@article{PollatosYeldesbayPikovskijetal.2014, author = {Pollatos, Olga and Yeldesbay, Azamat and Pikovskij, Arkadij and Rosenblum, Michael}, title = {How much time has passed? Ask your heart}, series = {Frontiers in neurorobotics}, volume = {8}, journal = {Frontiers in neurorobotics}, publisher = {Frontiers Research Foundation}, address = {Lausanne}, issn = {1662-5218}, doi = {10.3389/fnbot.2014.00015}, pages = {1 -- 9}, year = {2014}, abstract = {Internal signals like one's heartbeats are centrally processed via specific pathways and both their neural representations as well as their conscious perception (interoception) provide key information for many cognitive processes. Recent empirical findings propose that neural processes in the insular cortex, which are related to bodily signals, might constitute a neurophysiological mechanism for the encoding of duration. Nevertheless, the exact nature of such a proposed relationship remains unclear. We aimed to address this question by searching for the effects of cardiac rhythm on time perception by the use of a duration reproduction paradigm. Time intervals used were of 0.5, 2, 3, 7, 10, 14, 25, and 40s length. In a framework of synchronization hypothesis, measures of phase locking between the cardiac cycle and start/stop signals of the reproduction task were calculated to quantify this relationship. The main result is that marginally significant synchronization indices (Sls) between the heart cycle and the time reproduction responses for the time intervals of 2, 3, 10, 14, and 25s length were obtained, while results were not significant for durations of 0.5, 7, and 40s length. On the single participant level, several subjects exhibited some synchrony between the heart cycle and the time reproduction responses, most pronounced for the time interval of 25s (8 out of 23 participants for 20\% quantile). Better time reproduction accuracy was not related with larger degree of phase locking, but with greater vagal control of the heart. A higher interoceptive sensitivity (IS) was associated with a higher synchronization index (SI) for the 2s time interval only. We conclude that information obtained from the cardiac cycle is relevant for the encoding and reproduction of time in the time span of 2-25s. Sympathovagal tone as well as interoceptive processes mediate the accuracy of time estimation.}, language = {en} } @article{MengelLevermann2014, author = {Mengel, Matthias and Levermann, Anders}, title = {Ice plug prevents irreversible discharge from East Antarctica}, series = {Nature climate change}, volume = {4}, journal = {Nature climate change}, number = {6}, publisher = {Nature Publ. Group}, address = {London}, issn = {1758-678X}, doi = {10.1038/NCLIMATE2226}, pages = {451 -- 455}, year = {2014}, abstract = {Changes in ice discharge from Antarctica constitute the largest uncertainty in future sea-level projections, mainly because of the unknown response of its marine basins(1). Most of West Antarctica's marine ice sheet lies on an inland-sloping bed(2) and is thereby prone to a marine ice sheet instability(3-5). A similar topographic configuration is found in large parts of East Antarctica, which holds marine ice equivalent to 19 m of global sea-level rise(6), that is, more than five times that of West Antarctica. Within East Antarctica, the Wilkes Basin holds the largest volume of marine ice that is fully connected by subglacial troughs. This ice body was significantly reduced during the Pliocene epoch(7). Strong melting underneath adjacent ice shelves with similar bathymetry(8) indicates the ice sheet's sensitivity to climatic perturbations. The stability of the Wilkes marine ice sheet has not been the subject of any comprehensive assessment of future sea level. Using recently improved topographic data(6) in combination with ice-dynamic simulations, we show here that the removal of a specific coastal ice volume equivalent to less than 80 mm of global sea-level rise at the margin of the Wilkes Basin destabilizes the regional ice flow and leads to a self-sustained discharge of the entire basin and a global sea-level rise of 3-4 m. Our results are robust with respect to variation in ice parameters, forcing details and model resolution as well as increased surface mass balance, indicating that East Antarctica may become a large contributor to future sea-level rise on timescales beyond a century.}, language = {en} } @article{ShalomGuttentagFettkenhaueretal.2014, author = {Shalom, Menny and Guttentag, Miguel and Fettkenhauer, Christian and Inal, Sahika and Neher, Dieter and Llobet, Antoni and Antonietti, Markus}, title = {In situ formation of heterojunctions in modified graphitic carbon nitride: synthesis and noble metal free photocatalysis}, series = {Chemistry of materials : a publication of the American Chemical Society}, volume = {26}, journal = {Chemistry of materials : a publication of the American Chemical Society}, number = {19}, publisher = {American Chemical Society}, address = {Washington}, issn = {0897-4756}, doi = {10.1021/cm503258z}, pages = {5812 -- 5818}, year = {2014}, abstract = {Herein, we report the facile synthesis of an efficient roll-like carbon nitride (C3N4) photocatalyst for hydrogen production using a supramolecular complex composed of cyanuric acid, melamine, and barbituric acid as the starting monomers. Optical and photocatalytic investigations show, along with the known red shift of absorption into the visible region, that the insertion of barbituric acid results in the in situ formation of in-plane heterojuctions, which enhance the charge separation process under illumination. Moreover, platinum as the standard cocatalyst in photocatalysis could be successfully replaced with first row transition metal salts and complexes under retention of 50\% of the catalytic activity. Their mode of deposition and interaction with the semiconductor was studied in detail. Utilization of the supramolecular approach opens new opportunities to manipulate the charge transfer process within carbon nitride with respect to the design of a more efficient carbon nitride photocatalyst with controlled morphology and optical properties.}, language = {en} } @article{SaleemThungaKolloscheetal.2014, author = {Saleem, H. and Thunga, M. and Kollosche, Matthias and Kessler, M. R. and Laflamme, S.}, title = {Interfacial treatment effects on behavior of soft nano-composites for highly stretchable dielectrics}, series = {Polymer : the international journal for the science and technology of polymers}, volume = {55}, journal = {Polymer : the international journal for the science and technology of polymers}, number = {17}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-3861}, doi = {10.1016/j.polymer.2014.06.054}, pages = {4531 -- 4537}, year = {2014}, abstract = {We investigate the influence of interfacial treatment on the matrix filler interaction using a melt mixing process to fabricate robust and highly stretchable dielectrics. Silicone oil and silane coupling agent are studied as possible solutions to enhance the compatibility between the inorganic fillers and polymer matrix. Morphology, thermomechanical and dielectric behavior of the prepared specimens are studied. Results show that specimens filled with silicone oil coated particles have promising dielectric and thermal properties. The mechanical properties reveal a stiffness enhancement by 67\% with a high strain at break of 900\%. The relative permittivity of the specimens prepared with silicone oil increased by 45\% as observed from the dielectric analysis. (C) 2014 Elsevier Ltd. All rights reserved.}, language = {en} } @article{PradhanAlbrechtStilleretal.2014, author = {Pradhan, Basudev and Albrecht, Steve and Stiller, Burkhard and Neher, Dieter}, title = {Inverted organic solar cells comprising low-temperature-processed ZnO films}, series = {Applied physics : A, Materials science \& processing}, volume = {115}, journal = {Applied physics : A, Materials science \& processing}, number = {2}, publisher = {Springer}, address = {New York}, issn = {0947-8396}, doi = {10.1007/s00339-014-8373-8}, pages = {365 -- 369}, year = {2014}, abstract = {Inverted organic solar cells are fabricated using low-temperature-annealed ZnO film as an electron transport layer. Uniform ZnO films were prepared by spin coating a diethylzinc (DEZ) precursor solution in air, followed by annealing at 100 A degrees C. Organic solar cells prepared on these ZnO films with a 1:1 P3HT:PCBM blend as the active layer show a high power conversion efficiency of 4.03 \%, which is more than 10 \% higher than the PCE of solar cells comprising ZnO prepared via a high-temperature sol-gel route.}, language = {en} } @article{AliuArchambaultArlenetal.2014, author = {Aliu, E. and Archambault, S. and Arlen, T. and Aune, T. and Barnacka, Anna and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Cerruti, M. and Chen, X. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dumm, J. and Eisch, J. D. and Falcone, A. and Federici, S. and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hakansson, N. and Hanna, D. and Holder, J. and Hughes, G. and Hughes, Z. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kar, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Majumdar, P. and McArthur, S. and McCann, A. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nelson, T. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, M. and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sadun, A. and Santander, M. and Sembroski, G. H. and Shahinyan, K. and Sheidaei, F. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Theiling, M. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B. and Boettcher, Markus and Fumagalli, M.