@article{SchaalRutlohWeidenfeldetal.2018, author = {Schaal, Frederik and Rutloh, Michael and Weidenfeld, Susanne and Stumpe, Joachim and Michler, Peter and Pruss, Christof and Osten, Wolfgang}, title = {Optically addressed modulator for tunable spatial polarization control}, series = {Optics express : the international electronic journal of optics}, volume = {26}, journal = {Optics express : the international electronic journal of optics}, number = {21}, publisher = {Optical Society of America}, address = {Washington}, issn = {1094-4087}, doi = {10.1364/OE.26.028119}, pages = {28119 -- 28130}, year = {2018}, abstract = {We present an optically addressed non-pixelated spatial light modulator. The system is based on reversible photoalignment of a LC cell using a red light sensitive novel azobenzene photoalignment layer. It is an electrode-free device that manipulates the liquid crystal orientation and consequently the polarization via light without artifacts caused by electrodes. The capability to miniaturize the spatial light modulator allows the integration into a microscope objective. This includes a miniaturized 200 channel optical addressing system based on a VCSEL array and hybrid refractive-diffractive beam shapers. As an application example, the utilization as a microscope objective integrated analog phase contrast modulator is shown. (C) 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement}, language = {en} } @article{SchmaelzlinMoralejoGersondeetal.2018, author = {Schm{\"a}lzlin, Elmar Gerd and Moralejo, Benito and Gersonde, Ingo and Schleusener, Johannes and Darvin, Maxim E. and Thiede, Gisela and Roth, Martin M.}, title = {Nonscanning large-area Raman imaging for ex vivo/in vivo skin cancer discrimination}, series = {Journal of biomedical optics}, volume = {23}, journal = {Journal of biomedical optics}, number = {10}, publisher = {SPIE}, address = {Bellingham}, issn = {1083-3668}, doi = {10.1117/1.JBO.23.10.105001}, pages = {11}, year = {2018}, abstract = {Imaging Raman spectroscopy can be used to identify cancerous tissue. Traditionally, a step-by-step scanning of the sample is applied to generate a Raman image, which, however, is too slow for routine examination of patients. By transferring the technique of integral field spectroscopy (IFS) from astronomy to Raman imaging, it becomes possible to record entire Raman images quickly within a single exposure, without the need for a tedious scanning procedure. An IFS-based Raman imaging setup is presented, which is capable of measuring skin ex vivo or in vivo. It is demonstrated how Raman images of healthy and cancerous skin biopsies were recorded and analyzed. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License.}, language = {en} } @article{RichterFoxWakkeretal.2018, author = {Richter, Philipp and Fox, Andrew J. and Wakker, Bart P. and Howk, J. Christopher and Lehner, Nicolas and Barger, Kathleen A. and Lockman, Felix J.}, title = {New constraints on the nature and origin of the leading arm of the magellanic stream}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {865}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aadd0f}, pages = {16}, year = {2018}, abstract = {We present a new precision measurement of gas-phase abundances of S, O, N, Si, Fe, P, Al, Ca as well as molecular hydrogen (H-2) in the Leading Arm (region II, LA II) of the Magellanic Stream (MS) toward the Seyfert galaxy NGC 3783. The results are based on high-quality archival ultraviolet/optical/radio data from various different instruments (HST/STIS, FUSE, AAT, GBT, GB140 ft, ATCA). Our study updates previous results from lower-resolution data and provides for the first time a self-consistent component model of the complex multiphase absorber, delivering important constraints on the nature and origin of LA II. We derive a uniform, moderate a abundance in the two main absorber groups at +245 and +190 km s(-1) of alpha/H = 0.30 +/- 0.05 solar, a low nitrogen abundance of N/H = 0.05 +/- 0.01 solar, and a high dust content with substantial dust depletion values for Si, Fe, Al, and Ca. These a, N, and dust abundances in LA II are similar to those observed in the Small Magellanic Cloud (SMC). From the analysis of the H2 absorption, we determine a high thermal pressure of P/k approximate to 1680 K cm(-3) in LA II, in line with the idea that LA II is located in the inner Milky Way halo at a z-height of < 20 kpc, where it hydrodynamically interacts with the ambient hot coronal gas. Our study supports a scenario in which LA II stems from the breakup of a metal- and dust-enriched progenitor cloud that was recently (200-500 Myr ago) stripped from the SMC.}, language = {en} } @article{ThapaWyłomańskaSikoraetal.2021, author = {Thapa, Samudrajit and Wyłomańska, Agnieszka and Sikora, Grzegorz and Wagner, Caroline E. and Krapf, Diego and Kantz, Holger and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Leveraging large-deviation statistics to decipher the stochastic properties of measured trajectories}, series = {New Journal of Physics}, volume = {23}, journal = {New Journal of Physics}, publisher = {Dt. Physikalische Ges. ; IOP}, address = {Bad Honnef ; London}, issn = {1367-2630}, doi = {10.1088/1367-2630/abd50e}, pages = {22}, year = {2021}, abstract = {Extensive time-series encoding the position of particles such as viruses, vesicles, or individualproteins are routinely garnered insingle-particle tracking experiments or supercomputing studies.They contain vital clues on how viruses spread or drugs may be delivered in biological cells.Similar time-series are being recorded of stock values in financial markets and of climate data.Such time-series are most typically evaluated in terms of time-averaged mean-squareddisplacements (TAMSDs), which remain random variables for finite measurement times. Theirstatistical properties are different for differentphysical stochastic processes, thus allowing us toextract valuable information on the stochastic process itself. To exploit the full potential of thestatistical information encoded in measured time-series we here propose an easy-to-implementand computationally inexpensive new methodology, based on deviations of the TAMSD from itsensemble average counterpart. Specifically, we use the upper bound of these deviations forBrownian motion (BM) to check the applicability of this approach to simulated and real data sets.By comparing the probability of deviations fordifferent data sets, we demonstrate how thetheoretical bound for BM reveals additional information about observed stochastic processes. Weapply the large-deviation method to data sets of tracer beads tracked in aqueous solution, tracerbeads measured in mucin hydrogels, and of geographic surface temperature anomalies. Ouranalysis shows how the large-deviation properties can be efficiently used as a simple yet effectiveroutine test to reject the BM hypothesis and unveil relevant information on statistical propertiessuch as ergodicity breaking and short-time correlations.}, language = {en} } @article{WolfGuehr2019, author = {Wolf, Thomas and G{\"u}hr, Markus}, title = {Photochemical pathways in nucleobases measured with an X-ray FEL}, series = {Philosophical Transactions of the Royal Society of London, Series A : Mathematical, Physical and Engineering Sciences}, volume = {377}, journal = {Philosophical Transactions of the Royal Society of London, Series A : Mathematical, Physical and Engineering Sciences}, number = {2145}, publisher = {Royal Society}, address = {London}, issn = {1364-503X}, doi = {10.1098/rsta.2017.0473}, pages = {12}, year = {2019}, abstract = {The conversion of light energy into other molecular energetic degrees of freedom is often dominated by ultrafast, non-adiabatic processes. Femtosecond spectroscopy with optical pulses has helped in shaping our understanding of crucial processes in molecular energy-conversion. The advent of new, ultrashort and bright X-ray free electron laser sources opens the possibility to use X-ray-typical element and site sensitivity for ultrafast molecular research. We present two types of spectroscopy, ultrafast Auger and ultrafast X-ray absorption spectroscopy, and discuss their sensitivity to molecular processes. While Auger spectroscopy is able to monitor bond distance changes in the vicinity of an X-ray created core hole, near-edge absorption spectroscopy can deliver high-fidelity information on non-adiabatic transitions involving lone-pair orbitals. We demonstrate these features on the example of the UV-excited nucleobase thymine, investigated at the oxygen K-edge. We find a C-O bond elongation in the Auger data in addition to pi pi*/n pi* non-adiabatic transition in X-ray near-edge absorption. We compare the results from both methods and draw a conclusive scenario of non-adiabatic molecular relaxation after UV excitation.}, language = {en} } @article{StangeHintscheSachseetal.2017, author = {Stange, Maike and Hintsche, Marius and Sachse, Kirsten and Gerhardt, Matthias and Valleriani, Angelo and Beta, Carsten}, title = {Analyzing the spatial positioning of nuclei in polynuclear giant cells}, series = {Journal of Physics D: Applied Physics}, volume = {50}, journal = {Journal of Physics D: Applied Physics}, number = {46}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0022-3727}, doi = {10.1088/1361-6463/aa8da0}, pages = {8}, year = {2017}, abstract = {How cells establish and maintain a well-defined size is a fundamental question of cell biology. Here we investigated to what extent the microtubule cytoskeleton can set a predefined cell size, independent of an enclosing cell membrane. We used electropulse-induced cell fusion to form giant multinuclear cells of the social amoeba Dictyostelium discoideum. Based on dual-color confocal imaging of cells that expressed fluorescent markers for the cell nucleus and the microtubules, we determined the subcellular distributions of nuclei and centrosomes in the giant cells. Our two- and three-dimensional imaging results showed that the positions of nuclei in giant cells do not fall onto a regular lattice. However, a comparison with model predictions for random positioning showed that the subcellular arrangement of nuclei maintains a low but still detectable degree of ordering. This can be explained by the steric requirements of the microtubule cytoskeleton, as confirmed by the effect of a microtubule degrading drug.}, language = {en} } @article{RobradeOskinovaSchmittetal.2018, author = {Robrade, Jan and Oskinova, Lida and Schmitt, J. H. M. M. and Leto, Paolo and Trigilio, C.}, title = {Outstanding X-ray emission from the stellar radio pulsar CU Virginis}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {619}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201833492}, pages = {6}, year = {2018}, abstract = {Context. Among the intermediate-mass magnetic chemically peculiar (MCP) stars, CU Vir is one of the most intriguing objects. Its 100\% circularly polarized beams of radio emission sweep the Earth as the star rotates, thereby making this strongly magnetic star the prototype of a class of nondegenerate stellar radio pulsars. While CU Vir is well studied in radio, its high-energy properties are not known. Yet, X-ray emission is expected from stellar magnetospheres and confined stellar winds. Aims. Using X-ray data we aim to test CU Vir for intrinsic X-ray emission and investigate mechanisms responsible for its generation. Methods. We present X-ray observations performed with XMM-Newton and Chandra and study obtained X-ray images, light curves, and spectra. Basic X-ray properties are derived from spectral modelling and are compared with model predictions. In this context we investigate potential thermal and nonthermal X-ray emission scenarios. Results. We detect an X-ray source at the position of CU Vir. With LX approximate to 3 x 10(28) erg s(-1) it is moderately X-ray bright, but the spectrum is extremely hard compared to other Ap stars. Spectral modelling requires multi-component models with predominant hot plasma at temperatures of about T-X = 25MK or, alternatively, a nonthermal spectral component. Both types of model provide a virtually equivalent description of the X-ray spectra. The Chandra observation was performed six years later than those by XMM-Newton, yet the source has similar X-ray flux and spectrum, suggesting a steady and persistent X-ray emission. This is further confirmed by the X-ray light curves that show only mild X-ray variability. Conclusions. CU Vir is also an exceptional star at X-ray energies. To explain its full X-ray properties, a generating mechanism beyond standard explanations, like the presence of a low-mass companion or magnetically confined wind-shocks, is required. Magnetospheric activity might be present or, as proposed for fast-rotating strongly magnetic Bp stars, the X-ray emission of CU Vir is predominantly auroral in nature.}, language = {en} } @article{ShenDierckeDenker2019, author = {Shen, Z. and Diercke, Andrea and Denker, Carsten}, title = {Calibration of full-disk He i 10 830 angstrom filtergrams of the Chromospheric Telescope}, series = {Astronomische Nachrichten = Astronomical notes}, volume = {339}, journal = {Astronomische Nachrichten = Astronomical notes}, number = {9-10}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0004-6337}, doi = {10.1002/asna.201813536}, pages = {661 -- 671}, year = {2019}, abstract = {The Chromospheric Telescope (ChroTel) is a small 10-cm robotic telescope at Observatorio del Teide on Tenerife (Spain), which observes the entire sun in Hα, Ca ii K, and He i 10 830 {\AA}. We present a new calibration method that includes limb-darkening correction, removal of nonuniform filter transmission, and determination of He i Doppler velocities. Chromospheric full-disk filtergrams are often obtained with Lyot filters, which may display nonuniform transmission causing large-scale intensity variations across the solar disk. Removal of a 2D symmetric limb-darkening function from full-disk images results in a flat background. However, transmission artifacts remain and are even more distinct in these contrast-enhanced images. Zernike polynomials are uniquely appropriate to fit these large-scale intensity variations of the background. The Zernike coefficients show a distinct temporal evolution for ChroTel data, which is likely related to the telescope's alt-azimuth mount that introduces image rotation. In addition, applying this calibration to sets of seven filtergrams that cover the He i triplet facilitates the determination of chromospheric Doppler velocities. To validate the method, we use three datasets with varying levels of solar activity. The Doppler velocities are benchmarked with respect to cotemporal high-resolution spectroscopic data of the GREGOR Infrared Spectrograph (GRIS). Furthermore, this technique can be applied to ChroTel Hα and Ca ii K data. The calibration method for ChroTel filtergrams can be easily adapted to other full-disk data exhibiting unwanted large-scale variations. The spectral region of the He i triplet is a primary choice for high-resolution near-infrared spectropolarimetry. Here, the improved calibration of ChroTel data will provide valuable context data.}, language = {en} } @article{RychkovAltafim2018, author = {Rychkov, Dmitry and Altafim, Ruy Alberto Pisani}, title = {Template-based fluoroethylenepropylene ferroelectrets with enhanced thermal stability of piezoelectricity}, series = {Journal of applied physics}, volume = {124}, journal = {Journal of applied physics}, number = {17}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-8979}, doi = {10.1063/1.5041374}, pages = {5}, year = {2018}, abstract = {In ferroelectrets, the piezoelectricity stems from the charges of both polarities trapped on the inner surfaces of the cavities in the material, so that its thermal stability is defined by the stability of the respective charges. In the present work, a template-based lamination technique has been employed to fabricate tubular-channel ferroelectrets from fluoroethylenepropylene (FEP) films. It has been shown that the piezoelectricity in FEP ferroelectrets decays at relatively low temperatures due to the inherently lower thermal stability of the positive charge. In order to improve charge trapping, we have treated both FEP films and inner surfaces of the ferroelectret cavities with titanium-tetrachloride vapor, using the atomic-layer-deposition technique. Using surface-potential-decay measurements on FEP films, we have found that the charge-decay curves shift by more than 100 degrees C to the higher temperatures as a result of the surface treatment. Direct measurements of piezoelectric d(33) coefficients as a function of temperature have shown that the piezoelectric stability is likewise improved with the d(33)-decay curves shifted by 60 degrees C to the right. The improvement of electret/ferroelectret properties can be attributed to the formation of the deeper traps on the chemically modified FEP surface. SEM micrographs and EDS analysis reveal island-like structures with titanium- and oxygen-containing species that can be responsible for the deeper trapping of the electret charges. Published by AIP Publishing.}, language = {en} } @article{SposiniChechkinMetzler2018, author = {Sposini, Vittoria and Chechkin, Aleksei V. and Metzler, Ralf}, title = {First passage statistics for diffusing diffusivity}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {52}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {4}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8121/aaf6ff}, pages = {11}, year = {2018}, abstract = {A rapidly increasing number of systems is identified in which the stochastic motion of tracer particles follows the Brownian law < r(2)(t)> similar or equal to Dt yet the distribution of particle displacements is strongly non-Gaussian. A central approach to describe this effect is the diffusing diffusivity (DD) model in which the diffusion coefficient itself is a stochastic quantity, mimicking heterogeneities of the environment encountered by the tracer particle on its path. We here quantify in terms of analytical and numerical approaches the first passage behaviour of the DD model. We observe significant modifications compared to Brownian-Gaussian diffusion, in particular that the DD model may have a faster first passage dynamics. Moreover we find a universal crossover point of the survival probability independent of the initial condition.}, language = {en} } @article{JonscherFlemmingSchmittetal.2018, author = {Jonscher, Ernst and Flemming, Sven and Schmitt, Marius and Sabitzki, Ricarda and Reichard, Nick and Birnbaum, Jakob and Bergmann, B{\"a}rbel and H{\"o}hn, Katharina and Spielmann, Tobias}, title = {PfVPS45 Is Required for Host Cell Cytosol Uptake by Malaria Blood Stage Parasites}, series = {Cell host \& microbe}, volume = {25}, journal = {Cell host \& microbe}, number = {1}, publisher = {Cell Press}, address = {Cambridge}, issn = {1931-3128}, doi = {10.1016/j.chom.2018.11.010}, pages = {166 -- 173}, year = {2018}, abstract = {During development in human erythrocytes, the malaria parasite Plasmodium falciparum internalizes a large part of the cellular content of the host cell. The internalized cytosol, consisting largely of hemoglobin, is transported to the parasite's food vacuole where it is degraded, providing nutrients and space for growth. This host cell cytosol uptake (HCCU) is crucial for parasite survival but the parasite proteins mediating this process remain obscure. Here, we identify P. falciparum VPS45 as an essential factor in HCCU. Conditional inactivation of PfVPS45 led to an accumulation of host cell cytosol-filled vesicles within the parasite and inhibited the delivery of hemoglobin to the parasite's digestive vacuole, resulting in arrested parasite growth. A proportion of these HCCU vesicle intermediates was positive for phosphatidylinositol 3-phosphate, suggesting endosomal characteristics. Thus PfVPS45 provides insight into the elusive machinery of the ingestion pathway in a parasite that contains an endolysosomal system heavily repurposed for protein secretion.}, language = {en} } @article{DybiecCapalaChechkinetal.2018, author = {Dybiec, Bartlomiej and Capala, Karol and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Conservative random walks in confining potentials}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {52}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8121/aaefc2}, pages = {25}, year = {2018}, abstract = {Levy walks are continuous time random walks with spatio-temporal coupling of jump lengths and waiting times, often used to model superdiffusive spreading processes such as animals searching for food, tracer motion in weakly chaotic systems, or even the dynamics in quantum systems such as cold atoms. In the simplest version Levy walks move with a finite speed. Here, we present an extension of the Levy walk scenario for the case when external force fields influence the motion. The resulting motion is a combination of the response to the deterministic force acting on the particle, changing its velocity according to the principle of total energy conservation, and random velocity reversals governed by the distribution of waiting times. For the fact that the motion stays conservative, that is, on a constant energy surface, our scenario is fundamentally different from thermal motion in the same external potentials. In particular, we present results for the velocity and position distributions for single well potentials of different steepness. The observed dynamics with its continuous velocity changes enriches the theory of Levy walk processes and will be of use in a variety of systems, for which the particles are externally confined.