perturbation theory on top of Watanabe-Strogatz integrability
JF  - Journal of physics : A, Mathematical and theoretical
N2  - As has been shown by Watanabe and Strogatz (WS) (1993 Phys. Rev. Lett. 70 2391), a population of identical phase oscillators, sine-coupled to a common field, is a partially integrable system: for any ensemble size its dynamics reduce to equations for three collective variables. Here we develop a perturbation approach for weakly nonidentical ensembles. We calculate corrections to the WS dynamics for two types of perturbations: those due to a distribution of natural frequencies and of forcing terms, and those due to small white noise. We demonstrate that in both cases, the complex mean field for which the dynamical equations are written is close to the Kuramoto order parameter, up to the leading order in the perturbation. This supports the validity of the dynamical reduction suggested by Ott and Antonsen (2008 Chaos 18 037113) for weakly inhomogeneous populations.
KW  - Kuramoto model
KW  - oscillator populations
KW  - integrability
KW  - perturbation theory
Y1  - 2016
U6  - https://doi.org/10.1088/1751-8113/49/31/31LT02
SN  - 1751-8113
SN  - 1751-8121
VL  - 49
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Love, John A.
A1  - Chou, Shu-Hua
A1  - Huang, Ye
A1  - Bazan, Guillermo C.
A1  - Thuc-Quyen Nguyen, 
T1  - Effects of solvent additive on "s-shaped" curves in solution-processed small molecule solar cells
JF  - Beilstein journal of organic chemistry
N2  - A novel molecular chromophore, p-SIDT(FBTThCA8)(2), is introduced as an electron-donor material for bulk heterojunction (BHJ) solar cells with broad absorption and near ideal energy levels for the use in combination with common acceptor materials. It is found that films cast from chlorobenzene yield devices with strongly s-shaped current-voltage curves, drastically limiting performance. We find that addition of the common solvent additive diiodooctane, in addition to facilitating crystallization, leads to improved vertical phase separation. This yields much better performing devices, with improved curve shape, demonstrating the importance of morphology control in BHJ devices and improving the understanding of the role of solvent additives.
KW  - current voltage analysis
KW  - morphology
KW  - organic solar cells
Y1  - 2016
U6  - https://doi.org/10.3762/bjoc.12.249
SN  - 1860-5397
VL  - 12
SP  - 2543
EP  - 2555
PB  - Beilstein-Institut zur Förderung der Chemischen Wissenschaften
CY  - Frankfurt, Main
ER  - 
TY  - JOUR
A1  - Ge, J. X.
A1  - He, J. H.
A1  - Yan, Huirong
T1  - Effects of turbulent dust grain motion to interstellar chemistry
JF  - Monthly notices of the Royal Astronomical Society
N2  - Theoretical studies have revealed that dust grains are usually moving fast through the turbulent interstellar gas, which could have significant effects upon interstellar chemistry by modifying grain accretion. This effect is investigated in this work on the basis of numerical gas-grain chemical modelling. Major features of the grain motion effect in the typical environment of dark clouds (DC) can be summarized as follows: (1) decrease of gas-phase (both neutral and ionic) abundances and increase of surface abundances by up to 2-3 orders of magnitude; (2) shifts of the existing chemical jumps to earlier evolution ages for gas-phase species and to later ages for surface species by factors of about 10; (3) a few exceptional cases in which some species turn out to be insensitive to this effect and some other species can show opposite behaviours too. These effects usually begin to emerge from a typical DC model age of about 10(5) yr. The grain motion in a typical cold neutral medium (CNM) can help overcome the Coulomb repulsive barrier to enable effective accretion of cations on to positively charged grains. As a result, the grain motion greatly enhances the abundances of some gas-phase and surface species by factors up to 2-6 or more orders of magnitude in the CNM model. The grain motion effect in a typical molecular cloud (MC) is intermediate between that of the DC and CNM models, but with weaker strength. The grain motion is found to be important to consider in chemical simulations of typical interstellar medium.
KW  - astrochemistry
KW  - turbulence
KW  - ISM: abundances
KW  - ISM: clouds
KW  - dust, extinction
KW  - ISM: molecules
Y1  - 2016
U6  - https://doi.org/10.1093/mnras/stv2560
SN  - 0035-8711
SN  - 1365-2966
VL  - 455
SP  - 3570
EP  - 3587
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Kumph, Muir
A1  - Henkel, Carsten
A1  - Rabl, Peter
A1  - Brownnutt, Michael
A1  - Blatt, Rainer
T1  - Electric-field noise above a thin dielectric layer on metal electrodes
JF  - NEW JOURNAL OF PHYSICS
N2  - The electric-field noise above a layered structure composed of a planar metal electrode covered by a thin dielectric is evaluated and it is found that the dielectric film considerably increases the noise level, in proportion to its thickness. Importantly, even a thin (mono) layer of a low-loss dielectric can enhance the noise level by several orders of magnitude compared to the noise above a bare metal. Close to this layered surface, the power spectral density of the electric field varies with the inverse fourth power of the distance to the surface, rather than with the inverse square, as it would above a bare metal surface. Furthermore, compared to a clean metal, where the noise spectrum does not vary with frequency (in the radio-wave and microwave bands), the dielectric layer can generate electricfield noise which scales in inverse proportion to the frequency. For various realistic scenarios, the noise levels predicted from this model are comparable to those observed in trapped-ion experiments. Thus, these findings are of particular importance for the understanding and mitigation of unwanted heating and decoherence in miniaturized ion traps.
KW  - ion trap
KW  - electric field noise
KW  - fluctuation dissipation
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/2/023020
SN  - 1367-2630
VL  - 18
SP  - 1125
EP  - 1136
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Zehbe, Rolf
A1  - Mochales, Carolina
A1  - Radzik, Daniela
A1  - Mueller, Wolf-Dieter
A1  - Fleck, Claudia
T1  - Electrophoretic deposition of multilayered (cubic and tetragonal stabilized) zirconia ceramics for adapted crack deflection
JF  - Journal of the European Ceramic Society
N2  - The electrophoretic deposition process was used to produce multi-layered ceramics consisting of alternating layers of fully stabilized cubic zirconia and partially stabilized tetragonal zirconia to make use of their different mechanical behaviour, investigating the possibility to deflect advancing cracks at the interfaces of the different layers. This crack deflection is apparently impacted by a toughening mechanism only found in the tetragonal stabilized zirconia polymorph and is characterized by the stress induced transformation of the metastable tetragonal phase into the monoclinic one, which is accompanied by a volume increase resulting in a closing mechanism for advancing cracks. While improving the electrophoretic deposition process, we investigated the transformation toughening mechanism at the layer interfaces and their effect on crack propagation. Investigations involved a combination of different imaging methods, including light microscopy, white light interferometry, atomic force microscopy, scanning electron microscopy, energy dispersive X-ray spectroscopy and Raman spectroscopy. (C) 2015 Elsevier Ltd. All rights reserved.
KW  - Electrophoretic deposition
KW  - Yttria stabilized zirconia
KW  - Transformation toughening
KW  - Multilayer
KW  - Crack deflection
Y1  - 2016
U6  - https://doi.org/10.1016/j.jeurceramsoc.2015.08.022
SN  - 0955-2219
SN  - 1873-619X
VL  - 36
SP  - 357
EP  - 364
PB  - Elsevier
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Romita, Krista
A1  - Lada, Elizabeth
A1  - Cioni, Maria-Rosa L.
T1  - EMBEDDED CLUSTERS IN THE LARGE MAGELLANIC CLOUD USING THE VISTA MAGELLANIC CLOUDS SURVEY
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - We present initial results of the first large-scale survey of embedded star clusters in molecular clouds in the Large Magellanic Cloud (LMC) using near-infrared imaging from the Visible and Infrared Survey Telescope for Astronomy Magellanic Clouds Survey. We explored a ~1.65 deg2 area of the LMC, which contains the well-known star-forming region 30 Doradus as well as ~14% of the galaxy's CO clouds, and identified 67 embedded cluster candidates, 45 of which are newly discovered as clusters. We have determined the sizes, luminosities, and masses for these embedded clusters, examined the star formation rates (SFRs) of their corresponding molecular clouds, and made a comparison between the LMC and the Milky Way. Our preliminary results indicate that embedded clusters in the LMC are generally larger, more luminous, and more massive than those in the local Milky Way. We also find that the surface densities of both embedded clusters and molecular clouds is ~3 times higher than in our local environment, the embedded cluster mass surface density is ~40 times higher, the SFR is ~20 times higher, and the star formation efficiency is ~10 times higher. Despite these differences, the SFRs of the LMC molecular clouds are consistent with the SFR scaling law presented in Lada et al. This consistency indicates that while the conditions of embedded cluster formation may vary between environments, the overall process within molecular clouds may be universal.
KW  - galaxies: star clusters: general
KW  - Magellanic Clouds
KW  - stars: formation
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/821/1/51
SN  - 0004-637X
SN  - 1538-4357
VL  - 821
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Wenz, Leonie
A1  - Levermann, Anders
T1  - Enhanced economic connectivity to foster heat stress-related losses
JF  - Science Advances
N2  - Assessing global impacts of unexpected meteorological events in an increasingly connected world economy is important for estimating the costs of climate change. We show that since the beginning of the 21st century, the structural evolution of the global supply network has been such as to foster an increase of climate-related production losses. We compute first- and higher-order losses from heat stress-induced reductions in productivity under changing economic and climatic conditions between 1991 and 2011. Since 2001, the economic connectivity has augmented in such a way as to facilitate the cascading of production loss. The influence of this structural change has dominated over the effect of the comparably weak climate warming during this decade. Thus, particularly under future warming, the intensification of international trade has the potential to amplify climate losses if no adaptation measures are taken.
Y1  - 2016
U6  - https://doi.org/10.1126/sciadv.1501026
SN  - 2375-2548
VL  - 2
PB  - American Assoc. for the Advancement of Science
CY  - Washington
ER  - 
TY  - JOUR
A1  - Nishikawa, Ken-Ichi
A1  - Frederiksen, J. T.
A1  - Nordlund, A.
A1  - Mizuno, Y.
A1  - Hardee, P. E.
A1  - Niemiec, J.
