@article{ProctorAlbrechtKuiketal.2014, author = {Proctor, Christopher M. and Albrecht, Steve and Kuik, Martijn and Neher, Dieter and Thuc-Quyen Nguyen,}, title = {Overcoming geminate recombination and enhancing extraction in solution-processed small molecule solar cells}, series = {dvanced energy materials}, volume = {4}, journal = {dvanced energy materials}, number = {10}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1614-6832}, doi = {10.1002/aenm.201400230}, pages = {7}, year = {2014}, language = {en} } @misc{EschenlohrBattiatoMaldonadoetal.2014, author = {Eschenlohr, Andrea and Battiato, Mario and Maldonado, P. and Pontius, N. and Kachel, T. and Holldack, K. and Mitzner, Rolf and F{\"o}hlisch, Alexander and Oppeneer, P. M. and Stamm, Christian}, title = {Optical excitation of thin magnetic layers in multilayer structures Reply}, series = {Nature materials}, volume = {13}, journal = {Nature materials}, number = {2}, publisher = {Nature Publ. Group}, address = {London}, issn = {1476-1122}, doi = {10.1038/nmat3851}, pages = {102 -- 103}, year = {2014}, language = {en} } @phdthesis{Conrad2014, author = {Conrad, Claudia}, title = {Open cluster groups and complexes}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-77605}, school = {Universit{\"a}t Potsdam}, pages = {xii, 172}, year = {2014}, abstract = {It is generally agreed upon that stars typically form in open clusters and stellar associations, but little is known about the structure of the open cluster system. Do open clusters and stellar associations form isolated or do they prefer to form in groups and complexes? Open cluster groups and complexes could verify star forming regions to be larger than expected, which would explain the chemical homogeneity over large areas in the Galactic disk. They would also define an additional level in the hierarchy of star formation and could be used as tracers for the scales of fragmentation in giant molecular clouds? Furthermore, open cluster groups and complexes could affect Galactic dynamics and should be considered in investigations and simulations on the dynamical processes, such as radial migration, disc heating, differential rotation, kinematic resonances, and spiral structure. In the past decade there were a few studies on open cluster pairs (de La Fuente Marcos \& de La Fuente Marcos 2009a,b,c) and on open cluster groups and complexes (Piskunov et al. 2006). The former only considered spatial proximity for the identification of the pairs, while the latter also required tangential velocities to be similar for the members. In this work I used the full set of 6D phase-space information to draw a more detailed picture on these structures. For this purpose I utilised the most homogeneous cluster catalogue available, namely the Catalogue of Open Cluster Data (COCD; Kharchenko et al. 2005a,b), which contains parameters for 650 open clusters and compact associations, as well as for their uniformly selected members. Additional radial velocity (RV) and metallicity ([M/H]) information on the members were obtained from the RAdial Velocity Experiment (RAVE; Steinmetz et al. 2006; Kordopatis et al. 2013) for 110 and 81 clusters, respectively. The RAVE sample was cleaned considering quality parameters and flags provided by RAVE (Matijevič et al. 2012; Kordopatis et al. 2013). To ensure that only real members were included for the mean values, also the cluster membership, as provided by Kharchenko et al. (2005a,b), was considered for the stars cross-matched in RAVE. 6D phase-space information could be derived for 432 out of the 650 COCD objects and I used an adaption of the Friends-of-Friends algorithm, as used in cosmology, to identify potential groupings. The vast majority of the 19 identified groupings were pairs, but I also found four groups of 4-5 members and one complex with 15 members. For the verification of the identified structures, I compared the results to a randomly selected subsample of the catalogue for the Milky Way global survey of Star Clusters (MWSC; Kharchenko et al. 2013), which became available recently, and was used as reference sample. Furthermore, I implemented Monte-Carlo simulations with randomised samples created from two distinguished input distributions for the spatial and velocity parameters. On the one hand, assuming a uniform distribution in the Galactic disc and, on the other hand, assuming the COCD data distributions to be representative for the whole open cluster population. The results suggested that the majority of identified pairs are rather by chance alignments, but the groups and the complex seemed to be genuine. A comparison of my results to the pairs, groups and complexes proposed in the literature yielded a partial overlap, which was most likely because of selection effects and different parameters considered. This is another verification for the existence of such structures. The characteristics of the found groupings favour that members of an open cluster grouping originate from a common giant molecular cloud and formed in a single, but possibly sequential, star formation event. Moreover, the fact that the young open cluster population showed smaller spatial separations between nearest neighbours than the old cluster population indicated that the lifetime of open cluster groupings is most likely comparable to that of the Galactic open cluster population itself. Still even among the old open clusters I could identify groupings, which suggested that the detected structure could be in some cases more long lived as one might think. In this thesis I could only present a pilot study on structures in the Galactic open cluster population, since the data sample used was highly incomplete. For further investigations a far more complete sample would be required. One step in this direction would be to use data from large current surveys, like SDSS, RAVE, Gaia-ESO and VVV, as well as including results from studies on individual clusters. Later the sample can be completed by data from upcoming missions, like Gaia and 4MOST. Future studies using this more complete open cluster sample will reveal the effect of open cluster groupings on star formation theory and their significance for the kinematics, dynamics and evolution of the Milky Way, and thereby of spiral galaxies.}, language = {en} } @article{AlbrechtVandewalTumblestonetal.2014, author = {Albrecht, Steve and Vandewal, Koen and Tumbleston, John R. and Fischer, Florian S. U. and Douglas, Jessica D. and Frechet, Jean M. J. and Ludwigs, Sabine and Ade, Harald W. and Salleo, Alberto and Neher, Dieter}, title = {On the efficiency of charge transfer state splitting in polymer: Fullerene solar cells}, series = {Advanced materials}, volume = {26}, journal = {Advanced materials}, number = {16}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0935-9648}, doi = {10.1002/adma.201305283}, pages = {2533 -- 2539}, year = {2014}, language = {en} } @article{MkrtchianHenkel2014, author = {Mkrtchian, Vanik E. and Henkel, Carsten}, title = {On non-equilibrium photon distributions in the Casimir effect}, series = {Annalen der Physik}, volume = {526}, journal = {Annalen der Physik}, number = {1-2}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0003-3804}, doi = {10.1002/andp.201300135}, pages = {87 -- 101}, year = {2014}, abstract = {The electromagnetic field in a typical geometry of the Casimir effect is described in the Schwinger-Keldysh formalism. The main result is the photon distribution function (Keldysh Green function) in any stationary state of the field. A two-plate geometry with a sliding interface in local equilibrium is studied in detail, and full agreement with the results of Rytov fluctuation electrodynamics is found.}, language = {en} } @article{ReindlRauchWerneretal.2014, author = {Reindl, Nicole and Rauch, Thomas and Werner, Klaus and Kruk, J. W. and Todt, Helge Tobias}, title = {On helium-dominated stellar evolution: the mysterious role of the O(He)-type stars}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {566}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201423498}, pages = {23}, year = {2014}, abstract = {Context. About a quarter of all post-asymptotic giant branch (AGB) stars are hydrogen-deficient. Stellar evolutionary models explain the carbon-dominated H-deficient stars by a (very) late thermal pulse scenario where the hydrogen-rich envelope is mixed with the helium-rich intershell layer. Depending on the particular time at which the final flash occurs, the entire hydrogen envelope may be burned. In contrast, helium-dominated post-AGB stars and their evolution are not yet understood. Aims. A small group of very hot, helium-dominated stars is formed by O(He)-type stars. A precise analysis of their photospheric abundances will establish constraints to their evolution. Methods. We performed a detailed spectral analysis of ultraviolet and optical spectra of four O(He) stars by means of state-of-the-art non-LTE model-atmosphere techniques. Results. We determined effective temperatures, surface gravities, and the abundances of H, He, C, N, O, F, Ne, Si, P, S, Ar, and Fe. By deriving upper limits for the mass-loss rates of the O(He) stars, we found that they do not exhibit enhanced mass-loss. The comparison with evolutionary models shows that the status of the O(He) stars remains uncertain. Their abundances match predictions of a double helium white dwarf (WD) merger scenario, suggesting that they might be the progeny of the compact and of the luminous helium-rich sdO-type stars. The existence of planetary nebulae that do not show helium enrichment around every other O(He) star precludes a merger origin for these stars. These stars must have formed in a different way, for instance via enhanced mass-loss during their post-AGB evolution or a merger within a common-envelope (CE) of a CO-WD and a red giant or AGB star. Conclusions. A helium-dominated stellar evolutionary sequence exists that may be fed by different types of mergers or CE scenarios. It appears likely that all these pass through the O(He) phase just before they become WDs.}, language = {en} } @article{AliuAuneBeheraetal.2014, author = {Aliu, E. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Buckley, J. H. and Bugaev, V. and Cardenzana, J. V. and Cerruti, M. and Chen, X. and Ciupik, L. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kargaltsev, Oleg and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Lang, M. J. and Madhavan, A. S. and Maier, G. and Majumdar, P. and McCann, A. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Pandel, D. and Perkins, J. S. and Pohl, Manuela and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sembroski, G. H. and Skole, C. and Staszak, D. and Telezhinsky, Igor O. and Theiling, M. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vincent, S. and Wakely, S. P. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Williams, D. A. and Zitzer, B.}, title = {Observations of the unidentified gamm-ray source TeV J2032+4130 BY Veritas}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {783}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/783/1/16}, pages = {9}, year = {2014}, language = {en} } @article{DanehkarTodtErcolanoetal.2014, author = {Danehkar, A. and Todt, Helge Tobias and Ercolano, B. and Kniazev, A. Y.}, title = {Observations and three-dimensional photoionization modelling of the Wolf-Rayet planetary nebula Abell 48(star)}, series = {Monthly notices of the Royal Astronomical Society}, volume = {439}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu203}, pages = {3605 -- 3615}, year = {2014}, abstract = {Recent observations reveal that the central star of the planetary nebula Abell 48 exhibits spectral features similar to massive nitrogen-sequence Wolf-Rayet stars. This raises a pertinent question, whether it is still a planetary nebula or rather a ring nebula of a massive star. In this study, we have constructed a three-dimensional photoionization model of Abell 48, constrained by our new optical integral field spectroscopy. An analysis of the spatially resolved velocity distributions allowed us to constrain the geometry of Abell 48. We used the collisionally excited lines to obtain the nebular physical conditions and ionic abundances of nitrogen, oxygen, neon, sulphur and argon, relative to hydrogen. We also determined helium temperatures and ionic abundances of helium and carbon from the optical recombination lines. We obtained a good fit to the observations for most of the emission-line fluxes in our photoionization model. The ionic abundances deduced from our model are in decent agreement with those derived by the empirical analysis. However, we notice obvious discrepancies between helium temperatures derived from the model and the empirical analysis, as overestimated by our model. This could be due to the presence of a small fraction of cold metal-rich structures, which were not included in our model. It is found that the observed nebular line fluxes were best reproduced by using a hydrogen-deficient expanding model atmosphere as the ionizing source with an effective temperature of T-eff = 70 kK and a stellar luminosity of L-star = 5500 L-circle dot, which corresponds to a relatively low-mass progenitor star (similar to 3 M-circle dot) rather than a massive Pop I star.}, language = {en} } @article{AcciariArlenAuneetal.2014, author = {Acciari, V. A. and Arlen, T. and Aune, T. and Benbow, W. and Bird, R. and Bouvier, A. and Bradbury, S. M. and Buckley, J. H. and Bugaev, V. and de la Calle Perez, I. and Carter-Lewis, D. A. and Cesarini, A. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Falcone, A. and Federici, Simone and Fegan, D. J. and Fegan, S. J. and Finley, J. P. and Finnegan, G. and Fortson, L. and Gaidos, J. and Galante, N. and Gall, D. and Gibbs, K. and Gillanders, G. H. and Griffin, S. and Grube, J. and Gyuk, G. and Hanna, D. and Horan, D. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and McEnery, J. E. and Madhavan, A. S. and Moriarty, P. and Nelson, T. and Ong, R. A. and Orr, M. and Otte, A. N. and Perkins, J. S. and Petry, D. and Pichel, A. and Pohl, M. and Quinn, J. and Ragan, K. and Reynolds, T. and Roache, E. and Rovero, A. and Schroedter, M. and Sembroski, G. H. and Smith, A. and Telezhinsky, Igor O. and Theiling, M. and Toner, J. and Tyler, J. and Varlotta, A. and Vivier, M. and Wakely, S. P. and Ward, J. E. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Williams, D. A. and Wissel, S.}, title = {Observation of Markarian 421 in TeV gamma rays over a 14-year time span}, series = {Astroparticle physics}, volume = {54}, journal = {Astroparticle physics}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0927-6505}, doi = {10.1016/j.astropartphys.2013.10.004}, pages = {1 -- 10}, year = {2014}, abstract = {The variability of the blazar Markarian 421 in TeV gamma rays over a 14-year time period has been explored with the Whipple 10 m telescope. It is shown that the dynamic range of its flux variations is large and similar to that in X-rays. A correlation between the X-ray and TeV energy bands is observed during some bright flares and when the complete data sets are binned on long timescales. The main database consists of 878.4 h of observation with the Whipple telescope, spread over 783 nights. The peak energy response of the telescope was 400 GeV with 20\% uncertainty. This is the largest database of any TeV-emitting active galactic nucleus (AGN) and hence was used to explore the variability profile of Markarian 421. The tithe-averaged flux from Markarian 421 over this period was 0.446 +/- 0.008 Crab flux units. The flux exceeded 10 Crab flux units on three separate occasions. For the 2000-2001 season the average flux reached 1.86 Crab units, while in the 1996-1997 season the average flux was only 0.23 Crab units.}, language = {en} } @article{NezhadhaghighiChechkinMetzler2014, author = {Nezhadhaghighi, M. Ghasemi and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Numerical approach to unbiased and driven generalized elastic model}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {140}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {2}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.4858425}, pages = {9}, year = {2014}, abstract = {From scaling arguments and numerical simulations, we investigate the properties of the generalized elastic model (GEM) that is used to describe various physical systems such as polymers, membranes, single-file systems, or rough interfaces. We compare analytical and numerical results for the subdiffusion exponent beta characterizing the growth of the mean squared displacement <(delta h)(2)> of the field h described by the GEM dynamic equation. We study the scaling properties of the qth order moments with time, finding that the interface fluctuations show no intermittent behavior. We also investigate the ergodic properties of the process h in terms of the ergodicity breaking parameter and the distribution of the time averaged mean squared displacement. Finally, we study numerically the driven GEM with a constant, localized perturbation and extract the characteristics of the average drift for a tagged probe.}, language = {en} } @article{LepriPikovskij2014, author = {Lepri, Stefano and Pikovskij, Arkadij}, title = {Nonreciprocal wave scattering on nonlinear string-coupled oscillators}, series = {Chaos : an interdisciplinary journal of nonlinear science}, volume = {24}, journal = {Chaos : an interdisciplinary journal of nonlinear science}, number = {4}, publisher = {American Institute of Physics}, address = {Melville}, issn = {1054-1500}, doi = {10.1063/1.4899205}, pages = {9}, year = {2014}, abstract = {We study scattering of a periodic wave in a string on two lumped oscillators attached to it. The equations can be represented as a driven (by the incident wave) dissipative (due to radiation losses) system of delay differential equations of neutral type. Nonlinearity of oscillators makes the scattering non-reciprocal: The same wave is transmitted differently in two directions. Periodic regimes of scattering are analyzed approximately, using amplitude equation approach. We show that this setup can act as a nonreciprocal modulator via Hopf bifurcations of the steady solutions. Numerical simulations of the full system reveal nontrivial regimes of quasiperiodic and chaotic scattering. Moreover, a regime of a "chaotic diode," where transmission is periodic in one direction and chaotic in the opposite one, is reported. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{FoertigKniepertGlueckeretal.2014, author = {Foertig, Alexander and Kniepert, Juliane and Gluecker, Markus and Brenner, Thomas J. K. and Dyakonov, Vladimir and Neher, Dieter and Deibel, Carsten}, title = {Nongeminate and geminate recombination in PTB7: PCBM solar cells}, series = {Advanced functional materials}, volume = {24}, journal = {Advanced functional materials}, number = {9}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1616-301X}, doi = {10.1002/adfm.201302134}, pages = {1306 -- 1311}, year = {2014}, language = {en} } @article{CherstvyMetzler2014, author = {Cherstvy, Andrey G. and Metzler, Ralf}, title = {Nonergodicity, fluctuations, and criticality in heterogeneous diffusion processes}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {90}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {1}, publisher = {American Physical Society}, address = {College Park}, issn = {1539-3755}, doi = {10.1103/PhysRevE.90.012134}, pages = {11}, year = {2014}, abstract = {We study the stochastic behavior of heterogeneous diffusion processes with the power-law dependence D(x) similar to vertical bar x vertical bar(alpha) of the generalized diffusion coefficient encompassing sub- and superdiffusive anomalous diffusion. Based on statistical measures such as the amplitude scatter of the time-averaged mean-squared displacement of individual realizations, the ergodicity breaking and non-Gaussianity parameters, as well as the probability density function P(x, t), we analyze the weakly nonergodic character of the heterogeneous diffusion process and, particularly, the degree of irreproducibility of individual realizations. As we show, the fluctuations between individual realizations increase with growing modulus vertical bar alpha vertical bar of the scaling exponent. The fluctuations appear to diverge when the critical value alpha = 2 is approached, while for even larger alpha the fluctuations decrease, again. At criticality, the power-law behavior of the mean-squared displacement changes to an exponentially fast growth, and the fluctuations of the time-averaged mean-squared displacement do not converge for increasing number of realizations. From a systematic comparison we observe some striking similarities of the heterogeneous diffusion process with the familiar subdiffusive continuous time random walk process with power-law waiting time distribution and diverging characteristic waiting time.}, language = {en} } @phdthesis{Fischer2014, author = {Fischer, Jost Leonhardt}, title = {Nichtlineare Kopplungsmechanismen akustischer Oszillatoren am Beispiel der Synchronisation von Orgelpfeifen}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-71975}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {In dieser Arbeit werden nichtlineare Kopplungsmechanismen von akustischen Oszillatoren untersucht, die zu Synchronisation f{\"u}hren k{\"o}nnen. Aufbauend auf die Fragestellungen vorangegangener Arbeiten werden mit Hilfe theoretischer und experimenteller Studien sowie mit Hilfe numerischer Simulationen die Elemente der Tonentstehung in der Orgelpfeife und die Mechanismen der gegenseitigen Wechselwirkung von Orgelpfeifen identifiziert. Daraus wird erstmalig ein vollst{\"a}ndig auf den aeroakustischen und fluiddynamischen Grundprinzipien basierendes nichtlinear gekoppeltes Modell selbst-erregter Oszillatoren f{\"u}r die Beschreibung des Verhaltens zweier wechselwirkender Orgelpfeifen entwickelt. Die durchgef{\"u}hrten Modellrechnungen werden mit den experimentellen Befunden verglichen. Es zeigt sich, dass die Tonentstehung und die Kopplungsmechanismen von Orgelpfeifen durch das entwickelte Oszillatormodell in weiten Teilen richtig beschrieben werden. Insbesondere kann damit die Ursache f{\"u}r den nichtlinearen Zusammenhang von Kopplungsst{\"a}rke und Synchronisation des gekoppelten Zwei-Pfeifen Systems, welcher sich in einem nichtlinearen Verlauf der Arnoldzunge darstellt, gekl{\"a}rt werden. Mit den gewonnenen Erkenntnissen wird der Einfluss des Raumes auf die Tonentstehung bei Orgelpfeifen betrachtet. Daf{\"u}r werden numerische Simulationen der Wechselwirkung einer Orgelpfeife mit verschiedenen Raumgeometrien, wie z. B. ebene, konvexe, konkave, und gezahnte Geometrien, exemplarisch untersucht. Auch der Einfluss von Schwellk{\"a}sten auf die Tonentstehung und die Klangbildung der Orgelpfeife wird studiert. In weiteren, neuartigen Synchronisationsexperimenten mit identisch gestimmten Orgelpfeifen, sowie mit Mixturen wird die Synchronisation f{\"u}r verschiedene, horizontale und vertikale Pfeifenabst{\"a}nde in der Ebene der Schallabstrahlung, untersucht. Die dabei erstmalig beobachteten r{\"a}umlich isotropen Unstetigkeiten im Schwingungsverhalten der gekoppelten Pfeifensysteme, deuten auf abstandsabh{\"a}ngige Wechsel zwischen gegen- und gleichphasigen Sychronisationsregimen hin. Abschließend wird die M{\"o}glichkeit dokumentiert, das Ph{\"a}nomen der Synchronisation zweier Orgelpfeifen durch numerische Simulationen, also der Behandlung der kompressiblen Navier-Stokes Gleichungen mit entsprechenden Rand- und Anfangsbedingungen, realit{\"a}tsnah abzubilden. Auch dies stellt ein Novum dar.