}, language = {en} } @article{XueLiuWangetal.2019, author = {Xue, Rui and Liu, Ruo-Yu and Wang, Xiang-Yu and Yan, Huirong and B{\"o}ttcher, Markus}, title = {On the minimum jet power of TeV BL Lac objects in the p-gamma model}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {871}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aaf720}, pages = {10}, year = {2019}, abstract = {We study the requirement of the jet power in the conventional p-gamma models (photopion production and Bethe-Heitler pair production) for TeV BL Lac objects. We select a sample of TeV BL Lac objects whose spectral energy distributions are difficult to explain by the one-zone leptonic model. Based on the relation between the p-gamma interaction efficiency and the opacity of gamma gamma absorption, we find that the detection of TeV emission poses upper limits on the p-gamma interaction efficiencies in these sources and hence minimum jet powers can be derived accordingly. We find that the obtained minimum jet powers exceed the Eddington luminosity of the supermassive black holes (SMBHs). Implications for the accretion mode of the SMBHs in these BL Lac objects and the origin of their TeV emissions are discussed.}, language = {en} } @article{LiuYanWangetal.2019, author = {Liu, Ruo-Yu and Yan, Huirong and Wang, Xiang-Yu and Shao, Shi and Li, Hui}, title = {Gamma-Ray production in the extended halo of the galaxy and possible implications for the origin of galactic cosmic rays}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {871}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aaf567}, pages = {11}, year = {2019}, abstract = {Various studies have implied the existence of a gaseous halo around the Galaxy extending out to similar to 100 kpc. Galactic cosmic rays (CRs) that propagate to the halo, either by diffusion or by convection with the possibly existing large-scale Galactic wind, can interact with the gas therein and produce gamma-rays via proton-proton collision. We calculate the CR distribution in the halo and the gamma-ray flux, and explore the dependence of the result on model parameters such as diffusion coefficient, CR luminosity, and CR spectral index. We find that the current measurement of isotropic gamma-ray background (IGRB) at less than or similar to TeV with the Fermi Large Area Telescope already approaches a level that can provide interesting constraints on the properties of Galactic CR (e.g., with CR luminosity L-CR <= 1041 erg s(-1)). We also discuss the possibilities of the Fermi bubble and IceCube neutrinos originating from the proton-proton collision between CRs and gas in the halo, as well as the implication of our results for the baryon budget of the hot circumgalactic medium of our Galaxy. Given that the isotropic gamma-ray background is likely to be dominated by unresolved extragalactic sources, future telescopes may extract more individual sources from the IGRB, and hence put even more stringent restrictions on the relevant quantities (such as Galactic CR luminosity and baryon budget in the halo) in the presence of a turbulent halo that we consider.}, language = {en} } @article{BaranOstensenTeltingetal.2018, author = {Baran, Andrzej S. and Ostensen, R. H. and Telting, J. H. and Vos, Joris and Kilkenny, D. and Vuckovic, Maja and Reed, M. D. and Silvotti, R. and Jeffery, C. Simon and Parsons, Steven G. and Dhillon, V. S. and Marsh, T. R.}, title = {Pulsations and eclipse-time analysis of HW Vir}, series = {Monthly notices of the Royal Astronomical Society}, volume = {481}, journal = {Monthly notices of the Royal Astronomical Society}, number = {2}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/sty2473}, pages = {2721 -- 2735}, year = {2018}, abstract = {We analysed recent K2 data of the short-period eclipsing binary system HW Vir, which consists of a hot subdwarf-B type primary with an M-dwarf companion. We determined the mid-times of eclipses, calculated O-C diagrams, and an average shift of the secondary minimum. Our results show that the orbital period is stable within the errors over the course of the 70 days of observations. Interestingly, the offset from mid-orbital phase between the primary and the secondary eclipses is found to be 1.62 s. If the shift is explained solely by light-travel time, the mass of the sdB primary must be 0.26 M-circle dot, which is too low for the star to be core-helium burning. However, we argue that this result is unlikely to be correct and that a number of effects caused by the relative sizes of the stars conspire to reduce the effective light-travel time measurement. After removing the flux variation caused by the orbit, we calculated the amplitude spectrum to search for pulsations. The spectrum clearly shows periodic signal from close to the orbital frequency up to 4600 mu Hz, with the majority of peaks found below 2600 mu Hz. The amplitudes are below 0.1 part-per-thousand, too low to be detected with ground-based photometry. Thus, the high-precision data from the Kepler spacecraft has revealed that the primary of the HW Vir system is a pulsating sdBV star. We argue that the pulsation spectrum of the primary in HW Vir differs from that in other sdB stars due to its relatively fast rotation that is (nearly) phase-locked with the orbit.}, language = {en} } @article{GajdaWylomanskaKantzetal.2018, author = {Gajda, J. and Wylomanska, Agnieszka and Kantz, Holger and Chechkin, Aleksei V. and Sikora, Grzegorz}, title = {Large deviations of time-averaged statistics for Gaussian processes}, series = {Statistics \& Probability Letters}, volume = {143}, journal = {Statistics \& Probability Letters}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0167-7152}, doi = {10.1016/j.spl.2018.07.013}, pages = {47 -- 55}, year = {2018}, abstract = {In this paper we study the large deviations of time averaged mean square displacement (TAMSD) for Gaussian processes. The theory of large deviations is related to the exponential decay of probabilities of large fluctuations in random systems. From the mathematical point of view a given statistics satisfies the large deviation principle, if the probability that it belongs to a certain range decreases exponentially. The TAMSD is one of the main statistics used in the problem of anomalous diffusion detection. Applying the theory of generalized chi-squared distribution and sub-gamma random variables we prove the upper bound for large deviations of TAMSD for Gaussian processes. As a special case we consider fractional Brownian motion, one of the most popular models of anomalous diffusion. Moreover, we derive the upper bound for large deviations of the estimator for the anomalous diffusion exponent. (C) 2018 Elsevier B.V. All rights reserved.}, language = {en} } @article{MardoukhiChechkinMetzler2020, author = {Mardoukhi, Yousof and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Spurious ergodicity breaking in normal and fractional Ornstein-Uhlenbeck process}, series = {New Journal of Physics}, volume = {22}, journal = {New Journal of Physics}, publisher = {IOP}, address = {London}, issn = {1367-2630}, doi = {10.1088/1367-2630/ab950b}, pages = {18}, year = {2020}, abstract = {The Ornstein-Uhlenbeck process is a stationary and ergodic Gaussian process, that is fully determined by its covariance function and mean. We show here that the generic definitions of the ensemble- and time-averaged mean squared displacements fail to capture these properties consistently, leading to a spurious ergodicity breaking. We propose to remedy this failure by redefining the mean squared displacements such that they reflect unambiguously the statistical properties of any stochastic process. In particular we study the effect of the initial condition in the Ornstein-Uhlenbeck process and its fractional extension. For the fractional Ornstein-Uhlenbeck process representing typical experimental situations in crowded environments such as living biological cells, we show that the stationarity of the process delicately depends on the initial condition.}, language = {en} } @article{MakuchBrilliantovSremcevicetal.2006, author = {Makuch, Martin and Brilliantov, Nikolai V. and Sremcevic, Miodrag and Spahn, Frank and Krivov, Alexander V.}, title = {Stochastic circumplanetary dynamics of rotating non-spherical dust particles}, series = {Planetary and space science}, volume = {54}, journal = {Planetary and space science}, number = {9-10}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-0633}, doi = {10.1016/j.pss.2006.05.006}, pages = {855 -- 870}, year = {2006}, abstract = {We develop a model of stochastic radiation pressure for rotating non-spherical particles and apply the model to circumplanetary dynamics of dust grains. The stochastic properties of the radiation pressure are related to the ensemble-averaged characteristics of the rotating particles, which are given in terms of the rotational time-correlation function of a grain. We investigate the model analytically and show that an ensemble of particle trajectories demonstrates a diffusion-like behaviour. The analytical results are compared with numerical simulations, performed for the motion of the dusty ejecta from Deimos in orbit around Mars. We find that the theoretical predictions are in a good agreement with the simulation results. The agreement however deteriorates at later time, when the impact of non-linear terms, neglected in the analytic approach, becomes significant. Our results indicate that the stochastic modulation of the radiation pressure can play an important role in the circumplanetary dynamics of dust and may in case of some dusty systems noticeably alter an optical depth. (c) 2006 Elsevier Ltd. All rights reserved.}, language = {en} } @article{BeckerPettiniRafelskietal.2019, author = {Becker, George D. and Pettini, Max and Rafelski, Marc and Boera, Elisa and Christensen, Lise and Cupani, Guido and Ellison, Sara L. and Farina, Emanuele Paolo and Fumagalli, Michele and Lopez, Sebastian and Neeleman, Marcel and Ryan-Weber, Emma and Worseck, Gabor}, title = {The Evolution of OI over 3.2 < z < 6.5: Reionization of the Circumgalactic Medium}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {883}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/ab3eb5}, pages = {37}, year = {2019}, abstract = {We present a survey for metal absorption systems traced by neutral oxygen over 3.2 < z < 6.5. Our survey uses Keck/ESI and VLT/X-Shooter spectra of 199 QSOs with redshifts up to 6.6. In total, we detect 74 OI absorbers, of which 57 are separated from the background QSO by more than 5000 km s(-1). We use a maximum likelihood approach to fit the distribution of OI lambda 1302 equivalent widths in bins of redshift and from this determine the evolution in number density of absorbers with W-1302 > 0.05 angstrom, of which there are 49 nonproximate systems in our sample. We find that the number density does not monotonically increase with decreasing redshift, as would naively be expected from the buildup of metal-enriched circumgalactic gas with time. The number density over 4.9 < z < 5.7 is a factor of 1.7-4.1 lower (68\% confidence) than that over 5.7 < z < 6.5, with a lower value at z < 5.7 favored with 99\% confidence. This decrease suggests that the fraction of metals in a low-ionization phase is larger at z similar to 6 than at lower redshifts. Absorption from highly ionized metals traced by CIV is also weaker in higher-redshift OI systems, supporting this picture. The evolution of OI absorbers implies that metal-enriched circumgalactic gas at z similar to 6 is undergoing an ionization transition driven by a strengthening ultraviolet background. This in turn suggests that the reionization of the diffuse intergalactic medium may still be ongoing at or only recently ended by this epoch.}, language = {en} } @article{WilkinParrishYangetal.2019, author = {Wilkin, Kyle J. and Parrish, Robert M. and Yang, Jie and Wolf, Thomas J. A. and Nunes, J. Pedro F. and G{\"u}hr, Markus and Li, Renkai and Shen, Xiaozhe and Zheng, Qiang and Wang, Xijie and Martinez, Todd J. and Centurion, Martin}, title = {Diffractive imaging of dissociation and ground-state dynamics in a complex molecule}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {100}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9926}, doi = {10.1103/PhysRevA.100.023402}, pages = {10}, year = {2019}, abstract = {We have investigated the structural dynamics in photoexcited 1,2-diiodotetrafluoroethane molecules (C2F4I2) in the gas phase experimentally using ultrafast electron diffraction and theoretically using FOMO-CASCI excited-state dynamics simulations. The molecules are excited by an ultraviolet femtosecond laser pulse to a state characterized by a transition from the iodine 5p perpendicular to orbital to a mixed 5p parallel to sigma hole and CF2 center dot antibonding orbital, which results in the cleavage of one of the carbon-iodine bonds. We have observed, with sub-Angstrom resolution, the motion of the nuclear wave packet of the dissociating iodine atom followed by coherent vibrations in the electronic ground state of the C2F4I radical. The radical reaches a stable classical (nonbridged) structure in less than 200 fs.}, language = {en} } @article{WolfParrishMyhreetal.2019, author = {Wolf, Thomas J. A. and Parrish, Robert M. and Myhre, Rolf H. and Martinez, Todd J. and Koch, Henrik and G{\"u}hr, Markus}, title = {Observation of Ultrafast Intersystem Crossing in Thymine by Extreme Ultraviolet Time-Resolved Photoelectron Spectroscopy}, series = {The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment \& general theory}, volume = {123}, journal = {The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment \& general theory}, number = {32}, publisher = {American Chemical Society}, address = {Washington}, issn = {1089-5639}, doi = {10.1021/acs.jpca.9b05573}, pages = {6897 -- 6903}, year = {2019}, abstract = {We studied the photoinduced ultrafast relaxation dynamics of the nucleobase thymine using gas-phase time-resolved photoelectron spectroscopy. By employing extreme ultraviolet pulses from high harmonic generation for photoionization, we substantially extend our spectral observation window with respect to previous studies. This enables us to follow relaxation of the excited state population all the way to low-lying electronic states including the ground state. In thymine, we observe relaxation from the optically bright (1)pi pi* state of thymine to a dark (1)n pi* state within 80 +/- 30 fs. The (1)n pi* state relaxes further within 3.5 +/- 0.3 ps to a low-lying electronic state. By comparison with quantum chemical simulations, we can unambiguously assign its spectroscopic signature to the (3)pi pi* state. Hence, our study draws a comprehensive picture of the relaxation mechanism of thymine including ultrafast intersystem crossing to the triplet manifold.}, language = {en} } @article{RinaldiFormisanoKappeletal.2019, author = {Rinaldi, G. and Formisano, M. and Kappel, David and Capaccioni, F. and Bockelee-Morvan, D. and Cheng, Y-C and Vincent, J-B and Deshapriya, P. and Arnold, G. and Capria, M. T. and Ciarniello, M. and De Sanctis, M. C. and Doose, L. and Erard, S. and Federico, C. and Filacchione, G. and Fink, U. and Leyrat, C. and Longobardo, A. and Magni, G. and Mighorini, A. and Mottola, S. and Naletto, G. and Raponi, A. and Taylor, F. and Tosi, F. and Tozzi, G. P. and Salatti, M.}, title = {Analysis of night-side dust activity on comet 67P observed by VIRTIS-M}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {630}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201834907}, pages = {16}, year = {2019}, abstract = {On 2015 July 18, near perihelion at a heliocentric distance of 1.28 au, the Visible InfraRed Thermal Imaging Spectrometer (VIRTIS-M) on board the Rosetta spacecraft had the opportunity of observing dust activity in the inner coma with a view of the night side (shadowed side) of comet 67P/Churyumov-Gerasimenko. At the time of the measurements we present here, we observe a dust plume that originates on the far side of the nucleus. We are able to identify the approximate location of its source at the boundary between the Hapi and Anuket regions, and we find that it has been in darkness for some hours before the observation. Assuming that this time span is equal to the conductive time scale, we obtain a thermal inertia in the range 25-36 W K-1 m(-2) s(-1/2). These thermal inertia values can be used to verify with a 3D finite-element method (REM) numerical code whether the surface and subsurface temperatures agree with the values found in the literature. We explored three different configurations: (1) a layer of water ice mixed with dust beneath a dust mantle of 5 mm with thermal inertia of 36 J m(-2) K-1 S-0.5 ; (2) the same structure, but with thermal inertia of 100 J m(-2) K-1 S-0.5; (3) an ice-dust mixture that is directly exposed. Of these three configurations, the first seems to be the most reasonable, both for the low thermal inertia and for the agreement with the surface and subsurface temperatures that have been found for the comet 67P/Churyumov-Gerasimenko. The spectral properties of the plume show that the visible dust color ranged from 16 +/- 4.8\%/100 nm to 13 +/- 2.6\%/100 nm, indicating that this plume has no detectable color gradient. The morphology of the plume can be classified as a narrow jet that has an estimated total ejected mass of between 6 and 19 tons when we assume size distribution indices between -2.5 and -3.}, language = {en} } @article{TubianaRinaldiGuettleretal.2019, author = {Tubiana, C. and Rinaldi, G. and Guettler, C. and Snodgrass, C. and Shi, X. and Hu, X. and Marschall, R. and Fulle, M. and Bockeele-Morvan, D. and Naletto, G. and Capaccioni, F. and Sierks, H. and Arnold, G. and Barucci, M. A. and Bertaux, J-L and Bertini, I and Bodewits, D. and Capria, M. T. and Ciarniello, M. and Cremonese, G. and Crovisier, J. and Da Deppo, V and Debei, S. and De Cecco, M. and Deller, J. and De Sanctis, M. C. and Davidsson, B. and Doose, L. and Erard, S. and Filacchione, G. and Fink, U. and Formisano, M. and Fornasier, S. and Gutierrez, P. J. and Ip, W-H and Ivanovski, S. and Kappel, David and Keller, H. U. and Kolokolova, L. and Koschny, D. and Krueger, H. and La Forgia, F. and Lamy, P. L. and Lara, L. M. and Lazzarin, M. and Levasseur-Regourd, A. C. and Lin, Z-Y and Longobardo, A. and Lopez-Moreno, J. J. and Marzari, F. and Migliorini, A. and Mottola, S. and Rodrigo, R. and Taylor, F. and Toth, I and Zakharov, V}, title = {Diurnal variation of dust and gas production in comet 67P/Churyumov-Gerasimenko at the inbound equinox as seen by OSIRIS and VIRTIS-M on board Rosetta}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {630}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201834869}, pages = {14}, year = {2019}, abstract = {Context. On 27 April 2015, when comet 67P/Churyumov-Gerasimenko was at 1.76 au from the Sun and moving toward perihelion, the OSIRIS and VIRTIS-M instruments on board the Rosetta spacecraft simultaneously observed the evolving dust and gas coma during a complete rotation of the comet. Aims. We aim to characterize the spatial distribution of dust, H2O, and CO2 gas in the inner coma. To do this, we performed a quantitative analysis of the release of dust and gas and compared the observed H2O production rate with the rate we calculated using a thermophysical model. Methods. For this study we selected OSIRIS WAC images at 612 nm (dust) and VIRTIS-M image cubes at 612 nm, 2700 nm (H2O emission band), and 4200 nm (CO2 emission band). We measured the average signal in a circular annulus to study the spatial variation around the comet, and in a sector of the annulus to study temporal variation in the sunward direction with comet rotation, both at a fixed distance of 3.1 km from the comet center. Results. The spatial correlation between dust and water, both coming from the sunlit side of the comet, shows that water is the main driver of dust activity in this time period. The spatial distribution of CO2 is not correlated with water and dust. There is no strong temporal correlation between the dust brightness and water production rate as the comet rotates. The dust brightness shows a peak at 0 degrees subsolar longitude, which is not pronounced in the water production. At the same epoch, there is also a maximum in CO2 production. An excess of measured water production with respect to the value calculated using a simple thermophysical model is observed when the head lobe and regions of the southern hemisphere with strong seasonal variations are illuminated (subsolar longitude 270 degrees-50 degrees). A drastic decrease in dust production when the water production (both measured and from the model) displays a maximum occurs when typical northern consolidated regions are illuminated and the southern hemisphere regions with strong seasonal variations are instead in shadow (subsolar longitude 50 degrees-90 degrees). Possible explanations of these observations are presented and discussed.