@article{vanDrielGesztelyiBakerToeroeketal.2014, author = {van Driel-Gesztelyi, L. and Baker, Daniel N. and Toeroek, T. and Pariat, E. and Green, L. M. and Williams, D. R. and Carlyle, J. and Valori, G. and Demoulin, Pascal and Kliem, Bernhard and Long, D. M. and Matthews, S. A. and Malherbe, J. -M.}, title = {Coronal magnetic reconnection driven by CME expansion-the 2011 June 7 event}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {788}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/788/1/85}, pages = {12}, year = {2014}, abstract = {Coronal mass ejections (CMEs) erupt and expand in a magnetically structured solar corona. Various indirect observational pieces of evidence have shown that the magnetic field of CMEs reconnects with surrounding magnetic fields, forming, e.g., dimming regions distant from the CME source regions. Analyzing Solar Dynamics Observatory (SDO) observations of the eruption from AR 11226 on 2011 June 7, we present the first direct evidence of coronal magnetic reconnection between the fields of two adjacent active regions during a CME. The observations are presented jointly with a data-constrained numerical simulation, demonstrating the formation/intensification of current sheets along a hyperbolic flux tube at the interface between the CME and the neighboring AR 11227. Reconnection resulted in the formation of new magnetic connections between the erupting magnetic structure from AR 11226 and the neighboring active region AR 11227 about 200 Mm from the eruption site. The onset of reconnection first becomes apparent in the SDO/AIA images when filament plasma, originally contained within the erupting flux rope, is redirected toward remote areas in AR 11227, tracing the change of large-scale magnetic connectivity. The location of the coronal reconnection region becomes bright and directly observable at SDO/AIA wavelengths, owing to the presence of down-flowing cool, dense (1010 cm(-3)) filament plasma in its vicinity. The high-density plasma around the reconnection region is heated to coronal temperatures, presumably by slow-mode shocks and Coulomb collisions. These results provide the first direct observational evidence that CMEs reconnect with surrounding magnetic structures, leading to a large-scale reconfiguration of the coronal magnetic field.}, language = {en} } @article{AliuAuneBeheraetal.2014, author = {Aliu, E. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Connolly, M. P. and Cui, W. and Dumm, J. and Dwarkadas, Vikram V. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Gotthelf, E. V. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kargaltsev, O. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McArthur, S. and McCann, A. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Pandel, D. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Roberts, M. and Sembroski, G. H. and Shahinyan, K. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Tucci, J. V. and Tyler, J. and Vincent, S. and Wakely, S. P. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B.}, title = {Spatially resolving the very high energy emission from MRGO J2019+37 wih veritas}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {788}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/788/1/78}, pages = {10}, year = {2014}, abstract = {We present very high energy (VHE) imaging of MGRO J2019+37 obtained with the VERITAS observatory. The bright extended (similar to 2 degrees) unidentified Milagro source is located toward the rich star formation region Cygnus-X. MGRO J2019+37 is resolved into two VERITAS sources. The faint, point-like source VER J2016+371 overlaps CTB 87, a filled-center remnant (SNR) with no evidence of a supernova remnant shell at the present time. Its spectrum is well fit in the 0.65-10 TeV energy range by a power-law model with photon index 2.3 +/- 0.4. VER J2019+378 is a bright extended (similar to 1 degrees) source that likely accounts for the bulk of the Milagro emission and is notably coincident with PSR J2021+3651 and the star formation region Sh 2-104. Its spectrum in the range 1-30 TeV is well fit with a power-law model of photon index 1.75 +/- 0.3, among the hardest values measured in the VHE band, comparable to that observed near Vela-X. We explore the unusual spectrum and morphology in the radio and X-ray bands to constrain possible emission mechanisms for this source.