@misc{Steiglechner2018, type = {Master Thesis}, author = {Steiglechner, Peter}, title = {Estimating global warming from anthropogenic heat emissions}, doi = {10.25932/publishup-49886}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-498866}, school = {Universit{\"a}t Potsdam}, year = {2018}, abstract = {The forcing from the anthropogenic heat flux (AHF), i.e. the dissipation of primary energy consumed by the human civilisation, produces a direct climate warming. Today, the globally averaged AHF is negligibly small compared to the indirect forcing from greenhouse gas emissions. Locally or regionally, though, it has a significant impact. Historical observations show a constant exponential growth of worldwide energy production. A continuation of this trend might be fueled or even amplified by the exploration of new carbon-free energy sources like fusion power. In such a scenario, the impacts of the AHF become a relevant factor for anthropogenic post-greenhouse gas climate change on the global scale, as well. This master thesis aims at estimating the climate impacts of such a growing AHF forcing. In the first part of this work, the AHF is built into simple and conceptual, zero- and one-dimensional Energy Balance Models (EBMs), providing quick order of magnitude estimations of the temperature impact. In the one-dimensional EBM, the ice-albedo feedback from enhanced ice melting due to the AHF increases the temperature impact significantly compared to the zero-dimensional EBM. Additionally, the forcing is built into a climate model of intermediate complexity, CLIMBER-3α. This allows for the investigation of the effect of localised AHF and gives further insights into the impact of the AHF on processes like the ocean heat uptake, sea ice and snow pattern changes and the ocean circulation. The global mean temperature response from the AHF today is of the order of 0.010 - 0.016 K in all reasonable model configurations tested. A transient tenfold increase of this forcing heats up the Earth System additionally by roughly 0.1 - 0.2 K in the presented models. Further growth can also affect the tipping probability of certain climate elements. Most renewable energy sources do not or only partially contribute to the AHF forcing as the energy from these sources dissipates anyway. Hence, the transition to a (carbon-free) renewable energy mix, which, in particular, does not rely on nuclear power, eliminates the local and global climate impacts from the increasing AHF forcing, independent of the growth of energy production.}, language = {en} } @misc{ReindlFinchSchaffenrothetal.2018, author = {Reindl, Nicole and Finch, Nicolle L. and Schaffenroth, Veronika and Barstow, Martin A. and Casewell, Sarah L. and Geier, Stephan Alfred and Bertolami Miller, Marcelo Miguel and Taubenberger, Stefan}, title = {Revealing the true nature of Hen2-428}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {1129}, issn = {1866-8372}, doi = {10.25932/publishup-45970}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-459703}, pages = {9}, year = {2018}, abstract = {The nucleus of Hen 2-428 is a short orbital period (4.2 h) spectroscopic binary, whose status as potential supernovae type Ia progenitor has raised some controversy in the literature. We present preliminary results of a thorough analysis of this interesting system, which combines quantitative non-local thermodynamic (non-LTE) equilibrium spectral modelling, radial velocity analysis, multi-band light curve fitting, and state-of-the art stellar evolutionary calculations. Importantly, we find that the dynamical system mass that is derived by using all available He II lines does not exceed the Chandrasekhar mass limit. Furthermore, the individual masses of the two central stars are too small to lead to an SN Ia in case of a dynamical explosion during the merger process.}, language = {en} } @misc{ShanGuanHubaceketal.2018, author = {Shan, Yuli and Guan, Dabo and Hubacek, Klaus and Zheng, Bo and Davis, Steven J. and Jia, Lichao and Liu, Jianghua and Liu, Zhu and Fromer, Neil and Mi, Zhifu and Meng, Jing and Deng, Xiangzheng and Li, Yuan and Lin, Jintai and Schroeder, Heike and Weisz, Helga and Schellnhuber, Hans Joachim}, title = {City-level climate change mitigation in China}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {1096}, issn = {1866-8372}, doi = {10.25932/publishup-47154}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-471541}, pages = {18}, year = {2018}, abstract = {As national efforts to reduce CO2 emissions intensify, policy-makers need increasingly specific, subnational information about the sources of CO2 and the potential reductions and economic implications of different possible policies. This is particularly true in China, a large and economically diverse country that has rapidly industrialized and urbanized and that has pledged under the Paris Agreement that its emissions will peak by 2030. We present new, city level estimates of CO2 emissions for 182 Chinese cities, decomposed into 17 different fossil fuels, 46 socioeconomic sectors, and 7 industrial processes. We find that more affluent cities have systematically lower emissions per unit of gross domestic product (GDP), supported by imports from less affluent, industrial cities located nearby. In turn, clusters of industrial cities are supported by nearby centers of coal or oil extraction. Whereas policies directly targeting manufacturing and electric power infrastructure would drastically undermine the GDP of industrial cities, consumption based policies might allow emission reductions to be subsidized by those with greater ability to pay. In particular, sector based analysis of each city suggests that technological improvements could be a practical and effective means of reducing emissions while maintaining growth and the current economic structure and energy system. We explore city-level emission reductions under three scenarios of technological progress to show that substantial reductions (up to 31\%) are possible by updating a disproportionately small fraction of existing infrastructure.}, language = {en} } @misc{WoodfieldHorneGlauertetal.2018, author = {Woodfield, Emma E. and Horne, Richard B. and Glauert, Sarah A. and Menietti, John D. and Shprits, Yuri Y. and Kurth, William S.}, title = {Formation of electron radiation belts at Saturn by Z-mode wave acceleration}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {1032}, issn = {1866-8372}, doi = {10.25932/publishup-46834}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-468342}, pages = {9}, year = {2018}, abstract = {At Saturn electrons are trapped in the planet's magnetic field and accelerated to relativistic energies to form the radiation belts, but how this dramatic increase in electron energy occurs is still unknown. Until now the mechanism of radial diffusion has been assumed but we show here that in-situ acceleration through wave particle interactions, which initial studies dismissed as ineffectual at Saturn, is in fact a vital part of the energetic particle dynamics there. We present evidence from numerical simulations based on Cassini spacecraft data that a particular plasma wave, known as Z-mode, accelerates electrons to MeV energies inside 4 R-S (1 R-S = 60,330 km) through a Doppler shifted cyclotron resonant interaction. Our results show that the Z-mode waves observed are not oblique as previously assumed and are much better accelerators than O-mode waves, resulting in an electron energy spectrum that closely approaches observed values without any transport effects included.}, language = {en} } @misc{BouchouleSchemmerHenkel2018, author = {Bouchoule, Isabelle and Schemmer, Max and Henkel, Carsten}, title = {Cooling phonon modes of a Bose condensate with uniform few body losses}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {1029}, issn = {1866-8372}, doi = {10.25932/publishup-46881}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-468811}, pages = {20}, year = {2018}, abstract = {We present a general analysis of the cooling produced by losses on condensates or quasi-condensates. We study how the occupations of the collective phonon modes evolve in time, assuming that the loss process is slow enough so that each mode adiabatically follows the decrease of the mean density. The theory is valid for any loss process whose rate is proportional to the jth power of the density, but otherwise spatially uniform. We cover both homogeneous gases and systems confined in a smooth potential. For a low-dimensional gas, we can take into account the modified equation of state due to the broadening of the cloud width along the tightly confined directions, which occurs for large interactions. We find that at large times, the temperature decreases proportionally to the energy scale mc2, where m is the mass of the particles and c the sound velocity. We compute the asymptotic ratio of these two quantities for different limiting cases: a homogeneous gas in any dimension and a one-dimensional gas in a harmonic trap.}, language = {en} } @misc{RisbeyLewandowskyCowtanetal.2018, author = {Risbey, James S. and Lewandowsky, Stephan and Cowtan, Kevin and Oreskes, Naomi and Rahmstorf, Stefan and Jokim{\"a}ki, Ari and Foster, Grant}, title = {A fluctuation in surface temperature in historical context}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, volume = {13}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {1023}, issn = {1866-8372}, doi = {10.25932/publishup-46804}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-468041}, pages = {26}, year = {2018}, abstract = {This work reviews the literature on an alleged global warming 'pause' in global mean surface temperature (GMST) to determine how it has been defined, what time intervals are used to characterise it, what data are used to measure it, and what methods used to assess it. We test for 'pauses', both in the normally understood meaning of the term to mean no warming trend, as well as for a 'pause' defined as a substantially slower trend in GMST. The tests are carried out with the historical versions of GMST that existed for each pause-interval tested, and with current versions of each of the GMST datasets. The tests are conducted following the common (but questionable) practice of breaking the linear fit at the start of the trend interval ('broken' trends), and also with trends that are continuous with the data bordering the trend interval. We also compare results when appropriate allowance is made for the selection bias problem. The results show that there is little or no statistical evidence for a lack of trend or slower trend in GMST using either the historical data or the current data. The perception that there was a 'pause' in GMST was bolstered by earlier biases in the data in combination with incomplete statistical testing.