}, title = {Investigating broadband variability of the TeV blazar 1ES 1959+650}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {797}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {Veritas Collaboration}, issn = {0004-637X}, doi = {10.1088/0004-637X/797/2/89}, pages = {11}, year = {2014}, abstract = {We summarize broadband observations of the TeV-emitting blazar 1ES 1959+650, including optical R-band observations by the robotic telescopes Super-LOTIS and iTelescope, UV observations by Swift Ultraviolet and Optical Telescope, X-ray observations by the Swift X-ray Telescope, high-energy gamma-ray observations with the Fermi Large Area Telescope, and very-high-energy (VHE) gamma-ray observations by VERITAS above 315 GeV, all taken between 2012 April 17 and 2012 June 1 (MJD 56034 and 56079). The contemporaneous variability of the broadband spectral energy distribution is explored in the context of a simple synchrotron self Compton (SSC) model. In the SSC emission scenario, we find that the parameters required to represent the high state are significantly different than those in the low state. Motivated by possible evidence of gas in the vicinity of the blazar, we also investigate a reflected emission model to describe the observed variability pattern. This model assumes that the non-thermal emission from the jet is reflected by a nearby cloud of gas, allowing the reflected emission to re-enter the blob and produce an elevated gamma-ray state with no simultaneous elevated synchrotron flux. The model applied here, although not required to explain the observed variability pattern, represents one possible scenario which can describe the observations. As applied to an elevated VHE state of 66\% of the Crab Nebula flux, observed on a single night during the observation period, the reflected emission scenario does not support a purely leptonic non-thermal emission mechanism. The reflected emission model does, however, predict a reflected photon field with sufficient energy to enable elevated gamma-ray emission via pion production with protons of energies between 10 and 100 TeV.}, language = {en} } @article{AliuArchambaultAuneetal.2014, author = {Aliu, E. and Archambault, S. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Buckley, J. H. and Bugaev, V. and Cardenzana, J. V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dumm, J. and Dwarkadas, Vikram V. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gall, D. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krennrich, F. and Kumar, S. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McCann, A. J. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Pandel, D. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Ratliff, G. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Rousselle, J. and Sembroski, G. H. and Shahinyan, K. and Sheidaei, F. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Tsurusaki, K. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Ward, J. E. and Weinstein, A. and Welsing, R. and Wilhelm, Alina}, title = {Investigating the TeV morpholoy of MGRO J1908+06 with veritas}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {787}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/787/2/166}, pages = {7}, year = {2014}, abstract = {We report on deep observations of the extended TeV gamma-ray source MGRO J1908+06 made with the VERITAS very high energy gamma-ray observatory. Previously, the TeV emission has been attributed to the pulsar wind nebula (PWN) of the Fermi-LAT pulsar PSR J1907+0602. We detect MGRO J1908+06 at a significance level of 14 standard deviations (14 sigma) and measure a photon index of 2.20 +/- 0.10(stat) +/- 0.20(sys). The TeV emission is extended, covering the region near PSR J1907+0602 and also extending toward SNR G40.5-0.5. When fitted with a two-dimensional Gaussian, the intrinsic extension has a standard deviation of sigma(src) = 0 degrees.44 +/- 0 degrees.02. In contrast to other TeV PWNe of similar age in which the TeV spectrum softens with distance from the pulsar, the TeV spectrum measured near the pulsar location is consistent with that measured at a position near the rim of G40.5-0.5, 0 degrees.33 away.}, language = {en} } @phdthesis{Steyrleuthner2014, author = {Steyrleuthner, Robert}, title = {Korrelation von Struktur, optischen Eigenschaften und Ladungstransport in einem konjugierten Naphthalindiimid-Bithiophen Copolymer mit herausragender Elektronenmobilit{\"a}t}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-71413}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {Organische Halbleiter besitzen neue, bemerkenswerte Materialeigenschaften, die sie f{\"u}r die grundlegende Forschung wie auch aktuelle technologische Entwicklung (bsw. org. Leuchtdioden, org. Solarzellen) interessant werden lassen. Aufgrund der starken konformative Freiheit der konjugierten Polymerketten f{\"u}hrt die Vielzahl der m{\"o}glichen Anordnungen und die schwache intermolekulare Wechselwirkung f{\"u}r gew{\"o}hnlich zu geringer struktureller Ordnung im Festk{\"o}rper. Die Morphologie hat gleichzeitig direkten Einfluss auf die elektronische Struktur der organischen Halbleiter, welches sich meistens in einer deutlichen Reduktion der Ladungstr{\"a}gerbeweglichkeit gegen{\"u}ber den anorganischen Verwandten zeigt. So stellt die Beweglichkeit der Ladungen im Halbleiter einen der limitierenden Faktoren f{\"u}r die Leistungsf{\"a}higkeit bzw. den Wirkungsgrad von funktionellen organischen Bauteilen dar. Im Jahr 2009 wurde ein neues auf Naphthalindiimid und Bithiophen basierendes Dornor/Akzeptor Copolymer vorgestellt [P(NDI2OD‑T2)], welches sich durch seine außergew{\"o}hnlich hohe Ladungstr{\"a}germobilit{\"a}t auszeichnet. In dieser Arbeit wird die Ladungstr{\"a}germobilit{\"a}t in P(NDI2OD‑T2) bestimmt, und der Transport durch eine geringe energetischer Unordnung charakterisiert. Obwohl dieses Material zun{\"a}chst als amorph beschrieben wurde zeigt eine detaillierte Analyse der optischen Eigenschaften von P(NDI2OD‑T2), dass bereits in L{\"o}sung geordnete Vorstufen supramolekularer Strukturen (Aggregate) existieren. Quantenchemische Berechnungen belegen die beobachteten spektralen {\"A}nderungen. Mithilfe der NMR-Spektroskopie kann die Bildung der Aggregate unabh{\"a}ngig von optischer Spektroskopie best{\"a}tigt werden. Die Analytische Ultrazentrifugation an P(NDI2OD‑T2) L{\"o}sungen legt nahe, dass sich die Aggregation innerhalb der einzelnen Ketten unter Reduktion des hydrodynamischen Radius vollzieht. Die Ausbildung supramolekularen Strukturen nimmt auch eine signifikante Rolle bei der Filmbildung ein und verhindert gleichzeitig die Herstellung amorpher P(NDI2OD‑T2) Filme. Durch chemische Modifikation der P(NDI2OD‑T2)-Kette und verschiedener Prozessierungs-Methoden wurde eine {\"A}nderung des Kristallinit{\"a}tsgrades und gleichzeitig der Orientierung der kristallinen Dom{\"a}nen erreicht und mittels R{\"o}ntgenbeugung quantifiziert. In hochaufl{\"o}senden Elektronenmikroskopie-Messungen werden die Netzebenen und deren Einbettung in die semikristallinen Strukturen direkt abgebildet. Aus der Kombination der verschiedenen Methoden erschließt sich ein Gesamtbild der Nah- und Fernordnung in P(NDI2OD‑T2). {\"U}ber die Messung der Elektronenmobilit{\"a}t dieser Schichten wird die Anisotropie des Ladungstransports in den kristallographischen Raumrichtungen von P(NDI2OD‑T2) charakterisiert und die Bedeutung der intramolekularen Wechselwirkung f{\"u}r effizienten Ladungstransport herausgearbeitet. Gleichzeitig wird deutlich, wie die Verwendung von gr{\"o}ßeren und planaren funktionellen Gruppen zu h{\"o}heren Ladungstr{\"a}germobilit{\"a}ten f{\"u}hrt, welche im Vergleich zu klassischen semikristallinen Polymeren weniger sensitiv auf die strukturelle Unordnung im Film sind.}, language = {de} } @article{PalyulinChechkinMetzler2014, author = {Palyulin, Vladimir V. and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Levy flights do not always optimize random blind search for sparse targets}, series = {Proceedings of the National Academy of Sciences of the United States of America}, volume = {111}, journal = {Proceedings of the National Academy of Sciences of the United States of America}, number = {8}, publisher = {National Acad. of Sciences}, address = {Washington}, issn = {0027-8424}, doi = {10.1073/pnas.1320424111}, pages = {2931 -- 2936}, year = {2014}, abstract = {It is generally believed that random search processes based on scale-free, Levy stable jump length distributions (Levy flights) optimize the search for sparse targets. Here we show that this popular search advantage is less universal than commonly assumed. We study the efficiency of a minimalist search model based on Levy flights in the absence and presence of an external drift (underwater current, atmospheric wind, a preference of the walker owing to prior experience, or a general bias in an abstract search space) based on two different optimization criteria with respect to minimal search time and search reliability (cumulative arrival probability). Although Levy flights turn out to be efficient search processes when the target is far from the starting point, or when relative to the starting point the target is upstream, we show that for close targets and for downstream target positioning regular Brownian motion turns out to be the advantageous search strategy. Contrary to claims that Levy flights with a critical exponent alpha = 1 are optimal for the search of sparse targets in different settings, based on our optimization parameters the optimal a may range in the entire interval (1, 2) and especially include Brownian motion as the overall most efficient search strategy.}, language = {en} } @article{Goychuk2014, author = {Goychuk, Igor}, title = {Life and death of stationary linear response in anomalous continuous time random walk dynamics}, series = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, volume = {62}, journal = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, number = {4}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0253-6102}, pages = {497 -- 504}, year = {2014}, abstract = {Linear theory of stationary response in systems at thermal equilibrium requires to find equilibrium correlation function of unperturbed responding system. Studies of the response of the systems exhibiting anomalously slow dynamics are often based on the continuous time random walk description (CTRW) with divergent mean waiting times. The bulk of the literature on anomalous response contains linear response functions like one by Cole-Cole calculated from such a CTRW theory and applied to systems at thermal equilibrium. Here we show within a fairly simple and general model that for the systems with divergent mean waiting times the stationary response at thermal equilibrium is absent, in accordance with some recent studies. The absence of such stationary response (or dying to zero non-stationary response in aging experiments) would confirm CTRW with divergent mean waiting times as underlying physical relaxation mechanism, but reject it otherwise. We show that the absence of stationary response is closely related to the breaking of ergodicity of the corresponding dynamical variable. As an important new result, we derive a generalized Cole-Cole response within ergodic CTRW dynamics with finite waiting time. Moreover, we provide a physically reasonable explanation of the origin and wide presence of 1/f noise in condensed matter for ergodic dynamics close to normal, rather than strongly deviating.