TY - JOUR A1 - Schick, Daniel A1 - Le Guyader, Loic A1 - Pontius, Niko A1 - Radu, Ilie A1 - Kachel, Torsten A1 - Mitzner, Rolf A1 - Zeschke, Thomas A1 - Schuessler-Langeheine, Christian A1 - Föhlisch, Alexander A1 - Holldack, Karsten T1 - Analysis of the halo background in femtosecond slicing experiments JF - Journal of synchrotron radiation N2 - The slicing facility FemtoSpeX at BESSY II offers unique opportunities to study photo-induced dynamics on femtosecond time scales by means of X-ray magnetic circular dichroism, resonant and non-resonant X-ray diffraction, and X-ray absorption spectroscopy experiments in the soft X-ray regime. Besides femtosecond X-ray pulses, slicing sources inherently also produce a so-called `halo' background with a different time structure, polarization and pointing. Here a detailed experimental characterization of the halo radiation is presented, and a method is demonstrated for its correct and unambiguous removal from femtosecond time-resolved data using a special laser triggering scheme as well as analytical models. Examples are given for time-resolved measurements with corresponding halo correction, and errors of the relevant physical quantities caused by either neglecting or by applying a simplified model to describe this background are estimated. KW - femtosecond slicing KW - halo KW - pump-probe KW - XMCD KW - X-ray scattering Y1 - 2016 U6 - https://doi.org/10.1107/S160057751600401X SN - 1600-5775 VL - 23 SP - 700 EP - 711 PB - International Union of Crystallography CY - Chester ER - TY - JOUR A1 - Schick, Daniel A1 - Eckert, Sebastian A1 - Pontius, Niko A1 - Mitzner, Rolf A1 - Föhlisch, Alexander A1 - Holldack, Karsten A1 - Sorgenfrei, Florian T1 - Versatile soft X-ray-optical cross-correlator for ultrafast applications JF - Structural dynamics N2 - We present an X-ray-optical cross-correlator for the soft (> 150 eV) up to the hard X-ray regime based on a molybdenum-silicon superlattice. The cross-correlation is done by probing intensity and position changes of superlattice Bragg peaks caused by photoexcitation of coherent phonons. This approach is applicable for a wide range of X-ray photon energies as well as for a broad range of excitation wavelengths and requires no external fields or changes of temperature. Moreover, the cross-correlator can be employed on a 10 ps or 100 fs time scale featuring up to 50% total X-ray reflectivity and transient signal changes of more than 20%. (C) 2016 Author(s). Y1 - 2016 U6 - https://doi.org/10.1063/1.4964296 SN - 2329-7778 VL - 3 SP - 054304-1 EP - 054304-8 PB - American Institute of Physics CY - Melville ER - TY - GEN A1 - Schick, Daniel A1 - Eckert, Sebastian A1 - Pontius, Niko A1 - Mitzner, Rolf A1 - Föhlisch, Alexander A1 - Holldack, Karsten A1 - Sorgenfrei, Florian T1 - Versatile soft X-ray-optical cross-correlator for ultrafast applications T2 - Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe N2 - We present an X-ray-optical cross-correlator for the soft (> 150 eV) up to the hard X-ray regime based on a molybdenum-silicon superlattice. The cross-correlation is done by probing intensity and position changes of superlattice Bragg peaks caused by photoexcitation of coherent phonons. This approach is applicable for a wide range of X-ray photon energies as well as for a broad range of excitation wavelengths and requires no external fields or changes of temperature. Moreover, the cross-correlator can be employed on a 10 ps or 100 fs time scale featuring up to 50% total X-ray reflectivity and transient signal changes of more than 20%. (C) 2016 Author(s). T3 - Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe - 1331 Y1 - 2016 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-436962 SN - 1866-8372 IS - 1331 SP - 054304-1 EP - 054304-8 ER -