}, language = {de} } @article{ZinkWernerJechowetal.2014, author = {Zink, Christof and Werner, Nils and Jechow, Andreas and Heuer, Axel and Menzel, Ralf}, title = {Multi-wavelength operation of a single broad area diode laser by spectral beam combining}, series = {IEEE photonics technology letters}, volume = {26}, journal = {IEEE photonics technology letters}, number = {3}, publisher = {Inst. of Electr. and Electronics Engineers}, address = {Piscataway}, issn = {1041-1135}, doi = {10.1109/LPT.2013.2291963}, pages = {253 -- 256}, year = {2014}, abstract = {Stabilized multi-wavelength emission from a single emitter broad area diode laser (BAL) is realized by utilizing an external cavity with a spectral beam combining architecture. Self-organized emitters that are equidistantly spaced across the slow axis are enforced by the spatially distributed wavelength selectivity of the external cavity. This resulted in an array like near-field emission although the BAL is physically a single emitter without any epitaxial sub-structuring and only one electrical contact. Each of the self-organized emitters is operated at a different wavelength and the emission is multiplexed into one spatial mode with near-diffraction limited beam quality. With this setup, multi-line emission of 31 individual spectral lines centered around and a total spectral width of 3.6 nm is realized with a 1000 mu m wide BAL just above threshold. To the best of our knowledge, this is the first demonstration of such a self-organization of emitters by optical feedback utilizing a spectral beam combining architecture.}, language = {en} } @article{KustererNagelHartmannetal.2014, author = {Kusterer, D. -J. and Nagel, T. and Hartmann, S. and Werner, K. and Feldmeier, Achim}, title = {Monte Carlo radiation transfer in CV disk winds: application to the AM CVn prototype}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {561}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201321438}, pages = {10}, year = {2014}, abstract = {Context. AMCVn systems are ultracompact binaries in which a (semi-) degenerate star transfers helium-dominated matter onto a white dwarf. They are effective gravitational-wave emitters and potential progenitors of Type Ia supernovae. Aims. To understand the evolution of AMCVn systems it is necessary to determine their mass-loss rate through their radiation-driven accretion-disk wind. We constructed models to perform quantitative spectroscopy of P Cygni line profiles that were detected in UV spectra. Methods. We performed 2.5D Monte Carlo radiative transfer calculations in hydrodynamic wind structures by making use of realistic NLTE spectra from the accretion disk and by accounting for the white dwarf as an additional photon source. Results. We present first results from calculations in which LTE opacities are used in the wind model. A comparison with UV spectroscopy of the AMCVn prototype shows that the modeling procedure is potentially a good tool for determining mass-loss rates and abundances of trace metals in the helium-rich wind.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {31}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c4cp01234h}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, number = {16}, publisher = {the Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @misc{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor A. and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {Molecular motors pulling cargos in the viscoelastic cytosol: how power strokes beat subdiffusion}, series = {Physical Chemistry Chemical Physics}, journal = {Physical Chemistry Chemical Physics}, publisher = {The Royal Society of Chemistry}, address = {Cambridge}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76478}, pages = {16524 -- 16535}, year = {2014}, abstract = {The discovery of anomalous diffusion of larger biopolymers and submicron tracers such as endogenous granules, organelles, or virus capsids in living cells, attributed to the viscoelastic nature of the cytoplasm, provokes the question whether this complex environment equally impacts the active intracellular transport of submicron cargos by molecular motors such as kinesins: does the passive anomalous diffusion of free cargo always imply its anomalously slow active transport by motors, the mean transport distance along microtubule growing sublinearly rather than linearly in time? Here we analyze this question within the widely used two-state Brownian ratchet model of kinesin motors based on the continuous-state diffusion along microtubules driven by a flashing binding potential, where the cargo particle is elastically attached to the motor. Depending on the cargo size, the loading force, the amplitude of the binding potential, the turnover frequency of the molecular motor enzyme, and the linker stiffness we demonstrate that the motor transport may turn out either normal or anomalous, as indeed measured experimentally. We show how a highly efficient normal active transport mediated by motors may emerge despite the passive anomalous diffusion of the cargo, and study the intricate effects of the elastic linker. Under different, well specified conditions the microtubule-based motor transport becomes anomalously slow and thus significantly less efficient.}, language = {en} } @article{CherstvyPetrov2014, author = {Cherstvy, Andrey G. and Petrov, Eugene P.}, title = {Modeling DNA condensation on freestanding cationic lipid membranes}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {5}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c3cp53433b}, pages = {2020 -- 2037}, year = {2014}, abstract = {Motivated by recent experimental observations of a rapid spontaneous DNA coil-globule transition on freestanding cationic lipid bilayers, we propose simple theoretical models for DNA condensation on cationic lipid membranes. First, for a single DNA rod, we examine the conditions of full wrapping of a cylindrical DNA-like semi-flexible polyelectrolyte by an oppositely charged membrane. Then, for two parallel DNA rods, we self-consistently analyze the shape and the extent of the membrane enveloping them, focusing on membrane elastic deformations and the membrane-DNA embracing angle, which enables us to compute the membrane-mediated DNA-DNA interactions. We examine the effects of the membrane composition and its charge density, which are the experimentally tunable parameters. We show that membrane-driven rod-rod attraction is more pronounced for higher charge densities and for smaller surface tensions of the membrane. Thus, we demonstrate that for a long DNA chain adhered to a cationic lipid membrane, such membrane-induced DNA-DNA attraction can trigger compaction of DNA.}, language = {en} } @article{LiAbrechtYangetal.2014, author = {Li, Wentao and Abrecht, Steve and Yang, Liqiang and Roland, Steffen and Tumbleston, John R. and McAfee, Terry and Yan, Liang and Kelly, Mary Allison and Ade, Harald W. and Neher, Dieter and You, Wei}, title = {Mobility-controlled performance of thick solar cells based on fluorinated copolymers}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {44}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja5067724}, pages = {15566 -- 15576}, year = {2014}, abstract = {Developing novel materials and device architectures to further enhance the efficiency of polymer solar cells requires a fundamental understanding of the impact of chemical structures on photovoltaic properties. Given that device characteristics depend on many parameters, deriving structureproperty relationships has been very challenging. Here we report that a single parameter, hole mobility, determines the fill factor of several hundred nanometer thick bulk heterojunction photovoltaic devices based on a series of copolymers with varying amount of fluorine substitution. We attribute the steady increase of hole mobility with fluorine content to changes in polymer molecular ordering. Importantly, all other parameters, including the efficiency of free charge generation and the coefficient of nongeminate recombination, are nearly identical. Our work emphasizes the need to achieve high mobility in combination with strongly suppressed charge recombination for the thick devices required by mass production technologies.}, language = {en} } @article{ShinCherstvyMetzler2014, author = {Shin, Jaeoh and Cherstvy, Andrey G. and Metzler, Ralf}, title = {Mixing and segregation of ring polymers: spatial confinement and molecular crowding effects}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/5/053047}, pages = {19}, year = {2014}, abstract = {During the life cycle of bacterial cells the non-mixing of the two ring-shaped daughter genomes is an important prerequisite for the cell division process. Mimicking the environments inside highly crowded biological cells, we study the dynamics and statistical behavior of two flexible ring polymers in the presence of cylindrical confinement and crowding molecules. From extensive computer simulations we determine the degree of ring-ring overlap and the number of inter-monomer contacts for varying volume fractions phi of crowders. We also examine the entropic demixing of polymer rings in the presence of mobile crowders and determine the characteristic times of the internal polymer dynamics. Effects of the ring length on ring-ring overlap are also analyzed. In particular, on systematic variation of the fraction of crowding molecules, a (1 - phi)-scaling is found for the ring-ring overlap length along the cylinder axis, and a non-monotonic dependence of the 3D ring-ring contact number with a maximum at phi approximate to 0.2 is obtained. Our results demonstrate that polymer rings are demixed and separated by particular entropy-favourable partitioning of crowders along the axis of the cylindrical simulation box. These findings help to rationalize the implications of macromolecular crowding for circular DNA molecules in confined spaces inside bacteria as well as in localized cellular compartments inside eukaryotic cells.}, language = {en} } @article{EhlertLevermann2014, author = {Ehlert, D. and Levermann, Anders}, title = {Mechanism for potential strengthening of Atlantic overturning prior to collapse}, series = {Earth system dynamics}, volume = {5}, journal = {Earth system dynamics}, number = {2}, publisher = {Copernicus}, address = {G{\"o}ttingen}, issn = {2190-4979}, doi = {10.5194/esd-5-383-2014}, pages = {383 -- 397}, year = {2014}, abstract = {The Atlantic meridional overturning circulation (AMOC) carries large amounts of heat into the North Atlantic influencing climate regionally as well as globally. Palaeo-records and simulations with comprehensive climate models suggest that the positive salt-advection feedback may yield a threshold behaviour of the system. That is to say that beyond a certain amount of freshwater flux into the North Atlantic, no meridional overturning circulation can be sustained. Concepts of monitoring the AMOC and identifying its vicinity to the threshold rely on the fact that the volume flux defining the AMOC will be reduced when approaching the threshold. Here we advance conceptual models that have been used in a paradigmatic way to understand the AMOC, by introducing a density-dependent parameterization for the Southern Ocean eddies. This additional degree of freedom uncovers a mechanism by which the AMOC can increase with additional freshwater flux into the North Atlantic, before it reaches the threshold and collapses: an AMOC that is mainly wind-driven will have a constant upwelling as long as the Southern Ocean winds do not change significantly. The downward transport of tracers occurs either in the northern sinking regions or through Southern Ocean eddies. If freshwater is transported, either atmospherically or via horizontal gyres, from the low to high latitudes, this would reduce the eddy transport and by continuity increase the northern sinking which defines the AMOC until a threshold is reached at which the AMOC cannot be sustained. If dominant in the real ocean this mechanism would have significant consequences for monitoring the AMOC.}, language = {en} } @article{PapkeYadavalliHenkeletal.2014, author = {Papke, Thomas and Yadavalli, Nataraja Sekhar and Henkel, Carsten and Santer, Svetlana}, title = {Mapping a plasmonic hologram with photosensitive polymer films: standing versus propagating waves}, series = {ACS applied materials \& interfaces}, volume = {6}, journal = {ACS applied materials \& interfaces}, number = {16}, publisher = {American Chemical Society}, address = {Washington}, issn = {1944-8244}, doi = {10.1021/am503501y}, pages = {14174 -- 14180}, year = {2014}, abstract = {We use a photosensitive layer containing azobenzene moieties to map near-field intensity patterns in the vicinity of nanogrids fabricated within a thin silver layer. It is known that azobenzene containing films deform permanently during irradiation, following the pattern of the field intensity. The photosensitive material reacts only to stationary waves whose intensity patterns do not change in time. In this study, we have found a periodic deformation above the silver film outside the nanostructure, even if the latter consists of just one groove. This is in contradiction to the widely accepted viewpoint that propagating surface plasmon modes dominate outside nanogrids. We explain our observation based on an electromagnetic hologram formed by the constructive interference between a propagating surface plasmon wave and the incident light. This hologram contains a stationary intensity and polarization grating that even appears in the absence of the polymer layer.}, language = {en} } @article{ReibisVoellerGittetal.2014, author = {Reibis, Rona Katharina and V{\"o}ller, Heinz and Gitt, Anselm and Jannowitz, Christina and Halle, Martin and Pittrow, David and Hildemann, Steven}, title = {Management of patients with ST- segment elevation or non- ST- segment elevation acute coronary syndromes in cardiac rehabilitation centers}, series = {Clinical cardiology : international journal for cardiovascular diseases}, volume = {37}, journal = {Clinical cardiology : international journal for cardiovascular diseases}, number = {4}, publisher = {Wiley-Blackwell}, address = {Hoboken}, issn = {0160-9289}, doi = {10.1002/clc.22241}, pages = {213 -- 221}, year = {2014}, abstract = {BackgroundCurrent data on the management of patients in cardiac rehabilitation (CR) after an acute hospital stay due to ST-segment elevation or non-ST segment elevation acute coronary syndromes (STE-ACS or NSTE-ACS) are limited. We aimed to describe patient characteristics, risk factor management, and lipid target achievement of patients in CR in Germany and compare the 2 groups. HypothesisWith respect to the risk factor pattern and treatment effects during a CR stay, there are important differences between STE-ACS and NSTE-ACS patients. MethodsComparison of 7950 patients by STE-ACS or NSTE-ACS status in the Transparency Registry to Objectify Guideline-Oriented Risk Factor Management registry (2010) who underwent an inpatient CR period of about 3 weeks. ResultsSTE-ACS patients compared to NSTE-ACS patients were significantly younger (60.5 vs 64.4 years, P < 0.0001), and had diabetes mellitus, hypertension, or any risk factor (exception: smoking) less often. At discharge, in STE-ACS compared to NSTE-ACS patients, the low-density lipoprotein cholesterol (LDL-C) <100 mg/dL goal was achieved by 75.3\% and 76.2\%, respectively (LDL-C <70 mg/dL by 27.7\% and 27.4\%), the high-density lipoprotein cholesterol goal of >50 mg/dL in women and >40 mg/dL in men was achieved by 49.3\% and 49.0\%, respectively, and the triglycerides goal of <150 mg/dl was achievedby 72.3\% and 74.3\%, respectively (all comparisons not significant). Mean systolic and diastolic blood pressure were 121/74 and 123/74 mm Hg, respectively (P < 0.0001 systolic, diastolic not significant). The maximum exercise capacity was 110 and 102 W, respectively (P < 0.0001), and the maximum walking distance was 581 and 451 meters, respectively (P value not significant). ConclusionsPatients with STE-ACS and NSTE-ACS differed moderately in their baseline characteristics. Both groups benefited from the participation in CR, as their lipid profile, blood pressure, and physical fitness improved.}, language = {en} } @article{Levermann2014, author = {Levermann, Anders}, title = {Make supply chains climate-smart}, series = {Nature : the international weekly journal of science}, volume = {506}, journal = {Nature : the international weekly journal of science}, number = {7486}, publisher = {Nature Publ. Group}, address = {London}, issn = {0028-0836}, pages = {27 -- 29}, year = {2014}, language = {en} } @article{MizunoPohlNiemiecetal.2014, author = {Mizuno, Yosuke and Pohl, Martin and Niemiec, Jacek and Zhang, Bing and Nishikawa, Ken-Ichi and Hardee, Philip E.}, title = {Magnetic field amplification and saturation in turbulence behind a relativistic shock}, series = {Monthly notices of the Royal Astronomical Society}, volume = {439}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu196}, pages = {3490 -- 3503}, year = {2014}, abstract = {We have investigated via 2D relativistic magnetohydrodynamic simulations the long-term evolution of turbulence created by a relativistic shock propagating through an inhomogeneous medium. In the post-shock region, magnetic field is strongly amplified by turbulent motions triggered by pre-shock density inhomogeneities. Using a long-simulation box we have followed the magnetic field amplification until it is fully developed and saturated. The turbulent velocity is subrelativistic even for a strong shock. Magnetic field amplification is controlled by the turbulent motion and saturation occurs when the magnetic energy is comparable to the turbulent kinetic energy. Magnetic field amplification and saturation depend on the initial strength and direction of the magnetic field in the pre-shock medium, and on the shock strength. If the initial magnetic field is perpendicular to the shock normal, the magnetic field is first compressed at the shock and then can be amplified by turbulent motion in the post-shock region. Saturation occurs when the magnetic energy becomes comparable to the turbulent kinetic energy in the post-shock region. If the initial magnetic field in the pre-shock medium is strong, the post-shock region becomes turbulent but significant field amplification does not occur. If the magnetic energy after shock compression is larger than the turbulent kinetic energy in the post-shock region, significant field amplification does not occur. We discuss possible applications of our results to gamma-ray bursts and active galactic nuclei.}, language = {en} } @article{ChenChatterjeeZhangetal.2014, author = {Chen, Xuhui and Chatterjee, Ritaban and Zhang, Haocheng and Pohl, Martin and Fossati, Giovanni and Boettcher, Markus and Bailyn, Charles D. and Bonning, Erin W. and Buxton, Michelle and Coppi, Paolo and Isler, Jedidah and Maraschi, Laura and Urry, Meg}, title = {Magnetic field amplification and flat spectrum radio quasars}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu713}, pages = {2188 -- 2199}, year = {2014}, abstract = {We perform time-dependent, spatially resolved simulations of blazar emission to evaluate several flaring scenarios related to magnetic-field amplification and enhanced particle acceleration. The code explicitly accounts for light-travel-time effects and is applied to flares observed in the flat spectrum radio quasar (FSRQ) PKS 0208-512, which show optical/gamma-ray correlation at some times, but orphan optical flares at other times. Changes in both the magnetic field and the particle acceleration efficiency are explored as causes of flares. Generally, external Compton (EC) emission appears to describe the available data better than a synchrotron self-Compton (SSC) scenario, and in particular orphan optical flares are difficult to produce in the SSC framework. X-ray soft-excesses, gamma-ray spectral hardening, and the detections at very high energies of certain FSRQs during flares find natural explanations in the EC scenario with particle acceleration change. Likewise, optical flares with/without gamma-ray counterparts can be explained by different allocations of energy between the magnetization and particle acceleration, which may be related to the orientation of the magnetic field relative to the jet flow. We also calculate the degree of linear polarization and polarization angle as a function of time for a jet with helical magnetic field. Tightening of the magnetic helix immediately downstream of the jet perturbations, where flares occur, can be sufficient to explain the increases in the degree of polarization and a rotation by a parts per thousand yen180A degrees of the observed polarization angle, if light-travel-time effects are properly considered.}, language = {en} } @article{NishikawaHardeeDutanetal.2014, author = {Nishikawa, Ken-Ichi and Hardee, P. E. and Dutan, I. and Niemiec, J. and Medvedev, M. and Mizuno, Y. and Meli, A. and Sol, H. and Zhang, B. and Pohl, Martin and Hartmann, D. H.}, title = {Magnetic agnetic field generation in core-sheath jets via the kinetic Kelvin-Helmholtz instability}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {793}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/793/1/60}, pages = {16}, year = {2014}, abstract = {We have investigated magnetic field generation in velocity shears via the kinetic Kelvin-Helmholtz instability (kKHI) using a relativistic plasma jet core and stationary plasma sheath. Our three-dimensional particle-in-cell simulations consider plasma jet cores with Lorentz factors of 1.5, 5, and 15 for both electron-proton and electron-positron plasmas. For electron-proton plasmas, we find generation of strong large-scale DC currents and magnetic fields that extend over the entire shear surface and reach thicknesses of a few tens of electron skin depths. For electron-positron plasmas, we find generation of alternating currents and magnetic fields. Jet and sheath plasmas are accelerated across the shear surface in the strong magnetic fields generated by the kKHI. The mixing of jet and sheath plasmas generates a transverse structure similar to that produced by the Weibel instability.