}, language = {en} } @article{BaranTeltingJefferyetal.2019, author = {Baran, Andrzej S. and Telting, J. H. and Jeffery, C. Simon and Ostensen, R. H. and Vos, Joris and Reed, M. D. and Vŭcković, Maja}, title = {K2 observations of the sdBV plus dM/bd binaries PHL457 and EQPsc}, series = {Monthly notices of the Royal Astronomical Society}, volume = {489}, journal = {Monthly notices of the Royal Astronomical Society}, number = {2}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stz2209}, pages = {1556 -- 1571}, year = {2019}, abstract = {We present an analysis of two pulsating subdwarf B stars PHL 457 and EQ Psc observed during the K2 mission. The K2 light curves of both stars show variation consistent with irradiation of a cooler companion by the hot subdwarf. They also show higher frequency oscillations consistent with pulsation. Using new spectroscopic data, we measured the radial velocity, effective temperature, surface gravity, and helium abundance of both hot subdwarfs as a function of orbital phase. We confirm the previously published spectroscopic orbit of PHL 457, and present the first spectroscopic orbit of EQ Psc. The orbital periods are 0.313 and 0.801 d, respectively. For EQPsc, we find a strong correlation between T-eff and orbital phase, due to contribution of light from the irradiated companion. We calculated amplitude spectra, identified significant pulsation frequencies, and searched for multiplets and asymptotic period spacings. By means of multiplets and period spacing, we identified the degrees of several pulsation modes in each star. The g-mode multiplets indicate subsynchronous core rotation with periods of 4.6 d (PHL 457) and 9.4 d (EQ Psc). We made spectral energy disctribution (SED) fits of PHL 457 and EQ Psc using available broad-band photometry and Gaia data. While the SED of PHL 457 shows no evidence of a cool companion, the SED for EQPsc clearly shows an infrared (IR) access consistent with a secondary with a temperature of about 6800K and a radius of 0.23 R-circle dot. This is the first detection of an IR access in any sdB + dM binary.}, language = {en} } @article{EliazarMetzlerReuveni2019, author = {Eliazar, Iddo and Metzler, Ralf and Reuveni, Shlomi}, title = {Poisson-process limit laws yield Gumbel max-min and min-max}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {100}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {2470-0045}, doi = {10.1103/PhysRevE.100.022129}, pages = {12}, year = {2019}, abstract = {"A chain is only as strong as its weakest link" says the proverb. But what about a collection of statistically identical chains: How long till all chains fail? The answer to this question is given by the max-min of a matrix whose (i,j)entry is the failure time of link j of chain i: take the minimum of each row, and then the maximum of the rows' minima. The corresponding min-max is obtained by taking the maximum of each column, and then the minimum of the columns' maxima. The min-max applies to the storage of critical data. Indeed, consider multiple backup copies of a set of critical data items, and consider the (i,j) matrix entry to be the time at which item j on copy i is lost; then, the min-max is the time at which the first critical data item is lost. In this paper we address random matrices whose entries are independent and identically distributed random variables. We establish Poisson-process limit laws for the row's minima and for the columns' maxima. Then, we further establish Gumbel limit laws for the max-min and for the min-max. The limit laws hold whenever the entries' distribution has a density, and yield highly applicable approximation tools and design tools for the max-min and min-max of large random matrices. A brief of the results presented herein is given in: Gumbel central limit theorem for max-min and min-max}, language = {en} } @article{EliazarMetzlerReuveni2019, author = {Eliazar, Iddo and Metzler, Ralf and Reuveni, Shlomi}, title = {Gumbel central limit theorem for max-min and min-max}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {100}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {2470-0045}, doi = {10.1103/PhysRevE.100.020104}, pages = {6}, year = {2019}, abstract = {The max-min and min-max of matrices arise prevalently in science and engineering. However, in many real-world situations the computation of the max-min and min-max is challenging as matrices are large and full information about their entries is lacking. Here we take a statistical-physics approach and establish limit laws—akin to the central limit theorem—for the max-min and min-max of large random matrices. The limit laws intertwine random-matrix theory and extreme-value theory, couple the matrix dimensions geometrically, and assert that Gumbel statistics emerge irrespective of the matrix entries' distribution. Due to their generality and universality, as well as their practicality, these results are expected to have a host of applications in the physical sciences and beyond.}, language = {en} } @article{PoeschelBrilliantovFormella2006, author = {Poeschel, Thorsten and Brilliantov, Nikolai V. and Formella, Arno}, title = {Impact of high-energy tails on granular gas properties}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {74}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {4}, publisher = {The American Physical Society}, address = {College Park}, issn = {1539-3755}, doi = {10.1103/PhysRevE.74.041302}, pages = {5}, year = {2006}, abstract = {The velocity distribution function of granular gases in the homogeneous cooling state as well as some heated granular gases decays for large velocities as f proportional to exp(-const x nu). That is, its high-energy tail is overpopulated as compared with the Maxwell distribution. At the present time, there is no theory to describe the influence of the tail on the kinetic characteristics of granular gases. We develop an approach to quantify the overpopulated tail and analyze its impact on granular gas properties, in particular on the cooling coefficient. We observe and explain anomalously slow relaxation of the velocity distribution function to its steady state.}, language = {en} } @article{BaptistaGrebogiKoberle2006, author = {Baptista, Murilo da Silva and Grebogi, Celso and Koberle, Roland}, title = {Dynamically multilayered visual system of the multifractal fly}, series = {Physical review letters}, volume = {97}, journal = {Physical review letters}, number = {17}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.97.178102}, pages = {4}, year = {2006}, language = {en} } @article{HamannGraefenerLiermann2006, author = {Hamann, Wolf-Rainer and Graefener, G. and Liermann, A.}, title = {The galactic WN stars - Spectral analyses with line-blanketed model atmospheres versus stellar evolution models with and without rotation}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {457}, journal = {Astronomy and astrophysics : an international weekly journal}, number = {3}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361:20065052}, pages = {1015 -- 1031}, year = {2006}, abstract = {Context. Very massive stars pass through the Wolf-Rayet (WR) stage before they finally explode. Details of their evolution have not yet been safely established, and their physics are not well understood. Their spectral analysis requires adequate model atmospheres, which have been developed step by step during the past decades and account in their recent version for line blanketing by the millions of lines from iron and iron-group elements. However, only very few WN stars have been re-analyzed by means of line-blanketed models yet. Aims. The quantitative spectral analysis of a large sample of Galactic WN stars with the most advanced generation of model atmospheres should provide an empirical basis for various studies about the origin, evolution, and physics of the Wolf-Rayet stars and their powerful winds. Methods. We analyze a large sample of Galactic WN stars by means of the Potsdam Wolf-Rayet (PoWR) model atmospheres, which account for iron line blanketing and clumping. The results are compared with a synthetic population, generated from the Geneva tracks for massive star evolution. Results. We obtain a homogeneous set of stellar and atmospheric parameters for the GalacticWN stars, partly revising earlier results. Conclusions. Comparing the results of our spectral analyses of the Galactic WN stars with the predictions of the Geneva evolutionary calculations, we conclude that there is rough qualitative agreement. However, the quantitative discrepancies are still severe, and there is no preference for the tracks that account for the effects of rotation. It seems that the evolution of massive stars is still not satisfactorily understood.}, language = {en} } @article{ZaikinKurths2006, author = {Zaikin, Alexey and Kurths, J{\"u}rgen}, title = {Optimal length transportation hypothesis to model proteasome product size distribution}, series = {Journal of biological physics : emphasizing physical principles in biological research ; an international journal for the formulation and application of mathematical models in the biological sciences}, volume = {32}, journal = {Journal of biological physics : emphasizing physical principles in biological research ; an international journal for the formulation and application of mathematical models in the biological sciences}, number = {3-4}, publisher = {Springer}, address = {Dordrecht}, issn = {0092-0606}, doi = {10.1007/s10867-006-9014-z}, pages = {231 -- 243}, year = {2006}, abstract = {This paper discusses translocation features of the 20S proteasome in order to explain typical proteasome length distributions. We assume that the protein transport depends significantly on the fragment length with some optimal length which is transported most efficiently. By means of a simple one-channel model, we show that this hypothesis can explain both the one- and the three-peak length distributions found in experiments. A possible mechanism of such translocation is provided by so-called fluctuation-driven transport.}, language = {en} } @article{DierckeKuckeinDenker2019, author = {Diercke, Andrea and Kuckein, Christoph and Denker, Carsten}, title = {Dynamics and connectivity of an extended arch filament system}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {629}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201935583}, pages = {14}, year = {2019}, abstract = {Aims. In this study, we analyzed a filament system, which expanded between moving magnetic features (MMFs) of a decaying sunspot and opposite flux outside of the active region from the nearby quiet-Sun network. This configuration deviated from a classical arch filament system (AFS), which typically connects two pores in an emerging flux region. Thus, we called this system an extended AFS. We contrasted classical and extended AFSs with an emphasis on the complex magnetic structure of the latter. Furthermore, we examined the physical properties of the extended AFS and described its dynamics and connectivity. Methods. The extended AFS was observed with two instruments at the Dunn Solar Telescope (DST). The Rapid Oscillations in the Solar Atmosphere (ROSA) imager provided images in three different wavelength regions, which covered the dynamics of the extended AFS at different atmospheric heights. The Interferometric Bidimensional Spectropolarimeter (IBIS) provided spectroscopic Ha data and spectropolarimetric data that was obtained in the near-infrared (NIR) Call lambda 8542 angstrom line. We derived the corresponding line-of-sight (LOS) velocities and used He II lambda 304 angstrom extreme ultraviolet (EUV) images of the Atmospheric Imaging Assembly (AIA) and LOS magnetograms of the Helioseismic and Magnetic Imager (HMI) on board the Solar Dynamics Observatory (SDO) as context data. Results. The NIR Call Stokes-V maps are not suitable to definitively define a clear polarity inversion line and to classify this chromospheric structure. Nevertheless, this unusual AFS connects the MMFs of a decaying sunspot with the network field. At the southern footpoint, we measured that the flux decreases over time. We find strong downflow velocities at the footpoints of the extended AFS, which increase in a time period of 30 min. The velocities are asymmetric at both footpoints with higher velocities at the southern footpoint. An EUV brigthening appears in one of the arch filaments, which migrates from the northern footpoint toward the southern one. This activation likely influences the increasing redshift at the southern footpoint. Conclusions. The extended AFS exhibits a similar morphology as classical AFSs, for example, threaded filaments of comparable length and width. Major differences concern the connection from MMFs around the sunspot with the flux of the neighboring quietSun network, converging footpoint motions, and longer lifetimes of individual arch filaments of about one hour, while the extended AFS is still very dynamic.}, language = {en} } @article{SahaOwenOrretal.2019, author = {Saha, Sourav and Owen, Lewis A. and Orr, Elizabeth N. and Caffee, Marc W.}, title = {High-frequency Holocene glacier fluctuations in the Himalayan-Tibetan orogen}, series = {Quaternary science reviews : the international multidisciplinary research and review journal}, volume = {220}, journal = {Quaternary science reviews : the international multidisciplinary research and review journal}, publisher = {Elsevier}, address = {Oxford}, issn = {0277-3791}, doi = {10.1016/j.quascirev.2019.07.021}, pages = {372 -- 400}, year = {2019}, abstract = {Holocene glacial chronostratigraphies in glaciated valleys spread throughout the Himalayan-Tibetan orogen, including the Himalaya, Tibet, Pamir, and Tian Shan, are developed using a landsystems approach, detailed geomorphic mapping, and new and published Be-10 surface exposure dating. New studies in the Kulti valley of Lahul and the Parkachik valley of the Nun Kun massif of the Himalaya of northern India define three glacier advances at similar to 14.7, 12.2, 0.5 ka, in addition to one historically dated late 19th Century advance in the Kulti valley, and one Late Holocene advance at similar to 0.2 ka in the Parkachik valley. Three major climatic groups (subdivided into five climatic zones) are defined across the orogen using Cluster Analysis (CA) and Principal Component Analysis (PCA) to identify glaciated regions with comparable climatic characteristics to evaluate the timing, and extent of Holocene glacier advances across these regions. Our regional analyses across the Himalayan-Tibetan orogen suggest at least one Lateglacial (similar to 15.3-11.8 ka) and five Himalayan-Tibetan Holocene glacial stages (HTHS) at similar to 11.5-9.5, similar to 8.8-7.7, similar to 7.0-3.2, similar to 2.3-1.0, and <1 ka. The extent (amplitude) of glacier advances in 77 glaciated valleys is reconstructed and defined using equilibrium-line altitudes (ELAs). Modern glacier hypsometries are also assessed to help explain the intra-regional variations in glacier amplitudes during each regional glacier advance. A linear inverse glacier flow model is used to decipher the net changes in temperature (Delta T) between periods of reconstructed regional glacier advances in 66 glaciated valleys across different climatic regions throughout the orogen. The Be-10, ELAs, and Delta T data suggest enhanced monsoonal and increased precipitation during the Early Holocene, followed by relative cooling and increased aridity during the Mid- and Late Holocene that influenced glaciation. The sublimation-dominated cold-based glaciers in the northern regions of Himalayan-Tibetan orogen are more affected during these shifts in climate than the temperate glaciers in the south. (C) 2019 Elsevier Ltd. All rights reserved.}, language = {en} } @article{LiuYanZhang2019, author = {Liu, Ruo-Yu and Yan, Huirong and Zhang, Heshou}, title = {Role of Anisotropic Diffusion of Particles}, series = {Physical review letters}, volume = {123}, journal = {Physical review letters}, number = {22}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.123.221103}, pages = {5}, year = {2019}, abstract = {In this Letter, we propose that the x-ray and the TeV observations in the vicinity of Geminga can be understood in the framework of anisotropic diffusion of injected electrons or positrons. This interpretation only requires the turbulence in the vicinity of Geminga to be sub-Alfvenic with the local mean magnetic field direction approximately aligned with our line of sight towards Geminga, without invoking extreme conditions for the environment, such as an extremely small diffusion coefficient and a weak magnetic field of submicrogauss as suggested in previous literature.}, language = {en} } @article{LeverRamelowGuehr2019, author = {Lever, Fabiano and Ramelow, Sven and G{\"u}hr, Markus}, title = {Effects of time-energy correlation strength in molecular entangled photon spectroscopy}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {100}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {5}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9926}, doi = {10.1103/PhysRevA.100.053844}, pages = {6}, year = {2019}, abstract = {In this paper, we explore the time-energy domain quantum-classical transition comparing a classical pump-probe experiment on a diatomic molecule to its quantum enhanced counterpart, where the pump and probe pulses are substituted by the signal and idler beams of a spontaneous parametric down conversion (SPDC) source. Absorption of biphotons generated with SPDC exploits quantum time-energy entanglement to enhance the overall yield and selectivity of the process, when compared with a classical pump-probe setup, while maintaining femtosecond time resolution. We systematically study the effects of correlation strength on process efficiency and selectivity, comparing the results to classical pump-probe spectra. An excitation scheme to improve the yield based on spectral narrowing of biphotons is shown. The results indicate that the quantum improvements in yield are caused by a more efficient use of the total power available for the process.}, language = {en} } @article{BerrahSanchezGonzalezJureketal.2019, author = {Berrah, N. and S{\´a}nchez-Gonz{\´a}lez, {\´A}lvaro and Jurek, Zoltan and Obaid, Razib and Xiong, H. and Squibb, R. J. and Osipov, T. and Lutman, A. and Fang, L. and Barillot, T. and Bozek, J. D. and Cryan, J. and Wolf, T. J. A. and Rolles, Daniel and Coffee, R. and Schnorr, Kirsten and Augustin, S. and Fukuzawa, Hironobu and Motomura, K. and Niebuhr, Nina Isabelle and Frasinski, L. J. and Feifel, Raimund and Schulz, Claus-Peter and Toyota, Kenji and Son, Sang-Kil and Ueda, K. and Pfeifer, T. and Marangos, J. P. and Santra, Robin}, title = {Femtosecond-resolved observation of the fragmentation of buckminsterfullerene following X-ray multiphoton ionization}, series = {Nature physics}, volume = {15}, journal = {Nature physics}, number = {12}, publisher = {Nature Publ. Group}, address = {London}, issn = {1745-2473}, doi = {10.1038/s41567-019-0665-7}, pages = {1279 -- 1301}, year = {2019}, abstract = {X-ray free-electron lasers have, over the past decade, opened up the possibility of understanding the ultrafast response of matter to intense X-ray pulses. In earlier research on atoms and small molecules, new aspects of this response were uncovered, such as rapid sequences of inner-shell photoionization and Auger ionization. Here, we studied a larger molecule, buckminsterfullerene (C-60), exposed to 640 eV X-rays, and examined the role of chemical effects, such as chemical bonds and charge transfer, on the fragmentation following multiple ionization of the molecule. To provide time resolution, we performed femtosecond-resolved X-ray pump/X-ray probe measurements, which were accompanied by advanced simulations. The simulations and experiment reveal that despite substantial ionization induced by the ultrashort (20 fs) X-ray pump pulse, the fragmentation of C-60 is considerably delayed. This work uncovers the persistence of the molecular structure of C-60, which hinders fragmentation over a timescale of hundreds of femtoseconds. Furthermore, we demonstrate that a substantial fraction of the ejected fragments are neutral carbon atoms. These findings provide insights into X-ray free-electron laser-induced radiation damage in large molecules, including biomolecules.}, language = {en} } @article{RuedigerSchultz2019, author = {R{\"u}diger, G{\"u}nther and Schultz, M.}, title = {Non-diffusive angular momentum transport in rotating z-pinches}, series = {Journal of plasma physics}, volume = {85}, journal = {Journal of plasma physics}, number = {6}, publisher = {Cambridge Univ. Press}, address = {New York}, issn = {0022-3778}, doi = {10.1017/S0022377819000606}, pages = {16}, year = {2019}, abstract = {The stability of conducting Taylor-Couette flows under the presence of toroidal magnetic background fields is considered. For strong enough magnetic amplitudes such magnetohydrodynamic flows are unstable against non-axisymmetric perturbations which may also transport angular momentum. In accordance with the often used diffusion approximation, one expects the angular momentum transport to be vanishing for rigid rotation. In the sense of a non-diffusive Lambda effect, however, even for rigidly rotating z-pinches, an axisymmetric angular momentum flux appears which is directed outward (inward) for large (small) magnetic Mach numbers. The internal rotation in a magnetized rotating tank can thus never be uniform. Those particular rotation laws are used to estimate the value of the instability-induced eddy viscosity for which the non-diffusive Lambda effect and the diffusive shear-induced transport compensate each other. The results provide the Shakura \& Sunyaev viscosity ansatz leading to numerical values linearly growing with the applied magnetic field.