A1  - Gomez, J. L.
A1  - Dutan, I.
A1  - Meli, A.
A1  - Sol, H.
A1  - Pohl, Martin
A1  - Hartmann, D. H.
T1  - EVOLUTION OF GLOBAL RELATIVISTIC JETS: COLLIMATIONS AND EXPANSION WITH
kKHI AND THE WEIBEL INSTABILITY
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - In the study of relativistic jets one of the key open questions is their interaction with the environment. Here. we study the initial evolution of both electron-proton (e(-) - p(+)) and electron-positron (e(+/-)) relativistic jets, focusing on their lateral interaction with ambient plasma. We follow the evolution of toroidal magnetic fields generated by both the kinetic Kelvin-Helmholtz and Mushroom instabilities. For an e(-) - p(+) jet, the induced magnetic field collimates the jet and electrons are perpendicularly accelerated. As the instabilities saturate and subsequently weaken, the magnetic polarity switches from clockwise to counterclockwise in the middle of the jet. For an e(+/-) jet, we find strong mixing of electrons and positrons with the ambient plasma, resulting in the creation of a bow shock. The merging of current filaments generates density inhomogeneities that. initiate a forward shock. Strong jet-ambient plasma mixing prevents a full development of the jet (on the scale studied), revealing evidence for both jet collimation and particle acceleration in the forming bow shock. Differences in the magnetic field structure generated by e(-) - p(+) and e(+/-) jets may contribute to the polarization properties of the observed emission in AGN jets and gamma-ray bursts.
KW  - acceleration of particles
KW  - plasmas
KW  - radiation mechanisms: non-thermal
KW  - relativistic processes
KW  - stars: jets
KW  - Sun: magnetic fields
Y1  - 2016
U6  - https://doi.org/10.3847/0004-637X/820/2/94
SN  - 0004-637X
SN  - 1538-4357
VL  - 820
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Archambault, S.
A1  - Archer, A.
A1  - Aune, T.
A1  - Barnacka, Anna
A1  - Benbow, W.
A1  - Bird, R.
A1  - Buchovecky, M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cardenzana, J. V.
A1  - Cerruti, M.
A1  - Chen, Xuhui
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Dumm, J.
A1  - Eisch, J. D.
A1  - Falcone, A.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Flinders, A.
A1  - Fortin, P.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Gillanders, G. H.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Huetten, M.
A1  - Hakansson, Nils
A1  - Hanna, D.
A1  - Holder, J.
A1  - Humensky, T. B.
A1  - Johnson, C. A.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kelley-Hoskins, N.
A1  - Kertzman, M.
A1  - Khassen, Y.
A1  - Kieda, D.
A1  - Krause, M.
A1  - Krennrich, F.
A1  - Kumar, S.
A1  - Lang, M. J.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Meagher, K.
A1  - Millis, J.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, A. N.
A1  - Pandel, D.
A1  - Park, N.
A1  - Pelassa, V.
A1  - Pohl, Martin
A1  - Popkow, A.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Rousselle, J.
A1  - Rulten, C.
A1  - Santander, M.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Vincent, S.
A1  - Wakely, S. P.
A1  - Weiner, O. M.
A1  - Weinstein, A.
A1  - Wilhelm, Alina
A1  - Williams, D. A.
A1  - Zitzer, B.
T1  - EXCEPTIONALLY BRIGHT TEV FLARES FROM THE BINARY LS I+61 degrees 303
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters
N2  - The TeV binary system LS I +61 degrees 303 is known for its regular, non-thermal emission pattern that traces the orbital period of the compact object in its 26.5 day orbit around its B0 Ve star companion. The system typically presents elevated TeV emission around apastron passage with flux levels between 5% and 15% of the steady flux from the Crab Nebula (> 300 GeV). In this article, VERITAS observations of LS I + 61 degrees. 303 taken in late 2014 are presented, during which bright TeV flares around apastron at flux levels peaking above 30% of the Crab Nebula flux were detected. This is the brightest such activity from this source ever seen in the TeV regime. The strong outbursts have rise and fall times of less than a day. The short timescale of the flares, in conjunction with the observation of 10 TeV photons from LS I + 61 degrees 303 during the flares, provides constraints on the properties of the accelerator in the source.
KW  - binaries: general
KW  - gamma-rays: general
KW  - stars: individual (LS I+61 degrees 303, VER J0240+612)
KW  - X-rays: binaries
Y1  - 2016
U6  - https://doi.org/10.3847/2041-8205/817/1/L7
SN  - 2041-8205
SN  - 2041-8213
VL  - 817
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Wisotzki, Lutz
A1  - Bacon, Roland
A1  - Blaizot, J.
A1  - Brinchmann, Jarle
A1  - Herenz, Edmund Christian
A1  - Schaye, Joop
A1  - Bouche, Nicolas
A1  - Cantalupo, Sebastiano
A1  - Contini, Thierry
A1  - Carollo, C. M.
A1  - Caruana, Joseph
A1  - Courbot, J. -B.
A1  - Emsellem, E.
A1  - Kamann, S.
A1  - Kerutt, Josephine Victoria
A1  - Leclercq, F.
A1  - Lilly, S. J.
A1  - Patricio, V.
A1  - Sandin, C.
A1  - Steinmetz, Matthias
A1  - Straka, Lorrie A.
A1  - Urrutia, Tanya
A1  - Verhamme, A.
A1  - Weilbacher, Peter Michael
A1  - Wendt, Martin
T1  - Extended Lyman alpha haloes around individual high-redshift galaxies revealed by MUSE
JF  - Science
N2  - We report the detection of extended Ly alpha emission around individual star-forming galaxies at redshifts z = 3-6 in an ultradeep exposure of the Hubble Deep Field South obtained with MUSE on the ESO-VLT. The data reach a limiting surface brightness (1 sigma) of similar to 1 x 10(-19) erg s(-1) cm(-2) arcsec(-2) in azimuthally averaged radial profiles, an order of magnitude improvement over previous narrowband imaging. Our sample consists of 26 spectroscopically confirmed Ly alpha-emitting, but mostly continuum-faint (m(AB) greater than or similar to 27) galaxies. In most objects the Ly alpha emission is considerably more extended than the UV continuum light. While five of the faintest galaxies in the sample show no significantly detected Ly alpha haloes, the derived upper limits suggest that this is due to insufficient S/N. Ly alpha haloes therefore appear to be ubiquitous even for low-mass (similar to 10(8)-10(9) M-circle dot) star-forming galaxies at z > 3. We decompose the Ly alpha emission of each object into a compact component tracing the UV continuum and an extended halo component, and infer sizes and luminosities of the haloes. The extended Ly alpha emission approximately follows an exponential surface brightness distribution with a scale length of a few kpc. While these haloes are thus quite modest in terms of their absolute sizes, they are larger by a factor of 5-15 than the corresponding rest-frame UV continuum sources as seen by HST. They are also much more extended, by a factor similar to 5, than Ly alpha haloes around low-redshift star-forming galaxies. Between similar to 40% and greater than or similar to 90% of the observed Ly alpha flux comes from the extended halo component, with no obvious correlation of this fraction with either the absolute or the relative size of the Ly alpha halo. Our observations provide direct insights into the spatial distribution of at least partly neutral gas residing in the circumgalactic medium of low to intermediate mass galaxies at z > 3.
KW  - galaxies: high-redshift
KW  - galaxies: evolution
KW  - galaxies: formation
KW  - cosmology: observations
KW  - intergalactic medium
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527384
SN  - 1432-0746
VL  - 587
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Intravaia, F.
A1  - Behunin, R. O.
A1  - Henkel, Carsten
A1  - Busch, K.
A1  - Dalvit, D. A. R.
T1  - Failure of Local Thermal Equilibrium in Quantum Friction
JF  - Physical review letters
N2  - Recent progress in manipulating atomic and condensed matter systems has instigated a surge of interest in nonequilibrium physics, including many-body dynamics of trapped ultracold atoms and ions, near-field radiative heat transfer, and quantum friction. Under most circumstances the complexity of such nonequilibrium systems requires a number of approximations to make theoretical descriptions tractable. In particular, it is often assumed that spatially separated components of a system thermalize with their immediate surroundings, although the global state of the system is out of equilibrium. This powerful assumption reduces the complexity of nonequilibrium systems to the local application of well-founded equilibrium concepts. While this technique appears to be consistent for the description of some phenomena, we show that it fails for quantum friction by underestimating by approximately 80% the magnitude of the drag force. Our results show that the correlations among the components of driven, but steady-state, quantum systems invalidate the assumption of local thermal equilibrium, calling for a critical reexamination of this approach for describing the physics of nonequilibrium systems.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.117.100402
SN  - 0031-9007
SN  - 1079-7114
VL  - 117
SP  - 989
EP  - 1010
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Kim, Kyung-Chan
A1  - Shprits, Yuri Y.
A1  - Blake, J. Bernard
T1  - Fast injection of the relativistic electrons into the inner zone and the formation of the split-zone structure during the Bastille Day storm in July 2000
JF  - Journal of geophysical research : Space physics
N2  - During the July 2000 geomagnetic storm, known as the Bastille Day storm, Solar, Anomalous, and Magnetospheric Particle Explorer (SAMPEX)/Heavy Ion Large Telescope (HILT) observed a strong injection of similar to 1MeV electrons into the slot region (L similar to 2.5) during the storm main phase. Then, during the following month, electrons were clearly seen diffusing inward down to L=2 and forming a pronounced split structure encompassing a narrow, newly formed slot region around L=3. SAMPEX observations are first compared with electron and proton observations on HEO-3 and NOAA-15 to validate that the observed unusual dynamics was not caused by proton contamination of the SAMPEX instrument. The time-dependent 3-D Versatile Electron Radiation Belt (VERB) simulation of 1MeV electron flux evolution is compared with the SAMPEX/HILT observations. The results show that the VERB code predicts overall time evolution of the observed split structure. The simulated split structure is produced by pitch angle scattering into the Earth atmosphere of similar to 1MeV electrons by plasmaspheric hiss.