}, language = {en} } @article{ZhangZhangYouetal.2014, author = {Zhang, Xiaoqing and Zhang, Xinwu and You, Qiong and Sessler, Gerhard M.}, title = {Low- cost, large- area, stretchable piezoelectric films based on irradiation- crosslinked poly ( propylene)}, series = {Macromolecular materials and engineering}, volume = {299}, journal = {Macromolecular materials and engineering}, number = {3}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1438-7492}, doi = {10.1002/mame.201300161}, pages = {290 -- 295}, year = {2014}, abstract = {Low cost, large area, lightweight, stretchable piezoelectric films, based on space-charge electret with a foam structure (i.e., ferroelectrets or piezoelectrets), have been fabricated by using commercially available irradiation cross-linked poly(propylene) (IXPP) foam sheets. Piezoelectric d(33) coefficients are as high as 100pCN(-1). The piezoelectric performance in such IXPP films is well preserved for repeated strains of less than 10\%. Piezoelectric d(33) coefficients are frequency independent in the range from 2 to 100Hz. Such new class materials may be applied in sensory skins, smart clothing, bio-inspired systems, microenergy harvesters, and so on.}, language = {en} } @article{MarzeionLevermann2014, author = {Marzeion, Ben and Levermann, Anders}, title = {Loss of cultural world heritage and currently inhabited places to sea-level rise}, series = {Environmental research letters}, volume = {9}, journal = {Environmental research letters}, number = {3}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1748-9326}, doi = {10.1088/1748-9326/9/3/034001}, pages = {7}, year = {2014}, language = {en} } @article{AliuArchambaultAuneetal.2014, author = {Aliu, E. and Archambault, S. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Byrum, K. and Cerruti, M. and Chen, X. and Ciupik, L. and Connolly, M. P. and Cui, W. and Duke, C. and Dumm, J. and Errando, M. and Falcone, A. and Federici, S. and Feng, Q. and Finley, J. P. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Maier, G. and Majumdar, P. and McCann, A. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, M. and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Rousselle, J. and Sembroski, G. H. and Sheidaei, F. and Skole, C. and Smith, A. W. and Staszak, D. and Stroh, M. and Telezhinsky, Igor O. and Theiling, M. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vincent, S. and Wakely, S. P. and Weinstein, A. and Welsing, R. and Williams, D. A. and Zajczyk, A. and Zitzer, B. and Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Voelk, H. J. and Volpe, F. and Vorster, M. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Long-term TeV and X-RAY observations of the GAMMA- RAY binary hess J0632+057}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {780}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {VERITAS Collaboration, HESS Collaboration}, issn = {0004-637X}, doi = {10.1088/0004-637X/780/2/168}, pages = {14}, year = {2014}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and B{\"o}ttcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Forster, A. and Fuling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadsch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, Markus and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kiefeer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Kruger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puhlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schussler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and Van Eldik, C. and Van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Volk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Wornlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Long-term monitoring of PKS2155-304 with ATOM and HESS:investigation of optical/gamma-ray correlations in different spectral states}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {571}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, organization = {HESSS Collaboration}, issn = {0004-6361}, doi = {10.1051/0004-6361/201424142}, pages = {10}, year = {2014}, abstract = {In this paper we report on the analysis of all the available optical and very high-energy gamma-ray (> 200 GeV) data for the BL Lac object PKS 2155-304, collected simultaneously with the ATOM and H.E.S.S. telescopes from 2007 until 2009. This study also includes X-ray (RXTE, Swift) and high-energy gamma-ray (Fermi-LAT) data. During the period analysed, the source was transitioning from its flaring to quiescent optical states, and was characterized by only moderate flux changes at different wavelengths on the timescales of days and months. A flattening of the optical continuum with an increasing optical flux can be noted in the collected dataset, but only occasionally and only at higher flux levels. We did not find any universal relation between the very high-energy gamma-ray and optical flux changes on the timescales from days and weeks up to several years. On the other hand, we noted that at higher flux levels the source can follow two distinct tracks in the optical flux-colour diagrams, which seem to be related to distinct gamma-ray states of the blazar. The obtained results therefore indicate a complex scaling between the optical and gamma-ray emission of PKS 2155 304, with different correlation patterns holding at different epochs, and a gamma-ray flux depending on the combination of an optical flux and colour rather than a flux alone.}, language = {en} } @article{SchickHerzogWenetal.2014, author = {Schick, Daniel and Herzog, Marc and Wen, Haidan and Chen, Pice and Adamo, Carolina and Gaal, Peter and Schlom, Darrell G. and Evans, Paul G. and Li, Yuelin and Bargheer, Matias}, title = {Localized excited charge carriers generate ultrafast inhomogeneous strain in the multiferroic BiFeO3}, series = {Physical review letters}, volume = {112}, journal = {Physical review letters}, number = {9}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.112.097602}, pages = {6}, year = {2014}, abstract = {We apply ultrafast x-ray diffraction with femtosecond temporal resolution to monitor the lattice dynamics in a thin film of multiferroic BiFeO3 after above-band-gap photoexcitation. The sound-velocity limited evolution of the observed lattice strains indicates a quasi-instantaneous photoinduced stress which decays on a nanosecond time scale. This stress exhibits an inhomogeneous spatial profile evidenced by the broadening of the Bragg peak. These new data require substantial modification of existing models of photogenerated stresses in BiFeO3: the relevant excited charge carriers must remain localized to be consistent with the data.}, language = {en} } @article{GodecChechkinBarkaietal.2014, author = {Godec, Aljaz and Chechkin, Aleksei V. and Barkai, Eli and Kantz, Holger and Metzler, Ralf}, title = {Localisation and universal fluctuations in ultraslow diffusion processes}, series = {Journal of physics : A, Mathematical and theoretical}, volume = {47}, journal = {Journal of physics : A, Mathematical and theoretical}, number = {49}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1751-8113}, doi = {10.1088/1751-8113/47/49/492002}, pages = {10}, year = {2014}, abstract = {We study ultraslow diffusion processes with logarithmic mean squared displacement (MSD) < x(2)(t)> similar or equal to log(gamma)t. Comparison of annealed (renewal) continuous time random walks (CTRWs) with logarithmic waiting time distribution psi(tau) similar or equal to 1/(tau log(1+gamma)tau) and Sinai diffusion in quenched random landscapes reveals striking similarities, despite the great differences in their physical nature. In particular, they exhibit a weakly non-ergodic disparity of the time-averaged and ensemble-averaged MSDs. Remarkably, for the CTRW we observe that the fluctuations of time averages become universal, with an exponential suppression of mobile trajectories. We discuss the fundamental connection between the Golosov localization effect and non-ergodicity in the sense of the disparity between ensemble-averaged MSD and time-averaged MSD.}, language = {en} } @article{XuBrennerChabanneetal.2014, author = {Xu, Jingsan and Brenner, Thomas J. K. and Chabanne, Laurent and Neher, Dieter and Antonietti, Markus and Shalom, Menny}, title = {Liquid-Based growth of polymeric carbon nitride layers and their use in a mesostructured polymer solar cell with V-oc exceeding 1 V}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {39}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja508329c}, pages = {13486 -- 13489}, year = {2014}, abstract = {Herein we report a general liquid-mediated pathway for the growth of continuous polymeric carbon nitride (C3N4) thin films. The deposition method consists of the use of supramolecular complexes that transform to the liquid state before direct thermal condensation into C3N4 solid films. The resulting films exhibit continuous porous C3N4 networks on various substrates. Moreover, the optical absorption can be easily tuned to cover the solar spectrum by the insertion of an additional molecule into the starting complex. The strength of the deposition method is demonstrated by the use of the C3N4 layer as the electron acceptor in a polymer solar cell that exhibits a remarkable open-circuit voltage exceeding 1 V. The easy, safe, and direct synthesis of carbon nitride in a continuous layered architecture on different functional substrates opens new possibilities for the fabrication of many energy-related devices.}, language = {en} } @article{Goychuk2014, author = {Goychuk, Igor}, title = {Life and death of stationary linear response in anomalous continuous time random walk dynamics}, series = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, volume = {62}, journal = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, number = {4}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0253-6102}, pages = {497 -- 504}, year = {2014}, abstract = {Linear theory of stationary response in systems at thermal equilibrium requires to find equilibrium correlation function of unperturbed responding system. Studies of the response of the systems exhibiting anomalously slow dynamics are often based on the continuous time random walk description (CTRW) with divergent mean waiting times. The bulk of the literature on anomalous response contains linear response functions like one by Cole-Cole calculated from such a CTRW theory and applied to systems at thermal equilibrium. Here we show within a fairly simple and general model that for the systems with divergent mean waiting times the stationary response at thermal equilibrium is absent, in accordance with some recent studies. The absence of such stationary response (or dying to zero non-stationary response in aging experiments) would confirm CTRW with divergent mean waiting times as underlying physical relaxation mechanism, but reject it otherwise. We show that the absence of stationary response is closely related to the breaking of ergodicity of the corresponding dynamical variable. As an important new result, we derive a generalized Cole-Cole response within ergodic CTRW dynamics with finite waiting time. Moreover, we provide a physically reasonable explanation of the origin and wide presence of 1/f noise in condensed matter for ergodic dynamics close to normal, rather than strongly deviating.}, language = {en} } @article{PalyulinChechkinMetzler2014, author = {Palyulin, Vladimir V. and Chechkin, Aleksei V. and Metzler, Ralf}, title = {Levy flights do not always optimize random blind search for sparse targets}, series = {Proceedings of the National Academy of Sciences of the United States of America}, volume = {111}, journal = {Proceedings of the National Academy of Sciences of the United States of America}, number = {8}, publisher = {National Acad. of Sciences}, address = {Washington}, issn = {0027-8424}, doi = {10.1073/pnas.1320424111}, pages = {2931 -- 2936}, year = {2014}, abstract = {It is generally believed that random search processes based on scale-free, Levy stable jump length distributions (Levy flights) optimize the search for sparse targets. Here we show that this popular search advantage is less universal than commonly assumed. We study the efficiency of a minimalist search model based on Levy flights in the absence and presence of an external drift (underwater current, atmospheric wind, a preference of the walker owing to prior experience, or a general bias in an abstract search space) based on two different optimization criteria with respect to minimal search time and search reliability (cumulative arrival probability). Although Levy flights turn out to be efficient search processes when the target is far from the starting point, or when relative to the starting point the target is upstream, we show that for close targets and for downstream target positioning regular Brownian motion turns out to be the advantageous search strategy. Contrary to claims that Levy flights with a critical exponent alpha = 1 are optimal for the search of sparse targets in different settings, based on our optimization parameters the optimal a may range in the entire interval (1, 2) and especially include Brownian motion as the overall most efficient search strategy.}, language = {en} } @phdthesis{Steyrleuthner2014, author = {Steyrleuthner, Robert}, title = {Korrelation von Struktur, optischen Eigenschaften und Ladungstransport in einem konjugierten Naphthalindiimid-Bithiophen Copolymer mit herausragender Elektronenmobilit{\"a}t}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-71413}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {Organische Halbleiter besitzen neue, bemerkenswerte Materialeigenschaften, die sie f{\"u}r die grundlegende Forschung wie auch aktuelle technologische Entwicklung (bsw. org. Leuchtdioden, org. Solarzellen) interessant werden lassen. Aufgrund der starken konformative Freiheit der konjugierten Polymerketten f{\"u}hrt die Vielzahl der m{\"o}glichen Anordnungen und die schwache intermolekulare Wechselwirkung f{\"u}r gew{\"o}hnlich zu geringer struktureller Ordnung im Festk{\"o}rper. Die Morphologie hat gleichzeitig direkten Einfluss auf die elektronische Struktur der organischen Halbleiter, welches sich meistens in einer deutlichen Reduktion der Ladungstr{\"a}gerbeweglichkeit gegen{\"u}ber den anorganischen Verwandten zeigt. So stellt die Beweglichkeit der Ladungen im Halbleiter einen der limitierenden Faktoren f{\"u}r die Leistungsf{\"a}higkeit bzw. den Wirkungsgrad von funktionellen organischen Bauteilen dar. Im Jahr 2009 wurde ein neues auf Naphthalindiimid und Bithiophen basierendes Dornor/Akzeptor Copolymer vorgestellt [P(NDI2OD‑T2)], welches sich durch seine außergew{\"o}hnlich hohe Ladungstr{\"a}germobilit{\"a}t auszeichnet. In dieser Arbeit wird die Ladungstr{\"a}germobilit{\"a}t in P(NDI2OD‑T2) bestimmt, und der Transport durch eine geringe energetischer Unordnung charakterisiert. Obwohl dieses Material zun{\"a}chst als amorph beschrieben wurde zeigt eine detaillierte Analyse der optischen Eigenschaften von P(NDI2OD‑T2), dass bereits in L{\"o}sung geordnete Vorstufen supramolekularer Strukturen (Aggregate) existieren. Quantenchemische Berechnungen belegen die beobachteten spektralen {\"A}nderungen. Mithilfe der NMR-Spektroskopie kann die Bildung der Aggregate unabh{\"a}ngig von optischer Spektroskopie best{\"a}tigt werden. Die Analytische Ultrazentrifugation an P(NDI2OD‑T2) L{\"o}sungen legt nahe, dass sich die Aggregation innerhalb der einzelnen Ketten unter Reduktion des hydrodynamischen Radius vollzieht. Die Ausbildung supramolekularen Strukturen nimmt auch eine signifikante Rolle bei der Filmbildung ein und verhindert gleichzeitig die Herstellung amorpher P(NDI2OD‑T2) Filme. Durch chemische Modifikation der P(NDI2OD‑T2)-Kette und verschiedener Prozessierungs-Methoden wurde eine {\"A}nderung des Kristallinit{\"a}tsgrades und gleichzeitig der Orientierung der kristallinen Dom{\"a}nen erreicht und mittels R{\"o}ntgenbeugung quantifiziert. In hochaufl{\"o}senden Elektronenmikroskopie-Messungen werden die Netzebenen und deren Einbettung in die semikristallinen Strukturen direkt abgebildet. Aus der Kombination der verschiedenen Methoden erschließt sich ein Gesamtbild der Nah- und Fernordnung in P(NDI2OD‑T2). {\"U}ber die Messung der Elektronenmobilit{\"a}t dieser Schichten wird die Anisotropie des Ladungstransports in den kristallographischen Raumrichtungen von P(NDI2OD‑T2) charakterisiert und die Bedeutung der intramolekularen Wechselwirkung f{\"u}r effizienten Ladungstransport herausgearbeitet. Gleichzeitig wird deutlich, wie die Verwendung von gr{\"o}ßeren und planaren funktionellen Gruppen zu h{\"o}heren Ladungstr{\"a}germobilit{\"a}ten f{\"u}hrt, welche im Vergleich zu klassischen semikristallinen Polymeren weniger sensitiv auf die strukturelle Unordnung im Film sind.}, language = {de} } @article{AliuArchambaultAuneetal.2014, author = {Aliu, E. and Archambault, S. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Buckley, J. H. and Bugaev, V. and Cardenzana, J. V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dumm, J. and Dwarkadas, Vikram V. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gall, D. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krennrich, F. and Kumar, S. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McCann, A. J. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Pandel, D. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Ratliff, G. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Rousselle, J. and Sembroski, G. H. and Shahinyan, K. and Sheidaei, F. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Tsurusaki, K. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Ward, J. E. and Weinstein, A. and Welsing, R. and Wilhelm, Alina}, title = {Investigating the TeV morpholoy of MGRO J1908+06 with veritas}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {787}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/787/2/166}, pages = {7}, year = {2014}, abstract = {We report on deep observations of the extended TeV gamma-ray source MGRO J1908+06 made with the VERITAS very high energy gamma-ray observatory. Previously, the TeV emission has been attributed to the pulsar wind nebula (PWN) of the Fermi-LAT pulsar PSR J1907+0602. We detect MGRO J1908+06 at a significance level of 14 standard deviations (14 sigma) and measure a photon index of 2.20 +/- 0.10(stat) +/- 0.20(sys). The TeV emission is extended, covering the region near PSR J1907+0602 and also extending toward SNR G40.5-0.5. When fitted with a two-dimensional Gaussian, the intrinsic extension has a standard deviation of sigma(src) = 0 degrees.44 +/- 0 degrees.02. In contrast to other TeV PWNe of similar age in which the TeV spectrum softens with distance from the pulsar, the TeV spectrum measured near the pulsar location is consistent with that measured at a position near the rim of G40.5-0.5, 0 degrees.33 away.}, language = {en} } @article{AliuArchambaultArlenetal.2014, author = {Aliu, E. and Archambault, S. and Arlen, T. and Aune, T. and Barnacka, Anna and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Bouvier, A. and Buckley, J. H. and Bugaev, V. and Cerruti, M. and Chen, X. and Ciupik, L. and Collins-Hughes, E. and Connolly, M. P. and Cui, W. and Dumm, J. and Eisch, J. D. and Falcone, A. and Federici, S. and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hakansson, N. and Hanna, D. and Holder, J. and Hughes, G. and Hughes, Z. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kar, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Majumdar, P. and McArthur, S. and McCann, A. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nelson, T. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Perkins, J. S. and Pohl, M. and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sadun, A. and Santander, M. and Sembroski, G. H. and Shahinyan, K. and Sheidaei, F. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Theiling, M. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weekes, T. C. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B. and Boettcher, Markus and Fumagalli, M.}, title = {Investigating broadband variability of the TeV blazar 1ES 1959+650}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {797}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {Veritas Collaboration}, issn = {0004-637X}, doi = {10.1088/0004-637X/797/2/89}, pages = {11}, year = {2014}, abstract = {We summarize broadband observations of the TeV-emitting blazar 1ES 1959+650, including optical R-band observations by the robotic telescopes Super-LOTIS and iTelescope, UV observations by Swift Ultraviolet and Optical Telescope, X-ray observations by the Swift X-ray Telescope, high-energy gamma-ray observations with the Fermi Large Area Telescope, and very-high-energy (VHE) gamma-ray observations by VERITAS above 315 GeV, all taken between 2012 April 17 and 2012 June 1 (MJD 56034 and 56079). The contemporaneous variability of the broadband spectral energy distribution is explored in the context of a simple synchrotron self Compton (SSC) model. In the SSC emission scenario, we find that the parameters required to represent the high state are significantly different than those in the low state. Motivated by possible evidence of gas in the vicinity of the blazar, we also investigate a reflected emission model to describe the observed variability pattern. This model assumes that the non-thermal emission from the jet is reflected by a nearby cloud of gas, allowing the reflected emission to re-enter the blob and produce an elevated gamma-ray state with no simultaneous elevated synchrotron flux. The model applied here, although not required to explain the observed variability pattern, represents one possible scenario which can describe the observations. As applied to an elevated VHE state of 66\% of the Crab Nebula flux, observed on a single night during the observation period, the reflected emission scenario does not support a purely leptonic non-thermal emission mechanism. The reflected emission model does, however, predict a reflected photon field with sufficient energy to enable elevated gamma-ray emission via pion production with protons of energies between 10 and 100 TeV.