}, language = {en} } @article{XuBrennerChabanneetal.2014, author = {Xu, Jingsan and Brenner, Thomas J. K. and Chabanne, Laurent and Neher, Dieter and Antonietti, Markus and Shalom, Menny}, title = {Liquid-Based growth of polymeric carbon nitride layers and their use in a mesostructured polymer solar cell with V-oc exceeding 1 V}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {39}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja508329c}, pages = {13486 -- 13489}, year = {2014}, abstract = {Herein we report a general liquid-mediated pathway for the growth of continuous polymeric carbon nitride (C3N4) thin films. The deposition method consists of the use of supramolecular complexes that transform to the liquid state before direct thermal condensation into C3N4 solid films. The resulting films exhibit continuous porous C3N4 networks on various substrates. Moreover, the optical absorption can be easily tuned to cover the solar spectrum by the insertion of an additional molecule into the starting complex. The strength of the deposition method is demonstrated by the use of the C3N4 layer as the electron acceptor in a polymer solar cell that exhibits a remarkable open-circuit voltage exceeding 1 V. The easy, safe, and direct synthesis of carbon nitride in a continuous layered architecture on different functional substrates opens new possibilities for the fabrication of many energy-related devices.}, language = {en} } @article{GodecChechkinBarkaietal.2014, author = {Godec, Aljaz and Chechkin, Aleksei V. and Barkai, Eli and Kantz, Holger and Metzler, Ralf}, title = {Localisation and universal fluctuations in ultraslow diffusion processes}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {47}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {49}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8113/47/49/492002}, pages = {10}, year = {2014}, abstract = {We study ultraslow diffusion processes with logarithmic mean squared displacement (MSD) < x(2)(t)> similar or equal to log(gamma)t. Comparison of annealed (renewal) continuous time random walks (CTRWs) with logarithmic waiting time distribution psi(tau) similar or equal to 1/(tau log(1+gamma)tau) and Sinai diffusion in quenched random landscapes reveals striking similarities, despite the great differences in their physical nature. In particular, they exhibit a weakly non-ergodic disparity of the time-averaged and ensemble-averaged MSDs. Remarkably, for the CTRW we observe that the fluctuations of time averages become universal, with an exponential suppression of mobile trajectories. We discuss the fundamental connection between the Golosov localization effect and non-ergodicity in the sense of the disparity between ensemble-averaged MSD and time-averaged MSD.}, language = {en} } @article{SchickHerzogWenetal.2014, author = {Schick, Daniel and Herzog, Marc and Wen, Haidan and Chen, Pice and Adamo, Carolina and Gaal, Peter and Schlom, Darrell G. and Evans, Paul G. and Li, Yuelin and Bargheer, Matias}, title = {Localized excited charge carriers generate ultrafast inhomogeneous strain in the multiferroic BiFeO3}, series = {Physical review letters}, volume = {112}, journal = {Physical review letters}, number = {9}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.112.097602}, pages = {6}, year = {2014}, abstract = {We apply ultrafast x-ray diffraction with femtosecond temporal resolution to monitor the lattice dynamics in a thin film of multiferroic BiFeO3 after above-band-gap photoexcitation. The sound-velocity limited evolution of the observed lattice strains indicates a quasi-instantaneous photoinduced stress which decays on a nanosecond time scale. This stress exhibits an inhomogeneous spatial profile evidenced by the broadening of the Bragg peak. These new data require substantial modification of existing models of photogenerated stresses in BiFeO3: the relevant excited charge carriers must remain localized to be consistent with the data.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and B{\"o}ttcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Forster, A. and Fuling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadsch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, Markus and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kiefeer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Kruger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puhlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schussler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and Van Eldik, C. and Van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Volk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Wornlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Long-term monitoring of PKS2155-304 with ATOM and HESS:investigation of optical/gamma-ray correlations in different spectral states}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {571}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, organization = {HESSS Collaboration}, issn = {0004-6361}, doi = {10.1051/0004-6361/201424142}, pages = {10}, year = {2014}, abstract = {In this paper we report on the analysis of all the available optical and very high-energy gamma-ray (> 200 GeV) data for the BL Lac object PKS 2155-304, collected simultaneously with the ATOM and H.E.S.S. telescopes from 2007 until 2009. This study also includes X-ray (RXTE, Swift) and high-energy gamma-ray (Fermi-LAT) data. During the period analysed, the source was transitioning from its flaring to quiescent optical states, and was characterized by only moderate flux changes at different wavelengths on the timescales of days and months. A flattening of the optical continuum with an increasing optical flux can be noted in the collected dataset, but only occasionally and only at higher flux levels. We did not find any universal relation between the very high-energy gamma-ray and optical flux changes on the timescales from days and weeks up to several years. On the other hand, we noted that at higher flux levels the source can follow two distinct tracks in the optical flux-colour diagrams, which seem to be related to distinct gamma-ray states of the blazar. The obtained results therefore indicate a complex scaling between the optical and gamma-ray emission of PKS 2155 304, with different correlation patterns holding at different epochs, and a gamma-ray flux depending on the combination of an optical flux and colour rather than a flux alone.}, language = {en} } @article{AliuArchambaultAuneetal.2014, author = {Aliu, E. and Archambault, S. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Byrum, K. and Cerruti, M. and Chen, X. and Ciupik, L. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Errando, M. and Falcone, A. and Federici, S. and Feng, Q. and Finley, J. P. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Maier, G. and Majumdar, P. and McCann, A. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, M. and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Rousselle, J. and Sembroski, G. H. and Sheidaei, F. and Skole, C. and Smith, A. W. and Staszak, D. and Stroh, M. and Telezhinsky, Igor O. and Theiling, M. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vincent, S. and Wakely, S. P. and Weinstein, A. and Welsing, R. and Williams, D. A. and Zajczyk, A. and Zitzer, B. and Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Voelk, H. J. and Volpe, F. and Vorster, M. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Long-term TeV and X-RAY observations of the GAMMA- RAY binary hess J0632+057}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {780}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {VERITAS Collaboration, HESS Collaboration}, issn = {0004-637X}, doi = {10.1088/0004-637X/780/2/168}, pages = {14}, year = {2014}, language = {en} } @article{MarzeionLevermann2014, author = {Marzeion, Ben and Levermann, Anders}, title = {Loss of cultural world heritage and currently inhabited places to sea-level rise}, series = {Environmental research letters}, volume = {9}, journal = {Environmental research letters}, number = {3}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1748-9326}, doi = {10.1088/1748-9326/9/3/034001}, pages = {7}, year = {2014}, language = {en} } @article{ZhangZhangYouetal.2014, author = {Zhang, Xiaoqing and Zhang, Xinwu and You, Qiong and Sessler, Gerhard M.}, title = {Low- cost, large- area, stretchable piezoelectric films based on irradiation- crosslinked poly ( propylene)}, series = {Macromolecular materials and engineering}, volume = {299}, journal = {Macromolecular materials and engineering}, number = {3}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1438-7492}, doi = {10.1002/mame.201300161}, pages = {290 -- 295}, year = {2014}, abstract = {Low cost, large area, lightweight, stretchable piezoelectric films, based on space-charge electret with a foam structure (i.e., ferroelectrets or piezoelectrets), have been fabricated by using commercially available irradiation cross-linked poly(propylene) (IXPP) foam sheets. Piezoelectric d(33) coefficients are as high as 100pCN(-1). The piezoelectric performance in such IXPP films is well preserved for repeated strains of less than 10\%. Piezoelectric d(33) coefficients are frequency independent in the range from 2 to 100Hz. Such new class materials may be applied in sensory skins, smart clothing, bio-inspired systems, microenergy harvesters, and so on.