KW  - inner radiation zone and slot region
KW  - Bastille Day geomagnetic storm
KW  - 3-D diffusion simulation
KW  - plasmaspheric hiss
Y1  - 2016
U6  - https://doi.org/10.1002/2015JA022072
SN  - 2169-9380
SN  - 2169-9402
VL  - 121
SP  - 8329
EP  - 8342
PB  - American Geophysical Union
CY  - Washington
ER  - 
TY  - JOUR
A1  - Yang, Jie
A1  - Gühr, Markus
A1  - Vecchione, Theodore
A1  - Robinson, Matthew Scott
A1  - Li, Renkai
A1  - Hartmann, Nick
A1  - Shen, Xiaozhe
A1  - Coffee, Ryan
A1  - Corbett, Jeff
A1  - Fry, Alan
A1  - Gaffney, Kelly
A1  - Gorkhover, Tais
A1  - Hast, Carsten
A1  - Jobe, Keith
A1  - Makasyuk, Igor
A1  - Reid, Alexander
A1  - Robinson, Joseph
A1  - Vetter, Sharon
A1  - Wang, Fenglin
A1  - Weathersby, Stephen
A1  - Yoneda, Charles
A1  - Wang, Xijie
A1  - Centurion, Martin
T1  - Femtosecond gas phase electron diffraction with MeV electrons
JF  - Faraday discussions
N2  - We present results on ultrafast gas electron diffraction (UGED) experiments with femtosecond resolution using the MeV electron gun at SLAC National Accelerator Laboratory. UGED is a promising method to investigate molecular dynamics in the gas phase because electron pulses can probe the structure with a high spatial resolution. Until recently, however, it was not possible for UGED to reach the relevant timescale for the motion of the nuclei during a molecular reaction. Using MeV electron pulses has allowed us to overcome the main challenges in reaching femtosecond resolution, namely delivering short electron pulses on a gas target, overcoming the effect of velocity mismatch between pump laser pulses and the probe electron pulses, and maintaining a low timing jitter. At electron kinetic energies above 3 MeV, the velocity mismatch between laser and electron pulses becomes negligible. The relativistic electrons are also less susceptible to temporal broadening due to the Coulomb force. One of the challenges of diffraction with relativistic electrons is that the small de Broglie wavelength results in very small diffraction angles. In this paper we describe the new setup and its characterization, including capturing static diffraction patterns of molecules in the gas phase, finding time-zero with sub-picosecond accuracy and first time-resolved diffraction experiments. The new device can achieve a temporal resolution of 100 fs root-mean-square, and sub-angstrom spatial resolution. The collimation of the beam is sufficient to measure the diffraction pattern, and the transverse coherence is on the order of 2 nm. Currently, the temporal resolution is limited both by the pulse duration of the electron pulse on target and by the timing jitter, while the spatial resolution is limited by the average electron beam current and the signal-to-noise ratio of the detection system. We also discuss plans for improving both the temporal resolution and the spatial resolution.
Y1  - 2016
U6  - https://doi.org/10.1039/c6fd00071a
SN  - 1359-6640
SN  - 1364-5498
VL  - 194
SP  - 563
EP  - 581
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Godec, Aljaz
A1  - Metzler, Ralf
T1  - First passage time distribution in heterogeneity controlled kinetics: going beyond the mean first passage time
JF  - Scientific reports
N2  - The first passage is a generic concept for quantifying when a random quantity such as the position of a diffusing molecule or the value of a stock crosses a preset threshold (target) for the first time. The last decade saw an enlightening series of new results focusing mostly on the so-called mean and global first passage time (MFPT and GFPT, respectively) of such processes. Here we push the understanding of first passage processes one step further. For a simple heterogeneous system we derive rigorously the complete distribution of first passage times (FPTs). Our results demonstrate that the typical FPT significantly differs from the MFPT, which corresponds to the long time behaviour of the FPT distribution. Conversely, the short time behaviour is shown to correspond to trajectories connecting directly from the initial value to the target. Remarkably, we reveal a previously overlooked third characteristic time scale of the first passage dynamics mirroring brief excursion away from the target.
Y1  - 2016
U6  - https://doi.org/10.1038/srep20349
SN  - 2045-2322
VL  - 6
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Gonzalez Manrique, Sergio Javier
A1  - Kuckein, Christoph
A1  - Pastor Yabar, A.
A1  - Collados Vera, M.
A1  - Denker, Carsten
A1  - Fischer, C. E.
A1  - Gömöry, P.
A1  - Diercke, Andrea
A1  - Gonzalez, N. Bello
A1  - Schlichenmaier, R.
A1  - Balthasar, H.
A1  - Berkefeld, T.
A1  - Feller, A.
A1  - Hoch, S.
A1  - Hofmann, A.
A1  - Kneer, F.
A1  - Lagg, A.
A1  - Nicklas, H.
A1  - Orozco Suarez, D.
A1  - Schmidt, D.
A1  - Schmidt, W.
A1  - Sigwarth, M.
A1  - Sobotka, M.
A1  - Solanki, S. K.
A1  - Soltau, D.
A1  - Staude, J.
A1  - Strassmeier, Klaus G.
A1  - Verma, Meetu
A1  - Volkmer, R.
A1  - von der Lühe, O.
A1  - Waldmann, T.
T1  - Fitting peculiar spectral profiles in He I 10830 angstrom absorption features
JF  - Astronomische Nachrichten = Astronomical notes
N2  - The new generation of solar instruments provides better spectral, spatial, and temporal resolution for a better understanding of the physical processes that take place on the Sun. Multiple-component profiles are more commonly observed with these instruments. Particularly, the He i 10830 triplet presents such peculiar spectral profiles, which give information on the velocity and magnetic fine structure of the upper chromosphere. The purpose of this investigation is to describe a technique to efficiently fit the two blended components of the He i 10830 triplet, which are commonly observed when two atmospheric components are located within the same resolution element. The observations used in this study were taken on 2015 April 17 with the very fast spectroscopic mode of the GREGOR Infrared Spectrograph (GRIS) attached to the 1.5-m GREGOR solar telescope, located at the Observatorio del Teide, Tenerife, Spain. We apply a double-Lorentzian fitting technique using Levenberg-Marquardt least-squares minimization. This technique is very simple and much faster than inversion codes. Line-of-sight Doppler velocities can be inferred for a whole map of pixels within just a few minutes. Our results show sub-and supersonic downflow velocities of up to 32 km s(-1) for the fast component in the vicinity of footpoints of filamentary structures. The slow component presents velocities close to rest. (C) 2016 WILEY-VCH Verlag GmbH& Co. KGaA, Weinheim
KW  - Sun: chromosphere
KW  - methods: data analysis
KW  - techniques: spectroscopic
KW  - line: profiles
Y1  - 2016
U6  - https://doi.org/10.1002/asna.201512433
SN  - 0004-6337
SN  - 1521-3994
VL  - 337
SP  - 1057
EP  - 1063
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Verma, Meetu
A1  - Denker, Carsten
A1  - Böhm, F.
A1  - Balthasar, H.
A1  - Fischer, C. E.
A1  - Kuckein, Christoph
A1  - Gonzalez, N. Bello
A1  - Berkefeld, T.
A1  - Collados Vera, M.
A1  - Diercke, Andrea
A1  - Feller, A.
A1  - Gonzalez Manrique, Sergio Javier
A1  - Hofmann, A.
A1  - Lagg, A.
A1  - Nicklas, H.
A1  - Orozco Suarez, D.
A1  - Pator Yabar, A.
A1  - Rezaei, R.
A1  - Schlichenmaier, R.
A1  - Schmidt, D.
A1  - Schmidt, W.
A1  - Sigwarth, M.
A1  - Sobotka, M.
A1  - Solanki, S. K.
A1  - Soltau, D.
A1  - Staude, J.
A1  - Strassmeier, Klaus G.
A1  - Volkmer, R.
A1  - von der Lühe, O.
A1  - Waldmann, T.
T1  - Flow and magnetic field properties in the trailing sunspots of active region NOAA 12396
JF  - Astronomische Nachrichten = Astronomical notes
N2  - Improved measurements of the photospheric and chromospheric three-dimensional magnetic and flow fields are crucial for a precise determination of the origin and evolution of active regions. We present an illustrative sample of multi-instrument data acquired during a two-week coordinated observing campaign in August 2015 involving, among others, the GREGOR solar telescope (imaging and near-infrared spectroscopy) and the space missions Solar Dynamics Observatory (SDO) and Interface Region Imaging Spectrograph (IRIS). The observations focused on the trailing part of active region NOAA 12396 with complex polarity inversion lines and strong intrusions of opposite polarity flux. The GREGOR Infrared Spectrograph (GRIS) provided Stokes IQUV spectral profiles in the photospheric Si i.1082.7 nm line, the chromospheric He I lambda 1083.0 nm triplet, and the photospheric Ca I lambda 1083.9 nm line. Carefully calibrated GRIS scans of the active region provided maps of Doppler velocity and magnetic field at different atmospheric heights. We compare quick-look maps with those obtained with the " Stokes Inversions based on Response functions" (SIR) code, which furnishes deeper insight into the magnetic properties of the region. We find supporting evidence that newly emerging flux and intruding opposite polarity flux are hampering the formation of penumbrae, i.e., a penumbra fully surrounding a sunspot is only expected after cessation of flux emergence in proximity to the sunspots. (C) 2016 WILEY-VCH Verlag GmbH& Co.KGaA, Weinheim
KW  - Sun: magnetic fields
KW  - sunspots
KW  - methods: data analysis
KW  - techniques: polarimetric
KW  - techniques: spectroscopic
Y1  - 2016
U6  - https://doi.org/10.1002/asna.201612447
SN  - 0004-6337
SN  - 1521-3994
VL  - 337
SP  - 1090
EP  - 1098
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Fang, Lijia
A1  - Holzmueller, Felix
A1  - Matulaitis, Tomas
A1  - Baasner, Anne
A1  - Hauenstein, Christoph
A1  - Benduhn, Johannes
A1  - Schwarze, Martin
A1  - Petrich, Annett
A1  - Piersimoni, Fortunato
A1  - Scholz, Reinhard
A1  - Zeika, Olaf
A1  - Koerner, Christian
A1  - Neher, Dieter
A1  - Vandewal, Koen
A1  - Leo, Karl
T1  - Fluorine-containing low-energy-gap organic dyes with low voltage losses for organic solar cells
JF  - Synthetic metals : the journal of electronic polymers and electronic molecular materials
N2  - Fluorine-containing donor molecules TFTF, CNTF and PRTF are designed and isomer selectively synthesized for application in vacuum-deposited organic solar cells. These molecules comprise a donor acceptor molecular architecture incorporating thiophene and benzothiadiazole derivatives as the electron-donating and electron-withdrawing moieties, respectively. As opposed to previously reported materials from this class, PRTF can be purified by vacuum sublimation at moderate to high yields because of its higher volatility and better stabilization due to a stronger intramolecular hydrogen bond, as compared to TFTF and CNTF. The UV-vis absorption spectra of the three donors show an intense broadband absorption between 500 nm and 800 nm with, similar positions of their frontier energy levels. The photophysical properties of the three donor molecules are thoroughly tested and optimized in bulk heterojunction solar cells with C-60 as acceptor. PRTF shows the best performance, yielding power conversion efficiencies of up to 3.8%. Moreover, the voltage loss for the PRTF device due to the non radiative recombination of free charge carriers is exceptionally low (0.26 V) as compared to typical values for organic solar cells (>0.34V). (C) 2016 Published by Elsevier B.V.
