@misc{ZeuschnerMatternPudelletal.2021,
  author    = {Zeuschner, Steffen Peer and Mattern, Maximilian and Pudell, Jan-Etienne and Reppert, Alexander von and R{\"o}ssle, Matthias and Leitenberger, Wolfram and Schwarzkopf, Jutta and Boschker, Jos and Herzog, Marc and Bargheer, Matias},
  title     = {Reciprocal space slicing},
  series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe},
  journal   = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe},
  number    = {1137},
  issn      = {1866-8372},
  doi       = {10.25932/publishup-49976},
  url       = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-499761},
  pages     = {13},
  year      = {2021},
  abstract  = {An experimental technique that allows faster assessment of out-of-plane strain dynamics of thin film heterostructures via x-ray diffraction is presented. In contrast to conventional high-speed reciprocal space-mapping setups, our approach reduces the measurement time drastically due to a fixed measurement geometry with a position-sensitive detector. This means that neither the incident (ω) nor the exit (2θ) diffraction angle is scanned during the strain assessment via x-ray diffraction. Shifts of diffraction peaks on the fixed x-ray area detector originate from an out-of-plane strain within the sample. Quantitative strain assessment requires the determination of a factor relating the observed shift to the change in the reciprocal lattice vector. The factor depends only on the widths of the peak along certain directions in reciprocal space, the diffraction angle of the studied reflection, and the resolution of the instrumental setup. We provide a full theoretical explanation and exemplify the concept with picosecond strain dynamics of a thin layer of NbO2.},
  language  = {en}
}
@article{ZeuschnerMatternPudelletal.2021,
  author    = {Zeuschner, Steffen Peer and Mattern, Maximilian and Pudell, Jan-Etienne and Reppert, Alexander von and R{\"o}ssle, Matthias and Leitenberger, Wolfram and Schwarzkopf, Jutta and Boschker, Jos and Herzog, Marc and Bargheer, Matias},
  title     = {Reciprocal space slicing},
  series = {Structural dynamics},
  volume    = {8},
  journal   = {Structural dynamics},
  number    = {1},
  publisher = {AIP Publishing LLC},
  address   = {Melville, NY},
  issn      = {2329-7778},
  doi       = {10.1063/4.0000040},
  pages     = {10},
  year      = {2021},
  abstract  = {An experimental technique that allows faster assessment of out-of-plane strain dynamics of thin film heterostructures via x-ray diffraction is presented. In contrast to conventional high-speed reciprocal space-mapping setups, our approach reduces the measurement time drastically due to a fixed measurement geometry with a position-sensitive detector. This means that neither the incident (ω) nor the exit (2θ) diffraction angle is scanned during the strain assessment via x-ray diffraction. Shifts of diffraction peaks on the fixed x-ray area detector originate from an out-of-plane strain within the sample. Quantitative strain assessment requires the determination of a factor relating the observed shift to the change in the reciprocal lattice vector. The factor depends only on the widths of the peak along certain directions in reciprocal space, the diffraction angle of the studied reflection, and the resolution of the instrumental setup. We provide a full theoretical explanation and exemplify the concept with picosecond strain dynamics of a thin layer of NbO2.},
  language  = {en}
}
@article{HerzogReppertPudelletal.2022,
  author    = {Herzog, Marc and Reppert, Alexander von and Pudell, Jan-Etienne and Henkel, Carsten and Kronseder, Matthias and Back, Christian H. and Maznev, Alexei A. and Bargheer, Matias},
  title     = {Phonon-dominated energy transport in purely metallic heterostructures},
  series = {Advanced functional materials},
  volume    = {32},
  journal   = {Advanced functional materials},
  number    = {41},
  publisher = {Wiley-VCH},
  address   = {Weinheim},
  issn      = {1616-301X},
  doi       = {10.1002/adfm.202206179},
  pages     = {8},
  year      = {2022},
  abstract  = {Ultrafast X-ray diffraction is used to quantify the transport of energy in laser-excited nanoscale gold-nickel (Au-Ni) bilayers. Electron transport and efficient electron-phonon coupling in Ni convert the laser-deposited energy in the conduction electrons within a few picoseconds into a strong non-equilibrium between hot Ni and cold Au phonons at the bilayer interface. Modeling of the subsequent equilibration dynamics within various two-temperature models confirms that for ultrathin Au films, the thermal transport is dominated by phonons instead of conduction electrons because of the weak electron-phonon coupling in Au.},
  language  = {en}
}
@article{ZeuschnerParpiievPezeriletal.2019,
  author    = {Zeuschner, Steffen Peer and Parpiiev, Tymur and Pezeril, Thomas and Hillion, Arnaud and Dumesnil, Karine and Anane, Abdelmadjid and Pudell, Jan-Etienne and Willig, Lisa and R{\"o}ssle, Matthias and Herzog, Marc and Reppert, Alexander von and Bargheer, Matias},
  title     = {Tracking picosecond strain pulses in heterostructures that exhibit giant magnetostriction},
  series = {Structural Dynamics},
  volume    = {6},