}, language = {en} } @misc{CardinalettiKestersBerthoetal.2014, author = {Cardinaletti, Ilaria and Kesters, Jurgen and Bertho, Sabine and Conings, Bert and Piersimoni, Fortunato and Lutsen, Laurence and Nesladek, Milos and Van Mele, Bruno and Van Assche, Guy and Vandewal, Koen and Salleo, Alberto and Vanderzande, Dirk and Maes, Wouter and Manca, Jean V.}, title = {Toward bulk heterojunction polymer solar cells with thermally stable active layer morphology}, series = {Journal of photonics for energy}, volume = {4}, journal = {Journal of photonics for energy}, publisher = {SPIE}, address = {Bellingham}, issn = {1947-7988}, doi = {10.1117/1.JPE.4.040997}, pages = {12}, year = {2014}, abstract = {When state-of-the-art bulk heterojunction organic solar cells with ideal morphology are exposed to prolonged storage or operation at elevated temperatures, a thermally induced disruption of the active layer blend can occur, in the form of a separation of donor and acceptor domains, leading to diminished photovoltaic performance. Toward the long-term use of organic solar cells in real-life conditions, an important challenge is, therefore, the development of devices with a thermally stable active layer morphology. Several routes are being explored, ranging from the use of high glass transition temperature, cross-linkable and/or side-chain functionalized donor and acceptor materials, to light-induced dimerization of the fullerene acceptor. A better fundamental understanding of the nature and underlying mechanisms of the phase separation and stabilization effects has been obtained through a variety of analytical, thermal analysis, and electro-optical techniques. Accelerated aging systems have been used to study the degradation kinetics of bulk heterojunction solar cells in situ at various temperatures to obtain aging models predicting solar cell lifetime. The following contribution gives an overview of the current insights regarding the intrinsic thermally induced aging effects and the proposed solutions, illustrated by examples of our own research groups. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License.}, language = {en} } @article{ZinkNiebuhrJechowetal.2014, author = {Zink, Christof and Niebuhr, Mario and Jechow, Andreas and Heuer, Axel and Menzel, Ralf}, title = {Broad area diode laser with on-chip transverse Bragg grating stabilized in an off-axis external cavity}, series = {Optics express : the international electronic journal of optics}, volume = {22}, journal = {Optics express : the international electronic journal of optics}, number = {12}, publisher = {Optical Society of America}, address = {Washington}, issn = {1094-4087}, doi = {10.1364/OE.22.014108}, pages = {14108 -- 14113}, year = {2014}, abstract = {The emission characteristics of a novel, specially designed broad area diode laser (BAL) with on-chip transversal Bragg resonance (TBR) grating in lateral direction were investigated in an off-axis external cavity setup. The internal TBR grating defines a low loss transversal mode at a specific angle of incidence and a certain wavelength. By providing feedback at this specific angle with an external mirror, it is possible to select this low loss transverse mode and stabilize the BAL. Near diffraction limited emission with an almost single lobed far field pattern could be realized, in contrast to the double lobed far field pattern of similar setups using standard BALs or phase-locked diode laser arrays. Furthermore, we could achieve a narrow bandwidth emission with a simplified setup without external frequency selective elements. (C) 2014 Optical Society of America}, language = {en} } @article{ArchambaultArlenAuneetal.2014, author = {Archambault, S. and Arlen, T. and Aune, T. and Beilicke, M. and Benbow, W. and Bird, R. and Boettcher, Markus and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dickherber, R. and Dumm, J. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fortson, L. and Furniss, A. and Galante, N. and Gall, D. and Garson, A. III. and Gillanders, G. H. and Griffin, S. and Grube, J. and Gusbar, C. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Lamerato, A. and Lang, M. J. and Li, K. and Madhavan, A. S. and Maier, G. and Majumdar, P. and McArthur, S. and McCann, A. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Orr, M. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, Martin and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Roustazadeh, P. and Saxon, D. B. and Sembroski, G. H. and Senturk, G. D. and Skole, C. and Staszak, D. and Telezhinsky, Igor O. and Tesic, G. and Theiling, M. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weinstein, A. and Welsing, R. and Williams, D. A. and Zitzer, B.}, title = {Test of models of the cosmic infrared background with multiwavelength observations of the blazar 1ES 1218+30.4 IN 2009}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {788}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/788/2/158}, pages = {9}, year = {2014}, abstract = {We present the results of a multi-wavelength campaign targeting the blazar 1ES 1218+30.4 with observations with the 1.3 m McGraw-Hill optical telescope, the Rossi X-ray Timing Explorer (RXTE), the Fermi Gamma-Ray Space Telescope, and the Very Energetic Radiation Imaging Telescope Array System (VERITAS). The RXTE and VERITAS observations were spread over a 13 day period and revealed clear evidence for flux variability, and a strong X-ray and gamma-ray flare on 2009 February 26 (MJD 54888). The campaign delivered a well-sampled broadband energy spectrum with simultaneous RXTE and VERITAS very high energy (VHE, > 100 GeV) observations, as well as contemporaneous optical and Fermi observations. The 1ES 1218+30.4 broadband energy spectrum-the first with simultaneous X-ray and VHE gamma-ray energy spectra-is of particular interest as the source is located at a high cosmological redshift for a VHE source (z = 0.182), leading to strong absorption of VHE gamma rays by photons from the optical/infrared extragalactic background light (EBL) via gamma VHE +gamma EBL -> e(+) e(-)pair-creation processes. We model the data with a one-zone synchrotron self-Compton (SSC) emission model and with the extragalactic absorption predicted by several recent EBL models. We find that the observations are consistent with the SSC scenario and all the EBL models considered in this work. We discuss observational and theoretical avenues to improve on the EBL constraints.}, language = {en} } @article{ZhangChenBoettcher2014, author = {Zhang, Haocheng and Chen, Xuhui and Boettcher, Markus}, title = {Synchrotron polarization in blazars}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {789}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/789/1/66}, pages = {16}, year = {2014}, abstract = {We present a detailed analysis of time-and energy-dependent synchrotron polarization signatures in a shock-in-jet model for gamma-ray blazars. Our calculations employ a full three-dimensional radiation transfer code, assuming a helical magnetic field throughout the jet. The code considers synchrotron emission from an ordered magnetic field, and takes into account all light-travel-time and other relevant geometric effects, while the relevant synchrotron self-Compton and external Compton effects are handled with the two-dimensional Monte-Carlo/Fokker-Planck (MCFP) code. We consider several possible mechanisms through which a relativistic shock propagating through the jet may affect the jet plasma to produce a synchrotron and high-energy flare. Most plausibly, the shock is expected to lead to a compression of the magnetic field, increasing the toroidal field component and thereby changing the direction of the magnetic field in the region affected by the shock. We find that such a scenario leads to correlated synchrotron + synchrotron-self-Compton flaring, associated with substantial variability in the synchrotron polarization percentage and position angle. Most importantly, this scenario naturally explains large polarization angle rotations by greater than or similar to 180 degrees, as observed in connection with gamma-ray flares in several blazars, without the need for bent or helical jet trajectories or other nonaxisymmetric jet features.}, language = {en} } @article{KliemLinForbesetal.2014, author = {Kliem, Bernhard and Lin, J. and Forbes, T. G. and Priest, E. R. and Toeroek, T.}, title = {Catastrophe versus instability for the eruption of a toroadal solar magnetic flux}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {789}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/789/1/46}, pages = {13}, year = {2014}, abstract = {The onset of a solar eruption is formulated here as either a magnetic catastrophe or as an instability. Both start with the same equation of force balance governing the underlying equilibria. Using a toroidal flux rope in an external bipolar or quadrupolar field as a model for the current-carrying flux, we demonstrate the occurrence of a fold catastrophe by loss of equilibrium for several representative evolutionary sequences in the stable domain of parameter space. We verify that this catastrophe and the torus instability occur at the same point; they are thus equivalent descriptions for the onset condition of solar eruptions.