KW  - (Z)-isomer
KW  - Donor materials
KW  - CH center dot center dot center dot F hydrogen bonds
KW  - Sublimation with good yield
KW  - Low voltage losses
Y1  - 2016
U6  - https://doi.org/10.1016/j.synthmet.2016.10.025
SN  - 0379-6779
VL  - 222
SP  - 232
EP  - 239
PB  - Elsevier
CY  - Lausanne
ER  - 
TY  - JOUR
A1  - Hic, Ceren
A1  - Pradhan, Prajal
A1  - Rybski, Diego
A1  - Kropp, Jürgen
T1  - Food Surplus and Its Climate Burdens
JF  - Geological Society of America bulletin
N2  - Avoiding food loss and waste may counteract the increasing food demand and reduce greenhouse gas (GHG) emissions from the agricultural sector. This is crucial because of limited options available to increase food production. In the year 2010, food availability was 20% higher than was required on a global scale. Thus, a more sustainable food production and adjusted consumption would have positive environmental effects. This study provides a systematic approach to estimate consumer level food waste on a country scale and globally, based on food availability and requirements. The food requirement estimation considers demographic development, body weights, and physical activity levels. Surplus between food availability and requirements of a given country is considered as food waste. The global food requirement changed from 2,300 kcal/cap/day to 2,400 kcal/cap/day during the last 50 years, while food surplus grew from 310 kcal/cap/day to 510 kcal/cap/day. Similarly, GHG emissions related to the food surplus increased from 130 Mt CO2eq/yr to 530 Mt CO2eq/yr, an increase of more than 300%. Moreover, the global food surplus may increase up to 850 kcal/cap/day, while the total food requirement will increase only by 2%-20% by 2050. Consequently, GHG emissions associated with the food waste may also increase tremendously to 1.9-2.5 Gt CO2eq/yr.
Y1  - 2016
U6  - https://doi.org/10.1021/acs.est.5b05088
SN  - 0013-936X
SN  - 1520-5851
VL  - 50
SP  - 4269
EP  - 4277
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Parezanovic, Vladimir
A1  - Cordier, Laurent
A1  - Spohn, Andreas
A1  - Duriez, Thomas
A1  - Noack, Bernd R.
A1  - Bonnet, Jean-Paul
A1  - Segond, Marc
A1  - Abel, Markus
A1  - Brunton, Steven L.
T1  - Frequency selection by feedback control in a turbulent shear flow
JF  - Journal of fluid mechanics
N2  - Many previous studies have shown that the turbulent mixing layer under periodic forcing tends to adopt a lock-on state, where the major portion of the fluctuations in the flow are synchronized at the forcing frequency. The goal of this experimental study is to apply closed-loop control in order to provoke the lock-on state, using information from the flow itself. We aim to determine the range of frequencies for which the closed-loop control can establish the lock-on, and what mechanisms are contributing to the selection of a feedback frequency. In order to expand the solution space for optimal closed-loop control laws, we use the genetic programming control (CPC) framework. The best closed-loop control laws obtained by CPC are analysed along with the associated physical mechanisms in the mixing layer flow. The resulting closed-loop control significantly outperforms open-loop forcing in terms of robustness to changes in the free-stream velocities. In addition, the selection of feedback frequencies is not locked to the most amplified local mode, but rather a range of frequencies around it.
KW  - free shear layers
KW  - instability control
KW  - turbulence control
Y1  - 2016
U6  - https://doi.org/10.1017/jfm.2016.261
SN  - 0022-1120
SN  - 1469-7645
VL  - 797
SP  - 247
EP  - 283
PB  - Cambridge Univ. Press
CY  - New York
ER  - 
TY  - JOUR
A1  - Thiem, A.
A1  - Bagheri, M.
A1  - Grosse-Siestrup, C.
A1  - Zehbe, Rolf
T1  - Gelatin-poly(lactic-co-glycolic acid) scaffolds with oriented pore channel architecture - From in vitro to in vivo testing
JF  - Vision research : an international journal for functional aspects of vision.
N2  - A gelatin-poly(lactic-co-glycolic acid), PLGA, composite scaffold, featuring a highly oriented pore channel structure, was developed as a template for articular cartilage regeneration. As a design principle the composite scaffold was optimized to contain only medical grade educts and accordingly no chemical cross linking agents or other toxicological relevant substances or methods were used. Scaffolds were synthesized using a freeze structuring method combined with an electrochemical process followed by freeze-drying. Finally, cross linking was performed using dehydrothermal treatment, which was simultaneously used for sterilization purposes. These composite scaffolds were analyzed in regard to structural and biomechanical properties, and to their degradation behavior. Furthermore, cell culture performance was tested using chondrocytes originated from joint articular cartilage tissue from 6 to 10 months old domestic pigs. Finally, the scaffolds were tested for tissue biocompatibility and their ability for tissue integration in a rat model. The scaffolds showed both excellent functional performance and high biocompatibility in vitro and in vivo. We expect that these gelatin-PLGA scaffolds can effectively support chondrogenesis in vivo demonstrating great potential for the use in cartilage defect treatment. (C) 2016 Elsevier B.V. All rights reserved.
KW  - Gelatin-PLGA Scaffold
KW  - Dehydrothermal cross linking
KW  - Cartilage tissue engineering
KW  - Biomechanics
KW  - Rat model
Y1  - 2016
U6  - https://doi.org/10.1016/j.msec.2016.02.019
SN  - 0928-4931
SN  - 1873-0191
VL  - 62
SP  - 585
EP  - 595
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Kegeles, Alexander
A1  - Oriti, Daniele
T1  - Generalized conservation laws in non-local field theories
JF  - Journal of physics : A, Mathematical and theoretical
N2  - We propose a geometrical treatment of symmetries in non-local field theories, where the non-locality is due to a lack of identification of field arguments in the action. We show that the existence of a symmetry of the action leads to a generalized conservation law, in which the usual conserved current acquires an additional non-local correction term, obtaining a generalization of the standard Noether theorem. We illustrate the general formalism by discussing the specific physical example of complex scalar field theory of the type describing the hydrodynamic approximation of Bose-Einstein condensates. We expect our analysis and results to be of particular interest for the group field theory formulation of quantum gravity.
KW  - conservation laws
KW  - non-local field theory
KW  - Noether theorem
KW  - group field theory
Y1  - 2016
U6  - https://doi.org/10.1088/1751-8113/49/13/135401
SN  - 1751-8113
SN  - 1751-8121
VL  - 49
SP  - 119
EP  - 134
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Mazurek, P.
A1  - Yu, L.
A1  - Gerhard, Reimund
A1  - Wirges, Werner
A1  - Skov, A. L.
T1  - Glycerol as high-permittivity liquid filler in dielectric silicone elastomers
JF  - Journal of applied polymer science
N2  - A recently reported novel class of elastomers was tested with respect to its dielectric properties. The new elastomer material is based on a commercially available poly(dimethylsiloxane) composition, which has been modified by embedding glycerol droplets into its matrix. The approach has two major advantages that make the material useful in a dielectric actuator. First, the glycerol droplets efficiently enhance the dielectric constant, which can reach astonishingly high values in the composite. Second, the liquid filler also acts as a softener that effectively decreases the elastic modulus of the composite. In combination with very low cost and easy preparation, the two property enhancements lead to an extremely attractive dielectric elastomer material. Experimental permittivity data are compared to various theoretical models that predict relative permittivity changes as a function of filler loading, and the applicability of the models is discussed. (c) 2016 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2016, 133, 44153.
KW  - crosslinking
KW  - dielectric properties
KW  - elastomers
KW  - sensors and actuators
Y1  - 2016
U6  - https://doi.org/10.1002/app.44153
SN  - 0021-8995
SN  - 1097-4628
VL  - 133
PB  - Wiley-Blackwell
CY  - Hoboken
ER  - 
TY  - JOUR
A1  - Pavlenko, Elena S.
A1  - Sander, Mathias
A1  - Cui, Q.
A1  - Bargheer, Matias
T1  - Gold Nanorods Sense the Ultrafast Viscoelastic Deformation of Polymers upon Molecular Strain Actuation
JF  - The journal of physical chemistry : C, Nanomaterials and interfaces
N2  - On the basis of the layer-by-layer deposition of polyelectrolytes, we have designed hybrid nanolayer composites for integrated optoacoustic experiments. The femtosecond-laser-excitation of an Azo functionalized film launches nanoscale strain waves at GHz frequencies into a transparent polymer layer. Gold nanorods deposited on the surface sense the arrival of these hyper-sound-waves on the picosecond time scale via a modification of their longitudinal plasmon resonance. We simulated the strain waves using a simple linear masses-and-springs model, which yields good agreement with the observed time scales associated with the nanolayer thicknesses of the constituent materials. From systematic experiments with calibrated strain amplitudes we conclude that reversible viscoelastic deformations of the polyelectrolyte multilayers are triggered by ultrashort pressure transients of about 4 MPa. Our experiments show that strain-mediated interactions in nanoarchitectures composed of molecular photoswitches and plasmonic particles may be used to design new functionalities. The approach combines the highly flexible and cost-effective preparation of polyelectrolyte multilayers with ultrafast molecular strain actuation and plasmonic sensing. Although we use simple flat layered structures for demonstration, this new concept can be used for three-dimensional nanoassemblies with different functionalities. The ultrafast and reversible nature of the response is highly desirable, and the short wavelength associated with the high frequency of the hyper-sound-waves connecting photoactive molecules and nanoparticles inherently gives spectroscopic access to the nanoscale. High-frequency elastic moduli are derived from the ultrafast spectroscopy of the hypersonic response in polyelectrolyte multilayers.
