TY  - JOUR
A1  - Shayduk, Roman
A1  - Navirian, Hengameh
A1  - Leitenberger, Wolfram
A1  - Goldshteyn, Jevgenij
A1  - Vrejoiu, Ionela
A1  - Weinelt, Martin
A1  - Gaal, Peter
A1  - Herzog, Marc
A1  - von Korff Schmising, Clemens
A1  - Bargheer, Matias
T1  - Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction
JF  - New journal of physics : the open-access journal for physics
N2  - We report on synchrotron-based high-repetition rate ultrafast x-ray diffraction (UXRD) experiments monitoring the transport of heat from an epitaxial La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice (SL) into the substrate on timescales from 100 ps to 4 mu s. Transient thermal lattice expansion was determined with an accuracy of 10(-7), corresponding to a sensitivity to temperature changes down to 0.01 K. We follow the heat flow within the SL and into the substrate after the impulsive laser heating leads to a small temperature rise of Delta T = 6 K. The transient lattice temperature can be simulated very well using the bulk heat conductivities. This contradicts the interpretation of previous UXRD measurements, which predicted a long-lasting expansion of SrRuO(3) for more than 200 ps. The disagreement could be resolved by assuming that the heat conductivity changes in the first hundred picoseconds.
Y1  - 2011
U6  - https://doi.org/10.1088/1367-2630/13/9/093032
SN  - 1367-2630
VL  - 13
IS  - 11
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Navirian, Hengameh A.
A1  - Herzog, Marc
A1  - Goldshteyn, J.
A1  - Leitenberger, Wolfram
A1  - Vrejoiu, Ionella
A1  - Khakhulin, D.
A1  - Wulff, M.
A1  - Shayduk, Roman
A1  - Gaal, P.
A1  - Bargheer, Matias
T1  - Shortening x-ray pulses for pump-probe experiments at synchrotrons
JF  - Journal of applied physics
N2  - We implemented an experimental scheme for ultrafast x-ray diffraction at storage rings based on a laser-driven Bragg-switch that shortens the x-ray pulses emitted from an undulator. The increased time-resolution is demonstrated by observing changes of intensity, position and width of the diffraction peaks of a La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice sample after optical excitation, i.e., by quantitatively measuring the propagation of an expansion wave through the sample. These experimental transients with timescales of 35 to 60 ps evidence a reduction of the x-ray pulse duration by a factor of two.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3601057
SN  - 0021-8979
VL  - 109
IS  - 12
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Gruber, W.
A1  - Chakravarty, S.
A1  - Baehtz, C.
A1  - Leitenberger, Wolfram
A1  - Bruns, M.
A1  - Kobler, A.
A1  - Kübel, Christian
A1  - Schmidt, H.
T1  - Strain relaxation and vacancy creation in thin platinum films
JF  - Physical review letters
N2  - Synchrotron based combined in situ x-ray diffractometry and reflectometry is used to investigate the role of vacancies for the relaxation of residual stress in thin metallic Pt films. From the experimentally determined relative changes of the lattice parameter a and of the film thickness L the modification of vacancy concentration and residual strain was derived as a function of annealing time at 130 degrees C. The results indicate that relaxation of strain resulting from compressive stress is accompanied by the creation of vacancies at the free film surface. This proves experimentally the postulated dominant role of vacancies for stress relaxation in thin metal films close to room temperature.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevLett.107.265501
SN  - 0031-9007
VL  - 107
IS  - 26
PB  - American Physical Society
CY  - College Park
ER  -