}, language = {en} } @article{NuzaParisiScannapiecoetal.2014, author = {Nuza, Sebastian E. and Parisi, Florencia and Scannapieco, Cecilia and Richter, Philipp and Gottloeber, Stefan and Steinmetz, Matthias}, title = {The distribution of gas in the Local Group from constrained cosmological simulations: the case for Andromeda and the Milky Way galaxies}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu643}, pages = {2593 -- 2612}, year = {2014}, abstract = {We study the gas distribution in the Milky Way and Andromeda using a constrained cosmological simulation of the Local Group (LG) within the context of the CLUES (Constrained Local UniversE Simulations) project. We analyse the properties of gas in the simulated galaxies at z = 0 for three different phases: 'cold', 'hot' and H i, and compare our results with observations. The amount of material in the hot halo (M-hot a parts per thousand 4-5 x 10(10) M-aS (TM)), and the cold (M-cold(r a parts per thousand(2) 10 kpc) a parts per thousand 10(8) M-aS (TM)) and H i components displays reasonable agreement with observations. We also compute the accretion/ejection rates together with the H i (radial and all-sky) covering fractions. The integrated H i accretion rate within r = 50 kpc gives similar to 0.2-0.3 M-aS (TM) yr(-1), i.e. close to that obtained from high-velocity clouds in the Milky Way. We find that the global accretion rate is dominated by hot material, although ionized gas with T a parts per thousand(2) 10(5) K can contribute significantly too. The net accretion rates of all material at the virial radii are 6-8 M-aS (TM) yr(-1). At z = 0, we find a significant gas excess between the two galaxies, as compared to any other direction, resulting from the overlap of their gaseous haloes. In our simulation, the gas excess first occurs at z similar to 1, as a result of the kinematical evolution of the LG.}, language = {en} } @article{ChenChatterjeeZhangetal.2014, author = {Chen, Xuhui and Chatterjee, Ritaban and Zhang, Haocheng and Pohl, Martin and Fossati, Giovanni and Boettcher, Markus and Bailyn, Charles D. and Bonning, Erin W. and Buxton, Michelle and Coppi, Paolo and Isler, Jedidah and Maraschi, Laura and Urry, Meg}, title = {Magnetic field amplification and flat spectrum radio quasars}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu713}, pages = {2188 -- 2199}, year = {2014}, abstract = {We perform time-dependent, spatially resolved simulations of blazar emission to evaluate several flaring scenarios related to magnetic-field amplification and enhanced particle acceleration. The code explicitly accounts for light-travel-time effects and is applied to flares observed in the flat spectrum radio quasar (FSRQ) PKS 0208-512, which show optical/gamma-ray correlation at some times, but orphan optical flares at other times. Changes in both the magnetic field and the particle acceleration efficiency are explored as causes of flares. Generally, external Compton (EC) emission appears to describe the available data better than a synchrotron self-Compton (SSC) scenario, and in particular orphan optical flares are difficult to produce in the SSC framework. X-ray soft-excesses, gamma-ray spectral hardening, and the detections at very high energies of certain FSRQs during flares find natural explanations in the EC scenario with particle acceleration change. Likewise, optical flares with/without gamma-ray counterparts can be explained by different allocations of energy between the magnetization and particle acceleration, which may be related to the orientation of the magnetic field relative to the jet flow. We also calculate the degree of linear polarization and polarization angle as a function of time for a jet with helical magnetic field. Tightening of the magnetic helix immediately downstream of the jet perturbations, where flares occur, can be sufficient to explain the increases in the degree of polarization and a rotation by a parts per thousand yen180A degrees of the observed polarization angle, if light-travel-time effects are properly considered.