}, language = {en} } @misc{AlonsoStangeBeta2018, author = {Alonso, Sergio and Stange, Maike and Beta, Carsten}, title = {Modeling random crawling, membrane deformation and intracellular polarity of motile amoeboid cells}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch Naturwissenschaftliche Reihe}, number = {1014}, issn = {1866-8372}, doi = {10.25932/publishup-45974}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-459745}, pages = {24}, year = {2018}, abstract = {Amoeboid movement is one of the most widespread forms of cell motility that plays a key role in numerous biological contexts. While many aspects of this process are well investigated, the large cell-to-cell variability in the motile characteristics of an otherwise uniform population remains an open question that was largely ignored by previous models. In this article, we present a mathematical model of amoeboid motility that combines noisy bistable kinetics with a dynamic phase field for the cell shape. To capture cell-to-cell variability, we introduce a single parameter for tuning the balance between polarity formation and intracellular noise. We compare numerical simulations of our model to experiments with the social amoeba Dictyostelium discoideum. Despite the simple structure of our model, we found close agreement with the experimental results for the center-of-mass motion as well as for the evolution of the cell shape and the overall intracellular patterns. We thus conjecture that the building blocks of our model capture essential features of amoeboid motility and may serve as a starting point for more detailed descriptions of cell motion in chemical gradients and confined environments.}, language = {en} } @misc{MannRahmstorfKornhuberetal.2018, author = {Mann, Michael E. and Rahmstorf, Stefan and Kornhuber, Kai and Steinman, Byron A. and Miller, Sonya K. and Petri, Stefan and Coumou, Dim}, title = {Projected changes in persistent extreme summer weather events}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {994}, issn = {1866-8372}, doi = {10.25932/publishup-44641}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-446416}, pages = {12}, year = {2018}, abstract = {Persistent episodes of extreme weather in the Northern Hemisphere summer have been associated with high-amplitude quasi-stationary atmospheric Rossby waves, with zonal wave numbers 6 to 8 resulting from the phenomenon of quasi-resonant amplification (QRA). A fingerprint for the occurrence of QRA can be defined in terms of the zonally averaged surface temperature field. Examining state-of-the-art [Coupled Model Intercomparison Project Phase 5 (CMIP5)] climate model projections, we find that QRA events are likely to increase by similar to 50\% this century under business-as-usual carbon emissions, but there is considerable variation among climate models. Some predict a near tripling of QRA events by the end of the century, while others predict a potential decrease. Models with amplified Arctic warming yield the most pronounced increase in QRA events. The projections are strongly dependent on assumptions regarding the nature of changes in radiative forcing associated with anthropogenic aerosols over the next century. One implication of our findings is that a reduction in midlatitude aerosol loading could actually lead to Arctic de-amplification this century, ameliorating potential increases in persistent extreme weather events.}, language = {en} } @phdthesis{Leser2018, author = {Leser, Eva}, title = {Eta Carinae}, doi = {10.25932/publishup-42814}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-428141}, school = {Universit{\"a}t Potsdam}, pages = {X, 117}, year = {2018}, abstract = {Das außergew{\"o}hnliche Doppelsternsystem Eta Carinae fasziniert WissenschaftlerInnen und BeobachterInnen auf der s{\"u}dlichen Erdhalbkugel seit hunderten Jahren. Nach einem Supernova-{\"a}hnlichem Ausbruch war Eta Carinae zeitweise der hellste Stern am Nachthimmel. Heute sind durch zahlreiche Beobachtungen, von Radiowellen bis zu R{\"o}ntgenstrahlung, der Aufbau des Sternsystems und die Eigenschaften seiner Strahlung bis zu Energien von ~ 50 keV gut erforscht. Das Doppelsternsystem besteht aus zwei massiven Sternen (~ 30 und ~ 100 Sonnenmassen Gewicht) mit starken Sternwinden, {\"u}ber die sie kontinuierlich einen Teil ihrer Masse verlieren. Wenn diese Sternwinde kollidieren, entsteht auf beiden Seiten ein Kompressionsschock der das Plasma in der Kollisionszone aufheizt, was sich in R{\"o}ntgenstrahlung beobachten l{\"a}sst. Bei Energien oberhalb von ~ 50 keV ist der Ursprung der Strahlung nicht mehr thermisch: um ein Plasma auf die entsprechende Temperatur zu bringen, wird mehr mechanische Energie ben{\"o}tigt, als in den Sternwinden vorhanden. In hoch-energetischer Gamma-Strahlung ist Eta Carinae das einzige eindeutig detektierte Sternsystem seiner Art und sein Energiespektrum reicht bis zu ~ hundert GeV. Bodengebundene Gamma-Strahlungsexperimente haben in diesem Energiebereich den Vorteil von großen Detektorfl{\"a}chen. H.E.S.S. ist das einzige bodengebundene Gamma-Strahlungsexperiment auf der S{\"u}dhalbkugel und somit in der Lage, Eta Carinae in diesen Energien zu beobachten. H.E.S.S. misst Gamma-Strahlung mit Hilfe der elektromagnetischen Teilchenschauer, die sehr hoch-energetische Photonen in der Atmosph{\"a}re ausl{\"o}sen. Die gr{\"o}ßte Herausforderung der Messung von Eta Carinaes Strahlung mit H.E.S.S. ist die ultraviolette Strahlung des Carina Nebels, die zu einem Hintergrund f{\"u}hrt, der bis zu zehn mal st{\"a}rker ist als der Durchschnitt in H.E.S.S. In dieser Arbeit wird die erste Detektion eines Doppelsternsystems mit kollidierenden Sternwinden in sehr hoch-energetischer Gamma-Strahlung pr{\"a}sentiert und die Studien, die diese erm{\"o}glicht haben. Das differentielle Gamma-Strahlungsspektrum bis 700 GeV wird untersucht. Hadronische und leptonische Szenarios f{\"u}r den Ursprung der Gamma-Strahlung werden diskutiert und das hadronische Szenario wird aufgrund eines Vergleichs der K{\"u}hlzeiten bevorzugt.}, language = {en} } @phdthesis{TchoumbaKwamen2018, author = {Tchoumba Kwamen, Christelle Larodia}, title = {Investigating the dynamics of polarization reversal in ferroelectric thin films by time-resolved X-ray diffraction}, doi = {10.25932/publishup-42781}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-427815}, school = {Universit{\"a}t Potsdam}, pages = {xvii, 126, xxiii}, year = {2018}, abstract = {Ferroic materials have attracted a lot of attention over the years due to their wide range of applications in sensors, actuators, and memory devices. Their technological applications originate from their unique properties such as ferroelectricity and piezoelectricity. In order to optimize these materials, it is necessary to understand the coupling between their nanoscale structure and transient response, which are related to the atomic structure of the unit cell. In this thesis, synchrotron X-ray diffraction is used to investigate the structure of ferroelectric thin film capacitors during application of a periodic electric field. Combining electrical measurements with time-resolved X-ray diffraction on a working device allows for visualization of the interplay between charge flow and structural motion. This constitutes the core of this work. The first part of this thesis discusses the electrical and structural dynamics of a ferroelectric Pt/Pb(Zr0.2,Ti0.8)O3/SrRuO3 heterostructure during charging, discharging, and polarization reversal. After polarization reversal a non-linear piezoelectric response develops on a much longer time scale than the RC time constant of the device. The reversal process is inhomogeneous and induces a transient disordered domain state. The structural dynamics under sub-coercive field conditions show that this disordered domain state can be remanent and can be erased with an appropriate voltage pulse sequence. The frequency-dependent dynamic characterization of a Pb(Zr0.52,Ti0.48)O3 layer, at the morphotropic phase boundary, shows that at high frequency, the limited domain wall velocity causes a phase lag between the applied field and both the structural and electrical responses. An external modification of the RC time constant of the measurement delays the switching current and widens the electromechanical hysteresis loop while achieving a higher compressive piezoelectric strain within the crystal. In the second part of this thesis, time-resolved reciprocal space maps of multiferroic BiFeO3 thin films were measured to identify the domain structure and investigate the development of an inhomogeneous piezoelectric response during the polarization reversal. The presence of 109° domains is evidenced by the splitting of the Bragg peak. The last part of this work investigates the effect of an optically excited ultrafast strain or heat pulse propagating through a ferroelectric BaTiO3 layer, where we observed an additional current response due to the laser pulse excitation of the metallic bottom electrode of the heterostructure.}, language = {en} } @phdthesis{Hintsche2018, author = {Hintsche, Marius}, title = {Locomotion of a bacterium with a polar bundle of flagella}, doi = {10.25932/publishup-42697}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-426972}, school = {Universit{\"a}t Potsdam}, pages = {xi, 108}, year = {2018}, abstract = {Movement and navigation are essential for many organisms during some parts of their lives. This is also true for bacteria, which can move along surfaces and swim though liquid environments. They are able to sense their environment, and move towards environmental cues in a directed fashion. These abilities enable microbial lifecyles in biofilms, improved food uptake, host infection, and many more. In this thesis we study aspects of the swimming movement - or motility - of the soil bacterium (P. putida). Like most bacteria, P. putida swims by rotating its helical flagella, but their arrangement differs from the main model organism in bacterial motility research: (E. coli). P. putida is known for its intriguing motility strategy, where fast and slow episodes can occur after each other. Up until now, it was not known how these two speeds can be produced, and what advantages they might confer to this bacterium. Normally the flagella, the main component of thrust generation in bacteria, are not observable by ordinary light microscopy. In order to elucidate this behavior, we therefore used a fluorescent staining technique on a mutant strain of this species to specifically label the flagella, while leaving the cell body only faintly stained. This allowed us to image the flagella of the swimming bacteria with high spacial and temporal resolution with a customized high speed fluorescence microscopy setup. Our observations show that P. putida can swim in three different modes. First, It can swim with the flagella pushing the cell body, which is the main mode of swimming motility previously known from other bacteria. Second, it can swim with the flagella pulling the cell body, which was thought not to be possible in situations with multiple flagella. Lastly, it can wrap its flagellar bundle around the cell body, which results in a speed wich is slower by a factor of two. In this mode, the flagella are in a different physical conformation with a larger radius so the cell body can fit inside. These three swimming modes explain the previous observation of two speeds, as well as the non strict alternation of the different speeds. Because most bacterial swimming in nature does not occur in smoothly walled glass enclosures under a microscope, we used an artificial, microfluidic, structured system of obstacles to study the motion of our model organism in a structured environment. Bacteria were observed in microchannels with cylindrical obstacles of different sizes and with different distances with video microscopy and cell tracking. We analyzed turning angles, run times, and run length, which we compared to a minimal model for movement in