}, language = {en} } @article{NishikawaHardeeDutanetal.2014, author = {Nishikawa, Ken-Ichi and Hardee, P. E. and Dutan, I. and Niemiec, J. and Medvedev, M. and Mizuno, Y. and Meli, A. and Sol, H. and Zhang, B. and Pohl, Martin and Hartmann, D. H.}, title = {Magnetic agnetic field generation in core-sheath jets via the kinetic Kelvin-Helmholtz instability}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {793}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/793/1/60}, pages = {16}, year = {2014}, abstract = {We have investigated magnetic field generation in velocity shears via the kinetic Kelvin-Helmholtz instability (kKHI) using a relativistic plasma jet core and stationary plasma sheath. Our three-dimensional particle-in-cell simulations consider plasma jet cores with Lorentz factors of 1.5, 5, and 15 for both electron-proton and electron-positron plasmas. For electron-proton plasmas, we find generation of strong large-scale DC currents and magnetic fields that extend over the entire shear surface and reach thicknesses of a few tens of electron skin depths. For electron-positron plasmas, we find generation of alternating currents and magnetic fields. Jet and sheath plasmas are accelerated across the shear surface in the strong magnetic fields generated by the kKHI. The mixing of jet and sheath plasmas generates a transverse structure similar to that produced by the Weibel instability.}, language = {en} } @article{ChenChatterjeeZhangetal.2014, author = {Chen, Xuhui and Chatterjee, Ritaban and Zhang, Haocheng and Pohl, Martin and Fossati, Giovanni and Boettcher, Markus and Bailyn, Charles D. and Bonning, Erin W. and Buxton, Michelle and Coppi, Paolo and Isler, Jedidah and Maraschi, Laura and Urry, Meg}, title = {Magnetic field amplification and flat spectrum radio quasars}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu713}, pages = {2188 -- 2199}, year = {2014}, abstract = {We perform time-dependent, spatially resolved simulations of blazar emission to evaluate several flaring scenarios related to magnetic-field amplification and enhanced particle acceleration. The code explicitly accounts for light-travel-time effects and is applied to flares observed in the flat spectrum radio quasar (FSRQ) PKS 0208-512, which show optical/gamma-ray correlation at some times, but orphan optical flares at other times. Changes in both the magnetic field and the particle acceleration efficiency are explored as causes of flares. Generally, external Compton (EC) emission appears to describe the available data better than a synchrotron self-Compton (SSC) scenario, and in particular orphan optical flares are difficult to produce in the SSC framework. X-ray soft-excesses, gamma-ray spectral hardening, and the detections at very high energies of certain FSRQs during flares find natural explanations in the EC scenario with particle acceleration change. Likewise, optical flares with/without gamma-ray counterparts can be explained by different allocations of energy between the magnetization and particle acceleration, which may be related to the orientation of the magnetic field relative to the jet flow. We also calculate the degree of linear polarization and polarization angle as a function of time for a jet with helical magnetic field. Tightening of the magnetic helix immediately downstream of the jet perturbations, where flares occur, can be sufficient to explain the increases in the degree of polarization and a rotation by a parts per thousand yen180A degrees of the observed polarization angle, if light-travel-time effects are properly considered.}, language = {en} } @article{MizunoPohlNiemiecetal.2014, author = {Mizuno, Yosuke and Pohl, Martin and Niemiec, Jacek and Zhang, Bing and Nishikawa, Ken-Ichi and Hardee, Philip E.}, title = {Magnetic field amplification and saturation in turbulence behind a relativistic shock}, series = {Monthly notices of the Royal Astronomical Society}, volume = {439}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu196}, pages = {3490 -- 3503}, year = {2014}, abstract = {We have investigated via 2D relativistic magnetohydrodynamic simulations the long-term evolution of turbulence created by a relativistic shock propagating through an inhomogeneous medium. In the post-shock region, magnetic field is strongly amplified by turbulent motions triggered by pre-shock density inhomogeneities. Using a long-simulation box we have followed the magnetic field amplification until it is fully developed and saturated. The turbulent velocity is subrelativistic even for a strong shock. Magnetic field amplification is controlled by the turbulent motion and saturation occurs when the magnetic energy is comparable to the turbulent kinetic energy. Magnetic field amplification and saturation depend on the initial strength and direction of the magnetic field in the pre-shock medium, and on the shock strength. If the initial magnetic field is perpendicular to the shock normal, the magnetic field is first compressed at the shock and then can be amplified by turbulent motion in the post-shock region. Saturation occurs when the magnetic energy becomes comparable to the turbulent kinetic energy in the post-shock region. If the initial magnetic field in the pre-shock medium is strong, the post-shock region becomes turbulent but significant field amplification does not occur. If the magnetic energy after shock compression is larger than the turbulent kinetic energy in the post-shock region, significant field amplification does not occur. We discuss possible applications of our results to gamma-ray bursts and active galactic nuclei.}, language = {en} } @article{Levermann2014, author = {Levermann, Anders}, title = {Make supply chains climate-smart}, series = {Nature : the international weekly journal of science}, volume = {506}, journal = {Nature : the international weekly journal of science}, number = {7486}, publisher = {Nature Publ. Group}, address = {London}, issn = {0028-0836}, pages = {27 -- 29}, year = {2014}, language = {en} } @article{ReibisVoellerGittetal.2014, author = {Reibis, Rona Katharina and V{\"o}ller, Heinz and Gitt, Anselm and Jannowitz, Christina and Halle, Martin and Pittrow, David and Hildemann, Steven}, title = {Management of patients with ST- segment elevation or non- ST- segment elevation acute coronary syndromes in cardiac rehabilitation centers}, series = {Clinical cardiology : international journal for cardiovascular diseases}, volume = {37}, journal = {Clinical cardiology : international journal for cardiovascular diseases}, number = {4}, publisher = {Wiley-Blackwell}, address = {Hoboken}, issn = {0160-9289}, doi = {10.1002/clc.22241}, pages = {213 -- 221}, year = {2014}, abstract = {BackgroundCurrent data on the management of patients in cardiac rehabilitation (CR) after an acute hospital stay due to ST-segment elevation or non-ST segment elevation acute coronary syndromes (STE-ACS or NSTE-ACS) are limited. We aimed to describe patient characteristics, risk factor management, and lipid target achievement of patients in CR in Germany and compare the 2 groups. HypothesisWith respect to the risk factor pattern and treatment effects during a CR stay, there are important differences between STE-ACS and NSTE-ACS patients. MethodsComparison of 7950 patients by STE-ACS or NSTE-ACS status in the Transparency Registry to Objectify Guideline-Oriented Risk Factor Management registry (2010) who underwent an inpatient CR period of about 3 weeks. ResultsSTE-ACS patients compared to NSTE-ACS patients were significantly younger (60.5 vs 64.4 years, P < 0.0001), and had diabetes mellitus, hypertension, or any risk factor (exception: smoking) less often. At discharge, in STE-ACS compared to NSTE-ACS patients, the low-density lipoprotein cholesterol (LDL-C) <100 mg/dL goal was achieved by 75.3\% and 76.2\%, respectively (LDL-C <70 mg/dL by 27.7\% and 27.4\%), the high-density lipoprotein cholesterol goal of >50 mg/dL in women and >40 mg/dL in men was achieved by 49.3\% and 49.0\%, respectively, and the triglycerides goal of <150 mg/dl was achievedby 72.3\% and 74.3\%, respectively (all comparisons not significant). Mean systolic and diastolic blood pressure were 121/74 and 123/74 mm Hg, respectively (P < 0.0001 systolic, diastolic not significant). The maximum exercise capacity was 110 and 102 W, respectively (P < 0.0001), and the maximum walking distance was 581 and 451 meters, respectively (P value not significant). ConclusionsPatients with STE-ACS and NSTE-ACS differed moderately in their baseline characteristics. Both groups benefited from the participation in CR, as their lipid profile, blood pressure, and physical fitness improved.}, language = {en} } @article{PapkeYadavalliHenkeletal.2014, author = {Papke, Thomas and Yadavalli, Nataraja Sekhar and Henkel, Carsten and Santer, Svetlana}, title = {Mapping a plasmonic hologram with photosensitive polymer films: standing versus propagating waves}, series = {ACS applied materials \& interfaces}, volume = {6}, journal = {ACS applied materials \& interfaces}, number = {16}, publisher = {American Chemical Society}, address = {Washington}, issn = {1944-8244}, doi = {10.1021/am503501y}, pages = {14174 -- 14180}, year = {2014}, abstract = {We use a photosensitive layer containing azobenzene moieties to map near-field intensity patterns in the vicinity of nanogrids fabricated within a thin silver layer. It is known that azobenzene containing films deform permanently during irradiation, following the pattern of the field intensity. The photosensitive material reacts only to stationary waves whose intensity patterns do not change in time. In this study, we have found a periodic deformation above the silver film outside the nanostructure, even if the latter consists of just one groove. This is in contradiction to the widely accepted viewpoint that propagating surface plasmon modes dominate outside nanogrids. We explain our observation based on an electromagnetic hologram formed by the constructive interference between a propagating surface plasmon wave and the incident light. This hologram contains a stationary intensity and polarization grating that even appears in the absence of the polymer layer.