}, language = {en} } @article{SchroetterBoucheZabletal.2019, author = {Schroetter, Ilane and Bouche, Nicolas F. and Zabl, Johannes and Contini, Thierry and Wendt, Martin and Schaye, Joop and Mitchell, Peter and Muzahid, Sowgat and Marino, Raffaella Anna and Bacon, Roland and Lilly, Simon J. and Richard, Johan and Wisotzki, Lutz}, title = {MusE GAs FLOw andWind (MEGAFLOW)}, series = {Monthly notices of the Royal Astronomical Society}, volume = {490}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stz2822}, pages = {4368 -- 4381}, year = {2019}, abstract = {We present results from our on-going MusE GAs FLOw and Wind (MEGAFLOW) survey, which consists of 22 quasar lines of sight, each observed with the integral field unit MUSE and the UVES spectrograph at the ESO Very Large Telescopes (VLT). The goals of this survey are to study the properties of the circumgalactic medium around z similar to 1 star-forming galaxies. The absorption-line selected survey consists of 79 strong MgII absorbers (with rest-frame equivalent width greater than or similar to 0.3 angstrom) and, currently, 86 associated galaxies within 100 projected kpc of the quasar with stellar masses (M-star) from 109 to 1011 M-circle dot. We find that the cool halo gas traced by MgII is not isotropically distributed around these galaxies from the strong bi-modal distribution in the azimuthal angle of the apparent location of the quasar with respect to the galaxy major axis. This supports a scenario in which outflows are bi-conical in nature and co-exist with a co-planar gaseous structure extending at least up to 60-80 kpc. Assuming that absorbers near the minor axis probe outflows, the current MEGAFLOW sample allowed us to select 26 galaxy-quasar pairs suitable for studying winds. From this sample, using a simple geometrical model, we find that the outflow velocity only exceeds the escape velocity when M-star less than or similar to 4 x 10(9) M-circle dot, implying the cool material is likely to fall back except in the smallest haloes. Finally, we find that the mass loading factor., the ratio between the ejected mass rate and the star formation rate, appears to be roughly constant with respect to the galaxy mass.}, language = {en} } @article{PetitgirardSpiekermannGlazyrinetal.2019, author = {Petitgirard, Sylvain and Spiekermann, Georg and Glazyrin, Konstantin and Garrevoet, Jan and Murakami, Motohiko}, title = {Density of amorphous GeO2 to 133 GPa with possible pyritelike structure and stiffness at high pressure}, series = {Physical review : B, Condensed matter and materials physics}, volume = {100}, journal = {Physical review : B, Condensed matter and materials physics}, number = {21}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9950}, doi = {10.1103/PhysRevB.100.214104}, pages = {8}, year = {2019}, abstract = {Germanium oxide is a prototype network-forming oxide with pressure-induced structural changes similar to those found in crystals and amorphous silicate oxides at high pressure. Studying density and coordination changes in amorphous GeO2 allows for insight into structural changes in silicate oxides at very high pressure, with implications for the properties of planetary magmas. Here, we report the density of germanium oxide glass up to 133 GPa using the x-ray absorption technique, with very good agreement with previous experimental data at pressure below 40 GPa and recent calculation up to 140 GPa. Our data highlight four distinct compressibility domains, corresponding to changes of the local structure of GeO2. Above 80 GPa, our density data show a compressibility and bulk modulus similar to the counterpart crystal phase, and we propose that a compact distorted sixfold coordination, similar to the structural motif of the pyritelike crystalline GeO2 polymorph, is likely to be stable in that pressure range. Our density data point to a smooth continuous evolution of the average coordination for pressure above 20 GPa with persistent sixfold coordination, without sharp density or density slope discontinuities. These observations are in very good agreement with theoretical calculations and spectroscopic measurements, and our results indicate that glasses and melts may behave similarly to their high-pressure solid counterparts with comparable densities, compressibility, and possibly average coordination.}, language = {en} } @article{KrapfMetzler2019, author = {Krapf, Diego and Metzler, Ralf}, title = {Strange interfacial molecular dynamics}, series = {Physics today}, volume = {72}, journal = {Physics today}, number = {9}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0031-9228}, doi = {10.1063/PT.3.4294}, pages = {48 -- 54}, year = {2019}, language = {en} } @article{TeichmannRosenblum2019, author = {Teichmann, Erik and Rosenblum, Michael}, title = {Solitary states and partial synchrony in oscillatory ensembles with attractive and repulsive interactions}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {29}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {9}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/1.5118843}, pages = {11}, year = {2019}, abstract = {We numerically and analytically analyze transitions between different synchronous states in a network of globally coupled phase oscillators with attractive and repulsive interactions. The elements within the attractive or repulsive group are identical, but natural frequencies of the groups differ. In addition to a synchronous two-cluster state, the system exhibits a solitary state, when a single oscillator leaves the cluster of repulsive elements, as well as partially synchronous quasiperiodic dynamics. We demonstrate how the transitions between these states occur when the repulsion starts to prevail over attraction.}, language = {en} } @article{MeyerKreplinKrausetal.2019, author = {Meyer, Dominique M.-A. and Kreplin, Alexander and Kraus, S. and Vorobyov, E. I. and Haemmerl{\´e}, Lionel and Eisl{\"o}ffel, Jochen}, title = {On the ALMA observability of nascent massive multiple systems formed by gravitational instability}, series = {Monthly notices of the Royal Astronomical Society}, volume = {487}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stz1585}, pages = {4473 -- 4491}, year = {2019}, abstract = {Massive young stellar objects (MYSOs) form during the collapse of high-mass pre-stellar cores, where infalling molecular material is accreted through a centrifugally balanced accretion disc that is subject to efficient gravitational instabilities. In the resulting fragmented accretion disc of the MYSO, gaseous clumps and low-mass stellar companions can form, which will influence the future evolution of massive protostars in the Hertzsprung-Russell diagram. We perform dust continuum radiative transfer calculations and compute synthetic images of disc structures modelled by the gravito-radiation-hydrodynamics simulation of a forming MYSO, in order to investigate the Atacama Large Millimeter/submillimeter Array (alma) observability of circumstellar gaseous clumps and forming multiple systems. Both spiral arms and gaseous clumps located at similar or equal to a few from the protostar can be resolved by interferometric alma Cycle 7 C43-8 and C43-10 observations at band 6 (), using a maximal 0.015 aracsec beam angular resolution and at least exposure time for sources at distances of . Our study shows that substructures are observable regardless of their viewing geometry or can be inferred in the case of an edge-viewed disc. The observation probability of the clumps increases with the gradually increasing efficiency of gravitational instability at work as the disc evolves. As a consequence, large discs around MYSOs close to the zero-age-main-sequence line exhibit more substructures than at the end of the gravitational collapse. Our results motivate further observational campaigns devoted to the close surroundings of the massive protostars S255IR-NIRS3 and NGC 6334I-MM1, whose recent outbursts are a probable signature of disc fragmentation and accretion variability.}, language = {en} } @article{NivenAbelSchlegeletal.2019, author = {Niven, Robert K. and Abel, Markus and Schlegel, Michael and Waldrip, Steven H.}, title = {Maximum Entropy Analysis of Flow Networks: Theoretical Foundation and Applications}, series = {Entropy}, volume = {21}, journal = {Entropy}, number = {8}, publisher = {MDPI}, address = {Basel}, issn = {1099-4300}, doi = {10.3390/e21080776}, pages = {776}, year = {2019}, abstract = {The concept of a "flow network"-a set of nodes and links which carries one or more flows-unites many different disciplines, including pipe flow, fluid flow, electrical, chemical reaction, ecological, epidemiological, neurological, communications, transportation, financial, economic and human social networks. This Feature Paper presents a generalized maximum entropy framework to infer the state of a flow network, including its flow rates and other properties, in probabilistic form. In this method, the network uncertainty is represented by a joint probability function over its unknowns, subject to all that is known. This gives a relative entropy function which is maximized, subject to the constraints, to determine the most probable or most representative state of the network. The constraints can include "observable" constraints on various parameters, "physical" constraints such as conservation laws and frictional properties, and "graphical" constraints arising from uncertainty in the network structure itself. Since the method is probabilistic, it enables the prediction of network properties when there is insufficient information to obtain a deterministic solution. The derived framework can incorporate nonlinear constraints or nonlinear interdependencies between variables, at the cost of requiring numerical solution. The theoretical foundations of the method are first presented, followed by its application to a variety of flow networks.}, language = {en} } @article{SeilerSeissHoffmannetal.2019, author = {Seiler, Michael and Seiß, Martin and Hoffmann, Holger and Spahn, Frank}, title = {Hydrodynamic Simulations of Asymmetric Propeller Structures in Saturn's Rings}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Supplement series}, volume = {243}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Supplement series}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0067-0049}, doi = {10.3847/1538-4365/ab26b0}, pages = {16}, year = {2019}, abstract = {The observation of the non-Keplerian behavior of propeller structures in Saturn's outer A ring raises the question: how does the propeller respond to the wandering of the central embedded moonlet? Here, we study numerically how the structural imprint of the propeller changes for a libration of the moonlet. It turns out that the libration induces an asymmetry in the propeller, which depends on the libration period and amplitude of the moonlet. Further, we study the dependence of the asymmetry on the libration period and amplitude for a moonlet with a 400 m Hill radius, which is located in the outer A ring. This allows us to apply our findings to the largest known propeller Bl{\´e}riot, which is expected to be of a similar size. For Bl{\´e}riot, we can conclude that, supposing the moonlet is librating with the largest observed period of 11.1 yr and an azimuthal amplitude of about 1845 km, a small asymmetry should be measurable but depends on the moonlet's libration phase at the observation time. The longitude residuals of other trans-Encke propellers (e.g., Earhart) show amplitudes similar to Bl{\´e}riot, which might allow us to observe larger asymmetries due to their smaller azimuthal extent, allowing us to scan the whole gap structure for asymmetries in one observation. Although the librational model of the moonlet is a simplification, our results are a first step toward the development of a consistent model for the description of the formation of asymmetric propellers caused by a freely moving moonlet.}, language = {en} } @article{RichterVollhardt2006, author = {Richter, Lothar and Vollhardt, Dieter}, title = {Force measuring methods for determination of surface tension of liquids: A comparison}, series = {Tenside, surfactants, detergents}, volume = {43}, journal = {Tenside, surfactants, detergents}, number = {5}, publisher = {Hanser}, address = {M{\"u}nchen}, issn = {0932-3414}, doi = {10.3139/113.100314}, pages = {256 -- 261}, year = {2006}, abstract = {Three methods for the determination of the surface tension of liquids based on force measurements namely, the vertical plate method of Wilhelmy, the frame method of Lenard and the ring method of du Nouy are compared and studied in respect of a common principle of correction. It is shown that these three most important force-based methods allow the determination of the surface tension under static conditions. The force components of the corresponding liquid column below the measuring wire obtained for the straight part of the withdrawal curve up to the transition in its curved part provides exact surface tension values. The experimentally accessible value of the force component describes the physical background of the measured value correction contrary to the approximate equations obtained by mathematical way. Usually the determination of surface tension of liquids is based merely at the vertical plate method on exact equations thermodynamically derived whereas in the case of the frame and ring methods correction factors in approximate equations are used. At usual application of the force-based methods under the non-static condition of the withdrawal of a liquid column, the force maximum measured at withdrawal of the measuring object (plate, frame, or ring) is the basis for the determination of surface tension. In these cases, the measured surface tension values are compensated by correction equations for the frame and ring methods which are based on an correction factor and correction tables empirically obtained. The surface tension values obtained in this usual way agree with those obtained by using the force component of the corresponding liquid column below the measuring wire for the straight part of the withdrawal curve up to the transition in its curved part. Problems arising at the force measurements with increasing thickness of the measuring wires inside and outside the rings are discussed.}, language = {en} } @article{AssmannThielRomanoetal.2006, author = {Assmann, Birte and Thiel, Marco and Romano, Maria Carmen and Niemitz, Carsten}, title = {Recurrence plot analyses suggest a novel reference system involved in newborn spontaneous movements}, series = {Behavior research methods : a journal of the Psychonomic Society}, volume = {38}, journal = {Behavior research methods : a journal of the Psychonomic Society}, number = {3}, publisher = {Springer}, address = {New York}, issn = {1554-351X}, doi = {10.3758/BF03192793}, pages = {400 -- 406}, year = {2006}, abstract = {The movements of newborns have been thoroughly studied in terms of reflexes, muscle synergies, leg coordination, and target-directed arm/hand movements. Since these approaches have concentrated mainly on separate accomplishments, there has remained a clear need for more integrated investigations. Here, we report an inquiry in which we explicitly concentrated on taking such a perspective and, additionally, were guided by the methodological concept of home base behavior, which Ilan Golard developed for studies of exploratory behavior in animals. Methods from nonlinear dynamics, such as symbolic dynamics and recurrence plot analyses of kinematic data received from audiovisual newborn recordings, yielded new insights into the spatial and temporal organization of limb movements. In the framework of home base behavior, our approach uncovered a novel reference system of spontaneous newborn movements.}, language = {en} } @article{DiezTauerSchulz2006, author = {Diez, Isabel and Tauer, Klaus and Schulz, Burkhard}, title = {Unusual polymer dispersions-polypyrrole suspensions made of rings, frames, and platelets}, series = {Colloid and polymer science : official journal of the Kolloid-Gesellschaft}, volume = {284}, journal = {Colloid and polymer science : official journal of the Kolloid-Gesellschaft}, publisher = {Springer}, address = {New York}, issn = {0303-402X}, doi = {10.1007/s00396-006-1521-8}, pages = {1431 -- 1442}, year = {2006}, abstract = {Experimental results show that the polymerization of pyrrole in the presence of beta-naphthalenesulfonic acid and different fluorosurfactants like perfluorooctanesulfonic acid, perfluorooctyldiethanolamide, and ammonium perfluorooctanoate leads to polypyrrole with special morphologies, such as rings or disks and rectangular frames or plates. The formation of these unusually shaped particles of polymer dispersions is explained by the chemical and colloidal peculiarities of the oxidative pyrrole polymerization with ammonium peroxodisulfate in aqueous medium.}, language = {en} } @article{GiesersKamannDreizleretal.2019, author = {Giesers, Benjamin David and Kamann, Sebastian and Dreizler, Stefan and Husser, Tim-Oliver and Askar, Abbas and G{\"o}ttgens, Fabian and Brinchmann, Jarle and Latour, Marilyn and Weilbacher, Peter Michael and Wendt, Martin and Roth, Martin M.}, title = {A stellar census in globular clusters with MUSE: Binaries in NGC 3201}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {632}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201936203}, pages = {20}, year = {2019}, abstract = {We utilise multi-epoch MUSE spectroscopy to study binary stars in the core of the Galactic globular cluster NGC 3201. Our sample consists of 3553 stars with 54 883 spectra in total comprising 3200 main-sequence stars up to 4 magnitudes below the turn-off. Each star in our sample has between 3 and 63 (with a median of 14) reliable radial velocity measurements within five years of observations. We introduce a statistical method to determine the probability of a star showing radial velocity variations based on the whole inhomogeneous radial velocity sample. Using HST photometry and an advanced dynamical MOCCA simulation of this specific cluster we overcome observational biases that previous spectroscopic studies had to deal with. This allows us to infer a binary frequency in the MUSE field of view and enables us to deduce the underlying true binary frequency of (6.75 +/- 0.72)\% in NGC 3201. The comparison of the MUSE observations with the MOCCA simulation suggests a large portion of primordial binaries. We can also confirm a radial increase in the binary fraction towards the cluster centre due to mass segregation. We discovered that in the core of NGC 3201 at least (57.5 +/- 7.9)\% of blue straggler stars are in a binary system. For the first time in a study of globular clusters, we were able to fit Keplerian orbits to a significant sample of 95 binaries. We present the binary system properties of eleven blue straggler stars and the connection to SX Phoenicis-type stars. We show evidence that two blue straggler formation scenarios, the mass transfer in binary (or triple) star systems and the coalescence due to binary-binary interactions, are present in our data. We also describe the binary and spectroscopic properties of four sub-subgiant (or red straggler) stars. Furthermore, we discovered two new black hole candidates with minimum masses (M sin i) of (7.68 +/- 0.50)M-circle dot, (4.4 +/- 2.8)M-circle dot, and refine the minimum mass estimate on the already published black hole to (4.53 +/- 0.21)M-circle dot, These black holes are consistent with an extensive black hole subsystem hosted by NGC 3201.}, language = {en} } @article{LatourHusserGiesersetal.2019, author = {Latour, Marlyn and Husser, Tim Oliver and Giesers, Benjamin David and Kamann, S. and G{\"o}ttgens, Fabian and Dreizler, Stefan and Brinchmann, Jan and Bastian, Nate and Wendt, Martin and Weilbacher, Peter Michael and Molinski, N. S.}, title = {A stellar census in globular clusters with MUSE: multiple populations chemistry in NGC 2808 star star star}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {631}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201936242}, pages = {14}, year = {2019}, abstract = {Context. Galactic globular clusters (GCs) are now known to host multiple populations displaying particular abundance variations. The different populations within a GC can be well distinguished following their position in the pseudo two-colors diagrams, also referred to as "chromosome maps". These maps are constructed using optical and near-UV photometry available from the Hubble Space Telescope (HST) UV survey of GCs. However, the chemical tagging of the various populations in the chromosome maps is hampered by the fact that HST photometry and elemental abundances are both only available for a limited number of stars. Aims. The spectra collected as part of the MUSE survey of globular clusters provide a spectroscopic counterpart to the HST photometric catalogs covering the central regions of GCs. In this paper, we use the MUSE spectra of 1115 red giant branch (RGB) stars in NGC 2808 to characterize the abundance variations seen in the multiple populations of this cluster. Methods. We used the chromosome map of NGC 2808 to divide the RGB stars into their respective populations. We then combined the spectra of all stars belonging to a given population, resulting in one high signal-to-noise ratio spectrum representative of each population. Results. Variations in the spectral lines of O, Na, Mg, and Al are clearly detected among four of the populations. In order to quantify these variations, we measured equivalent width differences and created synthetic populations spectra that were used to determine abundance variations with respect to the primordial population of the cluster. Our results are in good agreement with the values expected from previous studies based on high-resolution spectroscopy. We do not see any significant variations in the spectral lines of Ca, K, and Ba. We also do not detect abundance variations among the stars belonging to the primordial population of NGC 2808. Conclusions. We demonstrate that in spite of their low resolution, the MUSE spectra can be used to investigate abundance variations in the context of multiple populations.}, language = {en} } @article{FoxRichterAshleyetal.2019, author = {Fox, Andrew J. and Richter, Philipp and Ashley, Trisha and Heckman, Timothy M. and Lehner, Nicolas and Werk, Jessica K. and Bordoloi, Rongmon and Peeples, Molly S.}, title = {The Mass Inflow and Outflow Rates of the Milky Way}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {884}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/ab40ad}, pages = {7}, year = {2019}, abstract = {We present new calculations of the mass inflow and outflow rates around the Milky Way (MW), derived from a catalog of ultraviolet metal-line high-velocity clouds (HVCs). These calculations are conducted by transforming the HVC velocities into the Galactic standard of rest (GSR) reference frame, identifying inflowing (vGSR.