structured geometries. Our findings show that hydrodynamic interactions with the walls lead to a guiding of the bacteria along obstacles. When comparing the observed behavior with the statics of a particle that is deflected with every obstacle contact, we find that cells run for longer distances than that model. Navigation in chemical gradients is one of the main applications of motility in bacteria. We studied the swimming response of P. putida cells to chemical stimuli (chemotaxis) of the common food preservative sodium benzoate. Using a microfluidic gradient generation device, we created gradients of varying strength, and observed the motion of cells with a video microscope and subsequent cell tracking. Analysis of different motility parameters like run lengths and times, shows that P. putida employs the classical chemotaxis strategy of E. coli: runs up the gradient are biased to be longer than those down the gradient. Using the two different run speeds we observed due to the different swimming modes, we classify runs into `fast' and `slow' modes with a Gaussian mixture model (GMM). We find no evidence that P. putida's uses its swimming modes to perform chemotaxis. In most studies of bacterial motility, cell tracking is used to gather trajectories of individual swimming cells. These trajectories then have to be decomposed into run sections and tumble sections. Several algorithms have been developed to this end, but most require manual tuning of a number of parameters, or extensive measurements with chemotaxis mutant strains. Together with our collaborators, we developed a novel motility analysis scheme, based on generalized Kramers-Moyal-coefficients. From the underlying stochastic model, many parameters like run length etc., can be inferred by an optimization procedure without the need for explicit run and tumble classification. The method can, however, be extended to a fully fledged tumble classifier. Using this method, we analyze E. coli chemotaxis measurements in an aspartate analog, and find evidence for a chemotactic bias in the tumble angles.}, language = {en} } @misc{SarhanKoopmanSchuetzetal.2018, author = {Sarhan, Radwan Mohamed and Koopman, Wouter-Willem Adriaan and Schuetz, Roman and Schmid, Thomas and Liebig, Ferenc and Koetz, Joachim and Bargheer, Matias}, title = {The importance of plasmonic heating for the plasmondriven photodimerization of 4-nitrothiophenol}, series = {Postprints der Universit{\"a}t Potsdam Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam Mathematisch-Naturwissenschaftliche Reihe}, number = {698}, issn = {1866-8372}, doi = {10.25932/publishup-42719}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-427197}, pages = {8}, year = {2018}, abstract = {Metal nanoparticles form potent nanoreactors, driven by the optical generation of energetic electrons and nanoscale heat. The relative influence of these two factors on nanoscale chemistry is strongly debated. This article discusses the temperature dependence of the dimerization of 4-nitrothiophenol (4-NTP) into 4,4′-dimercaptoazobenzene (DMAB) adsorbed on gold nanoflowers by Surface-Enhanced Raman Scattering (SERS). Raman thermometry shows a significant optical heating of the particles. The ratio of the Stokes and the anti-Stokes Raman signal moreover demonstrates that the molecular temperature during the reaction rises beyond the average crystal lattice temperature of the plasmonic particles. The product bands have an even higher temperature than reactant bands, which suggests that the reaction proceeds preferentially at thermal hot spots. In addition, kinetic measurements of the reaction during external heating of the reaction environment yield a considerable rise of the reaction rate with temperature. Despite this significant heating effects, a comparison of SERS spectra recorded after heating the sample by an external heater to spectra recorded after prolonged illumination shows that the reaction is strictly photo-driven. While in both cases the temperature increase is comparable, the dimerization occurs only in the presence of light. Intensity dependent measurements at fixed temperatures confirm this finding.}, language = {en} } @phdthesis{Hoischen2018, author = {Hoischen, Clemens}, title = {Multi-Messenger Astronomy with H.E.S.S: the Starburst Galaxy NGC253 and the Search for Short Time-Scale Transients}, doi = {10.25932/publishup-42452}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-424521}, school = {Universit{\"a}t Potsdam}, pages = {135}, year = {2018}, abstract = {Gamma-ray astronomy has proven to provide unique insights into cosmic-ray accelerators in the past few decades. By combining information at the highest photon energies with the entire electromagnetic spectrum in multi-wavelength studies, detailed knowledge of non-thermal particle populations in astronomical objects and systems has been gained: Many individual classes of gamma-ray sources could be identified inside our galaxy and outside of it. Different sources were found to exhibit a wide range of temporal evolution, ranging from seconds to stable behaviours over many years of observations. With the dawn of both neutrino- and gravitational wave astronomy, additional messengers have come into play over the last years. This development presents the advent of multi-messenger astronomy: a novel approach not only to search for sources of cosmic rays, but for astronomy in general. In this thesis, both traditional multi-wavelength studies and multi-messenger studies will be presented. They were carried out with the H.E.S.S. experiment, an imaging air Cherenkov telescope array located in the Khomas Highland of Namibia. H.E.S.S. has entered its second phase in 2012 with the addition of a large, fifth telescope. While the initial array was limited to the study of gamma-rays with energies above 100 GeV, the new instrument allows to access gamma-rays with energies down to a few tens of GeV. Strengths of the multi-wavelength approach will be demonstrated at the example of the galaxy NGC253, which is undergoing an episode of enhanced star-formation. The gamma-ray emission will be discussed in light of all the information on this system available from radio, infrared and X-rays. These wavelengths reveal detailed information on the population of supernova remnants, which are suspected cosmic-ray accelerators. A broad-band gamma-ray spectrum is derived from H.E.S.S. and Fermi-LAT data. The improved analysis of H.E.S.S. data provides a measurement which is no longer dominated by systematic uncertainties. The long-term behaviour of cosmic rays in the starburst galaxy NGC253 is finally characterised. In contrast to the long time-scale evolution of a starburst galaxy, multi-messenger studies are especially intriguing when shorter time-scales are being probed. A prime example of a short time-scale transient are Gamma Ray Bursts. The efforts to understand this phenomenon effectively founded the branch of gamma-ray astronomy. The multi-messenger approach allows for the study of illusive phenomena such as Gamma Ray Bursts and other transients using electromagnetic radiation, neutrinos, cosmic rays and gravitational waves contemporaneously. With contemporaneous observations getting more important just recently, the execution of such observation campaigns still presents a big challenge due to the different limitations and strengths of the infrastructures. An alert system for transient phenomena has been developed over the course of this thesis for H.E.S.S. It aims to address many follow-up challenges in order to maximise the science return of the new large telescope, which is able to repoint much faster than the initial four telescopes. The system allows for fully automated observations based on scientific alerts from any wavelength or messenger and allows H.E.S.S. to participate in multi-messenger campaigns. Utilising this new system, many interesting multi-messenger observation campaigns have been performed. Several highlight observations with H.E.S.S. are analysed, presented and discussed in this work. Among them are observations of Gamma Ray Bursts with low latency and low energy threshold, the follow-up of a neutrino candidate in spatial coincidence with a flaring active galactic nucleus and of the merger of two neutron stars, which was revealed by the coincidence of gravitational waves and a Gamma-Ray Burst.}, language = {en} } @phdthesis{RodriguezLoureiro2018, author = {Rodriguez Loureiro, Ignacio}, title = {Structural characterization of single and interacting soft interfaces displaying brushes of synthetic or biomolecular polymers}, doi = {10.25932/publishup-42367}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-423675}, school = {Universit{\"a}t Potsdam}, pages = {132}, year = {2018}, abstract = {The interaction between surfaces displaying end-grafted hydrophilic polymer brushes plays important roles in biology and in many wet-technological applications. The outer surfaces of Gram-negative bacteria, for example, are composed of lipopolysaccharide (LPS) molecules exposing oligo- and polysaccharides to the aqueous environment. This unique, structurally complex biological interface is of great scientific interest as it mediates the interaction of bacteria with neighboring bacteria in colonies and biofilms. The interaction between polymer-decorated surfaces is generally coupled to the distance-dependent conformation of the polymer chains. Therefore, structural insight into the interacting surfaces is a prerequisite to understand the interaction characteristics as well as the underlying physical mechanisms. This problem has been addressed by theory, but accurate experimental data on polymer conformations under confinement are rare, because obtaining perturbation-free structural insight into buried soft interfaces is inherently difficult. In this thesis, lipid membrane surfaces decorated with hydrophilic polymers of technological and biological relevance are investigated under controlled interaction conditions, i.e., at defined surface separations. For this purpose, dedicated sample architectures and experimental tools are developed. Via ellipsometry and neutron reflectometry pressure-distance curves and distance-dependent polymer conformations in terms of brush compression and reciprocative interpenetration are determined. Additional element-specific structural insight into the end-point distribution of interacting brushes is obtained by standing-wave x-ray fluorescence (SWXF). The methodology is first established for poly[ethylene glycol] (PEG) brushes of defined length and grafting density. For this system, neutron reflectometry revealed pronounced brush interpenetration, which is not captured in common brush theories and therefore motivates rigorous simulation-based treatments. In the second step the same approach is applied to realistic mimics of the outer surfaces of Gram-negative bacteria: monolayers of wild type LPSs extracted from E. Coli O55:B5 displaying strain-specific O-side chains. The neutron reflectometry experiments yield unprecedented structural insight into bacterial interactions, which are of great relevance for the properties of biofilms.