}, language = {en} } @article{EhlertLevermann2014, author = {Ehlert, D. and Levermann, Anders}, title = {Mechanism for potential strengthening of Atlantic overturning prior to collapse}, series = {Earth system dynamics}, volume = {5}, journal = {Earth system dynamics}, number = {2}, publisher = {Copernicus}, address = {G{\"o}ttingen}, issn = {2190-4979}, doi = {10.5194/esd-5-383-2014}, pages = {383 -- 397}, year = {2014}, abstract = {The Atlantic meridional overturning circulation (AMOC) carries large amounts of heat into the North Atlantic influencing climate regionally as well as globally. Palaeo-records and simulations with comprehensive climate models suggest that the positive salt-advection feedback may yield a threshold behaviour of the system. That is to say that beyond a certain amount of freshwater flux into the North Atlantic, no meridional overturning circulation can be sustained. Concepts of monitoring the AMOC and identifying its vicinity to the threshold rely on the fact that the volume flux defining the AMOC will be reduced when approaching the threshold. Here we advance conceptual models that have been used in a paradigmatic way to understand the AMOC, by introducing a density-dependent parameterization for the Southern Ocean eddies. This additional degree of freedom uncovers a mechanism by which the AMOC can increase with additional freshwater flux into the North Atlantic, before it reaches the threshold and collapses: an AMOC that is mainly wind-driven will have a constant upwelling as long as the Southern Ocean winds do not change significantly. The downward transport of tracers occurs either in the northern sinking regions or through Southern Ocean eddies. If freshwater is transported, either atmospherically or via horizontal gyres, from the low to high latitudes, this would reduce the eddy transport and by continuity increase the northern sinking which defines the AMOC until a threshold is reached at which the AMOC cannot be sustained. If dominant in the real ocean this mechanism would have significant consequences for monitoring the AMOC.}, language = {en} } @article{ShinCherstvyMetzler2014, author = {Shin, Jaeoh and Cherstvy, Andrey G. and Metzler, Ralf}, title = {Mixing and segregation of ring polymers: spatial confinement and molecular crowding effects}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/5/053047}, pages = {19}, year = {2014}, abstract = {During the life cycle of bacterial cells the non-mixing of the two ring-shaped daughter genomes is an important prerequisite for the cell division process. Mimicking the environments inside highly crowded biological cells, we study the dynamics and statistical behavior of two flexible ring polymers in the presence of cylindrical confinement and crowding molecules. From extensive computer simulations we determine the degree of ring-ring overlap and the number of inter-monomer contacts for varying volume fractions phi of crowders. We also examine the entropic demixing of polymer rings in the presence of mobile crowders and determine the characteristic times of the internal polymer dynamics. Effects of the ring length on ring-ring overlap are also analyzed. In particular, on systematic variation of the fraction of crowding molecules, a (1 - phi)-scaling is found for the ring-ring overlap length along the cylinder axis, and a non-monotonic dependence of the 3D ring-ring contact number with a maximum at phi approximate to 0.2 is obtained. Our results demonstrate that polymer rings are demixed and separated by particular entropy-favourable partitioning of crowders along the axis of the cylindrical simulation box. These findings help to rationalize the implications of macromolecular crowding for circular DNA molecules in confined spaces inside bacteria as well as in localized cellular compartments inside eukaryotic cells.}, language = {en} } @article{LiAbrechtYangetal.2014, author = {Li, Wentao and Abrecht, Steve and Yang, Liqiang and Roland, Steffen and Tumbleston, John R. and McAfee, Terry and Yan, Liang and Kelly, Mary Allison and Ade, Harald W. and Neher, Dieter and You, Wei}, title = {Mobility-controlled performance of thick solar cells based on fluorinated copolymers}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {44}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja5067724}, pages = {15566 -- 15576}, year = {2014}, abstract = {Developing novel materials and device architectures to further enhance the efficiency of polymer solar cells requires a fundamental understanding of the impact of chemical structures on photovoltaic properties. Given that device characteristics depend on many parameters, deriving structureproperty relationships has been very challenging. Here we report that a single parameter, hole mobility, determines the fill factor of several hundred nanometer thick bulk heterojunction photovoltaic devices based on a series of copolymers with varying amount of fluorine substitution. We attribute the steady increase of hole mobility with fluorine content to changes in polymer molecular ordering. Importantly, all other parameters, including the efficiency of free charge generation and the coefficient of nongeminate recombination, are nearly identical. Our work emphasizes the need to achieve high mobility in combination with strongly suppressed charge recombination for the thick devices required by mass production technologies.}, language = {en} } @article{CherstvyPetrov2014, author = {Cherstvy, Andrey G. and Petrov, Eugene P.}, title = {Modeling DNA condensation on freestanding cationic lipid membranes}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {5}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c3cp53433b}, pages = {2020 -- 2037}, year = {2014}, abstract = {Motivated by recent experimental observations of a rapid spontaneous DNA coil-globule transition on freestanding cationic lipid bilayers, we propose simple theoretical models for DNA condensation on cationic lipid membranes. First, for a single DNA rod, we examine the conditions of full wrapping of a cylindrical DNA-like semi-flexible polyelectrolyte by an oppositely charged membrane. Then, for two parallel DNA rods, we self-consistently analyze the shape and the extent of the membrane enveloping them, focusing on membrane elastic deformations and the membrane-DNA embracing angle, which enables us to compute the membrane-mediated DNA-DNA interactions. We examine the effects of the membrane composition and its charge density, which are the experimentally tunable parameters. We show that membrane-driven rod-rod attraction is more pronounced for higher charge densities and for smaller surface tensions of the membrane. Thus, we demonstrate that for a long DNA chain adhered to a cationic lipid membrane, such membrane-induced DNA-DNA attraction can trigger compaction of DNA.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {31}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c4cp01234h}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, number = {16}, publisher = {the Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @misc{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, publisher = {The Royal Society of Chemistry}, address = {Cambridge}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76478}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @article{KustererNagelHartmannetal.2014, author = {Kusterer, D. -J. and Nagel, T. and Hartmann, S. and Werner, K. and Feldmeier, Achim}, title = {Monte Carlo radiation transfer in CV disk winds: application to the AM CVn prototype}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {561}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201321438}, pages = {10}, year = {2014}, abstract = {Context. AMCVn systems are ultracompact binaries in which a (semi-) degenerate star transfers helium-dominated matter onto a white dwarf. They are effective gravitational-wave emitters and potential progenitors of Type Ia supernovae. Aims. To understand the evolution of AMCVn systems it is necessary to determine their mass-loss rate through their radiation-driven accretion-disk wind. We constructed models to perform quantitative spectroscopy of P Cygni line profiles that were detected in UV spectra. Methods. We performed 2.5D Monte Carlo radiative transfer calculations in hydrodynamic wind structures by making use of realistic NLTE spectra from the accretion disk and by accounting for the white dwarf as an additional photon source. Results. We present first results from calculations in which LTE opacities are used in the wind model. A comparison with UV spectroscopy of the AMCVn prototype shows that the modeling procedure is potentially a good tool for determining mass-loss rates and abundances of trace metals in the helium-rich wind.}, language = {en} } @article{ZinkWernerJechowetal.2014, author = {Zink, Christof and Werner, Nils and Jechow, Andreas and Heuer, Axel and Menzel, Ralf}, title = {Multi-wavelength operation of a single broad area diode laser by spectral beam combining}, series = {IEEE photonics technology letters}, volume = {26}, journal = {IEEE photonics technology letters}, number = {3}, publisher = {Inst. of Electr. and Electronics Engineers}, address = {Piscataway}, issn = {1041-1135}, doi = {10.1109/LPT.2013.2291963}, pages = {253 -- 256}, year = {2014}, abstract = {Stabilized multi-wavelength emission from a single emitter broad area diode laser (BAL) is realized by utilizing an external cavity with a spectral beam combining architecture. Self-organized emitters that are equidistantly spaced across the slow axis are enforced by the spatially distributed wavelength selectivity of the external cavity. This resulted in an array like near-field emission although the BAL is physically a single emitter without any epitaxial sub-structuring and only one electrical contact. Each of the self-organized emitters is operated at a different wavelength and the emission is multiplexed into one spatial mode with near-diffraction limited beam quality. With this setup, multi-line emission of 31 individual spectral lines centered around and a total spectral width of 3.6 nm is realized with a 1000 mu m wide BAL just above threshold. To the best of our knowledge, this is the first demonstration of such a self-organization of emitters by optical feedback utilizing a spectral beam combining architecture.