@article{AliuAuneBarnackaetal.2014, author = {Aliu, E. and Aune, T. and Barnacka, Anna and Beilicke, M. and Benbow, W. and Berger, K. and Biteau, Jonathan and Buckley, J. H. and Bugaev, V. and Byrum, K. and Cardenzana, J. V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Connaughton, V. and Cui, W. and Dickinson, H. J. and Eisch, J. D. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hakansson, Nils and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kar, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McArthur, S. and McCann, A. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Pueschel, Elisa and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sembroski, G. H. and Shahinyan, K. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weiner, O. M. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B. and McEnery, J. E. and Perkins, J. S. and Veres, P. and Zhu, S.}, title = {Constraints on very high energy emission from GRB 130427A}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, volume = {795}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {2041-8205}, doi = {10.1088/2041-8205/795/1/L3}, pages = {6}, year = {2014}, abstract = {Prompt emission from the very fluent and nearby (z = 0.34) gamma-ray burst GRB130427A was detected by several orbiting telescopes and by ground-based, wide-field-of-view optical transient monitors. Apart from the intensity and proximity of this GRB, it is exceptional due to the extremely long-lived high-energy (100 MeV to 100 GeV) gamma-ray emission, which was detected by the Large Area Telescope on the Fermi Gamma-Ray Space Telescope for similar to 70 ks after the initial burst. The persistent, hard-spectrum, high-energy emission suggests that the highest-energy gamma rays may have been produced via synchrotron self-Compton processes though there is also evidence that the high-energy emission may instead be an extension of the synchrotron spectrum. VERITAS, a ground-based imaging atmospheric Cherenkov telescope array, began follow-up observations of GRB130427A similar to 71 ks (similar to 20 hr) after the onset of the burst. The GRB was not detected with VERITAS; however, the high elevation of the observations, coupled with the low redshift of the GRB, make VERITAS a very sensitive probe of the emission from GRB130427A for E > 100 GeV. The non-detection and consequent upper limit derived place constraints on the synchrotron self-Compton model of high-energy gamma-ray emission from this burst.}, language = {en} } @article{SchmaelzlinMoralejoRutowskaetal.2014, author = {Schmaelzlin, Elmar and Moralejo, Benito and Rutowska, Monika and Monreal-Ibero, Ana and Sandin, Christer and Tarcea, Nicolae and Popp, Juergen and Roth, Martin M.}, title = {Raman imaging with a fiber-coupled multichannel spectrograph}, series = {Sensors}, volume = {14}, journal = {Sensors}, number = {11}, publisher = {MDPI}, address = {Basel}, issn = {1424-8220}, doi = {10.3390/s141121968}, pages = {21968 -- 21980}, year = {2014}, abstract = {Until now, spatially resolved Raman Spectroscopy has required to scan a sample under investigation in a time-consuming step-by-step procedure. Here, we present a technique that allows the capture of an entire Raman image with only one single exposure. The Raman scattering arising from the sample was collected with a fiber-coupled high-performance astronomy spectrograph. The probe head consisting of an array of 20 x 20 multimode fibers was linked to the camera port of a microscope. To demonstrate the high potential of this new concept, Raman images of reference samples were recorded. Entire chemical maps were received without the need for a scanning procedure.}, language = {en} } @article{PalyulinChechkinMetzler2014, author = {Palyulin, Vladimir V. and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Space-fractional Fokker-Planck equation and optimization of random search processes in the presence of an external bias}, series = {Journal of statistical mechanics: theory and experiment}, journal = {Journal of statistical mechanics: theory and experiment}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1742-5468}, doi = {10.1088/1742-5468/2014/11/P11031}, pages = {32}, year = {2014}, abstract = {Based on the space-fractional Fokker-Planck equation with a delta-sink term, we study the efficiency of random search processes based on Levy flights with power-law distributed jump lengths in the presence of an external drift, for instance, an underwater current, an airflow, or simply the preference of the searcher based on prior experience. While Levy flights turn out to be efficient search processes when the target is upstream relative to the starting point, in the downstream scenario, regular Brownian motion turns out to be advantageous. This is caused by the occurrence of leapovers of Levy flights, due to which Levy flights typically overshoot a point or small interval. Studying the solution of the fractional Fokker-Planck equation, we establish criteria when the combination of the external stream and the initial distance between the starting point and the target favours Levy flights over the regular Brownian search. Contrary to the common belief that Levy flights with a Levy index alpha = 1 (i.e. Cauchy flights) are optimal for sparse targets, we find that the optimal value for alpha may range in the entire interval (1, 2) and explicitly include Brownian motion as the most efficient search strategy overall.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and B{\"o}ttcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Forster, A. and Fuling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadsch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, Markus and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kiefeer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Kruger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puhlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schussler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and Van Eldik, C. and Van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Volk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Wornlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Long-term monitoring of PKS2155-304 with ATOM and HESS:investigation of optical/gamma-ray correlations in different spectral states}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {571}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, organization = {HESSS Collaboration}, issn = {0004-6361}, doi = {10.1051/0004-6361/201424142}, pages = {10}, year = {2014}, abstract = {In this paper we report on the analysis of all the available optical and very high-energy gamma-ray (> 200 GeV) data for the BL Lac object PKS 2155-304, collected simultaneously with the ATOM and H.E.S.S. telescopes from 2007 until 2009. This study also includes X-ray (RXTE, Swift) and high-energy gamma-ray (Fermi-LAT) data. During the period analysed, the source was transitioning from its flaring to quiescent optical states, and was characterized by only moderate flux changes at different wavelengths on the timescales of days and months. A flattening of the optical continuum with an increasing optical flux can be noted in the collected dataset, but only occasionally and only at higher flux levels. We did not find any universal relation between the very high-energy gamma-ray and optical flux changes on the timescales from days and weeks up to several years. On the other hand, we noted that at higher flux levels the source can follow two distinct tracks in the optical flux-colour diagrams, which seem to be related to distinct gamma-ray states of the blazar. The obtained results therefore indicate a complex scaling between the optical and gamma-ray emission of PKS 2155 304, with different correlation patterns holding at different epochs, and a gamma-ray flux depending on the combination of an optical flux and colour rather than a flux alone.}, language = {en} } @article{SchickHerzogBojahretal.2014, author = {Schick, Daniel and Herzog, Marc and Bojahr, Andre and Leitenberger, Wolfram and Hertwig, Andreas and Shayduk, Roman and Bargheer, Matias}, title = {Ultrafast lattice response of photoexcited thin films studied by X-ray diffraction}, series = {Structural dynamics}, volume = {1}, journal = {Structural dynamics}, number = {6}, publisher = {American Institute of Physics}, address = {Melville}, issn = {2329-7778}, doi = {10.1063/1.4901228}, pages = {13}, year = {2014}, abstract = {Using ultrafast X-ray diffraction, we study the coherent picosecond lattice dynamics of photoexcited thin films in the two limiting cases, where the photoinduced stress profile decays on a length scale larger and smaller than the film thickness. We solve a unifying analytical model of the strain propagation for acoustic impedance-matched opaque films on a semi-infinite transparent substrate, showing that the lattice dynamics essentially depend on two parameters: One for the spatial profile and one for the amplitude of the strain. We illustrate the results by comparison with high-quality ultrafast X-ray diffraction data of SrRuO3 films on SrTiO3 substrates. (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.