}, language = {en} } @phdthesis{Koc2018, author = {Ko{\c{c}}, Azize}, title = {Ultrafast x-ray studies on the non-equilibrium of the magnetic and phononic system in heavy rare-earths}, doi = {10.25932/publishup-42328}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-423282}, school = {Universit{\"a}t Potsdam}, pages = {ii, 117}, year = {2018}, abstract = {In this dissertation the lattice and the magnetic recovery dynamics of the two heavy rare-earth metals Dy and Gd after femtosecond photoexcitation are described. For the investigations, thin films of Dy and Gd were measured at low temperatures in the antiferromagnetic phase of Dy and close to room temperature in the ferromagnetic phase of Gd. Two different optical pump-x-ray probe techniques were employed: Ultrafast x-ray diffraction with hard x-rays (UXRD) yields the structural response of heavy rare-earth metals and resonant soft (elastic) x-ray diffraction (RSXD), which allows measuring directly changes in the helical antiferromagnetic order of Dy. The combination of both techniques enables to study the complex interaction between the magnetic and the phononic subsystems.}, language = {en} } @phdthesis{Codutti2018, author = {Codutti, Agnese}, title = {Behavior of magnetic microswimmers}, doi = {10.25932/publishup-42297}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-422976}, school = {Universit{\"a}t Potsdam}, pages = {iv, 142}, year = {2018}, abstract = {Microswimmers, i.e. swimmers of micron size experiencing low Reynolds numbers, have received a great deal of attention in the last years, since many applications are envisioned in medicine and bioremediation. A promising field is the one of magnetic swimmers, since magnetism is biocom-patible and could be used to direct or actuate the swimmers. This thesis studies two examples of magnetic microswimmers from a physics point of view. The first system to be studied are magnetic cells, which can be magnetic biohybrids (a swimming cell coupled with a magnetic synthetic component) or magnetotactic bacteria (naturally occurring bacteria that produce an intracellular chain of magnetic crystals). A magnetic cell can passively interact with external magnetic fields, which can be used for direction. The aim of the thesis is to understand how magnetic cells couple this magnetic interaction to their swimming strategies, mainly how they combine it with chemotaxis (the ability to sense external gradient of chemical species and to bias their walk on these gradients). In particular, one open question addresses the advantage given by these magnetic interactions for the magnetotactic bacteria in a natural environment, such as porous sediments. In the thesis, a modified Active Brownian Particle model is used to perform simulations and to reproduce experimental data for different systems such as bacteria swimming in the bulk, in a capillary or in confined geometries. I will show that magnetic fields speed up chemotaxis under special conditions, depending on parameters such as their swimming strategy (run-and-tumble or run-and-reverse), aerotactic strategy (axial or polar), and magnetic fields (intensities and orientations), but it can also hinder bacterial chemotaxis depending on the system. The second example of magnetic microswimmer are rigid magnetic propellers such as helices or random-shaped propellers. These propellers are actuated and directed by an external rotating magnetic field. One open question is how shape and magnetic properties influence the propeller behavior; the goal of this research field is to design the best propeller for a given situation. The aim of the thesis is to propose a simulation method to reproduce the behavior of experimentally-realized propellers and to determine their magnetic properties. The hydrodynamic simulations are based on the use of the mobility matrix. As main result, I propose a method to match the experimental data, while showing that not only shape but also the magnetic properties influence the propellers swimming characteristics.}, language = {en} } @phdthesis{vonNordheim2018, author = {von Nordheim, Danny}, title = {Dielectric non-linearities of P(VDF-TrFE) single and multilayers for memory applications}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-421778}, school = {Universit{\"a}t Potsdam}, pages = {XVI, 109}, year = {2018}, abstract = {Poly(vinylidene fluoride-trifluoroethylene) (P(VDF-TrFE)) ferroelectric thin films of different molar ratio have been studied with regard to data memory applications. Therefore, films with thicknesses of 200 nm and less have been spin coated from solution. Observations gained from single layers have been extended to multilayer capacitors and three terminal transistor devices. Besides conventional hysteresis measurements, the measurement of dielectric non-linearities has been used as a main tool of characterisation. Being a very sensitive and non-destructive method, non-linearity measurements are well suited for polarisation readout and property studies. Samples have been excited using a high quality, single-frequency sinusoidal voltage with an amplitude significantly smaller than the coercive field of the samples. The response was then measured at the excitation frequency and its higher harmonics. Using the measurement results, the linear and non-linear dielectric permittivities ɛ₁, ɛ₂ and ɛ₃ have been determined. The permittivities have been used to derive the temperature-dependent polarisation behaviour as well as the polarisation state and the order of the phase transitions. The coercive field in VDF-TrFE copolymers is high if compared to their ceramic competitors. Therefore, the film thickness had to be reduced significantly. Considering a switching voltage of 5 V and a coercive field of 50 MV/m, the film thickness has to be 100 nm and below. If the thickness becomes substantially smaller than the other dimensions, surface and interface layer effects become more pronounced. For thicker films of P(VDF-TrFE) with a molar fraction of 56/44 a second-order phase transition without a thermal hysteresis for an ɛ₁(T) temperature cycle has been predicted and observed. This however, could not be confirmed by the measurements of thinner films. A shift of transition temperatures as well as a temperature independent, non-switchable polarisation and a thermal hysteresis for P(VDF-TrFE) 56/44 have been observed. The impact of static electric fields on the polarisation and the phase transition has therefore been studied and simulated, showing that all aforementioned phenomena including a linear temperature dependence of the polarisation might originate from intrinsic electric fields. In further experiments the knowledge gained from single layer capacitors has been extended to bilayer copolymer thin films of different molar composition. Bilayers have been deposited by succeeding cycles of spin coating from solution. Single layers and their bilayer combination have been studied individually in order to prove the layers stability. The individual layers have been found to be physically stable. But while the bilayers reproduced the main ɛ₁(T) properties of the single layers qualitatively, quantitative numbers could not be explained by a simple serial connection of capacitors. Furthermore, a linear behaviour of the polarisation throughout the measured temperature range has been observed. This was found to match the behaviour predicted considering a constant electric field. Retention time is an important quantity for memory applications. Hence, the retention behaviour of VDF-TrFE copolymer thin films has been determined using dielectric non-linearities. The polarisation loss in P(VDF-TrFE) poled samples has been found to be less than 20\% if recorded over several days. The loss increases significantly if the samples have been poled with lower amplitudes, causing an unsaturated polarisation. The main loss was attributed to injected charges. Additionally, measurements of dielectric non-linearities have been proven to be a sensitive and non-destructive tool to measure the retention behaviour. Finally, a ferroelectric field effect transistor using mainly organic materials (FerrOFET) has been successfully studied. DiNaphtho[2,3-b:2',3'-f]Thieno[3,2-b]Thiophene (DNTT) has proven to be a stable, suitable organic semiconductor to build up ferroelectric memory devices. Furthermore, an oxidised aluminium bottom electrode and additional dielectric layers, i.e. parylene C, have proven to reduce the leakage current and therefore enhance the performance significantly.}, language = {en} } @phdthesis{Arora2018, author = {Arora, Ashima}, title = {Optical and electric field control of magnetism}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-421479}, school = {Universit{\"a}t Potsdam}, pages = {ii, 126}, year = {2018}, abstract = {Future magnetic recording industry needs a high-density data storage technology. However, switching the magnetization of small bits requires high magnetic fields that cause excessive heat dissipation. Therefore, controlling magnetism without applying external magnetic field is an important research topic for potential applications in data storage devices with low power consumption. Among the different approaches being investigated, two of them stand out, namely i) all-optical helicity dependent switching (AO-HDS) and ii) ferroelectric control of magnetism. This thesis aims to contribute towards a better understanding of the physical processes behinds these effects as well as reporting new and exciting possibility for the optical and/or electric control of magnetic properties. Hence, the thesis contains two differentiated chapters of results; the first devoted to AO-HDS on TbFe alloys and the second to the electric field control of magnetism in an archetypal Fe/BaTiO3 system. In the first part, the scalability of the AO-HDS to small laser spot-sizes of few microns in the ferrimagnetic TbFe alloy is investigated by spatially resolving the magnetic contrast with photo-emission electron microscopy (PEEM) and X-ray magnetic circular dichroism (XMCD). The results show that the AO-HDS is a local effect within the laser spot size that occurs in the ring-shaped region in the vicinity of thermal demagnetization. Within the ring region, the helicity dependent switching occurs via thermally activated domain wall motion. Further, the thesis reports on a novel effect of thickness dependent inversion of the switching orientation. It addresses some of the important questions like the role of laser heating and the microscopic mechanism driving AO-HDS. The second part of the thesis focuses on the electric field control of magnetism in an artificial multiferroic heterostructure. The sample consists of an Fe wedge with thickness varying between 0:5 nm and 3 nm, deposited on top of a ferroelectric and ferroelastic BaTiO3 [001]-oriented single crystal substrate. Here, the magnetic contrast is imaged via PEEM and XMCD as a function of out-of-plane voltage. The results show the evidence of the electric field control of superparamagnetism mediated by a ferroelastic modification of the magnetic anisotropy. The changes in the magnetoelastic anisotropy drive the transition from the superparamagnetic to superferromagnetic state at localized sample positions.