Y1  - 2016
U6  - https://doi.org/10.1021/acs.jpcc.6b06915
SN  - 1932-7447
VL  - 120
SP  - 24957
EP  - 24964
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Rätzel, Dennis
A1  - Wilkens, Martin
A1  - Menzel, Ralf
T1  - Gravitational properties of light
BT  - the gravitational field of a laser pulse
JF  - New journal of physics : the open-access journal for physics
N2  - The gravitational field of a laser pulse of finite lifetime, is investigated in the framework of linearized gravity. Although the effects are very small, they may be of fundamental physical interest. It is shown that the gravitational field of a linearly polarized light pulse is modulated as the norm of the corresponding electric field strength, while no modulations arise for circular polarization. In general, the gravitational field is independent of the polarization direction. It is shown that all physical effects are confined to spherical shells expanding with the speed of light, and that these shells are imprints of the spacetime events representing emission and absorption of the pulse. Nearby test particles at rest are attracted towards the pulse trajectory by the gravitational field due to the emission of the pulse, and they are repelled from the pulse trajectory by the gravitational field due to its absorption. Examples are given for the size of the attractive effect. It is recovered that massless test particles do not experience any physical effect if they are co-propagating with the pulse, and that the acceleration of massless test particles counter-propagating with respect to the pulse is four times stronger than for massive particles
at rest. The similarities between the gravitational effect of a laser pulse and Newtonian gravity in two dimensions are pointed out. The spacetime curvature close to the pulse is compared to that induced by gravitational waves from astronomical sources.
KW  - gravity
KW  - general relativity
KW  - laser pulses
KW  - electromagnetic radiation
KW  - linearized gravity
KW  - pp-wave solutions
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/2/023009
SN  - 1367-2630
VL  - 18
SP  - 1
EP  - 16
PB  - IOP Science
CY  - London
ER  - 
TY  - JOUR
A1  - Rätzel, Dennis
A1  - Wilkens, Martin
A1  - Menzel, Ralf
T1  - Gravitational properties of light-the gravitational field of a laser pulse
JF  - NEW JOURNAL OF PHYSICS
N2  - The gravitational field of a laser pulse of finite lifetime, is investigated in the framework of linearized gravity. Although the effects are very small, they may be of fundamental physical interest. It is shown that the gravitational field of a linearly polarized light pulse is modulated as the norm of the corresponding electric field strength, while no modulations arise for circular polarization. In general, the gravitational field is independent of the polarization direction. It is shown that all physical effects are confined to spherical shells expanding with the speed of light, and that these shells are imprints of the spacetime events representing emission and absorption of the pulse. Nearby test particles at rest are attracted towards the pulse trajectory by the gravitational field due to the emission of the pulse, and they are repelled from the pulse trajectory by the gravitational field due to its absorption. Examples are given for the size of the attractive effect. It is recovered that massless test particles do not experience any physical effect if they are co-propagating with the pulse, and that the acceleration of massless test particles counter-propagating with respect to the pulse is four times stronger than for massive particles at rest. The similarities between the gravitational effect of a laser pulse and Newtonian gravity in two dimensions are pointed out. The spacetime curvature close to the pulse is compared to that induced by gravitational waves from astronomical sources.
KW  - gravity
KW  - general relativity
KW  - laser pulses
KW  - electromagnetic radiation
KW  - linearized gravity
KW  - pp-wave solutions
Y1  - 2016
U6  - https://doi.org/10.1088/1367-2630/18/2/023009
SN  - 1367-2630
VL  - 18
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Schreck, Simon
A1  - Pietzsch, Annette
A1  - Kennedy, Brian
A1  - Sathe, Conny
A1  - Miedema, Piter S.
A1  - Techert, Simone
A1  - Strocov, Vladimir N.
A1  - Schmitt, Thorsten
A1  - Hennies, Franz
A1  - Rubensson, Jan-Erik
A1  - Föhlisch, Alexander
T1  - Ground state potential energy surfaces around selected atoms from resonant inelastic x-ray scattering
JF  - Scientific reports
N2  - Thermally driven chemistry as well as materials’ functionality are determined by the potential energy surface of a systems electronic ground state. This makes the potential energy surface a central and powerful concept in physics, chemistry and materials science. However, direct experimental access to the potential energy surface locally around atomic centers and to its long-range structure are lacking. Here we demonstrate how sub-natural linewidth resonant inelastic soft x-ray scattering at vibrational resolution is utilized to determine ground state potential energy surfaces locally and detect long-range changes of the potentials that are driven by local modifications. We show how the general concept is applicable not only to small isolated molecules such as O2 but also to strongly interacting systems such as the hydrogen bond network in liquid water. The weak perturbation to the potential energy surface through hydrogen bonding is observed as a trend towards softening of the ground state potential around the coordinating atom. The instrumental developments in high resolution resonant inelastic soft x-ray scattering are currently accelerating and will enable broad application of the presented approach. With this multidimensional potential energy surfaces that characterize collective phenomena such as (bio)molecular function or high-temperature superconductivity will become accessible in near future.
Y1  - 2016
U6  - https://doi.org/10.1038/srep20054
SN  - 2045-2322
VL  - 6
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Hassanin, Alshaimaa
A1  - Kliem, Bernhard
A1  - Seehafer, Norbert
T1  - Helical kink instability in the confined solar eruption on 2002 May 27
JF  - Astronomische Nachrichten = Astronomical notes
KW  - instabilities
KW  - magnetohydrodynamics (MHD)
KW  - Sun: corona
KW  - Sun: coronal mass ejections (CMEs)
KW  - Sun: flares
Y1  - 2016
U6  - https://doi.org/10.1002/asna.201612446
SN  - 0004-6337
SN  - 1521-3994
VL  - 337
SP  - 1082
EP  - 1089
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Abdalla, Hassan E.
A1  - Abramowski, Attila
A1  - Aharonian, Felix A.
A1  - Benkhali, Faical  Ait
A1  - Akhperjanian, A. G.
A1  - Andersson, T.
A1  - Angüner, Ekrem Oǧuzhan
A1  - Arrieta, M.
A1  - Aubert, Pierre
A1  - Backes, Michael
A1  - Balzer, Arnim
A1  - Barnard, Michelle
A1  - Becherini, Yvonne
A1  - Tjus, J. Becker
A1  - Berge, David
A1  - Bernhard, Sabrina
A1  - Bernlöhr, K.
A1  - Birsin, E.
A1  - Blackwell, R.
A1  - Boettcher, Markus
A1  - Boisson, Catherine
A1  - Bolmont, J.
A1  - Bordas, Pol
A1  - Bregeon, Johan
A1  - Brun, Francois
A1  - Brun, Pierre
A1  - Bryan, Mark
A1  - Bulik, Tomasz
A1  - Capasso, M.
A1  - Carr, John
A1  - Casanova, Sabrina
A1  - Chakraborty, N.
A1  - Chalme-Calvet, R.
A1  - Chaves, Ryan C. G.
A1  - Chen, Andrew
A1  - Chevalier, J.
A1  - Chretien, M.
A1  - Colafrancesco, Sergio
A1  - Cologna, Gabriele
A1  - Condon, B.
A1  - Conrad, Jan
A1  - Couturier, C.
A1  - Cui, Y.
A1  - Davids, I. D.
A1  - Degrange, B.
A1  - Deil, C.
A1  - Devin, J.
A1  - de Wilt, P.
A1  - Djannati-Ataie, A.
A1  - Domainko, W.
A1  - Donath, A.
A1  - Dubus, G.
A1  - Dutson, K.
A1  - Dyks, J.
A1  - Dyrda, M.
A1  - Edwards, T.
A1  - Egberts, Kathrin
A1  - Eger, P.
A1  - Ernenwein, J. -P.
A1  - Eschbach, S.
A1  - Farnier, C.
A1  - Fegan, S.
A1  - Fernandes, M. V.
A1  - Fiasson, A.
A1  - Fontaine, G.
A1  - Foerster, A.
A1  - Funk, S.
A1  - Fuessling, M.
A1  - Gabici, S.
A1  - Gajdus, M.
A1  - Gallant, Y. A.
A1  - Garrigoux, T.
A1  - Giavitto, G.
A1  - Giebels, B.
A1  - Glicenstein, J. F.
A1  - Gottschall, D.
A1  - Goyal, A.
A1  - Grondin, M. -H.
A1  - Grudzinska, M.
A1  - Hadasch, D.
A1  - Hahn, J.
A1  - Hawkes, J.
A1  - Heinzelmann, G.
A1  - Henri, G.
A1  - Hermann, G.
A1  - Hervet, O.
A1  - Hillert, A.
A1  - Hinton, James Anthony
A1  - Hofmann, W.
A1  - Hoischen, Clemens
A1  - Holler, M.
A1  - Horns, D.
A1  - Ivascenko, A.
A1  - Jacholkowska, A.
A1  - Jamrozy, M.
A1  - Janiak, M.
A1  - Jankowsky, D.
A1  - Jankowsky, F.
A1  - Jingo, M.
A1  - Jogler, T.
A1  - Jouvin, L.
A1  - Jung-Richardt, I.
A1  - Kastendieck, M. A.
A1  - Katarzynski, K.
A1  - Katz, U.
A1  - Kerszberg, D.
A1  - Khelifi, B.
A1  - Kieffer, M.
A1  - King, J.
A1  - Klepser, S.
A1  - Klochkov, D.
A1  - Kluzniak, W.
A1  - Kolitzus, D.
A1  - Komin, Nu.
A1  - Kosack, K.
A1  - Krakau, S.
A1  - Kraus, M.