}, language = {en} } @unpublished{HenkelPieplow2014, author = {Henkel, Carsten and Pieplow, Gregor}, title = {Reply to Comment on 'Fully covariant radiation force on a polarizable particle'}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/11/118002}, pages = {8}, year = {2014}, abstract = {We argue that the theories of Volokitin and Persson (2014 New J. Phys. 16 118001), Dedkov and Kyasov (2008 J. Phys.: Condens. Matter 20 354006), and Pieplow and Henkel (2013 New J. Phys. 15 023027) agree on the electromagnetic force on a small, polarizable particle that is moving parallel to a planar, macroscopic body, as far as the contribution of evanescent waves is concerned. The apparent differences are discussed in detail and explained by choices of units and integral transformations. We point out in particular the role of the Lorentz contraction in the procedure used by Volokitin and Persson, where a macroscopic body is 'diluted' to obtain the force on a small particle. Differences that appear in the contribution of propagating photons are briefly mentioned.}, language = {en} } @article{LiAbrechtYangetal.2014, author = {Li, Wentao and Abrecht, Steve and Yang, Liqiang and Roland, Steffen and Tumbleston, John R. and McAfee, Terry and Yan, Liang and Kelly, Mary Allison and Ade, Harald W. and Neher, Dieter and You, Wei}, title = {Mobility-controlled performance of thick solar cells based on fluorinated copolymers}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {44}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja5067724}, pages = {15566 -- 15576}, year = {2014}, abstract = {Developing novel materials and device architectures to further enhance the efficiency of polymer solar cells requires a fundamental understanding of the impact of chemical structures on photovoltaic properties. Given that device characteristics depend on many parameters, deriving structureproperty relationships has been very challenging. Here we report that a single parameter, hole mobility, determines the fill factor of several hundred nanometer thick bulk heterojunction photovoltaic devices based on a series of copolymers with varying amount of fluorine substitution. We attribute the steady increase of hole mobility with fluorine content to changes in polymer molecular ordering. Importantly, all other parameters, including the efficiency of free charge generation and the coefficient of nongeminate recombination, are nearly identical. Our work emphasizes the need to achieve high mobility in combination with strongly suppressed charge recombination for the thick devices required by mass production technologies.}, language = {en} } @article{ZamponiPenfoldNachtegaaletal.2014, author = {Zamponi, Flavio and Penfold, Thomas J. and Nachtegaal, Maarten and Luebcke, Andrea and Rittmann, Jochen and Milne, Chris J. and Chergui, Majed and van Bokhoven, Jeroen A.}, title = {Probing the dynamics of plasmon-excited hexanethiol-capped gold nanoparticles by picosecond X-ray absorption spectroscopy}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {42}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c4cp03301a}, pages = {23157 -- 23163}, year = {2014}, abstract = {Picosecond X-ray absorption spectroscopy (XAS) is used to investigate the electronic and structural dynamics initiated by plasmon excitation of 1.8 nm diameter Au nanoparticles (NPs) functionalised with 1-hexanethiol. We show that 100 ps after photoexcitation the transient XAS spectrum is consistent with an 8\% expansion of the Au-Au bond length and a large increase in disorder associated with melting of the NPs. Recovery of the ground state occurs with a time constant of similar to 1.8 ns, arising from thermalisation with the environment. Simulations reveal that the transient spectrum exhibits no signature of charge separation at 100 ps and allows us to estimate an upper limit for the quantum yield (QY) of this process to be <0.1.}, language = {en} } @article{QiuWirgesGerhard2014, author = {Qiu, Xunlin and Wirges, Werner and Gerhard, Reimund}, title = {Polarization and Hysteresis in Tubular-Channel Fluoroethylenepropylene-Copolymer Ferroelectrets}, series = {Ferroelectrics}, volume = {472}, journal = {Ferroelectrics}, number = {1}, publisher = {Routledge, Taylor \& Francis Group}, address = {Abingdon}, issn = {0015-0193}, doi = {10.1080/00150193.2014.964603}, pages = {100 -- 109}, year = {2014}, abstract = {Polarization-vs.-applied-voltage hysteresis curves are recorded on tubular-channel fluoroethylene-propylene (FEP) copolymer ferroelectrets by means of a modified Sawyer-Tower circuit. Dielectric barrier discharges (DBDs) inside the cavities are triggered when the applied voltage is sufficiently high. During the DBDs, the cavities become man-made macroscopic dipoles which build up an effective polarization in the ferroelectret. Therefore, a phenomenological hysteresis curve is observed. From the hysteresis loop, the remanent polarization and the coercive field can be determined. Furthermore, the polarization can be related to the respective piezoelectric coefficient of the ferroelectret. The proposed method is easy to implement and is useful for characterization, further development and optimization of ferro- or piezoelectrets.}, language = {en} } @unpublished{HilczerGerhardScott2014, author = {Hilczer, B{\"o}rn and Gerhard, Reimund and Scott, James F.}, title = {Special Issue of Ferroelectrics in Honor of S. B. Lang}, series = {Ferroelectrics}, volume = {472}, journal = {Ferroelectrics}, number = {1}, publisher = {Routledge, Taylor \& Francis Group}, address = {Abingdon}, issn = {0015-0193}, doi = {10.1080/00150193.2014.964099}, pages = {VII -- VIII}, year = {2014}, language = {en} } @unpublished{Gerhard2014, author = {Gerhard, Reimund}, title = {Sidney Lang - his collaboration with the University of Potsdam}, series = {Ferroelectrics}, volume = {472}, journal = {Ferroelectrics}, number = {1}, publisher = {Routledge, Taylor \& Francis Group}, address = {Abingdon}, issn = {0015-0193}, doi = {10.1080/00150193.2014.967090}, pages = {5 -- 5}, year = {2014}, language = {en} } @article{EvansMurphyWhitmoreetal.2014, author = {Evans, T. M. and Murphy, M. T. and Whitmore, J. B. and Misawa, T. and Centurion, Martin and Lopez, S. and Martins, C. J. A. P. and Molaro, P. and Petitjean, P. and Rahmani, H. and Srianand, R. and Wendt, Martin}, title = {The UVES Large Program for testing fundamental physics - III. Constraints on the fine-structure constant from three telescopes}, series = {Monthly notices of the Royal Astronomical Society}, volume = {445}, journal = {Monthly notices of the Royal Astronomical Society}, number = {1}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu1754}, pages = {128 -- 150}, year = {2014}, language = {en} } @article{SandersLomholtLizanaetal.2014, author = {Sanders, Lloyd P. and Lomholt, Michael A. and Lizana, Ludvig and Fogelmark, Karl and Metzler, Ralf and Ambjoernsson, Tobias}, title = {Severe slowing-down and universality of the dynamics in disordered interacting many-body systems: ageing and ultraslow diffusion}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/11/113050}, pages = {14}, year = {2014}, abstract = {Low-dimensional, many-body systems are often characterized by ultraslow dynamics. We study a labelled particle in a generic system of identical particles with hard-core interactions in a strongly disordered environment. The disorder is manifested through intermittent motion with scale-free sticking times at the single particle level. While for a non-interacting particle we find anomalous diffusion of the power-law form < x(2)(t)> similar or equal to t(alpha) of the mean squared displacement with 0 < alpha < 1, we demonstrate here that the combination of the disordered environment with the many-body interactions leads to an ultraslow, logarithmic dynamics < x(2)(t)> similar or equal to log(1/2)t with a universal 1/2 exponent. Even when a characteristic sticking time exists but the fluctuations of sticking times diverge we observe the mean squared displacement < x(2)(t)> similar or equal to t(gamma) with 0 < gamma < 1/2, that is slower than the famed Harris law < x(2)(t)> similar or equal to t(1/2) without disorder. We rationalize the results in terms of a subordination to a counting process, in which each transition is dominated by the forward waiting time of an ageing continuous time process.}, language = {en} } @article{LangeReiterPaetzeletal.2014, author = {Lange, Ilja and Reiter, Sina and Paetzel, Michael and Zykov, Anton and Nefedov, Alexei and Hildebrandt, Jana and Hecht, Stefan and Kowarik, Stefan and Woell, Christof and Heimel, Georg and Neher, Dieter}, title = {Tuning the work function of polar zinc oxide surfaces using modified phosphonic acid self-assembled monolayers}, series = {Advanced functional materials}, volume = {24}, journal = {Advanced functional materials}, number = {44}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1616-301X}, doi = {10.1002/adfm.201401493}, pages = {7014 -- 7024}, year = {2014}, abstract = {Zinc oxide (ZnO) is regarded as a promising alternative material for transparent conductive electrodes in optoelectronic devices. However, ZnO suffers from poor chemical stability. ZnO also has a moderate work function (WF), which results in substantial charge injection barriers into common (organic) semiconductors that constitute the active layer in a device. Controlling and tuning the ZnO WF is therefore necessary but challenging. Here, a variety of phosphonic acid based self-assembled monolayers (SAMs) deposited on ZnO surfaces are investigated. It is demonstrated that they allow the tuning the WF over a wide range of more than 1.5 eV, thus enabling the use of ZnO as both the hole-injecting and electron-injecting contact. The modified ZnO surfaces are characterized using a number of complementary techniques, demonstrating that the preparation protocol yields dense, well-defined molecular monolayers.