}, language = {en} } @phdthesis{Kegeles2018, author = {Kegeles, Alexander}, title = {Algebraic foundation of Group Field Theory}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-421014}, school = {Universit{\"a}t Potsdam}, pages = {124}, year = {2018}, abstract = {In this thesis we provide a construction of the operator framework starting from the functional formulation of group field theory (GFT). We define operator algebras on Hilbert spaces whose expectation values in specific states provide correlation functions of the functional formulation. Our construction allows us to give a direct relation between the ingredients of the functional GFT and its operator formulation in a perturbative regime. Using this construction we provide an example of GFT states that can not be formulated as states in a Fock space and lead to math- ematically inequivalent representations of the operator algebra. We show that such inequivalent representations can be grouped together by their symmetry properties and sometimes break the left translation symmetry of the GFT action. We interpret these groups of inequivalent representations as phases of GFT, similar to the classification of phases that we use in QFT's on space-time.}, language = {en} } @phdthesis{Quade2018, author = {Quade, Markus}, title = {Symbolic regression for identification, prediction, and control of dynamical systems}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-419790}, school = {Universit{\"a}t Potsdam}, pages = {xiii, 134}, year = {2018}, abstract = {In the present work, we use symbolic regression for automated modeling of dynamical systems. Symbolic regression is a powerful and general method suitable for data-driven identification of mathematical expressions. In particular, the structure and parameters of those expressions are identified simultaneously. We consider two main variants of symbolic regression: sparse regression-based and genetic programming-based symbolic regression. Both are applied to identification, prediction and control of dynamical systems. We introduce a new methodology for the data-driven identification of nonlinear dynamics for systems undergoing abrupt changes. Building on a sparse regression algorithm derived earlier, the model after the change is defined as a minimum update with respect to a reference model of the system identified prior to the change. The technique is successfully exemplified on the chaotic Lorenz system and the van der Pol oscillator. Issues such as computational complexity, robustness against noise and requirements with respect to data volume are investigated. We show how symbolic regression can be used for time series prediction. Again, issues such as robustness against noise and convergence rate are investigated us- ing the harmonic oscillator as a toy problem. In combination with embedding, we demonstrate the prediction of a propagating front in coupled FitzHugh-Nagumo oscillators. Additionally, we show how we can enhance numerical weather predictions to commercially forecast power production of green energy power plants. We employ symbolic regression for synchronization control in coupled van der Pol oscillators. Different coupling topologies are investigated. We address issues such as plausibility and stability of the control laws found. The toolkit has been made open source and is used in turbulence control applications. Genetic programming based symbolic regression is very versatile and can be adapted to many optimization problems. The heuristic-based algorithm allows for cost efficient optimization of complex tasks. We emphasize the ability of symbolic regression to yield white-box models. In contrast to black-box models, such models are accessible and interpretable which allows the usage of established tool chains.}, language = {en} } @phdthesis{SaadHassanin2018, author = {Saad Hassanin, Alshaimaa}, title = {Dynamic coronal mass ejection process and magnetic reconnection}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-419626}, school = {Universit{\"a}t Potsdam}, pages = {xix, 113}, year = {2018}, abstract = {The Sun is the nearest star to the Earth. It consists of an interior and an atmosphere. The convection zone is the outermost layer of the solar interior. A flux rope may emerge as a coherent structure from the convection zone into the solar atmosphere or be formed by magnetic reconnection in the atmosphere. A flux rope is a bundle of magnetic field lines twisting around an axis field line, creating a helical shape by which dense filament material can be supported against gravity. The flux rope is also considered as the key structure of the most energetic phenomena in the solar system, such as coronal mass ejections (CMEs) and flares. These magnetic flux ropes can produce severe geomagnetic storms. In particular, to improve the ability to forecast space weather, it is important to enrich our knowledge about the dynamic formation of flux ropes and the underlying physical mechanisms that initiate their eruption, such as a CME. A confined eruption consists of a filament eruption and usually an associated are, but does not evolve into a CME; rather, the moving plasma is halted in the solar corona and usually seen to fall back. The first detailed observations of a confined filament eruption were obtained on 2002 May 27by the TRACE satellite in the 195 A band. So, in the Chapter 3, we focus on a flux rope instability model. A twisted flux rope can become unstable by entering the kink instability regime. We show that the kink instability, which occurs if the twist of a flux rope exceeds a critical value, is capable of initiating of an eruption. This model is tested against the well observed confined eruption on 2002 May 27 in a parametric magnetohydrodynamic (MHD) simulation study that comprises all phases of the event. Very good agreement with the essential observed properties is obtained, only except for a relatively poor matching of the initial filament height. Therefore, in Chapter 4, we submerge the center point of the flux rope deeper below the photosphere to obtain a flatter coronal rope section and a better matching with the initial height profile of the erupting filament. This implies a more realistic inclusion of the photospheric line tying. All basic assumptions and the other parameter settings are kept the same as in Chapter 3. This complement of the parametric study shows that the flux rope instability model can yield an even better match with the observational data. We also focus in Chapters 3 and 4 on the magnetic reconnection during the confined eruption, demonstrating that it occurs in two distinct locations and phases that correspond to the observed brightenings and changes of topology, and consider the fate of the erupting flux, which can reform a (less twisted) flux rope. The Sun also produces series of homologous eruptions, i.e. eruptions which occur repetitively in the same active region and are of similar morphology. Therefore, in Chapter 5, we employ the reformed flux rope as a new initial condition, to investigate the possibility of subsequent homologous eruptions. Free magnetic energy is built up by imposing motions in the bottom boundary, such as converging motions, leading to flux cancellation. We apply converging motions in the sunspot area, such that a small part of the flux from the sunspots with different polarities is transported toward the polarity inversion line (PIL) and cancels with each other. The reconnection associated with the cancellation process forms more helical magnetic flux around the reformed flux rope, which leads to a second and a third eruption. In this study, we obtain the first MHD simulation results of a homologous sequence of eruptions that show a transition from a confined to two ejective eruptions, based on the reformation of a flux rope after each eruption.}, language = {en} } @phdthesis{Sander2018, author = {Sander, Mathias}, title = {Ultrafast tailored strain fields in nanostructures}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-417863}, school = {Universit{\"a}t Potsdam}, pages = {xvii, 119}, year = {2018}, abstract = {This publication based thesis, which consists of seven published articles, summarizes my contributions to the research field of laser excited ultrafast structural dynamics. The coherent and incoherent lattice dynamics on microscopic length scales are detected by ultrashort optical and X-ray pulses. The understanding of the complex physical processes is essential for future improvements of technological applications. For this purpose, tabletop soruces and large scale facilities, e.g. synchrotrons, are employed to study structural dynamics of longitudinal acoustic strain waves and heat transport. The investigated effects cover timescales from hundreds of femtoseconds up to several microseconds. The main part of this thesis is dedicated to the investigation of tailored phonon wave packets propagating in perovskite nanostructures. Tailoring is achieved either by laser excitation of nanostructured bilayer samples or by a temporal series of laser pulses. Due to the propagation of longitudinal acoustic phonons, the out-of-plane lattice spacing of a thin film insulator-metal bilayer sample is modulated on an ultrafast timescale. This leads to an ultrafast modulation of the X-ray diffraction efficiency which is employed as a phonon Bragg switch to shorten hard X-ray pulses emitted from a 3rd generation synchrotron. In addition, we have observed nonlinear mixing of high amplitude phonon wave packets which originates from an anharmonic interatomic potential. A chirped optical pulse sequence excites a narrow band phonon wave packet with specific momentum and energy. The second harmonic generation of these phonon wave packets is followed by ultrafast X-ray diffraction. Phonon upconversion takes place because the high amplitude phonon wave packet modulates the acoustic properties of the crystal which leads to self steepening and to the successive generation of higher harmonics of the phonon wave packet. Furthermore, we have demonstrated ultrafast strain in direction parallel to the sample surface. Two consecutive so-called transient grating excitations displaced in space and time are used to coherently control thermal gradients and surface acoustic modes. The amplitude of the coherent and incoherent surface excursion is disentangled by time resolved X-ray reflectivity measurements. We calibrate the absolute amplitude of thermal and acoustic surface excursion with measurements of longitudinal phonon propagation. In addition, we develop a diffraction model which allows for measuring the surface excursion on an absolute length scale with sub-{\"A}angstr{\"o}m precision. Finally, I demonstrate full coherent control of an excited surface deformation by amplifying and suppressing thermal and coherent excitations at the surface of a laser-excited Yttrium-manganite sample.