}, language = {en} } @article{PradhanAlbrechtStilleretal.2014, author = {Pradhan, Basudev and Albrecht, Steve and Stiller, Burkhard and Neher, Dieter}, title = {Inverted organic solar cells comprising low-temperature-processed ZnO films}, series = {Applied physics : A, Materials science \& processing}, volume = {115}, journal = {Applied physics : A, Materials science \& processing}, number = {2}, publisher = {Springer}, address = {New York}, issn = {0947-8396}, doi = {10.1007/s00339-014-8373-8}, pages = {365 -- 369}, year = {2014}, abstract = {Inverted organic solar cells are fabricated using low-temperature-annealed ZnO film as an electron transport layer. Uniform ZnO films were prepared by spin coating a diethylzinc (DEZ) precursor solution in air, followed by annealing at 100 A degrees C. Organic solar cells prepared on these ZnO films with a 1:1 P3HT:PCBM blend as the active layer show a high power conversion efficiency of 4.03 \%, which is more than 10 \% higher than the PCE of solar cells comprising ZnO prepared via a high-temperature sol-gel route.}, language = {en} } @article{SaleemThungaKolloscheetal.2014, author = {Saleem, H. and Thunga, M. and Kollosche, Matthias and Kessler, M. R. and Laflamme, S.}, title = {Interfacial treatment effects on behavior of soft nano-composites for highly stretchable dielectrics}, series = {Polymer : the international journal for the science and technology of polymers}, volume = {55}, journal = {Polymer : the international journal for the science and technology of polymers}, number = {17}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-3861}, doi = {10.1016/j.polymer.2014.06.054}, pages = {4531 -- 4537}, year = {2014}, abstract = {We investigate the influence of interfacial treatment on the matrix filler interaction using a melt mixing process to fabricate robust and highly stretchable dielectrics. Silicone oil and silane coupling agent are studied as possible solutions to enhance the compatibility between the inorganic fillers and polymer matrix. Morphology, thermomechanical and dielectric behavior of the prepared specimens are studied. Results show that specimens filled with silicone oil coated particles have promising dielectric and thermal properties. The mechanical properties reveal a stiffness enhancement by 67\% with a high strain at break of 900\%. The relative permittivity of the specimens prepared with silicone oil increased by 45\% as observed from the dielectric analysis. (C) 2014 Elsevier Ltd. All rights reserved.}, language = {en} } @article{ShalomGuttentagFettkenhaueretal.2014, author = {Shalom, Menny and Guttentag, Miguel and Fettkenhauer, Christian and Inal, Sahika and Neher, Dieter and Llobet, Antoni and Antonietti, Markus}, title = {In situ formation of heterojunctions in modified graphitic carbon nitride: synthesis and noble metal free photocatalysis}, series = {Chemistry of materials : a publication of the American Chemical Society}, volume = {26}, journal = {Chemistry of materials : a publication of the American Chemical Society}, number = {19}, publisher = {American Chemical Society}, address = {Washington}, issn = {0897-4756}, doi = {10.1021/cm503258z}, pages = {5812 -- 5818}, year = {2014}, abstract = {Herein, we report the facile synthesis of an efficient roll-like carbon nitride (C3N4) photocatalyst for hydrogen production using a supramolecular complex composed of cyanuric acid, melamine, and barbituric acid as the starting monomers. Optical and photocatalytic investigations show, along with the known red shift of absorption into the visible region, that the insertion of barbituric acid results in the in situ formation of in-plane heterojuctions, which enhance the charge separation process under illumination. Moreover, platinum as the standard cocatalyst in photocatalysis could be successfully replaced with first row transition metal salts and complexes under retention of 50\% of the catalytic activity. Their mode of deposition and interaction with the semiconductor was studied in detail. Utilization of the supramolecular approach opens new opportunities to manipulate the charge transfer process within carbon nitride with respect to the design of a more efficient carbon nitride photocatalyst with controlled morphology and optical properties.}, language = {en} } @article{MengelLevermann2014, author = {Mengel, Matthias and Levermann, Anders}, title = {Ice plug prevents irreversible discharge from East Antarctica}, series = {Nature climate change}, volume = {4}, journal = {Nature climate change}, number = {6}, publisher = {Nature Publ. Group}, address = {London}, issn = {1758-678X}, doi = {10.1038/NCLIMATE2226}, pages = {451 -- 455}, year = {2014}, abstract = {Changes in ice discharge from Antarctica constitute the largest uncertainty in future sea-level projections, mainly because of the unknown response of its marine basins(1). Most of West Antarctica's marine ice sheet lies on an inland-sloping bed(2) and is thereby prone to a marine ice sheet instability(3-5). A similar topographic configuration is found in large parts of East Antarctica, which holds marine ice equivalent to 19 m of global sea-level rise(6), that is, more than five times that of West Antarctica. Within East Antarctica, the Wilkes Basin holds the largest volume of marine ice that is fully connected by subglacial troughs. This ice body was significantly reduced during the Pliocene epoch(7). Strong melting underneath adjacent ice shelves with similar bathymetry(8) indicates the ice sheet's sensitivity to climatic perturbations. The stability of the Wilkes marine ice sheet has not been the subject of any comprehensive assessment of future sea level. Using recently improved topographic data(6) in combination with ice-dynamic simulations, we show here that the removal of a specific coastal ice volume equivalent to less than 80 mm of global sea-level rise at the margin of the Wilkes Basin destabilizes the regional ice flow and leads to a self-sustained discharge of the entire basin and a global sea-level rise of 3-4 m. Our results are robust with respect to variation in ice parameters, forcing details and model resolution as well as increased surface mass balance, indicating that East Antarctica may become a large contributor to future sea-level rise on timescales beyond a century.}, language = {en} } @article{PollatosYeldesbayPikovskijetal.2014, author = {Pollatos, Olga and Yeldesbay, Azamat and Pikovskij, Arkadij and Rosenblum, Michael}, title = {How much time has passed? Ask your heart}, series = {Frontiers in neurorobotics}, volume = {8}, journal = {Frontiers in neurorobotics}, publisher = {Frontiers Research Foundation}, address = {Lausanne}, issn = {1662-5218}, doi = {10.3389/fnbot.2014.00015}, pages = {1 -- 9}, year = {2014}, abstract = {Internal signals like one's heartbeats are centrally processed via specific pathways and both their neural representations as well as their conscious perception (interoception) provide key information for many cognitive processes. Recent empirical findings propose that neural processes in the insular cortex, which are related to bodily signals, might constitute a neurophysiological mechanism for the encoding of duration. Nevertheless, the exact nature of such a proposed relationship remains unclear. We aimed to address this question by searching for the effects of cardiac rhythm on time perception by the use of a duration reproduction paradigm. Time intervals used were of 0.5, 2, 3, 7, 10, 14, 25, and 40s length. In a framework of synchronization hypothesis, measures of phase locking between the cardiac cycle and start/stop signals of the reproduction task were calculated to quantify this relationship. The main result is that marginally significant synchronization indices (Sls) between the heart cycle and the time reproduction responses for the time intervals of 2, 3, 10, 14, and 25s length were obtained, while results were not significant for durations of 0.5, 7, and 40s length. On the single participant level, several subjects exhibited some synchrony between the heart cycle and the time reproduction responses, most pronounced for the time interval of 25s (8 out of 23 participants for 20\% quantile). Better time reproduction accuracy was not related with larger degree of phase locking, but with greater vagal control of the heart. A higher interoceptive sensitivity (IS) was associated with a higher synchronization index (SI) for the 2s time interval only. We conclude that information obtained from the cardiac cycle is relevant for the encoding and reproduction of time in the time span of 2-25s. Sympathovagal tone as well as interoceptive processes mediate the accuracy of time estimation.}, language = {en} } @article{GoychukKharchenkoMetzler2014, author = {Goychuk, Igor and Kharchenko, Vasyl O. and Metzler, Ralf}, title = {How Molecular Motors Work in the Crowded Environment of Living Cells: Coexistence and Efficiency of Normal and Anomalous Transport}, series = {PLoS one}, volume = {9}, journal = {PLoS one}, number = {3}, publisher = {PLoS}, address = {San Fransisco}, issn = {1932-6203}, doi = {10.1371/journal.pone.0091700}, pages = {7}, year = {2014}, abstract = {Recent experiments reveal both passive subdiffusion of various nanoparticles and anomalous active transport of such particles by molecular motors in the molecularly crowded environment of living biological cells. Passive and active microrheology reveals that the origin of this anomalous dynamics is due to the viscoelasticity of the intracellular fluid. How do molecular motors perform in such a highly viscous, dissipative environment? Can we explain the observed co-existence of the anomalous transport of relatively large particles of 100 to 500 nm in size by kinesin motors with the normal transport of smaller particles by the same molecular motors? What is the efficiency of molecular motors in the anomalous transport regime? Here we answer these seemingly conflicting questions and consistently explain experimental findings in a generalization of the well-known continuous diffusion model for molecular motors with two conformational states in which viscoelastic effects are included.}, language = {en} } @article{RichterFoxBenBekhtietal.2014, author = {Richter, Philipp and Fox, Andrew J. and Ben Bekhti, Nadya and Murphy, M. T. and Bomans, Dominik J. and Frank, S.}, title = {High-resolution absorption spectroscopy of the circumgalactic medium of the Milky Way}, series = {Astronomische Nachrichten = Astronomical notes}, volume = {335}, journal = {Astronomische Nachrichten = Astronomical notes}, number = {1}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0004-6337}, doi = {10.1002/asna.201312013}, pages = {92 -- 98}, year = {2014}, language = {en} } @article{CollaborationAbramowskiAharonianetal.2014, author = {Collaboration, H. E. S. S. and Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and de Wilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, Dieter and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, Kornelia and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {HESS observations of the Crab during its March 2013 GeV gamma-ray flare}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {562}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201323013}, pages = {5}, year = {2014}, abstract = {Context. On March 4, 2013 the Fermi-EAT and AGILE reported a flare from the direction of the Crab nebula in which the high-energy (HE; E > 100 MeV) flux was six times above its quiescent level. Simultaneous observations in other energy bands give us hints about the emission processes during the flare episode and the physics of pulsar wind nebulae in general. Aims. We search for variability in the emission of the Crab nebula at very-high energies (VHF,; E > 100 GeV), using contemporaneous data taken with the H.E.S.S. array of Cherenkov telescopes. Methods. Observational data taken with the H.E.S.S. instrument on five consecutive days during the flare were analysed for the flux and spectral shape of the emission from the Crab nebula. Night-wise light curves are presented with energy thresholds of 1 TeV and 5 TeV. Results. The observations conducted with H.E.S.S. on March 6 to March 10, 2013 show no significant changes in the flux. They limit the variation in the integral flux above 1 TeV to less than 63\% and the integral flux above 5 TeV to less than 78\% at a 95\% confidence level.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {HESS J1818-154, a new composite supernova remnant discovered in TeV gamma rays and X-rays}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {562}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, organization = {HESS Collaboration}, issn = {0004-6361}, doi = {10.1051/0004-6361/201322914}, pages = {10}, year = {2014}, abstract = {Composite supernova remnants (SNRs) constitute a small subclass of the remnants of massive stellar explosions where non-thermal radiation is observed from both the expanding shell-like shock front and from a pulsar wind nebula (PWN) located inside of the SNR. These systems represent a unique evolutionary phase of SNRs where observations in the radio, X-ray, and gamma-ray regimes allow the study of the co-evolution of both these energetic phenomena. In this article, we report results from observations of the shell-type SNR G15.4+0.1 performed with the High Energy Stereoscopic System (H. E. S. S.) and XMM-Newton. A compact TeV gamma-ray source, HESS J1818-154, located in the center and contained within the shell of G15.4+0.1 is detected by H. E. S. S. and featurs a spectrum best represented by a power-law model with a spectral index of -2.3 +/- 0.3(stat) +/- 0.2(sys) and an integral flux of F(>0.42 TeV) = (0.9 +/- 0.3(stat) +/- 0.2(sys)) x 10(-12) cm(-2) s(-1). Furthermore, a recent observation with XMM-Newton reveals extended X-ray emission strongly peaked in the center of G15.4+0.1. The X-ray source shows indications of an energy-dependent morphology featuring a compact core at energies above 4 keV and more extended emission that fills the entire region within the SNR at lower energies. Together, the X-ray and VHE gamma-ray emission provide strong evidence of a PWN located inside the shell of G15.4+0.1 and this SNR can therefore be classified as a composite based on these observations. The radio, X-ray, and gamma-ray emission from the PWN is compatible with a one-zone leptonic model that requires a low average magnetic field inside the emission region. An unambiguous counterpart to the putative pulsar, which is thought to power the PWN, has been detected neither in radio nor in X-ray observations of G15.4+0.1.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, Michael K. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, Marek and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, Krzysztof and Katz, Uli and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, Michael and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, Olaf and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, Christopher and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {HESS J1640-465-an exceptionally luminous TeV gamma-ray supernova remnant}, series = {Monthly notices of the Royal Astronomical Society}, volume = {439}, journal = {Monthly notices of the Royal Astronomical Society}, number = {3}, publisher = {Oxford Univ. Press}, address = {Oxford}, organization = {Hess Collaboration}, issn = {0035-8711}, doi = {10.1093/mnras/stu139}, pages = {2828 -- 2836}, year = {2014}, abstract = {The results of follow-up observations of the TeV gamma-ray source HESS J1640-465 from 2004 to 2011 with the High Energy Stereoscopic System (HESS) are reported in this work. The spectrum is well described by an exponential cut-off power law with photon index Gamma = 2.11 +/- 0.09(stat) +/- 0.10(sys), and a cut-off energy of E-2 = 6.0(-1.2)(+2.0) TeV. The TeV emission is significantly extended and overlaps with the northwestern part of the shell of the SNR G338.3-0.0. The new HESS results, a re-analysis of archival XMM-Newton data and multiwavelength observations suggest that a significant part of the gamma-ray emission from HESS J1640-465 originates in the supernova remnant shell. In a hadronic scenario, as suggested by the smooth connection of the GeV and TeV spectra, the product of total proton energy and mean target density could be as high as W(p)n(H) similar to 4 x 10(52)(d/10kpc)(2) erg cm(-3).}, language = {en} } @misc{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Dickinson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, Michael and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and de los Reyes, R. and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {HESS J1640-465 - an exceptionally luminous TeV gamma-ray supernova remnant (vol 439, pg 2828, 2014)}, series = {Monthly notices of the Royal Astronomical Society}, volume = {441}, journal = {Monthly notices of the Royal Astronomical Society}, number = {4}, publisher = {Oxford Univ. Press}, address = {Oxford}, organization = {HESS Collaboration}, issn = {0035-8711}, doi = {10.1093/mnras/stu826}, pages = {3640 -- 3642}, year = {2014}, language = {en} } @phdthesis{Mallonn2014, author = {Mallonn, Matthias}, title = {Ground-based transmission spectroscopy of three inflated Hot Jupiter exoplanets}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-74403}, school = {Universit{\"a}t Potsdam}, pages = {ix, 115}, year = {2014}, abstract = {The characterization of exoplanets is a young and rapidly expanding field in astronomy. It includes a method called transmission spectroscopy that searches for planetary spectral fingerprints in the light received from the host star during the event of a transit. This techniques allows for conclusions on the atmospheric composition at the terminator region, the boundary between the day and night side of the planet. Observationally a big challenge, first attempts in the community have been successful in the detection of several absorption features in the optical wavelength range. These are for example a Rayleighscattering slope and absorption by sodium and potassium. However, other objects show a featureless spectrum indicative for a cloud or haze layer of condensates masking the probable atmospheric layers. In this work, we performed transmission spectroscopy by spectrophotometry of three Hot Jupiter exoplanets. When we began the work on this thesis, optical transmission spectra have been available for two exoplanets. Our main goal was to advance the current sample of probed objects to learn by comparative exoplanetology whether certain absorption features are common. We selected the targets HAT-P-12b, HAT-P-19b and HAT-P-32b, for which the detection of atmospheric signatures is feasible with current ground-based instrumentation. In addition, we monitored the host stars of all three objects photometrically to correct for influences of stellar activity if necessary. The obtained measurements of the three objects all favor featureless spectra. A variety of atmospheric compositions can explain the lack of a wavelength dependent absorption. But the broad trend of featureless spectra in planets of a wide range of temperatures, found in this work and in similar studies recently published in the literature, favors an explanation based on the presence of condensates even at very low concentrations in the atmospheres of these close-in gas giants. This result points towards the general conclusion that the capability of transmission spectroscopy to determine the atmospheric composition is limited, at least for measurements at low spectral resolution. In addition, we refined the transit parameters and ephemerides of HAT-P-12b and HATP- 19b. Our monitoring campaigns allowed for the detection of the stellar rotation period of HAT-P-19 and a refined age estimate. For HAT-P-12 and HAT-P-32, we derived upper limits on their potential variability. The calculated upper limits of systematic effects of starspots on the derived transmission spectra were found to be negligible for all three targets. Finally, we discussed the observational challenges in the characterization of exoplanet atmospheres, the importance of correlated noise in the measurements and formulated suggestions on how to improve on the robustness of results in future work.}, language = {en} } @article{DiFlorioBruendermannYadavallietal.2014, author = {Di Florio, G. and Bruendermann, E. and Yadavalli, Nataraja Sekhar and Santer, Svetlana and Havenith, Martina}, title = {Graphene multilayer as nanosized optical strain gauge for polymer surface relief gratings}, series = {Nano letters : a journal dedicated to nanoscience and nanotechnology}, volume = {14}, journal = {Nano letters : a journal dedicated to nanoscience and nanotechnology}, number = {10}, publisher = {American Chemical Society}, address = {Washington}, issn = {1530-6984}, doi = {10.1021/nl502631s}, pages = {5754 -- 5760}, year = {2014}, abstract = {In this paper, we show how graphene can be utilized as a nanoscopic probe in order to characterize local opto-mechanical forces generated within photosensitive azobenzene containing polymer films. Upon irradiation with light interference patterns, photosensitive films deform according to the spatial intensity variation, leading to the formation of periodic topographies such as surface relief gratings (SRG). The mechanical driving forces inscribing a pattern into the films are supposedly fairly large, because the deformation takes place without photofluidization; the polymer is in a glassy state throughout. However, until now there has been no attempt to characterize these forces by any means. The challenge here is that the forces vary locally on a nanometer scale. Here, we propose to use Raman analysis of the stretching of the graphene layer adsorbed on top of polymer film under deformation in order to probe the strength of the material transport spatially resolved. With the well-known mechanical properties of graphene, we can obtain lower bounds on the forces acting within the film. Upon the basis of our experimental results, we can deduce that the internal pressure in the film due to grating formation can exceed 1 GPa. The graphene-based nanoscopic gauge opens new possibilities to characterize opto-mechanical forces generated within photosensitive polymer films.