}, language = {en} } @article{GerhardtWalzBeta2014, author = {Gerhardt, Matthias and Walz, Michael and Beta, Carsten}, title = {Signaling in chemotactic amoebae remains spatially confined to stimulated membrane regions}, series = {Journal of cell science}, volume = {127}, journal = {Journal of cell science}, number = {23}, publisher = {Company of Biologists Limited}, address = {Cambridge}, issn = {0021-9533}, doi = {10.1242/jcs.161133}, pages = {5115 -- 5125}, year = {2014}, abstract = {Recent work has demonstrated that the receptor-mediated signaling system in chemotactic amoeboid cells shows typical properties of an excitable system. Here, we delivered spatially confined stimuli of the chemoattractant cAMP to the membrane of differentiated Dictyostelium discoideum cells to investigate whether localized receptor stimuli can induce the spreading of excitable waves in the G-protein-dependent signal transduction system. By imaging the spatiotemporal dynamics of fluorescent markers for phosphatidylinositol (3,4,5)-trisphosphate (PIP3), PTEN and filamentous actin, we observed that the activity of the signaling pathway remained spatially confined to the stimulated membrane region. Neighboring parts of the membrane were not excited and no receptor-initiated spatial spreading of excitation waves was observed. To generate localized cAMP stimuli, either particles that carried covalently bound cAMP molecules on their surface were brought into contact with the cell or a patch of the cell membrane was aspirated into a glass micropipette to shield this patch against freely diffusing cAMP molecules in the surrounding medium. Additionally, the binding site of the cAMP receptor was probed with different surface-immobilized cAMP molecules, confirming results from earlier ligand-binding studies.}, language = {en} } @article{RichterZakrevskyyEiseleetal.2014, author = {Richter, Marcel and Zakrevskyy, Yuriy and Eisele, Michael and Lomadze, Nino and Santer, Svetlana and von Klitzing, Regine}, title = {Effect of pH, co-monomer content, and surfactant structure on the swelling behavior of microgel-azobenzene-containing surfactant complex}, series = {Polymer : the international journal for the science and technology of polymers}, volume = {55}, journal = {Polymer : the international journal for the science and technology of polymers}, number = {25}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-3861}, doi = {10.1016/j.polymer.2014.10.027}, pages = {6513 -- 6518}, year = {2014}, abstract = {The contraction/swelling transition of anionic PNIPAM-co-AAA particles can be manipulated by light using interactions with cationic azobenzene-containing surfactant. In this study the influence of pH-buffers and their concentrations, the charge density (AAA content) in microgel particles as well as the spacer length of the surfactant on the complex formation between the microgel and surfactant is investigated. It is shown that the presence of pH buffer can lead to complete blocking of the interactions in such complexes and the resulting microgel contraction/swelling response. There is a clear competition between the buffer ions and the surfactant molecules interacting with microgel particles. When working in pure water solutions with fixed concentration (charge density) of microgel, the contraction/swelling of the particles is controlled only by relative concentration (charge ratio) of the surfactant and AAA groups of the microgel. Furthermore, the particle contraction is more efficient for shorter spacer length of the surfactant. The onset point of the contraction process is not affected by the surfactant hydrophobicity. This work provides new insight into the interaction between microgel particles and photo-sensitive surfactants, which offers high potential in new sensor systems. (C) 2014 Elsevier Ltd. All rights reserved.}, language = {en} } @article{MetzlerSandersLomholtetal.2014, author = {Metzler, Ralf and Sanders, L. and Lomholt, M. A. and Lizana, L. and Fogelmark, K. and Ambjoernsson, Tobias}, title = {Ageing single file motion}, series = {The European physical journal}, volume = {223}, journal = {The European physical journal}, number = {14}, publisher = {Springer}, address = {Heidelberg}, issn = {1951-6355}, doi = {10.1140/epjst/e2014-02333-5}, pages = {3287 -- 3293}, year = {2014}, language = {en} } @article{LepriPikovskij2014, author = {Lepri, Stefano and Pikovskij, Arkadij}, title = {Nonreciprocal wave scattering on nonlinear string-coupled oscillators}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {24}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {4}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/1.4899205}, pages = {9}, year = {2014}, abstract = {We study scattering of a periodic wave in a string on two lumped oscillators attached to it. The equations can be represented as a driven (by the incident wave) dissipative (due to radiation losses) system of delay differential equations of neutral type. Nonlinearity of oscillators makes the scattering non-reciprocal: The same wave is transmitted differently in two directions. Periodic regimes of scattering are analyzed approximately, using amplitude equation approach. We show that this setup can act as a nonreciprocal modulator via Hopf bifurcations of the steady solutions. Numerical simulations of the full system reveal nontrivial regimes of quasiperiodic and chaotic scattering. Moreover, a regime of a "chaotic diode," where transmission is periodic in one direction and chaotic in the opposite one, is reported. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{ArridgeAchilleosAgarwaletal.2014, author = {Arridge, Christopher S. and Achilleos, N. and Agarwal, Jessica and Agnor, C. B. and Ambrosi, R. and Andre, N. and Badman, S. V. and Baines, K. and Banfield, D. and Barthelemy, M. and Bisi, M. M. and Blum, J. and Bocanegra-Bahamon, T. and Bonfond, B. and Bracken, C. and Brandt, P. and Briand, C. and Briois, C. and Brooks, S. and Castillo-Rogez, J. and Cavalie, T. and Christophe, B. and Coates, Andrew J. and Collinson, G. and Cooper, John F. and Costa-Sitja, M. and Courtin, R. and Daglis, I. A. and De Pater, Imke and Desai, M. and Dirkx, D. and Dougherty, M. K. and Ebert, R. W. and Filacchione, Gianrico and Fletcher, Leigh N. and Fortney, J. and Gerth, I. and Grassi, D. and Grodent, D. and Gr{\"u}n, Eberhard and Gustin, J. and Hedman, M. and Helled, R. and Henri, P. and Hess, Sebastien and Hillier, J. K. and Hofstadter, M. H. and Holme, R. and Horanyi, M. and Hospodarsky, George B. and Hsu, S. and Irwin, P. and Jackman, C. M. and Karatekin, O. and Kempf, Sascha and Khalisi, E. and Konstantinidis, K. and Kruger, H. and Kurth, William S. and Labrianidis, C. and Lainey, V. and Lamy, L. L. and Laneuville, Matthieu and Lucchesi, D. and Luntzer, A. and MacArthur, J. and Maier, A. and Masters, A. and McKenna-Lawlor, S. and Melin, H. and Milillo, A. and Moragas-Klostermeyer, Georg and Morschhauser, Achim and Moses, J. I. and Mousis, O. and Nettelmann, N. and Neubauer, F. M. and Nordheim, T. and Noyelles, B. and Orton, G. S. and Owens, Mathew and Peron, R. and Plainaki, C. and Postberg, F. and Rambaux, N. and Retherford, K. and Reynaud, Serge and Roussos, Elias and Russell, C. T. and Rymer, Am. and Sallantin, R. and Sanchez-Lavega, A. and Santolik, O. and Saur, J. and Sayanagi, Km. and Schenk, P. and Schubert, J. and Sergis, N. and Sittler, E. C. and Smith, A. and Spahn, Frank and Srama, Ralf and Stallard, T. and Sterken, V. and Sternovsky, Zoltan and Tiscareno, M. and Tobie, G. and Tosi, F. and Trieloff, M. and Turrini, D. and Turtle, E. P. and Vinatier, S. and Wilson, R. and Zarkat, P.}, title = {The science case for an orbital mission to Uranus: Exploring the origins and evolution of ice giant planets}, series = {Planetary and space science}, volume = {104}, journal = {Planetary and space science}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-0633}, doi = {10.1016/j.pss.2014.08.009}, pages = {122 -- 140}, year = {2014}, abstract = {Giant planets helped to shape the conditions we see in the Solar System today and they account for more than 99\% of the mass of the Sun's planetary system. They can be subdivided into the Ice Giants (Uranus and Neptune) and the Gas Giants (Jupiter and Saturn), which differ from each other in a number of fundamental ways. Uranus, in particular is the most challenging to our understanding of planetary formation and evolution, with its large obliquity, low self-luminosity, highly asymmetrical internal field, and puzzling internal structure. Uranus also has a rich planetary system consisting of a system of inner natural satellites and complex ring system, five major natural icy satellites, a system of irregular moons with varied dynamical histories, and a highly asymmetrical magnetosphere. Voyager 2 is the only spacecraft to have explored Uranus, with a flyby in 1986, and no mission is currently planned to this enigmatic system. However, a mission to the uranian system would open a new window on the origin and evolution of the Solar System and would provide crucial information on a wide variety of physicochemical processes in our Solar System. These have clear implications for understanding exoplanetary systems. In this paper we describe the science case for an orbital mission to Uranus with an atmospheric entry probe to sample the composition and atmospheric physics in Uranus' atmosphere. The characteristics of such an orbiter and a strawman scientific payload are described and we discuss the technical challenges for such a mission. This paper is based on a white paper submitted to the European Space Agency's call for science themes for its large-class mission programme in 2013.