TY - JOUR A1 - Jechow, Andreas A1 - Norton, B. G. A1 - Händel, S. A1 - Blums, V. A1 - Streed, E. W. A1 - Kielpinski, D. T1 - Controllable optical phase shift over one radian from a single isolated atom JF - Physical review letters N2 - Fundamental optics such as lenses and prisms work by applying phase shifts of several radians to incoming light, and rapid control of such phase shifts is crucial to telecommunications. However, large, controllable optical phase shifts have remained elusive for isolated quantum systems. We have used a single trapped atomic ion to induce and measure a large optical phase shift of 1.3 +/- 0.1 radians in light scattered by the atom. Spatial interferometry between the scattered light and unscattered illumination light enables us to isolate the phase shift in the scattered component. The phase shift achieves the maximum value allowed by atomic theory over the accessible range of laser frequencies, pointing out new opportunities in microscopy and nanophotonics. Single-atom phase shifts of this magnitude open up new quantum information protocols, in particular long-range quantum phase-shift-keying cryptography. DOI: 10.1103/PhysRevLett.110.113605 Y1 - 2013 U6 - https://doi.org/10.1103/PhysRevLett.110.113605 SN - 0031-9007 VL - 110 IS - 11 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Jechow, Andreas A1 - Seefeldt, Michael A1 - Kurzke, Henning A1 - Heuer, Axel A1 - Menzel, Ralf T1 - Enhanced two-photon excited fluorescence from imaging agents using true thermal light JF - Nature photonics N2 - Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy(1), but is still affected by photodamage to the probe. It has been proposed that TPEF can be enhanced using entangled photons(2,3), but this has proven challenging. Recently, it was shown that some features of entangled photons can be mimicked with thermal light, which finds application in ghost imaging(4), subwavelength lithography(5) and metrology(6). Here, we use true thermal light from a superluminescent diode to demonstrate TPEF that is enhanced compared to coherent light, using two common fluorophores and luminescent quantum dots, which suit applications in imaging and microscopy. We find that the TPEF rate is directly proportional to the measured(7) degree of second-order coherence, as predicted by theory. Our results show that photon bunching in thermal light can be exploited in two-photon microscopy, with the photon statistic providing a new degree of freedom. Y1 - 2013 U6 - https://doi.org/10.1038/NPHOTON.2013.271 SN - 1749-4885 SN - 1749-4893 VL - 7 IS - 12 SP - 973 EP - 976 PB - Nature Publ. Group CY - London ER -