<.0 km s(-1)) and outflowing (vGSR > 0 km s(-1)) populations, and using observational constraints on the distance, metallicity, dust content, covering fractions, and total silicon column density of each population. After removing HVCs associated with the Magellanic Stream and the Fermi Bubbles, we find inflow and outflow rates in cool (T similar to 10(4) K) ionized gas of dM(in)/dt greater than or similar to.(0.53 +/- 0.23)(d/12 kpc)(Z/0.2Z(circle dot))-1M(circle dot) yr(-1) and dM(out)/dt greater than or similar to (0.16 +/- 0.07)(d/12 kpc)(Z/0.5Z(circle dot))M--1(circle dot) yr(-1). The apparent excess of inflowing over outflowing gas suggests that the MW is currently in an inflow-dominated phase, but the presence of substantial mass flux in both directions supports a Galactic fountain model, in which gas is constantly recycled between the disk and the halo. We also find that the metal flux in both directions (in and out) is indistinguishable. By comparing the outflow rate to the Galactic star formation rate, we present the first estimate of the mass loading factor (eta(HVC)) of the disk-wide MW wind, finding eta(HVC) greater than or similar to (0.10 +/- 0.06)(d/12 kpc)(Z/0.5Z(circle dot))(-1). Including the contributions from low- and intermediatevelocity clouds and from hot gas would increase these inflow and outflow estimates.}, language = {en} } @article{MeiKochovskiRoaetal.2019, author = {Mei, Shilin and Kochovski, Zdravko and Roa, Rafael and Gu, Sasa and Xu, Xiaohui and Yu, Hongtao and Dzubiella, Joachim and Ballauff, Matthias and Lu, Yan}, title = {Enhanced Catalytic Activity of Gold@Polydopamine Nanoreactors with Multi-compartment Structure Under NIR Irradiation}, series = {Nano-Micro Letters}, volume = {11}, journal = {Nano-Micro Letters}, number = {1}, publisher = {Shanghai JIAO TONG univ press}, address = {Shanghai}, issn = {2311-6706}, doi = {10.1007/s40820-019-0314-9}, pages = {16}, year = {2019}, abstract = {Photothermal conversion (PTC) nanostructures have great potential for applications in many fields, and therefore, they have attracted tremendous attention. However, the construction of a PTC nanoreactor with multi-compartment structure to achieve the combination of unique chemical properties and structural feature is still challenging due to the synthetic difficulties. Herein, we designed and synthesized a catalytically active, PTC gold (Au)@polydopamine (PDA) nanoreactor driven by infrared irradiation using assembled PS-b-P2VP nanosphere as soft template. The particles exhibit multi-compartment structure which is revealed by 3D electron tomography characterization technique. They feature permeable shells with tunable shell thickness. Full kinetics for the reduction reaction of 4-nitrophenol has been investigated using these particles as nanoreactors and compared with other reported systems. Notably, a remarkable acceleration of the catalytic reaction upon near-infrared irradiation is demonstrated, which reveals for the first time the importance of the synergistic effect of photothermal conversion and complex inner structure to the kinetics of the catalytic reduction. The ease of synthesis and fresh insights into catalysis will promote a new platform for novel nanoreactor studies.}, language = {en} } @article{SahaOwenOrretal.2019, author = {Saha, Sourav and Owen, Lewis A. and Orr, Elizabeth N. and Caffee, Marc W.}, title = {Cosmogenic Be-10 and equilibrium-line altitude dataset of Holocene glacier advances in the Himalayan-Tibetan orogen}, series = {Data in brief}, volume = {26}, journal = {Data in brief}, publisher = {Elsevier}, address = {Amsterdam}, issn = {2352-3409}, doi = {10.1016/j.dib.2019.104412}, pages = {13}, year = {2019}, abstract = {A comprehensive analysis of the variable temporal and spatial responses of tropical-subtropical high-altitude glaciers to climate change is critical for successful model predictions and environmental risk assessment in the Himalayan-Tibetan orogen. High-frequency Holocene glacier chronostratigraphies are therefore reconstructed in 79 glaciated valleys across the orogen using 519 published and 16 new terrestrial cosmogenic 10Be exposure age dataset. Published 10Be ages are compiled only for moraine boulders (excluding bedrock ages). These ages are recalculated using the latest ICE-D production rate calibration database and the scaling scheme models. Outliers for the individual moraine are detected using the Chauvenet's criterion. In addition, past equilibrium-line altitudes (ELAs) are determined using the area-altitude (AA), area accumulation ratio (AAR), and toe-headwall accumulation ratio (THAR) methods for each glacier advance. The modern maximum elevations of lateral moraines (MELM) are also used to estimate modern ELAs and as an independent check on mean ELAs derived using the above three methods. These data may serve as an essential archive for future studies focusing on the cryospheric and environmental changes in the Himalayan-Tibetan orogen. A more comprehensive analysis of the published and new 10Be ages and ELA results and a list of references are presented in Saha et al. (2019, High-frequency Holocene glacier fluctuations in the Himalayan-Tibetan orogen. Quaternary Science Reviews, 220, 372-400).}, language = {en} } @article{TeomyMetzler2019, author = {Teomy, Eial and Metzler, Ralf}, title = {Transport in exclusion processes with one-step memory: density dependence and optimal acceleration}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {52}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {38}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8121/ab37e4}, pages = {19}, year = {2019}, abstract = {We study a lattice gas of persistent walkers, in which each site is occupied by at most one particle and the direction each particle attempts to move to depends on its last step. We analyse the mean squared displacement (MSD) of the particles as a function of the particle density and their persistence (the tendency to continue moving in the same direction). For positive persistence the MSD behaves as expected: it increases with the persistence and decreases with the density. However, for strong anti-persistence we find two different regimes, in which the dependence of the MSD on the density is non-monotonic. For very strong anti-persistence there is an optimal density at which the MSD reaches a maximum. In an intermediate regime, the MSD as a function of the density exhibits both a minimum and a maximum, a phenomenon which has not been observed before. We derive a mean-field theory which qualitatively explains this behaviour.}, language = {en} } @article{PalyulinBlackburnLomholtetal.2019, author = {Palyulin, Vladimir V. and Blackburn, George and Lomholt, Michael A. and Watkins, Nicholas W. and Metzler, Ralf and Klages, Rainer and Chechkin, Aleksei V.}, title = {First passage and first hitting times of Levy flights and Levy walks}, series = {New journal of physics : the open-access journal for physics}, volume = {21}, journal = {New journal of physics : the open-access journal for physics}, number = {10}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/ab41bb}, pages = {23}, year = {2019}, abstract = {For both L{\´e}vy flight and L{\´e}vy walk search processes we analyse the full distribution of first-passage and first-hitting (or first-arrival) times. These are, respectively, the times when the particle moves across a point at some given distance from its initial position for the first time, or when it lands at a given point for the first time. For L{\´e}vy motions with their propensity for long relocation events and thus the possibility to jump across a given point in space without actually hitting it ('leapovers'), these two definitions lead to significantly different results. We study the first-passage and first-hitting time distributions as functions of the L{\´e}vy stable index, highlighting the different behaviour for the cases when the first absolute moment of the jump length distribution is finite or infinite. In particular we examine the limits of short and long times. Our results will find their application in the mathematical modelling of random search processes as well as computer algorithms.}, language = {en} } @article{TeomyMetzler2019, author = {Teomy, Eial and Metzler, Ralf}, title = {Correlations and transport in exclusion processes with general finite memory}, series = {Journal of statistical mechanics: theory and experiment}, volume = {2019}, journal = {Journal of statistical mechanics: theory and experiment}, number = {10}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1742-5468}, doi = {10.1088/1742-5468/ab47fb}, pages = {31}, year = {2019}, language = {en} } @article{Lewandowski2022, author = {Lewandowski, Max}, title = {Hadamard states for bosonic quantum field theory on globally hyperbolic spacetimes}, series = {Journal of mathematical physics}, volume = {63}, journal = {Journal of mathematical physics}, number = {1}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0022-2488}, doi = {10.1063/5.0055753}, pages = {34}, year = {2022}, abstract = {According to Radzikowski's celebrated results, bisolutions of a wave operator on a globally hyperbolic spacetime are of the Hadamard form iff they are given by a linear combination of distinguished parametrices i2(G˜aF-G˜F+G˜A-G˜R) in the sense of Duistermaat and H{\"o}rmander [Acta Math. 128, 183-269 (1972)] and Radzikowski [Commun. Math. Phys. 179, 529 (1996)]. Inspired by the construction of the corresponding advanced and retarded Green operator GA, GR as done by B{\"a}r, Ginoux, and Pf{\"a}ffle {Wave Equations on Lorentzian Manifolds and Quantization [European Mathematical Society (EMS), Z{\"u}rich, 2007]}, we construct the remaining two Green operators GF, GaF locally in terms of Hadamard series. Afterward, we provide the global construction of i2(G˜aF-G˜F), which relies on new techniques such as a well-posed Cauchy problem for bisolutions and a patching argument using Čech cohomology. This leads to global bisolutions of the Hadamard form, each of which can be chosen to be a Hadamard two-point-function, i.e., the smooth part can be adapted such that, additionally, the symmetry and the positivity condition are exactly satisfied.}, language = {en} } @article{KurzkeKietheHeueretal.2017, author = {Kurzke, Henning and Kiethe, Jan and Heuer, Axel and Jechow, Andreas}, title = {Frequency doubling of incoherent light from a superluminescent diode in a periodically poled lithium niobate waveguide crystal}, series = {Laser physics letters}, volume = {14}, journal = {Laser physics letters}, publisher = {IOP Publ.}, address = {Bristol}, issn = {1612-2011}, doi = {10.1088/1612-202X/aa6889}, pages = {5}, year = {2017}, abstract = {The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a relatively broad spectral bandwidth and thermal-like photon statistics, as the measured degree of second order coherence, g((2))(0)= 1.9 +/- 0.1, indicates. Despite the non-optimized scenario in the spectral domain, we achieve six orders of magnitude higher conversion efficiency than previously reported with truly incoherent light. This is possible by using single spatial mode radiation and quasi phase matched material with a waveguide architecture. This work is a principle step towards efficient frequency conversion of temporally incoherent radiation in one spatial mode to access wavelengths where no radiation from superluminescent diodes is available, especially with tailored quasi phase matched crystals. The frequency doubled light might find application in imaging, metrology and quantum optics experiments.}, language = {en} } @article{KamannHusserDreizleretal.2017, author = {Kamann, Sebastian and Husser, T. -O. and Dreizler, S. and Emsellem, E. and Weilbacher, Peter Michael and Martens, S. and Bacon, R. and den Brok, M. and Giesers, B. and Krajnovic, Davor and Roth, Martin M. and Wendt, Martin and Wisotzki, Lutz}, title = {A stellar census in globular clusters with MUSE}, series = {Monthly notices of the Royal Astronomical Society}, volume = {473}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stx2719}, pages = {5591 -- 5616}, year = {2017}, abstract = {This is the first of a series of papers presenting the results from our survey of 25 Galactic globular clusters with the MUSE integral-field spectrograph. In combination with our dedicated algorithm for source deblending, MUSE provides unique multiplex capabilities in crowded stellar fields and allows us to acquire samples of up to 20 000 stars within the half-light radius of each cluster. The present paper focuses on the analysis of the internal dynamics of 22 out of the 25 clusters, using about 500 000 spectra of 200 000 individual stars. Thanks to the large stellar samples per cluster, we are able to perform a detailed analysis of the central rotation and dispersion fields using both radial profiles and two-dimensional maps. The velocity dispersion profiles we derive show a good general agreement with existing radial velocity studies but typically reach closer to the cluster centres. By comparison with proper motion data, we derive or update the dynamical distance estimates to 14 clusters. Compared to previous dynamical distance estimates for 47 Tuc, our value is in much better agreement with other methods. We further find significant (>3 sigma) rotation in the majority (13/22) of our clusters. Our analysis seems to confirm earlier findings of a link between rotation and the ellipticities of globular clusters. In addition, we find a correlation between the strengths of internal rotation and the relaxation times of the clusters, suggesting that the central rotation fields are relics of the cluster formation that are gradually dissipated via two-body relaxation.}, language = {en} } @article{MarschallSkorovZakharovetal.2020, author = {Marschall, Raphael and Skorov, Yuri and Zakharov, Vladimir and Rezac, Ladislav and Gerig, Selina-Barbara and Christou, Chariton and Dadzie, S. Kokou and Migliorini, Alessandra and Rinaldi, Giovanna and Agarwal, Jessica and Vincent, Jean-Baptiste and Kappel, David}, title = {Cometary comae-surface links the physics of gas and dust from the surface to a spacecraft}, series = {Space science reviews}, volume = {216}, journal = {Space science reviews}, number = {8}, publisher = {Springer}, address = {Dordrecht}, issn = {0038-6308}, doi = {10.1007/s11214-020-00744-0}, pages = {53}, year = {2020}, abstract = {A comet is a highly dynamic object, undergoing a permanent state of change. These changes have to be carefully classified and considered according to their intrinsic temporal and spatial scales. The Rosetta mission has, through its contiguous in-situ and remote sensing coverage of comet 67P/Churyumov-Gerasimenko (hereafter 67P) over the time span of August 2014 to September 2016, monitored the emergence, culmination, and winding down of the gas and dust comae. This provided an unprecedented data set and has spurred a large effort to connect in-situ and remote sensing measurements to the surface. In this review, we address our current understanding of cometary activity and the challenges involved when linking comae data to the surface. We give the current state of research by describing what we know about the physical processes involved from the surface to a few tens of kilometres above it with respect to the gas and dust emission from cometary nuclei. Further, we describe how complex multidimensional cometary gas and dust models have developed from the Halley encounter of 1986 to today. This includes the study of inhomogeneous outgassing and determination of the gas and dust production rates. Additionally, the different approaches used and results obtained to link coma data to the surface will be discussed. We discuss forward and inversion models and we describe the limitations of the respective approaches. The current literature suggests that there does not seem to be a single uniform process behind cometary activity. Rather, activity seems to be the consequence of a variety of erosion processes, including the sublimation of both water ice and more volatile material, but possibly also more exotic processes such as fracture and cliff erosion under thermal and mechanical stress, sub-surface heat storage, and a complex interplay of these processes. Seasons and the nucleus shape are key factors for the distribution and temporal evolution of activity and imply that the heliocentric evolution of activity can be highly individual for every comet, and generalisations can be misleading.}, language = {en} } @article{RousseauErardBecketal.2018, author = {Rousseau, Batiste and Erard, St{\´e}phane and Beck, P. and Quirico, Eric and Schmitt, B. and Brissaud, O. and Montes-Hernandez, G. and Capaccioni, F. and Filacchione, Gianrico and Bockelee-Morvan, Dominique and Leyrat, C. and Ciarniello, M. and Raponi, Andrea and Kappel, David and Arnold, G. and Moroz, L. V. and Palomba, Ernesto and Tosi, Federico}, title = {Laboratory simulations of the Vis-NIR spectra of comet 67P using sub-mu m sized cosmochemical analogues}, series = {Icarus : international journal of solar system studies}, volume = {306}, journal = {Icarus : international journal of solar system studies}, publisher = {Elsevier}, address = {San Diego}, organization = {VIRTIS Team}, issn = {0019-1035}, doi = {10.1016/j.icarus.2017.10.015}, pages = {306 -- 318}, year = {2018}, abstract = {Laboratory spectral measurements of relevant analogue materials were performed in the framework of the Rosetta mission in order to explain the surface spectral properties of comet 67P. Fine powders of coal, iron sulphides, silicates and their mixtures were prepared and their spectra measured in the Vis-IR range. These spectra are compared to a reference spectrum of 67P nucleus obtained with the VIRTIS/Rosetta instrument up to 2.7 mu m, excluding the organics band centred at 3.2 mu m. The species used are known to be chemical analogues for cometary materials which could be present at the surface of 67P. Grain sizes of the powders range from tens of nanometres to hundreds of micrometres. Some of the mixtures studied here actually reach the very low reflectance level observed by VIRTIS on 67P. The best match is provided by a mixture of sub-micron coal, pyrrhotite, and silicates. Grain sizes are in agreement with the sizes of the dust particles detected by the GIADA, MIDAS and COSIMA instruments on board Rosetta. The coal used in the experiment is responsible for the spectral slope in the visible and infrared ranges. Pyrrhotite, which is strongly absorbing, is responsible for the low albedo observed in the NIR. The darkest components dominate the spectra, especially within intimate mixtures. Depending on sample preparation, pyrrhotite can coat the coal and silicate aggregates. Such coating effects can affect the spectra as much as particle size. In contrast, silicates seem to play a minor role. (c) 2017 Elsevier Inc. All rights reserved.}, language = {en} } @article{HouCherstvyMetzleretal.2018, author = {Hou, Ru and Cherstvy, Andrey G. and Metzler, Ralf and Akimoto, Takuma}, title = {Biased continuous-time random walks for ordinary and equilibrium cases}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {20}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {32}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c8cp01863d}, pages = {20827 -- 20848}, year = {2018}, abstract = {We examine renewal processes with power-law waiting time distributions (WTDs) and non-zero drift via computing analytically and by computer simulations their ensemble and time averaged spreading characteristics. All possible values of the scaling exponent alpha are considered for the WTD psi(t) similar to 1/t(1+alpha). We treat continuous-time random walks (CTRWs) with 0 < alpha < 1 for which the mean waiting time diverges, and investigate the behaviour of the process for both ordinary and equilibrium CTRWs for 1 < alpha < 2 and alpha > 2. We demonstrate that in the presence of a drift CTRWs with alpha < 1 are ageing and non-ergodic in the sense of the non-equivalence of their ensemble and time averaged displacement characteristics in the limit of lag times much shorter than the trajectory length. In the sense of the equivalence of ensemble and time averages, CTRW processes with 1 < alpha < 2 are ergodic for the equilibrium and non-ergodic for the ordinary situation. Lastly, CTRW renewal processes with alpha > 2-both for the equilibrium and ordinary situation-are always ergodic. For the situations 1 < alpha < 2 and alpha > 2 the variance of the diffusion process, however, depends on the initial ensemble. For biased CTRWs with alpha > 1 we also investigate the behaviour of the ergodicity breaking parameter. In addition, we demonstrate that for biased CTRWs the Einstein relation is valid on the level of the ensemble and time averaged displacements, in the entire range of the WTD exponent alpha.