}, language = {en} } @phdthesis{Rafighi2018, author = {Rafighi, Iman}, title = {Plasma Instabilities from blazar-induced pair beams propagating through IGM}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-417428}, school = {Universit{\"a}t Potsdam}, pages = {ix, 114}, year = {2018}, abstract = {Modern gamma-ray telescopes, provide the main stream of data for astrophysicists in quest of detecting the sources of gamma rays such as active galactic nuclei (AGN). Many blazars have been detected with gamma-ray telescopes such as HESS, VERITAS, MAGIC and Fermi satellite as sources of gamma-rays with the energy E ≥ 100 GeV. These very-high-energy photons interact with extragalactic background light (EBL) producing ultra-relativistic electron-positron pairs. Observations with Fermi-LAT indicate that the GeV gamma-ray flux from some blazars is lower than that predicted from the full electromagnetic cascade. The pairs can induce electrostatic and electromagnetic instabilities. In this case, wave-particle interactions can reduce the energy of the pairs. Therefore, the collective plasma effects can also substantially suppress the GeV-band gamma-ray emission affecting as well the IGMF constraints. Using Particle in cell (PIC) simulations, we have revisited the issue of plasma instabilities induced by electron-positron beams in the fully ionized intergalactic medium. This problem is related to pair beams produced by TeV radiation of blazars. The main objective of our study is to clarify the feedback of the beam-driven instabilities on the pairs. The present dissertation provides new results regarding the plasma instabilities from blazar induced pair beams interacting with intergalactic medium. This clarifies the relevance of plasma instabilities and improves our understanding of blazars.}, language = {en} } @phdthesis{Feldmann2018, author = {Feldmann, David}, title = {Light-driven diffusioosmosis}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-417184}, school = {Universit{\"a}t Potsdam}, pages = {viii, 150}, year = {2018}, abstract = {The emergence of microfluidics created the need for precise and remote control of micron-sized objects. I demonstrate how light-sensitive motion can be induced at the micrometer scale by a simple addition of a photosensitive surfactant, which makes it possible to trigger hydrophobicity with light. With point-like laser irradiation, radial inward and outward hydrodynamic surface flows are remotely switched on and off. In this way, ensembles of microparticles can be moved toward or away from the irradiation center. Particle motion is analyzed according to varying parameters, such as surfactant and salt concentration, illumination condition, surface hydrophobicity, and surface structure. The physical origin of this process is the so-called light-driven diffusioosmosis (LDDO), a phenomenon that was discovered in the framework of this thesis and is described experimentally and theoretically in this work. To give a brief explanation, a focused light irradiation induces a local photoisomerization that creates a concentration gradient at the solid-liquid interface. To compensate for the change in osmotic pressure near the surface, a hydrodynamic flow along the surface is generated. Surface-surfactant interaction largely governs LDDO. It is shown that surfactant adsorption depends on the isomerization state of the surfactant. Photoisomerization, therefore, triggers a surfactant attachment or detachment from the surface. This change is considered to be one of the reasons for the formation of LDDO flow. These flows are introduced not only by a focused laser source but also by global irradiation. Porous particles show reversible repulsive and attractive interactions when dispersed in the solution of photosensitive surfactant. Repulsion and attraction is controlled by the irradiation wavelength. Illumination with red light leads to formation of aggregates, while illumination with blue light leads to the formation of a well-separated grid with equal interparticle distances, between 2µm and 80µm, depending on the particle surface density. These long-range interactions are considered to be a result of an increase or decrease of surfactant concentration around each particle, depending on the irradiation wavelength. Surfactant molecules adsorb inside the pores of the particles. A light-induced photoisomerization changes adsorption to the pores and drives surfactant molecules to the outside. The concentration gradients generate symmetric flows around each single particle resulting in local LDDO. With a break of the symmetry (i.e., by closing one side of the particle with a metal cap), one can achieve active self-propelled particle motion.}, language = {en} } @phdthesis{Ma2018, author = {Ma, Siyuan}, title = {Analysis of Teukolsky equations on slowly rotating Kerr spacetimes}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-414781}, school = {Universit{\"a}t Potsdam}, pages = {vi, 89}, year = {2018}, abstract = {In this thesis, we treat the extreme Newman-Penrose components of both the Maxwell field (s=±1) and the linearized gravitational perturbations (or "linearized gravity" for short) (s=±2) in the exterior of a slowly rotating Kerr black hole. Upon different rescalings, we can obtain spin s components which satisfy the separable Teukolsky master equation (TME). For each of these spin s components defined in Kinnersley tetrad, the resulting equations by performing some first-order differential operator on it once and twice (twice only for s=±2), together with the TME, are in the form of an "inhomogeneous spin-weighted wave equation" (ISWWE) with different potentials and constitute a linear spin-weighted wave system. We then prove energy and integrated local energy decay (Morawetz) estimates for this type of ISWWE, and utilize them to achieve both a uniform bound of a positive definite energy and a Morawetz estimate for the regular extreme Newman-Penrose components defined in the regular Hawking-Hartle tetrad. We also present some brief discussions on mode stability for TME for the case of real frequencies. This says that in a fixed subextremal Kerr spacetime, there is no nontrivial separated mode solutions to TME which are purely ingoing at horizon and purely outgoing at infinity. This yields a representation formula for solutions to inhomogeneous Teukolsky equations, and will play a crucial role in generalizing the above energy and Morawetz estimates results to the full subextremal Kerr case.}, language = {en} } @phdthesis{Paganini2018, author = {Paganini, Claudio Francesco}, title = {The role of trapping in black hole spacetimes}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-414686}, school = {Universit{\"a}t Potsdam}, pages = {v, 138}, year = {2018}, abstract = {In the here presented work we discuss a series of results that are all in one way or another connected to the phenomenon of trapping in black hole spacetimes. First we present a comprehensive review of the Kerr-Newman-Taub-NUT-de-Sitter family of black hole spacetimes and their most important properties. From there we go into a detailed analysis of the bahaviour of null geodesics in the exterior region of a sub-extremal Kerr spacetime. We show that most well known fundamental properties of null geodesics can be represented in one plot. In particular, one can see immediately that the ergoregion and trapping are separated in phase space. We then consider the sets of future/past trapped null geodesics in the exterior region of a sub-extremal Kerr-Newman-Taub-NUT spacetime. We show that from the point of view of any timelike observer outside of such a black hole, trapping can be understood as two smooth sets of spacelike directions on the celestial sphere of the observer. Therefore the topological structure of the trapped set on the celestial sphere of any observer is identical to that in Schwarzschild. We discuss how this is relevant to the black hole stability problem. In a further development of these observations we introduce the notion of what it means for the shadow of two observers to be degenerate. We show that, away from the axis of symmetry, no continuous degeneration exists between the shadows of observers at any point in the exterior region of any Kerr-Newman black hole spacetime of unit mass. Therefore, except possibly for discrete changes, an observer can, by measuring the black holes shadow, determine the angular momentum and the charge of the black hole under observation, as well as the observer's radial position and angle of elevation above the equatorial plane. Furthermore, his/her relative velocity compared to a standard observer can also be measured. On the other hand, the black hole shadow does not allow for a full parameter resolution in the case of a Kerr-Newman-Taub-NUT black hole, as a continuous degeneration relating specific angular momentum, electric charge, NUT charge and elevation angle exists in this case. We then use the celestial sphere to show that trapping is a generic feature of any black hole spacetime. In the last chapter we then prove a generalization of the mode stability result of Whiting (1989) for the Teukolsky equation for the case of real frequencies. The main result of the last chapter states that a separated solution of the Teukolsky equation governing massless test fields on the Kerr spacetime, which is purely outgoing at infinity, and purely ingoing at the horizon, must vanish. This has the consequence, that for real frequencies, there are linearly independent fundamental solutions of the radial Teukolsky equation which are purely ingoing at the horizon, and purely outgoing at infinity, respectively. This fact yields a representation formula for solutions of the inhomogenous Teukolsky equation, and was recently used by Shlapentokh-Rothman (2015) for the scalar wave equation.}, language = {en} } @phdthesis{Kotha2018, author = {Kotha, Sreeram Reddy}, title = {Quantification of uncertainties in seismic ground-motion prediction}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-415743}, school = {Universit{\"a}t Potsdam}, pages = {xii, 101}, year = {2018}, abstract = {The purpose of Probabilistic Seismic Hazard Assessment (PSHA) at a construction site is to provide the engineers with a probabilistic estimate of ground-motion level that could be equaled or exceeded at least once in the structure's design lifetime. A certainty on the predicted ground-motion allows the engineers to confidently optimize structural design and mitigate the risk of extensive damage, or in worst case, a collapse. It is therefore in interest of engineering, insurance, disaster mitigation, and security of society at large, to reduce uncertainties in prediction of design ground-motion levels. In this study, I am concerned with quantifying and reducing the prediction uncertainty of regression-based Ground-Motion Prediction Equations (GMPEs). Essentially, GMPEs are regressed best-fit formulae relating event, path, and site parameters (predictor variables) to observed ground-motion values at the site (prediction variable). GMPEs are characterized by a parametric median (μ) and a non-parametric variance (σ) of prediction. μ captures the known ground-motion physics i.e., scaling with earthquake rupture properties (event), attenuation with distance from source (region/path), and amplification due to local soil conditions (site); while σ quantifies the natural variability of data that eludes μ. In a broad sense, the GMPE prediction uncertainty is cumulative of 1) uncertainty on estimated regression coefficients (uncertainty on μ,σ_μ), and 2) the inherent natural randomness of data (σ). The extent of μ parametrization, the quantity, and quality of ground-motion data used in a regression, govern the size of its prediction uncertainty: σ_μ and σ. In the first step, I present the impact of μ parametrization on the size of σ_μ and σ. Over-parametrization appears to increase the σ_μ, because of the large number of regression coefficients (in μ) to be estimated with insufficient data. Under-parametrization mitigates σ_μ, but the reduced explanatory strength of μ is reflected in inflated σ. For an optimally parametrized GMPE, a ~10\% reduction in σ is attained by discarding the low-quality data