}, language = {en} } @phdthesis{Fischer2014, author = {Fischer, Jost Leonhardt}, title = {Nichtlineare Kopplungsmechanismen akustischer Oszillatoren am Beispiel der Synchronisation von Orgelpfeifen}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-71975}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {In dieser Arbeit werden nichtlineare Kopplungsmechanismen von akustischen Oszillatoren untersucht, die zu Synchronisation f{\"u}hren k{\"o}nnen. Aufbauend auf die Fragestellungen vorangegangener Arbeiten werden mit Hilfe theoretischer und experimenteller Studien sowie mit Hilfe numerischer Simulationen die Elemente der Tonentstehung in der Orgelpfeife und die Mechanismen der gegenseitigen Wechselwirkung von Orgelpfeifen identifiziert. Daraus wird erstmalig ein vollst{\"a}ndig auf den aeroakustischen und fluiddynamischen Grundprinzipien basierendes nichtlinear gekoppeltes Modell selbst-erregter Oszillatoren f{\"u}r die Beschreibung des Verhaltens zweier wechselwirkender Orgelpfeifen entwickelt. Die durchgef{\"u}hrten Modellrechnungen werden mit den experimentellen Befunden verglichen. Es zeigt sich, dass die Tonentstehung und die Kopplungsmechanismen von Orgelpfeifen durch das entwickelte Oszillatormodell in weiten Teilen richtig beschrieben werden. Insbesondere kann damit die Ursache f{\"u}r den nichtlinearen Zusammenhang von Kopplungsst{\"a}rke und Synchronisation des gekoppelten Zwei-Pfeifen Systems, welcher sich in einem nichtlinearen Verlauf der Arnoldzunge darstellt, gekl{\"a}rt werden. Mit den gewonnenen Erkenntnissen wird der Einfluss des Raumes auf die Tonentstehung bei Orgelpfeifen betrachtet. Daf{\"u}r werden numerische Simulationen der Wechselwirkung einer Orgelpfeife mit verschiedenen Raumgeometrien, wie z. B. ebene, konvexe, konkave, und gezahnte Geometrien, exemplarisch untersucht. Auch der Einfluss von Schwellk{\"a}sten auf die Tonentstehung und die Klangbildung der Orgelpfeife wird studiert. In weiteren, neuartigen Synchronisationsexperimenten mit identisch gestimmten Orgelpfeifen, sowie mit Mixturen wird die Synchronisation f{\"u}r verschiedene, horizontale und vertikale Pfeifenabst{\"a}nde in der Ebene der Schallabstrahlung, untersucht. Die dabei erstmalig beobachteten r{\"a}umlich isotropen Unstetigkeiten im Schwingungsverhalten der gekoppelten Pfeifensysteme, deuten auf abstandsabh{\"a}ngige Wechsel zwischen gegen- und gleichphasigen Sychronisationsregimen hin. Abschließend wird die M{\"o}glichkeit dokumentiert, das Ph{\"a}nomen der Synchronisation zweier Orgelpfeifen durch numerische Simulationen, also der Behandlung der kompressiblen Navier-Stokes Gleichungen mit entsprechenden Rand- und Anfangsbedingungen, realit{\"a}tsnah abzubilden. Auch dies stellt ein Novum dar.}, language = {de} } @article{CherstvyMetzler2014, author = {Cherstvy, Andrey G. and Metzler, Ralf}, title = {Nonergodicity, fluctuations, and criticality in heterogeneous diffusion processes}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {90}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {1}, publisher = {American Physical Society}, address = {College Park}, issn = {1539-3755}, doi = {10.1103/PhysRevE.90.012134}, pages = {11}, year = {2014}, abstract = {We study the stochastic behavior of heterogeneous diffusion processes with the power-law dependence D(x) similar to vertical bar x vertical bar(alpha) of the generalized diffusion coefficient encompassing sub- and superdiffusive anomalous diffusion. Based on statistical measures such as the amplitude scatter of the time-averaged mean-squared displacement of individual realizations, the ergodicity breaking and non-Gaussianity parameters, as well as the probability density function P(x, t), we analyze the weakly nonergodic character of the heterogeneous diffusion process and, particularly, the degree of irreproducibility of individual realizations. As we show, the fluctuations between individual realizations increase with growing modulus vertical bar alpha vertical bar of the scaling exponent. The fluctuations appear to diverge when the critical value alpha = 2 is approached, while for even larger alpha the fluctuations decrease, again. At criticality, the power-law behavior of the mean-squared displacement changes to an exponentially fast growth, and the fluctuations of the time-averaged mean-squared displacement do not converge for increasing number of realizations. From a systematic comparison we observe some striking similarities of the heterogeneous diffusion process with the familiar subdiffusive continuous time random walk process with power-law waiting time distribution and diverging characteristic waiting time.}, language = {en} } @article{FoertigKniepertGlueckeretal.2014, author = {Foertig, Alexander and Kniepert, Juliane and Gluecker, Markus and Brenner, Thomas J. K. and Dyakonov, Vladimir and Neher, Dieter and Deibel, Carsten}, title = {Nongeminate and geminate recombination in PTB7: PCBM solar cells}, series = {Advanced functional materials}, volume = {24}, journal = {Advanced functional materials}, number = {9}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1616-301X}, doi = {10.1002/adfm.201302134}, pages = {1306 -- 1311}, year = {2014}, language = {en} } @article{LepriPikovskij2014, author = {Lepri, Stefano and Pikovskij, Arkadij}, title = {Nonreciprocal wave scattering on nonlinear string-coupled oscillators}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {24}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {4}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/1.4899205}, pages = {9}, year = {2014}, abstract = {We study scattering of a periodic wave in a string on two lumped oscillators attached to it. The equations can be represented as a driven (by the incident wave) dissipative (due to radiation losses) system of delay differential equations of neutral type. Nonlinearity of oscillators makes the scattering non-reciprocal: The same wave is transmitted differently in two directions. Periodic regimes of scattering are analyzed approximately, using amplitude equation approach. We show that this setup can act as a nonreciprocal modulator via Hopf bifurcations of the steady solutions. Numerical simulations of the full system reveal nontrivial regimes of quasiperiodic and chaotic scattering. Moreover, a regime of a "chaotic diode," where transmission is periodic in one direction and chaotic in the opposite one, is reported. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{NezhadhaghighiChechkinMetzler2014, author = {Nezhadhaghighi, M. Ghasemi and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Numerical approach to unbiased and driven generalized elastic model}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {140}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {2}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.4858425}, pages = {9}, year = {2014}, abstract = {From scaling arguments and numerical simulations, we investigate the properties of the generalized elastic model (GEM) that is used to describe various physical systems such as polymers, membranes, single-file systems, or rough interfaces. We compare analytical and numerical results for the subdiffusion exponent beta characterizing the growth of the mean squared displacement <(delta h)(2)> of the field h described by the GEM dynamic equation. We study the scaling properties of the qth order moments with time, finding that the interface fluctuations show no intermittent behavior. We also investigate the ergodic properties of the process h in terms of the ergodicity breaking parameter and the distribution of the time averaged mean squared displacement. Finally, we study numerically the driven GEM with a constant, localized perturbation and extract the characteristics of the average drift for a tagged probe.}, language = {en} } @article{AcciariArlenAuneetal.2014, author = {Acciari, V. A. and Arlen, T. and Aune, T. and Benbow, W. and Bird, R. and Bouvier, A. and Bradbury, S. M. and Buckley, J. H. and Bugaev, V. and de la Calle Perez, I. and Carter-Lewis, D. A. and Cesarini, A. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Falcone, A. and Federici, Simone and Fegan, D. J. and Fegan, S. J. and Finley, J. P. and Finnegan, G. and Fortson, L. and Gaidos, J. and Galante, N. and Gall, D. and Gibbs, K. and Gillanders, G. H. and Griffin, S. and Grube, J. and Gyuk, G. and Hanna, D. and Horan, D. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and McEnery, J. E. and Madhavan, A. S. and Moriarty, P. and Nelson, T. and Ong, R. A. and Orr, M. and Otte, A. N. and Perkins, J. S. and Petry, D. and Pichel, A. and Pohl, M. and Quinn, J. and Ragan, K. and Reynolds, T. and Roache, E. and Rovero, A. and Schroedter, M. and Sembroski, G. H. and Smith, A. and Telezhinsky, Igor O. and Theiling, M. and Toner, J. and Tyler, J. and Varlotta, A. and Vivier, M. and Wakely, S. P. and Ward, J. E. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Williams, D. A. and Wissel, S.}, title = {Observation of Markarian 421 in TeV gamma rays over a 14-year time span}, series = {Astroparticle physics}, volume = {54}, journal = {Astroparticle physics}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0927-6505}, doi = {10.1016/j.astropartphys.2013.10.004}, pages = {1 -- 10}, year = {2014}, abstract = {The variability of the blazar Markarian 421 in TeV gamma rays over a 14-year time period has been explored with the Whipple 10 m telescope. It is shown that the dynamic range of its flux variations is large and similar to that in X-rays. A correlation between the X-ray and TeV energy bands is observed during some bright flares and when the complete data sets are binned on long timescales. The main database consists of 878.4 h of observation with the Whipple telescope, spread over 783 nights. The peak energy response of the telescope was 400 GeV with 20\% uncertainty. This is the largest database of any TeV-emitting active galactic nucleus (AGN) and hence was used to explore the variability profile of Markarian 421. The tithe-averaged flux from Markarian 421 over this period was 0.446 +/- 0.008 Crab flux units. The flux exceeded 10 Crab flux units on three separate occasions. For the 2000-2001 season the average flux reached 1.86 Crab units, while in the 1996-1997 season the average flux was only 0.23 Crab units.