}, language = {en} } @article{NagelGuvenThevesetal.2014, author = {Nagel, Oliver and Guven, Can and Theves, Matthias and Driscoll, Meghan and Losert, Wolfgang and Beta, Carsten}, title = {Geometry-driven polarity in motile amoeboid cells}, series = {PLoS one}, volume = {9}, journal = {PLoS one}, number = {12}, publisher = {PLoS}, address = {San Fransisco}, issn = {1932-6203}, doi = {10.1371/journal.pone.0113382}, pages = {20}, year = {2014}, abstract = {Motile eukaryotic cells, such as leukocytes, cancer cells, and amoeba, typically move inside the narrow interstitial spacings of tissue or soil. While most of our knowledge of actin-driven eukaryotic motility was obtained from cells that move on planar open surfaces, recent work has demonstrated that confinement can lead to strongly altered motile behavior. Here, we report experimental evidence that motile amoeboid cells undergo a spontaneous symmetry breaking in confined interstitial spaces. Inside narrow channels, the cells switch to a highly persistent, unidirectional mode of motion, moving at a constant speed along the channel. They remain in contact with the two opposing channel side walls and alternate protrusions of their leading edge near each wall. Their actin cytoskeleton exhibits a characteristic arrangement that is dominated by dense, stationary actin foci at the side walls, in conjunction with less dense dynamic regions at the leading edge. Our experimental findings can be explained based on an excitable network model that accounts for the confinement-induced symmetry breaking and correctly recovers the spatio-temporal pattern of protrusions at the leading edge. Since motile cells typically live in the narrow interstitial spacings of tissue or soil, we expect that the geometry-driven polarity we report here plays an important role for movement of cells in their natural environment.}, language = {en} } @phdthesis{Federici2014, author = {Federici, Simone}, title = {Gamma-ray studies of the young shell-type SNR RX J1713.7-3946}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-71734}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {One of the most significant current discussions in Astrophysics relates to the origin of high-energy cosmic rays. According to our current knowledge, the abundance distribution of the elements in cosmic rays at their point of origin indicates, within plausible error limits, that they were initially formed by nuclear processes in the interiors of stars. It is also believed that their energy distribution up to 1018 eV has Galactic origins. But even though the knowledge about potential sources of cosmic rays is quite poor above „ 1015 eV, that is the "knee" of the cosmic-ray spectrum, up to the knee there seems to be a wide consensus that supernova remnants are the most likely candidates. Evidence of this comes from observations of non-thermal X-ray radiation, requiring synchrotron electrons with energies up to 1014 eV, exactly in the remnant of supernovae. To date, however, there is not conclusive evidence that they produce nuclei, the dominant component of cosmic rays, in addition to electrons. In light of this dearth of evidence, γ-ray observations from supernova remnants can offer the most promising direct way to confirm whether or not these astrophysical objects are indeed the main source of cosmic-ray nuclei below the knee. Recent observations with space- and ground-based observatories have established shell-type supernova remnants as GeV-to- TeV γ-ray sources. The interpretation of these observations is however complicated by the different radiation processes, leptonic and hadronic, that can produce similar fluxes in this energy band rendering ambiguous the nature of the emission itself. The aim of this work is to develop a deeper understanding of these radiation processes from a particular shell-type supernova remnant, namely RX J1713.7-3946, using observations of the LAT instrument onboard the Fermi Gamma-Ray Space Telescope. Furthermore, to obtain accurate spectra and morphology maps of the emission associated with this supernova remnant, an improved model of the diffuse Galactic γ-ray emission background is developed. The analyses of RX J1713.7-3946 carried out with this improved background show that the hard Fermi-LAT spectrum cannot be ascribed to the hadronic emission, leading thus to the conclusion that the leptonic scenario is instead the most natural picture for the high-energy γ-ray emission of RX J1713.7-3946. The leptonic scenario however does not rule out the possibility that cosmic-ray nuclei are accelerated in this supernova remnant, but it suggests that the ambient density may not be high enough to produce a significant hadronic γ-ray emission. Further investigations involving other supernova remnants using the improved back- ground developed in this work could allow compelling population studies, and hence prove or disprove the origin of Galactic cosmic-ray nuclei in these astrophysical objects. A break- through regarding the identification of the radiation mechanisms could be lastly achieved with a new generation of instruments such as CTA.}, language = {en} } @article{Baushev2014, author = {Baushev, Anton N.}, title = {Galaxy halo formation in the absence of violent relaxation and a universal density profile of the halo center}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {786}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/786/1/65}, pages = {8}, year = {2014}, abstract = {While N-body simulations testify to a cuspy profile of the central region of dark matter halos, observations favor a shallow, cored density profile of the central region of at least some spiral galaxies and dwarf spheroidals. We show that a central profile, very close to the observed one, inevitably forms in the center of dark matter halos if we make a supposition about a moderate energy relaxation of the system during the halo formation. If we assume the energy exchange between dark matter particles during the halo collapse is not too intensive, the profile is universal: it depends almost not at all on the properties of the initial perturbation and is very akin, but not identical, to the Einasto profile with a small Einasto index n similar to 0.5. We estimate the size of the "central core" of the distribution, i.e., the extent of the very central region with a respectively gentle profile, and show that the cusp formation is unlikely, even if the dark matter is cold. The obtained profile is in good agreement with observational data for at least some types of galaxies but clearly disagrees with N-body simulations.}, language = {en} } @article{BonifacioRahmaniWhitmoreetal.2014, author = {Bonifacio, P. and Rahmani, H. and Whitmore, J. B. and Wendt, Martin and Centurion, Martin and Molaro, P. and Srianand, R. and Murphy, M. T. and Petitjean, P. and Agafonova, I. I. and Evans, T. M. and Levshakov, S. A. and Lopez, S. and Martins, C. J. A. P. and Reimers, D. and Vladilo, G.}, title = {Fundamental constants and high-resolution spectroscopy}, series = {Astronomische Nachrichten = Astronomical notes}, volume = {335}, journal = {Astronomische Nachrichten = Astronomical notes}, number = {1}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0004-6337}, doi = {10.1002/asna.201312005}, pages = {83 -- 91}, year = {2014}, language = {en} } @article{RolandSchubertCollinsetal.2014, author = {Roland, Steffen and Schubert, Marcel and Collins, Brian A. and Kurpiers, Jona and Chen, Zhihua and Facchetti, Antonio and Ade, Harald W. and Neher, Dieter}, title = {Fullerene-free polymer solar cells with highly reduced bimolecular recombination and field-independent charge carrier generation}, series = {The journal of physical chemistry letters}, volume = {5}, journal = {The journal of physical chemistry letters}, number = {16}, publisher = {American Chemical Society}, address = {Washington}, issn = {1948-7185}, doi = {10.1021/jz501506z}, pages = {2815 -- 2822}, year = {2014}, abstract = {Photogeneration, recombination, and transport of free charge carriers in all-polymer bulk heterojunction solar cells incorporating poly(3-hexylthiophene) (P3HT) as donor and poly([N,N'-bis(2-octyldodecyl)-naphthelene-1,4,5,8-bis(dicarboximide)-2,6-diyl]-alt-5,5'-(2,2'-bithiophene)) (P(NDI2OD-T2)) as acceptor polymer have been investigated by the use of time delayed collection field (TDCF) and time-of-flight (TOF) measurements. Depending on the preparation procedure used to dry the active layers, these solar cells comprise high fill factors (FFs) of up to 67\%. A strongly reduced bimolecular recombination (BMR), as well as a field-independent free charge carrier generation are observed, features that are common to high performance fullerene-based solar cells. Resonant soft X-ray measurements (R-SoXS) and photoluminescence quenching experiments (PQE) reveal that the BMR is related to domain purity. Our results elucidate the similarities of this polymeric acceptor with the superior recombination properties of fullerene acceptors.}, language = {en} } @phdthesis{Sorce2014, author = {Sorce, Jenny}, title = {From Spitzer mid-infrared observations and measurements of peculiar velocities to constrained simulations of the local universe}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-72486}, school = {Universit{\"a}t Potsdam}, pages = {xx, 303}, year = {2014}, abstract = {Galaxies are observational probes to study the Large Scale Structure. Their gravitational motions are tracers of the total matter density and therefore of the Large Scale Structure. Besides, studies of structure formation and galaxy evolution rely on numerical cosmological simulations. Still, only one universe observable from a given position, in time and space, is available for comparisons with simulations. The related cosmic variance affects our ability to interpret the results. Simulations constrained by observational data are a perfect remedy to this problem. Achieving such simulations requires the projects Cosmic flows and CLUES. Cosmic flows builds catalogs of accurate distance measurements to map deviations from the expansion. These measures are mainly obtained with the galaxy luminosity-rotation rate correlation. We present the calibration of that relation in the mid-infrared with observational data from Spitzer Space Telescope. Resulting accurate distance estimates will be included in the third catalog of the project. In the meantime, two catalogs up to 30 and 150 Mpc/h have been released. We report improvements and applications of the CLUES' method on these two catalogs. The technique is based on the constrained realization algorithm. The cosmic displacement field is computed with the Zel'dovich approximation. This latter is then reversed to relocate reconstructed three-dimensional constraints to their precursors' positions in the initial field. The size of the second catalog (8000 galaxies within 150 Mpc/h) highlighted the importance of minimizing the observational biases. By carrying out tests on mock catalogs, built from cosmological simulations, a method to minimize observational bias can be derived. Finally, for the first time, cosmological simulations are constrained solely by peculiar velocities. The process is successful as resulting simulations resemble the Local Universe. The major attractors and voids are simulated at positions approaching observational positions by a few megaparsecs, thus reaching the limit imposed by the linear theory.}, language = {en} } @phdthesis{Goldshteyn2014, author = {Goldshteyn, Jewgenij}, title = {Frequency-resolved ultrafast dynamics of phonon polariton wavepackets in the ferroelectric crystals LiNbO₃ and LiTaO₃}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-71623}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {During this work I built a four wave mixing setup for the time-resolved femtosecond spectroscopy of Raman-active lattice modes. This setup enables to study the selective excitation of phonon polaritons. These quasi-particles arise from the coupling of electro-magnetic waves and transverse optical lattice modes, the so-called phonons. The phonon polaritons were investigated in the optically non-linear, ferroelectric crystals LiNbO₃ and LiTaO₃. The direct observation of the frequency shift of the scattered narrow bandwidth probe pulses proofs the role of the Raman interaction during the probe and excitation process of phonon polaritons. I compare this experimental method with the measurement where ultra-short laser pulses are used. The frequency shift remains obscured by the relative broad bandwidth of these laser pulses. In an experiment with narrow bandwidth probe pulses, the Stokes and anti-Stokes intensities are spectrally separated. They are assigned to the corresponding counter-propagating wavepackets of phonon polaritons. Thus, the dynamics of these wavepackets was separately studied. Based on these findings, I develop the mathematical description of the so-called homodyne detection of light for the case of light scattering from counter propagating phonon polaritons. Further, I modified the broad bandwidth of the ultra-short pump pulses using bandpass filters to generate two pump pulses with non-overlapping spectra. This enables the frequency-selective excitation of polariton modes in the sample, which allows me to observe even very weak polariton modes in LiNbO₃ or LiTaO₃ that belong to the higher branches of the dispersion relation of phonon polaritons. The experimentally determined dispersion relation of the phonon polaritons could therefore be extended and compared to theoretical models. In addition, I determined the frequency-dependent damping of phonon polaritons.}, language = {en} } @article{AlbrechtLevermann2014, author = {Albrecht, Torsten and Levermann, Anders}, title = {Fracture-induced softening for large-scale ice dynamics}, series = {The Cryosphere : TC ; an interactive open access journal of the European Geosciences Union}, volume = {8}, journal = {The Cryosphere : TC ; an interactive open access journal of the European Geosciences Union}, number = {2}, publisher = {Copernicus}, address = {G{\"o}ttingen}, issn = {1994-0416}, doi = {10.5194/tc-8-587-2014}, pages = {587 -- 605}, year = {2014}, abstract = {Floating ice shelves can exert a retentive and hence stabilizing force onto the inland ice sheet of Antarctica. However, this effect has been observed to diminish by the dynamic effects of fracture processes within the protective ice shelves, leading to accelerated ice flow and hence to a sea-level contribution. In order to account for the macroscopic effect of fracture processes on large-scale viscous ice dynamics (i.e., ice-shelf scale) we apply a continuum representation of fractures and related fracture growth into the prognostic Parallel Ice Sheet Model (PISM) and compare the results to observations. To this end we introduce a higher order accuracy advection scheme for the transport of the two-dimensional fracture density across the regular computational grid. Dynamic coupling of fractures and ice flow is attained by a reduction of effective ice viscosity proportional to the inferred fracture density. This formulation implies the possibility of non-linear threshold behavior due to self-amplified fracturing in shear regions triggered by small variations in the fracture-initiation threshold. As a result of prognostic flow simulations, sharp across-flow velocity gradients appear in fracture-weakened regions. These modeled gradients compare well in magnitude and location with those in observed flow patterns. This model framework is in principle expandable to grounded ice streams and provides simple means of investigating climate-induced effects on fracturing (e. g., hydro fracturing) and hence on the ice flow. It further constitutes a physically sound basis for an enhanced fracture-based calving parameterization.}, language = {en} } @article{ChengDingZhangetal.2014, author = {Cheng, X. and Ding, M. D. and Zhang, J. and Sun, X. D. and Guo, Y. and Wang, Yi-Ming and Kliem, Bernhard and Deng, Y. Y.}, title = {Formation of a double-decker magnetic flux rope in the sigmoidal solar active region 11520}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {789}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/789/2/93}, pages = {12}, year = {2014}, abstract = {In this paper, we address the formation of a magnetic flux rope (MFR) that erupted on 2012 July 12 and caused a strong geomagnetic storm event on July 15. Through analyzing the long-term evolution of the associated active region observed by the Atmospheric Imaging Assembly and the Helioseismic and Magnetic Imager on board the Solar Dynamics Observatory, it is found that the twisted field of an MFR, indicated by a continuous S-shaped sigmoid, is built up from two groups of sheared arcades near the main polarity inversion line a half day before the eruption. The temperature within the twisted field and sheared arcades is higher than that of the ambient volume, suggesting that magnetic reconnection most likely works there. The driver behind the reconnection is attributed to shearing and converging motions at magnetic footpoints with velocities in the range of 0.1-0.6 km s(-1). The rotation of the preceding sunspot also contributes to the MFR buildup. Extrapolated three-dimensional non-linear force-free field structures further reveal the locations of the reconnection to be in a bald-patch region and in a hyperbolic flux tube. About 2 hr before the eruption, indications of a second MFR in the form of an S-shaped hot channel are seen. It lies above the original MFR that continuously exists and includes a filament. The whole structure thus makes up a stable double-decker MFR system for hours prior to the eruption. Eventually, after entering the domain of instability, the high-lying MFR impulsively erupts to generate a fast coronal mass ejection and X-class flare; while the low-lying MFR remains behind and continuously maintains the sigmoidicity of the active region.}, language = {en} } @phdthesis{Faber2014, author = {Faber, Michael}, title = {Folding dynamics of RNA secondary structures}, pages = {85}, year = {2014}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Anton, Gisela and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Bernl{\"o}hr, K. and Birsin, E. and Bissaldi, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Brucker, J. and Brun, Francois and Brun, Pierre and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Cerruti, M. and Chadwick, Paula M. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Cheesebrough, A. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Daniel, M. K. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Dicldnson, H. J. and Djannati-Ata{\"i}, A. and Domainko, W. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Grondin, M. -H. and Grudzinska, M. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kneiske, T. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lennarz, D. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Moderski, R. and Mohamed, M. and Moulin, Emmanuel and Murach, T. and Naumann, C. L. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Ohm, S. and Wilhelmi, E. de Ona and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Perez, J. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Raue, M. and Reimer, A. and Reimer, O. and Renaud, M. and Reyes, R. de Los and Rieger, F. and Rob, L. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Szostek, A. and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Venter, C. and Viana, A. and Vincent, P. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Zabalza, V. and Zacharias, M. and Zajczyk, A. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S.}, title = {Flux upper limits for 47 AGN observed with HESS in 2004-2011}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {564}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, organization = {HESS Collaboration}, issn = {0004-6361}, doi = {10.1051/0004-6361/201322897}, pages = {10}, year = {2014}, abstract = {Context. About 40\% of the observation time of the High Energy Stereoscopic System (H.E.S.S.) is dedicated to studying active galactic nuclei (AGN), with the aim of increasing the sample of known extragalactic very-high-energy (VHE, E > 100 GeV) sources and constraining the physical processes at play in potential emitters. Aims. H.E.S.S. observations of AGN, spanning a period from April 2004 to December 2011, are investigated to constrain their gamma-ray fluxes. Only the 47 sources without significant excess detected at the position of the targets are presented. Methods. Upper limits on VHE fluxes of the targets were computed and a search for variability was performed on the nightly time scale. Results. For 41 objects, the flux upper limits we derived are the most constraining reported to date. These constraints at VHE are compared with the flux level expected from extrapolations of Fermi-LAT measurements in the two-year catalog of AGN. The H.E.S.S. upper limits are at least a factor of two lower than the extrapolated Fermi-LAT fluxes for 11 objects Taking into account the attenuation by the extragalactic background light reduces the tension for all but two of them, suggesting intrinsic curvature in the high-energy spectra of these two AGN. Conclusions. Compilation efforts led by current VHE instruments are of critical importance for target-selection strategies before the advent of the Cherenkov Telescope Array (CTA).}, language = {en} } @article{KruesemannGodecMetzler2014, author = {Kr{\"u}semann, Henning and Godec, Aljaz and Metzler, Ralf}, title = {First-passage statistics for aging diffusion in systems with annealed and quenched disorder}, series = {Physical review : E, Statistical, nonlinear and soft matter physics}, volume = {89}, journal = {Physical review : E, Statistical, nonlinear and soft matter physics}, number = {4}, publisher = {American Physical Society}, address = {College Park}, issn = {1539-3755}, doi = {10.1103/PhysRevE.89.040101}, pages = {5}, year = {2014}, abstract = {Aging, the dependence of the dynamics of a physical process on the time t(a) since its original preparation, is observed in systems ranging from the motion of charge carriers in amorphous semiconductors over the blinking dynamics of quantum dots to the tracer dispersion in living biological cells. Here we study the effects of aging on one of the most fundamental properties of a stochastic process, the first-passage dynamics. We find that for an aging continuous time random walk process, the scaling exponent of the density of first-passage times changes twice as the aging progresses and reveals an intermediate scaling regime. The first-passage dynamics depends on t(a) differently for intermediate and strong aging. Similar crossovers are obtained for the first-passage dynamics for a confined and driven particle. Comparison to the motion of an aged particle in the quenched trap model with a bias shows excellent agreement with our analytical findings. Our results demonstrate how first-passage measurements can be used to unravel the age t(a) of a physical system.