from pan-European events with incorrect parametric values (of predictor variables). In case of regions with scarce ground-motion recordings, without under-parametrization, the only way to mitigate σ_μ is to substitute long-term earthquake data at a location with short-term samples of data across several locations - the Ergodic Assumption. However, the price of ergodic assumption is an increased σ, due to the region-to-region and site-to-site differences in ground-motion physics. σ of an ergodic GMPE developed from generic ergodic dataset is much larger than that of non-ergodic GMPEs developed from region- and site-specific non-ergodic subsets - which were too sparse to produce their specific GMPEs. Fortunately, with the dramatic increase in recorded ground-motion data at several sites across Europe and Middle-East, I could quantify the region- and site-specific differences in ground-motion scaling and upgrade the GMPEs with 1) substantially more accurate region- and site-specific μ for sites in Italy and Turkey, and 2) significantly smaller prediction variance σ. The benefit of such enhancements to GMPEs is quite evident in my comparison of PSHA estimates from ergodic versus region- and site-specific GMPEs; where the differences in predicted design ground-motion levels, at several sites in Europe and Middle-Eastern regions, are as large as ~50\%. Resolving the ergodic assumption with mixed-effects regressions is feasible when the quantified region- and site-specific effects are physically meaningful, and the non-ergodic subsets (regions and sites) are defined a priori through expert knowledge. In absence of expert definitions, I demonstrate the potential of machine learning techniques in identifying efficient clusters of site-specific non-ergodic subsets, based on latent similarities in their ground-motion data. Clustered site-specific GMPEs bridge the gap between site-specific and fully ergodic GMPEs, with their partially non-ergodic μ and, σ ~15\% smaller than the ergodic variance. The methodological refinements to GMPE development produced in this study are applicable to new ground-motion datasets, to further enhance certainty of ground-motion prediction and thereby, seismic hazard assessment. Advanced statistical tools show great potential in improving the predictive capabilities of GMPEs, but the fundamental requirement remains: large quantity of high-quality ground-motion data from several sites for an extended time-period.}, language = {en} } @phdthesis{Muench2018, author = {M{\"u}nch, Thomas}, title = {Interpretation of temperature signals from ice cores}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-414963}, school = {Universit{\"a}t Potsdam}, pages = {xxi, 197}, year = {2018}, abstract = {Earth's climate varies continuously across space and time, but humankind has witnessed only a small snapshot of its entire history, and instrumentally documented it for a mere 200 years. Our knowledge of past climate changes is therefore almost exclusively based on indirect proxy data, i.e. on indicators which are sensitive to changes in climatic variables and stored in environmental archives. Extracting the data from these archives allows retrieval of the information from earlier times. Obtaining accurate proxy information is a key means to test model predictions of the past climate, and only after such validation can the models be used to reliably forecast future changes in our warming world. The polar ice sheets of Greenland and Antarctica are one major climate archive, which record information about local air temperatures by means of the isotopic composition of the water molecules embedded in the ice. However, this temperature proxy is, as any indirect climate data, not a perfect recorder of past climatic variations. Apart from local air temperatures, a multitude of other processes affect the mean and variability of the isotopic data, which hinders their direct interpretation in terms of climate variations. This applies especially to regions with little annual accumulation of snow, such as the Antarctic Plateau. While these areas in principle allow for the extraction of isotope records reaching far back in time, a strong corruption of the temperature signal originally encoded in the isotopic data of the snow is expected. This dissertation uses observational isotope data from Antarctica, focussing especially on the East Antarctic low-accumulation area around the Kohnen Station ice-core drilling site, together with statistical and physical methods, to improve our understanding of the spatial and temporal isotope variability across different scales, and thus to enhance the applicability of the proxy for estimating past temperature variability. The presented results lead to a quantitative explanation of the local-scale (1-500 m) spatial variability in the form of a statistical noise model, and reveal the main source of the temporal variability to be the mixture of a climatic seasonal cycle in temperature and the effect of diffusional smoothing acting on temporally uncorrelated noise. These findings put significant limits on the representativity of single isotope records in terms of local air temperature, and impact the interpretation of apparent cyclicalities in the records. Furthermore, to extend the analyses to larger scales, the timescale-dependency of observed Holocene isotope variability is studied. This offers a deeper understanding of the nature of the variations, and is crucial for unravelling the embedded true temperature variability over a wide range of timescales.}, language = {en} } @phdthesis{Valliappan2018, author = {Valliappan, Senthamizh Pavai}, title = {Solar Activity Reconstruction from Historical Observations of Sunspots}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-413600}, school = {Universit{\"a}t Potsdam}, pages = {115}, year = {2018}, abstract = {The solar activity and its consequences affect space weather and Earth's climate. The solar activity exhibits a cyclic behaviour with a period of about 11 years. The solar cycle properties are governed by the dynamo taking place in the interior of the Sun, and they are distinctive. Extending the knowledge about solar cycle properties into the past is essential for understanding the solar dynamo and forecasting space weather. It can be acquired through the analysis of historical sunspot drawings. Sunspots are the dark areas, which are associated with strong magnetic fields, on the solar surface. Sunspots are the oldest and longest available observed features of solar activity. One of the longest available records of sunspot drawings is the collection by Samuel Heinrich Schwabe during 1825-1867. The sunspot sizes measured from digitized Schwabe drawings are not to scale and need to be converted into physical sunspot areas. We employed a statistical approach assuming that the area distribution of sunspots was the same in the 19th century as it was in the 20th century. Umbral areas for about 130 000 sunspots observed by Schwabe were obtained. The annually averaged sunspot areas correlate reasonably well with the sunspot number. Tilt angles and polarity separations of sunspot groups were calculated assuming them to be bipolar. There is, of course, no polarity information in the observations. We derived an average tilt angle by attempting to exclude unipolar groups with a minimum separation of the two surmised polarities and an outlier rejection method, which follows the evolution of each group and detects the moment, when it turns unipolar as it decays. As a result, the tilt angles, although displaying considerable natural scatter, are on average 5.85° ± 0.25°, with the leading polarity located closer to the equator, in good agreement with tilt angles obtained from 20th century data sets. Sources of uncertainties in the tilt angle determination are discussed and need to be addressed whenever different data sets are combined. Digital images of observations printed in the books Rosa Ursina and Prodromus pro sole mobili by Christoph Scheiner, as well as the drawings from Scheiner's letters to Marcus Welser, are analyzed to obtain information on the positions and sizes of sunspots that appeared before the Maunder minimum. In most cases, the given orientation of the ecliptic is used to set up the heliographic coordinate system for the drawings. Positions and sizes are measured manually displaying the drawings on a computer screen. Very early drawings have no indication of the solar orientation. A rotational matching using common spots of adjacent days is used in some cases, while in other cases, the assumption that images were aligned with a zenith-horizon coordinate system appeared to be the most likely. In total, 8167 sunspots were measured. A distribution of sunspot latitudes versus time (butterfly diagram) is obtained for Scheiner's observations. The observations of 1611 are very inaccurate, but the drawings of 1612 have at least an indication of the solar orientation, while the remaining part of the spot positions from 1618-1631 have good to very good accuracy. We also computed 697 tilt angles of apparent bipolar sunspot groups, which were observed in the period 1618-1631. We find that the average tilt angle of nearly 4° does not significantly differ from the 20th century values. The solar cycle properties seem to be related to the tilt angles of sunspot groups, and it is an important parameter in the surface flux transport models. The tilt angles of bipolar sunspot groups from various historical sets of solar drawings including from Schwabe and Scheiner are analyzed. Data by Scheiner, Hevelius, Staudacher, Zucconi, Schwabe, and Spörer deliver a series of average tilt angles spanning a period of 270 years, in addition to previously found values for 20th-century data obtained by other authors. We find that the average tilt angles before the Maunder minimum were not significantly different from modern values. However, the average tilt angles of a period 50 years after the Maunder minimum, namely for cycles 0 and 1, were much lower and near zero. The typical tilt angles before the Maunder minimum suggest that abnormally low tilt angles were not responsible for driving the solar cycle into a grand minimum. With the Schwabe (1826-1867) and Spörer (1866-1880) sunspot data, the butterfly diagram of sunspot groups extends back till 1826. A recently developed method, which separates the wings of the butterfly diagram based on the long gaps present in sunspot group occurrences at different latitudinal bands, is used to separate the wings of the butterfly diagram. The cycle-to-cycle variation in the start (F), end (L), and highest (H) latitudes of the wings with respect to the strength of the wings are analyzed. On the whole, the wings of the stronger cycles tend to start at higher latitudes and have a greater extent. The time spans of the wings and the time difference between the wings in the northern hemisphere display a quasi-periodicity of 5-6 cycles. The average wing overlap is zero in the southern hemisphere, whereas it is 2-3 months in the north. A marginally significant oscillation of about 10 solar cycles is found in the asymmetry of the L latitudes. This latest, extended database of butterfly wings provides new observational constraints, regarding the spatio-temporal distribution of sunspot occurrences over the solar cycle, to solar dynamo models.