A1  - Krayzel, F.
A1  - Krueger, P. P.
A1  - Laffon, H.
A1  - Lamanna, G.
A1  - Lau, J.
A1  - Lees, J. -P.
A1  - Lefaucheur, J.
A1  - Lefranc, V.
A1  - Lemiere, A.
A1  - Lemoine-Goumard, M.
A1  - Lenain, J. -P.
A1  - Leser, Eva
A1  - Liu, R.
A1  - Lohse, T.
A1  - Lorentz, M.
A1  - Lypova, I.
A1  - Marandon, V.
A1  - Marcowith, Alexandre
A1  - Mariaud, C.
A1  - Marx, R.
A1  - Maurin, G.
A1  - Maxted, N.
A1  - Mayer, Michael
A1  - Meintjes, P. J.
A1  - Meyer, M.
A1  - Mitchell, A. M. W.
A1  - Moderski, R.
A1  - Mohamed, M.
A1  - Mora, K.
A1  - Moulin, Emmanuel
A1  - Murach, T.
A1  - de Naurois, M.
A1  - Niederwanger, F.
A1  - Niemiec, J.
A1  - Oakes, L.
A1  - Odaka, H.
A1  - Ohm, S.
A1  - Ostrowski, M.
A1  - Oettl, S.
A1  - Oya, I.
A1  - Padovani, M.
A1  - Panter, M.
A1  - Parsons, R. D.
A1  - Arribas, M. Paz
A1  - Pekeur, N. W.
A1  - Pelletier, G.
A1  - Perennes, C.
A1  - Petrucci, P. -O.
A1  - Peyaud, B.
A1  - Pita, S.
A1  - Poon, H.
A1  - Prokhorov, D.
A1  - Prokoph, H.
A1  - Puehlhofer, G.
A1  - Punch, M.
A1  - Quirrenbach, A.
A1  - Raab, S.
A1  - Reimer, A.
A1  - Reimer, O.
A1  - Renaud, M.
A1  - Reyes, R. de los
A1  - Rieger, F.
A1  - Romoli, C.
A1  - Rosier-Lees, S.
A1  - Rowell, G.
A1  - Rudak, B.
A1  - Rulten, C. B.
A1  - Sahakian, V.
A1  - Salek, D.
A1  - Sanchez, David M.
A1  - Santangelo, A.
A1  - Sasaki, M.
A1  - Schlickeiser, R.
A1  - Schuessler, F.
A1  - Schulz, A.
A1  - Schwanke, U.
A1  - Schwemmer, S.
A1  - Settimo, M.
A1  - Seyffert, A. S.
A1  - Shafi, N.
A1  - Shilon, I.
A1  - Simoni, R.
A1  - Sol, H.
A1  - Spanier, F.
A1  - Spengler, G.
A1  - Spies, F.
A1  - Stawarz, L.
A1  - Steenkamp, R.
A1  - Stegmann, Christian
A1  - Stinzing, F.
A1  - Stycz, K.
A1  - Sushch, Iurii
A1  - Tavernet, J. -P.
A1  - Tavernier, T.
A1  - Taylor, A. M.
A1  - Terrier, R.
A1  - Tibaldo, L.
A1  - Tluczykont, M.
A1  - Trichard, C.
A1  - Tuffs, R.
A1  - van der Walt, J.
A1  - van Eldik, C.
A1  - van Soelen, B.
A1  - Vasileiadis, G.
A1  - Veh, J.
A1  - Venter, C.
A1  - Viana, A.
A1  - Vincent, P.
A1  - Vink, J.
A1  - Voisin, F.
A1  - Voelk, H. J.
A1  - Vuillaume, T.
A1  - Wadiasingh, Z.
A1  - Wagner, S. J.
A1  - Wagner, P.
A1  - Wagner, R. M.
A1  - White, R.
A1  - Wierzcholska, A.
A1  - Willmann, P.
A1  - Woernlein, A.
A1  - Wouters, D.
A1  - Yang, R.
A1  - Zabalza, V.
A1  - Zaborov, D.
A1  - Zacharias, M.
A1  - Zdziarski, A. A.
A1  - Zech, Alraune
A1  - Zefi, F.
A1  - Ziegler, A.
A1  - Zywucka, N.
T1  - HESS Limits on Linelike Dark Matter Signatures in the 100 GeV to 2 TeV Energy Range Close to the Galactic Center
JF  - Physical review letters
N2  - A search for dark matter linelike signals iss performed in the vicinity of the Galactic Center by the H.E.S.S. experiment on observational data taken in 2014. An unbinned likelihood analysis iss developed to improve the sensitivity to linelike signals. The upgraded analysis along with newer data extend the energy coverage of the previous measurement down to 100 GeV. The 18 h of data collected with the H.E.S.S. array allow one to rule out at 95% C.L. the presence of a 130 GeV line (at l = -1.5 degrees, b = 0 degrees and for a dark matter profile centered at this location) previously reported in Fermi-LAT data. This new analysis overlaps significantly in energy with previous Fermi-LAT and H.E.S.S. results. No significant excess associated with dark matter annihilations was found in the energy range of 100 GeV to 2 TeV and upper limits on the gamma-ray flux and the velocity weighted annihilation cross section are derived adopting an Einasto dark matter halo profile. Expected limits for present and future large statistics H.E.S.S. observations are also given.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.117.151302
SN  - 0031-9007
SN  - 1079-7114
VL  - 117
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Geiger, Tobias
A1  - Frieler, Katja
A1  - Levermann, Anders
T1  - High-income does not protect against hurricane losses
JF  - Environmental research letters
N2  - Damage due to tropical cyclones accounts for more than 50% of all meteorologically-induced economic losses worldwide. Their nominal impact is projected to increase substantially as the exposed population grows, per capita income increases, and anthropogenic climate change manifests. So far, historical losses due to tropical cyclones have been found to increase less than linearly with a nation's affected gross domestic product (GDP). Here we show that for the United States this scaling is caused by a sub-linear increase with affected population while relative losses scale super-linearly with per capita income. The finding is robust across a multitude of empirically derived damage models that link the storm's wind speed, exposed population, and per capita GDP to reported losses. The separation of both socio-economic predictors strongly affects the projection of potential future hurricane losses. Separating the effects of growth in population and per-capita income, per hurricane losses with respect to national GDP are projected to triple by the end of the century under unmitigated climate change, while they are estimated to decrease slightly without the separation.
KW  - climate change
KW  - tropical cyclones
KW  - damage
KW  - meteorological extremes
KW  - vulnerability
Y1  - 2016
U6  - https://doi.org/10.1088/1748-9326/11/8/084012
SN  - 1748-9326
VL  - 11
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Ryabchun, Alexander
A1  - Kollosche, Matthias
A1  - Wegener, Michael
A1  - Sakhno, Oksana
T1  - Holographic Structuring of Elastomer Actuator: First True Monolithic Tunable Elastomer Optics
JF  - Advanced materials
N2  - Volume diffraction gratings (VDGs) are inscribed selectively by diffusive introduction of benzophenone and subsequent UV-holographic structuring into an electroactive dielectric elastomer actuator (DEA), to afford a continuous voltage-controlled grating shift of 17%. The internal stress coupling of DEA and optical domain allows for a new generation of true monolithic tunable elastomer optics with voltage controlled properties.
Y1  - 2016
U6  - https://doi.org/10.1002/adma.201602881
SN  - 0935-9648
SN  - 1521-4095
VL  - 28
SP  - 10217
EP  - 10223
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Verma, Meetu
A1  - Denker, Carsten
A1  - Balthasar, H.
A1  - Kuckein, Christoph
A1  - González Manrique, Sergio Javier
A1  - Sobotka, M.
A1  - Gonzalez, N. Bello
A1  - Hoch, S.
A1  - Diercke, Andrea
A1  - Kummerow, Philipp
A1  - Berkefeld, T.
A1  - Collados Vera, M.
A1  - Feller, A.
A1  - Hofmann, A.
A1  - Kneer, F.
A1  - Lagg, A.
A1  - Löhner-Böttcher, J.
A1  - Nicklas, H.
A1  - Pastor Yabar, A.
A1  - Schlichenmaier, R.
A1  - Schmidt, D.
A1  - Schmidt, W.
A1  - Schubert, M.
A1  - Sigwarth, M.
A1  - Solanki, S. K.
A1  - Soltau, D.
A1  - Staude, J.
A1  - Strassmeier, Klaus G.
A1  - Volkmer, R.
A1  - von der Lühe, O.
A1  - Waldmann, T.
T1  - Horizontal flow fields in and around a small active region The transition period between flux emergence and decay
JF  - Polymers
N2  - Context. The solar magnetic field is responsible for all aspects of solar activity. Thus, emergence of magnetic flux at the surface is the first manifestation of the ensuing solar activity. Aims. Combining high-resolution and synoptic observations aims to provide a comprehensive description of flux emergence at photospheric level and of the growth process that eventually leads to a mature active region. Methods. The small active region NOAA 12118 emerged on 2014 July 17 and was observed one day later with the 1.5-m GREGOR solar telescope on 2014 July 18. High-resolution time-series of blue continuum and G-band images acquired in the blue imaging channel (BIC) of the GREGOR Fabry-Perot Interferometer (GFPI) were complemented by synoptic line-of-sight magnetograms and continuum images obtained with the Helioseismic and Magnetic Imager (HMI) onboard the Solar Dynamics Observatory (SDO). Horizontal proper motions and horizontal plasma velocities were computed with local correlation tracking (LCT) and the differential affine velocity estimator (DAVE), respectively. Morphological image processing was employed to measure the photometric and magnetic area, magnetic flux, and the separation profile of the emerging flux region during its evolution. Results. The computed growth rates for photometric area, magnetic area, and magnetic flux are about twice as high as the respective decay rates. The space-time diagram using HMI magnetograms of five days provides a comprehensive view of growth and decay. It traces a leaf-like structure, which is determined by the initial separation of the two polarities, a rapid expansion phase, a time when the spread stalls, and a period when the region slowly shrinks again. The separation rate of 0.26 km s(-1) is highest in the initial stage, and it decreases when the separation comes to a halt. Horizontal plasma velocities computed at four evolutionary stages indicate a changing pattern of inflows. In LCT maps we find persistent flow patterns such as outward motions in the outer part of the two major pores, a diverging feature near the trailing pore marking the site of upwelling plasma and flux emergence, and low velocities in the interior of dark pores. We detected many elongated rapidly expanding granules between the two major polarities, with dimensions twice as large as the normal granules.
