TY - JOUR A1 - Winkler, M. A1 - Abel, M. W. T1 - Mixing in thermal convection of very thin free-standing films JF - PHYSICA SCRIPTA N2 - Thin liquid films serve as the paradigms of atmospheric convection, thermal convection in the Earth’s mantle or turbulence in magnetohydrodynamics, thereby connecting with typical systems exhibiting turbulent mixing. In addition, recent research on colloids, interfaces and nanofluids led to advances in the development of micro-mixers (lab-on-a-chip devices). By the thermal forcing of a film, one can reach Rayleigh numbers in the turbulent regime, such that the experiment may serve as a prototype of a mixer on the basis of thermally induced turbulence in free-standing thin liquid films with thicknesses in the nanometer range. Here, the specific experimental results of a setup with a focus on the mixing statistics of a thermally driven two-dimensional thin film are presented. Our setup allows us to capture thin film interference patterns under controlled surface and atmospheric conditions. The convection is realized by placing a cooled copper rod in the center of the film. The temperature gradient between the rod and the atmosphere results in a density gradient in the liquid film, so that the varying buoyancy induces turbulent motion. The flow field is characterized by a newly developed algorithm-color imaging velocimetry (CIV). This analysis determines not only the velocity, but also the full deformation tensor in the Lagrangian frame. On the basis of these insights, the flow in the experiment was investigated with respect to its mixing properties: we calculated the mixing efficiency and entropy of the flow scheme to sufficiently high accuracy. Y1 - 2013 U6 - https://doi.org/10.1088/0031-8949/2013/T155/014020 SN - 0031-8949 VL - T155 IS - 7 PB - IOP PUBLISHING LTD CY - BRISTOL ER - TY - JOUR A1 - Winkler, M. A1 - Kofod, G. A1 - Krastev, R. A1 - Stoeckle, S. A1 - Abel, M. W. T1 - Exponentially Fast Thinning of Nanoscale Films by Turbulent Mixing JF - PHYSICAL REVIEW LETTERS N2 - Films are nanoscopic elements of foams, emulsions, and suspensions that form a paradigm for nanochannel transport that eventually tests the limits of hydrodynamic descriptions. Here, we study the collapse of a freestanding film to its equilibrium. The generation of nanoscale films usually is a slow linear process; using thermal forcing we find unprecedented dynamics with exponentially fast thinning. The complex interplay of thermal convection, interface, and gravitational forces yields optimal turbulent mixing and transport. Domains of collapsed film are generated, elongated, and convected in a beautiful display of chaotic mixing. With a time scale analysis, we identify mixing as the dominant dynamical process responsible for exponential thinning. DOI: 10.1103/PhysRevLett.110.094501 Y1 - 2013 U6 - https://doi.org/10.1103/PhysRevLett.110.094501 SN - 0031-9007 VL - 110 IS - 9 PB - AMER PHYSICAL SOC CY - COLLEGE PK ER -