TY  - JOUR
A1  - Tockhorn, Philipp
A1  - Sutter, Johannes
A1  - Cruz Bournazou, Alexandros
A1  - Wagner, Philipp
A1  - Jäger, Klaus
A1  - Yoo, Danbi
A1  - Lang, Felix
A1  - Grischek, Max
A1  - Li, Bor
A1  - Li, Jinzhao
A1  - Shargaieva, Oleksandra
A1  - Unger, Eva
A1  - Al-Ashouri, Amran
A1  - Köhnen, Eike
A1  - Stolterfoht, Martin
A1  - Neher, Dieter
A1  - Schlatmann, Rutger
A1  - Rech, Bernd
A1  - Stannowski, Bernd
A1  - Albrecht, Steve
A1  - Becker, Christiane
T1  - Nano-optical designs for high-efficiency monolithic perovskite-silicon tandem solar cells
JF  - Nature nanotechnology
N2  - Designing gentle sinusoidal nanotextures enables the realization of high-efficiency perovskite-silicon solar cells <br /> Perovskite-silicon tandem solar cells offer the possibility of overcoming the power conversion efficiency limit of conventional silicon solar cells. Various textured tandem devices have been presented aiming at improved optical performance, but optimizing film growth on surface-textured wafers remains challenging. Here we present perovskite-silicon tandem solar cells with periodic nanotextures that offer various advantages without compromising the material quality of solution-processed perovskite layers. We show a reduction in reflection losses in comparison to planar tandems, with the new devices being less sensitive to deviations from optimum layer thicknesses. The nanotextures also enable a greatly increased fabrication yield from 50% to 95%. Moreover, the open-circuit voltage is improved by 15 mV due to the enhanced optoelectronic properties of the perovskite top cell. Our optically advanced rear reflector with a dielectric buffer layer results in reduced parasitic absorption at near-infrared wavelengths. As a result, we demonstrate a certified power conversion efficiency of 29.80%.
Y1  - 2022
U6  - https://doi.org/10.1038/s41565-022-01228-8
SN  - 1748-3387
SN  - 1748-3395
VL  - 17
IS  - 11
SP  - 1214
EP  - 1221
PB  - Nature Publishing Group
CY  - London [u.a.]
ER  - 
TY  - JOUR
A1  - Roland, Steffen
A1  - Neubert, Sebastian
A1  - Albrecht, Steve
A1  - Stannowski, Bernd
A1  - Seger, Mark
A1  - Facchetti, Antonio
A1  - Schlatmann, Rutger
A1  - Rech, Bernd
A1  - Neher, Dieter
T1  - Hybrid Organic/Inorganic Thin-Film Multijunction Solar Cells Exceeding 11% Power Conversion Efficiency
JF  - Advanced materials
N2  - Hybrid multijunction solar cells comprising hydrogenated amorphous silicon and an organic bulk heterojunction are presented, reaching 11.7% power conversion efficiency. The benefits of merging inorganic and organic subcells are pointed out, the optimization of the cells, including optical modeling predictions and tuning of the recombination contact are described, and an outlook of this technique is given.
Y1  - 2015
U6  - https://doi.org/10.1002/adma.201404698
SN  - 0935-9648
SN  - 1521-4095
VL  - 27
IS  - 7
SP  - 1262
EP  - 1267
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Albrecht, Steve
A1  - Grootoonk, Bjorn
A1  - Neubert, Sebastian
A1  - Roland, Steffen
A1  - Wordenweber, Jan
A1  - Meier, Matthias
A1  - Schlatmann, Rutger
A1  - Gordijn, Aad
A1  - Neher, Dieter
T1  - Efficient hybrid inorganic/organic tandem solar cells with tailored recombination contacts
JF  - Solar energy materials & solar cells : an international journal devoted to photovoltaic, photothermal, and photochemical solar energy conversion
N2  - In this work, the authors present a 7.5% efficient hybrid tandem solar cell with the bottom cell made of amorphous silicon and a Si-PCPDTBT:PC70BM bulk heterojunction top cell. Loss-free recombination contacts were realized by combing Al-doped ZnO with either the conducting polymer composite PEDOT:PSS or with a bilayer of ultrathin Al and MoO3. Optimization of these contacts results in tandem cells with high fill factors of 70% and an open circuit voltage close to the sum of those of the sub-cells. This is the best efficiency reported for this type of hybrid tandem cell so far. Optical and electrical device modeling suggests that the efficiency can be increased to similar to 12% on combining a donor polymer with suitable absorption onset with PCBM. We also describe proof-of-principle studies employing light trapping in hybrid tandem solar cells, suggesting that this device architecture has the potential to achieve efficiencies well above 12%. (C) 2014 Elsevier B.V. All rights reserved.
KW  - Hybrid solar cells
KW  - Tandem solar cells
KW  - Organic solar cells
KW  - Bulk heterojunction
KW  - Efficiency optimization
Y1  - 2014
U6  - https://doi.org/10.1016/j.solmat.2014.04.020
SN  - 0927-0248
SN  - 1879-3398
VL  - 127
SP  - 157
EP  - 162
PB  - Elsevier
CY  - Amsterdam
ER  -