}, language = {en} } @article{DanehkarTodtErcolanoetal.2014, author = {Danehkar, A. and Todt, Helge Tobias and Ercolano, B. and Kniazev, A. Y.}, title = {Observations and three-dimensional photoionization modelling of the Wolf-Rayet planetary nebula Abell 48(star)}, series = {Monthly notices of the Royal Astronomical Society}, volume = {439}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu203}, pages = {3605 -- 3615}, year = {2014}, abstract = {Recent observations reveal that the central star of the planetary nebula Abell 48 exhibits spectral features similar to massive nitrogen-sequence Wolf-Rayet stars. This raises a pertinent question, whether it is still a planetary nebula or rather a ring nebula of a massive star. In this study, we have constructed a three-dimensional photoionization model of Abell 48, constrained by our new optical integral field spectroscopy. An analysis of the spatially resolved velocity distributions allowed us to constrain the geometry of Abell 48. We used the collisionally excited lines to obtain the nebular physical conditions and ionic abundances of nitrogen, oxygen, neon, sulphur and argon, relative to hydrogen. We also determined helium temperatures and ionic abundances of helium and carbon from the optical recombination lines. We obtained a good fit to the observations for most of the emission-line fluxes in our photoionization model. The ionic abundances deduced from our model are in decent agreement with those derived by the empirical analysis. However, we notice obvious discrepancies between helium temperatures derived from the model and the empirical analysis, as overestimated by our model. This could be due to the presence of a small fraction of cold metal-rich structures, which were not included in our model. It is found that the observed nebular line fluxes were best reproduced by using a hydrogen-deficient expanding model atmosphere as the ionizing source with an effective temperature of T-eff = 70 kK and a stellar luminosity of L-star = 5500 L-circle dot, which corresponds to a relatively low-mass progenitor star (similar to 3 M-circle dot) rather than a massive Pop I star.}, language = {en} } @article{AliuAuneBeheraetal.2014, author = {Aliu, E. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Buckley, J. H. and Bugaev, V. and Cardenzana, J. V. and Cerruti, M. and Chen, X. and Ciupik, L. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kargaltsev, Oleg and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Lang, M. J. and Madhavan, A. S. and Maier, G. and Majumdar, P. and McCann, A. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Pandel, D. and Perkins, J. S. and Pohl, Manuela and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sembroski, G. H. and Skole, C. and Staszak, D. and Telezhinsky, Igor O. and Theiling, M. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vincent, S. and Wakely, S. P. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Williams, D. A. and Zitzer, B.}, title = {Observations of the unidentified gamm-ray source TeV J2032+4130 BY Veritas}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {783}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/783/1/16}, pages = {9}, year = {2014}, language = {en} } @article{ReindlRauchWerneretal.2014, author = {Reindl, Nicole and Rauch, Thomas and Werner, Klaus and Kruk, J. W. and Todt, Helge Tobias}, title = {On helium-dominated stellar evolution: the mysterious role of the O(He)-type stars}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {566}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201423498}, pages = {23}, year = {2014}, abstract = {Context. About a quarter of all post-asymptotic giant branch (AGB) stars are hydrogen-deficient. Stellar evolutionary models explain the carbon-dominated H-deficient stars by a (very) late thermal pulse scenario where the hydrogen-rich envelope is mixed with the helium-rich intershell layer. Depending on the particular time at which the final flash occurs, the entire hydrogen envelope may be burned. In contrast, helium-dominated post-AGB stars and their evolution are not yet understood. Aims. A small group of very hot, helium-dominated stars is formed by O(He)-type stars. A precise analysis of their photospheric abundances will establish constraints to their evolution. Methods. We performed a detailed spectral analysis of ultraviolet and optical spectra of four O(He) stars by means of state-of-the-art non-LTE model-atmosphere techniques. Results. We determined effective temperatures, surface gravities, and the abundances of H, He, C, N, O, F, Ne, Si, P, S, Ar, and Fe. By deriving upper limits for the mass-loss rates of the O(He) stars, we found that they do not exhibit enhanced mass-loss. The comparison with evolutionary models shows that the status of the O(He) stars remains uncertain. Their abundances match predictions of a double helium white dwarf (WD) merger scenario, suggesting that they might be the progeny of the compact and of the luminous helium-rich sdO-type stars. The existence of planetary nebulae that do not show helium enrichment around every other O(He) star precludes a merger origin for these stars. These stars must have formed in a different way, for instance via enhanced mass-loss during their post-AGB evolution or a merger within a common-envelope (CE) of a CO-WD and a red giant or AGB star. Conclusions. A helium-dominated stellar evolutionary sequence exists that may be fed by different types of mergers or CE scenarios. It appears likely that all these pass through the O(He) phase just before they become WDs.}, language = {en} } @article{MkrtchianHenkel2014, author = {Mkrtchian, Vanik E. and Henkel, Carsten}, title = {On non-equilibrium photon distributions in the Casimir effect}, series = {Annalen der Physik}, volume = {526}, journal = {Annalen der Physik}, number = {1-2}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0003-3804}, doi = {10.1002/andp.201300135}, pages = {87 -- 101}, year = {2014}, abstract = {The electromagnetic field in a typical geometry of the Casimir effect is described in the Schwinger-Keldysh formalism. The main result is the photon distribution function (Keldysh Green function) in any stationary state of the field. A two-plate geometry with a sliding interface in local equilibrium is studied in detail, and full agreement with the results of Rytov fluctuation electrodynamics is found.}, language = {en} } @article{AlbrechtVandewalTumblestonetal.2014, author = {Albrecht, Steve and Vandewal, Koen and Tumbleston, John R. and Fischer, Florian S. U. and Douglas, Jessica D. and Frechet, Jean M. J. and Ludwigs, Sabine and Ade, Harald W. and Salleo, Alberto and Neher, Dieter}, title = {On the efficiency of charge transfer state splitting in polymer: Fullerene solar cells}, series = {Advanced materials}, volume = {26}, journal = {Advanced materials}, number = {16}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0935-9648}, doi = {10.1002/adma.201305283}, pages = {2533 -- 2539}, year = {2014}, language = {en} } @phdthesis{Conrad2014, author = {Conrad, Claudia}, title = {Open cluster groups and complexes}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-77605}, school = {Universit{\"a}t Potsdam}, pages = {xii, 172}, year = {2014}, abstract = {It is generally agreed upon that stars typically form in open clusters and stellar associations, but little is known about the structure of the open cluster system. Do open clusters and stellar associations form isolated or do they prefer to form in groups and complexes? Open cluster groups and complexes could verify star forming regions to be larger than expected, which would explain the chemical homogeneity over large areas in the Galactic disk. They would also define an additional level in the hierarchy of star formation and could be used as tracers for the scales of fragmentation in giant molecular clouds? Furthermore, open cluster groups and complexes could affect Galactic dynamics and should be considered in investigations and simulations on the dynamical processes, such as radial migration, disc heating, differential rotation, kinematic resonances, and spiral structure. In the past decade there were a few studies on open cluster pairs (de La Fuente Marcos \& de La Fuente Marcos 2009a,b,c) and on open cluster groups and complexes (Piskunov et al. 2006). The former only considered spatial proximity for the identification of the pairs, while the latter also required tangential velocities to be similar for the members. In this work I used the full set of 6D phase-space information to draw a more detailed picture on these structures. For this purpose I utilised the most homogeneous cluster catalogue available, namely the Catalogue of Open Cluster Data (COCD; Kharchenko et al. 2005a,b), which contains parameters for 650 open clusters and compact associations, as well as for their uniformly selected members. Additional radial velocity (RV) and metallicity ([M/H]) information on the members were obtained from the RAdial Velocity Experiment (RAVE; Steinmetz et al. 2006; Kordopatis et al. 2013) for 110 and 81 clusters, respectively. The RAVE sample was cleaned considering quality parameters and flags provided by RAVE (Matijevič et al. 2012; Kordopatis et al. 2013). To ensure that only real members were included for the mean values, also the cluster membership, as provided by Kharchenko et al. (2005a,b), was considered for the stars cross-matched in RAVE. 6D phase-space information could be derived for 432 out of the 650 COCD objects and I used an adaption of the Friends-of-Friends algorithm, as used in cosmology, to identify potential groupings. The vast majority of the 19 identified groupings were pairs, but I also found four groups of 4-5 members and one complex with 15 members. For the verification of the identified structures, I compared the results to a randomly selected subsample of the