  journal   = {Structural Dynamics},
  number    = {2},
  publisher = {AIP Publishing LLC},
  address   = {Melville, NY},
  issn      = {2329-7778},
  doi       = {10.1063/1.5084140},
  pages     = {9},
  year      = {2019},
  abstract  = {We combine ultrafast X-ray diffraction (UXRD) and time-resolved Magneto-Optical Kerr Effect (MOKE) measurements to monitor the strain pulses in laser-excited TbFe2/Nb heterostructures. Spatial separation of the Nb detection layer from the laser excitation region allows for a background-free characterization of the laser-generated strain pulses. We clearly observe symmetric bipolar strain pulses if the excited TbFe2 surface terminates the sample and a decomposition of the strain wavepacket into an asymmetric bipolar and a unipolar pulse, if a SiO2 glass capping layer covers the excited TbFe2 layer. The inverse magnetostriction of the temporally separated unipolar strain pulses in this sample leads to a MOKE signal that linearly depends on the strain pulse amplitude measured through UXRD. Linear chain model simulations accurately predict the timing and shape of UXRD and MOKE signals that are caused by the strain reflections from multiple interfaces in the heterostructure.},
  language  = {en}
}
@article{ReppertMatternPudelletal.2020,
  author    = {Reppert, Alexander von and Mattern, Maximilian and Pudell, Jan-Etienne and Zeuschner, Steffen Peer and Dumesnil, Karine and Bargheer, Matias},
  title     = {Unconventional picosecond strain pulses resulting from the saturation of magnetic stress within a photoexcited rare earth layer},
  series = {Structural Dynamics},
  volume    = {7},
  journal   = {Structural Dynamics},
  number    = {024303},
  publisher = {AIP Publishing LLC},
  address   = {Melville, NY},
  issn      = {2329-7778},
  doi       = {10.1063/1.5145315},
  pages     = {13},
  year      = {2020},
  abstract  = {Optical excitation of spin-ordered rare earth metals triggers a complex response of the crystal lattice since expansive stresses from electron and phonon excitations compete with a contractive stress induced by spin disorder. Using ultrafast x-ray diffraction experiments, we study the layer specific strain response of a dysprosium film within a metallic heterostructure upon femtosecond laser-excitation. The elastic and diffusive transport of energy to an adjacent, non-excited detection layer clearly separates the contributions of strain pulses and thermal excitations in the time domain. We find that energy transfer processes to magnetic excitations significantly modify the observed conventional bipolar strain wave into a unipolar pulse. By modeling the spin system as a saturable energy reservoir that generates substantial contractive stress on ultrafast timescales, we can reproduce the observed strain response and estimate the time- and space dependent magnetic stress. The saturation of the magnetic stress contribution yields a non-monotonous total stress within the nanolayer, which leads to unconventional picosecond strain pulses.},
  language  = {en}
}
@article{SarhanKoopmanPudelletal.2019,
  author    = {Sarhan, Radwan Mohamed and Koopman, Wouter-Willem Adriaan and Pudell, Jan-Etienne and Stete, Felix and R{\"o}ssle, Matthias and Herzog, Marc and Schmitt, Clemens Nikolaus Zeno and Liebig, Ferenc and Koetz, Joachim and Bargheer, Matias},
  title     = {Scaling up nanoplasmon catalysis},
  series = {The journal of physical chemistry : C, Nanomaterials and interfaces},
  volume    = {123},
  journal   = {The journal of physical chemistry : C, Nanomaterials and interfaces},
  number    = {14},
  publisher = {American Chemical Society},
  address   = {Washington},
  issn      = {1932-7447},
  doi       = {10.1021/acs.jpcc.8b12574},
  pages     = {9352 -- 9357},
  year      = {2019},
  abstract  = {Nanoscale heating by optical excitation of plasmonic nanoparticles offers a new perspective of controlling chemical reactions, where heat is not spatially uniform as in conventional macroscopic heating but strong temperature gradients exist around microscopic hot spots. In nanoplasmonics, metal particles act as a nanosource of light, heat, and energetic electrons driven by resonant excitation of their localized surface plasmon resonance. As an example of the coupling reaction of 4-nitrothiophenol into 4,4′-dimercaptoazobenzene, we show that besides the nanoscopic heat distribution at hot spots, the microscopic distribution of heat dictated by the spot size of the light focus also plays a crucial role in the design of plasmonic nanoreactors. Small sizes of laser spots enable high intensities to drive plasmon-assisted catalysis. This facilitates the observation of such reactions by surface-enhanced Raman scattering, but it challenges attempts to scale nanoplasmonic chemistry up to large areas, where the excess heat must be dissipated by one-dimensional heat transport.},
  language  = {en}
}
@misc{PavlenkoSanderMitzscherlingetal.2016,
  author    = {Pavlenko, Elena S. and Sander, Mathias and Mitzscherling, Steffen and Pudell, Jan-Etienne and Zamponi, Flavio and R{\"o}ssle, Matthias and Bojahr, Andre and Bargheer, Matias},
  title     = {Azobenzene - functionalized polyelectrolyte nanolayers as ultrafast optoacoustic transducers},