}, language = {en} } @article{TobieTeanbyCoustenisetal.2014, author = {Tobie, G. and Teanby, N. A. and Coustenis, A. and Jaumann, Ralf and Raulin, E. and Schmidt, J. and Carrasco, N. and Coates, Andrew J. and Cordier, D. and De Kok, R. and Geppert, W. D. and Lebreton, J. -P. and Lefevre, A. and Livengood, T. A. and Mandt, K. E. and Mitri, G. and Nimmo, F. and Nixon, C. A. and Norman, L. and Pappalardo, R. T. and Postberg, F. and Rodriguez, S. and SchuizeMakuch, D. and Soderblom, J. M. and Solomonidou, A. and Stephan, K. and Stofan, E. R. and Turtle, E. P. and Wagner, R. J. and West, R. A. and Westlake, J. H.}, title = {Science goals and mission concept for the future exploration of Titan and Enceladus}, series = {Planetary and space science}, volume = {104}, journal = {Planetary and space science}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-0633}, doi = {10.1016/j.pss.2014.10.002}, pages = {59 -- 77}, year = {2014}, language = {en} } @article{MiedemaBeyeKoenneckeetal.2014, author = {Miedema, Piter Sybren and Beye, Martin and Koennecke, R. and Schiwietz, Gregor and F{\"o}hlisch, Alexander}, title = {Thermal evolution of the band edges of 6H-SiC: X-ray methods compared to the optical band gap}, series = {Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy}, volume = {197}, journal = {Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0368-2048}, doi = {10.1016/j.elspec.2014.08.003}, pages = {37 -- 42}, year = {2014}, abstract = {The band gap of semiconductors like silicon and silicon carbide (SIC) is the key for their device properties. In this research, the band gap of 6H-SiC and its temperature dependence were analyzed with silicon 2p X-ray absorption spectroscopy (XAS), X-ray emission spectroscopy (XES) and resonant inelastic X-ray scattering (RIXS) allowing for a separate analysis of the conduction-band minimum (CBM) and valence-band maximum (VBM) components of the band gap. The temperature-dependent asymmetric band gap shrinking of 6H-SiC was determined with a valence-band slope of +2.45 x 10(-4) eV/K and a conduction-band slope of -1.334 x 10(-4) eV/K. The apparent asymmetry, e.g., that two thirds of the band-gap shrinking with increasing temperature is due to the VBM evolution in 6H-SiC, is similar to the asymmetry obtained for pure silicon before. The overall band gap temperature-dependence determined with XAS and nonresonant XES is compared to temperature-dependent optical studies. The core-excitonic binding energy appearing in the Si 2p XAS is extracted as the main difference. In addition, the energy loss of the onset of the first band in RIXS yields to values similar to the optical band gap over the tested temperature range. (C) 2014 Elsevier B.V. All rights reserved.}, language = {en} } @article{MeierKriegelMotschmannetal.2014, author = {Meier, Patrick and Kriegel, Hendrik and Motschmann, Uwe and Schmidt, J{\"u}rgen and Spahn, Frank and Hill, Thomas W. and Dong, Yaxue and Jones, Geraint H.}, title = {A model of the spatial and size distribution of Enceladus' dust plume}, series = {Planetary and space science}, volume = {104}, journal = {Planetary and space science}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-0633}, doi = {10.1016/j.pss.2014.09.016}, pages = {216 -- 233}, year = {2014}, language = {en} } @article{ToenjesSokolovPostnikov2014, author = {Toenjes, Ralf and Sokolov, Igor M. and Postnikov, Eugene B.}, title = {Spectral properties of the fractional Fokker-Planck operator for the Levy flight in a harmonic potential}, series = {The European physical journal}, volume = {87}, journal = {The European physical journal}, number = {12}, publisher = {Springer}, address = {New York}, issn = {1434-6028}, doi = {10.1140/epjb/e2014-50558-5}, pages = {11}, year = {2014}, abstract = {We present a detailed analysis of the eigenfunctions of the Fokker-Planck operator for the LevyOrnstein- Uhlenbeck process, their asymptotic behavior and recurrence relations, explicit expressions in coordinate space for the special cases of the Ornstein-Uhlenbeck process with Gaussian and with Cauchy white noise and for the transformation kernel, which maps the fractional Fokker-Planck operator of the Cauchy-Ornstein-Uhlenbeck process to the non-fractional Fokker-Planck operator of the usual Gaussian Ornstein-Uhlenbeck process. We also describe how non-spectral relaxation can be observed in bounded random variables of the Levy-Ornstein-Uhlenbeck process and their correlation functions.}, language = {en} } @article{CherstvyChechkinMetzler2014, author = {Cherstvy, Andrey G. and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Ageing and confinement in non-ergodic heterogeneous diffusion processes}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {47}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {48}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8113/47/48/485002}, pages = {18}, year = {2014}, abstract = {We study the effects of ageing-the time delay between initiation of the physical process at t = 0 and start of observation at some time t(a) > 0-and spatial confinement on the properties of heterogeneous diffusion processes (HDPs) with deterministic power-law space-dependent diffusivities, D(x) = D-0 vertical bar x vertical bar(alpha). From analysis of the ensemble and time averaged mean squared displacements and the ergodicity breaking parameter quantifying the inherent degree of irreproducibility of individual realizations of the HDP we obtain striking similarities to ageing subdiffusive continuous time random walks with scale-free waiting time distributions. We also explore how both processes can be distinguished. For confined HDPs we study the long-time saturation of the ensemble and time averaged particle displacements as well as the magnitude of the inherent scatter of time averaged displacements and contrast the outcomes to the results known for other anomalous diffusion processes under confinement.}, language = {en} } @article{NagelGuvenThevesetal.2014, author = {Nagel, Oliver and Guven, Can and Theves, Matthias and Driscoll, Meghan and Losert, Wolfgang and Beta, Carsten}, title = {Geometry-driven polarity in motile amoeboid cells}, series = {PLoS one}, volume = {9}, journal = {PLoS one}, number = {12}, publisher = {PLoS}, address = {San Fransisco}, issn = {1932-6203}, doi = {10.1371/journal.pone.0113382}, pages = {20}, year = {2014}, abstract = {Motile eukaryotic cells, such as leukocytes, cancer cells, and amoeba, typically move inside the narrow interstitial spacings of tissue or soil. While most of our knowledge of actin-driven eukaryotic motility was obtained from cells that move on planar open surfaces, recent work has demonstrated that confinement can lead to strongly altered motile behavior. Here, we report experimental evidence that motile amoeboid cells undergo a spontaneous symmetry breaking in confined interstitial spaces. Inside narrow channels, the cells switch to a highly persistent, unidirectional mode of motion, moving at a constant speed along the channel. They remain in contact with the two opposing channel side walls and alternate protrusions of their leading edge near each wall. Their actin cytoskeleton exhibits a characteristic arrangement that is dominated by dense, stationary actin foci at the side walls, in conjunction with less dense dynamic regions at the leading edge. Our experimental findings can be explained based on an excitable network model that accounts for the confinement-induced symmetry breaking and correctly recovers the spatio-temporal pattern of protrusions at the leading edge. Since motile cells typically live in the narrow interstitial spacings of tissue or soil, we expect that the geometry-driven polarity we report here plays an important role for movement of cells in their natural environment.}, language = {en} } @article{KraffertSteyrleuthnerAlbrechtetal.2014, author = {Kraffert, Felix and Steyrleuthner, Robert and Albrecht, Steve and Neher, Dieter and Scharber, Markus C. and Bittl, Robert and Behrends, Jan}, title = {Charge Separation in PCPDTBT : PCBM Blends from an EPR Perspective}, series = {The journal of physical chemistry}, volume = {118}, journal = {The journal of physical chemistry}, number = {49}, publisher = {American Chemical Society}, address = {Washington}, issn = {1932-7447}, doi = {10.1021/jp509650v}, pages = {28482 -- 28493}, year = {2014}, language = {en} } @article{GodecChechkinBarkaietal.2014, author = {Godec, Aljaz and Chechkin, Aleksei V. and Barkai, Eli and Kantz, Holger and Metzler, Ralf}, title = {Localisation and universal fluctuations in ultraslow diffusion processes}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {47}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {49}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8113/47/49/492002}, pages = {10}, year = {2014}, abstract = {We study ultraslow diffusion processes with logarithmic mean squared displacement (MSD) < x(2)(t)> similar or equal to log(gamma)t. Comparison of annealed (renewal) continuous time random walks (CTRWs) with logarithmic waiting time distribution psi(tau) similar or equal to 1/(tau log(1+gamma)tau) and Sinai diffusion in quenched random landscapes reveals striking similarities, despite the great differences in their physical nature. In particular, they exhibit a weakly non-ergodic disparity of the time-averaged and ensemble-averaged MSDs. Remarkably, for the CTRW we observe that the fluctuations of time averages become universal, with an exponential suppression of mobile trajectories. We discuss the fundamental connection between the Golosov localization effect and non-ergodicity in the sense of the disparity between ensemble-averaged MSD and time-averaged MSD.