catalogue for the Milky Way global survey of Star Clusters (MWSC; Kharchenko et al. 2013), which became available recently, and was used as reference sample. Furthermore, I implemented Monte-Carlo simulations with randomised samples created from two distinguished input distributions for the spatial and velocity parameters. On the one hand, assuming a uniform distribution in the Galactic disc and, on the other hand, assuming the COCD data distributions to be representative for the whole open cluster population. The results suggested that the majority of identified pairs are rather by chance alignments, but the groups and the complex seemed to be genuine. A comparison of my results to the pairs, groups and complexes proposed in the literature yielded a partial overlap, which was most likely because of selection effects and different parameters considered. This is another verification for the existence of such structures. The characteristics of the found groupings favour that members of an open cluster grouping originate from a common giant molecular cloud and formed in a single, but possibly sequential, star formation event. Moreover, the fact that the young open cluster population showed smaller spatial separations between nearest neighbours than the old cluster population indicated that the lifetime of open cluster groupings is most likely comparable to that of the Galactic open cluster population itself. Still even among the old open clusters I could identify groupings, which suggested that the detected structure could be in some cases more long lived as one might think. In this thesis I could only present a pilot study on structures in the Galactic open cluster population, since the data sample used was highly incomplete. For further investigations a far more complete sample would be required. One step in this direction would be to use data from large current surveys, like SDSS, RAVE, Gaia-ESO and VVV, as well as including results from studies on individual clusters. Later the sample can be completed by data from upcoming missions, like Gaia and 4MOST. Future studies using this more complete open cluster sample will reveal the effect of open cluster groupings on star formation theory and their significance for the kinematics, dynamics and evolution of the Milky Way, and thereby of spiral galaxies.}, language = {en} } @misc{EschenlohrBattiatoMaldonadoetal.2014, author = {Eschenlohr, Andrea and Battiato, Mario and Maldonado, P. and Pontius, N. and Kachel, T. and Holldack, K. and Mitzner, Rolf and F{\"o}hlisch, Alexander and Oppeneer, P. M. and Stamm, Christian}, title = {Optical excitation of thin magnetic layers in multilayer structures Reply}, series = {Nature materials}, volume = {13}, journal = {Nature materials}, number = {2}, publisher = {Nature Publ. Group}, address = {London}, issn = {1476-1122}, doi = {10.1038/nmat3851}, pages = {102 -- 103}, year = {2014}, language = {en} } @article{ProctorAlbrechtKuiketal.2014, author = {Proctor, Christopher M. and Albrecht, Steve and Kuik, Martijn and Neher, Dieter and Thuc-Quyen Nguyen,}, title = {Overcoming geminate recombination and enhancing extraction in solution-processed small molecule solar cells}, series = {dvanced energy materials}, volume = {4}, journal = {dvanced energy materials}, number = {10}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1614-6832}, doi = {10.1002/aenm.201400230}, pages = {7}, year = {2014}, language = {en} } @misc{MouleNeherTurner2014, author = {Moule, Adam J. and Neher, Dieter and Turner, Sarah T.}, title = {P3HT-Based solar cells: structural properties and photovoltaic performance}, series = {Advances in Polymer Science}, volume = {265}, journal = {Advances in Polymer Science}, editor = {Ludwigs, S}, publisher = {Springer}, address = {Berlin}, isbn = {978-3-662-45145-8; 978-3-662-45144-1}, issn = {0065-3195}, doi = {10.1007/12_2014_289}, pages = {181 -- 232}, year = {2014}, abstract = {Each year we are bombarded with B.Sc. and Ph.D. applications from students that want to improve the world. They have learned that their future depends on changing the type of fuel we use and that solar energy is our future. The hope and energy of these young people will transform future energy technologies, but it will not happen quickly. Organic photovoltaic devices are easy to sketch, but the materials, processing steps, and ways of measuring the properties of the materials are very complicated. It is not trivial to make a systematic measurement that will change the way other research groups think or practice. In approaching this chapter, we thought about what a new researcher would need to know about organic photovoltaic devices and materials in order to have a good start in the subject. Then, we simplified that to focus on what a new researcher would need to know about poly-3-hexylthiophene: phenyl-C61-butyric acid methyl ester blends (P3HT: PCBM) to make research progress with these materials. This chapter is by no means authoritative or a compendium of all things on P3HT: PCBM. We have selected to explain how the sample fabrication techniques lead to control of morphology and structural features and how these morphological features have specific optical and electronic consequences for organic photovoltaic device applications.}, language = {en} } @article{CherstvyChechkinMetzler2014, author = {Cherstvy, Andrey G. and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Particle invasion, survival, and non-ergodicity in 2D diffusion processes with space-dependent diffusivity}, series = {Soft matter}, volume = {10}, journal = {Soft matter}, number = {10}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1744-683X}, doi = {10.1039/c3sm52846d}, pages = {1591 -- 1601}, year = {2014}, abstract = {We study the thermal Markovian diffusion of tracer particles in a 2D medium with spatially varying diffusivity D(r), mimicking recently measured, heterogeneous maps of the apparent diffusion coefficient in biological cells. For this heterogeneous diffusion process (HDP) we analyse the mean squared displacement (MSD) of the tracer particles, the time averaged MSD, the spatial probability density function, and the first passage time dynamics from the cell boundary to the nucleus. Moreover we examine the non-ergodic properties of this process which are important for the correct physical interpretation of time averages of observables obtained from single particle tracking experiments. From extensive computer simulations of the 2D stochastic Langevin equation we present an in-depth study of this HDP. In particular, we find that the MSDs along the radial and azimuthal directions in a circular domain obey anomalous and Brownian scaling, respectively. We demonstrate that the time averaged MSD stays linear as a function of the lag time and the system thus reveals a weak ergodicity breaking. Our results will enable one to rationalise the diffusive motion of larger tracer particles such as viruses or submicron beads in biological cells.}, language = {en} } @article{ZakrevskyyTitovLomadzeetal.2014, author = {Zakrevskyy, Yuriy and Titov, Evgenii and Lomadze, Nino and Santer, Svetlana}, title = {Phase diagrams of DNA-photosensitive surfactant complexes: Effect of ionic strength and surfactant structure}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {141}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {16}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.4899281}, pages = {8}, year = {2014}, abstract = {Realization of all-optically controlled and efficient DNA compaction is the major motivation in the study of interactions between DNA and photosensitive surfactants. In this article, using recently published approach of phase diagram construction [Y. Zakrevskyy, P. Cywinski, M. Cywinska, J. Paasche, N. Lomadze, O. Reich, H.-G. Lohmannsroben, and S. Santer, J. Chem. Phys. 140, 044907 (2014)], a strategy for substantial reduction of compaction agent concentration and simultaneous maintaining the light-induced decompaction efficiency is proposed. The role of ionic strength (NaCl concentration), as a very important environmental parameter, and surfactant structure (spacer length) on the changes of positions of phase transitions is investigated. Increase of ionic strength leads to increase of the surfactant concentration needed to compact DNA molecule. However, elongation of the spacer results to substantial reduction of this concentration. DNA compaction by surfactants with longer tails starts to take place in diluted solutions at charge ratios Z < 1 and is driven by azobenzene-aggregation compaction mechanism, which is responsible for efficient decompaction. Comparison of phase diagrams for different DNA-photosensitive surfactant systems allowed explanation and proposal of a strategy to overcome previously reported limitations of the light-induced decompaction for complexes with increasing surfactant hydrophobicity. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{HeuerRaabeMenzel2014, author = {Heuer, Axel and Raabe, S. and Menzel, Ralf}, title = {Phase memory across two single-photon interferometers including wavelength conversion}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {90}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {4}, publisher = {American Physical Society}, address = {College Park}, issn = {1050-2947}, doi = {10.1103/PhysRevA.90.045803}, pages = {4}, year = {2014}, abstract = {Spontaneous parametric down-conversion (SPDC) in a nonlinear crystal generates two single photons (signal and idler) with random phases. Thus, no first-order interference between them occurs. However, coherence can be induced in a cascaded setup of two crystals if, e.g., the idler modes of both crystals are aligned to be indistinguishable. Due to the effect of phase memory it is found that the first-order interference of the signal beams can be controlled by the phase delay between the pump beams. Even for pump photon delays much larger than the coherence length of the SPDC photons, the visibility is above 90\%. The high visibilities reported here prove an almost perfect phase memory effect across the two interferometers for the pump and the signal photon modes.}, language = {en} }