  volume    = {8},
  doi       = {10.1039/C6NR01448H},
  url       = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-101996},
  pages     = {13297 -- 13302},
  year      = {2016},
  abstract  = {We introduce azobenzene-functionalized polyelectrolyte multilayers as efficient, inexpensive optoacoustic transducers for hyper-sound strain waves in the GHz range. By picosecond transient reflectivity measurements we study the creation of nanoscale strain waves, their reflection from interfaces, damping by scattering from nanoparticles and propagation in soft and hard adjacent materials like polymer layers, quartz and mica. The amplitude of the generated strain ε ∼ 5 × 10-4 is calibrated by ultrafast X-ray diffraction.},
  language  = {en}
}
@article{MatternPudellLaskinetal.2021,
  author    = {Mattern, Maximilian and Pudell, Jan-Etienne and Laskin, Gennadii and Reppert, Alexander von and Bargheer, Matias},
  title     = {Analysis of the temperature- and fluence-dependent magnetic stress in laser-excited SrRuO3},
  series = {Structural dynamics},
  volume    = {8},
  journal   = {Structural dynamics},
  number    = {2},
  publisher = {AIP Publishing LLC},
  address   = {Melville, NY},
  issn      = {2329-7778},
  doi       = {10.1063/4.0000072},
  pages     = {9},
  year      = {2021},
  abstract  = {We use ultrafast x-ray diffraction to investigate the effect of expansive phononic and contractive magnetic stress driving the picosecond strain response of a metallic perovskite SrRuO3 thin film upon femtosecond laser excitation. We exemplify how the anisotropic bulk equilibrium thermal expansion can be used to predict the response of the thin film to ultrafast deposition of energy. It is key to consider that the laterally homogeneous laser excitation changes the strain response compared to the near-equilibrium thermal expansion because the balanced in-plane stresses suppress the Poisson stress on the picosecond timescale. We find a very large negative Gr{\"u}neisen constant describing the large contractive stress imposed by a small amount of energy in the spin system. The temperature and fluence dependence of the strain response for a double-pulse excitation scheme demonstrates the saturation of the magnetic stress in the high-fluence regime.},
  language  = {en}
}
@article{PudellSanderBaueretal.2019,
  author    = {Pudell, Jan-Etienne and Sander, M. and Bauer, R. and Bargheer, Matias and Herzog, Marc and Ga{\´a}l, Peter},
  title     = {Full Spatiotemporal Control of Laser-Excited Periodic Surface Deformations},
  series = {Physical review applied},
  volume    = {12},
  journal   = {Physical review applied},
  number    = {2},
  publisher = {American Physical Society},
  address   = {College Park},
  issn      = {2331-7019},
  doi       = {10.1103/PhysRevApplied.12.024036},
  pages     = {11},
  year      = {2019},
  abstract  = {We demonstrate full control of acoustic and thermal periodic deformations at solid surfaces down to subnanosecond time scales and few-micrometer length scales via independent variation of the temporal and spatial phase of two optical transient grating (TG) excitations. For this purpose, we introduce an experimental setup that exerts control of the spatial phase of subsequent time-delayed TG excitations depending on their polarization state. Specific exemplary coherent control cases are discussed theoretically and corresponding experimental data are presented in which time-resolved x-ray reflectivity measures the spatiotemporal surface distortion of nanolayered heterostructures. Finally, we discuss examples where the application of our method may enable the control of functional material properties via tailored spatiotemporal strain fields.},
  language  = {en}
}
@misc{MatternPudellDumesniletal.2023,
  author    = {Mattern, Maximilian and Pudell, Jan-Etienne and Dumesnil, Karine and Reppert, Alexander von and Bargheer, Matias},
  title     = {Towards shaping picosecond strain pulses via magnetostrictive transducers},
  series = {Zweitver{\"o}ffentlichungen der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe},
  journal   = {Zweitver{\"o}ffentlichungen der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe},
  number    = {1321},
  issn      = {1866-8372},
  doi       = {10.25932/publishup-58886},
  url       = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-588868},
  pages     = {7},
  year      = {2023},
  abstract  = {Using time-resolved x-ray diffraction, we demonstrate the manipulation of the picosecond strain response of a metallic heterostructure consisting of a dysprosium (Dy) transducer and a niobium (Nb) detection layer by an external magnetic field. We utilize the first-order ferromagnetic-antiferromagnetic phase transition of the Dy layer, which provides an additional large contractive stress upon laser excitation compared to its zerofield response. This enhances the laser-induced contraction of the transducer and changes the shape of the picosecond strain pulses driven in Dy and detected within the buried Nb layer. Based on our experiment with rare-earth metals we discuss required properties for functional transducers, which may allow for novel field-control of the emitted picosecond strain pulses.},
  language  = {en}
}