}, language = {en} } @article{CuiYashchenokZhangetal.2014, author = {Cui, Qianling and Yashchenok, Alexey and Zhang, Lu and Li, Lidong and Masic, Admir and Wienskol, Gabriele and Moehwald, Helmuth and Bargheer, Matias}, title = {Fabrication of Bifunctional Gold/Gelatin Hybrid Nanocomposites and Their Application}, series = {ACS applied materials \& interfaces}, volume = {6}, journal = {ACS applied materials \& interfaces}, number = {3}, publisher = {American Chemical Society}, address = {Washington}, issn = {1944-8244}, doi = {10.1021/am5000068}, pages = {1999 -- 2002}, year = {2014}, abstract = {Herein, a facile method is presented to integrate large gold nanoflowers (similar to 80 nm) and small gold nanoparticles (2-4 nm) into a single entity, exhibiting both surface-enhanced Raman scattering (SERS) and catalytic activity. The as-prepared gold nanoflowers were coated by a gelatin layer, in which the gold precursor was adsorbed and in situ reduced into small gold nanoparticles. The thickness of the gelatin shell is controlled to less than 10 nm, ensuring that the small gold nanoparticles are still in a SERS-active range of the inner Au core. Therefore, the reaction catalyzed by these nanocomposites can be monitored in situ using label-free SERS spectroscopy. In addition, these bifunctional nanocomposites are also attractive candidates for application in SERS monitoring of bioreactions because of their excellent biocompatibility.}, language = {en} } @article{CuiShenYanetal.2014, author = {Cui, Qianling and Shen, Guizhi and Yan, Xuehai and Li, Lidong and Moehwald, Helmuth and Bargheer, Matias}, title = {Fabrication of Au@Pt multibranched nanoparticles and their application to in situ SERS monitoring}, series = {ACS applied materials \& interfaces}, volume = {6}, journal = {ACS applied materials \& interfaces}, number = {19}, publisher = {American Chemical Society}, address = {Washington}, issn = {1944-8244}, doi = {10.1021/am504709a}, pages = {17075 -- 17081}, year = {2014}, abstract = {Here, we present an Au@Pt core-shell multibranched nanoparticle as a new substrate capable of in situ surface-enhanced Raman scattering (SERS), thereby enabling monitoring of the catalytic reaction on the active surface. By careful control of the amount of Pt deposited bimetallic Au@Pt, nanoparticles with moderate performance both for SERS and catalytic activity were obtained. The Pt-catalyzed reduction of 4-nitrothiophenol by borohydride was chosen as the model reaction. The intermediate during the reaction was captured and clearly identified via SERS spectroscopy. We established in situ SERS spectroscopy as a promising and powerful technique to investigate in situ reactions taking place in heterogeneous catalysis.}, language = {en} } @article{ChuBrennerChenetal.2014, author = {Chu, X. -L. and Brenner, Thomas J. K. and Chen, X. -W. and Ghosh, Y. and Hollingsworth, J. A. and Sandoghdar, Vahid and Goetzinger, S.}, title = {Experimental realization of an optical antenna designed for collecting 99\% of photons from a quantum emitter}, series = {Optica}, volume = {1}, journal = {Optica}, number = {4}, publisher = {Optical Society of America}, address = {Washington}, issn = {2334-2536}, doi = {10.1364/OPTICA.1.000203}, pages = {203 -- 208}, year = {2014}, abstract = {A light source that emits single photons at well-defined times and into a well-defined mode would be a decisive asset for quantum information processing, quantum metrology, and sub-shot-noise detection of absorption. One of the central challenges in the realization of such a deterministic device based on a single quantum emitter concerns the collection of the photons, which are radiated into a 4 pi solid angle. Here, we present the fabrication and characterization of an optical antenna designed to convert the dipolar radiation of an arbitrarily oriented quantum emitter to a directional beam with more than 99\% efficiency. Our approach is extremely versatile and can be used for more efficient detection of nanoscopic emitters ranging from semiconductor quantum dots to dye molecules, color centers, or rare-earth ions in various environments. Having addressed the issue of collection efficiency, we also discuss the photophysical limitations of the existing quantum emitters for the realization of a deterministic single-photon source. (C) 2014 Optical Society of America}, language = {en} } @article{FangGuerreroMarquezLugoetal.2014, author = {Fang, X. and Guerrero, Mart{\´i}n A. and Marquez-Lugo, R. A. and Toala, Jes{\´u}s Alberto and Arthur, S. J. and Chu, Y.-H. and Blair, William P. and Gruendl, R. A. and Hamann, Wolf-Rainer and Oskinova, Lida and Todt, Helge Tobias}, title = {Expansion of hydrogen-poor knots in the born-again planetary nebulae A30 and A78}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {797}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {2}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/797/2/100}, pages = {11}, year = {2014}, abstract = {We analyze the expansion of hydrogen-poor knots and filaments in the born-again planetary nebulae A30 and A78 based on Hubble Space Telescope ( HST) images obtained almost 20 yr apart. The proper motion of these features generally increases with distance to the central star, but the fractional expansion decreases, i.e., the expansion is not homologous. As a result, there is not a unique expansion age, which is estimated to be 610-950 yr for A30 and 600-1140 yr for A78. The knots and filaments have experienced complex dynamical processes: the current fast stellar wind is mass loaded by the material ablated from the inner knots; the ablated material is then swept up until it shocks the inner edges of the outer, hydrogen-rich nebula. The angular expansion of the outer filaments shows a clear dependence on position angle, indicating that the interaction of the stellar wind with the innermost knots channels the wind along preferred directions. The apparent angular expansion of the innermost knots seems to be dominated by the rocket effect of evaporating gas and by the propagation of the ionization front inside them. Radiation-hydrodynamical simulations show that a single ejection of material followed by a rapid onset of the stellar wind and ionizing flux can reproduce the variety of clumps and filaments at different distances from the central star found in A30 and A78.}, language = {en} } @phdthesis{Lange2014, author = {Lange, Ilja}, title = {Energetische Struktur von Schichten organischer Halbleiter und ihr fundamentaler Einfluss auf die physikalischen Eigenschaften organischer elektronischer Bauteile}, school = {Universit{\"a}t Potsdam}, pages = {105}, year = {2014}, language = {de} } @phdthesis{Schubert2014, author = {Schubert, Marcel}, title = {Elementary processes in layers of electron transporting Donor-acceptor copolymers : investigation of charge transport and application to organic solar cells}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-70791}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {Donor-acceptor (D-A) copolymers have revolutionized the field of organic electronics over the last decade. Comprised of a electron rich and an electron deficient molecular unit, these copolymers facilitate the systematic modification of the material's optoelectronic properties. The ability to tune the optical band gap and to optimize the molecular frontier orbitals as well as the manifold of structural sites that enable chemical modifications has created a tremendous variety of copolymer structures. Today, these materials reach or even exceed the performance of amorphous inorganic semiconductors. Most impressively, the charge carrier mobility of D-A copolymers has been pushed to the technologically important value of 10 cm^{2}V^{-1}s^{-1}. Furthermore, owed to their enormous variability they are the material of choice for the donor component in organic solar cells, which have recently surpassed the efficiency threshold of 10\%. Because of the great number of available D-A copolymers and due to their fast chemical evolution, there is a significant lack of understanding of the fundamental physical properties of these materials. Furthermore, the complex chemical and electronic structure of D-A copolymers in combination with their semi-crystalline morphology impede a straightforward identification of the microscopic origin of their superior performance. In this thesis, two aspects of prototype D-A copolymers were analysed. These are the investigation of electron transport in several copolymers and the application of low band gap copolymers as acceptor component in organic solar cells. In the first part, the investigation of a series of chemically modified fluorene-based copolymers is presented. The charge carrier mobility varies strongly between the different derivatives, although only moderate structural changes on the copolymers structure were made. Furthermore, rather unusual photocurrent transients were observed for one of the copolymers. Numerical simulations of the experimental results reveal that this behavior arises from a severe trapping of electrons in an exponential distribution of trap states. Based on the comparison of simulation and experiment, the general impact of charge carrier trapping on the shape of photo-CELIV and time-of-flight transients is discussed. In addition, the high performance naphthalenediimide (NDI)-based copolymer P(NDI2OD-T2) was characterized. It is shown that the copolymer posses one of the highest electron mobilities reported so far, which makes it attractive to be used as the electron accepting component in organic photovoltaic cells.\par Solar cells were prepared from two NDI-containing copolymers, blended with the hole transporting polymer P3HT. I demonstrate that the use of appropriate, high boiling point solvents can significantly increase the power conversion efficiency of these devices. Spectroscopic studies reveal that the pre-aggregation of the copolymers is suppressed in these solvents, which has a strong impact on the blend morphology. Finally, a systematic study of P3HT:P(NDI2OD-T2) blends is presented, which quantifies the processes that limit the efficiency of devices. The major loss channel for excited states was determined by transient and steady state spectroscopic investigations: the majority of initially generated electron-hole pairs is annihilated by an ultrafast geminate recombination process. Furthermore, exciton self-trapping in P(NDI2OD-T2) domains account for an additional reduction of the efficiency. The correlation of the photocurrent to microscopic morphology parameters was used to disclose the factors that limit the charge generation efficiency. Our results suggest that the orientation of the donor and acceptor crystallites relative to each other represents the main factor that determines the free charge carrier yield in this material system. This provides an explanation for the overall low efficiencies that are generally observed in all-polymer solar cells.}, language = {en} } @article{Cherstvy2014, author = {Cherstvy, Andrey G.}, title = {Electrostatics and charge regulation in polyelectrolyte multi layered assembly}, series = {The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces \& biophysical chemistry}, volume = {118}, journal = {The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces \& biophysical chemistry}, number = {17}, publisher = {American Chemical Society}, address = {Washington}, issn = {1520-6106}, doi = {10.1021/jp502460v}, pages = {4552 -- 4560}, year = {2014}, abstract = {We examine the implications of electrostatic interactions on formation of polyelectrolyte multilayers, in application to field-effect based biosensors for label-free detection of charged macromolecules. We present a quantitative model to describe the experimental potentiometric observations and discuss its possibilities and limitations for detection of polyelectrolyte adsorption. We examine the influence of the ionic strength and pH on the sensor response upon polyelectrolyte layer-by-layer formation. The magnitude of potential oscillations on the sensor-electrolyte interface predicted upon repetitive adsorption charge-alternating polymers agrees satisfactorily with experimental results. The model accounts for different screening by mobile ions in electrolyte and inside tightly interdigitated multilayered structure. In particular, we show that sensors' potential oscillations are larger and more persistent at lower salt conditions, while they decay faster with the number of layers at higher salt conditions, in agreement with experiments. The effects of polyelectrolyte layer thickness, substrate potential, and charge regulation on the sensor surface triggered by layer-by-layer deposition are also analyzed.}, language = {en} } @article{CherstvyTeif2014, author = {Cherstvy, Andrey G. and Teif, Vladimir B.}, title = {Electrostatic effect of H1-histone protein binding on nucleosome repeat length}, series = {Physical biology : a journal for the fundamental understanding of biological systems}, volume = {11}, journal = {Physical biology : a journal for the fundamental understanding of biological systems}, number = {4}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1478-3967}, doi = {10.1088/1478-3975/11/4/044001}, pages = {6}, year = {2014}, abstract = {Within a simple biophysical model we describe the effect of electrostatic binding of H1 histone proteins on the nucleosome repeat length in chromatin. The length of wrapped DNA optimizes its binding energy to the histone core and the elastic energy penalty of DNA wrapping. The magnitude of the effect predicted from our model is in agreement with the systematic experimental data on the linear variation of nucleosome repeat lengths with H1/nucleosome ratio (Woodcock C L et al 2006 Chromos. Res. 14 17-25). We compare our model to the data for different cell types and organisms, with a widely varying ratio of bound H1 histones per nucleosome. We underline the importance of this non-specific histone-DNA charge-balance mechanism in regulating the positioning of nucleosomes and the degree of compaction of chromatin fibers in eukaryotic cells.}, language = {en} } @article{BronnerUtechtHaaseetal.2014, author = {Bronner, Christopher and Utecht, Manuel Martin and Haase, Anton and Saalfrank, Peter and Klamroth, Tillmann and Tegeder, Petra}, title = {Electronic structure changes during the surface-assisted formation of a graphene nanoribbon}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {140}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {2}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.4858855}, pages = {7}, year = {2014}, abstract = {High conductivity and a tunability of the band gap make quasi-one-dimensional graphene nanoribbons (GNRs) highly interesting materials for the use in field effect transistors. Especially bottom-up fabricated GNRs possess well-defined edges which is important for the electronic structure and accordingly the band gap. In this study we investigate the formation of a sub-nanometer wide armchair GNR generated on a Au(111) surface. The on-surface synthesis is thermally activated and involves an intermediate non-aromatic polymer in which the molecular precursor forms polyanthrylene chains. Employing angle-resolved two-photon photoemission in combination with density functional theory calculations we find that the polymer exhibits two dispersing states which we attribute to the valence and the conduction band, respectively. While the band gap of the non-aromatic polymer obtained in this way is relatively large, namely 5.25 +/- 0.06 eV, the gap of the corresponding aromatic GNR is strongly reduced which we attribute to the different degree of electron delocalization in the two systems.}, language = {en} } @article{AlbrechtGrootoonkNeubertetal.2014, author = {Albrecht, Steve and Grootoonk, Bjorn and Neubert, Sebastian and Roland, Steffen and Wordenweber, Jan and Meier, Matthias and Schlatmann, Rutger and Gordijn, Aad and Neher, Dieter}, title = {Efficient hybrid inorganic/organic tandem solar cells with tailored recombination contacts}, series = {Solar energy materials \& solar cells : an international journal devoted to photovoltaic, photothermal, and photochemical solar energy conversion}, volume = {127}, journal = {Solar energy materials \& solar cells : an international journal devoted to photovoltaic, photothermal, and photochemical solar energy conversion}, publisher = {Elsevier}, address = {Amsterdam}, issn = {0927-0248}, doi = {10.1016/j.solmat.2014.04.020}, pages = {157 -- 162}, year = {2014}, abstract = {In this work, the authors present a 7.5\% efficient hybrid tandem solar cell with the bottom cell made of amorphous silicon and a Si-PCPDTBT:PC70BM bulk heterojunction top cell. Loss-free recombination contacts were realized by combing Al-doped ZnO with either the conducting polymer composite PEDOT:PSS or with a bilayer of ultrathin Al and MoO3. Optimization of these contacts results in tandem cells with high fill factors of 70\% and an open circuit voltage close to the sum of those of the sub-cells. This is the best efficiency reported for this type of hybrid tandem cell so far. Optical and electrical device modeling suggests that the efficiency can be increased to similar to 12\% on combining a donor polymer with suitable absorption onset with PCBM. We also describe proof-of-principle studies employing light trapping in hybrid tandem solar cells, suggesting that this device architecture has the potential to achieve efficiencies well above 12\%. (C) 2014 Elsevier B.V. All rights reserved.}, language = {en} } @article{VandewalAlbrechtHokeetal.2014, author = {Vandewal, Koen and Albrecht, Steve and Hoke, Eric T. and Graham, Kenneth R. and Widmer, Johannes and Douglas, Jessica D. and Schubert, Marcel and Mateker, William R. and Bloking, Jason T. and Burkhard, George F. and Sellinger, Alan and Frechet, Jean M. J. and Amassian, Aram and Riede, Moritz K. and McGehee, Michael D. and Neher, Dieter and Salleo, Alberto}, title = {Efficient charge generation by relaxed charge-transfer states at organic interfaces}, series = {Nature materials}, volume = {13}, journal = {Nature materials}, number = {1}, publisher = {Nature Publ. Group}, address = {London}, issn = {1476-1122}, doi = {10.1038/NMAT3807}, pages = {63 -- 68}, year = {2014}, abstract = {carriers on illumination. Efficient organic solar cells require a high yield for this process, combined with a minimum of energy losses. Here, we investigate the role of the lowest energy emissive interfacial charge-transfer state (CT1) in the charge generation process. We measure the quantum yield and the electric field dependence of charge generation on excitation of the charge-transfer (CT) state manifold viaweakly allowed, low-energy optical transitions. For a wide range of photovoltaic devices based on polymer: fullerene, small-molecule:C-60 and polymer: polymer blends, our study reveals that the internal quantum efficiency (IQE) is essentially independent of whether or not D, A or CT states with an energy higher than that of CT1 are excited. The best materials systems show an IQE higher than 90\% without the need for excess electronic or vibrational energy.}, language = {en} } @article{GehrigRolandHowardetal.2014, author = {Gehrig, Dominik W. and Roland, Steffen and Howard, Ian A. and Kamm, Valentin and Mangold, Hannah and Neher, Dieter and Laquai, Frederic}, title = {Efficiency-limiting processes in low-bandgap polymer:Perylene diimide photovoltaic blends}, series = {The journal of physical chemistry : C, Nanomaterials and interfaces}, volume = {118}, journal = {The journal of physical chemistry : C, Nanomaterials and interfaces}, number = {35}, publisher = {American Chemical Society}, address = {Washington}, issn = {1932-7447}, doi = {10.1021/jp503366m}, pages = {20077 -- 20085}, year = {2014}, abstract = {The charge generation and recombination processes following photo-excitation of a low-bandgap polymer:perylene diimide photovoltaic blend are investigated by transient absorption pump-probe spectroscopy covering a dynamic range from femto-to microseconds to get insight into the efficiency-limiting photophysical processes. The several tens of picoseconds, and its efficiency is only half of that in a polymer:fullerene photoinduced electron transfer from the polymer to the perylene acceptor takes up to blend. This reduces the short-circuit current. Time-delayed collection field experiments reveal that the subsequent charge separation is strongly field-dependent, limiting the fill factor and lowering the short-circuit current in polymer:PDI devices. Upon excitation of the acceptor in the low-bandgap polymer blend, the PDI exciton undergoes charge transfer on a time scale of several tens of picoseconds. However, a significant fraction of the charges generated at the interface are quickly lost because of fast geminate recombination. This reduces the short-circuit current even further, leading to a scenario in which only around 2596 of the initial photoexcitations generate free charges that can potentially contribute to the photocurrent. In summary, the key photophysical limitations of perylene diimide as an acceptor in low-bandgap polymer blends appear at the interface between the materials, with the kinetics of both charge generation and separation inhibited as compared to that of fullerenes.}, language = {en} } @article{RichterZakrevskyyEiseleetal.2014, author = {Richter, Marcel and Zakrevskyy, Yuriy and Eisele, Michael and Lomadze, Nino and Santer, Svetlana and von Klitzing, Regine}, title = {Effect of pH, co-monomer content, and surfactant structure on the swelling behavior of microgel-azobenzene-containing surfactant complex}, series = {Polymer : the international journal for the science and technology of polymers}, volume = {55}, journal = {Polymer : the international journal for the science and technology of polymers}, number = {25}, publisher = {Elsevier}, address = {Oxford}, issn = {0032-3861}, doi = {10.1016/j.polymer.2014.10.027}, pages = {6513 -- 6518}, year = {2014}, abstract = {The contraction/swelling transition of anionic PNIPAM-co-AAA particles can be manipulated by light using interactions with cationic azobenzene-containing surfactant. In this study the influence of pH-buffers and their concentrations, the charge density (AAA content) in microgel particles as well as the spacer length of the surfactant on the complex formation between the microgel and surfactant is investigated. It is shown that the presence of pH buffer can lead to complete blocking of the interactions in such complexes and the resulting microgel contraction/swelling response. There is a clear competition between the buffer ions and the surfactant molecules interacting with microgel particles. When working in pure water solutions with fixed concentration (charge density) of microgel, the contraction/swelling of the particles is controlled only by relative concentration (charge ratio) of the surfactant and AAA groups of the microgel. Furthermore, the particle contraction is more efficient for shorter spacer length of the surfactant. The onset point of the contraction process is not affected by the surfactant hydrophobicity. This work provides new insight into the interaction between microgel particles and photo-sensitive surfactants, which offers high potential in new sensor systems. (C) 2014 Elsevier Ltd. All rights reserved.