}, language = {en} } @article{CherstvyThapaMardoukhietal.2018, author = {Cherstvy, Andrey G. and Thapa, Samudrajit and Mardoukhi, Yousof and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Time averages and their statistical variation for the Ornstein-Uhlenbeck process}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {98}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {2470-0045}, doi = {10.1103/PhysRevE.98.022134}, pages = {15}, year = {2018}, abstract = {How ergodic is diffusion under harmonic confinements? How strongly do ensemble- and time-averaged displacements differ for a thermally-agitated particle performing confined motion for different initial conditions? We here study these questions for the generic Ornstein-Uhlenbeck (OU) process and derive the analytical expressions for the second and fourth moment. These quantifiers are particularly relevant for the increasing number of single-particle tracking experiments using optical traps. For a fixed starting position, we discuss the definitions underlying the ensemble averages. We also quantify effects of equilibrium and nonequilibrium initial particle distributions onto the relaxation properties and emerging nonequivalence of the ensemble- and time-averaged displacements (even in the limit of long trajectories). We derive analytical expressions for the ergodicity breaking parameter quantifying the amplitude scatter of individual time-averaged trajectories, both for equilibrium and outof-equilibrium initial particle positions, in the entire range of lag times. Our analytical predictions are in excellent agreement with results of computer simulations of the Langevin equation in a parabolic potential. We also examine the validity of the Einstein relation for the ensemble- and time-averaged moments of the OU-particle. Some physical systems, in which the relaxation and nonergodic features we unveiled may be observable, are discussed.}, language = {en} } @article{SchaererIzotovNakajimaetal.2018, author = {Schaerer, Daniel and Izotov, Yuri I. and Nakajima, K. and Worseck, Gabor and Chisholm, J. and Verhamme, A. and Thuan, T. X. and de Barros, S.}, title = {Intense C III] lambda lambda 1907,1909 emission from a strong Lyman continuum emitting galaxy}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {616}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {1432-0746}, doi = {10.1051/0004-6361/201833823}, pages = {5}, year = {2018}, abstract = {We have obtained the first complete ultraviolet (UV) spectrum of a strong Lyman continuum (LyC) emitter at low redshift - the compact, low-metallicity, star-forming galaxy J1154+2443 - with a Lyman continuum escape fraction of 46\% discovered recently. The Space Telescope Imaging Spectrograph spectrum shows strong Ly alpha and C III] lambda 1909 emission, as well as O III] lambda 1666. Our observations show that strong LyC emitters can have UV emission lines with a high equivalent width (e.g. EW(C III]) = 11.7 +/- 2.9 angstrom rest-frame), although their equivalent widths should be reduced due to the loss of ionizing photons. The intrinsic ionizing photon production efficiency of J1154+2443 is high, log(xi(0)(ion)) = 25.56 erg(-1) Hz, comparable to that of other recently discovered z similar to 0.3-0.4 LyC emitters. Combining our measurements and earlier determinations from the literature, we find a trend of increasing xi(0)(ion) with increasing C III] lambda 1909 equivalent width, which can be understood by a combination of decreasing stellar population age and metallicity. Simple ionization and density-bounded photoionization models can explain the main observational features including the UV spectrum of J1154+2443.}, language = {en} } @article{BattistoniDuerrGuehretal.2018, author = {Battistoni, A. and D{\"u}rr, H. A. and G{\"u}hr, Markus and Wolf, Thomas J. A.}, title = {A tilted pulse-front setup for femtosecond transient grating spectroscopy in highly non-collinear geometries}, series = {Journal of optics}, volume = {20}, journal = {Journal of optics}, number = {9}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {2040-8978}, doi = {10.1088/2040-8986/aad60a}, pages = {5}, year = {2018}, abstract = {We demonstrate a tilted pulse-front transient grating (TG) technique that allows to optimally utilize time resolution as well as TG line density while probing under grazing incidence as typically done in extreme ultraviolet (EUV) or soft x-ray (SXR) experiments. Our optical setup adapts the pulse front tilt of the two pulses that create the TG to the grazing incident pulse. We demonstrate the technique using all 800 nm femtosecond laser pulses for TG generation on a vanadium dioxide film. We probe that grating via diffraction of a third 800 nm pulse. The time resolution of 90 fs is an improvement by a factor of 30 compared to our previous experiments on the same system. The scheme paves the way for EUV and SXR probing of optically induced TGs on any material.}, language = {en} } @article{BustamanteSparreSpringeletal.2018, author = {Bustamante, Sebastian and Sparre, Martin and Springel, Volker and Grand, Robert J. J.}, title = {Merger-induced metallicity dilution in cosmological galaxy formation simulations}, series = {Monthly notices of the Royal Astronomical Society}, volume = {479}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/sty1692}, pages = {3381 -- 3392}, year = {2018}, abstract = {Observational studies have revealed that galaxy pairs tend to have lower gas-phase metallicity than isolated galaxies. This metallicity deficiency can be caused by inflows of low-metallicity gas due to the tidal forces and gravitational torques associated with galaxy mergers, diluting the metal content of the central region. In this work we demonstrate that such metallicity dilution occurs in state-of-the-art cosmological simulations of galaxy formation. We find that the dilution is typically 0.1 dex for major mergers, and is noticeable at projected separations smaller than 40 kpc. For minor mergers the metallicity dilution is still present, even though the amplitude is significantly smaller. Consistent with previous analysis of observed galaxies we find that mergers are outliers from the fundamental metallicity relation, with deviations being larger than expected for a Gaussian distribution of residuals. Our large sample of mergers within full cosmological simulations also makes it possible to estimate how the star formation rate enhancement and gas consumption timescale behave as a function of the merger mass ratio. We confirm that strong starbursts are likely to occur in major mergers, but they can also arise in minor mergers if more than two galaxies are participating in the interaction, a scenario that has largely been ignored in previous work based on idealised isolated merger simulations.}, language = {en} } @article{CecchiniThielSchelteretal.2018, author = {Cecchini, Gloria and Thiel, Marco and Schelter, Bj{\"o}rn and Sommerlade, Linda}, title = {Improving network inference}, series = {Journal of neuroscience methods}, volume = {307}, journal = {Journal of neuroscience methods}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0165-0270}, doi = {10.1016/j.jneumeth.2018.06.011}, pages = {31 -- 36}, year = {2018}, abstract = {Background: A reliable inference of networks from data is of key interest in the Neurosciences. Several methods have been suggested in the literature to reliably determine links in a network. To decide about the presence of links, these techniques rely on statistical inference, typically controlling the number of false positives, paying little attention to false negatives. New method: In this paper, by means of a comprehensive simulation study, we analyse the influence of false positive and false negative conclusions about the presence or absence of links in a network on the network topology. We show that different values to balance false positive and false negative conclusions about links should be used in order to reliably estimate network characteristics. We propose to run careful simulation studies prior to making potentially erroneous conclusion about the network topology. Results: Our analysis shows that optimal values to balance false positive and false negative conclusions about links depend on the network topology and characteristic of interest. Comparison with existing methods: Existing methods rely on a choice of the rate for false positive conclusions. They aim to be sure about individual links rather than the entire network. The rate of false negative conclusions is typically not investigated. Conclusions: Our investigation shows that the balance of false positive and false negative conclusions about links in a network has to be tuned for any network topology that is to be estimated. Moreover, within the same network topology, the results are qualitatively the same for each network characteristic, but the actual values leading to reliable estimates of the characteristics are different.}, language = {en} } @article{HeintzWatsonJakobssonetal.2018, author = {Heintz, Kasper Elm and Watson, D. and Jakobsson, P. and Fynbo, J. P. U. and Bolmer, J. and Arabsalmani, M. and Cano, Zach and Covino, S. and Gomboc, A. and Japelj, J. and Kaper, L. and Krogager, J. -K. and Pugliese, G. and Sanchez-Ramirez, R. and Selsing, J. and Sparre, Martin and Tanvir, N. R. and Thone, C. C. and de Ugarte Postigo, A. and Vergani, S. D.}, title = {Highly ionized metals as probes of the circumburst gas in the natal regions of gamma-ray bursts}, series = {Monthly notices of the Royal Astronomical Society}, volume = {479}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/sty1447}, pages = {3456 -- 3476}, year = {2018}, abstract = {We present here a survey of high-ionization absorption lines in the afterglow spectra of long-duration gamma-ray bursts (GRBs) obtained with the VLT/X-shooter spectrograph. Our main goal is to investigate the circumburst medium in the natal regions of GRBs. Our primary focus is on the N vλλ 1238, 1242 line transitions, but we also discuss other high-ionization lines such as O vi, C iv, and Si iv. We find no correlation between the column density of N v and the neutral gas properties such as metallicity, H i column density, and dust depletion; however, the relative velocity of N v, typically a blueshift with respect to the neutral gas, is found to be correlated with the column density of H i. This may be explained if the N v gas is part of an H ii region hosting the GRB, where the region's expansion is confined by dense, neutral gas in the GRB's host galaxy. We find tentative evidence (at 2σ significance) that the X-ray derived column density, NH, X, may be correlated with the column density of N v, which would indicate that both measurements are sensitive to the column density of the gas located in the vicinity of the GRB. We investigate the scenario where N v (and also O vi) is produced by recombination after the corresponding atoms have been stripped entirely of their electrons by the initial prompt emission, in contrast to previous models where highly ionized gas is produced by photoionization from the GRB afterglow.}, language = {en} } @article{LebigaSantosLimaYan2018, author = {Lebiga, O. and Santos-Lima, Reinaldo and Yan, Huirong}, title = {Kinetic-MHD simulations of gyroresonance instability driven by CR pressure anisotropy}, series = {Monthly notices of the Royal Astronomical Society}, volume = {476}, journal = {Monthly notices of the Royal Astronomical Society}, number = {2}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/sty309}, pages = {2779 -- 2791}, year = {2018}, abstract = {The transport of cosmic rays (CRs) is crucial for the understanding of almost all high-energy phenomena. Both pre-existing large-scale magnetohydrodynamic (MHD) turbulence and locally generated turbulence through plasma instabilities are important for the CR propagation in astrophysical media. The potential role of the resonant instability triggered by CR pressure anisotropy to regulate the parallel spatial diffusion of low-energy CRs (less than or similar to 100 GeV) in the interstellar and intracluster medium of galaxies has been shown in previous theoretical works. This work aims to study the gyroresonance instability via direct numerical simulations, in order to access quantitatively the wave-particle scattering rates. For this, we employ a 1D PIC-MHD code to follow the growth and saturation of the gyroresonance instability. We extract from the simulations the pitch-angle diffusion coefficient D-mu mu produced by the instability during the linear and saturation phases, and a very good agreement (within a factor of 3) is found with the values predicted by the quasi-linear theory (QLT). Our results support the applicability of the QLT for modelling the scattering of low-energy CRs by the gyroresonance instability in the complex interplay between this instability and the large-scale MHD turbulence.}, language = {en} } @article{ElNagarLauermannSarhanetal.2018, author = {El-Nagar, Gumaa A. and Lauermann, Iver and Sarhan, Radwan Mohamed and Roth, Christina}, title = {Hierarchically structured iron-doped silver (Ag-Fe) lotus flowers for an efficient oxygen reduction reaction}, series = {Nanoscale}, volume = {10}, journal = {Nanoscale}, number = {15}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {2040-3364}, doi = {10.1039/c8nr00020d}, pages = {7304 -- 7310}, year = {2018}, abstract = {The development of cheap and efficient electrocatalysts for the oxygen reduction reaction (ORR) is vital for the immediate commercialization of fuel cells which are still limited by the high cost and low performance of the utilized commercial Pt-based electrodes. As a promising alternative, this study reports on the synthesis of hierarchical iron-doped silver lotus flowers (AgFelotus) by a facile chemical procedure as robust and efficient ORR electrocatalysts. Succinic acid was used as a structure directing agent to tune the morphology of undoped and iron-doped silver particles. In the absence of succinic acid, ball-like silver particles were obtained, while using 2 mM succinic acid led to peony-like flower structures. The doping of silver peony-flowers with iron resulted in lotus-like flower structures with high electrocatalytic activity for ORR together with outstanding tolerance against poisoning with various hydrocarbon (HC) impurities, in situ generated during fuel cell operation, as well as different fuels from anodic crossover. AgFelotus exhibited a superior ORR activity with more than 40 times higher stability than the commercial Pt/C catalyst in alkaline media. This substantial performance enhancement is attributed to the unique lotus-like flower structures providing more electroactive surface sites, in addition to the iron dopants which facilitate ORR charge transfer.}, language = {en} } @article{ZhangYanRichter2018, author = {Zhang, Heshou and Yan, Huirong and Richter, Philipp}, title = {The influence of atomic alignment on absorption and emission spectroscopy}, series = {Monthly notices of the Royal Astronomical Society}, volume = {479}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/sty1594}, pages = {3923 -- 3935}, year = {2018}, abstract = {Spectroscopic observations play essential roles in astrophysics. They are crucial for determining physical parameters in our Universe, providing information about the chemistry of various astronomical environments. The proper execution of the spectroscopic analysis requires accounting for all the physical effects that are compatible to the signal-to-noise ratio. We find in this paper the influence on spectroscopy from the atomic/ground state alignment owing to anisotropic radiation and modulated by interstellar magnetic field, has significant impact on the study of interstellar gas. In different observational scenarios, we comprehensively demonstrate how atomic alignment influences the spectral analysis and provide the expressions for correcting the effect. The variations are even more pronounced for multiplets and line ratios. We show the variation of the deduced physical parameters caused by the atomic alignment effect, including alpha-to-iron ratio ([X/Fe]) and ionization fraction. Synthetic observations are performed to illustrate the visibility of such effect with current facilities. A study of Photodissociation regions in rho Ophiuchi cloud is presented to demonstrate how to account for atomic alignment in practice. Our work has shown that due to its potential impact, atomic alignment has to be included in an accurate spectroscopic analysis of the interstellar gas with current observational capability.}, language = {en} } @article{SchmidtHennawiWorsecketal.2018, author = {Schmidt, Tobias M. and Hennawi, Joseph F. and Worseck, Gabor and Davies, Frederick B. and Lukic, Zarija and O{\~n}orbe, Jose}, title = {Modeling the HeII transverse proximity effect}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {861}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aac8e4}, pages = {20}, year = {2018}, abstract = {The He II transverse proximity effect-enhanced He II Ly alpha transmission in a background sightline caused by the ionizing radiation of a foreground quasar-offers a unique opportunity to probe the emission properties of quasars, in particular the emission geometry (obscuration, beaming) and the quasar lifetime. Building on the foreground quasar survey published in Schmidt et al., we present a detailed model of the He II transverse proximity effect, specifically designed to include light travel time effects, finite quasar ages, and quasar obscuration. We postprocess outputs from a cosmological hydrodynamical simulation with a fluctuating He II ultraviolet background model, with the added effect of the radiation from a single bright foreground quasar. We vary the age t(age) and obscured sky fractions Omega(obsc) of the foreground quasar, and explore the resulting effect on the He II transverse proximity effect signal. Fluctuations in intergalactic medium density and the ultraviolet background, as well as the unknown orientation of the foreground quasar, result in a large variance of the He II Ly alpha transmission along the background sightline. We develop a fully Bayesian statistical formalism to compare far-ultraviolet He II Ly alpha transmission spectra of the background quasars to our models, and extract joint constraints on t(age) and Omega(obsc) for the six Schmidt et al. foreground quasars with the highest implied He II photoionization rates. Our analysis suggests a bimodal distribution of quasar emission properties, whereby one foreground quasar, associated with a strong He II transmission spike, is relatively old (22 Myr) and unobscured (Omega(obsc) < 35\%), whereas three others are either younger than 10 Myr or highly obscured (Omega(obsc) > 70\%).}, language = {en} } @article{YangZhuWolfetal.2018, author = {Yang, Jie and Zhu, Xiaolei and Wolf, Thomas J. A. and Li, Zheng and Nunes, Jo{\~a}o Pedro Figueira and Coffee, Ryan and Cryan, James P. and G{\"u}hr, Markus and Hegazy, Kareem and Heinz, Tony F. and Jobe, Keith and Li, Renkai and Shen, Xiaozhe and Veccione, Theodore and Weathersby, Stephen and Wilkin, Kyle J. and Yoneda, Charles and Zheng, Qiang and Martinez, Todd J. and Centurion, Martin and Wang, Xijie}, title = {Imaging CF3I conical intersection and photodissociation dynamics with ultrafast electron diffraction}, series = {Science}, volume = {361}, journal = {Science}, number = {6397}, publisher = {American Assoc. for the Advancement of Science}, address = {Washington}, issn = {0036-8075}, doi = {10.1126/science.aat0049}, pages = {64 -- 67}, year = {2018}, abstract = {Conical intersections play a critical role in excited-state dynamics of polyatomic molecules because they govern the reaction pathways of many nonadiabatic processes. However, ultrafast probes have lacked sufficient spatial resolution to image wave-packet trajectories through these intersections directly. Here, we present the simultaneous experimental characterization of one-photon and two-photon excitation channels in isolated CF3I molecules using ultrafast gas-phase electron diffraction. In the two-photon channel, we have mapped out the real-space trajectories of a coherent nuclear wave packet, which bifurcates onto two potential energy surfaces when passing through a conical intersection. In the one-photon channel, we have resolved excitation of both the umbrella and the breathing vibrational modes in the CF3 fragment in multiple nuclear dimensions. These findings benchmark and validate ab initio nonadiabatic dynamics calculations.}, language = {en} } @article{OhmHoischen2018, author = {Ohm, Stefan and Hoischen, Clemens}, title = {On the expected gamma-ray emission from nearby flaring stars}, series = {Monthly notices of the Royal Astronomical Society}, volume = {474}, journal = {Monthly notices of the Royal Astronomical Society}, number = {1}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stx2806}, pages = {1335 -- 1341}, year = {2018}, abstract = {Stellar flares have been extensively studied in soft X-rays (SXRs) by basically every X-ray mission. Hard X-ray (HXR) emission from stellar superflares, however, have only been detected from a handful of objects over the past years. One very extreme event was the superflare from the young M-dwarf DGCVn binary star system, which triggered Swift/BAT as if it was a gamma-ray burst. In this work, we estimate the expected gamma-ray emission from DGCVn and the most extreme stellar flares by extrapolating from solar flares based on measured solar energetic particles (SEPs), as well as thermal and non-thermal emission properties. We find that ions are plausibly accelerated in stellar superflares to 100 GeV energies, and possibly up to TeV energies in the associated coronal mass ejections. The corresponding pi(0)-decay gamma-ray emission could be detectable from stellar superflares with ground-based gamma-ray telescopes. On the other hand, the detection of gamma-ray emission implies particle densities high enough that ions suffer significant losses due to inelastic proton-proton scattering. The next-generation Cherenkov Telescope Array (CTA) should be able to probe superflares from M dwarfs in the solar neighbourhood and constrain the energy in interacting cosmic rays and/or their maximum energy. The detection of gamma-ray emission from stellar flares would open a new window for the study of stellar physics, the underlying physical processes in flares and their impact on habitability of planetary systems.