}, language = {en} } @article{MassaOskinovaFullertonetal.2014, author = {Massa, D. and Oskinova, Lidia M. and Fullerton, A. W. and Prinja, R. K. and Bohlender, D. A. and Morrison, N. D. and Blake, M. and Pych, W.}, title = {CIR modulation of the X-ray flux from the O7.5 III(n)((f)) star xi Persei(a similar to...)?}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu565}, pages = {2173 -- 2180}, year = {2014}, abstract = {We analyse a 162 ks high energy transmission grating Chandra observation of the O7.5 III(n)((f)) star xi Per, together with contemporaneous H alpha observations. The X-ray spectrum of this star is similar to other single O stars, and not pathological in any way. Its UV wind lines are known to display cyclical time variability, with a period of 2.086 d, which is thought to be associated with corotating interaction regions (CIRs). We examine the Chandra and H alpha data for variability on this time-scale. We find that the X-rays vary by similar to 15 per cent over the course of the observations and that this variability is out of phase with variable absorption on the blue wing of the H alpha profiles (assumed to be a surrogate for the UV absorption associated with CIRs). While not conclusive, both sets of data are consistent with models where the CIRs are either a source of X-rays or modulate them.}, language = {en} } @article{GaoWangLinetal.2014, author = {Gao, Guan-Nan and Wang, Min and Lin, Jun and Wu, Ning and Tan, Cheng-Ming and Kliem, Bernhard and Su, Yang}, title = {Radio observations of the fine structure inside a post-CME current sheet}, series = {Research in astronomy and astrophysics : a publication of the Chinese Astronomical Society and National Astronomical Observatories, Chinese Academy of Sciences}, volume = {14}, journal = {Research in astronomy and astrophysics : a publication of the Chinese Astronomical Society and National Astronomical Observatories, Chinese Academy of Sciences}, number = {7}, publisher = {Chinese Astronomical Society and National Astronomical Observatories, Chinese Academy of Sciences}, address = {Beijing}, issn = {1674-4527}, doi = {10.1088/1674-4527/14/7/006}, pages = {843 -- 854}, year = {2014}, abstract = {A solar radio burst was observed in a coronal mass ejection/flare event by the Solar Broadband Radio Spectrometer at the Huairou Solar Observing Station on 2004 December 1. The data exhibited various patterns of plasma motions, suggestive of the interaction between sunward moving plasmoids and the flare loop system during the impulsive phase of the event. In addition to the radio data, the associated white-light, H alpha, extreme ultraviolet light, and soft and hard X-rays were also studied.}, language = {en} } @article{BeshnovaCherstvyVainshteinetal.2014, author = {Beshnova, Daria A. and Cherstvy, Andrey G. and Vainshtein, Yevhen and Teif, Vladimir B.}, title = {Regulation of the nucleosome repeat length in vivo by the DNA sequence, protein concentrations and long-range interactions}, series = {PLoS Computational Biology : a new community journal}, volume = {10}, journal = {PLoS Computational Biology : a new community journal}, number = {7}, publisher = {PLoS}, address = {San Fransisco}, issn = {1553-734X}, doi = {10.1371/journal.pcbi.1003698}, pages = {14}, year = {2014}, abstract = {The nucleosome repeat length (NRL) is an integral chromatin property important for its biological functions. Recent experiments revealed several conflicting trends of the NRL dependence on the concentrations of histones and other architectural chromatin proteins, both in vitro and in vivo, but a systematic theoretical description of NRL as a function of DNA sequence and epigenetic determinants is currently lacking. To address this problem, we have performed an integrative biophysical and bioinformatics analysis in species ranging from yeast to frog to mouse where NRL was studied as a function of various parameters. We show that in simple eukaryotes such as yeast, a lower limit for the NRL value exists, determined by internucleosome interactions and remodeler action. For higher eukaryotes, also the upper limit exists since NRL is an increasing but saturating function of the linker histone concentration. Counterintuitively, smaller H1 variants or non-histone architectural proteins can initiate larger effects on the NRL due to entropic reasons. Furthermore, we