KW  - Sun: photosphere
KW  - Sun: magnetic fields
KW  - techniques: image processing
KW  - methods: data analysis
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201628380
SN  - 1432-0746
VL  - 596
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Sandin, C.
A1  - Steffen, M.
A1  - Schoenberner, D.
A1  - Rühling, Ute
T1  - Hot bubbles of planetary nebulae with hydrogen-deficient winds I. Heat conduction in a chemically stratified plasma
JF  - Frontiers in psychology
N2  - Heat conduction has been found a plausible solution to explain discrepancies between expected and measured temperatures in hot bubbles of planetary nebulae (PNe). While the heat conduction process depends on the chemical composition, to date it has been exclusively studied for pure hydrogen plasmas in PNe. A smaller population of PNe show hydrogen-deficient and helium-and carbon-enriched surfaces surrounded by bubbles of the same composition; considerable differences are expected in physical properties of these objects in comparison to the pure hydrogen case. The aim of this study is to explore how a chemistry-dependent formulation of the heat conduction affects physical properties and how it affects the X-ray emission from PN bubbles of hydrogen-deficient stars. We extend the description of heat conduction in our radiation hydrodynamics code to work with any chemical composition. We then compare the bubble-formation process with a representative PN model using both the new and the old descriptions. We also compare differences in the resulting X-ray temperature and luminosity observables of the two descriptions. The improved equations show that the heat conduction in our representative model of a hydrogen-deficient PN is nearly as efficient with the chemistry-dependent description; a lower value on the diffusion coefficient is compensated by a slightly steeper temperature gradient. The bubble becomes somewhat hotter with the improved equations, but differences are otherwise minute. The observable properties of the bubble in terms of the X-ray temperature and luminosity are seemingly unaffected.
KW  - conduction
KW  - hydrodynamics
KW  - planetary nebulae: general
KW  - stars: AGB and post-AGB
KW  - stars: Wolf-Rayet
KW  - X-rays: stars
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201527357
SN  - 1432-0746
VL  - 586
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Lechleitner, Franziska A.
A1  - Baldini, James U. L.
A1  - Breitenbach, Sebastian Franz Martin
A1  - Fohlmeister, Jens Bernd
A1  - McIntyre, Cameron
A1  - Goswami, Bedartha
A1  - Jamieson, Robert A.
A1  - van der Voort, Tessa S.
A1  - Prufer, Keith
A1  - Marwan, Norbert
A1  - Culleton, Brendan J.
A1  - Kennett, Douglas J.
A1  - Asmerom, Yemane
A1  - Polyak, Victor
A1  - Eglinton, Timothy I.
T1  - Hydrological and climatological controls on radiocarbon concentrations in a tropical stalagmite
JF  - Geochimica et cosmochimica acta : journal of the Geochemical Society and the Meteoritical Society
N2  - Precisely-dated stalagmites are increasingly important archives for the reconstruction of terrestrial paleoclimate at very high temporal resolution. In-depth understanding of local conditions at the cave site and of the processes driving stalagmite deposition is of paramount importance for interpreting proxy signals incorporated in stalagmite carbonate. Here we present a sub-decadally resolved dead carbon fraction (DCF) record for a stalagmite from Yok Balum Cave (southern Belize). The record is coupled to parallel stable carbon isotope (delta C-13) and U/Ca measurements, as well as radiocarbon (C-14) measurements from soils overlying the cave system. Using a karst carbon cycle model we disentangle the importance of soil and karst processes on stalagmite DCF incorporation, revealing a dominant host rock dissolution control on total DCF. Covariation between DCF, delta C-13, and U/Ca indicates that karst processes are a common driver of all three parameters, suggesting possible use of delta C-13 and trace element ratios to independently quantify DCF variability. A statistically significant multi-decadal lag of variable length exists between DCF and reconstructed solar activity, suggesting that solar activity influenced regional precipitation in Mesoamerica over the past 1500 years, but that the relationship was non-static. Although the precise nature of the observed lag is unclear, solar-induced changes in North Atlantic oceanic and atmospheric dynamics may play a role. (C) 2016 Elsevier Ltd. All rights reserved.
KW  - Stalagmite
KW  - Tropics
KW  - Radiocarbon
KW  - Trace elements
KW  - Hydroclimate
Y1  - 2016
U6  - https://doi.org/10.1016/j.gca.2016.08.039
SN  - 0016-7037
SN  - 1872-9533
VL  - 194
SP  - 233
EP  - 252
PB  - Elsevier
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Shashev, Yury
A1  - Kupsch, Andreas
A1  - Lange, Axel
A1  - Müller, Bernd R.
A1  - Bruno, Giovanni
T1  - Improving the visibility of phase gratings for Talbot-Lau X-ray imaging
JF  - Materials testing : Materialprüfung ; materials and components, technology and application
N2  - Talbot-Lau interferometry provides X-ray imaging techniques with significant enhancement of the radiographic contrast of weakly absorbing objects. The grating based technique allows separation of absorption, refraction and small angle scattering effects. The different efficiency of rectangular and triangular shaped phase gratings at varying detector distances is investigated. The interference patterns (Talbot carpets) are modeled for parallel monochromatic radiation and measured by synchrotron radiation. In comparison to rectangular shapes of phase gratings much higher visibility is obtained for triangular shapes which yield enhanced contrast of a glass capillary test specimen.
KW  - Talbot-Lau interferometry
KW  - phase grating
KW  - synchrotron imaging
KW  - visibility
KW  - X-ray refraction
Y1  - 2016
U6  - https://doi.org/10.3139/120.110948
SN  - 0025-5300
VL  - 58
SP  - 970
EP  - 974
PB  - Hanser
CY  - München
ER  - 
TY  - JOUR
A1  - Martinez Gonzalez, M. J.
A1  - Pastor Yabar, A.
A1  - Lagg, A.
A1  - Asensio Ramos, A.
A1  - Collados Vera, M.
A1  - Solanki, S. K.
A1  - Balthasar, H.
A1  - Berkefeld, T.
A1  - Denker, Carsten
A1  - Doerr, H. P.
A1  - Feller, A.
A1  - Franz, M.
A1  - González Manrique, Sergio Javier
A1  - Hofmann, A.
A1  - Kneer, F.
A1  - Kuckein, Christoph
A1  - Louis, R.
A1  - von der Lühe, O.
A1  - Nicklas, H.
A1  - Orozco, D.
A1  - Rezaei, R.
A1  - Schlichenmaier, R.
A1  - Schmidt, D.
A1  - Schmidt, W.
A1  - Sigwarth, M.
A1  - Sobotka, M.
A1  - Soltau, D.
A1  - Staude, J.
A1  - Strassmeier, Klaus G.
A1  - Verma, Meetu
A1  - Waldman, T.
A1  - Volkmer, R.
T1  - Inference of magnetic fields in the very quiet Sun
JF  - Journal of geophysical research : Earth surface
N2  - Context. Over the past 20 yr, the quietest areas of the solar surface have revealed a weak but extremely dynamic magnetism occurring at small scales (<500 km), which may provide an important contribution to the dynamics and energetics of the outer layers of the atmosphere. Understanding this magnetism requires the inference of physical quantities from high-sensitivity spectro-polarimetric data with high spatio-temporal resolution. Aims. We present high-precision spectro-polarimetric data with high spatial resolution (0.4") of the very quiet Sun at 1.56 mu m obtained with the GREGOR telescope to shed some light on this complex magnetism. Methods. We used inversion techniques in two main approaches. First, we assumed that the observed profiles can be reproduced with a constant magnetic field atmosphere embedded in a field-free medium. Second, we assumed that the resolution element has a substructure with either two constant magnetic atmospheres or a single magnetic atmosphere with gradients of the physical quantities along the optical depth, both coexisting with a global stray-light component. Results. Half of our observed quiet-Sun region is better explained by magnetic substructure within the resolution element. However, we cannot distinguish whether this substructure comes from gradients of the physical parameters along the line of sight or from horizontal gradients (across the surface). In these pixels, a model with two magnetic components is preferred, and we find two distinct magnetic field populations. The population with the larger filling factor has very weak (similar to 150 G) horizontal fields similar to those obtained in previous works. We demonstrate that the field vector of this population is not constrained by the observations, given the spatial resolution and polarimetric accuracy of our data. The topology of the other component with the smaller filling factor is constrained by the observations for field strengths above 250 G: we infer hG fields with inclinations and azimuth values compatible with an isotropic distribution. The filling factors are typically below 30%. We also find that the flux of the two polarities is not balanced. From the other half of the observed quiet-Sun area similar to 50% are two-lobed Stokes V profiles, meaning that 23% of the field of view can be adequately explained with a single constant magnetic field embedded in a non-magnetic atmosphere. The magnetic field vector and filling factor are reliable inferred in only 50% based on the regular profiles. Therefore, 12% of the field of view harbour hG fields with filling factors typically below 30%. At our present spatial resolution, 70% of the pixels apparently are non-magnetised.
KW  - Sun: atmosphere
KW  - Sun: magnetic fields
KW  - techniques: polarimetric
KW  - methods: observational
Y1  - 2016
U6  - https://doi.org/10.1051/0004-6361/201628449
SN  - 1432-0746
VL  - 596
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Holländer, Lars
A1  - Kossack, Wilhelm
A1  - Kollosche, Matthias
A1  - Wirges, Werner
A1  - Kremer, Friedrich
A1  - Gerhard, Reimund
T1  - Influence of the remanent polarisation on the liquid crystal alignment in composite films of ferroelectric poly(vinylidene fluoride-trifluoroethylene) and a cyanobiphenyl-based liquid crystal
JF  - Liquid crystals : an international journal of science and technology
N2  - Polymer-dispersed liquid crystals (PDLCs) of ferroelectric poly(vinylidene fluoride-trifluoroethylene) and nematic 4-cyano-4&#697;-n-hexylbiphenyl (6CB) or 4-cyano-4&#697;-n-pentylbiphenyl (5CB) were prepared to study the effect of the remanent polarisation of the polymer on the liquid crystal alignment. We measured the macroscopic alignment of the liquid crystal molecules in the thickness direction by means of Infrared Transition-Moment Orientational Analysis. Electrical poling at 100 V/µm caused an increased order parameter up to 0.15. After subsequent annealing above the nematic-to-isotropic phase-transition temperature, the order parameter was reduced to 0.02. Nevertheless, the order parameter was still higher than for non-poled film indicating a slight orientation in thickness direction. Both values are lower than those expected from model calculations. In agreement with dielectric measurements, we attribute this result to the shielding effect of mobile charge carriers within the liquid crystal inclusions.