}, language = {en} } @misc{YadavalliLoebnerPapkeetal.2018, author = {Yadavalli, Nataraja Sekhar and Loebner, Sarah and Papke, Thomas and Sava, Elena and Hurduc, Nicolae and Santer, Svetlana}, title = {A comparative study of photoinduced deformation in azobenzene containing polymer films}, series = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, journal = {Postprints der Universit{\"a}t Potsdam : Mathematisch-Naturwissenschaftliche Reihe}, number = {458}, issn = {1866-8372}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-413510}, year = {2018}, abstract = {In this paper two groups supporting different views on the mechanism of light induced polymer deformation argue about the respective underlying theoretical conceptions, in order to bring this interesting debate to the attention of the scientific community. The group of Prof. Nicolae Hurduc supports the model claiming that the cyclic isomerization of azobenzenes may cause an athermal transition of the glassy azobenzene containing polymer into a fluid state, the so-called photo-fluidization concept. This concept is quite convenient for an intuitive understanding of the deformation process as an anisotropic flow of the polymer material. The group of Prof. Svetlana Santer supports the re-orientational model where the mass-transport of the polymer material accomplished during polymer deformation is stated to be generated by the light-induced re-orientation of the azobenzene side chains and as a consequence of the polymer backbone that in turn results in local mechanical stress, which is enough to irreversibly deform an azobenzene containing material even in the glassy state. For the debate we chose three polymers differing in the glass transition temperature, 32 °C, 87 °C and 95 °C, representing extreme cases of flexible and rigid materials. Polymer film deformation occurring during irradiation with different interference patterns is recorded using a homemade set-up combining an optical part for the generation of interference patterns and an atomic force microscope for acquiring the kinetics of film deformation. We also demonstrated the unique behaviour of azobenzene containing polymeric films to switch the topography in situ and reversibly by changing the irradiation conditions. We discuss the results of reversible deformation of three polymers induced by irradiation with intensity (IIP) and polarization (PIP) interference patterns, and the light of homogeneous intensity in terms of two approaches: the re-orientational and the photo-fluidization concepts. Both agree in that the formation of opto-mechanically induced stresses is a necessary prerequisite for the process of deformation. Using this argument, the deformation process can be characterized either as a flow or mass transport.}, language = {en} } @phdthesis{Gidion2018, author = {Gidion, Gunnar}, title = {Akustische Resonatoren zur Analyse und Kontrolle von schwingungsf{\"a}higen Systemen am Beispiel von Streichinstrumenten und Dielektrischen Elastomeraktoren}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-411772}, school = {Universit{\"a}t Potsdam}, pages = {190}, year = {2018}, abstract = {Die Klangeigenschaften von Musikinstrumenten werden durch das Zusammenwirken der auf ihnen anregbaren akustischen Schwingungsmoden bestimmt, welche sich wiederum aus der geometrischen Struktur des Resonators in Kombination mit den verwendeten Materialien ergeben. In dieser Arbeit wurde das Schwingungsverhalten von Streichinstrumenten durch den Einsatz minimal-invasiver piezoelektrischer Polymerfilmsensoren untersucht. Die studierten Kopplungsph{\"a}nomene umfassen den sogenannten Wolfton und Schwingungstilger, die zu dessen Abschw{\"a}chung verwendet werden, sowie die gegenseitige Beeinflussung von Bogen und Instrument beim Spielvorgang. An Dielektrischen Elastomeraktormembranen wurde dagegen der Einfluss der elastischen Eigenschaften des Membranmaterials auf das akustische und elektromechanische Schwingungsverhalten gezeigt. Die Dissertation gliedert sich in drei Teile, deren wesentliche Ergebnisse im Folgenden zusammengefasst werden. In Teil I wurde die Funktionsweise eines abstimmbaren Schwingungstilgers zur D{\"a}mpfung von Wolft{\"o}nen auf Streichinstrumenten untersucht. Durch Abstimmung der Resonanzfrequenz des Schwingungstilgers auf die Wolftonfrequenz kann ein Teil der Saitenschwingungen absorbiert werden, so dass die zu starke Anregung der Korpusresonanz vermieden wird, die den Wolfton verursacht. Der Schwingungstilger besteht aus einem „Wolft{\"o}ter", einem Massest{\"u}ck, welches auf der Nachl{\"a}nge der betroffenen Saite (zwischen Steg und Saitenhalter) installiert wird. Hier wurde gezeigt, wie die Resonanzen dieses Schwingungstilgers von der Masse des Wolft{\"o}ters und von dessen Position auf der Nachl{\"a}nge abh{\"a}ngen. Aber auch die Geometrie des Wolft{\"o}ters stellte sich als ausschlaggebend heraus, insbesondere bei einem nicht-rotationssymmetrischen Wolft{\"o}ter: In diesem Fall entsteht - basierend auf den zu erwartenden nicht-harmonischen Moden einer massebelasteten Saite - eine zus{\"a}tzliche Mode, die von der Polarisationsrichtung der Saitenschwingung abh{\"a}ngt. Teil II der Dissertation befasst sich mit Elastomermembranen, die als Basis von Dielektrischen Elastomeraktoren dienen, und die wegen der Membranspannung auch akustische Resonanzen aufweisen. Die Ansprache von Elastomeraktoren h{\"a}ngt unter anderem von der Geschwindigkeit der elektrischen Anregung ab. Die damit zusammenh{\"a}ngenden viskoelastischen Eigenschaften der hier verwendeten Elastomere, Silikon und Acrylat, wurden einerseits in einer frequenzabh{\"a}ngigen dynamisch-mechanischen Analyse des Elastomers erfasst, andererseits auch optisch an vollst{\"a}ndigen Aktoren selbst gemessen. Die h{\"o}here Viskosit{\"a}t des Acrylats, das bei tieferen Frequenzen h{\"o}here Aktuationsdehnungen als das Silikon zeigt, f{\"u}hrt zu einer Verminderung der Dehnungen bei h{\"o}heren Frequenzen, so dass {\"u}ber etwa 40 Hertz mit Silikon gr{\"o}ßere Aktuationsdehnungen erreicht werden. Mit den untersuchten Aktoren konnte die Gitterkonstante weicher optischer Beugungsgitter kontrolliert werden, die als zus{\"a}tzlicher Film auf der Membran installiert wurden. {\"U}ber eine Messung der akustischen Resonanzfrequenz von Elastomermebranen aus Acrylat in 1Abh{\"a}ngigkeit von ihrer Vorstreckung konnte in Verbindung mit einer Modellierung des hyperelastischen Verhaltens des Elastomers (Ogden-Modell) der Schermodul bestimmt werden. Schließlich wird in Teil III die Untersuchung von Geigen und ihrer Streichanregung mit Hilfe minimal-invasiver piezoelektrischer Polymerfilme geschildert. Es konnten am Bogen und am Steg von Geigen - unter den beiden F{\"u}ßen des Stegs - jeweils zwei Filmsensoren installiert werden. Mit den beiden Sensoren am Steg wurden Frequenzg{\"a}nge von Geigen gemessen, welche eine Bestimmung der frequenzabh{\"a}ngigen Stegbewegung erlaubten. Diese Methode erm{\"o}glicht damit auch eine umfassende Charakterisierung der Signaturmoden in Bezug auf die Stegdynamik. Die Ergebnisse der komplement{\"a}ren Methoden von Impulsanregung und nat{\"u}rlichem Spielen der Geigen konnten dank der Sensoren verglichen werden. F{\"u}r die Nutzung der Sensoren am Bogen - insbesondere f{\"u}r eine Messung des Bogendrucks - wurde eine Kalibrierung des Bogen-Sensor-Systems mit Hilfe einer Materialpr{\"u}fmaschine durchgef{\"u}hrt. Bei einer Messung w{\"a}hrend des nat{\"u}rlichen Spielens wurde mit den Sensoren am Bogen einerseits die {\"U}bertragung der Saitenschwingung auf den Bogen festgestellt. Dabei konnten außerdem longitudinale Bogenhaarresonanzen identifiziert werden, die von der Position der Saite auf dem Bogen abh{\"a}ngen. Aus der Analyse dieses Ph{\"a}nomens konnte die longitudinale Wellengeschwindigkeit der Bogenhaare bestimmt werden, die eine wichtige Gr{\"o}ße f{\"u}r die Kopplung zwischen Saite und Bogen ist. Mit Hilfe des Systems aus Sensoren an Bogen und Steg werden auf Grundlage der vorliegenden Arbeit Studien an Streichinstrumenten vorgeschlagen, in denen die Bespielbarkeit der Instrumente zu den jeweils angeregten Steg- und Bogenschwingungen in Beziehung gesetzt werden kann. Damit k{\"o}nnte nicht zuletzt auch die bisher nicht vollst{\"a}ndig gekl{\"a}rte Rolle des Bogens f{\"u}r Klang und Bespielbarkeit besser beurteilt werden}, language = {de} } @misc{SposiniChechkinFlavioetal.2018, author = {Sposini, Vittoria and Chechkin, Aleksei V. and Flavio, Seno and Pagnini, Gianni and Metzler, Ralf}, title = {Random diffusivity from stochastic equations}, series = {New Journal of Physics}, journal = {New Journal of Physics}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-409743}, pages = {33}, year = {2018}, abstract = {Brownian yet non-Gaussian dynamics was observed. These are processes characterised by a linear growth in time of the mean squared displacement, yet the probability density function of the particle displacement is distinctly non-Gaussian, and often of exponential(Laplace) shape. This apparently ubiquitous behaviour observed in very different physical systems has been interpreted as resulting from diffusion in inhomogeneous environments and mathematically represented through a variable, stochastic diffusion coefficient. Indeed different models describing a fluctuating diffusivity have been studied. Here we present a new view of the stochastic basis describing time dependent random diffusivities within a broad spectrum of distributions. Concretely, our study is based on the very generic class of the generalised Gamma distribution. Two models for the particle spreading in such random diffusivity settings are studied. The first belongs to the class of generalised grey Brownian motion while the second follows from the idea of diffusing diffusivities. The two processes exhibit significant characteristics which reproduce experimental results from different biological and physical systems. We promote these two physical models for the description of stochastic particle motion in complex environments.}, language = {en} } @misc{ŚlęzakMetzlerMagdziarz2018, author = {Ślęzak, Jakub and Metzler, Ralf and Magdziarz, Marcin}, title = {Superstatistical generalised Langevin equation}, url = {http://nbn-resolving.de/urn:nbn:de:kobv:517-opus4-409315}, pages = {25}, year = {2018}, abstract = {Recent advances in single particle tracking and supercomputing techniques demonstrate the emergence of normal or anomalous, viscoelastic diffusion in conjunction with non-Gaussian distributions in soft, biological, and active matter systems. We here formulate a stochastic model based on a generalised Langevin equation in which non-Gaussian shapes of the probability density function and normal or anomalous diffusion have a common origin, namely a random parametrisation of the stochastic force. We perform a detailed analysis demonstrating how various types of parameter distributions for the memory kernel result in exponential, power law, or power-log law tails of the memory functions. The studied system is also shown to exhibit a further unusual property: the velocity has a Gaussian one point probability density but non-Gaussian joint distributions. This behaviour is reflected in the relaxation from a Gaussian to a non-Gaussian distribution observed for the position variable. We show that our theoretical results are in excellent agreement with stochastic simulations.}, language = {en} }