demonstrate that different regimes of the NRL dependence on histone concentrations exist depending on whether DNA sequence-specific effects dominate over boundary effects or vice versa. We consider several classes of genomic regions with apparently different regimes of the NRL variation. As one extreme, our analysis reveals that the period of oscillations of the nucleosome density around bound RNA polymerase coincides with the period of oscillations of positioning sites of the corresponding DNA sequence. At another extreme, we show that although mouse major satellite repeats intrinsically encode well-defined nucleosome preferences, they have no unique nucleosome arrangement and can undergo a switch between two distinct types of nucleosome positioning.}, language = {en} } @article{SchubertCollinsMangoldetal.2014, author = {Schubert, Marcel and Collins, Brian A. and Mangold, Hannah and Howard, Ian A. and Schindler, Wolfram and Vandewal, Koen and Roland, Steffen and Behrends, Jan and Kraffert, Felix and Steyrleuthner, Robert and Chen, Zhihua and Fostiropoulos, Konstantinos and Bittl, Robert and Salleo, Alberto and Facchetti, Antonio and Laquai, Frederic and Ade, Harald W. and Neher, Dieter}, title = {Correlated donor/acceptor crystal orientation controls photocurrent generation in all-polymer solar cells}, series = {Advanced functional materials}, volume = {24}, journal = {Advanced functional materials}, number = {26}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1616-301X}, doi = {10.1002/adfm.201304216}, pages = {4068 -- 4081}, year = {2014}, abstract = {New polymers with high electron mobilities have spurred research in organic solar cells using polymeric rather than fullerene acceptors due to their potential of increased diversity, stability, and scalability. However, all-polymer solar cells have struggled to keep up with the steadily increasing power conversion efficiency of polymer: fullerene cells. The lack of knowledge about the dominant recombination process as well as the missing concluding picture on the role of the semi-crystalline microstructure of conjugated polymers in the free charge carrier generation process impede a systematic optimization of all-polymer solar cells. These issues are examined by combining structural and photo-physical characterization on a series of poly(3-hexylthiophene) (donor) and P(NDI2OD-T2) (acceptor) blend devices. These experiments reveal that geminate recombination is the major loss channel for photo-excited charge carriers. Advanced X-ray and electron-based studies reveal the effect of chloronaphthalene co-solvent in reducing domain size, altering domain purity, and reorienting the acceptor polymer crystals to be coincident with those of the donor. This reorientation correlates well with the increased photocurrent from these devices. Thus, effi cient split-up of geminate pairs at polymer/polymer interfaces may necessitate correlated donor/acceptor crystal orientation, which represents an additional requirement compared to the isotropic fullerene acceptors.}, language = {en} } @article{KruglovKuznetsovPikovskij2014, author = {Kruglov, Vyacheslav P. and Kuznetsov, Sergey P. and Pikovskij, Arkadij}, title = {Attractor of Smale - Williams type in an autonomous distributed system}, series = {Regular and chaotic dynamics : international scientific journal}, volume = {19}, journal = {Regular and chaotic dynamics : international scientific journal}, number = {4}, publisher = {Pleiades Publ.}, address = {New York}, issn = {1560-3547}, doi = {10.1134/S1560354714040042}, pages = {483 -- 494}, year = {2014}, abstract = {We consider an autonomous system of partial differential equations for a one-dimensional distributed medium with periodic boundary conditions. Dynamics in time consists of alternating birth and death of patterns with spatial phases transformed from one stage of activity to another by the doubly expanding circle map. So, the attractor in the Poincar, section is uniformly hyperbolic, a kind of Smale - Williams solenoid. Finite-dimensional models are derived as ordinary differential equations for amplitudes of spatial Fourier modes (the 5D and 7D models). Correspondence of the reduced models to the original system is demonstrated numerically. Computational verification of the hyperbolicity criterion is performed for the reduced models: the distribution of angles of intersection for stable and unstable manifolds on the attractor is separated from zero, i.e., the touches are excluded. The example considered gives a partial justification for the old hopes that the chaotic behavior of autonomous distributed systems may be associated with uniformly hyperbolic attractors.