}, language = {en} } @article{SchreckPietzschKunnusetal.2014, author = {Schreck, Simon and Pietzsch, Annette and Kunnus, Kristjan and Kennedy, Brian and Quevedo, Wilson and Miedema, Piter S. and Wernet, Philippe and F{\"o}hlisch, Alexander}, title = {Dynamics of the OH group and the electronic structure of liquid alcohols}, series = {Structural dynamics}, volume = {1}, journal = {Structural dynamics}, number = {5}, publisher = {American Institute of Physics}, address = {Melville}, issn = {2329-7778}, doi = {10.1063/1.4897981}, pages = {14}, year = {2014}, abstract = {In resonant inelastic soft x-ray scattering (RIXS) from molecular and liquid systems, the interplay of ground state structural and core-excited state dynamical contributions leads to complex spectral shapes that partially allow for ambiguous interpretations. In this work, we dissect these contributions in oxygen K-edge RIXS from liquid alcohols. We use the scattering into the electronic ground state as an accurate measure of nuclear dynamics in the intermediate core-excited state of the RIXS process. We determine the characteristic time in the core-excited state until nuclear dynamics give a measurable contribution to the RIXS spectral profiles to tau(dyn) = 1.2 +/- 0.8 fs. By detuning the excitation energy below the absorption resonance we reduce the effective scattering time below sdyn, and hence suppress these dynamical contributions to a minimum. From the corresponding RIXS spectra of liquid methanol, we retrieve the "dynamic-free" density of states and find that it is described solely by the electronic states of the free methanol molecule. From this and from the comparison of normal and deuterated methanol, we conclude that the split peak structure found in the lone-pair emission region at non-resonant excitation originates from dynamics in the O-H bond in the core-excited state. We find no evidence that this split peak feature is a signature of distinct ground state structural complexes in liquid methanol. However, we demonstrate how changes in the hydrogen bond coordination within the series of linear alcohols from methanol to hexanol affect the split peak structure in the liquid alcohols. (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.}, language = {en} } @article{HaakhHenkelSpagnoloetal.2014, author = {Haakh, Harald R. and Henkel, Carsten and Spagnolo, Salvatore and Rizzuto, Lucia and Passante, Roberto}, title = {Dynamical Casimir-Polder interaction between an atom and surface plasmons}, series = {Physical review : A, Atomic, molecular, and optical physics}, volume = {89}, journal = {Physical review : A, Atomic, molecular, and optical physics}, number = {2}, publisher = {American Physical Society}, address = {College Park}, issn = {1050-2947}, doi = {10.1103/PhysRevA.89.022509}, pages = {11}, year = {2014}, abstract = {We investigate the time-dependent Casimir-Polder potential of a polarizable two-level atom placed near a surface of arbitrary material, after a sudden change in the parameters of the system. Different initial conditions are taken into account. For an initially bare ground-state atom, the time-dependent Casimir-Polder energy reveals how the atom is "being dressed" by virtual, matter-assisted photons. We also study the transient behavior of the Casimir-Polder interaction between the atom and the surface starting from a partially dressed state, after an externally induced change in the atomic level structure or transition dipoles. The Heisenberg equations are solved through an iterative technique for both atomic and field operators in the medium-assisted electromagnetic field quantization scheme. We analyze, in particular, how the time evolution of the interaction energy depends on the optical properties of the surface, in particular on the dispersion relation of surface plasmon polaritons. The physical significance and the limits of validity of the obtained results are discussed in detail.}, language = {en} } @article{ToeroekLeakeTitovetal.2014, author = {Toeroek, T. and Leake, J. E. and Titov, Viacheslav S. and Archontis, V. and Mikic, Z. and Linton, M. G. and Dalmasse, K. and Aulanier, Guillaume and Kliem, Bernhard}, title = {Distribution of electric currents in solar active regions}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, volume = {782}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {2041-8205}, doi = {10.1088/2041-8205/782/1/L10}, pages = {6}, year = {2014}, language = {en} } @article{OskinovaNazeTodtetal.2014, author = {Oskinova, Lida and Naze, Yael and Todt, Helge Tobias and Huenemoerder, David P. and Ignace, Richard and Hubrig, Swetlana and Hamann, Wolf-Rainer}, title = {Discovery of X-ray pulsations from a massive star}, series = {Nature Communications}, volume = {5}, journal = {Nature Communications}, publisher = {Nature Publ. Group}, address = {London}, issn = {2041-1723}, doi = {10.1038/ncomms5024}, pages = {9}, year = {2014}, abstract = {X-ray emission from stars much more massive than the Sun was discovered only 35 years ago. Such stars drive fast stellar winds where shocks can develop, and it is commonly assumed that the X-rays emerge from the shock-heated plasma. Many massive stars additionally pulsate. However, hitherto it was neither theoretically predicted nor observed that these pulsations would affect their X-ray emission. All X-ray pulsars known so far are associated with degenerate objects, either neutron stars or white dwarfs. Here we report the discovery of pulsating X-rays from a non-degenerate object, the massive B-type star xi(1) CMa. This star is a variable of beta Cep-type and has a strong magnetic field. Our observations with the X-ray Multi-Mirror (XMM-Newton) telescope reveal X-ray pulsations with the same period as the fundamental stellar oscillations. This discovery challenges our understanding of stellar winds from massive stars, their X-ray emission and their magnetism.}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Uner, E. O. Ang and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Dalton, M. and Davids, I. D. and Degrange, B. and Deil, C. and deWilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadasch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, Markus and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, M. and Janiak, M. and Jankowsky, F. and Jung-Richardt, I. and Kastendieck, M. A. and Katarzynski, K. and Katz, U. and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lau, J. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, M. and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, O. and Renaud, M. and Reyes, R. de Los and Rieger, F. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, F. and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and Van Eldik, C. and van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S. and Fukui, Y. and Sano, H. and Fukuda, T. and Yoshiike, S.}, title = {Discovery of the hard spectrum VHE gamma-ray source Hess J1641-463}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, volume = {794}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {HESS Collaboration}, issn = {2041-8205}, doi = {10.1088/2041-8205/794/1/L1}, pages = {6}, year = {2014}, abstract = {This Letter reports the discovery of a remarkably hard spectrum source, HESS J1641-463, by the High Energy Stereoscopic System (H.E.S.S.) in the very high energy (VHE) domain. HESS J1641-463 remained unnoticed by the usual analysis techniques due to confusion with the bright nearby source HESS J1640-465. It emerged at a significance level of 8.5 standard deviations after restricting the analysis to events with energies above 4 TeV. It shows a moderate flux level of phi(E > 1TeV) = (3.64 +/- 0.44(stat)+/- 0.73(sys)) x 10(-13) cm(-2) s(-1), corresponding to 1.8\% of the Crab Nebula flux above the same energy, and a hard spectrum with a photon index of Gamma = 2.07 +/- 0.11(stat)+/- 0.20(sys). It is a point-like source, although an extension up to a Gaussian width of sigma = 3 arcmin cannot be discounted due to uncertainties in the H.E.S.S. point-spread function. The VHE gamma-ray flux of HESS J1641-463 is found to be constant over the observed period when checking time binnings from the year-by-year to the 28 minute exposure timescales. HESS J1641-463 is positionally coincident with the radio supernova remnant SNR G338.5+0.1. No X-ray candidate stands out as a clear association; however, Chandra and XMM-Newton data reveal some potential weak counterparts. Various VHE gamma-ray production scenarios are discussed. If the emission from HESS J1641-463 is produced by cosmic ray protons colliding with the ambient gas, then their spectrum must extend close to 1 PeV. This object may represent a source population contributing significantly to the galactic cosmic ray flux around the knee.}, language = {en} } @article{GvaramadzeCheneKniazevetal.2014, author = {Gvaramadze, V. V. and Chene, A.-N. and Kniazev, A. Y. and Schnurr, O. and Shenar, Tomer and Sander, Andreas Alexander Christoph and Hainich, Rainer and Langer, N. and Hamann, Wolf-Rainer and Chu, Y.-H. and Gruendl, R. A.}, title = {Discovery of a new Wolf-Rayet star and a candidate star cluster in the Large Magellanic Cloud with Spitzer}, series = {Monthly notices of the Royal Astronomical Society}, volume = {442}, journal = {Monthly notices of the Royal Astronomical Society}, number = {2}, publisher = {Oxford Univ. Press}, address = {Oxford}, issn = {0035-8711}, doi = {10.1093/mnras/stu909}, pages = {929 -- 945}, year = {2014}, abstract = {We report the first-ever discovery of a Wolf-Rayet (WR) star in the Large Magellanic Cloud via detection of a circular shell with the Spitzer Space Telescope. Follow-up observations with Gemini-South resolved the central star of the shell into two components separated from each other by a parts per thousand 2 arcsec (or a parts per thousand 0.5 pc in projection). One of these components turns out to be a WN3 star with H and He lines both in emission and absorption (we named it BAT99 3a using the numbering system based on extending the Breysacher et al. catalogue). Spectroscopy of the second component showed that it is a B0 V star. Subsequent spectroscopic observations of BAT99 3a with the du Pont 2.5-m telescope and the Southern African Large Telescope revealed that it is a close, eccentric binary system, and that the absorption lines are associated with an O companion star. We analysed the spectrum of the binary system using the non-LTE Potsdam WR (powr) code, confirming that the WR component is a very hot (a parts per thousand 90 kK) WN star. For this star, we derived a luminosity of log L/ L-aS (TM) = 5.45 and a mass-loss rate of 10(- 5.8) M-aS (TM) yr(- 1), and found that the stellar wind composition is dominated by helium with 20 per cent of hydrogen. Spectroscopy of the shell revealed an He iii region centred on BAT99 3a and having the same angular radius (a parts per thousand 15 arcsec) as the shell. We thereby add a new example to a rare class of high-excitation nebulae photoionized by WR stars. Analysis of the nebular spectrum showed that the shell is composed of unprocessed material, implying that the shell was swept-up from the local interstellar medium. We discuss the physical relationship between the newly identified massive stars and their possible membership of a previously unrecognized star cluster.}, language = {en} } @article{BauerGodecMetzler2014, author = {Bauer, Maximilian and Godec, Aljaž and Metzler, Ralf}, title = {Diffusion of finite-size particles in two-dimensional channels with random wall configurations}, series = {Physical chemistry, chemical physics : PCCP ; a journal of European chemical societies}, volume = {16}, journal = {Physical chemistry, chemical physics : PCCP ; a journal of European chemical societies}, number = {13}, publisher = {RSC Publications}, address = {Cambridge}, issn = {1463-9084}, doi = {10.1039/C3CP55160A}, pages = {6118 -- 6128}, year = {2014}, abstract = {Diffusion of chemicals or tracer molecules through complex systems containing irregularly shaped channels is important in many applications. Most theoretical studies based on the famed Fick-Jacobs equation focus on the idealised case of infinitely small particles and reflecting boundaries. In this study we use numerical simulations to consider the transport of finite-size particles through asymmetrical two-dimensional channels. Additionally, we examine transient binding of the molecules to the channel walls by applying sticky boundary conditions. We consider an ensemble of particles diffusing in independent channels, which are characterised by common structural parameters. We compare our results for the long-time effective diffusion coefficient with a recent theoretical formula obtained by Dagdug and Pineda [J. Chem. Phys., 2012, 137, 024107].}, language = {en} } @misc{BauerGodecMetzler2014, author = {Bauer, Maximilian and Godec, Aljaž and Metzler, Ralf}, title = {Diffusion of finite-size particles in two-dimensional channels with random wall configurations}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-76199}, year = {2014}, abstract = {Diffusion of chemicals or tracer molecules through complex systems containing irregularly shaped channels is important in many applications. Most theoretical studies based on the famed Fick-Jacobs equation focus on the idealised case of infinitely small particles and reflecting boundaries. In this study we use numerical simulations to consider the transport of finite-size particles through asymmetrical two-dimensional channels. Additionally, we examine transient binding of the molecules to the channel walls by applying sticky boundary conditions. We consider an ensemble of particles diffusing in independent channels, which are characterised by common structural parameters. We compare our results for the long-time effective diffusion coefficient with a recent theoretical formula obtained by Dagdug and Pineda [J. Chem. Phys., 2012, 137, 024107].}, language = {en} } @article{AbramowskiAharonianBenkhalietal.2014, author = {Abramowski, Attila and Aharonian, Felix A. and Benkhali, Faical Ait and Akhperjanian, A. G. and Ang{\"u}ner, Ekrem Oǧuzhan and Backes, Michael and Balenderan, Shangkari and Balzer, Arnim and Barnacka, Anna and Becherini, Yvonne and Tjus, J. Becker and Berge, David and Bernhard, Sabrina and Bernl{\"o}hr, K. and Birsin, E. and Biteau, Jonathan and Boettcher, Markus and Boisson, Catherine and Bolmont, J. and Bordas, Pol and Bregeon, Johan and Brun, Francois and Brun, Pierre and Bryan, Mark and Bulik, Tomasz and Carrigan, Svenja and Casanova, Sabrina and Chadwick, Paula M. and Chakraborty, N. and Chalme-Calvet, R. and Chaves, Ryan C. G. and Chretien, M. and Colafrancesco, Sergio and Cologna, Gabriele and Conrad, Jan and Couturier, C. and Cui, Y. and Davids, I. D. and Degrange, B. and Deil, C. and dewilt, P. and Djannati-Ata{\"i}, A. and Domainko, W. and Donath, A. and Dubus, G. and Dutson, K. and Dyks, J. and Dyrda, M. and Edwards, T. and Egberts, Kathrin and Eger, P. and Espigat, P. and Farnier, C. and Fegan, S. and Feinstein, F. and Fernandes, M. V. and Fernandez, D. and Fiasson, A. and Fontaine, G. and Foerster, A. and Fuessling, M. and Gabici, S. and Gajdus, M. and Gallant, Y. A. and Garrigoux, T. and Giavitto, G. and Giebels, B. and Glicenstein, J. F. and Gottschall, D. and Grondin, M. -H. and Grudzinska, M. and Hadasch, D. and Haeffner, S. and Hahn, J. and Harris, J. and Heinzelmann, G. and Henri, G. and Hermann, G. and Hervet, O. and Hillert, A. and Hinton, James Anthony and Hofmann, W. and Hofverberg, P. and Holler, M. and Horns, D. and Ivascenko, A. and Jacholkowska, A. and Jahn, C. and Jamrozy, Marek and Janiak, M. and Jankowsky, F. and Jung-Richardt, I. and Kastendieck, M. A. and Katarzynski, Krzysztof and Katz, Uli and Kaufmann, S. and Khelifi, B. and Kieffer, M. and Klepser, S. and Klochkov, D. and Kluzniak, W. and Kolitzus, D. and Komin, Nu. and Kosack, K. and Krakau, S. and Krayzel, F. and Krueger, P. P. and Laffon, H. and Lamanna, G. and Lefaucheur, J. and Lefranc, V. and Lemiere, A. and Lemoine-Goumard, M. and Lenain, J. -P. and Lohse, T. and Lopatin, A. and Lu, C. -C. and Marandon, V. and Marcowith, Alexandre and Marx, R. and Maurin, G. and Maxted, N. and Mayer, M. and McComb, T. J. L. and Mehault, J. and Meintjes, P. J. and Menzler, U. and Meyer, M. and Mitchell, A. M. W. and Moderski, R. and Mohamed, M. and Mora, K. and Moulin, Emmanuel and Murach, T. and de Naurois, M. and Niemiec, J. and Nolan, S. J. and Oakes, L. and Odaka, H. and Ohm, S. and Opitz, B. and Ostrowski, M. and Oya, I. and Panter, M. and Parsons, R. D. and Arribas, M. Paz and Pekeur, N. W. and Pelletier, G. and Petrucci, P. -O. and Peyaud, B. and Pita, S. and Poon, H. and Puehlhofer, G. and Punch, Michael and Quirrenbach, A. and Raab, S. and Reichardt, I. and Reimer, A. and Reimer, Olaf and Renaud, M. and de los Reyes, R. and Rieger, F. and Romoli, C. and Rosier-Lees, S. and Rowell, G. and Rudak, B. and Rulten, C. B. and Sahakian, V. and Salek, D. and Sanchez, David M. and Santangelo, Andrea and Schlickeiser, R. and Schuessler, Fabian and Schulz, A. and Schwanke, U. and Schwarzburg, S. and Schwemmer, S. and Sol, H. and Spanier, F. and Spengler, G. and Spies, F. and Stawarz, L. and Steenkamp, R. and Stegmann, Christian and Stinzing, F. and Stycz, K. and Sushch, Iurii and Tavernet, J. -P. and Tavernier, T. and Taylor, A. M. and Terrier, R. and Tluczykont, M. and Trichard, C. and Valerius, K. and van Eldik, Christopher and van Soelen, B. and Vasileiadis, G. and Veh, J. and Venter, C. and Viana, A. and Vincent, P. and Vink, J. and Voelk, H. J. and Volpe, F. and Vorster, M. and Vuillaume, T. and Wagner, S. J. and Wagner, P. and Wagner, R. M. and Ward, M. and Weidinger, M. and Weitzel, Q. and White, R. and Wierzcholska, A. and Willmann, P. and Woernlein, A. and Wouters, D. and Yang, R. and Zabalza, V. and Zaborov, D. and Zacharias, M. and Zdziarski, A. A. and Zech, Alraune and Zechlin, H. -S. and Fukui, Y.}, title = {Diffuse Galactic gamma-ray emission with HESS}, series = {Physical review : D, Particles, fields, gravitation, and cosmology}, volume = {90}, journal = {Physical review : D, Particles, fields, gravitation, and cosmology}, number = {12}, publisher = {American Physical Society}, address = {College Park}, organization = {HESS Collaboration}, issn = {1550-7998}, doi = {10.1103/PhysRevD.90.122007}, pages = {8}, year = {2014}, abstract = {Diffuse gamma-ray emission is the most prominent observable signature of celestial cosmic-ray interactions at high energies. While already being investigated at GeVenergies over several decades, assessments of diffuse gamma-ray emission at TeVenergies remain sparse. After completion of the systematic survey of the inner Galaxy, the H.E.S.S. experiment is in a prime position to observe large-scale diffuse emission at TeVenergies. Data of the H.E.S.S. Galactic Plane Survey are investigated in regions off known gamma-ray sources. Corresponding gamma-ray flux measurements were made over an extensive grid of celestial locations. Longitudinal and latitudinal profiles of the observed gamma-ray fluxes show characteristic excess emission not attributable to known gamma-ray sources. For the first time large-scale gamma-ray emission along the Galactic plane using imaging atmospheric Cherenkov telescopes has been observed. While the background subtraction technique limits the ability to recover modest variation on the scale of the H.E.S.S. field of view or larger, which is characteristic of the inverse Compton scatter-induced Galactic diffuse emission, contributions of neutral pion decay as well as emission from unresolved gamma-ray sources can be recovered in the observed signal to a large fraction. Calculations show that the minimum gamma-ray emission from pi(0) decay represents a significant contribution to the total signal. This detection is interpreted as a mix of diffuse Galactic gamma-ray emission and unresolved sources.}, language = {en} } @article{GhoshCherstvyMetzler2014, author = {Ghosh, Surya K. and Cherstvy, Andrey G. and Metzler, Ralf}, title = {Deformation propagation in responsive polymer network films}, series = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, volume = {141}, journal = {The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr}, number = {7}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0021-9606}, doi = {10.1063/1.4893056}, pages = {9}, year = {2014}, abstract = {We study the elastic deformations in a cross-linked polymer network film triggered by the binding of submicron particles with a sticky surface, mimicking the interactions of viral pathogens with thin films of stimulus-responsive polymeric materials such as hydrogels. From extensive Langevin Dynamics simulations we quantify how far the network deformations propagate depending on the elasticity parameters of the network and the adhesion strength of the particles. We examine the dynamics of the collective area shrinkage of the network and obtain some simple relations for the associated characteristic decay lengths. A detailed analysis elucidates how the elastic energy of the network is distributed between stretching and compression modes in response to the particle binding. We also examine the force-distance curves of the repulsion or attraction interactions for a pair of sticky particles in the polymer network film as a function of the particle-particle separation. The results of this computational study provide new insight into collective phenomena in soft polymer network films and may, in particular, be applied to applications for visual detection of pathogens such as viruses via a macroscopic response of thin films of cross-linked hydrogels. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{ArchambaultAuneBeheraetal.2014, author = {Archambault, S. and Aune, T. and Behera, B. and Beilicke, M. and Benbow, W. and Berger, K. and Bird, R. and Biteau, Jonathan and Bugaev, V. and Byrum, K. and Cardenzana, J. V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Connolly, M. P. and Cui, Wei and Dumm, J. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Kumar, S. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McCann, A. and Meagher, K. and Moriarty, P. and Mukherjee, R. and Nieto, Daniel and Ong, R. A. and Otte, A. N. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sembroski, G. H. and Shahinyan, K. and Staszak, D. and Telezhinsky, Igor O. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Ackermann, Margit and Ajello, M. and Albert, A. and Baldini, L. and Bastieri, D. and Bellazzini, R. and Bissaldi, E. and Bregeon, Johan and Buehler, R. and Buson, S. and Caliandro, G. A. and Cameron, R. A. and Caraveo, P. A. and Cavazzuti, E. and Charles, E. and Chiang, J. and Ciprini, S. and Claus, R. and Cutini, S. and de Angelis, A. and de Palma, F. and Dermer, C. D. and Digel, S. W. and Di Venere, L. and Drell, P. S. and Favuzzi, C. and Franckowiak, A. and Fusco, P. and Gargano, F. and Gasparrini, D. and Giglietto, N. and Giordano, F. and Giroletti, M. and Grenier, I. A. and Guiriec, S. and Jogler, T. and Kuss, M. and Larsson, S. and Latronico, L. and Longo, F. and Loparco, F. and Lubrano, P. and Madejski, G. M. and Mayer, M. and Mazziotta, Mario Nicola and Michelson, P. F. and Mizuno, T. and Monzani, M. E. and Morselli, Aldo and Murgia, S. and Nuss, E. and Ohsugi, T. and Ormes, J. F. and Paneque, D. and Perkins, J. S. and Piron, F. and Pivato, G. and Raino, S. and Razzano, M. and Reimer, A. and Reimer, Olaf and Ritz, S. and Schaal, M. and Sgro, C. and Siskind, E. J. and Spinelli, P. and Takahashi, H. and Tibaldo, L. and Tinivella, M. and Troja, E. and Vianello, G. and Werner, M. and Wood, M.}, title = {Deep broadband observations of the distant gamma-ray blazar PKS 1424+240}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, volume = {785}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, organization = {VERITAS Collaboration, Fermi LAT Collaboration}, issn = {2041-8205}, doi = {10.1088/2041-8205/785/1/L16}, pages = {8}, year = {2014}, abstract = {We present deep VERITAS observations of the blazar PKS 1424+240, along with contemporaneous Fermi Large Area Telescope, Swift X-ray Telescope, and Swift UV Optical Telescope data between 2009 February 19 and 2013 June 8. This blazar resides at a redshift of z >= 0.6035, displaying a significantly attenuated gamma-ray flux above 100 GeV due to photon absorption via pair-production with the extragalactic background light. We present more than 100 hr of VERITAS observations over three years, a multiwavelength light curve, and the contemporaneous spectral energy distributions. The source shows a higher flux of (2.1 +/- 0.3) x 10(-7) photons m(-2) s(-1) above 120 GeV in 2009 and 2011 as compared to the flux measured in 2013, corresponding to (1.02 +/- 0.08) x 10-7 photons m(-2) s(-1) above 120 GeV. The measured differential very high energy (VHE; E >= 100 GeV) spectral indices are Gamma = 3.8 +/- 0.3, 4.3 +/- 0.6 and 4.5 +/- 0.2 in 2009, 2011, and 2013, respectively. No significant spectral change across the observation epochs is detected. We find no evidence for variability at gamma-ray opacities of greater than tau = 2, where it is postulated that any variability would be small and occur on timescales longer than a year if hadronic cosmic-ray interactions with extragalactic photon fields provide a secondary VHE photon flux. The data cannot rule out such variability due to low statistics.}, language = {en} } @article{deCarvalhoMetzlerCherstvy2014, author = {de Carvalho, Sidney J. and Metzler, Ralf and Cherstvy, Andrey G.}, title = {Critical adsorption of polyelectrolytes onto charged Janus nanospheres}, series = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, volume = {16}, journal = {Physical chemistry, chemical physics : a journal of European Chemical Societies}, number = {29}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, issn = {1463-9076}, doi = {10.1039/c4cp02207f}, pages = {15539 -- 15550}, year = {2014}, abstract = {Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two equally but oppositely charged hemispheres. The critical binding conditions for polyelectrolyte chains are analysed as function of the radius of the Janus particle and its surface charge density, as well as the salt concentration in the ambient solution. Specifically for the adsorption of finite-length polyelectrolyte chains onto Janus nanoparticles, we demonstrate that the critical adsorption conditions drastically differ when the size of the Janus particle or the screening length of the electrolyte are varied. We compare the scaling laws obtained for the adsorption-desorption threshold to the known results for uniformly charged spherical particles, observing significant disparities. We also contrast the changes to the polyelectrolyte chain conformations close to the surface of the Janus nanoparticles as compared to those for simple spherical particles. Finally, we discuss experimentally relevant physicochemical systems for which our simulations results may become important. In particular, we observe similar trends with polyelectrolyte complexation with oppositely but heterogeneously charged proteins.}, language = {en} } @misc{deCarvalhoMetzlerCherstvy2014, author = {de Carvalho, Sidney J. and Metzler, Ralf and Cherstvy, Andrey G.}, title = {Critical adsorption of polyelectrolytes onto charged Janus nanospheres}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-98783}, pages = {12}, year = {2014}, abstract = {Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two equally but oppositely charged hemispheres. The critical binding conditions for polyelectrolyte chains are analysed as function of the radius of the Janus particle and its surface charge density, as well as the salt concentration in the ambient solution. Specifically for the adsorption of finite-length polyelectrolyte chains onto Janus nanoparticles, we demonstrate that the critical adsorption conditions drastically differ when the size of the Janus particle or the screening length of the electrolyte are varied. We compare the scaling laws obtained for the adsorption-desorption threshold to the known results for uniformly charged spherical particles, observing significant disparities. We also contrast the changes to the polyelectrolyte chain conformations close to the surface of the Janus nanoparticles as compared to those for simple spherical particles. Finally, we discuss experimentally relevant physico-chemical systems for which our simulations results may become important. In particular, we observe similar trends with polyelectrolyte complexation with oppositely but heterogeneously charged proteins.}, language = {en} } @phdthesis{Balzer2014, author = {Balzer, Arnim}, title = {Crab flare observations with H.E.S.S. phase II}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-72545}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {The H.E.S.S. array is a third generation Imaging Atmospheric Cherenkov Telescope (IACT) array. It is located in the Khomas Highland in Namibia, and measures very high energy (VHE) gamma-rays. In Phase I, the array started data taking in 2004 with its four identical 13 m telescopes. Since then, H.E.S.S. has emerged as the most successful IACT experiment to date. Among the almost 150 sources of VHE gamma-ray radiation found so far, even the oldest detection, the Crab Nebula, keeps surprising the scientific community with unexplained phenomena such as the recently discovered very energetic flares of high energy gamma-ray radiation. During its most recent flare, which was detected by the Fermi satellite in March 2013, the Crab Nebula was simultaneously observed with the H.E.S.S. array for six nights. The results of the observations will be discussed in detail during the course of this work. During the nights of the flare, the new 24 m × 32 m H.E.S.S. II telescope was still being commissioned, but participated in the data taking for one night. To be able to reconstruct and analyze the data of the H.E.S.S. Phase II array, the algorithms and software used by the H.E.S.S. Phase I array had to be adapted. The most prominent advanced shower reconstruction technique developed by de Naurois and Rolland, the template-based model analysis, compares real shower images taken by the Cherenkov telescope cameras with shower templates obtained using a semi-analytical model. To find the best fitting image, and, therefore, the relevant parameters that describe the air shower best, a pixel-wise log-likelihood fit is done. The adaptation of this advanced shower reconstruction technique to the heterogeneous H.E.S.S. Phase II array for stereo events (i.e. air showers seen by at least two telescopes of any kind), its performance using MonteCarlo simulations as well as its application to real data will be described.}, language = {en} } @article{SandevMetzlerTomovski2014, author = {Sandev, Trifce and Metzler, Ralf and Tomovski, Zivorad}, title = {Correlation functions for the fractional generalized Langevin equation in the presence of internal and external noise}, series = {Journal of mathematical physics}, volume = {55}, journal = {Journal of mathematical physics}, number = {2}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0022-2488}, doi = {10.1063/1.4863478}, pages = {23}, year = {2014}, abstract = {We study generalized fractional Langevin equations in the presence of a harmonic potential. General expressions for the mean velocity and particle displacement, the mean squared displacement, position and velocity correlation functions, as well as normalized displacement correlation function are derived. We report exact results for the cases of internal and external friction, that is, when the driving noise is either internal and thus the fluctuation-dissipation relation is fulfilled or when the noise is external. The asymptotic behavior of the generalized stochastic oscillator is investigated, and the case of high viscous damping (overdamped limit) is considered. Additional behaviors of the normalized displacement correlation functions different from those for the regular damped harmonic oscillator are observed. In addition, the cases of a constant external force and the force free case are obtained. The validity of the generalized Einstein relation for this process is discussed. The considered fractional generalized Langevin equation may be used to model anomalous diffusive processes including single file-type diffusion.}, language = {en} } @article{SchubertCollinsMangoldetal.2014, author = {Schubert, Marcel and Collins, Brian A. and Mangold, Hannah and Howard, Ian A. and Schindler, Wolfram and Vandewal, Koen and Roland, Steffen and Behrends, Jan and Kraffert, Felix and Steyrleuthner, Robert and Chen, Zhihua and Fostiropoulos, Konstantinos and Bittl, Robert and Salleo, Alberto and Facchetti, Antonio and Laquai, Frederic and Ade, Harald W. and Neher, Dieter}, title = {Correlated donor/acceptor crystal orientation controls photocurrent generation in all-polymer solar cells}, series = {Advanced functional materials}, volume = {24}, journal = {Advanced functional materials}, number = {26}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {1616-301X}, doi = {10.1002/adfm.201304216}, pages = {4068 -- 4081}, year = {2014}, abstract = {New polymers with high electron mobilities have spurred research in organic solar cells using polymeric rather than fullerene acceptors due to their potential of increased diversity, stability, and scalability. However, all-polymer solar cells have struggled to keep up with the steadily increasing power conversion efficiency of polymer: fullerene cells. The lack of knowledge about the dominant recombination process as well as the missing concluding picture on the role of the semi-crystalline microstructure of conjugated polymers in the free charge carrier generation process impede a systematic optimization of all-polymer solar cells. These issues are examined by combining structural and photo-physical characterization on a series of poly(3-hexylthiophene) (donor) and P(NDI2OD-T2) (acceptor) blend devices. These experiments reveal that geminate recombination is the major loss channel for photo-excited charge carriers. Advanced X-ray and electron-based studies reveal the effect of chloronaphthalene co-solvent in reducing domain size, altering domain purity, and reorienting the acceptor polymer crystals to be coincident with those of the donor. This reorientation correlates well with the increased photocurrent from these devices. Thus, effi cient split-up of geminate pairs at polymer/polymer interfaces may necessitate correlated donor/acceptor crystal orientation, which represents an additional requirement compared to the isotropic fullerene acceptors.}, language = {en} } @article{vanDrielGesztelyiBakerToeroeketal.2014, author = {van Driel-Gesztelyi, L. and Baker, Daniel N. and Toeroek, T. and Pariat, E. and Green, L. M. and Williams, D. R. and Carlyle, J. and Valori, G. and Demoulin, Pascal and Kliem, Bernhard and Long, D. M. and Matthews, S. A. and Malherbe, J. -M.}, title = {Coronal magnetic reconnection driven by CME expansion-the 2011 June 7 event}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {788}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/788/1/85}, pages = {12}, year = {2014}, abstract = {Coronal mass ejections (CMEs) erupt and expand in a magnetically structured solar corona. Various indirect observational pieces of evidence have shown that the magnetic field of CMEs reconnects with surrounding magnetic fields, forming, e.g., dimming regions distant from the CME source regions. Analyzing Solar Dynamics Observatory (SDO) observations of the eruption from AR 11226 on 2011 June 7, we present the first direct evidence of coronal magnetic reconnection between the fields of two adjacent active regions during a CME. The observations are presented jointly with a data-constrained numerical simulation, demonstrating the formation/intensification of current sheets along a hyperbolic flux tube at the interface between the CME and the neighboring AR 11227. Reconnection resulted in the formation of new magnetic connections between the erupting magnetic structure from AR 11226 and the neighboring active region AR 11227 about 200 Mm from the eruption site. The onset of reconnection first becomes apparent in the SDO/AIA images when filament plasma, originally contained within the erupting flux rope, is redirected toward remote areas in AR 11227, tracing the change of large-scale magnetic connectivity. The location of the coronal reconnection region becomes bright and directly observable at SDO/AIA wavelengths, owing to the presence of down-flowing cool, dense (1010 cm(-3)) filament plasma in its vicinity. The high-density plasma around the reconnection region is heated to coronal temperatures, presumably by slow-mode shocks and Coulomb collisions. These results provide the first direct observational evidence that CMEs reconnect with surrounding magnetic structures, leading to a large-scale reconfiguration of the coronal magnetic field.}, language = {en} } @article{BeimGraben2014, author = {Beim Graben, Peter}, title = {Contextual emergence of intentionality}, series = {Journal of consciousness studies : controversies in science \& the humanities ; an international multi-disciplinary journal}, volume = {21}, journal = {Journal of consciousness studies : controversies in science \& the humanities ; an international multi-disciplinary journal}, number = {5-6}, publisher = {Imprint Academic}, address = {Exeter}, issn = {1355-8250}, pages = {75 -- 96}, year = {2014}, abstract = {By means of an intriguing physical example, magnetic surface swimmers, that can be described in terms of Dennett's intentional stance, I reconstruct a hierarchy of necessary and sufficient conditions for the applicability of the intentional strategy. It turns out that the different levels of the intentional hierarchy are contextually emergent from their respective subjacent levels by imposing stability constraints upon them. At the lowest level of the hierarchy, phenomenal physical laws emerge for the coarse-grained description of open, nonlinear, and dissipative non-equilibrium systems in critical states. One level higher, dynamic patterns, such as, for example, magnetic surface swimmers, are contextually emergent as they are invariant under certain symmetry operations. Again one level up, these patterns behave apparently rationally by selecting optimal pathways for the dissipation of energy that is delivered by external gradients. This is in accordance with the restated Second Law of thermodynamics as a stability criterion. At the highest level, true believers are intentional systems that are stable under exchanging their observation conditions.}, language = {en} } @phdthesis{Steinhaus2014, author = {Steinhaus, Sebastian Peter}, title = {Constructing quantum spacetime}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus-72558}, school = {Universit{\"a}t Potsdam}, year = {2014}, abstract = {Despite remarkable progress made in the past century, which has revolutionized our understanding of the universe, there are numerous open questions left in theoretical physics. Particularly important is the fact that the theories describing the fundamental interactions of nature are incompatible. Einstein's theory of general relative describes gravity as a dynamical spacetime, which is curved by matter and whose curvature determines the motion of matter. On the other hand we have quantum field theory, in form of the standard model of particle physics, where particles interact via the remaining interactions - electromagnetic, weak and strong interaction - on a flat, static spacetime without gravity. A theory of quantum gravity is hoped to cure this incompatibility by heuristically replacing classical spacetime by quantum spacetime'. Several approaches exist attempting to define such a theory with differing underlying premises and ideas, where it is not clear which is to be preferred. Yet a minimal requirement is the compatibility with the classical theory, they attempt to generalize. Interestingly many of these models rely on discrete structures in their definition or postulate discreteness of spacetime to be fundamental. Besides the direct advantages discretisations provide, e.g. permitting numerical simulations, they come with serious caveats requiring thorough investigation: In general discretisations break fundamental diffeomorphism symmetry of gravity and are generically not unique. Both complicates establishing the connection to the classical continuum theory. The main focus of this thesis lies in the investigation of this relation for spin foam models. This is done on different levels of the discretisation / triangulation, ranging from few simplices up to the continuum limit. In the regime of very few simplices we confirm and deepen the connection of spin foam models to discrete gravity. Moreover, we discuss dynamical, e.g. diffeomorphism invariance in the discrete, to fix the ambiguities of the models. In order to satisfy these conditions, the discrete models have to be improved in a renormalisation procedure, which also allows us to study their continuum dynamics. Applied to simplified spin foam models, we uncover a rich, non--trivial fixed point structure, which we summarize in a phase diagram. Inspired by these methods, we propose a method to consistently construct the continuum theory, which comes with a unique vacuum state.}, language = {en} } @article{AliuAuneBarnackaetal.2014, author = {Aliu, E. and Aune, T. and Barnacka, Anna and Beilicke, M. and Benbow, W. and Berger, K. and Biteau, Jonathan and Buckley, J. H. and Bugaev, V. and Byrum, K. and Cardenzana, J. V. and Cerruti, M. and Chen, Xuhui and Ciupik, L. and Connaughton, V. and Cui, W. and Dickinson, H. J. and Eisch, J. D. and Errando, M. and Falcone, A. and Federici, Simone and Feng, Q. and Finley, J. P. and Fleischhack, H. and Fortin, P. and Fortson, L. and Furniss, A. and Galante, N. and Gillanders, G. H. and Griffin, S. and Griffiths, S. T. and Grube, J. and Gyuk, G. and Hakansson, Nils and Hanna, D. and Holder, J. and Hughes, G. and Humensky, T. B. and Johnson, C. A. and Kaaret, P. and Kar, P. and Kertzman, M. and Khassen, Y. and Kieda, D. and Krawczynski, H. and Krennrich, F. and Lang, M. J. and Madhavan, A. S. and Maier, G. and McArthur, S. and McCann, A. and Meagher, K. and Millis, J. and Moriarty, P. and Mukherjee, R. and Nieto, D. and Ong, R. A. and Otte, A. N. and Park, N. and Pohl, Martin and Popkow, A. and Prokoph, H. and Pueschel, Elisa and Quinn, J. and Ragan, K. and Rajotte, J. and Reyes, L. C. and Reynolds, P. T. and Richards, G. T. and Roache, E. and Sembroski, G. H. and Shahinyan, K. and Smith, A. W. and Staszak, D. and Telezhinsky, Igor O. and Tucci, J. V. and Tyler, J. and Varlotta, A. and Vassiliev, V. V. and Vincent, S. and Wakely, S. P. and Weiner, O. M. and Weinstein, A. and Welsing, R. and Wilhelm, Alina and Williams, D. A. and Zitzer, B. and McEnery, J. E. and Perkins, J. S. and Veres, P. and Zhu, S.}, title = {Constraints on very high energy emission from GRB 130427A}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, volume = {795}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {2041-8205}, doi = {10.1088/2041-8205/795/1/L3}, pages = {6}, year = {2014}, abstract = {Prompt emission from the very fluent and nearby (z = 0.34) gamma-ray burst GRB130427A was detected by several orbiting telescopes and by ground-based, wide-field-of-view optical transient monitors. Apart from the intensity and proximity of this GRB, it is exceptional due to the extremely long-lived high-energy (100 MeV to 100 GeV) gamma-ray emission, which was detected by the Large Area Telescope on the Fermi Gamma-Ray Space Telescope for similar to 70 ks after the initial burst. The persistent, hard-spectrum, high-energy emission suggests that the highest-energy gamma rays may have been produced via synchrotron self-Compton processes though there is also evidence that the high-energy emission may instead be an extension of the synchrotron spectrum. VERITAS, a ground-based imaging atmospheric Cherenkov telescope array, began follow-up observations of GRB130427A similar to 71 ks (similar to 20 hr) after the onset of the burst. The GRB was not detected with VERITAS; however, the high elevation of the observations, coupled with the low redshift of the GRB, make VERITAS a very sensitive probe of the emission from GRB130427A for E > 100 GeV. The non-detection and consequent upper limit derived place constraints on the synchrotron self-Compton model of high-energy gamma-ray emission from this burst.}, language = {en} } @article{Wendt2014, author = {Wendt, Martin}, title = {Constraints on variations of m(p)/m(e) based on UVES observations of H-2}, series = {Astronomische Nachrichten = Astronomical notes}, volume = {335}, journal = {Astronomische Nachrichten = Astronomical notes}, number = {1}, publisher = {Wiley-VCH}, address = {Weinheim}, issn = {0004-6337}, doi = {10.1002/asna.201312008}, pages = {106 -- 112}, year = {2014}, abstract = {This article summarizes the latest results on the proton-to-electron mass ratio derived from H-2 observations at high redshift in the light of possible variations of fundamental physical constants. The focus lies on UVES observations of the past years as enormous progress was achieved since the first positive results on / were published. With the better understanding of systematics, dedicated observation runs, and numerous approaches to improve wavelength calibration accuracy, all current findings are in reasonable good agreement with no variation and provide an upper limit of / < 1 x 10(-5) for the redshift range of 2 < z < 3. ((}, language = {en} }