}, language = {en} } @article{KomarovPikovskij2014, author = {Komarov, Maxim and Pikovskij, Arkadij}, title = {The Kuramoto model of coupled oscillators with a bi-harmonic coupling function}, series = {Physica : D, Nonlinear phenomena}, volume = {289}, journal = {Physica : D, Nonlinear phenomena}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0167-2789}, doi = {10.1016/j.physd.2014.09.002}, pages = {18 -- 31}, year = {2014}, abstract = {We study synchronization in a Kuramoto model of globally coupled phase oscillators with a bi-harmonic coupling function, in the thermodynamic limit of large populations. We develop a method for an analytic solution of self-consistent equations describing uniformly rotating complex order parameters, both for single-branch (one possible state of locked oscillators) and multi-branch (two possible values of locked phases) entrainment. We show that synchronous states coexist with the neutrally linearly stable asynchronous regime. The latter has a finite life time for finite ensembles, this time grows with the ensemble size as a power law. (C) 2014 Elsevier B.V. All rights reserved.}, language = {en} } @article{FangGuerreroMarquezLugoetal.2014, author = {Fang, X. and Guerrero, Mart{\´i}n A. and Marquez-Lugo, R. A. and Toala, Jes{\´u}s Alberto and Arthur, S. J. and Chu, Y.-H. and Blair, William P. and Gruendl, R. A. and Hamann, Wolf-Rainer and Oskinova, Lidia M. and Todt, Helge Tobias}, title = {Expansion of hydrogen-poor knots in the born-again planetary nebulae A30 and A78}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {797}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/797/2/100}, pages = {11}, year = {2014}, abstract = {We analyze the expansion of hydrogen-poor knots and filaments in the born-again planetary nebulae A30 and A78 based on Hubble Space Telescope ( HST) images obtained almost 20 yr apart. The proper motion of these features generally increases with distance to the central star, but the fractional expansion decreases, i.e., the expansion is not homologous. As a result, there is not a unique expansion age, which is estimated to be 610-950 yr for A30 and 600-1140 yr for A78. The knots and filaments have experienced complex dynamical processes: the current fast stellar wind is mass loaded by the material ablated from the inner knots; the ablated material is then swept up until it shocks the inner edges of the outer, hydrogen-rich nebula. The angular expansion of the outer filaments shows a clear dependence on position angle, indicating that the interaction of the stellar wind with the innermost knots channels the wind along preferred directions. The apparent angular expansion of the innermost knots seems to be dominated by the rocket effect of evaporating gas and by the propagation of the ionization front inside them. Radiation-hydrodynamical simulations show that a single ejection of material followed by a rapid onset of the stellar wind and ionizing flux can reproduce the variety of clumps and filaments at different distances from the central star found in A30 and A78.}, language = {en} } @article{AliuArchambaultArlenetal.2014, author = {Aliu, E. and Archambault, S. and Arlen, T. and Aune, T. and Barnacka, Anna and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Cerruti, M. and Chen, X. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dumm, J. and Eisch, J. D. and Falcone, A. and Federici, S. and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hakansson, N. and Hanna, D. and Holder, J. and Hughes, G. and Hughes, Z. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kar, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Majumdar, P. and McArthur, S. and McCann, A. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nelson, T. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, M. and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sadun, A. and Santander, M. and Sembroski, G. H. and Shahinyan, K. and Sheidaei, F. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Theiling, M. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B. and Boettcher, Markus and Fumagalli, M.}, title = {Investigating broadband variability of the TeV blazar 1ES 1959+650}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {797}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {Veritas Collaboration}, issn = {0004-637X}, doi = {10.1088/0004-637X/797/2/89}, pages = {11}, year = {2014}, abstract = {We summarize broadband observations of the TeV-emitting blazar 1ES 1959+650, including optical R-band observations by the robotic telescopes Super-LOTIS and iTelescope, UV observations by Swift Ultraviolet and Optical Telescope, X-ray observations by the Swift X-ray Telescope, high-energy gamma-ray observations with the Fermi Large Area Telescope, and very-high-energy (VHE) gamma-ray observations by VERITAS above 315 GeV, all taken between 2012 April 17 and 2012 June 1 (MJD 56034 and 56079). The contemporaneous variability of the broadband spectral energy distribution is explored in the context of a simple synchrotron self Compton (SSC) model. In the SSC emission scenario, we find that the parameters required to represent the high state are significantly different than those in the low state. Motivated by possible evidence of gas in the vicinity of the blazar, we also investigate a reflected emission model to describe the observed variability pattern. This model assumes that the non-thermal emission from the jet is reflected by a nearby cloud of gas, allowing the reflected emission to re-enter the blob and produce an elevated gamma-ray state with no simultaneous elevated synchrotron flux. The model applied here, although not required to explain the observed variability pattern, represents one possible scenario which can describe the observations. As applied to an elevated VHE state of 66\% of the Crab Nebula flux, observed on a single night during the observation period, the reflected emission scenario does not support a purely leptonic non-thermal emission mechanism. The reflected emission model does, however, predict a reflected photon field with sufficient energy to enable elevated gamma-ray emission via pion production with protons of energies between 10 and 100 TeV.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Goudelis, A. and Grondin, M. -H. and Grudzinska, M. and Hadsch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, Olaf and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, Fabian and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Serpico, P. and Sol, H. and Spanier, F. and Spengler, G. and Spiess, F. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Search for dark matter annihilation signatures in HESS observations of dwarf spheroidal galaxies}, series = {Physical review : D, Particles, fields, gravitation, and cosmology}, volume = {90}, journal = {Physical review : D, Particles, fields, gravitation, and cosmology}, number = {11}, publisher = {American Physical Society}, address = {College Park}, organization = {HESS Collaboration}, issn = {1550-7998}, doi = {10.1103/PhysRevD.90.112012}, pages = {15}, year = {2014}, abstract = {Dwarf spheroidal galaxies of the Local Group are close satellites of the Milky Way characterized by a large mass-to-light ratio and are not expected to be the site of nonthermal high-energy gamma-ray emission or intense star formation. Therefore they are among the most promising candidates for indirect dark matter searches. During the last years the High Energy Stereoscopic System (H.E.S.S.) of imaging atmospheric Cherenkov telescopes observed five of these dwarf galaxies for more than 140 hours in total, searching for TeV gamma-ray emission from annihilation of dark matter particles. The new results of the deep exposure of the Sagittarius dwarf spheroidal galaxy, the first observations of the Coma Berenices and Fornax dwarves and the reanalysis of two more dwarf spheroidal galaxies already published by the H.E.S.S. Collaboration, Carina and Sculptor, are presented. In the absence of a significant signal new constraints on the annihilation cross section applicable to weakly interacting massive particles (WIMPs) are derived by combining the observations of the five dwarf galaxies. The combined exclusion limit depends on the WIMP mass and the best constraint is reached at 1-2 TeV masses with a cross-section upper bound of similar to 3.9 x 10(-24) cm(3) s(-1) at a 95\% confidence level.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadasch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, Marek and Janiak, M. and Jankowsky, F. and Jung-Richardt, I. and Kastendieck, M. A. and Katarzynski, Krzysztof and Katz, Uli and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, Michael and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, Olaf and Renaud, M. and de los Reyes, R. and Rieger, F. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, Fabian and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, Christopher and van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S. and Fukui, Y.}, title = {Diffuse Galactic gamma-ray emission with HESS}, series = {Physical review : D, Particles, fields, gravitation, and cosmology}, volume = {90}, journal = {Physical review : D, Particles, fields, gravitation, and cosmology}, number = {12}, publisher = {American Physical Society}, address = {College Park}, organization = {HESS Collaboration}, issn = {1550-7998}, doi = {10.1103/PhysRevD.90.122007}, pages = {8}, year = {2014}, abstract = {Diffuse gamma-ray emission is the most prominent observable signature of celestial cosmic-ray interactions at high energies. While already being investigated at GeVenergies over several decades, assessments of diffuse gamma-ray emission at TeVenergies remain sparse. After completion of the systematic survey of the inner Galaxy, the H.E.S.S. experiment is in a prime position to observe large-scale diffuse emission at TeVenergies. Data of the H.E.S.S. Galactic Plane Survey are investigated in regions off known gamma-ray sources. Corresponding gamma-ray flux measurements were made over an extensive grid of celestial locations. Longitudinal and latitudinal profiles of the observed gamma-ray fluxes show characteristic excess emission not attributable to known gamma-ray sources. For the first time large-scale gamma-ray emission along the Galactic plane using imaging atmospheric Cherenkov telescopes has been observed. While the background subtraction technique limits the ability to recover modest variation on the scale of the H.E.S.S. field of view or larger, which is characteristic of the inverse Compton scatter-induced Galactic diffuse emission, contributions of neutral pion decay as well as emission from unresolved gamma-ray sources can be recovered in the observed signal to a large fraction. Calculations show that the minimum gamma-ray emission from pi(0) decay represents a significant contribution to the total signal. This detection is interpreted as a mix of diffuse Galactic gamma-ray emission and unresolved sources.}, language = {en} } @book{Pohl2014, author = {Pohl, Martin}, title = {Physik f{\"u}r alle}, series = {Verdammt clever}, journal = {Verdammt clever}, publisher = {Wiley}, address = {Hoboken}, isbn = {978-3-527-41235-8}, pages = {268 S.}, year = {2014}, language = {de} } @article{DiFlorioBruendermannYadavalletal.2014, author = {DiFlorio, Giuseppe and Br{\"u}ndermann, Erik and Yadavall, Nataraja Sekhar and Santer, Svetlana and Havenith, Martina}, title = {Polarized 3D Raman and nanoscale near-field optical microscopy of optically inscribed surface relief gratings: chromophore orientation in azo-doped polymer films}, issn = {1744-683x}, doi = {10.1039/c3sm51787j}, year = {2014}, abstract = {We have used polarized confocal Raman microspectroscopy and scanning near-field optical microscopy with a resolution of 60 nm to characterize photoinscribed grating structures of azobenzene doped polymer films on a glass support. Polarized Raman microscopy allowed determining the reorientation of the chromophores as a function of the grating phase and penetration depth of the inscribing laser in three dimensions. We found periodic patterns, which are not restricted to the surface alone, but appear also well below the surface in the bulk of the material. Near-field optical microscopy with nanoscale resolution revealed lateral two-dimensional optical contrast, which is not observable by atomic force and Raman microscopy.}, language = {en} } @misc{deCarvalhoMetzlerCherstvy2014, author = {de Carvalho, Sidney J. and Metzler, Ralf and Cherstvy, Andrey G.}, title = {Critical adsorption of polyelectrolytes onto charged Janus nanospheres}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-98783}, pages = {12}, year = {2014}, abstract = {Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two equally but oppositely charged hemispheres. The critical binding conditions for polyelectrolyte chains are analysed as function of the radius of the Janus particle and its surface charge density, as well as the salt concentration in the ambient solution. Specifically for the adsorption of finite-length polyelectrolyte chains onto Janus nanoparticles, we demonstrate that the critical adsorption conditions drastically differ when the size of the Janus particle or the screening length of the electrolyte are varied. We compare the scaling laws obtained for the adsorption-desorption threshold to the known results for uniformly charged spherical particles, observing significant disparities. We also contrast the changes to the polyelectrolyte chain conformations close to the surface of the Janus nanoparticles as compared to those for simple spherical particles. Finally, we discuss experimentally relevant physico-chemical systems for which our simulations results may become important. In particular, we observe similar trends with polyelectrolyte complexation with oppositely but heterogeneously charged proteins.}, language = {en} } @misc{LiuTkachovKomberetal.2014, author = {Liu, W. and Tkachov, R. and Komber, H. and Senkovskyy, V. and Schubert, M. and Wei, Z. and Facchetti, A. and Neher, Dieter and Kiriy, A.}, title = {Chain-growth polycondensation of perylene diimide-based copolymers}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-98724}, pages = {8}, year = {2014}, abstract = {Herein, we report the chain-growth tin-free room temperature polymerization method to synthesize n-type perylene diimide-dithiophene-based conjugated polymers (PPDIT2s) suitable for solar cell and transistor applications. The palladium/electron-rich tri-tert-butylphosphine catalyst is effective to enable the chain-growth polymerization of anion-radical monomer Br-TPDIT-Br/Zn to PPDIT2 with a molecular weight up to Mw ≈ 50 kg mol-1 and moderate polydispersity. This is the second example of the polymerization of unusual anion-radical aromatic complexes formed in a reaction of active Zn and electron-deficient diimide-based aryl halides. As such, the discovered polymerization method is not a specific reactivity feature of the naphthalene-diimide derivatives but is rather a general polymerization tool. This is an important finding, given the significantly higher maximum external quantum efficiency that can be reached with PDI-based copolymers (32-45\%) in all-polymer solar cells compared to NDI-based materials (15-30\%). Our studies revealed that PPDIT2 synthesized by the new method and the previously published polymer prepared by step-growth Stille polycondensation show similar electron mobility and all-polymer solar cell performance. At the same time, the polymerization reported herein has several technological advantages as it proceeds relatively fast at room temperature and does not involve toxic tin-based compounds. Because several chain-growth polymerization reactions are well-suited for the preparation of well-defined multi-functional polymer architectures, the next target is to explore the utility of the discovered polymerization in the synthesis of end-functionalized polymers and block copolymers. Such materials would be helpful to improve the nanoscale morphology of polymer blends in all-polymer solar cells.}, language = {en} } @phdthesis{Brem2014, author = {Brem, Patrick}, title = {Compact objects in dense astrophysical environments}, school = {Universit{\"a}t Potsdam}, pages = {173}, year = {2014}, language = {en} } @phdthesis{Zhou2014, author = {Zhou, Xu}, title = {Atmospheric interactions with land surface in the arctic based on regional climate model solutions}, pages = {143}, year = {2014}, language = {en} } @phdthesis{Goswami2014, author = {Goswami, Bedartha}, title = {Uncertainties in climate data analysis}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-78312}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {Scientific inquiry requires that we formulate not only what we know, but also what we do not know and by how much. In climate data analysis, this involves an accurate specification of measured quantities and a consequent analysis that consciously propagates the measurement errors at each step. The dissertation presents a thorough analytical method to quantify errors of measurement inherent in paleoclimate data. An additional focus are the uncertainties in assessing the coupling between different factors that influence the global mean temperature (GMT). Paleoclimate studies critically rely on `proxy variables' that record climatic signals in natural archives. However, such proxy records inherently involve uncertainties in determining the age of the signal. We present a generic Bayesian approach to analytically determine the proxy record along with its associated uncertainty, resulting in a time-ordered sequence of correlated probability distributions rather than a precise time series. We further develop a recurrence based method to detect dynamical events from the proxy probability distributions. The methods are validated with synthetic examples and demonstrated with real-world proxy records. The proxy estimation step reveals the interrelations between proxy variability and uncertainty. The recurrence analysis of the East Asian Summer Monsoon during the last 9000 years confirms the well-known `dry' events at 8200 and 4400 BP, plus an additional significantly dry event at 6900 BP. We also analyze the network of dependencies surrounding GMT. We find an intricate, directed network with multiple links between the different factors at multiple time delays. We further uncover a significant feedback from the GMT to the El Ni{\~n}o Southern Oscillation at quasi-biennial timescales. The analysis highlights the need of a more nuanced formulation of influences between different climatic factors, as well as the limitations in trying to estimate such dependencies.