}, language = {en} } @article{BeniniSchenkelSchreiber2018, author = {Benini, Marco and Schenkel, Alexander and Schreiber, Urs}, title = {The Stack of Yang-Mills Fields on Lorentzian Manifolds}, series = {Communications in mathematical physics}, volume = {359}, journal = {Communications in mathematical physics}, number = {2}, publisher = {Springer}, address = {New York}, issn = {0010-3616}, doi = {10.1007/s00220-018-3120-1}, pages = {765 -- 820}, year = {2018}, abstract = {We provide an abstract definition and an explicit construction of the stack of non-Abelian Yang-Mills fields on globally hyperbolic Lorentzian manifolds. We also formulate a stacky version of the Yang-Mills Cauchy problem and show that its well-posedness is equivalent to a whole family of parametrized PDE problems. Our work is based on the homotopy theoretical approach to stacks proposed in Hollander (Isr. J. Math. 163:93-124, 2008), which we shall extend by further constructions that are relevant for our purposes. In particular, we will clarify the concretification of mapping stacks to classifying stacks such as BG (con).}, language = {en} } @article{KoopmanMucciniToffanin2018, author = {Koopman, Wouter-Willem Adriaan and Muccini, Michele and Toffanin, Stefano}, title = {High-resolution photoluminescence electro-modulation microscopy by scanning lock-in}, series = {Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques}, volume = {89}, journal = {Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques}, number = {4}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0034-6748}, doi = {10.1063/1.5010281}, pages = {7}, year = {2018}, abstract = {Morphological inhomogeneities and structural defects in organic semiconductors crucially determine the charge accumulation and lateral transport in organic thin-film transistors. Photoluminescence Electro-Modulation (PLEM) microscopy is a laser-scanning microscopy technique that relies on the modulation of the thin-film fluorescence in the presence of charge-carriers to image the spatial distribution of charges within the active organic semiconductor. Here, we present a lock-in scheme based on a scanning beam approach for increasing the PLEM microscopy resolution and contrast. The charge density in the device is modulated by a sinusoidal electrical signal, phase-locked to the scanning beam of the excitation laser. The lock-in detection scheme is achieved by acquiring a series of images with different phases between the beam scan and the electrical modulation. Application of high resolution PLEM to an organic transistor in accumulation mode demonstrates its potential to image local variations in the charge accumulation. A diffraction-limited precision of sub-300 nm and a signal to noise ratio of 21.4 dB could be achieved. Published by AIP Publishing.}, language = {en} } @article{MorHerzogNoacketal.2018, author = {Mor, Selene and Herzog, Marc and Noack, Johannes and Katayama, Naoyuki and Nohara, Minoru and Takagi, Hide and Trunschke, Annette and Mizokawa, Takashi and Monney, Claude and St{\"a}hler, Julia}, title = {Inhibition of the photoinduced structural phase transition in the excitonic insulator Ta2NiSe5}, series = {Physical review : B, Condensed matter and materials physics}, volume = {97}, journal = {Physical review : B, Condensed matter and materials physics}, number = {11}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9950}, doi = {10.1103/PhysRevB.97.115154}, pages = {5}, year = {2018}, abstract = {Femtosecond time-resolved midinfrared reflectivity is used to investigate the electron and phonon dynamics occurring at the direct band gap of the excitonic insulator Ta2NiSe5 below the critical temperature of its structural phase transition. We find that the phonon dynamics show a strong coupling to the excitation of free carriers at the Gamma point of the Brillouin zone. The optical response saturates at a critical excitation fluence F-C = 0.30 +/- 0.08 mJ/cm(2) due to optical absorption saturation. This limits the optical excitation density in Ta2NiSe5 so that the system cannot be pumped sufficiently strongly to undergo the structural change to the high-temperature phase. We thereby demonstrate that Ta2NiSe5 exhibits a blocking mechanism when pumped in the near-infrared regime, preventing a nonthermal structural phase transition.}, language = {en} } @article{AydinerCherstvyMetzler2018, author = {Aydiner, Ekrem and Cherstvy, Andrey G. and Metzler, Ralf}, title = {Wealth distribution, Pareto law, and stretched exponential decay of money}, series = {Physica : europhysics journal ; A, Statistical mechanics and its applications}, volume = {490}, journal = {Physica : europhysics journal ; A, Statistical mechanics and its applications}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0378-4371}, doi = {10.1016/j.physa.2017.08.017}, pages = {278 -- 288}, year = {2018}, abstract = {We study by Monte Carlo simulations a kinetic exchange trading model for both fixed and distributed saving propensities of the agents and rationalize the person and wealth distributions. We show that the newly introduced wealth distribution - that may be more amenable in certain situations - features a different power-law exponent, particularly for distributed saving propensities of the agents. For open agent-based systems, we analyze the person and wealth distributions and find that the presence of trap agents alters their amplitude, leaving however the scaling exponents nearly unaffected. For an open system, we show that the total wealth - for different trap agent densities and saving propensities of the agents - decreases in time according to the classical Kohlrausch-Williams-Watts stretched exponential law. Interestingly, this decay does not depend on the trap agent density, but rather on saving propensities. The system relaxation for fixed and distributed saving schemes are found to be different.}, language = {en} } @article{TotzEliseevPetrietal.2018, author = {Totz, Sonja Juliana and Eliseev, Alexey V. and Petri, Stefan and Flechsig, Michael and Caesar, Levke and Petoukhov, Vladimir and Coumou, Dim}, title = {The dynamical core of the Aeolus 1.0 statistical-dynamical atmosphere model}, series = {Geoscientific model development : an interactive open access journal of the European Geosciences Union}, volume = {11}, journal = {Geoscientific model development : an interactive open access journal of the European Geosciences Union}, number = {2}, publisher = {Copernicus}, address = {G{\"o}ttingen}, issn = {1991-959X}, doi = {10.5194/gmd-11-665-2018}, pages = {665 -- 679}, year = {2018}, abstract = {Here, we present novel equations for the large-scale zonal-mean wind as well as those for planetary waves. Together with synoptic parameterization (as presented by Coumou et al., 2011), these form the mathematical description of the dynamical core of Aeolus 1.0. The regions of high azonal wind velocities (planetary waves) are accurately captured for all validation experiments. The zonal-mean zonal wind and the integrated lower troposphere mass flux show good results in particular in the Northern Hemisphere. In the Southern Hemisphere, the model tends to produce too-weak zonal-mean zonal winds and a too-narrow Hadley circulation. We discuss possible reasons for these model biases as well as planned future model improvements and applications.}, language = {en} } @article{XiongFangOsipovetal.2018, author = {Xiong, Hui and Fang, Li and Osipov, Timur and Kling, Nora G. and Wolf, Thomas J. A. and Sistrunk, Emily and Obaid, Razib and G{\"u}hr, Markus and Berrah, Nora}, title = {Fragmentation of endohedral fullerene Ho3N@C-80 in an intense femtosecond near-infrared laser field}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {97}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9926}, doi = {10.1103/PhysRevA.97.023419}, pages = {7}, year = {2018}, abstract = {The fragmentation of gas phase endohedral fullerene, Ho3N@C-80, was investigated using femtosecond near-infrared laser pulses with an ion velocity map imaging spectrometer. We observed that Ho+ abundance associated with carbon cage opening dominates at an intensity of 1.1 x 10(14) W/cm(2). As the intensity increases, the Ho+ yield associated with multifragmentation of the carbon cage exceeds the prominence of Ho+ associated with the gentler carbon cage opening. Moreover, the power law dependence of Ho+ on laser intensity indicates that the transition of the most likely fragmentation mechanisms occurs around 2.0 x 10(14) W/cm(2).}, language = {en} } @article{FoxBargerWakkeretal.2018, author = {Fox, Andrew J. and Barger, Kathleen A. and Wakker, Bart P. and Richter, Philipp and Antwi-Danso, Jacqueline and Casetti-Dinescu, Dana I. and Howk, J. Christopher and Lehner, Nicolas and Crowther, Paul A. and Lockman, Felix J.}, title = {Chemical Abundances in the Leading Arm of the Magellanic Stream}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {854}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aaa9bb}, pages = {14}, year = {2018}, abstract = {The Leading Arm (LA) of the Magellanic Stream is a vast debris field of H I clouds connecting the Milky Way and the Magellanic Clouds. It represents an example of active gas accretion onto the Galaxy. Previously, only one chemical abundance measurement had been made in the LA. Here we present chemical abundance measurements using Hubble Space Telescope/Cosmic Origins Spectrograph and Green Bank Telescope spectra of four AGN sightlines passing through the LA and three nearby sightlines that may trace outer fragments of the LA. We find low oxygen abundances, ranging from 4.0+(2.0)(2.0)\% 12.6(4.1)(6.0)\% solar, in the confirmed LA directions, with the lowest values found in the region known as LA III, farthest from the LMC. These abundances are substantially lower than the single previous measurement, S/H = 35 +/- 7\% solar, but are in agreement with those reported in the SMC filament of the trailing Stream, supporting a common origin in the SMC (not the LMC) for the majority of the LA and trailing Stream. This provides important constraints for models of the formation of the Magellanic System. Finally, two of the three nearby sightlines show high-velocity clouds with H I columns, kinematics, and oxygen abundances consistent with LA membership. This suggests that the LA is larger than traditionally thought, extending at least 20 degrees further to the Galactic northwest.}, language = {en} } @article{YoungUedaGuehretal.2018, author = {Young, Linda and Ueda, Kiyoshi and G{\"u}hr, Markus and Bucksbaum, Philip H. and Simon, Marc and Mukamel, Shaul and Rohringer, Nina and Prince, Kevin C. and Masciovecchio, Claudio and Meyer, Michael and Rudenko, Artem and Rolles, Daniel and Bostedt, Christoph and Fuchs, Matthias and Reis, David A. and Santra, Robin and Kapteyn, Henry and Murnane, Margaret and Ibrahim, Heide and Legare, Francois and Vrakking, Marc and Isinger, Marcus and Kroon, David and Gisselbrecht, Mathieu and W{\"o}rner, Hans Jakob and Leone, Stephen R.}, title = {Roadmap of ultrafast x-ray atomic and molecular physics}, series = {Journal of physics : B, Atomic, molecular and optical physics}, volume = {51}, journal = {Journal of physics : B, Atomic, molecular and optical physics}, number = {3}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0953-4075}, doi = {10.1088/1361-6455/aa9735}, pages = {45}, year = {2018}, abstract = {X-ray free-electron lasers (XFELs) and table-top sources of x-rays based upon high harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and molecular physics, largely due to an explosive growth in capabilities in the past decade. XFELs now provide unprecedented intensity (10(20) W cm(-2)) of x-rays at wavelengths down to similar to 1 Angstrom, and HHG provides unprecedented time resolution (similar to 50 attoseconds) and a correspondingly large coherent bandwidth at longer wavelengths. For context, timescales can be referenced to the Bohr orbital period in hydrogen atom of 150 attoseconds and the hydrogen-molecule vibrational period of 8 femtoseconds; wavelength scales can be referenced to the chemically significant carbon K-edge at a photon energy of similar to 280 eV (44 Angstroms) and the bond length in methane of similar to 1 Angstrom. With these modern x-ray sources one now has the ability to focus on individual atoms, even when embedded in a complex molecule, and view electronic and nuclear motion on their intrinsic scales (attoseconds and Angstroms). These sources have enabled coherent diffractive imaging, where one can image non-crystalline objects in three dimensions on ultrafast timescales, potentially with atomic resolution. The unprecedented intensity available with XFELs has opened new fields of multiphoton and nonlinear x-ray physics where behavior of matter under extreme conditions can be explored. The unprecedented time resolution and pulse synchronization provided by HHG sources has kindled fundamental investigations of time delays in photoionization, charge migration in molecules, and dynamics near conical intersections that are foundational to AMO physics and chemistry. This roadmap coincides with the year when three new XFEL facilities, operating at Angstrom wavelengths, opened for users (European XFEL, Swiss-FEL and PAL-FEL in Korea) almost doubling the present worldwide number of XFELs, and documents the remarkable progress in HHG capabilities since its discovery roughly 30 years ago, showcasing experiments in AMO physics and other applications. Here we capture the perspectives of 17 leading groups and organize the contributions into four categories: ultrafast molecular dynamics, multidimensional x-ray spectroscopies; high-intensity x-ray phenomena; attosecond x-ray science.}, language = {en} } @article{MyhreWolfChengetal.2018, author = {Myhre, Rolf H. and Wolf, Thomas J. A. and Cheng, Lan and Nandi, Saikat and Coriani, Sonia and G{\"u}hr, Markus and Koch, Henrik}, title = {A theoretical and experimental benchmark study of core-excited states in nitrogen}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {148}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {6}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.5011148}, pages = {7}, year = {2018}, abstract = {The high resolution near edge X-ray absorption fine structure spectrum of nitrogen displays the vibrational structure of the core-excited states. This makes nitrogen well suited for assessing the accuracy of different electronic structure methods for core excitations. We report high resolution experimental measurements performed at the SOLEIL synchrotron facility. These are compared with theoretical spectra calculated using coupled cluster theory and algebraic diagrammatic construction theory. The coupled cluster singles and doubles with perturbative triples model known as CC3 is shown to accurately reproduce the experimental excitation energies as well as the spacing of the vibrational transitions. The computational results are also shown to be systematically improved within the coupled cluster hierarchy, with the coupled cluster singles, doubles, triples, and quadruples method faithfully reproducing the experimental vibrational structure. Published by AIP Publishing.}, language = {en} } @article{ZellmeierBrennerJanietzetal.2018, author = {Zellmeier, M. and Brenner, Thomas J. K. and Janietz, Silvia and Nickel, N. H. and Rappich, J.}, title = {Polythiophenes as emitter layers for crystalline silicon solar cells}, series = {Journal of applied physics}, volume = {123}, journal = {Journal of applied physics}, number = {3}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-8979}, doi = {10.1063/1.5006625}, pages = {5}, year = {2018}, abstract = {We investigated the influence of the emitter (amorphous-Si, a-Si, or polythiophene derivatives: poly(3-hexylthiophene), P3HT, and poly(3-[3,6-dioxaheptyl]-thiophene), P3DOT) and the interface passivation (intrinsic a-Si or SiOX and methyl groups or SiOX) on the c-Si based 1 × 1 cm2 planar hybrid heterojunction solar cell parameters. We observed higher short circuit currents for the P3HT or P3DOT/c-Si solar cells than those obtained for a-Si/c-Si devices, independent of the interface passivation. The obtained VOC of 659 mV for the P3DOT/SiOX/c-Si heterojunction solar cell with hydrophilic 3,6-dioxaheptyl side chains is among the highest reported for c-Si/polythiophene devices. The maximum power conversion efficiency, PCE, was 11\% for the P3DOT/SiOX/c-Si heterojunction solar cell. Additionally, our wafer lifetime measurements reveal a field effect passivation in the wafer induced by the polythiophenes when deposited on c-Si.}, language = {en} } @article{SawickiAbelSchoell2018, author = {Sawicki, Jakub and Abel, Markus and Sch{\"o}ll, Eckehard}, title = {Synchronization of organ pipes}, series = {The European physical journal : B, Condensed matter and complex systems}, volume = {91}, journal = {The European physical journal : B, Condensed matter and complex systems}, number = {2}, publisher = {Springer}, address = {New York}, issn = {1434-6028}, doi = {10.1140/epjb/e2017-80485-8}, pages = {9}, year = {2018}, abstract = {We investigate synchronization of coupled organ pipes. Synchronization and reflection in the organ lead to undesired weakening of the sound in special cases. Recent experiments have shown that sound interaction is highly complex and nonlinear, however, we show that two delay-coupled Van-der-Pol oscillators appear to be a good model for the occurring dynamical phenomena. Here the coupling is realized as distance-dependent, or time-delayed, equivalently. Analytically, we investigate the synchronization frequency and bifurcation scenarios which occur at the boundaries of the Arnold tongues. We successfully compare our results to experimental data.}, language = {en} } @article{KrapfMarinariMetzleretal.2018, author = {Krapf, Diego and Marinari, Enzo and Metzler, Ralf and Oshanin, Gleb and Xu, Xinran and Squarcini, Alessio}, title = {Power spectral density of a single Brownian trajectory}, series = {New journal of physics : the open-access journal for physics}, volume = {20}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/aaa67c}, pages = {30}, year = {2018}, abstract = {The power spectral density (PSD) of any time-dependent stochastic processX (t) is ameaningful feature of its spectral content. In its text-book definition, the PSD is the Fourier transform of the covariance function of X-t over an infinitely large observation timeT, that is, it is defined as an ensemble-averaged property taken in the limitT -> infinity. Alegitimate question is what information on the PSD can be reliably obtained from single-trajectory experiments, if one goes beyond the standard definition and analyzes the PSD of a single trajectory recorded for a finite observation timeT. In quest for this answer, for a d-dimensional Brownian motion (BM) we calculate the probability density function of a single-trajectory PSD for arbitrary frequency f, finite observation time T and arbitrary number k of projections of the trajectory on different axes. We show analytically that the scaling exponent for the frequency-dependence of the PSD specific to an ensemble of BM trajectories can be already obtained from a single trajectory, while the numerical amplitude in the relation between the ensemble-averaged and single-trajectory PSDs is afluctuating property which varies from realization to realization. The distribution of this amplitude is calculated exactly and is discussed in detail. Our results are confirmed by numerical simulations and single-particle tracking experiments, with remarkably good agreement. In addition we consider a truncated Wiener representation of BM, and the case of a discrete-time lattice random walk. We highlight some differences in the behavior of a single-trajectory PSD for BM and for the two latter situations. The framework developed herein will allow for meaningful physical analysis of experimental stochastic trajectories.}, language = {en} } @article{LeiendeckerLichtBorghsetal.2018, author = {Leiendecker, Mai-Thi and Licht, Christopher J. and Borghs, Jannik and Mooney, David J. and Zimmermann, Marc and B{\"o}ker, Alexander}, title = {Physical polyurethane hydrogels via charge shielding through acids or salts}, series = {Macromolecular rapid communications}, volume = {39}, journal = {Macromolecular rapid communications}, number = {7}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1022-1336}, doi = {10.1002/marc.201700711}, pages = {5}, year = {2018}, abstract = {Physical hydrogels with tunable stress-relaxation and excellent stress recovery are formed from anionic polyurethanes via addition of acids, monovalent salts, or divalent salts. Gel properties can be widely adjusted through pH, salt valence, salt concentration, and monomer composition. We propose and investigate a novel gelation mechanism based on a colloidal system interacting through charge repulsion and chrage shielding, allowing a broad use of the material, from acidic (pH 4-5.5) to pH-neutral hydrogels with Young's moduli ranging from 10 to 140 kPa.