KW  - Polymer-dispersed liquid crystal
KW  - ferroelectric polymer
KW  - remanent polarisation
KW  - liquid crystal alignment
Y1  - 2016
U6  - https://doi.org/10.1080/02678292.2016.1185174
SN  - 0267-8292
SN  - 1366-5855
VL  - 43
SP  - 1514
EP  - 1521
PB  - Editions Rodopi BV
CY  - Abingdon
ER  - 
TY  - JOUR
A1  - Ghosh, Surya K.
A1  - Cherstvy, Andrey G.
A1  - Petrov, Eugene P.
A1  - Metzler, Ralf
T1  - Interactions of rod-like particles on responsive elastic sheets
JF  - Soft matter
N2  - What are the physical laws of the mutual interactions of objects bound to cell membranes, such as various membrane proteins or elongated virus particles? To rationalise this, we here investigate by extensive computer simulations mutual interactions of rod-like particles adsorbed on the surface of responsive elastic two-dimensional sheets. Specifically, we quantify sheet deformations as a response to adhesion of such filamentous particles. We demonstrate that tip-to-tip contacts of rods are favoured for relatively soft sheets, while side-by-side contacts are preferred for stiffer elastic substrates. These attractive orientation-dependent substrate-mediated interactions between the rod-like particles on responsive sheets can drive their aggregation and self-assembly. The optimal orientation of the membrane-bound rods is established via responding to the elastic energy profiles created around the particles. We unveil the phase diagramme of attractive–repulsive rod–rod interactions in the plane of their separation and mutual orientation. Applications of our results to other systems featuring membrane-associated particles are also discussed.
Y1  - 2016
U6  - https://doi.org/10.1039/C6SM01522K
SN  - 1744-6848
SN  - 1744-683X
PB  - RSC
CY  - London
ER  - 
TY  - JOUR
A1  - Ghosh, Surya K.
A1  - Cherstvy, Andrey G.
A1  - Petrov, Eugene P.
A1  - Metzler, Ralf
T1  - Interactions of rod-like particles on responsive elastic sheets
JF  - Soft matter
N2  - What are the physical laws of the mutual interactions of objects bound to cell membranes, such as various membrane proteins or elongated virus particles? To rationalise this, we here investigate by extensive computer simulations mutual interactions of rod-like particles adsorbed on the surface of responsive elastic two-dimensional sheets. Specifically, we quantify sheet deformations as a response to adhesion of such filamentous particles. We demonstrate that tip-to-tip contacts of rods are favoured for relatively soft sheets, while side-by-side contacts are preferred for stiffer elastic substrates. These attractive orientation-dependent substrate-mediated interactions between the rod-like particles on responsive sheets can drive their aggregation and self-assembly. The optimal orientation of the membrane-bound rods is established via responding to the elastic energy profiles created around the particles. We unveil the phase diagramme of attractive-repulsive rod-rod interactions in the plane of their separation and mutual orientation. Applications of our results to other systems featuring membrane-associated particles are also discussed.
Y1  - 2016
U6  - https://doi.org/10.1039/c6sm01522k
SN  - 1744-683X
SN  - 1744-6848
VL  - 12
SP  - 7908
EP  - 7919
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Pimenova, Anastasiya V.
A1  - Goldobin, Denis S.
A1  - Rosenblum, Michael
A1  - Pikovskij, Arkadij
T1  - Interplay of coupling and common noise at the transition to synchrony in oscillator populations
JF  - Scientific reports
N2  - There are two ways to synchronize oscillators: by coupling and by common forcing, which can be pure noise. By virtue of the Ott-Antonsen ansatz for sine-coupled phase oscillators, we obtain analytically tractable equations for the case where both coupling and common noise are present. While noise always tends to synchronize the phase oscillators, the repulsive coupling can act against synchrony, and we focus on this nontrivial situation. For identical oscillators, the fully synchronous state remains stable for small repulsive coupling; moreover it is an absorbing state which always wins over the asynchronous regime. For oscillators with a distribution of natural frequencies, we report on a counter-intuitive effect of dispersion (instead of usual convergence) of the oscillators frequencies at synchrony; the latter effect disappears if noise vanishes.
Y1  - 2016
U6  - https://doi.org/10.1038/srep38518
SN  - 2045-2322
VL  - 6
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Zehbe, Kerstin
A1  - Kollosche, Matthias
A1  - Lardong, Sebastian
A1  - Kelling, Alexandra
A1  - Schilde, Uwe
A1  - Taubert, Andreas
T1  - Ionogels Based on Poly(methyl methacrylate) and Metal-Containing Ionic Liquids: Correlation between Structure and Mechanical and Electrical Properties
JF  - International journal of molecular sciences
N2  - Ionogels (IGs) based on poly(methyl methacrylate) (PMMA) and the metal-containing ionic liquids (ILs) bis-1-butyl-3-methlimidazolium tetrachloridocuprate(II), tetrachloride cobaltate(II), and tetrachlorido manganate(II) have been synthesized and their mechanical and electrical properties have been correlated with their microstructure. Unlike many previous examples, the current IGs show a decreasing stability in stress-strain experiments on increasing IL fractions. The conductivities of the current IGs are lower than those observed in similar examples in the literature. Both effects are caused by a two-phase structure with micrometer-sized IL-rich domains homogeneously dispersed an IL-deficient continuous PMMA phase. This study demonstrates that the IL-polymer miscibility and the morphology of the IGs are key parameters to control the (macroscopic) properties of IGs.
KW  - microstructure
KW  - ionogels
KW  - ionic liquids
KW  - phase separation
KW  - mechanical properties
KW  - ionic conductivity
Y1  - 2016
U6  - https://doi.org/10.3390/ijms17030391
SN  - 1422-0067
VL  - 17
PB  - MDPI
CY  - Basel
ER  - 
TY  - JOUR
A1  - Schreck, Simon
A1  - Wernet, Philippe
T1  - Isotope effects in liquid water probed by transmission mode x-ray absorption spectroscopy at the oxygen K-edge
JF  - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr
N2  - The effects of isotope substitution in liquid water are probed by x-ray absorption spectroscopy at the O K-edge as measured in transmission mode. Confirming earlier x-ray Raman scattering experiments, the D2O spectrum is found to be blue shifted with respect to H2O, and the D2O spectrum to be less broadened. Following the earlier interpretations of UV and x-ray Raman spectra, the shift is related to the difference in ground-state zero-point energies between D2O and H2O, while the difference in broadening is related to the difference in ground-state vibrational zero-point distributions. We demonstrate that the transmission-mode measurements allow for determining the spectral shapes with unprecedented accuracy. Owing in addition to the increased spectral resolution and signal to noise ratio compared to the earlier measurements, the new data enable the stringent determination of blue shift and broadening in the O K-edge x-ray absorption spectrum of liquid water upon isotope substitution. The results are compared to UV absorption data, and it is discussed to which extent they reflect the differences in zero-point energies and vibrational zero-point distributions in the ground-states of the liquids. The influence of the shape of the final-state potential, inclusion of the Franck-Condon structure, and differences between liquid H2O and D2O resulting from different hydrogen-bond environments in the liquids are addressed. The differences between the O K-edge absorption spectra of water from our transmission-mode measurements and from the state-of-the-art x-ray Raman scattering experiments are discussed in addition. The experimentally extracted values of blue shift and broadening are proposed to serve as a test for calculations of ground-state zero-point energies and vibrational zero-point distributions in liquid H2O and D2O. This clearly motivates the need for new calculations of the O K-edge x-ray absorption spectrum of liquid water. Published by AIP Publishing.
Y1  - 2016
U6  - https://doi.org/10.1063/1.4962237
SN  - 0021-9606
SN  - 1089-7690
VL  - 145
SP  - 24
EP  - 32
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Rettig, L.
A1  - Dornes, C.
A1  - Thielemann-Kuehn, Nele
A1  - Pontius, N.
A1  - Zabel, Hartmut
A1  - Schlagel, D. L.
A1  - Lograsso, T. A.
A1  - Chollet, M.
A1  - Robert, A.
A1  - Sikorski, M.
A1  - Song, S.
A1  - Glownia, J. M.
A1  - Schuessler-Langeheine, Christian
A1  - Johnson, S. L.
A1  - Staub, U.
T1  - Itinerant and Localized Magnetization Dynamics in Antiferromagnetic Ho
JF  - Physical review letters
N2  - Using femtosecond time-resolved resonant magnetic x-ray diffraction at the Ho L-3 absorption edge, we investigate the demagnetization dynamics in antiferromagnetically ordered metallic Ho after femtosecond optical excitation. Tuning the x-ray energy to the electric dipole (E1, 2p -> 5d) or quadrupole (E2, 2p -> 4f) transition allows us to selectively and independently study the spin dynamics of the itinerant 5d and localized 4f electronic subsystems via the suppression of the magnetic (2 1 3-tau) satellite peak. We find demagnetization time scales very similar to ferromagnetic 4f systems, suggesting that the loss of magnetic order occurs via a similar spin-flip process in both cases. The simultaneous demagnetization of both subsystems demonstrates strong intra-atomic 4f-5d exchange coupling. In addition, an ultrafast lattice contraction due to the release of magneto-striction leads to a transient shift of the magnetic satellite peak.
Y1  - 2016
U6  - https://doi.org/10.1103/PhysRevLett.116.257202
SN  - 0031-9007
SN  - 1079-7114
VL  - 116
SP  - 6382
EP  - 6389
PB  - American Physical Society
CY  - College Park
ER  -