}, language = {en} } @phdthesis{Conrad2014, author = {Conrad, Claudia}, title = {Open cluster groups and complexes}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-77605}, school = {Universit{\"a}t Potsdam}, pages = {xii, 172}, year = {2014}, abstract = {It is generally agreed upon that stars typically form in open clusters and stellar associations, but little is known about the structure of the open cluster system. Do open clusters and stellar associations form isolated or do they prefer to form in groups and complexes? Open cluster groups and complexes could verify star forming regions to be larger than expected, which would explain the chemical homogeneity over large areas in the Galactic disk. They would also define an additional level in the hierarchy of star formation and could be used as tracers for the scales of fragmentation in giant molecular clouds? Furthermore, open cluster groups and complexes could affect Galactic dynamics and should be considered in investigations and simulations on the dynamical processes, such as radial migration, disc heating, differential rotation, kinematic resonances, and spiral structure. In the past decade there were a few studies on open cluster pairs (de La Fuente Marcos \& de La Fuente Marcos 2009a,b,c) and on open cluster groups and complexes (Piskunov et al. 2006). The former only considered spatial proximity for the identification of the pairs, while the latter also required tangential velocities to be similar for the members. In this work I used the full set of 6D phase-space information to draw a more detailed picture on these structures. For this purpose I utilised the most homogeneous cluster catalogue available, namely the Catalogue of Open Cluster Data (COCD; Kharchenko et al. 2005a,b), which contains parameters for 650 open clusters and compact associations, as well as for their uniformly selected members. Additional radial velocity (RV) and metallicity ([M/H]) information on the members were obtained from the RAdial Velocity Experiment (RAVE; Steinmetz et al. 2006; Kordopatis et al. 2013) for 110 and 81 clusters, respectively. The RAVE sample was cleaned considering quality parameters and flags provided by RAVE (Matijevič et al. 2012; Kordopatis et al. 2013). To ensure that only real members were included for the mean values, also the cluster membership, as provided by Kharchenko et al. (2005a,b), was considered for the stars cross-matched in RAVE. 6D phase-space information could be derived for 432 out of the 650 COCD objects and I used an adaption of the Friends-of-Friends algorithm, as used in cosmology, to identify potential groupings. The vast majority of the 19 identified groupings were pairs, but I also found four groups of 4-5 members and one complex with 15 members. For the verification of the identified structures, I compared the results to a randomly selected subsample of the catalogue for the Milky Way global survey of Star Clusters (MWSC; Kharchenko et al. 2013), which became available recently, and was used as reference sample. Furthermore, I implemented Monte-Carlo simulations with randomised samples created from two distinguished input distributions for the spatial and velocity parameters. On the one hand, assuming a uniform distribution in the Galactic disc and, on the other hand, assuming the COCD data distributions to be representative for the whole open cluster population. The results suggested that the majority of identified pairs are rather by chance alignments, but the groups and the complex seemed to be genuine. A comparison of my results to the pairs, groups and complexes proposed in the literature yielded a partial overlap, which was most likely because of selection effects and different parameters considered. This is another verification for the existence of such structures. The characteristics of the found groupings favour that members of an open cluster grouping originate from a common giant molecular cloud and formed in a single, but possibly sequential, star formation event. Moreover, the fact that the young open cluster population showed smaller spatial separations between nearest neighbours than the old cluster population indicated that the lifetime of open cluster groupings is most likely comparable to that of the Galactic open cluster population itself. Still even among the old open clusters I could identify groupings, which suggested that the detected structure could be in some cases more long lived as one might think. In this thesis I could only present a pilot study on structures in the Galactic open cluster population, since the data sample used was highly incomplete. For further investigations a far more complete sample would be required. One step in this direction would be to use data from large current surveys, like SDSS, RAVE, Gaia-ESO and VVV, as well as including results from studies on individual clusters. Later the sample can be completed by data from upcoming missions, like Gaia and 4MOST. Future studies using this more complete open cluster sample will reveal the effect of open cluster groupings on star formation theory and their significance for the kinematics, dynamics and evolution of the Milky Way, and thereby of spiral galaxies.}, language = {en} } @phdthesis{Lange2014, author = {Lange, Ilja}, title = {Energetische Struktur von Schichten organischer Halbleiter und ihr fundamentaler Einfluss auf die physikalischen Eigenschaften organischer elektronischer Bauteile}, school = {Universit{\"a}t Potsdam}, pages = {105}, year = {2014}, language = {de} } @phdthesis{Hutter2014, author = {Hutter, Anne}, title = {Unveiling the epoch of reionization by simulations and high-redshift galaxies}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76998}, school = {Universit{\"a}t Potsdam}, pages = {vi, 155}, year = {2014}, abstract = {The Epoch of Reionization marks after recombination the second major change in the ionization state of the universe, going from a neutral to an ionized state. It starts with the appearance of the first stars and galaxies; a fraction of high-energy photons emitted from galaxies permeate into the intergalactic medium (IGM) and gradually ionize the hydrogen, until the IGM is completely ionized at z~6 (Fan et al., 2006). While the progress of reionization is driven by galaxy evolution, it changes the ionization and thermal state of the IGM substantially and affects subsequent structure and galaxy formation by various feedback mechanisms. Understanding this interaction between reionization and galaxy formation is further impeded by a lack of understanding of the high-redshift galactic properties such as the dust distribution and the escape fraction of ionizing photons. Lyman Alpha Emitters (LAEs) represent a sample of high-redshift galaxies that are sensitive to all these galactic properties and the effects of reionization. In this thesis we aim to understand the progress of reionization by performing cosmological simulations, which allows us to investigate the limits of constraining reionization by high-redshift galaxies as LAEs, and examine how galactic properties and the ionization state of the IGM affect the visibility and observed quantities of LAEs and Lyman Break galaxies (LBGs). In the first part of this thesis we focus on performing radiative transfer calculations to simulate reionization. We have developed a mapping-sphere-scheme, which, starting from spherically averaged temperature and density fields, uses our 1D radiative transfer code and computes the effect of each source on the IGM temperature and ionization (HII, HeII, HeIII) profiles, which are subsequently mapped onto a grid. Furthermore we have updated the 3D Monte-Carlo radiative transfer pCRASH, enabling detailed reionization simulations which take individual source characteristics into account. In the second part of this thesis we perform a reionization simulation by post-processing a smoothed-particle hydrodynamical (SPH) simulation (GADGET-2) with 3D radiative transfer (pCRASH), where the ionizing sources are modelled according to the characteristics of the stellar populations in the hydrodynamical simulation. Following the ionization fractions of hydrogen (HI) and helium (HeII, HeIII), and temperature in our simulation, we find that reionization starts at z~11 and ends at z~6, and high density regions near sources are ionized earlier than low density regions far from sources. In the third part of this thesis we couple the cosmological SPH simulation and the radiative transfer simulations with a physically motivated, self-consistent model for LAEs, in order to understand the importance of the ionization state of the IGM, the escape fraction of ionizing photons from galaxies and dust in the interstellar medium (ISM) on the visibility of LAEs. Comparison of our models results with the LAE Lyman Alpha (Lya) and UV luminosity functions at z~6.6 reveals a three-dimensional