TY  - JOUR
A1  - Huber, C.
A1  - Klamroth, Tillmann
T1  - Simulation of two-photon-photoelectron spectra at a jellium-vacuum interface
N2  - In this paper we report on time dependent configuration interaction singles (TD-CIS) calculations aimed at simulating two-photon-photoelectron emission (2PPE) spectra of metal films, the latter treated within a one-dimensional jellium model. The method is based on a many-electron approach in which electron-electron-scattering is approximately accounted for and no artificial lifetimes have to be assumed for excited electrons. This contrasts with one-electron models where lifetimes and "dissipation" have to be introduced. The driving force for the photoelectron ejection in 2PPE experiments is the electric field of two laser pulses that are generally separated by a delay time, Delta t. To compute energy- and time-resolved 2PPE signals P(E, Delta t), a new scheme based on the time-energy method is proposed to analyze electronic wave packets in asymptotic regions of the potential
Y1  - 2005
ER  - 
TY  - JOUR
A1  - Saalfrank, Peter
A1  - Klamroth, Tillmann
A1  - Huber, C.
A1  - Krause, Pascal
T1  - Laser-driven electron dynamics at interfaces
N2  - In this paper we present time-dependent, quantum-dynamical simulations of photoinduced processes at solid surfaces involving nonadiabatic transitions of electrons to and from short-lived intermediate excited states. In particular, two-photon photoemission (2PPE) spectra of naked metal surfaces and free-standing metal films are considered. One major problem in both cases is the presence of electron-electron scattering, which is treated here in various ways. The first way is to adopt an open-system density matrix approach, in which a single electron is weakly coupled to a "bath" of other electrons. The second approach is based on a many-electron Schrodinger equation, which is solved with the help of a time-dependent configuration interactions singles (TD-CIS) method
Y1  - 2005
SN  - 0021-2148
ER  -