}, language = {en} } @article{Sachse2018, author = {Sachse, Manuel}, title = {A planetary dust ring generated by impact-ejection from the Galilean satellites}, series = {Icarus : international journal of solar system studies}, volume = {303}, journal = {Icarus : international journal of solar system studies}, publisher = {Elsevier}, address = {San Diego}, issn = {0019-1035}, doi = {10.1016/j.icarus.2017.10.011}, pages = {166 -- 180}, year = {2018}, abstract = {All outer planets in the Solar System are surrounded by a ring system. Many of these rings are dust rings or they contain at least a high proportion of dust. They are often formed by impacts of micro-meteoroids onto embedded bodies. The ejected material typically consists of micron-sized charged particles, which are susceptible to gravitational and non-gravitational forces. Generally, detailed information on the dynamics and distribution of the dust requires expensive numerical simulations of a large number of particles. Here we develop a relatively simple and fast, semi-analytical model for an impact-generated planetary dust ring governed by the planet's gravity and the relevant perturbation forces for the dynamics of small charged particles. The most important parameter of the model is the dust production rate, which is a linear factor in the calculation of the dust densities. We apply our model to dust ejected from the Galilean satellites using production rates obtained from flybys of the dust sources. The dust densities predicted by our model are in good agreement with numerical simulations and with in situ measurements by the Galileo spacecraft. The lifetimes of large particles are about two orders of magnitude greater than those of small ones, which implies a flattening of the size distribution in circumplanetary space. Information about the distribution of circumplanetary dust is also important for the risk assessment of spacecraft orbits in the respective regions.}, language = {en} } @article{ChengKliemDing2018, author = {Cheng, Xin and Kliem, Bernhard and Ding, Mingde}, title = {Unambiguous evidence of filament splitting-induced partial eruptions}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {856}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.3847/1538-4357/aab08d}, pages = {15}, year = {2018}, abstract = {Coronal mass ejections are often considered to result from the full eruption of a magnetic flux rope (MFR). However, it is recognized that, in some events, the MFR may release only part of its flux, with the details of the implied splitting not completely established due to limitations in observations. Here, we investigate two partial eruption events including a confined and a successful one. Both partial eruptions are a consequence of the vertical splitting of a filament-hosting MFR involving internal reconnection. A loss of equilibrium in the rising part of the magnetic flux is suggested by the impulsive onset of both events and by the delayed onset of reconnection in the confined event. The remaining part of the flux might be line-tied to the photosphere in a bald patch (BP) separatrix surface, and we confirm the existence of extended BP sections for the successful eruption. The internal reconnection is signified by brightenings in the body of one filament and between the rising and remaining parts of both filaments. It evolves quickly into the standard current sheet reconnection in the wake of the eruption. As a result, regardless of being confined or successful, both eruptions produce hard X-ray sources and flare loops below the erupting but above the surviving flux, as well as a pair of flare ribbons enclosing the latter.}, language = {en} } @article{BaushevBarkov2018, author = {Baushev, Anton N. and Barkov, M. V.}, title = {Why does Einasto profile index n similar to 6 occur so frequently?}, series = {Journal of cosmology and astroparticle physics}, journal = {Journal of cosmology and astroparticle physics}, number = {3}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1475-7516}, doi = {10.1088/1475-7516/2018/03/034}, pages = {15}, year = {2018}, abstract = {We consider the behavior of spherically symmetric Einasto halos composed of gravitating particles in the Fokker-Planck approximation. This approach allows us to consider the undesirable influence of close encounters in the N-body simulations more adequately than the generally accepted criteria. The Einasto profile with index n approximate to 6 is a stationary solution of the Fokker-Planck equation in the halo center. There are some reasons to believe that the solution is an attractor. Then the Fokker-Planck diffusion tends to transform a density profile to the equilibrium one with the Einasto index n approximate to 6. We suggest this effect as a possible reason why the Einasto index n approximate to 6 occurs so frequently in the interpretation of N-body simulation results. The results obtained cast doubt on generally accepted criteria of N-body simulation convergence.}, language = {en} } @article{HaniSparreEllisonetal.2017, author = {Hani, Maan H. and Sparre, Martin and Ellison, Sara L. and Torrey, Paul and Vogelsberger, Mark}, title = {Galaxy mergers moulding the circum-galactic medium}, series = {Monthly notices of the Royal Astronomical Society}, volume = {475}, journal = {Monthly notices of the Royal Astronomical Society}, number = {1}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stx3252}, pages = {1160 -- 1176}, year = {2017}, abstract = {Galaxies are surrounded by sizeable gas reservoirs which host a significant amount of metals: the circum-galactic medium (CGM). The CGM acts as a mediator between the galaxy and the extragalactic medium. However, our understanding of how galaxy mergers, a major evolutionary transformation, impact the CGM remains deficient. We present a theoretical study of the effect of galaxy mergers on the CGM. We use hydrodynamical cosmological zoom-in simulations of a major merger selected from the Illustris project such that the z = 0 descendant has a halo mass and stellar mass comparable to the Milky Way. To study the CGM we then re-simulated this system at a 40 times better mass resolution, and included detailed post-processing ionization modelling. Our work demonstrates the effect the merger has on the characteristic size of the CGM, its metallicity, and the predicted covering fraction of various commonly observed gas-phase species, such as H I, C IV, and O VI. We show that merger-induced outflows can increase the CGM metallicity by 0.2-0.3 dex within 0.5 Gyr post-merger. These effects last up to 6 Gyr post-merger. While the merger increases the total metal covering fractions by factors of 2-3, the covering fractions of commonly observed UV ions decrease due to the hard ionizing radiation from the active galactic nucleus, which we model explicitly. Our study of the single simulated major merger presented in this work demonstrates the significant impact that a galaxy interaction can have on the size, metallicity, and observed column densities of the CGM.}, language = {en} } @article{UolaLeverGuehneetal.2018, author = {Uola, Roope and Lever, Fabiano and G{\"u}hne, Otfried and Pellonpaa, Juha-Pekka}, title = {Unified picture for spatial, temporal, and channel steering}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {97}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {3}, publisher = {American Physical Society}, address = {College Park}, issn = {2469-9926}, doi = {10.1103/PhysRevA.97.032301}, pages = {6}, year = {2018}, abstract = {Quantum steering describes how local actions on a quantum system can affect another, spacelike separated, quantum state. Lately, quantum steering has been formulated also for timelike scenarios and for quantum channels. We approach all the three scenarios as one using tools from Stinespring dilations of quantum channels. By applying our technique we link all three steering problems one-to-one with the incompatibility of quantum measurements, a result formerly known only for spatial steering. We exploit this connection by showing how measurement uncertainty relations can be used as tight steering inequalities for all three scenarios. Moreover, we show that certain notions of temporal and spatial steering are fully equivalent and prove a hierarchy between temporal steering and macrorealistic hidden variable models.}, language = {en} } @article{Goychuk2018, author = {Goychuk, Igor}, title = {Sensing magnetic fields with magnetosensitive ion channels}, series = {Sensors}, volume = {18}, journal = {Sensors}, number = {3}, publisher = {MDPI}, address = {Basel}, issn = {1424-8220}, doi = {10.3390/s18030728}, pages = {19}, year = {2018}, abstract = {Magnetic nanoparticles are met across many biological species ranging from magnetosensitive bacteria, fishes, bees, bats, rats, birds, to humans. They can be both of biogenetic origin and due to environmental contamination, being either in paramagnetic or ferromagnetic state. The energy of such naturally occurring single-domain magnetic nanoparticles can reach up to 10-20 room k(B)T in the magnetic field of the Earth, which naturally led to supposition that they can serve as sensory elements in various animals. This work explores within a stochastic modeling framework a fascinating hypothesis of magnetosensitive ion channels with magnetic nanoparticles serving as sensory elements, especially, how realistic it is given a highly dissipative viscoelastic interior of living cells and typical sizes of nanoparticles possibly involved.}, language = {en} } @article{HaubitzFudickarLinkeretal.2020, author = {Haubitz, Toni and Fudickar, Werner and Linker, Torsten and Kumke, Michael Uwe}, title = {pH-sensitive fluorescence switching of pyridylanthracenes}, series = {The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment \& general theory}, volume = {124}, journal = {The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment \& general theory}, number = {52}, publisher = {American Chemical Society}, address = {Washington}, issn = {1089-5639}, doi = {10.1021/acs.jpca.0c09911}, pages = {11017 -- 11024}, year = {2020}, abstract = {9,10-substituted anthracenes are known for their useful optical properties like fluorescence, which makes them frequently used probes in sensing applications. In this article, we investigate the fundamental photophysical properties of three pyridyl-substituted variants. The nitrogen atoms in the pyridinium six-membered rings are located in the ortho-, meta-, and para-positions in relation to the anthracene core. Absorption, fluorescence, and transient absorption measurements were carried out and were complemented by theoretical calculations. We monitored the photophysics of the anthracene derivatives in chloroform and water investigating the protonated as well as their nonprotonated forms. We found that the optical properties of the nonprotonated forms are strongly determined by the anthracene chromophore, with only small differences to other 9,10-substituted anthracenes, for example diphenyl anthracene. In contrast, protonation leads to a strong decrease in fluorescence intensity and lifetime. Transient absorption measurements and theoretical calculations revealed the formation of a charge-transfer state in the protonated chromophores, where electron density is shifted from the anthracene moiety toward the protonated pyridyl substituents. While the para- and ortho-derivatives' charge transfer is still moderately fluorescent, the meta-derivative is affected much stronger and shows nearly no fluorescence. This nitrogen-atom-position-dependent sensitivity to hydronium activity makes a combination of these fluorophores very attractive for pH-sensing applications covering a broadened pH range.}, language = {en} } @article{MalassTarkhanov2020, author = {Malass, Ihsane and Tarkhanov, Nikolaj Nikolaevič}, title = {A perturbation of the de Rham complex}, series = {Journal of Siberian Federal University : Mathematics \& Physics}, volume = {13}, journal = {Journal of Siberian Federal University : Mathematics \& Physics}, number = {5}, publisher = {Siberian Federal University}, address = {Krasnojarsk}, issn = {1997-1397}, doi = {10.17516/1997-1397-2020-13-5-519-532}, pages = {519 -- 532}, year = {2020}, abstract = {We consider a perturbation of the de Rham complex on a compact manifold with boundary. This perturbation goes beyond the framework of complexes, and so cohomology does not apply to it. On the other hand, its curvature is "small", hence there is a natural way to introduce an Euler characteristic and develop a Lefschetz theory for the perturbation. This work is intended as an attempt to develop a cohomology theory for arbitrary sequences of linear mappings.}, language = {en} } @article{AbdallaAdamAharonianetal.2020, author = {Abdalla, Hassan E. and Adam, Remi and Aharonian, Felix A. and Benkhali, Faical Ait and Ang{\"u}ner, Ekrem Oǧuzhan and Arakawa, Masanori and Arcaro, C and Armand, Catherine and Armstrong, T. and Egberts, Kathrin}, title = {Very high energy γ-ray emission from two blazars of unknown redshift and upper limits on their distance}, series = {Monthly Notices of the Royal Astronomical Society}, volume = {494}, journal = {Monthly Notices of the Royal Astronomical Society}, number = {4}, publisher = {Wiley-Blackwell}, address = {Oxford}, pages = {13}, year = {2020}, abstract = {We report on the detection of very high energy (VHE; E > 100 GeV) gamma-ray emission from the BL Lac objects KUV 00311-1938 and PKS 1440-389 with the High Energy Stereoscopic System (H.E.S.S.). H.E.S.S. observations were accompanied or preceded by multiwavelength observations with Fermi/LAT, XRT and UVOT onboard the Swift satellite, and ATOM. Based on an extrapolation of the Fermi/LAT spectrum towards the VHE gamma-ray regime, we deduce a 95 per cent confidence level upper limit on the unknown redshift of KUV 00311-1938 of z < 0.98 and of PKS 1440-389 of z < 0.53. When combined with previous spectroscopy results, the redshift of KUV 00311-1938 is constrained to 0.51 <= z < 0.98 and of PKS 1440-389 to 0.14 (sic) z < 0.53.}, language = {en} } @article{Teichmann2021, author = {Teichmann, Erik}, title = {Using phase dynamics to study partial synchrony}, series = {European physical journal special topics}, volume = {230}, journal = {European physical journal special topics}, number = {14-15}, publisher = {Springer}, address = {Heidelberg}, issn = {1951-6355}, doi = {10.1140/epjs/s11734-021-00156-3}, pages = {2833 -- 2842}, year = {2021}, abstract = {Partial synchronous states appear between full synchrony and asynchrony and exhibit many interesting properties. Most frequently, these states are studied within the framework of phase approximation. The latter is used ubiquitously to analyze coupled oscillatory systems. Typically, the phase dynamics description is obtained in the weak coupling limit, i.e., in the first-order in the coupling strength. The extension beyond the first-order represents an unsolved problem and is an active area of research. In this paper, three partially synchronous states are investigated and presented in order of increasing complexity. First, the usage of the phase response curve for the description of macroscopic oscillators is analyzed. To achieve this, the response of the mean-field oscillations in a model of all-to-all coupled limit-cycle oscillators to pulse stimulation is measured. The next part treats a two-group Kuramoto model, where the interaction of one attractive and one repulsive group results in an interesting solitary state, situated between full synchrony and self-consistent partial synchrony. In the last part, the phase dynamics of a relatively simple system of three Stuart-Landau oscillators are extended beyond the weak coupling limit. The resulting model contains triplet terms in the high-order phase approximation, though the structural connections are only pairwise. Finally, the scaling of the new terms with the coupling is analyzed.}, language = {en} } @article{Schirdewahn2020, author = {Schirdewahn, Daniel}, title = {Stability of a parametric harmonic oscillator with dichotomic noise}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {30}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {9}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/5.0012946}, pages = {7}, year = {2020}, abstract = {The harmonic oscillator is a powerful model that can appear as a limit case when examining a nonlinear system. A well known fact is that, without driving, the inclusion of a friction term makes the origin of the phase space-which is a fixed point of the system-linearly stable. In this work, we include a telegraph process as perturbation of the oscillator's frequency, for example, to describe the motion of a particle with fluctuating charge gyrating in an external magnetic field. Increasing intensity of this colored noise is capable of changing the quality of the fixed point. To characterize the stability of the system, we use a stability measure that describes the growth of the displacement of the system's phase space position and express it in a closed form. We expand the respective exponent for light friction and low noise intensity and compare both the exact analytic solution and the expansion to numerical values. Our findings allow stability predictions for several physical systems.}, language = {en} } @article{Rosenblum2020, author = {Rosenblum, Michael}, title = {Controlling collective synchrony in oscillatory ensembles by precisely timed pulses}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {30}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {9}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/5.0019823}, pages = {9}, year = {2020}, abstract = {We present an efficient technique for control of synchrony in a globally coupled ensemble by pulsatile action. We assume that we can observe the collective oscillation and can stimulate all elements of the ensemble simultaneously. We pay special attention to the minimization of intervention into the system. The key idea is to stimulate only at the most sensitive phase. To find this phase, we implement an adaptive feedback control. Estimating the instantaneous phase of the collective mode on the fly, we achieve efficient suppression using a few pulses per oscillatory cycle. We discuss the possible relevance of the results for neuroscience, namely, for the development of advanced algorithms for deep brain stimulation, a medical technique used to treat Parkinson's disease.}, language = {en} } @article{BetaKruse2017, author = {Beta, Carsten and Kruse, Karsten}, title = {Intracellular oscillations and waves}, series = {Annual review of condensed matter physics}, volume = {8}, journal = {Annual review of condensed matter physics}, publisher = {Annual Reviews}, address = {Palo Alto}, isbn = {978-0-8243-5008-6}, issn = {1947-5454}, doi = {10.1146/annurev-conmatphys-031016-025210}, pages = {239 -- 264}, year = {2017}, abstract = {Dynamic processes in living cells are highly organized in space and time. Unraveling the underlying molecular mechanisms of spatiotemporal pattern formation remains one of the outstanding challenges at the interface between physics and biology. A fundamental recurrent pattern found in many different cell types is that of self-sustained oscillations. They are involved in a wide range of cellular functions, including second messenger signaling, gene expression, and cytoskeletal dynamics. Here, we review recent developments in the field of cellular oscillations and focus on cases where concepts from physics have been instrumental for understanding the underlying mechanisms. We consider biochemical and genetic oscillators as well as oscillations that arise from chemo-mechanical coupling. Finally, we highlight recent studies of intracellular waves that have increasingly moved into the focus of this research field.}, language = {en} } @article{RubioAndersCorrea2021, author = {Rubio, Jes{\´u}s and Anders, Janet and Correa, Luis A.}, title = {Global quantum thermometry}, series = {Physical review letters / publ. by the American Physical Society}, volume = {127}, journal = {Physical review letters / publ. by the American Physical Society}, number = {19}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.127.190402}, pages = {6}, year = {2021}, abstract = {A paradigm shift in quantum thermometry is proposed. To date, thermometry has relied on local estimation, which is useful to reduce statistical fluctuations once the temperature is very well known. In order to estimate temperatures in cases where few measurement data or no substantial prior knowledge are available, we build instead a method for global quantum thermometry. Based on scaling arguments, a mean logarithmic error is shown here to be the correct figure of merit for thermometry. Its full minimization provides an operational and optimal rule to postprocess measurements into a temperature reading, and it establishes a global precision limit. We apply these results to the simulated outcomes of measurements on a spin gas, finding that the local approach can lead to biased temperature estimates in cases where the global estimator converges to the true temperature. The global framework thus enables a reliable approach to data analysis in thermometry experiments.}, language = {en} } @article{PalyulinAlaNissilaMetzler2014, author = {Palyulin, Vladimir V. and Ala-Nissila, Tapio and Metzler, Ralf}, title = {Polymer translocation: the first two decades and the recent diversification}, series = {Soft matter}, volume = {45}, journal = {Soft matter}, number = {10}, editor = {Metzler, Ralf}, publisher = {the Royal Society of Chemistry}, address = {Cambridge}, issn = {1744-683X}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76266}, pages = {9016 -- 9037}, year = {2014}, abstract = {Probably no other field of statistical physics at the borderline of soft matter and biological physics has caused such a flurry of papers as polymer translocation since the 1994 landmark paper by Bezrukov, Vodyanoy, and Parsegian and the study of Kasianowicz in 1996. Experiments, simulations, and theoretical approaches are still contributing novel insights to date, while no universal consensus on the statistical understanding of polymer translocation has been reached. We here collect the published results, in particular, the famous-infamous debate on the scaling exponents governing the translocation process. We put these results into perspective and discuss where the field is going. In particular, we argue that the phenomenon of polymer translocation is non-universal and highly sensitive to the exact specifications of the models and experiments used towards its analysis.}, language = {en} }