degeneracy between the ionization state of the IGM, the ionizing photons escape fraction and the ISM dust distribution, which implies that LAEs act not only as tracers of reionization but also of the ionizing photon escape fraction and of the ISM dust distribution. This degeneracy does not even break down when we compare simulated with observed clustering of LAEs at z~6.6. However, our results show that reionization has the largest impact on the amplitude of the LAE angular correlation functions, and its imprints are clearly distinguishable from those of properties on galactic scales. These results show that reionization cannot be constrained tightly by exclusively using LAE observations. Further observational constraints, e.g. tomographies of the redshifted hydrogen 21cm line, are required. In addition we also use our LAE model to probe the question when a galaxy is visible as a LAE or a LBG. Within our model galaxies above a critical stellar mass can produce enough luminosity to be visible as a LBG and/or a LAE. By finding an increasing duty cycle of LBGs with Lya emission as the UV magnitude or stellar mass of the galaxy rises, our model reveals that the brightest (and most massive) LBGs most often show Lya emission. Predicting the Lya equivalent width (Lya EW) distribution and the fraction of LBGs showing Lya emission at z~6.6, we reproduce the observational trend of the Lya EWs with UV magnitude. However, the Lya EWs of the UV brightest LBGs exceed observations and can only be reconciled by accounting for an increased Lya attenuation of massive galaxies, which implies that the observed Lya brightest LAEs do not necessarily coincide with the UV brightest galaxies. We have analysed the dependencies of LAE observables on the properties of the galactic and intergalactic medium and the LAE-LBG connection, and this enhances our understanding of the nature of LAEs.}, language = {en} } @phdthesis{Schreck2014, author = {Schreck, Simon Frederik}, title = {Potential energy surfaces, femtosecond dynamics and nonlinear X-Ray-Matter interactions from resonant inelastic soft x-Ray scattering}, pages = {164}, year = {2014}, language = {en} } @misc{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, publisher = {The Royal Society of Chemistry}, address = {Cambridge}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76478}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, number = {16}, publisher = {the Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @misc{JeonChechkinMetzler2014, author = {Jeon, Jae-Hyung and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Scaled Brownian motion: a paradoxical process with a time dependent diffusivity for the description of anomalous diffusion}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76302}, pages = {15811 -- 15817}, year = {2014}, abstract = {Anomalous diffusion is frequently described by scaled Brownian motion (SBM){,} a Gaussian process with a power-law time dependent diffusion coefficient. Its mean squared displacement is ?x2(t)? [similar{,} equals] 2K(t)t with K(t) [similar{,} equals] t[small alpha]-1 for 0 < [small alpha] < 2. SBM may provide a seemingly adequate description in the case of unbounded diffusion{,} for which its probability density function coincides with that of fractional Brownian motion. Here we show that free SBM is weakly non-ergodic but does not exhibit a significant amplitude scatter of the time averaged mean squared displacement. More severely{,} we demonstrate that under confinement{,} the dynamics encoded by SBM is fundamentally different from both fractional Brownian motion and continuous time random walks. SBM is highly non-stationary and cannot provide a physical description for particles in a thermalised stationary system. Our findings have direct impact on the modelling of single particle tracking experiments{,} in particular{,} under confinement inside cellular compartments or when optical tweezers tracking methods are used.}, language = {en} } @article{JeonChechkinMetzler2014, author = {Jeon, Jae-Hyung and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Scaled Brownian motion: a paradoxical process with a time dependent diffusivity for the description of anomalous diffusion}, series = {Physical chemistry, chemical physics : PCCP}, volume = {30}, journal = {Physical chemistry, chemical physics : PCCP}, number = {16}, publisher = {The Royal Society of Chemistry}, address = {Cambridge}, doi = {10.1039/C4CP02019G}, pages = {15811 -- 15817}, year = {2014}, abstract = {Anomalous diffusion is frequently described by scaled Brownian motion (SBM){,} a Gaussian process with a power-law time dependent diffusion coefficient. Its mean squared displacement is ?x2(t)? [similar{,} equals] 2K(t)t with K(t) [similar{,} equals] t[small alpha]-1 for 0 < [small alpha] < 2. SBM may provide a seemingly adequate description in the case of unbounded diffusion{,} for which its probability density function coincides with that of fractional Brownian motion. Here we show that free SBM is weakly non-ergodic but does not exhibit a significant amplitude scatter of the time averaged mean squared displacement. More severely{,} we demonstrate that under confinement{,} the dynamics encoded by SBM is fundamentally different from both fractional Brownian motion and continuous time random walks. SBM is highly non-stationary and cannot provide a physical description for particles in a thermalised stationary system. Our findings have direct impact on the modelling of single particle tracking experiments{,} in particular{,} under confinement inside cellular compartments or when optical tweezers tracking methods are used.}, language = {en} } @misc{PalyulinAlaNissilaMetzler2014, author = {Palyulin, Vladimir V. and Ala-Nissila, Tapio and Metzler, Ralf}, title = {Polymer translocation: the first two decades and the recent diversification}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76287}, pages = {9016 -- 9037}, year = {2014}, abstract = {Probably no other field of statistical physics at the borderline of soft matter and biological physics has caused such a flurry of papers as polymer translocation since the 1994 landmark paper by Bezrukov, Vodyanoy, and Parsegian and the study of Kasianowicz in 1996. Experiments, simulations, and theoretical approaches are still contributing novel insights to date, while no universal consensus on the statistical understanding of polymer translocation has been reached. We here collect the published results, in particular, the famous-infamous debate on the scaling exponents governing the translocation process. We put these results into perspective and discuss where the field is going. In particular, we argue that the phenomenon of polymer translocation is non-universal and highly sensitive to the exact specifications of the models and experiments used towards its analysis.}, language = {en} } @article{PalyulinAlaNissilaMetzler2014, author = {Palyulin, Vladimir V. and Ala-Nissila, Tapio and Metzler, Ralf}, title = {Polymer translocation: the first two decades and the recent diversification}, series = {Soft matter}, volume = {45}, journal = {Soft matter}, number = {10}, editor = {Metzler, Ralf}, publisher = {the Royal Society of Chemistry}, address = {Cambridge}, issn = {1744-683X}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76266}, pages = {9016 -- 9037}, year = {2014}, abstract = {Probably no other field of statistical physics at the borderline of soft matter and biological physics has caused such a flurry of papers as polymer translocation since the 1994 landmark paper by Bezrukov, Vodyanoy, and Parsegian and the study of Kasianowicz in 1996. Experiments, simulations, and theoretical approaches are still contributing novel insights to date, while no universal consensus on the statistical understanding of polymer translocation has been reached. We here collect the published results, in particular, the famous-infamous debate on the scaling exponents governing the translocation process. We put these results into perspective and discuss where the field is going. In particular, we argue that the phenomenon of polymer translocation is non-universal and highly sensitive to the exact specifications of the models and experiments used towards its analysis.}, language = {en} } @misc{BauerGodecMetzler2014, author = {Bauer, Maximilian and Godec, Aljaž and Metzler, Ralf}, title = {Diffusion of finite-size particles in two-dimensional channels with random wall configurations}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76199}, year = {2014}, abstract = {Diffusion of chemicals or tracer molecules through complex systems containing irregularly shaped channels is important in many applications. Most theoretical studies based on the famed Fick-Jacobs equation focus on the idealised case of infinitely small particles and reflecting boundaries. In this study we use numerical simulations to consider the transport of finite-size particles through asymmetrical two-dimensional channels. Additionally, we examine transient binding of the molecules to the channel walls by applying sticky boundary conditions. We consider an ensemble of particles diffusing in independent channels, which are characterised by common structural parameters. We compare our results for the long-time effective diffusion coefficient with a recent theoretical formula obtained by Dagdug and Pineda [J. Chem. Phys., 2012, 137, 024107].}, language = {en} }