}, language = {en} } @article{ZhaoDunlopQiuetal.2014, author = {Zhao, Qiang and Dunlop, John William Chapman and Qiu, Xunlin and Huang, Feihe and Zhang, Zibin and Heyda, Jan and Dzubiella, Joachim and Antonietti, Markus and Yuan, Jiayin}, title = {An instant multi-responsive porous polymer actuator driven by solvent molecule sorption}, series = {Nature Communications}, volume = {5}, journal = {Nature Communications}, publisher = {Nature Publ. Group}, address = {London}, issn = {2041-1723}, doi = {10.1038/ncomms5293}, pages = {8}, year = {2014}, abstract = {Fast actuation speed, large-shape deformation and robust responsiveness are critical to synthetic soft actuators. A simultaneous optimization of all these aspects without trade-offs remains unresolved. Here we describe porous polymer actuators that bend in response to acetone vapour (24 kPa, 20 degrees C) at a speed of an order of magnitude faster than the state-of-the-art, coupled with a large-scale locomotion. They are meanwhile multi-responsive towards a variety of organic vapours in both the dry and wet states, thus distinctive from the traditional gel actuation systems that become inactive when dried. The actuator is easy-to-make and survives even after hydrothermal processing (200 degrees C, 24 h) and pressing-pressure (100 MPa) treatments. In addition, the beneficial responsiveness is transferable, being able to turn 'inert' objects into actuators through surface coating. This advanced actuator arises from the unique combination of porous morphology, gradient structure and the interaction between solvent molecules and actuator materials.}, language = {en} } @article{ChengDingZhangetal.2014, author = {Cheng, X. and Ding, M. D. and Zhang, J. and Sun, X. D. and Guo, Y. and Wang, Yi-Ming and Kliem, Bernhard and Deng, Y. Y.}, title = {Formation of a double-decker magnetic flux rope in the sigmoidal solar active region 11520}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {789}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/789/2/93}, pages = {12}, year = {2014}, abstract = {In this paper, we address the formation of a magnetic flux rope (MFR) that erupted on 2012 July 12 and caused a strong geomagnetic storm event on July 15. Through analyzing the long-term evolution of the associated active region observed by the Atmospheric Imaging Assembly and the Helioseismic and Magnetic Imager on board the Solar Dynamics Observatory, it is found that the twisted field of an MFR, indicated by a continuous S-shaped sigmoid, is built up from two groups of sheared arcades near the main polarity inversion line a half day before the eruption. The temperature within the twisted field and sheared arcades is higher than that of the ambient volume, suggesting that magnetic reconnection most likely works there. The driver behind the reconnection is attributed to shearing and converging motions at magnetic footpoints with velocities in the range of 0.1-0.6 km s(-1). The rotation of the preceding sunspot also contributes to the MFR buildup. Extrapolated three-dimensional non-linear force-free field structures further reveal the locations of the reconnection to be in a bald-patch region and in a hyperbolic flux tube. About 2 hr before the eruption, indications of a second MFR in the form of an S-shaped hot channel are seen. It lies above the original MFR that continuously exists and includes a filament. The whole structure thus makes up a stable double-decker MFR system for hours prior to the eruption. Eventually, after entering the domain of instability, the high-lying MFR impulsively erupts to generate a fast coronal mass ejection and X-class flare; while the low-lying MFR remains behind and continuously maintains the sigmoidicity of the active region.}, language = {en} } @misc{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, Michael and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {HESS J1640-465 - an exceptionally luminous TeV gamma-ray supernova remnant (vol 439, pg 2828, 2014)}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, organization = {HESS Collaboration}, issn = {0035-8711}, doi = {10.1093/mnras/stu826}, pages = {3640 -- 3642}, year = {2014}, language = {en} } @article{TremelFischerKayunkidetal.2014, author = {Tremel, Kim and Fischer, Florian S. U. and Kayunkid, Navaphun and Di Pietro, Riccardo and Tkachov, Roman and Kiriy, Anton and Neher, Dieter and Ludwigs, Sabine and Brinkmann, Martin}, title = {Charge transport anisotropy in highly oriented thin films of the acceptor polymer P(NDI2OD-T2)}, series = {dvanced energy materials}, volume = {4}, journal = {dvanced energy materials}, number = {10}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1614-6832}, doi = {10.1002/aenm.201301659}, pages = {13}, year = {2014}, abstract = {The nanomorphology of the high mobility polymer poly{[N,N'-bis(2-octyldodecyl)-1,4,5,8-naphthalenedicarboximide-2,6-diyl]-alt-5,5'-(2,2'-bithiophene)} P(NDI2OD-T2) in thin films is explored as a function of different annealing conditions and correlated to optical and electrical properties. While nanofibrils with face-on orientation in form I are obtained directly after spin-coating and annealing below the melt transition temperature, clear evidence of lamellar structures is found after melt-annealing followed by slow cooling to room temperature. Interestingly these structural changes are accompanied by distinct changes in the absorption patterns. Electron diffraction measurements further show clear transitions towards predominant edge-on oriented chains in form II upon melt-annealing. Large-scale alignment with dichroic ratios up to 10 and improved order is achieved by high temperature rubbing and subsequent post-rubbing annealing. These highly oriented morphologies allow anisotropic in-plane charge transport to be probed with top-gate transistors parallel and perpendicular to the polymer chain direction. Mobilities up to 0.1 cm(2) V-1 s(-1) are observed parallel to the polymer chain, which is up to 10 times higher than those perpendicular to the polymer chain.}, language = {en} } @article{ProctorAlbrechtKuiketal.2014, author = {Proctor, Christopher M. and Albrecht, Steve and Kuik, Martijn and Neher, Dieter and Thuc-Quyen Nguyen,}, title = {Overcoming geminate recombination and enhancing extraction in solution-processed small molecule solar cells}, series = {dvanced energy materials}, volume = {4}, journal = {dvanced energy materials}, number = {10}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1614-6832}, doi = {10.1002/aenm.201400230}, pages = {7}, year = {2014}, language = {en} } @article{YadavalliKorolkovMoulinetal.2014, author = {Yadavalli, Nataraja Sekhar and Korolkov, Denis and Moulin, Jean-Francois and Krutyeva, Margarita and Santer, Svetlana}, title = {Probing opto-mechanical stresses within azobenzene-containing photosensitive polymer films by a thin metal film placed above}, series = {ACS applied materials \& interfaces}, volume = {6}, journal = {ACS applied materials \& interfaces}, number = {14}, publisher = {American Chemical Society}, address = {Washington}, issn = {1944-8244}, doi = {10.1021/am501870t}, pages = {11333 -- 11340}, year = {2014}, abstract = {Azo-modified photosensitive polymers offer the interesting possibility to reshape bulk polymers and thin films by UV-irradiation while being in the solid glassy state. The polymer undergoes considerable mass transport under irradiation with a light interference pattern resulting in the formation of surface relief grating (SRG). The forces inscribing this SRG pattern into a thin film are hard to assess experimentally directly. In the current study, we are proposing a method to probe opto-mechanical stresses within polymer films by characterizing the mechanical response of thin metal films (10 nm) deposited on the photosensitive polymer. During irradiation, the metal film not only deforms along with the SRG formation but ruptures in a regular and complex manner. The morphology of the cracks differs strongly depending on the electrical field distribution in the interference pattern, even when the magnitude and the kinetics of the strain are kept constant. This implies a complex local distribution of the opto-mechanical stress along the topography grating. In addition, the neutron reflectivity measurements of the metal/polymer interface indicate the penetration of a metal layer within the polymer, resulting in a formation of a bonding layer that confirms the transduction of light-induced stresses in the polymer layer to a metal film.}, language = {en} }